Text

10CFR61 Radwaste Classification Scaling Factor Evaluation.
	ML18149A105
Person / Time
Site:	Surry
Issue date:	09/30/1985
From:	; VIRGINIA POWER (VIRGINIA ELECTRIC & POWER CO.)
To:	;
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References
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- - - - ....i'1 VIRGINIA POWER SURRY POWER STATION 10CFR61 RADIOACTIVE WASTE CLASSIFICATION SCALING FACTOR EVALUATION SEPTEMBER, 1985

I

'I

- - __ 1

Ca-2:'13 CCa-2ff) in Priaa.ry Resin CX:ey Isotope : Co-60)

The unmodified S.F. was 1.lE-06; however, this resulted in a no.nconserva.tive calculated isotopic concentration for samples 10446, and 10556, of which only 105S6 was out of spec. Since 61-1088 was the only sample containing a <LLD value for the isotope, it was eliminated from the calculations to provide a ---------

conservative scaling factor of l.9E-06. - -----------

/_

- -. - - ., - - * .. - - - ... . . lllllllt .... ....

VIRGINIA POWER SURRY POWER STATION 10CFR61 RADIOACTIVE WASTE CLASSIFICATION SCALING FACTOR EVALUATION SEPTEMBER, 1985

- -~- - - - - - - - - '- - - --

~

10CFR61.55, "Waste Classification", provides in part that, "The concentration of a radionuclide may be determined by indirect methods such as the use of scaling factors which relate the inferred concentration of one radionuclide to another that is measured, .... if there is reasonable assurance that the indirect methods can be correlated with actual measurements".

Based on recent NRC guidance which suggested that Scaling Factor (S.F .) correlations, wherever possible, be accurate within a factor of 10, the station's S.F. development methodology was modified to improve results. Using log normal averaging of inferred nuclide to scaling nuclide ratios, the waste sample analysis data compiled during the two year collection period of 1983 and 1984 was evaluated to determine S.F .s which would most accurately correlate with sample results. This evaluation provided acceptable S.F .s for classification of wastes in four distinct waste streams; dry active waste (DAW), liquid waste processing resins (Liquid Waste), primary loop filter media (Primary Filter) and primary loop purification resins (Primary. Resins).

DISCUSSION A review of the data collected during 1983 and 1984 was performed initially to ensure awareness of those factors with potential for undue influence on correlation accuracy. These factors included: sample size, activity and representativeness, laboratory analysis sensitivity and the percentage of positive analytical results vs. those below the lower limit of detection

(<LLD) for samples within each waste stream. The factors identified as having greatest influence on correlation accuracy are as follows.

(i) The samples collected during 1983 and 1984 were analyzed by two different vendor laboratories. Sample quantities provided to the laboratory utilized during 1983 were extremely small due to activity restrictions contained in the vendor's by-product material license. For 1984, a different vendor was located with far less restrictive license con-ditiom;. The analysis results reported l5y these two vendors were observed in several instances to compare unfavorably due to the effect on analytical sensitivity of reduced sample quantity.

(ii)

Samples collected from the Liquid Waste stream during 1983 and 1984 were observed to correlate poorly for several radionuclides. Investigation revealed that the 1983 samples consisted of small quantities of specific types of ion ex-change resin media (e.g., anion, cation, etc.). In 1984, a sample of mixed resin was obtained from an actual shipment container. This type of sample is considered more representative of typical waste shipments and, thus, was given more weight during scaling factor evaluation.

()Jjjc.e.,,

The development of scaling factors required a two phase evaluation. First, alJ sample data was assembled by waste stream and nuclide of interest. The log normal average of all inferred nuclides to scaling nuclide ratios was calculated for each group of data. This value (the scaling factor) was then used to calculate inferred nuclide concentrations. The factor difference between measured and calculated nuclide concentrations was determined to assess correlation accuracy, with a negative sign applied to nonconservative correlations. In the second phase, correlation accuracy was reviewed for each data grdup. In each case where nonconservative correlations were observed to exceed a factor of 10, the data group was reevaluated to determine if improvement was possible. The influence of <LLD results and sample results with question-able reliability or representativeness were observed to contribute to poor correlation in a number of data groups requiring reevaluation. Where improvement would occur, these results were eliminated from the data group and a modified scaling factor was calculated. In several cases, however, elimination of <LLD results would have provided further nonconservatism thus, the original scaling factor was retained. Additionally, a small number of cases which were reevaluated* exhibited no suspect data and presented no logical* method for improving correlations. Here also, the original scaling factor was retained.

.. - - - .... 91! ---

Displayed in the attached tables are the results of the scaling .factor development described above. The first table provides a summary of the final waste classification scaling factors_ for each of the four waste streams. The tables which follow provide detailed calculational results of the evaluation, organized by waste stream and radionuclide. Footnotes are provided, as necessary, to describe the results of reevaluations performed to address nonconservative correlations.

CONCLUSIONS:

While the S.F. development methodology used was unable to achieve total conformance with the correlation accuracy goal, those few correlations which remain nonconservative by greater than a factor of 10 were closely evaluated and are not considered to invalidate the final S.F.s accepted. S.F.s will be reevaluated and updated on an annual basis to assure currency.

.. -* ---- ...... Surry Power St.ation Rad. 1d

. . . .j

. assification Sea ling Factors 10 CFR 61 : : :

. . . .1.S:.Q~9P~.... : . ~.e:Y. !~9f9P.~. : ..... I? .Pi':,*( . .... : .. ~j\l, ':,'( ?P.t.e: .. : . F'.t:ir:r1 .f. i.lt!:'r: . : .F'.t:i'T! .g~,s:.iri..

. .. .?.r.-:*~.Q .... : ... !=:~:-.1.~7 ... : ...!:? :r:;:~f;-:-Q:;:.. : .. .4:O~f;7Q? .. : ...4:Q~f;-:-Q4 .. : ...4,:;i~f;:-Q:;: ..

. .. .T~-:'?.':! .... :... !=:~:-.1.?,7 ... : .. -~ ,?,~f; :-Q4.. : ...~ :?,~f; :-Q4..: .. .1.-.~~-~ "!'PQ.. : ...!:? ,$~f; :-Q9 ..

. . . . .1:-.1.4~ .... : ... !=:~:-.1.'.?J: ... : .. .4,4Qf;:-Q4 .. : ...::? :O~~ :-Q4..: ... 1. ,Q~f;:-Q?,,.: ...~,(;:~f;:-Q9, .

. .. . .G:-.1.4..... : .... r.Q-:'?P .... : ...~, Mf;:-Q1 .. : ... 1. ,?,~~:-Q:?..: ...4,$~~:-Q? .. : ... 1.:?~f;:-Q4..

. . . .f!:':-:9~ .... : .... r.Q-:'?P .... : ...~:4~f;:-Q1 .. : .. .'?,!;i?!;:-Q1 .. : .. kQ7~:-Q1 .. : ...::?,~f-!f;:-Q?..

. . . . Ni.--:9~ .... : .... 9.C!-:'?.Q .... :.. _q ,r;,~f; :-Q 1.. : ...4,Q~f; -:-Q1 .. : ... 1. :$:'1:f; 7Q 1.. : .. _q :~~f; :-Q 1..

. . . P.*r~4.1 .... : ... !=:~:-.1.4~ ... : ...1...!:?~.~"!'QQ .. : .. ."?:~*7~:-Q1 .. : .. _q:?-~;:-Q1 .. : .. k?Q~:-Q1 ..

. . . . . . . . . . . . . . . : .... r.Q-:'?.G .... :.. _q ,r:;:~; :-Q? .. : .. -~, 1~~ 7Q?,.. : ...::? ,1~;:-P?.. : .. :? k1.f; :-Q4..

. ..i;:ro:-.4f4 ... : ... !=:~:-.1.4~ ... : .. -~ ,$f-!f;:-Q9 .. : ... 1. ,9f.!f;:-Q? .. : ...4,9Qf;:-Q9_.: .. .4,4Rf;:-Q?..

. .. . . . . . . . . . . . . : .... r.Q:'?.Q .... :... 1.:4~~:-Q4.. : .. .1. ,9:2:~:-Q4.. : ... 1. :?f-!;:-P?.. : ...!:?:$~~:-Q9..

. . . F'. 1~:-~9~ ... : ... !=:~:-.1.4~ ... : ... 1. :O~f;:-Q? .. : ...7., 1.1.f;:-Q?, .. : .. .4,9~f;:-Q?,.. : .. _q :~~f; :-Q9 ..

. .. . . . . . . . . . . . . :.... r.Q:'?.Q .... :.. _q ,r:;:Qf; :-P4..: ...~ ,f::!f;:-Q9.. : ... 1. ,9~f;:-Q!:?.. : .. -~ :9~f;:-Q?..

. ..~rri.--:?~l ... : ... G~:-.1.4~ ... : ...~,4.1.~:-Q? .. : ...~, 1~~:-Q9 .. : .. .1., l ~~:-Q?.. : .. .EL~!:!~:-Q4..

. . . . . . . . . .. .. . . :.... r.C!-:'?P .... : ...1.:?~;:-Q4.. : ...q,?~;7Q!;i.. : ...7., 1~~:-Q~* .. : ...::?,Q~;:-Q?..

. . . F'.1.J:-~?,~ ... : ... !'.=:~:-.1.4~ ... : .. .1. :7~;:-Q?.. : ...!:?,$7;:-Q?-.. : .. .1.* ~.1.f;:-Q?.. : ...4: 1l;:-Q?, ..

. . . .f5.... F.tJ:-~4Q: .... r.C!:'?.Q .... :...~,~~f;:-Q4 .. : ...7. ,QQ;:-Q9 .. : ... 1. ,?Q;:-Q!;i .. : .. _q, 1Rf;:-Q? ..

. .. P.*~:-~4~ ... : ... !'.=:~:-.1.4::1: ... : ...~:9!:!;:-Q4 .. : ...4,!;if-!;:-Q4..: .. ,q :~*~;:-Q!;i,.: ...4, 1i:;:-Q9 ..

. . . -~-. NP.:-~?-l: .... r.C?-:'?.Q .... :...~, 1~;:-Q!;i.. : ...!:?,4 !'.;:-P?.. : ...::?,?-~;:-Q?.. : ...~ ,$~;:-Q$..

. ..Gro:-.4~.q ... : ... !'.=:~7.1.4~ ... : ...l.:$~;7Q?, .. : ...q,$'.:i;:-Q? .. : ...~ ,Q.1.;7!'.N .. : ...4,r;,R;:-Q4 ..

& Cm-244: Co-60 : 6.72E-05 : 4.59E-05 : 5.68E-06 : 1 .88E-06 September., 1985

-- ' ............ .. I DRW Scaling Factor Evaluation

___J

.. ---,-* Sr-9 Cs-137

.. , ... ,, .......... ; ............................................. :. ............... :. ..AY.E!l'.'~9.E: ..S9~.T l,:'19. . ;C. ~-1P.41.<!t.~ d*..* I!>.C! .{~

....C~JP.*.

$~.rrm\~ri:i~.E:I'.' . !~'?~PP.~ .CP.r!Q, . l<.E:Y. !~9... C9.r!Q, l.~<?I.IS,Y. .l~~~j9: .1<?9. !~9/~~.Y.: ..... f~P.t.cir: ........ !~9... CP.r!Q, ..... f ~P.t.cir: ... .

.. .. .. ........... L-~~:-Rt........=?,1 ~.-:9J....... !;5*. :r:~:-R':l.... :.... :-.~.:?...... :.... !;5.. '.::!~:-R~........ ,..~~:-R~........ to.~..... .

03~~......... ~.-~~:-R~....... .1.,~~:-:9~ ...... 7.-~~:-Q~.... : .... *:-.::?,1.. .. : 5.9E-03

.... !.... 7.5E-05 -1.3 61-1093 1.6E-02 3.4E-01 4.7E-02 : .:.1.3 .. : .... s. 9E.:.ai........ 2. aE.:.ai ....... :.a:o......

No out of spec. nonoonserv ative oorre latior,s are observed J

To-9

......................................C~.'":1 ~7 ................... : ............... :~Y~t:"a9.e S0:alin9. Calculated ls:o vs. Cale.

~:a.rrP.1.~

10397 N':lro~.~t:' . ,~9~~.P.~ .C~.rl<?: . ~.~Y. !~9... C!='.11'?: l.~'?/.l'StY. gJ~j9:.1'?9. ,~o/Key is~'.'c~~~: .... "i:~~t'~~ .. ...

Fa~t*~~ .. . .. '*' ......................

.. "1 '03'99" .... ~ ..

................. ~

~**~~:Q~...... " 4 : ~.:o.1....... ~.. Q~:-Q~, .. * (.... :-.~:?.......... '?.,::\~:-Q~.......... J..~~:-Q~.......~ . ~......

1

.....R~. R~ ....... .1.*~~..o;;::., .... , .. ~~:-R~... ;: .... :-.4,e.......... '?.. ::\~7Q~.......... ~...1.~7Q9...... :-.4:~.... ..

61-1093 2.BE-04 3.4E-01 8.2E-04 : -3.1 6.4E-04 2.2E-04 -1 .3

.. - - .. ,- - .. - .. - .. -\ - - .... -~*

Sinoe 1-129 was <LLD in all samples, no o~her sa~isfac~ory Scaling Fao~or oan be re.alized.

.. .. .... - ... .. - - .. - C-1 1111 -

. . . . C 60 . .

................. : . : ............... : . : ...... '?:-........ : ............... : ............... : .~Y.E!~ fl9.E! .~9:a.lji:ig : ..C:a.lP.41.~~~~.. : .IF.Q .'{f,. i:;:,~JP.*.

$l9.l'DP.1~

.... i *a:!~* ..... 1. 1.. r:~=~!* . *[*

10 Nyro~~(.: !~9t!>.P.~ .(;!>.I'!<?::. :~.E!Y. !~9, ,i:;:,:inq: :1.~i:;,(.~,Y. .~fl~i9: .1'?9.1~9/~"°*Y ....................................................

I .. : =:~*:

Factor : lso. Cono. : Factor .

0~.... j .. ?.*~~ :.QP.... j.... :.o. ~....... ;.... ~..,1.~ :R 1...... ;.... ~.. Q~:-R~.. ;.... :-.4 :~..... .

.. . .. . .. .. .. . .. .. . .. .. .. *.................. :. ~..Q~ ....... 1.. ~~. Q1.. ........ .0:7..... :... 8.1 E 01

6.SE-03

4.3 61-1093 :<: 1.4E-03 : : 2.9E-01 : El;minated: N.A. *: *e:1.'1e::01""":""2*.4e::01":""1*6e.'1'-""

See aUaohed exp la nation

-- C-14 in DAW-Unm Sc.a ling F.actor 60

............*.*.. :. . :' ......*........ :. * :. ..*..C-:-9:-........ :' ............... :' .......*....... : ..~Y.E:t:' ~9.E: .~9~.111'.'19. . .C~.lP.41.~~~~- . : .l~.Q .~f:. C~JP.*.

~~.l'flP.ci\*~~ro~.e:(. \!~9~PP.~.Cpn<;\. \KE:Y. !~9... C~n<?: ?~Q/.t~'?!I. g~~w .1<?9. !~9/~1?.Y.: ..... f~P.t.Qt:' ........ !~9:.CPn<?: .. :... f~P.t.Qt:' ... .

.. .. 1. ...~?...... :.:.. ~--~~ :-Q 1.... : .: .. -~ /~~:-:9~ .... : .. ~)!?~ t.QP.... : ..... 9. 9....... :.... 1.-~~:-R 1.. . . .. . ... t~~ :-R?.. :... :-:~~ .,q ... ..

. . .. !.Q~.~f;3...... -1 * \ *. L-~~:-R~.... :.: ...~.~~."".0~ .... : .. , .. ~~:-Ql .... : .... :-.Q:7...... :.... L-~~:-Ql .......... t~~:-R~.. :.... :-.1. :~.... ..

61-1093 *<* 1 .4E-03 : : 2.9E-01 : 4.8E-03 : -2.3 1.5E-01 4.3E-02 : 30.5

C-11 in DAY The unmodified S.F. was l.5E-0I; however, this resulted in a nonconservative calculated isotopic concentration for sample 10397, due to the influence of the

<LLD value of sample 61-1093 .. Therefore, the S.F. was recalculated using the values of samples 10397 and 10398, resulting* with a conservative factor of 8.lE-01.

Fe-55

Ill ..,- - - .. - - .. - - .. - -* Ni-63

.................._( ................ : .... .G9:-.~9..... ............... :............... lr'f.e.r: J9.~ .~9~.ljrig ..C~.lP.41.~~~~- ..Ii>.~."!,: -~~JP.*.

~~.rfl.P.l.~

10397 N':lfl'.lt:i.~r: . :. !~9~!>P.~

4 E .C!>.!"Kl:

O . *:l:<.~Y. !~9:.~!='nq: 1.~Q/.ISfY. .~J~j9:* .1Q9. .lso/Key

. . . . . . . . . . . . . .Factor lso. Conn.

. . . . . . . . . . . . . . .......... Factor

'I'. * * * **************

10398 . : .... -~.".'

8 7 -03 .. ~ ..... :

...~:~~:-:Q~;

- ..... , .. ~~:-Q1..

+ .. :

.... :-.Q 13.. 3.7E-01 3.6E-02 -1.2

..........................~ ............ ,!:;I :~~..Q~.... .. 1.-~ ..Q9.... : .....0. 9 ~.7E-01 3.1 E-03 -2 .8 61-1093 : 3.1E-02 : 2.9E-01 1.1E-01 : . -1.6...... "":o'.1e::o; .......... ,...,.e::o, .. ""'i,4"""'

- - .. - - - .. - Pu-241 in DA 'w' otcipe : Ce-144)

................. : . : ........... ; ... : . : ....C!?:: 1~'f................... : ............... : .i'~Y.E!'7J9.E! .~9:a.li".'19.: ..C:a.lP.41.~,~~.. .l!>.C! .-<,,.C:a.lP.*.

$:arnP.1.E! N':lro!:i.E!i::.: !~9~!>P.~ .C!>.t"!Q,:. :l<.E!Y. !~9... CP.t"!Q, l,~q/.lS,Y. .f?.il~i9:, Jqg, ,~9/~!?.Y.: ..... f~P.t.QI'." ...... : .. !!r9:.CP.t"!Q, ..... .F:'ilP.t.QI'." ... .

.. .. !.Q~~?...... : .: .. J** ~~-:-R~ .... :.: .. .1.*~~;:Q~ ...... 7.-~~-:-Ql .... : .... :-P,1 ...... :.... L-~~t-.Q9...... :.... ~.. Q~:-Q~.......~.-L .... ..

10398 : : 3.6E-03 : <: 9.SE-05 3.7E+01 : 1.6 : 1.6E+OO : 1.5E~04 -23.3 61-1093 : : 9.4E-03 : : 6.5E-02 1.4E-01 -0.8 1.6E+OO 1.0E-01 10.9 Elimination of the Ce-144 <LLD value of :s:arnple 10398 would result in a less conservative Scaling Faofor

- -~ - - - - .. - - *- - - -*-

Pu-241 inDA'w'(K tope : Co-60)

. . . . C 60 . * .

. . . . . . . . . . . . . . . . . : . : ............... : . : ...... 9:-........ : ............... : ............... : l~Y.~~ ~9.~ .~9~.lji:ig : ..C~.lp,41;~1ft~ .. : .1~.q .\!f,.. C~.19.,.

$~.l'flP.1.~

10397 N':lro~.~r::* . :* l~9~P.P.ft E .CP.l'}q, *: . :* ~.~Y. !~9... C9.'1<?, :* I.~'? I.IStY. .~~~j9:* .1'?9. !~o/~eiy : F.actor

. . .......... : lso. Cone. : F.actor .

...*, *03'90* ..... :.: .. J..~. :-R~.... :.: ...~.~~::O~ .... :*

L-~~:-Q?. * **: * ** *:-.1. ,e. *****(***.~A~~:-Q?. * * * * * (* ** .~..~~:-Q~. *: * ** *.'J. J. ** ** **

- - 61 ~*frjcji * * *1 * ! * *t:t:~l * *: *: * ~::~*:Zf **** *:J~:§1-*** :*~t *****: ****;*::~:§~* *****: ****t~:§i* * *~~s~* ** .

1* 1* * *

1* **

Cm-242 in DAW (Ke pe : Ce-144)

\.

.. * * .... * * ...... * * ................ j ....C~.":1 ~~ ................... : ................~Y.E!(fl9.E! .~9~.lji:-,9.: .. C~.lP.41.~~~~ .. .1~.Q .'{J:.C~.19.*.

$~.rfl.P.l.e:

10397 N'ilro~.e:i: . !~9~!>.P.~

1 6E-05 .C!>."!<?: . *:l;-:.e:y. !~9:

- .C!>.1"!<?: 1.~<d.~fY. ~fl~j9:* .1Q9. !~9/~~.Y. . ......... Faofor :

lso. Cone. ..............

_. ........ :*************** Fao~or .

10398 . .... *...........

8 SE 07 . :

... 1.:~~ .. 0~ ...... f;l.. ~~:-Q~ .... :

.... :-.:?:1 3.9E-03 , 7.4E-06 -2.2

................. ~ ........ :-....... ~: .. ~:e~.":0~ .... ,,f;l,}~:-Q~ .... : .... :-.2:1 3.9E-03 : 3.SE-07 - -2.2 61""1093 s.2E-os = 6.sE-02 e.oE-o4 : -ix ..... .... 3..siE.:.03...... :.... 2..sE.:.04.......-i.i .... ..

- -~ -*-*- - ... Cm-242 in DA'w' (I<

tope : Co-60)

.......................................G9:-.Ei-9.................... :. . . .. . . .. . .. . . ~ye~age Scaling Calculated lso vs. Cale.

$~,ITIP.1~

10397 N':lro!>.~~ . !~9~!>P.~

1 6E-05 .C!>.r"!Q: . l<.~Y. !~9:.C!>.r"!Q,

- I.S;Q/.IS~Y. .R~tio:

. . .. : . log

. . . .lso. . ./Key

. . . . . .. . . ... . .F. ac*t*~~.... . . i.~.~*.

. . . . . . . . . . . . .. *c~~~: ...... Fa~*t~~.: ...

.. .. 1..0398

. . . . .. .. . .. . .. 8.. *...............

5 - ~.~~..- 0~ ...... 1 .6E-04

............. :* . . . . .-3.8

. . . . . . . . . . .. . . . 1

. ..4E-04

... ...... .. .. . . . . 1.4E-05 -1 :1......

.. .. .. . .. . .. .. .. . ~ .......~. Q7........~.~~..0~ ...... J,.Q~:-Q~ * -4.0 1.4E-04 1.2E-06 14 61-1093 5.2E-05 2.9E-01 1.eE-04"":'"':..'i:7'""' ""1'.4E:04"'"' .... 4..2E:o~:;" ":..(2"""

- ---- Pu-238 in Dl'o\'f (.

.otopE" : Ce,-1 44)

.................................. : ....C!?;:M"................... :................~Y.E:'7J9.E: .S!'?~.lji:-i9. ..C~.lP.41.~~~~: . .l!>.Q .\!~:.C~.lP.*.

~:arr,.P.1.E: N':lro~.E:17 . ,~9~!>.P.~ .C!>.r!C?: . :.l<.E:Y. ,~9: .C!'.l"!C?, ,.~Q/.IS~Y. .l~~~j,;,: .1Q9. ,~9/~!?.Y ...... -~ Jp,t_q17 ........ ,~9: .CPnC?, .*... f JP.t,q17 ... .

. .. . 1.Q~.~7...... . .. J..~~:-P.!;i..... : .. .1.* ~~."'.0~.... . .?.. ~~:-Q~.... : .... :-.:.? ,1.......... L,Q~:-Q?... '... .. .. 7.. Q~:-Q~....... L~...... .

. . .. J.Q~~~-..... . . J...1.~:-P.9 .... ~: ...~.f?~."'.Ol:! ...... J...1.~:-Q1. ... : .... :-.0.~.......... J..Q~:-Q? .......... J.. Q~:-P.~......"'.lP.*.~ .... .

61-1093 8.5E-05 : 6.5E-02 1.3E-03 -2.9 1.0E-02 6.7E-04 7.8 Elimination of the, valuH of sample, 10398 due, to <LLD of Ce-144 would provide, a lE-ss: cons:e,rvatin Scaling Factor

- - - - - - - - - - - - - - -*- Pu-:238 ;n DAW ( ~ope : Co-60)

.... *.... * .............................G9:-~9.................... :............... *"'Y.~~~9.~ .~9~.lj,:ig, ..C~.lP.41.~~~~- . .l!>.C! .~,:.9~.lP.*.

$~.rri.P.1.~

10397 Nt,1IT1~.~~ . !~9~P..P.~

1 4E-05 .CP.'"!t.?, . ~-~Y. !~9-... 9p.r,t.;i, 1.S:<?l.~fY. g~~j9:* .1<?9. !~9/Key Fao~or lso. Cone. Fao~or . *

....foigif ......................... ~.~~- .9~ ...... 1.-~~:-R'f.... : .... :-.~,e.......... ?:.-~~:-Q'f.......... ?:.-~~:-R9.......?.. ?..... ..

* .................. J. ..1.~:-Q~........E;l,'f~.-:0;!; ...... J..~~:-R~.... : .... :-.~.~- ......... ?:)~~:-P4 3.:2E-06 -3,5 61-1093 8.5E-05 2.9E-01 :2.9E-04 : -3.5 3.SE-04****** ****;*:1*E.:.04** *****1".3"******

.I .

- - ------ - - - - - - - *- -~ Am-241 in DA\v' (K. ope : Ce-144)

................. :. .:. ............... :. . :. .....C,.-:1 ~':l.,... :* ...............* *:............... :* l~Y.~r:-a9.e

- - - r03,97******:*:**:* ~r i:lf"!Q Scalinn: Calculated : ls:o vs. Cale.

S.am le Number: : Is t C : : * ........ ;:,. : * ...... * * .. " .. : * .. * * * * " " " "

=: * : ~.~Y. !~9,. CPnQ, :1.~Q !.ISfY. g?~~'?: .1<?9. !~9/~!?.Y : : ..... f ?P.t.cir:- ...... : .. !~'?,.Cpnq, .. :... f ~P.t.cir:- ... .

.. .. . . .. . .. .. .. .. : . : .... *.. ::*....... :.: ...1. 1~~-:Q;!

2.2E-03 * -2.7

3.4E-03 : 6 SE-06 : 16

10398 .. 23E- * * . *****:***************:***************:*******************:***********************'********

................. : . : ....*.... Rt$ .... :~: .. .'~,e~.-:0:S

2.3E-02 * -1 .6

3.4E-03

3 3E-07 : -6 9 61-1093 : : s .1 E-os : : 6 .sE-02 .... : .. 1*.aE.:.04.... :.... :.*i:; *.... *: .... 3°.4E.:.oi:' .... *: .... 2*:2E:-:.04.. :.... *4*i *.. *..

- - - - - ----- - - - - -*- -~ *. Am-241 in DA'w' (l.tope : Co-:-60)

.. .. C60. . .

. . . . . . . . . . . . . . . . . : . : ....... ,- ....... : . : ...... 9:-........ : ............... : ............... : lr:t.E!t:~9.E! .~9:9,1jri9.: ..C:9.lP.41.~~~~-.: .l~.q -~~,.C:9.lP.*.

$:9.l"fl.P.l.E! .~':lro~.E!t::.: !~9~P.P.~ .CP.r'!Q::. :l:<.E!Y. !~9,.CP.F'!Q, :l.~<?l.~fY. g~~j9: .1<?9. !~9/~!?.Y.: : .. .. f JP.t,q,:- ..... : . lso. Cone. : Faotor 10397 : : 4 1E-06 : : - : - : - . ~ . : .............. : ............. ..

.... 1*03*90" .... :.: .. :{iE:06* .. *: *: **.~.~~*..:9~.... :* *~--~~:R9.* .. :* .. *:.*4:'f.... **: * .. -'--~~: Q'f.... * *: * * *

L-~~:-R9.. :.....l-9..... ..

........................*.................~,'f~..0~ ...... -~--~~- Q.,_ .... : ..... ,q,~...... : .... L~~- Q.,_...... : ... 1 .1 E-06 * -2.2 61-1093 : : 5.1E-05 : : 2.9E-01 : 1..8E-04 : -3.8 : 1.!E-04 . i.1E:05":'"':.*;:4"""

- -~ - - - - - - - - - ------ Pu-239 (Pu-240) in [) A Isotope : Ce-144)

.. . .. .. .. .. ; ..................... :. . :. .....C~.-: 144 ........ :' ............... :* ...............

. Average Scaling Calculated ls:o vs. Cale.

$:a.rr*P.l.E! N':lro~.'=!t:' . !~9~!>.P.~ .C!>r!Q,:. :~.E!Y. !~9:.C!>.l"!Q, :f.~Q/.il;,Y. git~j9; .1Q9. ,~o/Key ..... °Fao't'~~.... . . j;~:

I 0397 4 3E-05 : : 9 - : - *

c~~~: ..... °F~~*t*~~ ... .

10398 .. .. .. .. . . .. .. *................

6 3E-06 * * .1.,. ~.. 9R .......

~.. ~~. R? .... :

..... .1. ,'$... . 1.7E-02 3.3E-05 -1 .3

.................................. :~: ...~,e~.-:Ol:! .... : .. ~..:'\~:-!'.!?.... : .... :-.1.,:?. 1.7E-02 1.7E-06 -37 61-1093 2.3E-o4 : : 6.5E-02 : 3.5E-o::i: : -2.5 ......... , .. 1E.:.02.......... ,.:1*E.:.oi* .....4. 9.......

- - ------ Pu-239 (Pu-240) in* D

. Isotope : Co-60) 1111111. - *- - -

.;" ................................... .G9:-.~9..... ............... :............... ~v.erag_e Scaling_ Calculated ls:o vs. Cale.

.-:&.rriP.1.~

10397 N':'ro~.~r: . !!?9t!>P.~

4 3E-05 *- .CP."!Q, l.~<?I.IS,Y.

.Q!>m, . i:::.~Y. ,~9: - .~ftj9:* .1<?9 :..!!?9/Key . . . *Fac't'~~.... . . i~~*.. c~*~~: ..... *F~~*{~~ ... ..

107 98 .................

6 3E-06 ... ~,~~

8 .. 9~ ...... ~.. ~~.QcJ-.... :

...... q,4... 6.4E-04 6.3E-05

................................................... 1.5 . .

..................... ................. .... ,'f~.-:O;!i ....* .. 7.. ~;:-Q'f .... : .... :-.~,1...... 6.4E-04

5.3E-06 -1 2 61-1093 2.:a:E-04 2.9E-01 7.9E-04 : -3.1 .... 6.. 4E.:.04"'.*" ****;*.9e:.:.04** "**:...,-:i'*****

- --* ------ ---------- Pu-242 (Np-237) ;n D y Isotope : Ce-144)

Ce-144 : *"'Y.~t:'~9.~ .~9,l,lj~Q. .. l;il.lP.41.~~~~.. : .1~.Q .~, .. .l'.;~.lP.*.

~~:fTlP.l:~ N~ro~~~i: 1ii9~PP.~:c;,:~q; 1: i~Y: !~9:.:c;,:~q; i:~(d~~M :~~~j9(: lqg: ii9i~~:.,;: ..... f ~P.t.Qt: ........ !~9,.1'.;~nq, .. :... f ~P.t.Qt; ... .

.. .. !.Q~7...... :~: .. J..;!i~:-R'?.... :.: .. .1. -.~~.-:Q;!i ...... ~--~~-:-R':l .... : .... :-.~,?...... . .. .f:3.-~~:-Q~......... .1 .-~~-:-Q~.. :..... L~..... ..

.. .. LQ~~?...... :~: .. , .. ~~:-Pl?.... :~: ...~.e~.-:o~ ...... 1.-~~:-R?.... : .... :-.1.*e.......... ?.-~~:-R~.......... ~.. ~~-:-Re.. :....-:1 !=!-.? .... .

61-1093 :<: 4.2E-06 : : 6.5E-02 6.5E-05 : -4.2 8.6E-04

5.6E-05 : 13.3 EHminatfon ofthe <LLD values of sample 10398 would result ;n a less conservat;ve Sea ling Factor

- - -* - - - - - ------- Pu-242 (Np-237) ;n D y lsofope : Co-60)

.**.. **...... :. *:..*: ...... ******.. ,:..*:, .....C9:-.~0...... : ... ; ........... : ............... : ,.t,Y.~~~9.~ .~9~.1ji:-i9.:. ,r:;~.lp,41.~~~~.. : .1~.Q ."<,: .C~JP.*.

5. ~.ITlP.1.~ -~;ro~.~(. j !~9~!>P., .l:;!>.I"!'?: j. (~-~y. !~9: .C!>.l"!Q: jl.~C? /.!SfY.. -~~~i9(. l<?9. !~9/~!l'.Y.: .... of ~P.~.Q~ ...... : .. !~9...C!>.l"!Q: .. : .. *. f ~P.~.Q~ ... .

- **1.Q~~ *..... :~: .. 1.-~~:-R~.... : . : .. -~=~~:-:o~ .... : .. L-~~:-R~ .... :... ;:-.4:~...... : ... ;~.-~~:-R~...... : .... ~...t.~:-R~.. :.....:?. ~...... .

. .... !.Q~.~8 ....... :~: .. J..,~:-R~ .... :.: ...~,tf~.--:0~ .... : .. J.. ~~:-Qtf.... : .. -3:e... : 3.2E-05 : 2.7E-07 : -5.3 61-109! :<: 4.2E-06 : : 2.9E-01 : 1.4E-05 : .. :..4.8 "':""i2E:05""":""9'.2i:06":""'i.2"""'

- -~ - - - ---,-- - - - - - -- Cm-243 (Cm-244) ;n D~ y lsofope : Ce-144)

.. .. .. .. .. .. .. .. ... : . : ............... .. : . : .....C~."'.1. ~1-.... :. ............... :........ : Avera9.e, ScaHn9.: Calculated : lso vs. Cale.

$~.l"fl.P.l.E:

10397 N':lf'l'.'l~.E:r::.:

.. 3

!~9~!)P.~ .C!).l'!Q::.:

. * ~.E:Y. !~9 ... C~.l'!Q: :l,:;:q

/.~tY. g~tjo: log lso'iK~*y*.: ......Fact*~~.... :.. i~~: *c~*~~: .. :...

. *:*** ............................................................. 'i:~~*t*~~ ... ..

.. .. ..10398

... .. .. .. .. :* .:. ..... ~~:-R9 8 2E 07 .... :.:

* .. .1. :'?~."'.0;!: .... :* .. J..~~:-P3 ...... :* ..................................................................

-2.7 : 1 .SE-03 : 3.5E-06 : 1.0 .

................. :~: ....*... :-....... : ~: ...~ ,l;l~."'.0::i .... : .. ~.. ~;:-Q~.... : ... -.2 .1 : 1 .8E-03 : 1 .SE-07 : -4 .6 61-1093 : : 2.e.E-05 : : 6.5E-02 : 4.oE-o4 :* ~ix ..... :.... 1..aE.:.oi ...... :.... 1. 2E.:.04": .....4. s.......

Cm-243 (Cm-244) ;n . l ? Y Isotope : Co-60)

- -~ - - - - - - - - - - - - -. -

Liquid Waste Scaling Factor Evaluation

- -" - - - - ... - - - - - - -~.-

'w' .aste .*

......................................i:;:~.--: 1R7.... . .............. :................it,Y.E:(J9.E: .~'?i1.ljr:i9. ..Cil.lP.41.~,~~.. .1~.C! ."<~, .(;:/1.lP.*.

$?1.l"fl.P. l.e: N':'ro~.E:( . !~'?~PP.~ .CP.l'!Q, . l<.E:Y. !~9: ,,:;;~M, l.~9 l~~Y. .~~~i9: .199. !~9/~~.Y. .. .. J ~P.t..Q(. .. .. . .. !~9,. ,:;;~m, .. .. . f ~P.t.ci~ .. ..

. . . . !.Q~:4~...... ~ .. ~.. ~~:-R9........~, 1~:-:0~ ......~li.rri.;ri.~~~~.. : ..... ~.. ~ *......... 7.. Q;:-Q?.......... '?.. ;3:;:-Q~...... 7Q:'~ ..... .

.. .. !.Q~.4~......... ~.. ~~:-R~........4,~~.--:0.1 .......~1imiri.~~~1.. : ..... ~...~ .......... ~.. Q~:-R?.......... 9.. ~~:-R~ ..... .1.?~ . Ei .... .

.. .. !.Q~.4~......... !.. ~~:-R9 ........E;I, 1~:-:0~ ...... ~.. ~~:-R?.... : .... :-.1. ,'? .......... ~.-R~:-R?......... J .. l~:-R9...... :-.1., 1.. .. ..

61-1091 9.8E-03 5.SE-01 1.8E-02: -1.7 2.0E-02 1.1E-02 1.1.

see .attached exp1.an.atfon

................. : . : ............... : . : .... C~.-: 1~?.... :............... :............... :l'1Y.e.r. ~9.e. .~'?~.lji;l9.: ..C~.lP.41.<l~~':i.. : .l~.t! .'(f, .C~JP.*.

~~.rPP.1.e. N':lro~.e.r.::: ,~9~PP.~ .CP.F'!<?,:.: ~.e.Y. ,~9 . .CPn<1, :l.~q IK,Y. R~~i9: .1<?9. !~9/1'.='.!?.Y.: ..... f ~P~.Qr. ...... : .. !~9 ...CP.'1<1, .. : ... f ~P.~.C!r. ... .

10443 :<: 8.9E-06 : : 3.1E-02 : 2.9E-04 : -3.5 : 2.1E-03 : 6.5E-05 : 7.3

.... i'04'44' ..... :.: .. 4°.2E:05' ... :.: .. '2 :e.e:*..:0*1*.: .. :.. i *.6E:ij4' ... :.... :.ie' ..... :.... :i.'t'E:oi ..... :*.... 5*.4E:04": .... i i:6" .. ..

.. .. ,*044s .... *: *: .. ;*.9E:os* ***:*:***a: 1e:*..:04 .... =* **2;3e::oi ***: ****:.*,. :6* *.... :****2*xE:ai *.... :*.. *, *.1E:oe.* *:* .. *..:fr .'1' * .. ..

.. *61 :.*fr19i *.. *: *: .. 9*.eE:oi ***: *: .. "s:ii..:01* ...... *; *.eE:oi ********:.*1* :1 .......... *2'.'1*E:ai *........ *; *.2E:o~.. :*.. *:.*a:4* *.. ..

Se::20 in Liguid :Waste The unmodified S.F. was 2.IE-03: however, this resulted in a nonconservative*

calculated isotopic concentration for sample 10+48. . Therefore. the S.F. was recalculated using the values of samples10-448 and 61-1091, resulting with a co.nservative factor of 2.0E-02. .

- -. To-99 in

................. : .:............... : . : ....C~:: 1~7.... : ............... :............... :.~Y~I'.'~9.E! .~9fj!Jjl'.'IQ. : ..Cfj!JP.'~1.~~~~.. : .l!>.Q .'{f... C~.lP.*.

$~rriP.1.e: N~ro~.E!I'.':.: ,~9~PP.~ .CPJ"!t.?::. :~.E!Y. !~9... Cpnq, :l.~q/.l,;tY. -~~~j9: .1'-?9. ,~9/~~.Y.: ..... f ~P.t..QI'.' ...... : .. !~9: ,l.;pnq, .. : ... f fP.t..QI'.' ... .

.. .. !.Q~~~- ..... :~: .. ~.. ~~:-Q~.... :.: ...~: 1~:-:0~ .... :.. l?.. ~~:-R1 .... :.... :-.~: 1...... :.... '?.*~~:-Q1...... :.... L.~~:-R?.. :.... :-.1. :~.... ; .

. . .. !.Q~~~...... :( .. ~.-~~:-R?.... :.: ...:?,1$~.:0.1 ..... :.. ~.-!~:-R? .... :.... :-.4,Q...... :.... '?.*~~:-Rf ..... :.... J.. ~~".'R1 .. :.... .t? . ~...... .

. . .. J.Q~~~- ..... :~: .. ~.-~~:-Q~.... :.: ...f!,1 ~:-:9~ .... :.. ~.. Q~:-~r~:.... : .... :-.:?,1 ...... :.... P.*~~7Q1...... : .... !;i.. J.~:-R7 .. :... :-:1~ . "? .... .

61-1091 : : 1.4E-04 : : 5.5E-01 : 2.5E-04 -3.6 6.3E-04 !.5E-04 : 2.5 Due to influence of <LLD v alue:s: of Tc-99 J no ot.her s:at.is:fa,::it.or-y S:l.a ling Fact.ors o.an be determined

1-129 in

................. : . : ............... : . : .... Cf-:1 ~7.... :............... :............... :l~Y.~t:"~9.~ .~'?:a.lj,:-i9.: ..C!l.lP.'~1.~~,~-.: .l~.Q -~~ ... C:aJP.*.

$:a.rrrP.1.~ N\lro~~r::.: !~9~PP.~ .CP.1"!C?1:. :~.~Y. !~9... Cpnq, :l.~Q(.~fY. .~~~i9: .1<?9. !~9.l~,.Y.: ..... -~~P.t.Qt:" ...... : .. !~9...CPM: .. : ... f fP~.QI'." ... .

10443 :<: 1.7E-06 : : 3.1 E-02 : 5.6E-05 : -4.3 : 2.1 E-04 : 6.4E-06 : 3.8

- - - 0444* ** ** *
      
      <: **;*.1E:oe.* ***: *: **ie.E*.:0*1* ****: *.6. 6E:os* ***:****:.ii*****:*** *2*:1*E:04* *****:* ***i::i.4E:os* *: ****3*1 :-r* *** **

i:Qi4~:::::: 1: 1:: i.i:!~7i:!~:::: 1: 1:: :~; i~:~o~:::: 1:: ~-~~7Ri::: 1:::: ~:1:; i:::::: 1::: :iJ~7Q~:::::: 1::::; :.j~7Rf: 1:: :~~:1: f:,:::::

61-1091 :<: 3.3E-05 : : 5.5E-01 : 6.0E-05 -4.2 2.1E-04 1.tE-04 : 3.5 see attached discussion*

1-129 in Liui.4 Yaste The reported concentration of the key isotope of sample lO+tS is suspect due to its low concentration relative to the other samples. As stated in the discussion, the most representative sample is 61-1091 due to its mixture characteristics as per typical shipmen ts.

- -~ .. C-14 in L

'aste

.............*.... :;: ............... :.: .....G9:-.~9..... : ............... : ............... : .~Y.E:r:J9.E: .~9".lji;i9.: ..C".lP.41.~~~~.. : .l~.q .'!,... C".lP.*.

$~.l"fl.P.l.e: N':lro~.e:r::.: !~9~P.P.~ .C!>.l'!Q::.: l:<.e:Y. !~9... CP.l'!Q: :l.~<?/.~f!J. gf~j9: .1<?9. !~9/'>,.Y.: ..... f fP.t.qr; ...... : .. !~9... CP.r!Q: .. : ... ff P.t.cir: .. ..

... 'i10443

'04'44 ...... :.:: : 1.SE-04 : : 4.8E-02

.. 7.2E:.04' ... :.: .. *; :2E~cfr .... :: .. 3.7E-03 6 OE:.oi ... :: .... :.:2

-2.4

'i' ..... :: ... *;1.3E-02

!E:.oi' ..... ::... *;6.4E-04

&:.oi.:: .... ':i'3.5i' ..... .

::::;:rj~:4~:::::: 1: 1:: :,j~~ij,f::: 1: 1::) ;~~:~o~:::: 1:: ~:\~i~Ri:::: 1:::: ~)}::::: 1:::: L~i~Ri::::: 1::: :i\i~R~:: 1:::: ~i{:::::

61-1091 : : 2.0E..;02 : : 6.8E-01 : 2.9E-02 -1.5 1.3E-02 9.0E-03 : -2.2

-- - ' - 1]11111 Fe-55 ;n U

................. : . : ............... : . : .....G9:-~9..... : ............... : ............... : .~Y.E!l'.'~9.E! .~9~.1ji;i9.: .. c;::~JP.41.~~~~-.: .1~.Q .'<~: ,c;::~.lP.*.

$~,ITIP.1.E! N1,1ro~.E!I'.':.: !~9~!>.P.~ ,c;::!>.l'!C?::. :l:<.E!Y. ,~9: ,c;::!>nC?: :I.S;q/.lS,~ .~J~i9: .1Q9. !~9/~!?.Y.: ..... f ~P.~.QI'.' ...... : .. !~9.. ,c;::p.riq: .. : ... f ~P.~.QI'.' ... .

10443 : : 4.1E-02 : : 4.SE-02 : 8.6E-01 : -0.1 : 7.6E-01 : 3.6E-02 : -1.1

.. ,*0444 .... *: *: .. 2.9E:.o:i' .. *: *: .. *; :2E*.:(fr .. **: **2.4£:.01 .... :.. **:.:ai *.... :****1*.e:E:01 ****.. :****9*.oE:oi *:* .. *IX ......

.:::(q~:'l~: :: :::1 :1 ::f~i7Ri : :1 :1:: :1: ;~~:~o~:::: 1: :i~i~:tjp:: : 1::: j,)( :: ::::1::: ):.~~7Rt:::::: 1:::: (ii~Ri: 1:::: ~ii:::::

61-1091 : : 4.oE-01 : : 6.8E-01 : 6.oE-01 : -0.2 : 7.6E-01 : 5.2E-01 : 1.2

-.-~ - Ni-63 in 'w'aste

. . ................ : . : ............... : . : .....G9:--.l:?9..... :.... *........... : ................~Y.e.r.~9.~ .~9~.lj,:.9.: .. C~.lP.41.~~'?~.. : .IF.C! .'<f... C:a.lP.*.

$:a!'l'li'ci~-~~n;l~~r:\. i !~9~PP.~ .CP.1'19, (. (~-~Y. !~9... Cpnq, /~1-?(~~Y. R~~i9( .1t-?9. !~9/~!!'.'J° ...... f ~P.t.C?r: ...... : .. !~9:.GPf!<l, .. : ... f ~P~.C!I'.' .. ..

. .. .. 1..0444

.. .. .. .. .. . .:~:. .. 1L-~~-:-R' 9E O f .... :.: * * ...i,e~.-:9~ .... :* ..~lt,rn1ri.~~'?d.

* . . *: . . . . . N.A. 4.0E-01 1.9E-02 : 120.5 .

1044~ ,.:.: .... -... -:- .. 'f .... :.: ... 1.,:?~.-:9.1..... : ..~11rri1ri.ated,. N.A. 4.0E-01 . 4.8E-02

. . ...................................................................... : 252.6 .

- - s1 ~*1*09i* ** */ *1 *1:~~:gr * * *l::~*:z~ * ** *i*:;~:m ****i * ** *:g:;, ***** ****:*:§~:m ******:. **1:9~:§r-* :. * *Y=t **

l

1*

1*

see at.taohed e,xp lanat.ion

- - - ---- .. - - Ni-6! in Liquid 'v.'as:~e- ified Sea ling Factor

. . . . C 60 . . .

. . . . . . . . . . . . . . . . . : . : ............... : . : ...... 9:-........ : ............... : ............... : ...~Y.E:l'.'~9.E: .~9~.1)1'.'19.: .. C~.lP.41.~~~~.. : .l~.Q .'<~ ... C~JP.*.

$~.rnP.1.ie: .~l,lfl'.l~f:!1'.':.: !~'?~PP.~ .CP.l"f<?::.: KE:Y. !~9... C?n<?: :l~q /.~~Y. .~~~)'?: .199. !~9/1$!?.Y.: ..... f ~P.~.Qt:' ...... : .. !~'? ... 9P.l"f<?: .. : ... f ~P.~.Qt:' ... .

.. .. J.Q~.4~...... :~: .. J..R;:-R~.... :.: ...'Le~:-:9~ .... : .. ~.. R;:-R~.... : .... :-14:~ ...... : .... ~.-.1.;:-Q? ...... : .... J..~~7Q~ .. : .....~ . L .... ..

.. . . !.Q~.4~...... :.: .. J..~;:-Q~.... :.: .. .1.*:?~:-:9.1 ..... : .. 1.,R;':'Q~.... : .... :-.:?,e...... :.... ~...t.;:-R:? ...... : .... ~A=:;:-R~.. : .... r~: 1..... .

. . .. J.Q~.4~...... :.: .. ~.,R;:-R~ .... :.: ...1.*~~:-:9~ .... : .. ~/~~:-R1 .... : .... :-.Qi~ ...... : .... ~.. J.;:-Q?...... : .... ~.. l;:-Q~.. : ....'":rn..1. ... ..

61-1091 : : 2.0E-01 : : 6.8E-01 : 2.9E-01 : -0.5 : 3.1E-02 : 2.1E-02 : -9.6

lfi-63 in Liguid Jfaste The unmodified S.F. was 3.lE-02: however, this resulted in a nonconservative calculated isotopic concentration for sample 10.<<8. Therefore. the S.F. was recalculated using the values of samples 10<<8 and 61-1091, resultins with a conservative factorof .f.OE-01. .

- - - - - - - _... .. - - ..... - - - sofope : Ce-1 44)

................. :. . :. ............... :. . :. .....C~:-: 144

........ :. .... :.......... :. ............... : *"Y.e.r. ~9.e. .~9~.lj,:ig :.. r;~JP.41.~~,~- . :.l~.Q .'<~:. Cil.lP.*.

$~.'Tine. -~~ro~.e.r.:. :!~9~P.P.ct .CP.l"!Q:: . :Ke.Y. !~9:. CP.r!Q: :I.S:Q m~Y. .l~~~j9: .1Q9. !~9/~!?.Y. : ..... f ~P.t.qr, ...... : .. !~9: .l;Pf!Q, .. : ... f ~P~.QI'.' ... .

.. . .. ..~- ........ :.: .. ~.-.1.t*R4.... :.: ..."? :9~::9~ .... : .. ~--~~:-R1 .... :.... :-.Q:?...... : .... 7.."J.~:-Q1 ...... : .... ~--~~:-Q4.. :..... 1. ~...... .

. . ... LQ~.4,...... :.: .. 7.-~~:-Rf ... : ~: ...:?:~~::9~ .... : .. :;2.. !~:-Ql .... :.... :-.Q:~...... : .... 7.,!~:-Q1 ...... : .... f .. ~~:-Rl.: .... .~:~...... .

.... ,.o~.4~...... :.: .. , .. ~~:-R4.... :.: ...4:~~::0~ .... :.. ~--~~:-Ql .... :.... :-.0,?...... : .... 7..'J.~:-Ql ...... :.... i .. Q~:-Q4.. :..... 1. i ...... .

61-1091 : : 8.lE-03 : : 2.oE-05 : 5.5E+OO : 0.5 : 7.7E-01 : 1.SE-05 : -4.6

- - - -* - ... - .. Pu-241 in Liquid Was:t Isotope, : Co-60)

IIIJ

. . . . C 60 . .

, , .... , ... , , , , , .. : . : ............... : . : ...... 9:-........ : ............... : ............... : l'!'Y~r:~g-~ .~9~.lji;ig: .. C~,lp,i~l.~~~~ .. : .l!>.Q .'(~ ... r;~,lp,.,

10l,e; .~':l~~.e:r::

$il.l'fl.P. 43 .:!~9~PP., .C~:in<?:: . :~.E!Y. !~'?... r;pnq: :I.S;q I.IS'?Y. g~~j9: .1<?9. !~9 /.K,.Y Factor : lso. Cone.

- - - - : Factor .

.. .. .. .~\ ....... :.: .. , ...t.~:-Rt. ... :.: ...4:f=3~::9~ .... :.. ~.*R~:-Q? .... :.... :-.4: 1...... :.... ~.. ~~:-Q? ...... :.... ~.. ~~:-Q4 .. :..... LL .... ..

. .. .. !.0.~. . 4...... . : . : .. 7.. ~~:-R4.... :.: .. .1. :?~::OJ. .... :.. ~.*R~:-P?.... :.... :-.4:?...... :.... ~.. ~~:-Ql ..... : .... J...1.~:-Q~ .. :..... 1..f .... ..

10 4 4 8 : : 1 .GE-04 : : 1.6E-02 : 1 OE-02 : -2 0 : 9 2E-03 : 1 4E-04 : -1 1

.. *ti, ~*fr;9; ****: *: .. e*:1*E:oi .. *: *: .. i:eE*~o*1* .... :**;*:~if:i:ii' *.. :*.. *:.:,. \~* ***.. :*.. *9*:2E:oi...... :*.. *s*:2E:oi *: *.. *~*1* '.i *....

- - ----*- .. .. - - *- - - Cm-242 ;n Uqu;d 'w'asi Isotope : Ce-1 44)

. . . . C 144 . . .A S 1' . C .

.. * * .. .. .. * * .. .. *: *: ............... : * : ..... !?."": ........ : ............... : ............... : ** Y.e:r.?19.E: .. 9~. ,i:-9.: ... ~.lP.1..11.-,~~~ .. : .l~.C! x~ ... C~.lP.*.

$~.rri.P.1.e: N'='ro~~r.:.: !lf9~!>.P.~ ,i;:!>.l"!Q,:. :~.E:Y. !~9: .CP.l"!Q, :l.~q/J~tY. g?i~j9: .1Q9. !~9/~l?.Y.: ...... ~ f P.i.Qr. ...... :.. !~9: .CP.l"!Q, .. : ... ff P~.C!r. .. ..

.. .. LQ~.4~...... :.: .. ~--~~:-R9 .... :.: .. :u;.1~.'":9~ .... :.. t~~:-Q?.... : .... :-.1.* ~ ...... :.... L-~~:-Q?...... : .... ~.-:!!~:-Q9.. :..... L9..... ..

. .. .. LQ~.4~...... :.: .. ~.J:~:-R~.... :.: ...~,~~.'":9~ .... :.. 1.. ~~:-Q?.... :.... :-.1.*~...... :... .1.-~~:-Q?...... : .... ~.. ~~:-Q~ .. :..... LL .... ..

.... J.04.4~...... : .: .. i ..R~:-R~ .... :.: ...4,9~."'.9~ .... : .. 7..l~:-Q~.... : .... :-.::?,1 ...... :.... 1.-~~:-R4...... : .... ~.. ~~:-Re. .. :..... 1:~... ... .

61-1091 * : : 6.2E-05 : : 2.3E-03 : 2.7E-02 :* -1.6 : 1.4E-02 : 3.1E-05 : -2.0 *

-- - - - - 1111 . .

Cm-242 in Liquid Was:

Isotope : Co-60)

. . . . C 60 . . .. . . .

................. : . : ............... : . : ...... 9:-........ : ............... : ............... : /w.e.r. ~9.e. .~911.l1i:i9. : .. C11.1p_41.~~~~- . : .1~.C! .'{~:.C~.lP.*.

$11.l'fl.P.1.e. N':'ITl~.e.r.:.: !~9t!>.P.~ .C!>r!Q::. :~.t?.Y. !~'?: .CPr!Q: :l.~q/.lStY. -~~tj'?:. lqg, !~9/~!?.Y.: ..... f ~P.t,qr, ...... : .. !~'?: .CP.r'!Q: .. : ... f ~P~.C!r. ... .

.. .. LQ~.4~...... :.: .. ~-.~~:-R~ .... :.: ...4:~~.-:0~ .... :.. L-~~:-Rf ... :.... :-.q:7...... :.... 1A~:-R'1...... :.... 7.. J:~:-R~ .. :.... :-.1. :?..... .

.. .. !.Qf4~...... :.: .. ~.-~~:-R!:?.... :.: .. .1. :?~.-:0.1..... :.. ~.. Q~:-R'1.... :.... :-.q:!:?...... :.... U=!~:-R'1...... :... J .. ~~:-R!:? .. :.... :-.1. :~.... ..

. . . . J.Q,.4~...... :.: .. f .. Q~:-R~ .... :.: .. .1. =~~:-:0~ .... : .. L-~~:-Q'1.... : .... :-.~:~...... : .... U=i~:-Q'1 ...... :... -~--~~:-R~.. : ..... 1.. ~... ..

61-1091 : : 6.2E-05 : : 6.SE-01 : 9.1E-05 : -4.0 : 1.6E-04 : 1.1E-04 : 1.8 ..

- - - - - ..... - - - -*- - -,; - Pu-238 in Liqui~ Wast Isotope : Ce-1 44)

.................:. .:. ............... .:.:' .....C~."'. 144

........ :. ............... :. ............... :. .i',Y.E!r:~9.E! .~9~.1]1'.'19. : ..C~.lP.41.~~~~-. : .l,.Q ."<~:. C~.lP.*.

$~.rflm~*:~ro~.e:r:j. ! !~r;~!tfl<?, ! '. jl<,ef bi~o~onq, /'*~~l.~:_~1ol~~j91 .1Q9:_!~~-:-~!?.Y. j..... J~P!.Qr: ...... (.. !~9:.CP~Q, .. (... f ~P.t.Qr: ... .

.... .. . . . . .. .. .. .: .:... ,*,, ................ :............... ,*, .................4: ............ 7.-.1.~. !=!9...... : ... -~--!=!~.QI!? .. :..... 1:?...... .

.. .. J.0~.4~...... :.: .. ~.-~~:-R~.... :.: .. ~.~~."'.O;!i .... : .. ~.. Q~:-!=!9 .... :.... :-.::?.~...... :.... 7...t.~:-Q9...... : .... ~.-.1.~:-Q~.. :..... ?. ~..... .

.. .. J.0~.4~...... ! . ! .. 7.-~~:-R?.... :.: ...=?,11?~.-:Q~ .... :.. i .. ~~:-Q~.... : .... :-.=?.~...... :.... 7.-.1J:-Q~...... : .... 1..~~:-RII?.. :.....~. ~- ..... :

61-1091 1.6E-04 * : : 2.:0E-03 : 7.0E-02 : -1.2 : 7.1E-03 1.6E-05 : -9.8

- - ------ - - - - - - -.r - _Pu-239 in Liquid 'vr' as lso~ope : Co-60)

................. : . : ................ : .....G9:-.~9..... :............... :............ ;.. : l~Y.~t:'~9.~ .~9i1.lji;i9.: ..Cil.lP.41.~~~~-.: .1,,q .'{~:.Cil.lP.*.

$~.l'flP.l.~ Ni,,ro~.~t:':.: !~9~P.P.~ .CP.l'lQ: . :l.<.~Y. !~9,.C9.1"!Q, :I.S:Q/.~,Y. -~~~j9: .1Q9. !~9/~l!'.Y.: ..... f ~P.~.Qt:' ...... : .. !~9,.Q91'!Q: .. : ... f?P~.Qt:' ... .

10443 . : : 2.9E-06 I00000000IIOOIOOOIIOIOIOII001111111 000110 4.SE-02 1110 11010000

6.1 E-05 110010010010 1111101111

-4.2 I

9.5E-05 IIOIIIIIOIOOIIOOOII

4.1 E-06 :

IIIOIIIIIIIOIIIIIOIOIIIIIOOOIOIIOI 1.4 10111111

.... J.Q~.4~...... :.: .. ~.-!:!~:-Rt? ..... : .. .1..?~.":9.1..... :.. 7.-~~:-R~.... :.... :-.4:1 ...... :.... ~..:=~~:-R~...... : .... LR~:-R~.. : ..... L!. .... ..

.. .. J.Q~.4~...... :.: .. 7.-!=:~:-R?..... : .. .1. :E?~.":0~ .... :.. ~--~~:-Q9 .... : .... :--.'L~...... : ... ,1;3):i~:-Q9...... : ... J .-~~:-Q9.. : ..... L?..... ..

61-1091 . : : I .6E-04 : 6.SE-01 : 2.4E-04 -3.6 8.5E-05 5.SE-05 : -2.8

- - - *- - - - .. ----*-- - - *~ Isotope : Ce-144)

................. : .: ................ : . : ....C,.-.1 ~':l................... : ............... :."iY.e.r:~9.~ .~9~.ljr:ig,: ..C~.lP.'~1.~~~~ .. :.ll>.C!X~:.C~.lP.*.

~~rriP.1.~ Ni,aro~.~r::.: !!!~~PP.~ .CP.r!q::. :l<.~Y. !!!9: .CPn<?: ,.~<;i/.lS,Y. g~~]9: .1Q9. ,~9/~~.Y.: ..... f ~P.\C!r: ...... :.. ,~9,.Cpnq: .. : ... f ~P.t.C!r: ... .

. ... !.Q1~~- ..... :.: .. L-~~:-R~.... :.: ..."UJ~:-:0~ ..... J .. ~~:-Q~ .... :.: .. -:-~:? ...... : ... -~--~~-:-!=!~ ...... : ... -~--~~-:-Qi;, .. : ..... 1.-7..... ..

.... 10444 : : 4.4E-06 i044Ei ..... :.:

0

: 2.9E-03

.. fsE.:.07' ... :.: 1.5E-03

.. iei..:04 ...... 9°.6E.:.04' ... :: .... :..*io'

-2.8

..... :: .... ~;°.2E.:.oi 3.2E-03

..... :: .... ~i.2E.:.07'.:

9.1E-06 :

.... i2.13' ..... .

.. *6; ~*,o*9i ... *: *: **s*.4E.:.i:ii ***: *: ***2:ir*..:oi **** **i1E.:.oi' ***: ****:. .*1 :4* *****: ***:i2e::. oi *****:* ***1.~E.:.06* *:* .. *..:; *;*.i ****

Since there is no influence from <LLD values, there is no obvious route to modify Soa ling Factor

- - ------ - - - - - - -**- - Am-241 ;n Liqu;d Wa . y Isotope : Co-60)

./

. . . . . . . . . . . . . . . . . . .: ............... .: . .: ......C9:-..60...... .: ............... :. ............... :. ..AY.E:t:-J9.E: ..S9:a.1'1r,9. :. . ;C

. :a.1P.',~1.~\~~

.. : .li>,q .'l!f: .C:a.lP.*.

~:arriP.1.e: N':lrot,~r;- . : !~9~!>.P.~ .C!>.l'l<?,: . : ~.E:Y. !~9: .CP.I'!<?, :l.~c;i /.IStY. .~,~j9: .1C?9. !~9/~,.Y.: ..... f JP~.qr: ...... : .. !:!!9: .CP.1'!<?: .. : ... f ?P~.o/. ... .

.. .. !.Q~.4~....... : .. J..~~:-R9.... :.: ...4,~~::9~ .... :.. ~.,:7'.~:-R9.... : .... :-.4,9...... :.... ~A=!~:-!=!9...... : .... J..!;:!~:-RE?.. :..... 1. , ...... .

.. .. !.Q~.4~....... : .. ~.. ~~:-R9.... ~.: ...1. ,4~."":9.1..... : .. ~..J:~:-R9.... : .... :-.4,~...... :.... ~A:~~:-Q9 ...... : ....i:i..~~:-RE? .. :..... 1:0...... .

.. .. !.Q~.4~....... : .. i ..~~:-R7. ... :.: .. .1. ,E?~."":9~ .... :.. J..~~:-Q9.... :.... :-.4,e...... :.... ~.. !;:!~:-Q9...... :.... !;i..!;:!~:-Q7.. :.....:?. ~..... ..

61-1091 : 8.4E-05 : :

6.SE-01 : 1.2E-04 : -3.9 : 3.SE-05 : 2.6E-05 : -3.3 *

- -~ - - - ---,--- - - - -.- - Pu-239 (Pu-240) in Liquid ' (K,e,y Isotope : Ce-144)

...r

. . . . C 144 . .

................. : . : ............... : . : ..... ~.-: ........ : ............... : ............... : ."~Y.!17 ?9.~ .~9~.ljl)g_ : ..C~.lP.41.~~~9.. .11>.C! .°'<~: .G~JP.*.

$~.rPP.1.! .~\IITl~.~r::.: !~9~P.P.~ .CP.11C?,:.: ~-~Y. !~9: .GP.1'1'1, :l.~9 mfY. .~{l~j9: .199. !~9/f-::'.!?.Y.: ..... f ~P~.C!I'. ...... : .. !~9, .Gpnq: ..... f ilP~.C!I'. ... .

.. .. 1.Qf49...... :.: .. 7.-R~:-R9.... :.: .. ."?:0~.-:0~ .... : .. i .. ~~:-R~ .... : ... : :-.:?:9...... : .... ?.-~~:-R~...... :.... ~.-.1.~:-Q9..... .. ?. 1. .... ..

.. .. J.Q~.4~...... : .: .. ~.-~~:-R9.... :.: ...4,~~.-:0~ .... :. -~--~~:-Q~.... : .... :-.4:9...... :.... ?.-~~:-Q~...... : .... L-l~:-Q!;i .......?. !;)..... ..

.. .. !.Q~.4~...... : .: .. i ...t.~:-R9.... : .: ...:?,9~:-:0~ .... : .. ~.-.1.~-:-Q~.... : .... :-.4,1 ...... : .... ?.-~~-:-R~...... :.... L.~~:-Q9...... :-.1.* ~ .... ..

61-1091 : : 5.0E-05 : : 2.oE-03 : 2.2E-02 : -1 .7 : 5.9E-03 : 1.5E-05 -3.7

- ---- - -1*- - -

Pu-239 (Pu-240) in Liquid (Key Isotope : Co-60)

.. .. .. .. .. .. . .. . .: .: ............... : .: .... .G9:-.~9..... :............... :............... :.i'~Y.E!t:-i19.E! .~i;:~Jii;i9.:. Calculated : lso vs. Cale.

$~.rrm~-~in:i~.e:r: 1.1,~rPP.!.CP.r'!<?, 1.~ l<.E!Y. ,~9, .C9M, 11.~q 1.~,Y. R~~i9~ .1<?9.,~91~,.Y .1 ..... f ~P~.Qt: .. : ... 1. :i~9:. :GP.rl<?::: 1::: i ~9:t:q~:: ::

................. : .: .... -R~. R~ .... :.: ...4:f;:!~:-:0~ .... : .. ~--~~:-R~ .... :.... :-.4 ,~...... :.... 7.-R~:-R~...... :.... ~--~;:-Qt$ .. :..... 1. 7... .

10444

.: 6 -...........

BE-06 . * ...1.,.~.-:

.: 2 0. .1 ..... *: .. !;5.. !~:-J:!5 . . ** -4.2 ** 7.0E-05 ** ,

8.oE-06 ** 1.2 ...

10448 : : 2.lE-06 : : 1.6E-02 : 1 4E-04 .. :* .. *:_*.;.*.;"*"*:""1***o*E**:.'0'5""'":""'"1*E*:*****:****:_**********

................. : * : ...................................... ,*, ................ -~:? ............ ,*, ................. , ...... Qt$ .. : ..... .1.*~ .... ..

61-1091 5.0E-05 .. 6.8E-01 : 7.4E-05 : -4.1 : 7.0E-05 4.SE-05 -1.1

- - - - - - -:- -**- - -*- - ** Pu-242 (Np-237) in Liquid e (Key l:s:ot.ope : Ce-1 44)

............ ;.... : . :.................... C~.--:1 ~4 ............... :... : ............... : ."~Y.~t:~9.~ .~9!1.lii:-t9.: ..!;!1.lP.41.~~~~ .. : .1~.C! .'{?:.C:a.lP.*.

$:afflP. l.~ .~ ... ro~.~r:: .: !~9~9P.~. f,;p,riq: . l<.~Y. !~9,.(,;pf!q, l.~9 l.l~~Y.* .~11~i9: .199. ,~9 /~!?.Y . : ..... f ~P.t..QI'." ...... : .. !~9,. CPM, .. : ... f ~P.t..Qt: ... .

.. .. !.Q~.4~...... :.: .. u~~:-R?........( ,or--:o~ ...... 1..:-i:~:-R4.... : .... :-~.~- ..... : .... i:'-.-~~:-R'f ...... : .... ~.. ~~:-R7 .. : .....~ . 7..... ..

. . . . !.Q~.4~...... :.: .. !.-.1.~-:-R7........4,~r--:OR ...... ~.-~~-:-R~ .... : .... :-.4,4...... : .... ~-.~~:-Q<f ...... : .... !.*R~:-Q9.. : .... J.4, 1..... .

. . . . LQ~.4\3...... :~: .. ~)~~-:-Q7 ........4,9~::9~ ...... J...1.~:-Q~.... : .... :-.~,Q...... : .... ~.. ~~-:-r.:!4 ...... : .... J..~~:-r.:!7.. : .... :-.4,4.... ..

61-1091 :<: 1.4E-05 2.3E-03 6.1E-03 : -2.2 : 4.6E-04 : 1.lE-06 : -13.3 Eliminat.ion of <LLD v alue:s: for :s:amp Jes 10448 and 61 -1 091 would rl?sult. in a le:s::s: c:onserv ative Soa ling Fact.or

- - - - - - - - -- -- -'- - -- -~ Pu-242 (Np-237) ;n L;qu;.e, (Key Isotope : Co-60)

.................................. : .....G9:-.'~9..... :............... :............... : .l,Y.~r:ft!l~ .~9~.lj('l9.: ..C~.lP.41.~~~~ .. : .l!>.Q ."<, ... C~JP.*.

~~.rri.P.1.~ N':'ro~~r: . !~9~!>.P.~ .C!>.11Q: . :K~Y. !~9... C9f!Q: :l.~Q !.IStY. .~fl~j*i .1<?9. !~9/~,.Y. : ..... f flP.t.cir: ...... : .. !~9: .C~>nQ: .. : ... f ftP.t.qr: ... .

. . . . !.Q~.4~........ *. !.-~~:-R?..... : ...4,e~::Q~ .... : .. i .. ~~:-R9 .... : .... :-.~:9...... :.... !?.-~~:-R9...... : .... ~.. ~~:-R7.. :.....4:f...... ..

. . . . !.Q~.4~......... J..J.~:-Q7. .... : .. .1. ,4~.-:9.1..... :.. ~.. ~~:-Q?. ... : .... :-.~.Q...... : .... !?)~~:-Q9...... : .... '?.. ~~:-R7.. :.....~.. ~- ..... .

.. ..!.Q~~~- ..... ~ .. f ..~~:-R?. .... : .. .1. ,l:?~.-:Q~ .... : .. J.. ~~:-Q~ .... : .... :-.4:7...... : .... ~.. ~~:-R~ ...... : .... (3..~~:-R~.. : .... :-.~.-:J..... .

61-1091 < 1 .4E-05 : 6.8E-01 : 2.1 E:-05 : -4.7 : 5.5E-06 : 3.7E-06 : -3.8

- -* ------ - -**- - - - - --- Cm-243 (Cm-244) ;n Uqu;d Key Isotope : Ce-1 44)

................. :. . :. ............... :. . :. .....Cf:'.-. 144 .. Y.E:I'.' 'i19.E: ..S9~.1'1r:i9. :. .. C~.lP.41,i!~~~ .. :* .l~.C! ."<~:. C~JP.*.

........ ,:. ............... :. ............... :'A

$~.rr*P.l.e: N':'ro~.e:r::.: !~9~!>P.~ .C!>.r!Q,:. :KE:Y. !~9: .C!>f!Q, :l.~q/KfY. .l~~~jf, 1<?9. !~9 /~,.Y.: ..... f ~p~~I'.' ...... : .. !~9 ...Cs:inq,;.: .. .f~P~.C!I'.' .. ..

. . . . !.Q~:4~...... :.: .. J..~~:-1=!9 .... :.: ...1 ,Q~.-.O~ .... : .. ~..J.~:-R~ .... :.... -:-.~:?...... :.... 9.*~~:-Q9...... : .... i.}F;:-Q9.. :..... 1. ~...... .

.. ..rn,.4~...... :.: .. ~. ~F;:-A9.... :.: ...~.~~.-.Q~ .... : .. J..~F;:-R~.... :.... -:-~.~...... : .... 9..'.=~F;:-R~...... : .... J...1.~:-R~.. : .....?. ?...... .

. . .. !.Q~.'l~...... :.: .. 7A=:~:-A7.... :.: ...~,9~.-.Q~ .... :. ,:;?,.~F;:-Q9.... :.... -:-.=?,9...... :.... 9.. ~F;:-Q9...... :.... J.. QF;:-QE;>.. :..... 1.. ~...... .

61 -1 091 : : 6 .OE-05 : : 2 .3E-03 : 2 .6E-02 : -1 .6 : 3. 9E-03 : 8. 9E-06 : -6 .8

- - ------ ------- Cm-243 (Cm-244) in Liqui e (Key Isotope : Co-60) r

... ;........... :.: . ' 60

......C9:-........ :' ............... :. ............... :. ..AY~r:-!19.e. ..S9~.1',1'.'19.:. .. c~.1P.41.~~~~ .. .: .1,.C! .-<?: .c~.1P.*.

8. ~!'flP.cie. N~ro~~I'.' j. \!:!!9~!>P.~ ,(;frtfi: \. ~~.e.y. !:!!9, .(;Pf!<?: 11.~q /.1-~~Y. Pil~i9i .1qg, !:!!9/t::'.!!'.Y

1* .... f i!P.t.C!r: ...... : .. !:!!9, ,(;pnq: .. : ... f ~P.t.C!r: ... .

. . *. J.. ~.4 ....... :.: .. J.* ~~:-Rr;,.... : . : ...4:!;:l~.-:9~ .... : .. ?:...1J:-R9.... :.... :-.4,9...... : ... -~--R~:-R9 ...... :... -~--~~:-R9.. : ..... 1. ~...... .

**rn::t *** *) *[**t~~:§~* ** *) *) ** -~-:~~-:g~ * * *t;~:§;* ** )* * -~:i* *

j* j * *. -~--~~:R9 ...... j .... ~.-~t:R!? .. /* .. *:.Lf ..... .

.. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . ,............. ~.-~~. R9........... 7.-.1.~. R7........ .I., 1..... .

61-1091 : : 6.0E-05 : : 6.8E-01 : 8.SE-05 : -4.1 : 4.6E-05 : 3.1E-05 : -1.9

Primary Filter Scaling Factor Evaluation

- - \- - - - - - --- - - - - -. -- Sr-90 in Pr, Fmer

............ : .... :. : ............... : . : ....C~:-: 1~?.... :............... :............... :.~Y~r: ~9.~ .~9i'.lji:i9. : ..Ci'.lP.41:~~~~-. : .li>.C! .'<:P:, ,i'.;i9.1P.*.

$i\l.l'flP.l.~ .~i,iro~.~r::.: !~9~!>.P.~ .C!>.11<?::. :~.~Y. !~9, .C!>.l"!Q: :l.~q/.lStY. .l~~~j9: .11?9. !~9/~~.Y.: ..... f JP.~.C!r: ...... : .. !~9, .C!>.I"!<?: *. : ..* ff P.~.C!r: .. ..

.. . . !R?.~J. ..... :~: .. !.-~~:-R?.... : ~: .. .1. :~~.":O.Q .... : .. J.-~~:-R?.... : .... :-.1. :~ ...... : .... ~--R~:-R?...... : ... -~--~~:-R?.. : ...*..?i, J. ..... .

.. .. J.Q9_~i...... :.: .. J..:i'.~:-R1 .... : ~: .. .1.: 1~:t:O.Q .... : .. J..~~:-R1 .... :.... :-.Q :e...... :.... ~--R~:-R?...... :.... ~--~~:-Q?.. :.... :-.~ =~* .... .

.. .. LQ?.~9...... :.: .. ?.-.1.~:-R?.... : ~: .. .1. :e~.-1:0.Q .... : .. 1..1~:-R?.... :.... :-.1. :e...... :.... ~--R~:-R?...... :.... 7.-~~:-R? .. :.....?,9..... ..

.. ..!.Q?.~~- ..... :.: .. u:1~:-R?i.... : ~: ...4i~~:-:O~ .... :. -~--~~:-R?.... :.... :-.1. :9...... :.... ~--R~:-Q?...... :.... J.. J'.~:-R~.. :..... 1,7...... .

.. .. J.Q?.~~- ..... : . : .. J.-~~:-R?.... : ~= .. .'..?:?~.-:0.1..... :. -~--~~:-R? .... :.... :-.1. :?i...... :... -~--R~:-R? ...... :... -~--:-.1'.~:-R?i.. :.... :-.1. :?i..... .

.. . .!.Q~.~'?...... :.:. -~--~~:-Rl ... : ~: ...1. :'f~:-:Q.1 ..... : .. 7.-~~:-R? .... : .... :-.1. :9..*... : .... ~..Q~:-R?...... :.... ~-.~~:-R?i.. : ..... 1,7...... .

.. .~ 1:-.1. O.~~- ... : .: .. '?.-i!i~:-Rl ... : .: ...~ :?Kt:O.Q .... : .. 7.. Q~:-R?.... :.... :-.1. :?...... : .... ~.. Q~:-Q?...... : .... J.-~~:-R1 .. : .....?. O..... ..

.. . ~-1 :-.1. 9.~0.... :. :.. ~--R~ :-R?.... : . : ...~ :~~:-:0.1..... :.. ~--~~ :-R?.... :.... :-.1. =~ ...... : .... ~.. Q~:-R?...... :.... ~--!'.~ :-R?.. :.... :-.1. 1..... . =

61.=1092 _ 6.6E-O~ 2.2E--02._ : 3.0E-01 : -0.5 : 4.0E-02 : S.SE-04 :_ -7.5

- - - - - - -*- -----*-- -- To-99 in Pr Filter

......: ......... : . : ............... : . : ....c~.'": 1~?.... :............... :............... :l~Y.e:r: ~9.e: .~i;,i:1Jjr;'l9. : ..ci:1Jp_41.~1~~-.: .1~.Q .-<,: .ci:1Ji:i.. .

$~.l"fl.P.l.e: .~'iJro~.e:r::.: !~9~!>.R~ .C!>nC?::. :l<.E:Y. !~9 *. CP.l'!'-1: :I.~<? !.ISfY. .l~~~j9: .1<?9. !~9/~~.Y.: ..... -~ ~P.t.Qr: ...... : .. !~9 *. Cs>nC?: .. :... { f~.t.Qr: ... .

.. .. !.Q~.~L ..... :~:. -~--~~:-R~ .... : ~: .. .1. :~~:t:9.Q .... : ..~1i.rnin~t,~~-.: ..... ~.. /~: ..... :.... L-~~t.Q9...... :....?.~.~tQ9.. :... ~~~-.E! ... ..

. . . . !.Q~.~~- ..... :~: .. ~--~~:-R~.... :~: .. .1.: 1~.i;9.Q .... :. Jli.fTl.ifv~t,~~-.: .... .~../~: ..... : .... J.-~~t.Q9...... :....?,9.~tQ9.. :... ;.?;~~JJ .... .

.. .. !.Q~.~~- ..... :~: .. ~--~~:-R~.... : ~: ...1. :e~.i;9.Q .... : ..~1imiri."~~~ .. :..... ~.. /~: ..... :.... J.-~~t.Q9...... :....~:~.~tQ9.. :... i!:4.1...~ .... .

.. .. !.Q~.~~- ..... :f .. !.-~~:-R'f.... : ~: ...4:~~."":9~ .... : ..~1i.fTl.iri.~~~~ .. :..... ~.. /~: ..... :.... L-~~t.Q9...... :.... 7.. ~~:-Q?.. :... ~ 1~ . ::? .... .

.. . . !.Q~.~~- ..... :~: .. 9.-i!if:*Rf ... : ~: ...~.?~:-:9.1..... : .. ~li.fTl.in"1fl~ .. : ..... ~.-l~: ..... :.... JA~~t.Q9...... : ... .~.-~~:-Ql .. : ... ~?~-.:? .... .

.. .. !.Q~.~9...... :~: .. !.-H:-R~.... : ~: .. .1. :'f~."":9.1..... : ..~hfTl.il'l."~~~.. :..... R.~, ..... :.... J..~~:+-.Q9...... :.... i .. ~~:-Q1 .. :... ;2;~.1...E! ... ..

.. .~1 :-.1.9.~~- ... :.: .. ~.. ~~t.Q! .... :.: ...~.?~.i;9.Q .... : .. 7.. ~~:+-.Q9.... :..... 9. ~....... :.... J..!~~:t".Q9...... :....~.~.~tQ9 .. :.... :-.~.~- .... .

.. .~1 :-.1.9.~9.... :.: .. ~-.~~:-R1 .... :.: ...~.~~."":9.1 ..... : .. ~.. ;2;~:-Ql .... : ..... 9. 9....... : .... U~~:t".Q9...... : .... 1.7.~tQO.. :.....?. 9...... .

61-1092 : : 2.DE-02 : : 2.2E-02 9.1 E-01 0.0 1 .8E+OO 4.0E-02 : 2.0

see attached explanation

- - ------ - - *- - - - - -* dified So.aling Factor

................. : .: ............... : . :.*... C.s.--: 1R7 ... :: .' .............. :............... :l~Y.e:r:~9.E: .~91'.li".'19.: ..C;.Jp,1~1.~~~~-.: .I.S.C! .\'.~... <;;.JP.*.

$;..rriP.1.e: .~':1!1l~~r::.: !~9~PP.~ .<;P.l'!q::.: ~.E:Y. !~9. _<;p,riq: :I.S:Q f.~,Y. -~~~i9: .1Q9. !~9/t::~.Y.: ..... f ~~.t.C!t:" ...... : .. !~9 ... CPM: .. : ... f ~~.t.C!t:" ... .

. . .. !.Q9.~!. ..... :~:. -~--R~:-R~.... : ~: .. .1. :9~:t9.Q .... : .. ~.-.1.~:-Q9 .... : .... :-.4:<J...... :.... 9.-!=:~:-Q?...... : ... -~--l~:-Q?.. :.....~ . ~- ..... .

.. .. !.Q9.~~- ..... :~: .. ~--~~:-R~ .... : ~: .. .1.: 1~:t:9.Q .... : .. ?A~:-Q~ .... :.... :-.4: 1...... :.... 9.-!=:~:-Q?...... :.... ~.. Q~:-Q?.. :.....4. 7...... .

.. .. !.Q9.~~- ..... :~: .. '?.-!=:~:-R~.... : ~: .. .1.*e~:t:9.Q .... :.. !;>** ;:~:-Q9.... :.... :-.4:~...... :.... 9.-!=:~:-Q?...... :.... '?):~~:-Q?.. : ..... '? . ~...... .

. . .. LQ~.~~- ..... :~: .. !.-~~:-Rf ... :~: ...4:~~.--:Qg .... :. -~--~~:-Q~ .... : .... :-.4,4 ...... : ... -~--!=:~7Q?...... : .... L-~~:-Q9.. : ..... ~ . !. .... ..

.. .. !.Q~.~9...... :~: .. '?.-~~:-R4 .... : ~: ...::?,?~:-:0.1..... :. -~--?!~:-Q~.... :.... :-.4:9...... :... -~--~~:-Q?...... :.... ?A~~:-R~.. : .... 1.::?:l .... .

..,.. LQ9.~'?...... :~: .. L-.1.~:-R~.... : ~: .. .1. :4~.--:0.1..... : .. 7.-~~:-Q~.... : .... :-.4:1 ...... :.: .. ~A~:-Q?...... :.... !;>*. Q~:-Q9 .. :..... 4. '?..... ..

.. . ~ 1:-.1. 9.~'?.... :.: .. ~--R~T.Q !. ... : . : ...~ :?r-t:9.Q .... : .. 7.-~~T.Q9.... : ..... 9.. '?....... :.... ~.-!=:~:-Q?...... :.... 1.-~~:-Q1..: ...: 1~'?.*!=: ... .

.. .~1 :-.1.9.~9.... : . : .. ~.-!=:~:-Rl. ... :.: ...~,9~.--:0.1..... : .. '?.)~~:-Ql .... :..... 9. 9....... : .... 9.-!=:~:-Q?...... :.... 9.*R~:-Q?.. : ....--:?~-.'? .... .

61-1092 : :

2.0E-02 : : 2.2E-02 : 9.1E-01 : 0.0 : 3.6E-02 : 7.9E-04 : -25.3

Jc-99 in P,:iau:y Filter The unmodified S.F. was 3.6E-02; however. this resulted in a nonconservative calculated* isotopic concentration for samples 61-1089. 61-1090, and 61-1092; none of which contained <LLD values. Therefore, the S.F. was recalculated using only the positive values of samples 61-1089. 61-1090. and 61-1092, resulting with a conservative factor of 1.8£ ... 00.

- - --*-' - - - - - - - - - -*- - 1-1 29 in ry Filter

................. : . : ............... : . : .... C~:-:1 ;!:7.... :............... : .......... .' .... : /w_e,r,{lge, .~9~.lji:ag: ..C~.lP.41.~~i!t~ .. : .1~.C! .'<~ ... C~.lP.*.

$?f'f!P. ~ N1:1ro~.e.r.: . : !~9~P.P.i!t .CP.I'!<?: : . :Ke.Y. !~,;,... CPn<?, :I.~<? /.IStY. g{l~19: .1<?9. !~9 /~!?.Y . : ..... f {IP.t.Qr. ...... : .. !~9,.. CP.1'!<?.: .. : ... f {IP.t.Qr, ... .

.. .. !.Q9~J. ..... :~: .. i ..~~:-R:? .... : ~: ...1.*~~-~op .... :.. u~~:-R?.... : .... :-.1. ,7...... : .... tR~:-R9...... : .... J..;!:~:-Q~.. : ....":P:-.~ .... .

.... !.Q~~~. :.... : . : .. L-~~:-Rl ... : ~: .. .1., 1~:t:9.Q .... :. J ..~~:-Q?.... :*.... :-.U~ ...... : ... J ..Q~:-Q~...... : .... J.-.1.~:-Q~.. : ....":1 ~..1.... ..

.. .. l'.Q9.~9...... :.: .. i .. ~~:-R~.... : ~: .. .1. ,~~-~9.Q .... :.. , .. ~~:-Q9 .... : .... :-.4,~...... : .... LQ~:-Q~ ...... : .... L~~:-Q~ .. :.... ~.1.:? .... ..

. . .. !.Q9~~...... :~: .. U5!~:-R4.... : ~: ...4,~~.":9~ .... : .. ~.. ~~:-!=!~.... :.... :-.4,'t...... : .... J..Q~:-Q~...... : .... ~.. ~~:-!=!::>.. :.... :-.4:~..... .

.. .. !.Q9~?...... :~: .. L.~~:-R't.... : ~: ...::?:?~.-:9.1 ..... : .. ~.. ~~:-Q't.... : .... :-.~,?...... : .... J..Q~:-Q~...... :: ... ~.. ~~:-Q't.. : ..... 1..~..... ..

.. .. !.Q~~9...... :~: .. !.-~~:-P4 .... : ~: .. .1. ,'t~:-:9.1..... : .. !.. Q~:-Q~; ... : .... :-~,Q ...... : .... J*. Q~:-Q~...... : .... J.. ~~:-Q, .. :..... 1. 9...... .

61-1089 :<: 7.5E-05 : : 3.2E+OO : 2.3E-05 : -4.6 . : 1.0E-03 *: 3.3E-03 : 43.9

. . . ~1 :-.1.9.~9.... :~: .. ~.-~~:-R!:?.... :.: ...~.~~.-:9.1..... : .. ~.. ~~:-Q9.... :.... :-.4,?.. ; ... : .... J..Q~:-Q~...... : .... ~.. ~~:-Q~.. :..:. !:?,,..... .

61-1092 :<: 2.2E-05 : : 2.2E-02 : 1.0E-03 : -3.0 : 1.0E-03 : 2.3E-05 : 1.0 Due to <LLD values exhibited in samples, no ot.her sat.isfact.ory Sea ling Fact.ors oa_n be determined

- -. - - - - *- - C-14 ;n Pr Filter la°* -

................. : .: ............... : .: .... .G9:-.~9..... : ............... :............... : .~Y.E:r: ~ge: .~9~.lji;ig : ..C~.lP.41.<41~~-. : .1,.C! .\:':f,. ,(;i!l.lP.. .

$~.l"flP.l.E: .~':Jro~.E:r::.: 1~9~PP.~ .CPn<?::. :~.E:Y.1~9... CPn<?: :I.S:Q/.IS~Y. g~~j9: .1Q9. l~9/~!!'.Y.: ..... -~ ~P.t,q,: ...... : .. 1~9... CPJ'!<?, .. : ... f ~P.t,q,: ... .

. . . . J.Q~.~J. ..... : .: . ,f,..Qt-Q1 .... : .: .. ~=~~.-t:9~ .... : ..~1i.rri.ifl.~~~ .. : ..... N..l~: ..... :.... ~..~~:-!=!?...... : .... 1. 7~tR1 .. :.... ~.1:~..... .

.. . . LQ~.~~- ..... : .: .. ~.-~~:-Q 1.... : . : .. ~ :?~.-t:9.4 .... : ..~1trri.in<41~~- . : ..... N...~, ..... : .... ~.-~~ :-R?...... : .... 1. !;>.~ tR 1.. : .... ~.4: 1..... .

.. .. LQ~.~~...... :.: .. ~.. ~~:t".Q9.... :.: .. ~.!;i~.-t:9.~ .... :. J1i.rri.i!'l.~~~~ .. : ..... N..l~: ..... :.... ~.. ~~:-!=!?...... :....7. 9.~tR1 .. :.... :?.1. :1 ..... .

. .. . J.Q~.~,...... :.: .. 9.*~~:-R?.... :.: ...4,°'~.-t:9.1..... : ..~1i.rri.in~1~~ .. : .... .N...~ ...... :... .~.-~~:-!=!?...... : .... '?.,~~:-R1 .. :.... J.Q,Q..... .

e.

.. .. !.Q~.~~- ..... :.: .. 7.. ~~:-R1 .... :.: .. .4,~~:t:9.4 .... : ..~1imifl.~~~~ .. : ..... N...l'.i, ..... : .... ~.-~~:-!=!?...... : .... ~.~tRO.. :.... J.1. .~..... .

.. .. !.Q~.~9...... :.: .. ~t~~:-R? .... : .: .. .1. :1 ~:+:9.4 .... : ..~1i.rri.ifl.~,~~-.: ..... N...~ *..... : .... ~.. ~~:-!=!? ...... : ....~ . J~tRO.. : .... 7.Q,~.... ..

.. . ~1 :-.1.9.~~.... :.: .. ~...1J:t".Q!. ... :.: ...'l,1 ~:+:9.4'. ... : .. !;5*..1.~:-R?.... :.... :-.1.* ~...... : .... ~*. ~~7R?...... : .... 1. ~.~tR1 .. :.... :-.1. ,e.... ..

.. . ~1 :-.\9.~9.... :.: .. ~tQ~:t".09.... :.: ...4,~~.-t:9.4 .... : .. J.J:~:-Q?. .- .. :.... :-.1. :e...... :.... ~. ~~:-!=!?...... :....E? .. !;5.~tRO.. :..... 1. 9...... .

61-1092 : : 1 .4E+OO : : 5.5E+01 : 2.5E-02 : -1 .6 : 2.8E-02 : 1 .6E+OO : 1.1 See attached exp la nation

- - - - - - - ...- -- -*-* - - - C-14 in Prim-:iry Filter dified Sc-:iling Factor

................. : ................ : . : .....G9:-.tf9..... : ............... : ............... : lrY.~".'~9.~ .~'??.ljrig_: .. C?.lP.~1.~~,~-.: .1~.C! ."<f: .C?.lP.*.

~?.l'flP.l.~ N1:1roP.~".':. l:!i9~PP.~ .CP."lt.?,:.: l<.~Y. ,~9: .l:;Pnt.?, :I.~(? /.1<;,Y. g~~j9: .1<?9. !:!19/'>!?.'d.: ..... f ~~.t.C!".' ...... : .. l:!19, ,1:;pnq, .. : ... f ~P.t.C!".' ... .

.. .. LQ?.~!. ..... : ... '?.,RF;:-R1 .... :.: .. ,q,~~.-t:9.4 .... : .. J.. QF;:-R~.... :.... :-.:;;,Q...... :.... ?.-~F;:-R~ ...... : ....?:9.~tRO.. :..... ~ . ?...... .

.... !.Q?.~:?...... : ... 9.-~F;:-R1. ... :.: .. _q,?~.-t:9.4 .... : .. '?.)'.F;:-R'f .... : .... :-.~,?...... : .... ?.*~F;:-R9...... : .... 1:~-~tRO.. : .... .~:9...... .

.... !.Q?.~9...... : ... ?.*~~:+-P9.... :.: ...4,9~.-t:9.~ .... :.. J.. ~F;:-R~ .... :.... :-.4,~...... : .... ?.-~F;:-R9...... : ....$:~.~tRO.. :.... .?:'?...... .

.... !.Q?.~~- ..... : ... '?.-~F;:-R? .... :.: ...4,'t~.-t:9.1..... : .. :?A~F;:-Q9.... :.... :-.4,9...... :.... ?.*~F;:-R9 ...... :.... ?.. ~F;:-R?.. :..... 1..;2...... .

.. .. J.Q?.~?...... :. . .7.-?:F;:-R1 .... :.:: ..4:'=~tt:9.4 .... : .. 7.-~F;:-R9 .... : .... :-,4 ,9 ...... : .... ?.-~F;:-R9 ...... : .... ?.. ~F;:-R1 .. : ..... 1. f ..... .

.. .. !.Q?.~'?...... :. . .~--~F;:-R? .... :.: .. .1., 1~.-t:9.4 .... : .. ~.. QF;:-R'f .... : .... :-.:;; ,'f ...... :.... ?.*~F;:-R9 ...... :.... ?.,!F;:-R1 .. :.....~ . ~...... .

. .. !=:1 :-.1.9.E;I?.... : ... :?...t.F;:+-.cn. ... :.: ...4:1 ~.-t:9.4 .... :. ,;i,.,1,F;:-R?.... :.... :-.1. :9...... :.... ?.-~F;:-R9...... :.... 1A~tRQ .. :...."":rn..t.... ..

.. . !=:1 :-.1.9.~9.... : ... ~.. RF;:+-.Q9.... : . : ...4,9~.-t:9.4 .... : .. J../F;:-R?.... :.... :-.1. ,$...... : .... ?.*~F;:-R9 ...... : .... 7A::!F;:-R1 .. :.... :-.e';,,1 .... ..

61-1092 : 1.4E+OO : : 5.5E+01 : 2.SE-02 : -1.6 : 3.4E-03 : 1.9E-01 : -7.5

- - *- - .. - - -* .. --*-- -* --*- *- ~

c-11 in Priaaa Filter The unmodified S.F. was 3.4E-03; however, this resulted in a nonconservative calculated isotopic concentration for samples 61-1089, 61-1090, and 61-1092, of which 61-1089 was the only nonconservative out of spec. result. Therefore. the S.F. was .recalculated usins the values of samples 61-1089, 61-1090, and 61-1092,

.resulti.ns with a conservative factor of 2.SE-02.

~-- - - - - - .. -- Fe-55 i n * * ~ Filter all' -

............ :.... : . : ............... : . : .....G9:-.~9..... :............... :............... : l'f'!.e.r.fl9.e. .~9fll.lil;l9.: ..Cfl.1P.4V~~~~-.: .l~.Q Xf, .Cfl.lP.*.

~flfflP. l.e. n':lro~.e.r.: . : !~9~PP.~ .CP.r'!Q: : * : l<,e,y. ,~9:.Ci:>f!Q: :l.~<?/.l<;tY. .~fl~i9: .lQ9. !~9/'>"'.Y . :..... f flP.t,qr, ...... : .. !~9,.Ci:>.l"!Q: .. : *.. -~ flP.t.Qr, .*..

10391 : : 1 .5E+01 : : 5.9E+02 : 2.6E-02 : -1 .6 : 3.1 E-01 : 1.8E+02 : 11 .9

.. .. J.Q9.~~- ..... :.: .. !;i.. ~~:t'.Q~.... :.: .. .~:?~:t:9.4 .... :.. L..1.~:t'.Q9.... :..... 9. 9....... :.... 9.-.1.~:-Rl ...... : .... 1,9.~tR? .. : .... :-.~:'t ..... .

.. .. !.Q9.~~- ..... :.: .. !.-~~:t'.Q~.... :.: .. .4 ,9~:t:9.~ .... :.. 7.-~~:-!=!1 .... :.... :-.Q, 1...... :.... ?...t.~:-!=!1 ...... : ....7,9.~tR?.. :.... :-.4:'t .... ..

10394

2.2E+Ot : : 2.4E+01 : 9.0E-01 : 0.0 .............................

- - - - : 3.1 E-01 : ******

7.4E+OO********: .............

-2.9 .

.. .. J.Q?>.~?...... :.: .. i .. i:;:+-.Q, .... :.: .. .4 =~~:t:9.4 .... : .. ?.. .1.;:-R?.... : .... :-.t. ,Q...... : .... ?>.. .1.;:-R1. ..... : ....e,?.~tR1 .. : ..... ~ .. "- .... ..

.. . . J.Q?>.~9...... :.: .. 7.-~~:i-.Qi.... :.: ...1.: 1~.-t:9.4 .... : .. ~.-.1J:t'.Q9.... :..... 9. ?>....... :.... 9...t.~:-Pl ...... : .... ~,?>.~tP1 .. :.... :-.~:7..... .

.. .-~ 1:-.1. 9.~?.... :.: .. J.-~~:'".Q7.... :.: ...4, 1~.-t:9.4 .... :.. ?>.. ;;;;~:-Pl .... :.... :-.Q :?...... : .... ?>.-.1.~:-Pl ...... :.... 1. ?.~tQ?.. :.... :-.1.:Q.... ..

.. . ~1 :-.1.9.~9. ... :.: .. ~--~~:'".QJ. ... :.: .. .4 ,~~.-t:9.4 .... :.. ~..:;:~:-Rl .... :.... :-.Q:?...... :.... ?...t.~:-P1 ...... :.....7. J.~tPl .. :..... 1. J. .... ..

61-1092 : : 4.5E+OO : : 5.5E+01 : 8.2E-02 : -1.1 : 3.1 E-01 : 1.7E+01 : 3.7 No out of spec. nono.onserv atin correlations: are observed

................. : .: ;.............. : . : .....G9:-.~9..... : ............... :............. :.: l~Y.~l'.'~9.~ .~9i:1.lj('l9.: ..Ci:i.lP.41.<4~'~-.: .l~,q .'<~... r;.aJP.*.

$.&.rflP.l.~ N':lro~.~I'.':.: !~9~PP.~ .CP.riq::. :K~Y. !~9... Cpnq, :l.~<?l.!c;fY. R~~j9: .1<?9. !~9/'>~.Y.: ..... f ~p~_q( ...... : .. !~9,.CPM, .. : ... f ~P.t,ql'.' ... .

.. . . !.Q~.~, ...... :.: .. ~--~F;t.Q! .... :.: ...~.~~.-t:9.:? .... : .. ~--~F;:-Q?.... : .... :-.1.: 1...... : .... J.. ~F;:-Ql ...... : .... 1,, .~tQ?.. :.....?. 7...... .

.. .. !.Q~.~:;2...... :.: .. :;2..J.F;t.Q:;2.... :.: ...~:?~.-t:9.:? .... : .. ~.-.1.F;:-R1 .... : .... :-.Q,4...... : .... J..~F;:-Q1 ...... : ....~,9.~tQ1 .. : .... :-~,?.... ..

.. .. ! .Q~.~~- ..... :.: .. ,.-i'.f;t.Q:;2.... :.: .. .4:9~.-t:9.~ .... : .. J/~; :-Ql .... : .... :-.Q :7. ..... :... J .. ~F; :-Ql ...... : ....4. '?.~ tQ? .. : .... :-.1. :0.... ..

.. .. !.Q~.~~- ..... :.: .. ~.-l;t.QP.... :.: ...:?,4~.-t:9.1..... : .. :;2.JF;:-R1 .... : .... :-Pk ..... : .... J..~F;:-Q1 ...... : ....4:~-~tQO .. : .... :-.1. ,~..... .

.. .. !.Q?>.~!;5...... : . : .. ~.. ;:l~-r.Q!. ... :.: ...:?.~~.-t:9.:? .... :. -~--R~:-R'.? .... : .... :-.1. ,1 ...... : .... U=!~:-Q1 ...... : ....9,f~tQ1 .. :..... '.? .. !. .... ..

.. .. !.Q~.~9...... : . : ,,:;2,.gF;t.Q!. ... :.: .. .1. :1 ~.-t:9.:? .... :. ,:;2,.QF;:-Q1 .... :.... :-.Q,7...... : .... J..~F;:-Q1 ...... : ....?:9~tQ1 .. : .... :-.1. ,1 .... ..

. . . ~ 1:*-.1.9.~~- ... :.: .. !.-~F;t.Q:;2.... :.: ...'t: 1~.-t:9.:? .... : .. ~--~F;:-Q1 .... : .... :-.Q,!;i...... : .... J.. ~F;:-Q1 ...... : ....7. ~.~tQ1 .. :.... :-.1.* ~ ..... .

.. . ~, :-.1.9.~9.... :.: .. , .. ~F;t.Q!. ... :.: ...4:~~.-t:9.:? .... :. ,:;2,.QF;:-Q1 .... : .... :-.Q,7...... : .... J..~f;:-Q1 ...... : ....4/;2.~tQ1 .. : .... :-.1. ,1 .... ..

61-1092 : : 7.5E+OO : : 5.5E+01 : 1.4E-01 : -0.9 : 1.SE-01 : 1.0E+01 : 1.4 J

- - - - - - - - - - - - - -. - Pu-241 ;n Pr;mary Filt Isotope : Ce-144)

................. : . : ............... : . : : ... Cf!'.-: M'J.. .. . .............. :.............. ;:.'~Y.e:r: J9.e: .~9!1.lj~9. : ..C!i.lP.41.~~~~.. : .lii:.C! x,,.. C~JP.*.

$~fflP. l.e: .~':IITl~.e:r:: . : !~9~PP.~ .CP.F'!Q: : . :~.e:Y. !~9,. CP.l'!Q: 1.S;'? /.~,Y. .~~~j9: .1"?9. !~9/~fl'.Y . : ..... f ~P.t.C?r: ...... : .. !~9... CPf!Q: .. : .... ~ ~P.t.C?r: ... .

.. .. !.Q~.~!. ..... : .: .. J..~~:-R1 .... : ~: ...~:e~:t:9.Q ...... ~t~~:-R? .... : .... :-.1. :'9: ...... : .... ~.. ~~:-R1 ...... :.... 1. ~.~tRO.. :.....e. 9....... *

.... J.Q?.~~...... :.: .. !;i..~~ffi9.... :.: ...:?,O~.-t:9.1....... 7.}~:-Q1 .... : .... :-.Q,9...... :.... ?.. ~~:-~H ...... : ....9,'?.~~QO.. : ..... 1..~...... .

10393 * : : 2.0E+oO : <: 4.3E+OO 4.6E-01 .: -0.3 : 3.4E-01 : 1.4E+OO : -1 .4

- .. i*03.94* *. ***:: *: **a*.4E:oi

- - - - ***: *: **'i:a{.:02 **** ,*1*.2E+.cio' ***: *****c/ i***.. **: ****i4E:oi ******: ****iie::oi *:****:.*ii* ....

.... LQ?.~!;i...... :.: .. J..H:-R 1. ... :.: ...~ .~~.-:0.1..... . .?.*~~:-~H .... : .... :-P :~...... : .... ?.*~~:-Q1 ...... : ... .1 ...1.~:-Q1 .. : .... :-.1. :0......

10396 : : 2.4E-01 : : 1 .5E+OO . 1 .6E-01

..................................................................................... : -0.8 **********************

3.4E-01 : ........ **********

5.1 E-01 : ************

2.2 *

... ~ 1:-.1. 9.E;l?.... :.: .. ~..?i~t.Q9.... :.: ...'f =~~.-t:9.Q.... . .'?.,i'.~:-Q1 .... : .... :-P:?...... : .... ?.*~~:-Q1 ...... : .... 1,'?.~tQO.. : .... :-.:? :9..... .

.. . ~ 1:-.Hl.~9.... :.: .. ?.. ~~:-R1 .... :.: .. .1.*7~.-t:9.Q.... .. ~..!=~~:-Q1 .... : .... :-.Q :?...... :.... ?.*~~:-Q1 ...... : .... ~.-l~:-Q1 .. : .... :-.1. :7.... ..

61-1092 : : 2.1E-01 5.2E-01 4.0E-01 -0.4 . 3.4E-01 1-.7E-01 : -1.2

- - *- .. 1- .. - - -*- - Pu-241 in Primary. Filte Isotope : Co-60)

................. : . : ....... : ....... : . : .....G9:-.~9..... : ............... :............... : .l,Y.~~J9.~ .$9~Jj,:i9.: ..C~:lP.41.-!1~~.. : .l~.Q .'{f,.C~JP.*.

$~.l'TlP.1.~ .~\Jf'l'.l~.~~:.: !~9~PP.~ .CP.1'!<?::. :l.<.~Y. !~9,.CP.1'!<?: :1.S:QmfY. .l~~~j9; .1Q9. !~9/~!?.Y.: ..... f JP.t.Qr:- *..... : .. !~9,.CP.1"!<?: .. : ... f JP.t,qr:- *...

.. .. J.Q~~J. ..... :.: .. !,.~;:-Q1 .... :.: ...~:'~~:t:9.4 .... : .. 7.,l;:-Q~.... : .... :-.~:~...... : .... 7.,.1.;:-Q~ ...... : .... 1,7.~TQO .. : ..... ?. ~..... ..

.. .. LQ?.~f...... :.: .. !;>** ~;:+-.Q9.... :.: .. ~/?~:t:9.4 .... :.. J..Q~:-P.?.... : .... :-.4:0...... : .... 7...1.~:-Q~...... : .... 1:J.~TQO.. : .... :-:4:~ .... ..

. . . . J.Q~.~~...... :.: .. f .. Q~:+-.Q9.... :.: ...4:9~:t:9.~ .... : .. ?.. Q~:-Q~ .... : .... :-.~: 1...... : .... 7.-.1.~:-Q~ ...... : ....~,~~TP.0 .. : .....?,9...... .

.. .. LQ?.~~...... :.: .. ~.. ~;:-Q? .... :.: ...4:~~:t:9.1. .... : .. ?.-~~:-Q~.... : .... :-.4:9...... : ... ,:;2,.J.~:-Q~...... : ... ,!;:i,.~;:-Q?.. : .... :-.1. :~.... ..

.. . . LQ~~?...... :.: .. J...1.~:-P.1. ... :.: ...~:~~:t:9.4 .... : .. ~.. '.::!~:-Q~.... : .... :-.~:~...... : .... ?...1.~:-Q~...... : .... ~.. ~~:-P.1 .. : ..... !;I .., ..... ..

.. . . LQ?.~9...... :.: .. i .. ~;:-P.1. ... :.: .. .1.: 1~:t:9.4 .... : .. i ..~;:-Q~ .... :.... :-~:? ...... : .... i .. .t.~:-Q~..... :: .... :;?..;!i~:-P.1 .. : .... :-.1. :0.... ..

61-1089 : : 3.3E+OO . : : 4.1E+02 : 8.0E-03 : -2.1 : 2.1E-03 : 8.7E-01 :. -3.8

)1 ~:1:ti:~o: :: :1 :1 ::~)~~Rt::::! :1: :i~~:~pf::: 1: :~)~~Q~:: :: 1: :: >f{: :: :: 1: :: iJt~R~:: :: :: 1:: ::~)~~!-ii ::1: :: :~io:: ::::

61-1092 : : 2.1E-01 : : 5.5E+01 : 3.8E-03 : -2.4 : 2.1E-03 : 1.2E-01 : -1.8

- - - - *- - - - - -*- - - - -. - Cm-242 in Primary Filte Isotope : Ce-144)

................. : . : ............... : . : ....C~.-:1 ~':l.... : ............... :................~Y.E!l'.'~9.E! .~9i1.ljr;i9.: ..Ci1.1P.i~1.~~~~-.: .I~.'=! ."<~... Ci1.1P.*.

$!1ffl.P.l.E! N':lro~~t;:.: !,9~!>.P.~ .C!>.'l<?::. :~.E!Y. !,9,. .C!'.'l<?, :l.~q/.lStY. .l~~~j9: .1Q9. !,9/~,.Y ...... J ~P.t.QI'.' ...... : .. !~9, .C!'M: .. :... f ~~JQI'.' ... .

.. .. ! Q~~ !...... : .: .. ~--R~:-Q9 .... : ~: .. ~:1;1~:t:99 .... : .. J...1.~ :-Q9 .. ,. : .... :-.~ :0. . . . .. . ... i .. i=!~ :-Rl ..... : .... ?.-i=!~ :-R9.. :..... ?. 1...... .

. . . . LQ~.~i...... : . : .. '?.*R~:-R?.... : .: ...:?,O~:t:9.1..... :. -~--~~:-Q9.... : .... :-.:?.~ .......... i .. ~~:-R9...... : .... ~.-~~:-Q?.. :.... :-.1. ,9.... ..

. . . . J.Q~.~~- ..... :.: .. ~.. ;i;~:-R9.... : ~: ...4:9~:t:9.Q .... : .. J.. g~:-Q9.... : .... :-.:?,';l .......... i .. ~~:-i::'.!9...... : .... J...1.~:-Q?.. :..... ?. L ..... .

. . . . LQ~.~~- ..... : . : .. ~--~~:-R't .... : .: .. ~ .er*:O;i; .... : .. !?.-~~:-Q9.... :.... :-.:? :9. . . . .. . ... i .. ~~:-i::'.!9...... : .... J*. l~ :-Rf. :.... :-.:? ,1..... .

.. .. LQ~.~~- ..... : . : .. ~-.~~:-R9.... :.: .. ~:9~.-:0.1..... : .. J.. ~~:-Q?.... : .... :-.1. ,e......... -~--~~:-Q9...... : ... J3.. ~~:-Q~.. :.... :-.!!?,e.... ..

. . . . 1.Q~.~~...... : . : .. !.-~~:-Rl ... :.: .. .1. ,9~.-t:9.Q .... : .. J...1.~:-Q9 .... : .... :-°R:9 .......... i ..~~:-R9 ...... : ... -~--~~:-i::'.!9 .. :.....?. ~..... ..

.. . ~ 1:-.1.9.~?.... :.: .. !.. g~:-R?.... :.: ...4,';l~.-t:9.Q .... :.. i .. ~~:-Q9.... :.... :-.:?.~.......... i .. ~~:-R9...... : .... J.. ~~:-Q?.. :..... 1. 9...... .

. .. ~1 :*J.9.~9.... : .: .. 7...1.~:-!=!9.... :.: .. .1. ,7~:t:9.Q .... : .. ~.. ~~:-Q9.... :.... :-.4,':l.......... i .. ~~:-R9...... : ... -~--~~:-Rl. :.... :-.1. ,7..... .

61-1 092 : : 5 .6E-04 : : 5 .2E-O 1 : 1.1 E-03 : -3 .0 2 .SE-03 : 1.3E-03 : 2 .3

- -. - - - - - - - - - - - - -*- - Cm-242 ;n Pr;mary Fm y Isotope : Co-60)

................. : .: ............... : .: .....G'?:-.~9..... : ............... :............... : l~Y.~1'.' fl9.~ .~'?~.lil'.19. : ..C~.lP.41.~~~~ .. : .l!>.Q :~~ ... C~.lP.*.

$~fflP.l.~ N':lro~.~I'.':.: !~9~!>.P.~ .(;!>.IW,:.: K~Y. !~9 ... (;9.rW, :I.S;q /.IS~Y. gfl~i9: .1<?9. !~9/~!!'.Y.: ..... f flP.t.QI'.' ...... : .. !~9, ,,;9nq, .. : ... f flP~.QI'.' ... .

.. .. !.Q?.~L ..... :.: .. , .. R~-:'Rl ... :.: ...~,'.7~.-t:9.4 .... :.. ~.. ~~:-Q9 .... :.... :-.~,?...... :.... J..R;:-P?...... : ... .'~.. ~;:-Q9 .. :..... ?. ~..... ..

.. . . !.Q?.~?:...... :.: .. ~A=i;:-R?.... :.: ...~ ,?~.-t:9.4 .... :.. J.-~~:-Q4.... :.... :-.~ ,'.? ...... :.... J.,R;:-Q?...... : .... l?.. ~;:-Q9 .. : .... :-:? .~..... .

.. .. !.Q?.~9...... : .: .. ~.. ~~:-R~ .... : .: ...4,?~.-t:9.~ .... : .. ~...1.;:-Q~.... : .... :-.~.?...... : .... J.. !S:;:-Q;i...... :.... ~.. ~;:-Q? .. :.....7. ~..... ..

. . . . J.Q?.~,...... :.: .. ~--~;:-R4 .... :.: ...4,4~.-t:9.1..... :.. J.. ~;:-Q? .... :.... :-.4,$...... :.... J.. ~;:-Q?...... : .... ~-*~;:-Q4 .. : ..... 1. J...... .

10395...... ..: ....

.......... : 4.9E-03 : : 2'.9E+02

.. ****************** : 1 .7E-05

.................. . : -4.8 : 1 .6E-05 : 4.6E-03 :

- (** ............................ ****** ............. ********* ................. .

-1 .1 .

. . . . !.Q~.~'?...... : .: .. J.. ~~:-R~ .... : .: ...1. ,1 ~.-t:9.4 .... : .. J..~;:-Q? .... :.... :-.4,$...... :.... J.. R;:-Q~...... : .... J.. l;:-Q9.. :..... 1. J...... .

.. .R1 :-.1.9.~~- ... : .: .. J.. g~:-R?.... : .: ...4,1 ~.-t:9.4 .... : .. ~.. ~;:-Q?.... : .... :-.4,9...... : .... J..R;:-Q? ...... :.... '?.. ~;:-Q~ .. :.... :-.1.* ~ .... ..

.. . R1 :-.1.9.~9.... : .: .. ?.. H:-Rl ... : . : ...4,9~.-t:9.4 .... : .. ?..,1,;:-P9.... : .... :-.4,?...... :.... J.. R;:-Q?...... :." .}.!S:;:-Q~ .. :.... :-.:?:O .... ..

61-1092 : : 5.6E-04 : : 5.5E+01 : 1.0E-05 : -5.0 : 1.6E-05 : 8.7E-04 : 1.5

- - -*- - - - - - - - - - - --- Pu-238 in Primary Filte Isotope : Ce-144)

................. : . : ............... : .: .... (;:~."'.1 ~'t.... : ............... :............. : . :,1~Y.E:1'.'{19.E: .~9~.lj('lg : ..r;:~JP.41.(j~~~ .. : .l~.Q .':'1:. (;:~.lP.*.

$~.rfl.P.l.e: .~':IITl~.e:r::.: !~9~PP.~ ,r;:pnq::.: ~.E:Y. !~9:.(;:Pf!<?: :l.~qm,Y. .~{1~19: .1qg, !~9/~!?.':J.: ..... f flP.t,qr:- ...... : .. !~9: .(;:S>n<?: .. : ... f fp~~I'.' .. ..

.. .. J.Q~.~J. ..... :.: .. J..H:-R~.... : ~: .. ,q:e~:t:9.Q .... : .. i .. ~;:-Q'f .... :.... :-.~:9...... :.... i.-R;:-Q9...... : ... J .. Q;:-R? .. :... ..~:L .... ..

10392

..... *:: *:: .. 5.9E-02

- 1*039! 7.4E:oi .. : : 2.0E+01

(: .. *4:iE*+oo .... : 3.0E-03

**,*.1E:oi *.. :

*.. *-2.5

2:a ...... :

.. 2.6E-03

2.sE:oi * *** :

****5.2E-02 :

1*E

02

...... **** **** .......................................................... ************** ......................... .. : .....-1.2

1. s..... ...

.. . . J.Q~.~~- ..... :.: .. 9.-~~:-R~ .... :.: .. R:~~."'.0~ .... :.. ?..~;:-R9.... : .... :-.~:O...... :.... ~..R;:-Q9...... : .... U~;:-R't.. :.... :-.q:~.... ..

10395 : : 1 .SE-03 : : 3.3E-01 : 4.5E-03 : -2.3 : 2.6E-03 : 8.SE-04 : -1 .7

...::~1;:gi~~:: :-: :1: 1: }:~~~R~: :: :1 :1: ;~~:~9:q:::: 1:: ;:.~~7~i::: 1: : :~f~:::: : i::: }.~~7Ri::::: 1: :: :~:.R~~Ri: 1: : ::1 i:: : :

1:

-.1.9.F.;l?.... :.: .. J.-~~:-R?.... : .: ...4:~~:t:9.Q .... :.. i .. ~;:-R9 .... :.... :-.~:9...... :.... ~.*R~:-Q9 ...... : .... L,?i~:-Q?.. :.... :-.1. :1 ..... .

.. . ~ 1:-.1. 9.~9.... :.: .. ?.-~~:-R~ .... :.: .. .1. :7~:t:9.Q .... : .. ~.. ~~:-R9.... : .... :-.:?:9...... :.... ~.-R~:-Q9, ..*... : .... ~--~~:-99.. :.... :-.:?: 1..... .

61-1092 : : 2.2E-03 : : 5.2E-01 : 4.2E-03 : -2.4 : 2.6E-03 : 1 .4E-03 : -1 .6

- ------ --------- Pu-238 ;n Primary Fflt y Isotope : Co-60)

................. : . : ............... : .: .....G9:-.~9..... : ............... :............... : lw.e.r. ~9.e. .~9~.ljrr9. :*..C~.lP.1.!1.~~I?~.. : .l~.C! -~~: .C~JP.*.

$~.l'fl.P. l.e. N1,1roP.e.r.:.: !~9~PP.I? .CP.l'!Q::.: ~.e.Y. !~'?: .CPnq, :l.~Q I.IS~Y. g~~j'?: .1Q9. !~9/'>!?.Y.: ..... .F: ~P.1.C!r. ...... : .. !~'?, .Cimq: .. : ... f ~P~.C!r. ... .

.. . . J.Q?.~l. ..... :.: .. !...1.~:-R~.... :.: .. -~=~~.-t:9.4 .... : .. J..'.~~:P9.... :.... :-.~:?...... :.... J..f'.;:-Q9...... :.... ~.-!:!;:-Q9 .. :.....!;!,'?..... ..

.. .. !.Q?.~7...... :.: .. !?.-~~:-R:?.... : .: .. -~=?~.-t:9.:? .... : .. J...1.;:-Q~.... : .... :-.~:~...... : .... J..f'.;:-Q9 ...... : .... ~.. ~;:-Q9 .. : .... -:-~:~ ... . ..

... . J.Q9.~~...... :.: .. ?.. ~~:-Rl ... : .: ...4:~~.-t:9.~ .... :.. 9.. Q~:-Q9.... :.... :-.~:9...... :.... J.. f'.~:-Q9 ...... : .... ~...lJ:-Q?.. :.....!? . '?...... .

.. .. J.Q?.~~- ..... :.: .. '?.-~;:-R4 .... :.: ...4,4~.-t:9.1..... :.. ~.. ~~:-Q~.... :.... :-.4k ..... : .... J..7~:-Q9 ...... : .... ~..Q~:-Q4 .. :.... :-.1. ,~..... .

.. .. J.Q?.~!?...... :.: .. L-~;:-Rl ... :.: ...4,~~.-t:9.4 .... :.. ~.. ~;:-Q~.... : .... :-.~,~...... : .... J.. !'.~:-Q?...... : .... ~.. !:!;:-Q9.. :..... ~ . ~..... ..

.. . . J.Q~.~~- ..... :.: .. 7.. g~:-Rl ... :.: .. .1., 1~.-t:9.4 .... :.. ~.. Q~:-Q~ .... :.... :-.4 :7...... :.... J.. 7~:-Q9...... : .... J..!:!~:-99.. : .... :-.1. ,?.... ..

.. . ~1 :-.1.9.E;I'?.... :.: .. !.. ~~:-R~.... :.: ...4,1 ~.-t:9.4 .... :.. ~.. ~~:-Q9.... :.... :-.4,9...... : .... J.. 7~:-Q9...... :.... i;... !:!~:-Q9 .. :.... :-.4,1. ... ..

.. . ~1 :-.1.9.~9.... :.: .. ?.. ;;::~:-R~.... : .: ...4,~r-t:9.4 .... :.. ~.. Q~:-Q~.... :.... :-.4,4...... : .... J.. 7:~:-Q!:? ...... : .... ?.-!:!~:-Q9 .. :.... -:-~,4 .... ..

61-1092 : : 2.2E-03 : : 5.5E+01 : 4.0E-05 : -4.4 : 1 .7E-05 : 9.1 E-04 : -2.4

- - - - - - - - - - - - *- -*- - Am-241 in Primary Fi ey Isotope : Ce-144)

... : ............. : . : ............... : . : .... C~.-: 1~~ .... : ............... : ............... : .~Y.~t:' f9.~ .~9,1,lji;i9.: ..9!1.lP.41.~~~~.. : .1!>.Q -~~: .Ci1.1P.*.

~il.l'flP.l.~ .~':lro~.~r:-:.: l~9~PP., .CP.rl<?::. :~.~y .1~9 ...C?n<?: :l.~q/K,Y. Rf~19: .11?9. !!f9/.~!!'.Y.: ..... f fp,t,qr:- ...... : .. !!f9... C?.rl<?: .. : ... f fP.t,qr:- ... .

. ... !.Q?.~J ...... : .: .. 7.-~~:-Ri. ... : ~: .. .~.e~:~9.Q .... : .. i ...1.~:-Q'f.... : .... -:-.~:?...... : .... J...1.~:-Q~...... : .... ~J..~~:-Q~ .. : .....~ ..~- .... ..

. . . . J.Q~.~~- ..... :.: .. '?.-!~:-R~ .... :.: ....~:O~:t9.1..... :.. ~.. ~~:-R~ .... :.... :-.~:~...... : .... J...1J:-Q~...... : .... ~.-~~:-Q?.. : .... :-~.9..... .

.. .. J.Q9.~~...... :.: .. ~--R~:-R~.... : ~: .. .ii~~:~9.Q .... : .. ~--~~:-Rf ... : .... :-.~,Q.: .... : .... J...1.~:-Q~...... : .... ~.. ~~:-R~ .. : ..... 1:i...... .

.. .. !.Q~.~~...... :.: .. ~.-?i~:-R~.... :.: ...~:e~.-:9~ .... :.. ~--~~:-Q~.... : .... :-~:l ..... : .... J...1J:-Ql ..... : .... 7.. ~~:-Q~.. : .... :-.i,~.... ..

. . . . J.Q~.~~- ..... :.: .. ~.. ?;~:-R~ .... :.: ...~:~~.-:9.1 ..... : .. ~.-~~:-R1 .... :. *... :-~.Q...... : .... J..J.~:-R~ ...... :.... ?.-~~,R~ .. :..... 1,'?....... .

. . . . J.Q~.~'?...... :.: .. ~.-~~:-R4. ... :.: .. .1.*~~:~9.Q .... : .. J.. ~~:-Q'f .... : .... :-~.e...... :.... J...1.~:-Q~...... : .... J.}~:-R~.. : ..... ~ .. ~- .... ..

. . . ~ 1:-.1. 9~~.... :.: .. '?.-~~:-Rl ... :.: ...4 .~~.-+:9.Q .... :.. L-~~:-Ql ... : .... :-.~ .~...... : .. :. J...1J:-Q~...... : .... !;:i**~~:-Q~ .. : .... :-.1. ,'?...... .

. . . ~ 1:-.1.9.~9.... :.: .. '?.-~~:-Rl ... :.: .. .1.*7~.-+:9.Q .... :.. ?.*~~:-R~.... :.... :-.4:'f...... : .... J. ..1J:-Q~...... : .... J..~~:-Q~.. :.... :-.~.~..... .

61 .. 1092 :: 6.2E-04 :: 5.2E-01 : 1.2E-03 : -2.9- : 1.1E-03 : *5.9E-04: -1.0

- -- ------- - --- - - - - - - Am-241 in Primary F1 ey l:s:otope : Co-60)

................. : .: ............... : .: .... .G9:-.~9. .... :....... :....... :............... : lf'f.e.r: J9.~ .~9~.lji:i9. : ..C~.lP.41.ci~,~.. : .I~!~.~~... C~.lP.*.

$~P.1.~ N':Jro~r::.: !,9~PP.~ .CP.r!Q::. :l<.~Y. !,9... C~.l'!Q: :l.~Q/.!S,Y. .~J~j*?:. lQ9. !,9/~,.Y.: ..... f fP.t.QI'.' ...... : .. !~9... CP.l'!Q, .. : ... f f9~.Qr; ... .

.. .. LQ~.~L ..... :.: .. 7.. ~~:-R'4. ... :.: ...~,~~.-t:9.4 .... :. J .. ~~:-QI?.... : .... :-.!:?.~...... :.... 7.,g~:-Rf? ...... :.... o:1-** g~:-R~.. : ..... ~ . ~- .... ..

- 10392

........ : : 6.7E-02

- - - - : : 5.2E+02

.......... ********** : 1.3E-04

- - - - : -3.9 ****** ...................................................

.................. : 7.2E-06 : 3.7E-03 : -17.9 .

.. .. !.Q~.~~...... :.: .. ~.-R~:-R~ .... :.: ...:?:~~.-t:9.~ .... :.. J..~~:-Rf?.... : .... :-.~.i;i...... :.... 7.. g~:-RI?...... :.... J..!:~~:-R~ .. : ..... 4. ~...... .

10394 : : 3.3E-04 : : 2.4E+01 : 1.4E-05 : -4.9 : 7.2E-06 : 1.7E-04 : -1.9

i:Q~~~: :::: :! :! ::~j~~i:!4::: :! :! :: :~;~~:~~:?: :: i: :;:J~~i:!~:: :: i: :: :~:~;~:: :: :: 1: :: :i~~~Q~:: :: ::1: :: :i\~~Q~:: 1: :: ::~) :::: ::

.... !.Q~.~P...... :.: .. f .. ~~:-R4.... :.: .. .1., 1~.-t:9.4 .... :.. ~.. ~~:-QI?.... :.... :-.~:'?...... :.... 7.. ~~:-RI?...... :.... 7..!:~~:-R4.. :..... ~. L ..... .

.. .!=!1 :-.1.9.~~.... :.: .. P.*~~:-R~.... : .: ..."l, 1~:t:9.4 .... : .. L~~:-R~.... :.... :-."l,e...... :.... 7.. g~:-Rf? ...... :.... ~.. ~~:-R~.. :.... :-.:?.~.... ..

61-1090 : : 6.6E-03 : : 2.3E+02 : 2.9E-05 : . -4.5 : 7.2E-06 : 1.7E-03 : -4.0 0

61 :.:1ogi' ... :.: .. 6°.2E:.04' .. ':.: .. *5:5E+01 .... :. *;*:1*E:.05" .. :.... :.:4:9* ..... :.... 7°.2E:.oi ..... :... 4.0E:.04": .... -.:; :i;," ....

0 Sinc:e there i:s: no int1uerioe of <LLD values, there is no obvious route to modify Scaling Faotor

Pu-239 (Pu-240) ;n Pr;m.ar r (Key Isotope : Ce-144)

.................. : . : ............... : . : ....C!:'::1 ~4 .... :............... :.. : ............ : itY~~J9.~ .~9fl.lji;-i9.: ..Cfl.lP.41.~~~~ .. : .1,.Q .~, ... Cii.lP.*.

$fl.rflP.l.~ .~':IITI~.~~:.: !~9~PP.~ .CP.l'lE?,:. :l:<.~Y. !~9 ... CPnE?, :l.~9/.l~tY. .~~~j9: .199. !~9/~~.Y.: ..... f {IP.t.Q~ ...... : .. !~9: .CPf!E?, .. : ... f JP.t.Q~ ... .

.. .. !.Q9~!. ..... : .: .. ~..~~:-R4 .... : ~: .. ~.e~.-t:99 .... : .. L-~~:-Q4 .... :.... :-~:~...... : .... L-~~:-Q9, ..... : .... 7.. ~~:-Q9.. : .... J~:1 .... ..

.. .. !.Q9.~i...... :.: .. f}~:-R?-.... :.: ...~:9~.-t:9.1..... : .. i .. ~~:-!l~.... :.... :-.4,I?...... : .... '-*~~:-Ql ..... :.... 9.. J'.~:-Q~.. :.... :-.1. ,9.... ..

.. .. LQ9.~9...... :.: .. '?.-l~:-R9.... : ~: ...4,;;:~.-t:9.Q .... : .. J.-~~:-Q9.... :.... :-.4:e...... : .... J.. ~~:-!=!9 ...... : .... ?..~~:-!=!9 .. :..... Li..... ..

.. .. LQ~.~~- ..... :.: .. ~.. ~~:-R4.... :.: ...~.e~.-:9~ .... :.. ?.. ~~:-Q9 .... : .... :-.4, 1...... :.... , .. ~~:-R;;:...... :.... , .. ~~:-Q4.. :.... :-.4,!;i..... .

. . . . J.Q9.~!;5...... :.: .. ~.. ~f;:-Q4 .... :.: ...~.~~.-:9.1 ..... :.. ~...1.f;:-9.9.... :.... -:-.'4,7 ...... :.... ,..~f;:-Q~...... : .... ~.. ~~:-Q4 .. :.... :-.1., 1..... .

.. .. !.Q9~'?...... :.: .. J.;~~:-R~.... :.: .. .1. ,9~.-t:9.Q .... : .. J..~~:-Q~ .... : .... :-.4 :~ ...... : .... J.. ~f;:-9.~ ...... : .... :?..~;-:-!=!~ .. : ..... L~..... ..

.. .~1 :-.1.9.~?.... :.: .. , .. .1.~:-Q?-.... :.: ...4:~~.-t:9.Q .... :.. i .. ~~:-Q~.... : .... :-.4:9...... : .... J..~~:'Q~...... : .... ?.. ~~:-Q~.. : .... :-J. ,?-..... .

.. .~1 :-.1.9.~9.... : . : .. ?.. ~~:-R~ .... :.: .. .1. ,?~:t:9.Q .... : .. ~.. ~~:-R9 .... :.... :-.4,9...... :.... J.. ~F;:-R9...... : .... 9.*~~:-R9.. :.... :-.4,4.... ..

61-1092 : : 1 .7E-03 : : !5.2E-01 : 3.3E-03 : -2.!5 : 1.9E-03 : 9.9E-04 * : -1 .7 rnm;natfon of <LLD values would result ;n a less oonseorvat;ve ScaHng Factor and no out of spec. ,nonoonseorvat;ve, correlation values are observed

- - ---*--- --------- Pu-239 (Pu-240) ;n Prima r (Key Isotope : Co-60)

................. : .: ............... : .: .....G9:-.~9..... :........... ;... :........... :... *"'Y.E!l'.'{19.E! .~9~.lji;ig_: ..C~.lP.41.~~~~ .. : .l~.ci .'<1: .i;:i'i.lP.*.

$i'ifflP.l.E! N1,1ro~.E!I'.':.: !~9~P.P.~ .CP.l'!Q::. :~.E!Y. !~9... CPM: :l.~9/.~tY. g{l~i9: .199. !~9/~!!'.Y. . .... f JP.t.QI'.' ...... : .. !~9... CP.l"!Q: .. : ... f {IP.t,qr: .. ..

.. .. !.Q~.~J ...... :.: .. , ..l:!~:-Rf ... :.: ...~:~~:t:9.t ... :.. 7..~;:-Q?.... :.... :-.~: 1.......... J..~;:-R9...... :.... 7...1.;:-Q~.. :.... L~:7.... ..

10392 : : 4.7E-02 : : 5.2E+02

.................................................................. : 9.0E-05 ******** : ...............................

-4.0 1.2E-05 : 6.3E-03 :

- - - - -7.5

.. .. J.Q~.~~...... :.: .. 9,.j'.~:-Rl ... :.: ...4:9~:t:9.~ .... : .. 7..;;:-Q~.... :.... :-.~.r9.......... J.*~~:-R9...... :.... ~.. Q~:-Q?.. :..... f.,...... .

.... J.Q~.~~...... : . : .. ?.,!:!~:-Rf ... :.: ...:?:'f~:t:9.1..... : .. 7..:4;;:-Q9.... :.... :-:4:9.......... J.. ~;:-Q9...... : .... 7.. ~;:-Q'f.. :.... :-.:?:9..... .

.. .. !.Q~.~~...... :.: .. 9.,li!~:-R't. ... :.: ...:?:~~.-+:9.::? .... : .. :;2*. :4;~:-R9.... :.... :-.!:;i:9.......... J..~;:-Q~...... :.... ~.. ~~:-!=!~.. :..... ~ . 9...... .

.. .. !.Q~.~9...... :.: .. J..li!~:-R~.... :.: .. .1.: 1~:t:9.4 .... :.. J..;~:-R9.... :.... :-.'Le.......... J.. ~~:-R~...... : .... J..~~:-R~.. :.... :-.1. :-, ..... .

.. . ~ 1:-.1. 9.~~.... : .: .. J..H:-R~.... : .: ...4: 1~.-+:9.:? .... : .. 7.-7~:-Q!;i .... :.... :-.4 :1$. . . . . . . ... J.. ~~ :-R~...... :.... ~.. ~~ :-R~.. :.... :-.:? :?..... .

.. .!=!1 ~.1.9.~9.... :.: .. 7..li!~:-R~ .... :.: ...:?:~~.-+:9.:? .... : .. ~..:4;~:-R9.... :.... :-:4:!;i.......... J.. ~~:-R~...... : .... 7A:~~:-Q~.. :.... :-.:?:'~..... .

61-1092 : : 1.7E-03 : : 5.5E+01 : 3.1 E-05 : -4.5 1 .2E-05 : 6.6E-04 : -2.6 No out of spec:. nonconserv at;vt c:orre lations are observed

-- ---- - -1*-*- -

Pu-242 (Np-237) ;n Prim.ar r (K,e,y Isotope : Ce-144)

................. : . : ............... : . : .... C~:-: 1~~ .... :............... : ............... : AY.E!~ ~9.E! .~9~.lii;l9. : ..C~.lP.41.~~~~.. : .1~.Q :-<~ ... C:a.lP.*.

$~.rri.P.1.e: .~':lro~.e:(.: !~9~P.P.~ .CP.1'!<?::.: l<.E!Y. !~9 ... CP!l<?: :1.~q/.~,Y. .~~~i9: .1<?9. ,~9/~!:'.Y.: ..... f ~P.t.QI'.' ...... : .. !~9 ... CPn<?: .. : ... f ~P.t.Q~ ... .

10391 :<: 2.4E-b4 : <: 3.8E+OO ................................................................

- - - - : 6.3E-05 : -4.2 : 3.7E-05 : 1.4E-04 : -1 .7 ****

.... !.Q~.~~...... :.: .. ~A=!~:-R~.... :.: ...:? :O~:t:9.1..... :.. J.* ~~:-R~ .... :.... :-.~ ,$ ...... : .... ~.. J'.~:-R?...... :.... 7.. ~~:-R" .. :.... :-.~ .~..... .

.... l.Q~.~~...... :.: .. ?.. ~~:-Q!;i.... : ~: ...4:~~:t:9.Q .... :.. J.. ~~:-Q!;i.... :.... :-.4:$...... :.... ~.. J'.~:-R?...... :.... J.. ~~:-Q~ .. : .....:? . J...... .

.. .. !.Q~.~~...... :~: .. J..Q~:-Q!;i.... :.: ...E?:$~:-:0~ .... :. J .. ~~:-R" .... :.... :-~ :$...... : .... ~..J'.~:-R?...... :.... ~.. ~~:-Qt;,.. : .... :-.4 ,9.... ..

10395 : : 9.SE-06 : : 3.3E-01 : 2.9E-05 : -4.5 : 3.7E-05 : 1.2E-05 : 1.3 .

.. i*03.96. *****: *: .. ;i.aE:06* ***: *: ***,- :ii..:o*o ****: **i2E:06.... :****:.s:s* *****: ****3*.:.;E:o~i *.. **: ****5°.6e::05*

1*1 ::,* *****

........................................................................................................................................... =* * *

61-1089

- - - - :<: 8.7E-05 ******

4.9E+OO : 1.SE-05 : -4.8 : 3.7E-05 ************************************

1.8E-04 : 2.1

.. :~1 :-.1.9.~0.... :~: .. ~.. .1.~:-lH.... :.: .. .1. :7~:t:9.Q .... :.. J..~~:-Q"* ... :.... :-.'~:7...... : .... ~3~:-Q!;i...... :.... ~.. ~~:-Q~.. : .... :-.4.~..... .

61-1092 :<: 9.4E-06 : : 5.2E-01 : 1.8E-05 : -4.7 : 3.7E-05 : 1.9E-05 : 2.0 No out of spec. nonoonseorv.at;ve oorrel.atfons .are observed

- - - - - -------- - - *- - - - .. Pu-242 (Np-237) in Prim.ter (Key Isotope : Co-60) r"

................ , : . : ................ : .....G9:-.E?9..... : ............... : ............... : hY.~l'.'J9.EL~9i-!.1ji;-i9.: .. Ci-!.lP.41.~~~~.. : .l~.Q x~ ...Ci-!.lP.*.

$i-!.ITIP.1.~ N':lro~~( .: !~9~PP.~ .CP.1"!<?: . : l<.~Y. !~9... CPM: :I.~<? /.~~Y. g{l~j9: .1<?9. !~9/~!!'.Y. : ...... ~ f P.t.QI'.' ...... : .. !~9,. .C~>r!<?: .. : ... ff P.t.QI'.' ... .

.. .. !.Q~~! ...... :~: .. ?.. ~~:-R~ ..... : .. ~=~~.-t:9.~ .... : .. , ...1.~:-R? .... :.... :-~:4 ...... : .... :?..~~:-R? ...... : .... ! ..~~:-R~ .. : .... :-.1. :e..... .

I 0392 : : 2.SE-03 : 5.2E+02 : 5.4E-06 : -5.3 : 2.3E-07 : 1.2E-04 : . -23.1

.. ,. io39i .... *: *: **fG{-05* *** *: ***2:5E*.;o*i .. **: **i*1*E:ae* ***: ****::1:5* *.... :***'iiE:01* *****: ***'i:i.aE:04* *: *.. **1*.6* .... ..

.:.. i'o~94' ..... :<: .. i*.oE:05' .... :.. 'i:4E +01 .... :.. 4'.'1*E:07' ... :.... :..*6:4* ..... :.... 2°.3E:01' ..... :.... 5°.7E:o,s'.: .... :.:; :S- ... ..

0

.....:: !.Q~~~ :: :: :1:.:: I::.. f~~~~i:::

i:o~~~:...... :i:: :~;~~:~9i:::: i: :i~~~i:ie:::: 1::: :~:1;~:: :: :: 1::: :i~~~Rf::: :: 1::: :~:.ij~~R~:: 1: :: :i~: : : ::

~..!:!~:-Q~ ..... : .. .1.: 1[t:9~ .... : .. , .. ~~:-Re .... : .... :-."? :4 ...... : .... :?.. ~~:-Q7 ...... : .... 7..~~:-Q~ .. : .....~ . ~.......

61-1089 :<: 8.7E-05 : 4.1E+02 : 2.1E-07 : -6.7 : 2.3E-07 : 9.5E-05: 1.1

... 61 :.*10*90' *". :<: .. iXE:04' .... : .. 'i:iE'+oi .. *-: .. i°.3E:i::i,s' ... : .... :.si ..... : ... 2°.!E:07' ..... : ... S .4E:o:s": .... :.s:e" 0 0 0 61-1092 :<: 9.4E-06 : 5.5E+01 : 1.7E-07 : -6.8 : 2.3E-07 : 1.3E-05 : 1.4 There is no obvious route to modify So.aling F.aotor to eliminate the out of spec. nonconservative oorri?lation

- - ------ - - *- - - -*- - - Cm-243 (Cm-244) in Primary * (Key Isotope : Ce-144)

................. : . : ............... : . : ....C,."'.1 ~~- ... : ............... :............... :.~Y.E:'=J9.E: .~9~.11~9.: ..C~.lP.41.~~'~*.: ,l:;,q x~ ... C~.lP.. .

$~,FTlP.1.e: N1:1ro~.E:'=: . : !~9~P.P., .CPrtQ, : . :l<.E:Y. !~9:.<;:pnq: :1.~9 l.~tY. g~~19: .199. !~9 /~,.Y . :..... f JP.t.Q~ ...... : .. !~9... CPnQ: .. : ... f ~P.t.qr: .. ..

.. .. J.Q9.~L ..... : .: .. ~.-~~:-P4. ... : ~: .. ~=~~:1:0.Q .... : .. J..Q~:-Q~.... : .... :-.4,0...... :.... ?.. Q~:-Q~...... : .... 9.*~~:-!=!9 .. : .....~ . ?...... .

.. .. !.Q9.~i...... :~: .. L.~~:-R?.... :.: .. .~ ,O~:f:9.1..... :.. ?.. J'.~:-Qf ... :.... :-.~,9...... :.... ?.. Q~:-Q~ ...... :.... ,A~~:-Q?.. :.... :-.1., 1.... ..

.. .. !.Q9.~~...... :.: .. ~.. Q~:-R~ .... :.: ...4:~~:f:0.Q .... :.. L-~~:-Q9.... :.... :-~,~- ..... : ... .?.. Q~:-R~ ...... : .... 9.. ~~:-R9 .. :.... :-.1. ,~ .... ..

10394 : : 1.SE-04 : :

6.SE;,.02 : 2.6E-03 : -2.6 : 9.0E-04 : 6.1E-05 : -2.9

.. ** ,*03*9~; **.. *: *: *-~i.1E:04* .. *: *: ***i:~i..:cfr ****: **1*.1E:oi ***: ****:.:i:a* *****=* * * *9*.oE:04* *****=* * * *ioE:04* *: *.. *:.*, :9.. **..

.... ,*a3.96. ** ** *= * =**2'.iE:04* .. *= *: ** *; :5E*+a*o** ** :* *,*.sE:04* *** :* ***:.*ia** .. ** :* ** *9*.oE:04* *****: *** *,*.4E:oi* =* ** **6*.;* ** ** **

:~1~)9~?: :::1: 1::~j~~Ri :: :1 :1 :: 4;~~:~9:q:: :: 1:: (~~~Ri: :: 1::: :~~i: : : 1: :: :~:.Q~~Q~:::::: 1: :: :~:.~~~R~::1: :: :~:1: i: :: ::

... ~ 1:-.1. 9.<E!O.... : . : .. 9..~~ :-R~ .... : . : .. .1. ,7~:t:9.Q .... : .. 9.*~~ :-Q9.... :.... :-.~,~ ...... :.... ?.. Q~ :-Q~...... : .... L.~~:-Q9.. :.... :-.4 ,?.... ..

61-1092 : : 4.9E-04 : : 5.2E-01 : 9.4E-04 : -3.0 : 9.0E-04 : 4.7E-04 : -1 .0

- - ----*-- - -*- - - - - - - Cm-243 (Cm-244) in Primar (Key Isotope : Co-60)

................. : ................ : .: .....G9:-.E?9..... : ............... : ............... : .~Y.E:17~9.E: .~9~.ljtl9.:. ,c;i),lp,41,~,~~-.: .1~.C! ."<~:.C~.19.:.

$~.l'flP.l.e: .~':lro~.~17:. !~9~PP.~ .!;P.I'!<?::. :l:<.E:Y. !~9... C9.1'!Q: :l.~9(,IStY. .~1~j9: .199. !~9/~~.Y.: ... :. f 1P.t.Q17 .. ; ... : .. !~9... C9n<?: .. :: .. f ~P.t.Q17 ... .

. .. .. J.Q?.~L ..... : .. -~--~~:-R~ .... :.: ...!:?.~~.-t:9.4 .... : .. ~.-R;:-Q7.... :.... :-.E?:? ...... : .... 9.-l~:-Q9...... : .... ?.-:!i~:-Q~.. : ..... 9..... .. e.

... . LQ?.~~- ..... :~ .. !.-~~:-R:?.... :.: .. .~.?~:t:9.4 .... :..?.*R~:-Q9 .... :.... :-.'l,., ...... :.... 9.-l;:-Q9, ..... :.... ?.,Q;:-Q~.. : .... :-.E?.~ .... ..

1039! : 5.0E-03 : : 2.5E+03 : 2.0E-06 :. -5.7 *: 5.7E-06 : 1.4E-02 : 2.8 .

....:::fq~:~~:::: :*: 1: ::i:.ij~7R,f::: 1: 1:: i4~:~~1::::: 1:: ~-,:.~i7~i::: 1:::: ~ii:::::: 1::: :~j~7R~:::::: 1:::: ;:.~~7R4:: 1:::: ~:,: i:::::

~ ~

!.Q:P~?...... : ... ?.-7:~:-R'f .... :.: .. ~.~~:t:9.4 .... : .. .. Q~:-Qi;,.... : .... -:-.~.?...... : .... ..:;:~:-Qi;,...... : .... J..l~:-Q~.. : .....?. ..... .. ~

.. : . J.Q?.~P...... :... ~--~~:-Rf ... :.: .. .1.: 1~:t:9.4 .... : .. i .. J.~:-Q9.... :.... :-.~ ,7...... :.... ~--l~:-A9 ...... :.... ~--~~:-Q~.. : .....?. ?..... ..

. .. R1 :-.1.9.E;I~.... : ... P.-~~:-Rl ... :.: ...4,1 ~:t:9.4 .... : .. J.* l;:-Q9.... : .... :-.'l,e...... : .... ?.-:?:;:-Q9...... :.... 7.-:!i~:-Q~.. : .... -:-.q,Q .... ..

.. . ~ 1:-. Hl.~9.... : . . .P.-~~:-R~.... : .: .. .4.~~:t:9.4 .. .. :.. 7A;!; :-Q9.... :.... :-.'l ,,;,...... :.... ?.,:?:;:-Q9, ..... :.... J..:!i;:-Q~.. :.... :-.4 .~..... .

61-1092 : 4.9E-04 5.5E+01 : 8.9E-06 : -5.1 : 5.7E-06 : 3.1E-04 : -1.6

I - -

Primary Resin. Scaling Factor Evaluation

- - - - - - - - - - - - -*- -.- - Sr-90 in ry Resin

................. : . : ............... :. : .... Ci>."'.1 R7.... : ............... : ............... : ,",y,e.r.~9.~ .~'?~.tji:ig : ..C~.lP.41.~~~~.. : .lis.ci .'{~... C~JP.*.

~~.rfl.P.l.~ N':lro~.~t::.: !~9~P.P.~ .CP.1"!<?::. :~.~Y. !~9,.CPJW: :l.~91.~~Y. g~~i9: .199. !~9/~,.Y.: ...... ~~P.t..cir: ...... : .. !!19:.CPT!<?: .. : ... f ~P~.C!t: ... .

.. .. !.Q~~~...... :.: .. ~.. ~;-:-Q? .... :.: .. .1. :f;!~:t9.1..... : .. :;?A~;-:-R9.... :.... :-.'4:7...... : .... ~..'.~;-:-R9 ...... : .... ?.. ~~-:-R?.. :..... ?. , ..... ..

... . !.Q~.i9...... :.: .. ~.-~;-:-R1 .... :.: .. .1.: 1~:t9.'4 .... :.. ~.. ~;-:-R9.... :.... :-.'4:~...... :..... ~.. ~~-:-R?i... : .. :.... ~.*R~-:-Rl .. :..... 1:,..... ..

10447 : : 2.6E-01 : : 2.7E+01 : 9.7E-03 : -2.0 : 4.9E-03. : 1.3E-01 : -2.0 i:q~~~: :: :: :;: :1

::61-1087 ::i:.~~~i:i~:::: 1:: :\:: :8.0E+OO

3.3E-01

.~~7q~

::: :1: :: :~ii:::::

,: ;~~:~9:1: : : :\:: 4.1E-02 -1.4 1::::

~jt7q~:::::: 1:::

4.9E-03. :

i~t7Ri:

3.9E-02 :

1::: )ii::::::

-8.5

.. *6; ~*,o'ae ***: *: .. 4*.oE.:.i:ii ***: *: ***; :~i*+clo ****: **i°.1E.:.oi ***: ****~-, i *****: ****4°.9E.:.oi *****: *. ***1'.iE.:.oi.. :****~s:5.. ****

No out. of speo. noncons:erv at.ive co:,rre lat.ions are obse-rved

-* .. - -- Tc-99 ;n P Resin

................. :. . :. ............... .. : . : .....C~:-: 1~ 7..... : ............... : . . . . . . . . . . . . . . . .,*'r:t.~I'.' ~9.~ .~9~.lji;i9. : ..C~.lP.41.~~~~- . : .l!>.Q ."{~,. C~JP*.

~~fflP.~~ N~ro~.~I'.':.: !~9~P.P.~ .CP.r!Q,:. :l<.~Y. !~9... CP.r!Q, :I.S:Q/.~~Y. -~~~j9: .11?9. !~9/~!!'.Y ...... f ~P.~.QI'.' ...... : .. !~9... C9.1'1Q, .. : ... f ~P.\QI'.' ... .

.. . .L. ~.4 ....... :~: .. ?.J'.~:-R~ .... :.: .. .1. ,~~.-+:9.1..... : ..~1i.rri.iM~ll~ .. : .... -~--l~, ..... .... ?.. ~~:-Q~ ...... : .... J.. R~:-Rl .. :... .1.1?~-E! ..

.. .. !.Q1.4'?...... :1: .. !.. ~~:-R~ .... : .: .. .1. ,1 ~.-+:9.4 .... : ..~li.l'fl.ifl.~~~~-.: .... -~---~, ......... ?.. ~~:-Q~ ...... : .... '?.. ~~:-Rl .. : ...

.... LQ~.4r ..... :~: .. J..i'.~:-R~.... :.: .. -.4,7~.-+:9.t..... :. Jli.l'fl.iri.~~ll~ .. : ..... ~.-.A., ......... ?.. ~~:-R~...... :.... , .. ~~:-Rl .. :... -~-~.'?..... .

~~~.:"l .. :::

...J;°:.~i*a1* ... ( .. !A~~:~t. ... 1. 1.. .1. :~~-:9.1..... 1.. ~imi~.~~~~-. [ .... :.~.-.A.: ......... ?.. ~~=Q~...... \.... ?.. ~~=Q:? .. \... ~~~.,1. .... .

.. .. .. .. .. .. ... . .. .. .. ~.-R ....:?..........~,O~.. 9.Q ...... ,.,..,.;:~. Q~...........4,!;i .......... ~.. ~~- Q~ ...... : .... ~.. 7:~. Q?.. : ..... L~...... .

61-1088 : : I .6E-D2 : : 1 .5E+OO : 1 .1 E-02 : -2.0 5.9E-03 : 8.8E-03 : -1 .8 See .aUached exp 1ana1ion

- - - - **-' - - - - - - -: - - .. - *- - Tc-99 in Prim.ary Re-sin difie-d Soaling Factor

........... :..... :.: ............... :.:....c;:~:-: rn7 .... :............... :............... :lr:t~r:fi9.~ .~9~.1il;l9.: ..C~.lP.41.~~~'if .. : .l~.C! .\'.f, .C~JP.*.

$~.rrrP.1.e: N':lroP.e:r::.: !~9~P.P.~ .CP.rl9,:. :~.E:Y. !~9, .CP.r'!<?: :1.:s;q/.~~Y. g~~)9: .1Q9. !~9/'>!l'.Y.: ...... ~ ~P.t.C!I'.' ...... : .. !~9 . ,i:;:PM, .. :.:. f fiP.t.C!I'.' .*..

.. .. !.Q~.4?...... :~: .. ?.. ~~:-Q4 .... :.: .. .1. :~~.-t:9.1..... : .. 9.,g~:-Q~ .... :.; .. :-.4:~ ...... : .... J..~~:-Q4...... : .... f .. ~~:-Q~ .. : .....4. ~.......

10446 :<: 1.4E-03 : : 1.1E+02 : 1.3E~05 : -4.9 : 1.5E-04 : 1.6E-02 : 11.6

.... ;*0441* .... *:<: * * ,*.1E:oi .. *: *: ** *i:1r*+o"1 ** **: * *6*.iE:05* ** *: **** :.*4:i° ***.. : *** *; *.sE:04* *** .. : ****4*.oE:oi

*.... '.i°.4. ***...

. . . . !.Q~.!;;19...... :~: .. L.~~:-Q4 .... :.: ...1. :9~:i:9.1..... : .. J.. g~:-Q!;i .... : .... :".4,~...... : .... J.. ~~:-Q4...... : .... :?.. Q~:-Q~.. :.... L~:4 ...... .

61-1087

......... : .: 2.E,E-02

- - - .************ : : 8.0E+OO

.. ****** .......... : . 3.3E-03 **************

- - - - .............. : -2.5 ................

1.5E-04 : 1.2E-03 : -21.9 61-1088 : : 1.6E-02 : : 1.5E+OO : 1.1E-02 : -2.0 : 1.5E-04 : 2.2E-04: -71.8

Jc-99 in PJ:i eu:,: Resin The unmodified S,F. was l.5E-04: however, this resulted in a nonconservative calculated isotopic concentration for samples 61-1087 and 61-1088: neither of which contained <LLD values. Therefore, the S.F. was recalculated using only the positive values of samples 61-1087, and 61-1088. resulting with a conservative factor of S.9E-03.

-. - - - - -*--- -*-*- -* - - .. 1-129 in Pr Resin I

. : : Cs-1 37 : :

. . . . . . . . . . . . . . . . . . ................................................................... :. ..AY.~I'.' "9.~ ..

S'?fl.1'J1;'19. :' ***Cfl.1P.41.~t.~ d

... :' .l!>.Q .'<,: ..Cfl.1P.*.

$flfflP.l.~ N':lro~.~I'.' .: !~9~PP.~ .CP.l'!Q::. :K~Y. !~9:.CP.IW: .S:Q/.~fY. -~"~j9: .1<?9.1~9/~!l'.Y.: ..... f "P.t,q,: ...... : .. !~9... CPM: .. : ... f "P~.QI'.' .. ..

.. .. LQ~.4?. .. . . . . :.. ~--~F;:-Q!;i.... : . : .. .1. :!$~:t:9.1. . . . . . .~j::F;:-Q9.... : .... :-~ ::;: ...... :.... ':SA:!F;:-Q9..... c-: .... , .. ~F;:-Q4.. :..... 1. ?...... .

.... LQ~.4~....... :.. ~--~F;:-R4 .... : .: ...1. :1 ~:t:9.:? .... .. ~.-~F;:-R9.... :.... :-.~:1 ....... :.... ':SA:!F;:-R9...... :.... 7.-~F;:-R4.. :.... :-.1. :?.... ..

.. .. 1LQ~:H Q556

.......<:: .. 4J..~F;:-R4 2E-04

.... :.: ...4:7~:+:0.1.... , .. !;5}~F;:-Q9

: 1 3E +O 1 3 1E-

.... :: .... :-.5.2 : 6.SE-06 : 1 .9E-04 :

1.2

...61 ............... ,', ................. :.............. ,', ... 99 ...........4 :9...... : .. .lf?o):~F;. QE;i, ****** : **** ?.-~F;:-Q9.. : .... :-.4:9..... .

- *61~-}g:~- *** r**t~~:§~*** -i

i * * *1:~r:g-g .. ** **;*::~:§t ** i- ** *:*;t* *

i *

t::~:§t***

i- * * }:8~:§~** 1* ** -t~* * *

I I

I I

II

................. :. : ............... : .: .....G9:-f/J..... :............... : ............... /: lr:t.~t:{19.~ .~9i!.ljr;i9.: ..i;i!JP.41.~~~~ .. : .l!>.Q x~ ... i:;:~JP.*.

$~.rflP. l.~ .~l,l!'D~.~t:: . : !~9~PP.~ .i;pnq: : . :l<.~Y. !~9,. i:;:pnq: :1.:::q (.t.;~Y. g{l~j,;,; .lqg, !~9/~~.Y .1: ..... f {19.\Qt:' ...... : .. !~9,. i:;:pnq: .. : ... f {lp,t_qt: ... .

10445

.**.********.*..** :<: 9.5E-02 ,, ***********.***..********.**.**

,, .**********. : : 7.3E+01 : 1.3E-03, ******..**********

-2.9 1

1.8E-04

- I** .*******.* : ,, *.1.3E-02:

,, *****.** -7.2 10446 :<: 2.5E-01 : : 1 .1 E+02 : 2.4E-03 : -2.6 r: 1.8E-04 : 1.9E-02 : -13.1

:: i:rj~i/:: :: :: :1 ::i~i~f-ii :: :1 :1:: i~f~0:i:: :: 1: :~)i~i:i6:: :: 1:::: ~:4:i:::: :r :: :(~i~R4:::: :: 1::: :1)i~Ri: 1::: :ih: :: :: ::

.... l.Q?.!:i~...... :.: .. J..!::~-:-P.~ .... :.: ...1. =~~.-t:9Q .... : .. '?,'~~-:-:-!<f .... : .... :-.~,O..... : .... U:~~-:-:-!~ ...... : .... ?.. ~~-:-:-!~ .. : .... :-.!:;i:9 ......

61-1087 ....................

.. ************ : : 2.2E-03 : ..............................

1.7E+02 : 1.3E-05' .....................................................................

-4.9 : 1.8E-04 : 3.1E-02 : 13.9 .

61-1088 :<: 3.2E-04 : : 3.2E+01 : 1.0E-05 : -5.0 ,: 1.8E-04 : 5.7E-03 : 17.9 I

I II I'

I I

II Eliminatfon of th'=' <LLD val*Je:s: for C-14 in sampl'='s 10445, 10446 wouldlre:s:ult in a less c:onservative Scaling Factor I

I

................. : .: ............... : .: .... .G9:-.~9..... :.......... ; .... :. .. .. . . .. .. .. . . ..',Y.~1'.' ft9.~ .~9~.lj1;"19. : .. C~.lP.41.<!~~~.. : .1~.C! -~~:. C~.lP.*.

$~.l'!'lP.1.~ N':lro~.~I'.':.: l:!f9~PP.~ .CP.11<?,:. :K~Y. !:!f9: .C!>f!Q, .~Q !.IS~Y. -~~~i9: .1Q9. !:!f9/~,.Y ...... f ~P.~.C!I'.' ...... : .. !:!f9: .C~nq, .. :... f ~9.~.C!I'.' ... ;

10445 : : 3.7E+OO : : 7.!E+Ot 5.0E-02 : -1.3 3.0E-02 : 2.2E+OO : -1.7

.... J.Qi:l.4~...... :.: .. J.-~~T.QJ .... :.: .. .1., 1~:t:9~.... . .J.-~~:-Q1 .... : .... :-Q .~...... . .. -~--9.~:-P.? ...... :....~:~~tP.0.. :.... :-~ .~ ..... .

. .. . 104i7 : : 2.3E+OO : : 3.9E+02 5.9E-03 : -2.2 3.0E-02 : 1 .2E+01 : 5.1

.... ;:g~~~:::::: 1: i: )j~~i:!i: :: :! :1:: :,: ;~~:~9:Q:::: ::;:.~~7R1:: :: 1: :: :~~re:::::: :::i-R~7Ri::::: 1::: :~:.j~~Ri:: 1:::: ~~;e:::: :

~

... R1 :-.1.9.E:i?. ... :.: .. .. ~~T.Q9.... :.: .. .1. ,7~:t:9.4 ...... U5!~:-P.?.... : .... :-.1. ,7......... -~--9.~:-P.? ...... :....9:J~tP.0.. :..... L~...... .

61-1088 : : 2.4E-01 : : 3.2E+01 7.5E-03 : -2.1 3.0E-02 : 9.5E-01 : 4.0

(

-- -- - Ni-63 in P

- r - - - - -*- -

Resin I

................. :.: ............... : .: .... ~9:-~9..... :............... :............... :.~Y~~J9.~ .~9~.lj~9.: ..(;~.lP.l!l.~~Et~ .. : .IF.Q .'<~:.C~JP.*.

$~.F'fl.P.l.~ .~\JITI~.~~:.: !~9~P.P.~ .CP.l"!C?::. :l:<.~Y. !~9:.CPnq: :1.S;<?/.IS,Y. .~~~j9:. lQ9. !~9/~,.Y.: J.... f ~9.~.Q~ ...... : .. !~9:.CP.'"!Q: .. : ... f ~P.~.Q~ ... .

10445 : : !.6E+01 : : 7 .3E+01 : 4.9E-01 : -0.3 :I 3.6E-01 : 2.6E+01 : -1 .4

qi4~

:::: \: 1:: i\~t:q;:::: 1: 1:: :1:;1~:~9i::: i~~7R1:::: ~::::~RI:.::::~ Ii::: i~~7R1:::::: ~:: *: i~~tQi:: ~:::: ~:1:; i::::::

10447 : : 1 .OE+02 : :

3.9E+02 ' : 2.5E-01 : -0.6 : 3.6E-01 : 1 .4E+02 : 1 .4

- .. ;*0556 .... *: *: **;.4E:o, .. **: *: .. *; :9E+cici .. ** i4E:a1 ****: *.. *:.o:s...... i ***i6E:a, .... **: *.. *6°.eE:o, .. :*.... ,.; *......

* *

~ i ~:i of,::::~:~:: ;:.R~t9~:::: ~: :1~:~~ii:::: ~j~7Q1:::: 1:::: ~R :i::::::)::: i~~7R1:::::: i::: i.o:~tQ1:: ~:::: ~\}:::::

61-1088 : : 6.BE+OO : : 3.2E+01 : 2.1E-01 : -0.7 :/ 3.6E-01 : 1.1E+01 : 1.7

- - - -** - - -***- --------- Pu-241 in Primary Resi lsotop* : c.L 44)

- ** ** ** * ** * ** ** *: * : ** ** ** ** ** * * ** *: .: .... (;~.--: 1~~-: .. : ............... :............... : .A,. Y.~r: ~9.~ .~9~.lj~g : . .c;;~JP.41.~1~~-. : ,li,,q .'<~: .(;~JP.. .

!;:~.rriP.1.~ .r~~ro~.~r::.: !~9~PP.~ ,c;;p,11Q,:.: K~Y. !~9 . ,(;:!)f!Q, :l.~c;i !.~~Y. g~~j*?:. lQ9. !~9/~~.Y.: ..... -~ ~P.~_qr: ...... : .. !~9 .. ,c;;pnq: .. :, .. f ~P.t,qr: ... .

10445 : : 1 .7E-02 : : 6.1 E-02 : 2.8E-01 : -0.5 : 1 3.2E-01 : 2.0E-02 : 1 .1

- .. ;*04.46. **.. *: *: .. 2..2{:.o,* .. *: *: .. i:2E*~o*1* .... :**i*,*E.:.o, **.. :****:.o:s* *.. **:r **3*.2E.:.o; .. ****: *.. *2*.iE.:.o, .. :* .... ;'.ci ......

- - - *044
      
      *1 *****: *: **i.sE.:.o; ****: *: **2:oE*~o,* ****: **; *.1E+*oo* ***: *****o'.i* ******: i2E.:.o, ******: ****6*.sE.:.oi' *: ****:.*si *****

1 * * *

.... ;*oi:5s6* *.. **: *: .. ioE.:.oi .. *: *: ***; :aE*~o2 .... :**1*.6E.:.o; **.. :*.. *:.*a:e* *.. **: i ***i2E.:.o; .. ****: *.. *s*.9E.:.oi *:* .. ..i'.o* ......

- - e:; ~, o'ei ***: *: **9.e:E.:.oi' ***: *: **'i:iE~o*1* ****: **4°.2E.:.o; ****: ****:.*a:4* *****: i***i2E.:.o, ******: ****7.4e:.:.oi' *: ****:.*; i *****

- - e:; :.*; o* *a****:*:**; *.6E.:.oi' ***: (: ***; :~i~o*1* ****: **1*:1*E.:.o; ****: ****:.*; :o* *****: i***i2E.:.o, ******: ****4*: *E.:.oi' *: ****i.o* ******

- -. -*- - - - -*- - -- - -*- - 11111 Pu-241 in Primary Resi Isotope : Co-60)

. . . . C 6n . ' .

. . . . . . . . . . . . . . . . :: . : ............... : . : ...... 9:-.. 'l-'***** : *************** : *************** : .PJY.e.r. fl9.E! .~9~.lj~9. : ..9~.lP.41.~~~~- . : .l~.C! -~~:. f:;~.lP.*

~~.rr1P.l.e: N':lro~.E!t:':.: !~9~!>P.~ .9!>.11<?,:. :l.<.E!Y. !~9, .C!>.f'!Q, :l.~C? /.!S,Y. gfl~j9: .1<?9. !~9/'>!l'.Y.:. J**.. ~ f!P.t.Qt:' ...... : .. !~9,.C!>.f'!Q, .. : ... f flP~.C!t:' ... :

.... !.Q~::l~...... :.: .. !.-i'.~:-Rl ... :.: ..."? .~~:t:0.1..... : .. 7.-~~:-Q~ .... : .... :-.~,f? ...... :. J .. 7A~~:-Q~...... :.... !;5.,R~:-Q? .. :..... ~ . ~- ..... .

.. .. LQ~.4~...... :.:. -~--~~:-R1 .... :.: .. .1., 1~:t:O~ .... : .. 7.-.1.~:-Q~ .... : .... :-.~.7 ...... :. l .. 7.-R~:-Q~ ...... : .... ~...1.~:-Q? .. :.... :-~ ,7 ..... .

.. . . !.Q~.47...... :.: .. ~--~~:-R1 .... :.: ...~.~~.-t:O.:? .... :.. ~--~~:-Q~.... : .... :-.~, 1...... :. l .. 7.-!=:~:-Q~...... : .... ~.. Q~:-Rl .. :.... :-.1. ,?..... .

.. .. LQ!;i~~- ..... : .: .. ~.. Q~:-Q~.... : . : .. .1.*~~.-t:O.Q .... : .. J.-!S:~:-Q~.... : .... :-.'.:?,~ ...... :.1... 7.-R~:-R~ ...... : .... J.. ~~:-Q~.. : .... :-~,1 ..... .

. . . !=: 1:-.1. 0.1;17.... :.: .. ~--!=:~:-R? .... :.: .. .1.* 7~.-t:0.:? .... : .. !;5.. !=:~:-Q~ .... : .... :-.~ ,?...... : ./... 7.-!=:~:-Q~...... : .... J.-~~:-Q1 .. : ..... 1.-~...... .

61-1088 : : 1 .6E-02 : : 3.2E+01 : 5.0E-04 : -3.3 : I 7.6E-04 : 2.4E-02 : 1.5

- - ------ - - .... .. -- --- - Cm-242 in Primary Re ey Isotope : Ce-144)

................. : . : ............... : . : .... C~.-:1 ~~ .... :............... :............... : /1,y,e,r;~9.e, .~9~.ljri9.: ..C~.lP.41.-,1~~.. : .l~.C! .'!,... ~~.l~.. .

$~P.l.e. N':lro~.e.r::.: 1~9~P.P.~ .CP.11<?,:. :~.e.Y .1~9... ~~>nq, :1.~Q/.~,Y. .l~~~j9: .1Q9.1~9/~,.Y.: ..... f ~P.t.Qr:- ...... :.. !~9... CP.l'!Q: .. : ... f ~P.t.Qt:" ... .

.. .. J.Q1.4?...... :.: .. J..~~:-Q~ .... :.: ...~, 1~.-:9~ .... : .. i .. ~~:-R? .... :.... :-.1.* ~ ...... : .... f .. ~~:-R9...... :... J .. ~~:-Q~.. : .... :-.~, 1.. .. ..

. . .. J.Q1.4~...... :.: .. ?)~;:-Qf ... :.: ..."? ,?~.-:9.1..... :.. 7.,!=:;:-Qf ... :.... :-.~, 1...... :.... f .. ~;:-R9...... :.... U~;:-Ql.: ..... ~ . ~...... .

.. .. !.Q~.47...... : .: .. U~~:-R~: ... :.: ...4,0~.-:9.1..... :.. ~.. .1.~:-Ql ... :.... :-.:?,Q...... : .... i .. ~~:-R9...... :.... !?.. Q~:-Q~.. :.... :-.~,?.... ..

.. .. !.Q!?~~...... : . : .. J..~~ :-R~.... : . : .. .1. ,$~.-:9g .... : . J .. Q~ :-Q?.... :.... :-.:? ,9...... : .... i .. ~~>:*Ql ..... :.... ~.-~~ :-Q9.. : .... :-.4 ,?.... ..

.. .!=:l ~.1.9.~7.... : .: .. ~..~;:-Q~ .... :.: ...4,~~.-:9.1..... :.. ,...1.;:-Q9.... :.... :-.~:9...... :.... i .. ~~:-R9...... :.... !?.. ~;:-Q~ .. :..... ?. ~...... .

61-1088 : : 1.9E-05 :<: 1.5E-01 : 1.3E-04 : -3.9 : 2.5E-03 : 3.7E-04: 19.4 No out of spec. nonconservative correletions are observed

-- Cm-242 in Primary ey Isotope : Co-60)

................. : .: ............... : .: .....G9:-~9..... : ............... : ............... : ."~Y.~r:~9.~ .~9i!.lii:i9.: ..Cit.lP.41.~~~,;f .. : .lf.Q ."<i ... Cit.19.. .

$ittn.P.1.~ N':Jro~r::.: !~9~PP.~ .CP.l'!Q::. :l:<.~Y. !~9... CPnQ: :l.:s:q(.l<;tY. g~~i9: .1<?9. !~9/~!!'.Y.: ..... f ~P.t.Q,:" ...... : .. !~9... Cpf!Q: .. : ... f ~P.t,qr:- ... .

.. .. !.Q~;'l?...... :.: .. J..~~-:-R~.... :.: .. ."?:~[+:9.1..... : .. J..~~:-R~ .... : .... :-4:7...... : .... ?.. ~~:-R9 ...... : .... ~.. ~~:-R':l .. : .... :-~ ::? .... ..

.. .. !.Q~P...... : .: .. ?.,i:!~ -:-R':l.... : . : .. .1. :.1 ~:+:9.4 .... :.. ?..,1,~:-R9.... : .... :-~ :~...... :.... ?.. ~~ :-R9...... : .... 9.,g~ :-R'f.. :..... 1.. L .... ..

.. .. !.Q~47...... :.: .. J.. ~~:-R~.... :.: .. ,q:~~:+:9:4 .... : .. ~.}~:-R9 .... : .... :-~.~...... : .... !;5.. ~~:'R9 ...... : .... :?..~~:-R~ .. :..... 1. ~...... .

.. .. !.Q!;:i~~...... : . : .. J..~~-:-R~.... :.: .. .1. :~~:+:9.Q .... : .. J.. Q~:-R':l .... :.... :-.4:9...... : .... !;5.. ~~-:-R9...... : .... L.1.~:-R~.. :....~F . ~ ... ..

61-1087 : : 2.5E-04 : : 1 .7E+02

......................................................... : 1.5E-06

-5.8 ..........................

- : 5.8E-06 :****************

9.9E-04 :...............

4.0 .

61-1088 : : 1.9E-05 : : 3.2E+01 : 5.9E-07 : -6.2 : 5.8E-06 : 1.9E-04 : 9.8 Since there is no influence from <LLD values, 'there is no obvious route to modify Scaling Factor ,

- - - -* - - - - - - - - ... - - -*- Pu-238 in Primary Resi lso~ope : Ce-144)

................. : .:............... : .:... ,c;,.--: 1~4 .... : ............... :............... :liY.e.r: ~9.~ .~9i1Jji:a9. : ..Ci1.1P.41.~~~~.. : .I~.<! .'<f, .c;~JP.*.

~~.r(l.P.1.~ .~i..iro~.~I'.':.: !~9~PP.~ .CP.r!Q::.: l<.~Y. !~9 ... CPnQ: :l.~Q l.~tY. .F~~~j9: .1Q9. !~9/i>,.Y.: ...... ~ ftP.~.Qt:'.; .... : .. !~9 ... CP.l'lQ: .. : ... f {tP.~.QI'.' ... .

.. .. !.Q~.4~...... :.: .. J..g~:-1=!4.... :.: .. ~:1 ~:-:Qg .... : .-.7.. Q~7Q9, ... : .... :-:4:? ...... :.... ~.. Q~:-Ql ..... : .... :?..~~:-Q4 .. :.....?. 9..... ..

.. .. J.Q~.4~...... :.: .. ~.. Q~:-R9 .... :.: .. .1 :?~:-:9.1..... : .. ~.. ~~::R9.... :.... :-'4:4...... :.... ~.. Q~:-Q~...... : .... 7..!=~~:-Q9.. :.... :-.1. :1 .... ..

.. .. !.Q~:47...... :.: .. !.. ~~:-R9 .... :.: .. :4 :O~:-:Q.1..... : .. 7,.~~:-Q9 .... :.... :-:4 :1 ...... :.... ~..Q~::Q9, ..... : .... ?...1.~:-Q4 .. :.... :-.1. :~.... : .

.. .. !.Q~.!:?~...... : .: .. , .. ~~:-R~.... : .: .. .1. :e~.-:Q~ .... : .. ?.. ~~ ::R9.... :.... :-.:? :'?...... :.... ~A~~ :-Q9, ..... :.... 7.. ~~ :-Q~.. :..... 1. 7...... .

.. .~1 :-.1.9~7.... : .: .. !.. ~~:-R9 .... :.: ...4,9~.-:Q.1 ..... : .. 7..Q~:-Q9 .... : .... :-:4:?-...... :.... ~.. Q~:-Q9 ...... : .... ~...1.~:-Q4 .. :.... :-.1. :e ..... .

61-1088 : : 5.9E-04 : <: 1 .5E-01 : 3.9E-03 : -2.4 : 4.0E-03 : !5.9E-04 : 1.0

- - - - - - - -* Pu-238 ;n Pr;mary Res y Isotope : Co-60)

................. : .: ............... : .: .....G9:-~9..... : ............... :............... :.~Y~r:~9.~ .~9~.lir:i9.: . .i:;:~JP.41.~~~9.. : .l~.Q ."<f,.C~JP.. .

$~.l'flP.l.~ .~':lro~.~r::.: !~9~PP.~ .CP.IW::. :l:<.~Y. !~9... CP.f'!Q: :l.~Q/.~tY. -~~~i9: .1Q9. !~9/~!!'.Y.: ..... f ~P.t.Qr: ...... : .. !~9,.CP.IW: .. : ... f ~P.t.Qr: ... .

.. . . !.Q~4!?...... :.: .. ! .. ~~:-R4 .... :.: .. J :9~:t:9.1..... : .. J.-R~:-Q9 .... :.... :-.~ :~...... : .... ~.. ~~:-R9 ...... : .... '?)~~:-Q4 .. :.....~..7...... .

.. .. J.Q~.4~...... :.: .. ~.-R~:-R9.... :.: .. .1. :1 ~:t:9.4 .... : .. ~.-~~:-Q~.... :.... :-.4:~...... :... -~--~~:-R9 ...... :.. :. J.. Q~:-R9.. :.... :-.~:9.... ..

.. .. !.Q~.47...... :.: .. U~~:-R~ .... :.: .. ~.~~:t:9.4 .... : .. ~A~~:-R9 .... :.... :-.~,4...... : ... -~--~~:-R9 ...... : .... ?<~~:-Q9 .. :.....f . ~..... ..

10556 * ; : 4.2E-05 ; : 1 .9E+OO : 2.2E-05 : -4.7 . : 9.4E-06 : 1.8E-05 : -2.4

.. . ~1 :-.1.9.!;!7. ... :.: .. !.-~~:-Rl ... :.: .. .1. ,7~:t:9.4 .... :. -~--~~:-R9 .... :.... :-.~,Q...... : ... -~--~~:-R9 ...... : .... J..~~:-Q~.. : .... :-.1. :0 ......

61-1088 : : 5.9E-04 : : 3.2E+Ol : 1 .SE-05 : -4.7 : 9.4E-06 : 3.0E-04 : -2.0

- - - - - --- --- - --- - - *- - Am-241 in Primary Resi . lso~ope : Ce-144)

................ :: .: ............... : . : ....C~:-: M.,.... : ............... :............... : hY.~17 ;9.~ -~9,1,ljl;l9. : .. C~.lP.41.~~~i;I.. : .IF.C! ."<f: .C'1.1P.*.

$,1.rrif ci~ .~':lroP.~'=).) !~9~PP.~ ,l'.;P.l"!C?:). \~-~Y. !~9...CP!l'1: ?~q(,l<;~Y. .Fi!;~j9( .1Q9. !~9/~~-Y.: ..... f ;p.~_q17 ...... : .. !~9... CP.1"!<?: .. : ... f ;p,~,q~ ... .

.. *. . fl~...... :.: .. l;l..~~:-R?.... :.: ...~:l~.":0~ .... :.. L-~~:-Q~... ,. :.... :-.4:~...... :... -~--!S:~:-Q.,...... : .... !;>.*~~:-!=!?.. :.... :-.1. :9.... ..

. . . .1

..0.. .1....... :.: .. ~--R~:-R'J .... :.: .. J =~~.":0.1 ..... : .. !;>*.R~:-Q., .... : .... :-~ :~...... :.... ~--R~:-Q'f ...... : .... ~-.J.~:-Q., .. :..... 1.,!?...... .

......*6i-g;-~r ..... :. (. L-~~:-R'f.... :.: ...4:0~.":0.1..... :.. 9)~~:-Q'f.... :.... :-.~ ::?...... :.... ~--!S:~:-Q'f...... :.... L.~~:-Q'f.. :..... 1..~..... ..

t... oei ... :.: .. ~.}~:-R9.... :.: .. .t. :e~:-:0~ .... :.. ?.-~~:-!=!1.... :.... :-~ =~* ..... : .... ~--!S:~:-Q.,...... : .... J.-!S:~:-R?.. :..... LP..... ..

.. .. .. :-.1......... :.: .. , ..R~:-R-,.... :.: ...4:~~.":0.1 ..... : .. L-l~:-Q~.... : .... :-.4:$...... :... -~--!S:~:-Q'f...... : .... i .. Q~:-Q'f .. :.... :-.4:0..... .

61-1088 : : 1.3E-04 :<: 1.5E-01 : 8.7E-04 :. -3.1 8.6E-04 1.!E-04: -1.0

- - ------ - - - - - *- -*- - Am-241 ;n Pr;mary Res y Isotope : Co-60)

................. : . : ............... : . : .....G9:-.E?9..... :............... :............... : .~Y.e.r. ~9.e. .~9~.lji:-r9. : ..C~.lP.41.~~'i;j*. : .1!>.C! .~,,. C~.lP.*.

$~.rflP. l.e. .~':IITl~.e.( . : ,~9~PP., .CPn<?:: . : l<.e.Y. !:!!9,. CPn<?: :1,~,.?f.~~Y. g~~i9: .199. !~9 /~~-Y . : ...... ~ ~P.t.Qr. ...... : .. !:!!'?:.Cpnq: .. : ... f {IP~.Qr. ... .

10445 : : 8.4E-05 : : 7 .!E+Ol : 1.1 E-06 : -5.9 : 2.0E-06 : 1 .5E-04 : 1.8

.... i*04.46.... **: *: .. 4*.oE:04* .. *: *: .. *,-: fr+cii ****: **iaE:oe: *.. :****:_*5 x *.. **: ****i'.oE:06* *.. **: ****2*.2E:04 .. :*.. *:_*,-:a-* ....

00000000000IIOOOIIOIOO 00000000 00 0001 000000000000000IOOOo lOIOOO I 0011000 0000 010100000111II000I00000000100001 0000010000100000 000000000oll 0000 10447 : : 1:2:E-04 : : 3.9E+02 : 3.4E-07 : -6.5 : 2.0E-06 : 8.0E-04. : 6.0

.... i*osse: .... *: *: .. 9*_1E:oi* .. *: *: ***,- :9£.+iio ****: **~i:,*E:06* *.. :*.. *::5j...... :****ioE:o.s* *.... :****i9E:oi.. :.. **:_is......

I0000IOII00000IOI00110000000 110000 100110 oOOO 100000 II O o 01 0000000 0000001 OOOOOOOOOOOI 0000000 I IOOOOOOOOOooOOOoOo 00000000000III00000o 00 oooOOoOo

... ~1 :-.1.9.~7.... : .: .. , ..R;:-R't .... : .: ...1. :7~:1:9.~ .... : .. i .. ~;:-Qi;i .... : .... :-.!:?,i;i ...... : .... i .. Q~:-Ri;i...... : ... -~--~~:-R't .. :.... :-.1.*~ ......

61-1088 : : 1.!E-04 : : 3.2E+01 : 4.1E-06 : -5.4 : ,2.0E-06 : 6.SE-05 : -2.0

- - - - - - - -*-*- - - - -*- - Pu-239 (Pu-240) in Primary (Key ls:otope : Ce- I 44)

................. : . : ............... : . : .... I'.;~;: 1~4 .... : ............... : ............... : lf'!.e.r. ~9.e. .~9iii.ljl'.l9.: ..Ciii.lP.41.~~~~-.: .l!>.Q .'ff. ,t;:i:IJP.-.

$iiifflP.l.e. N':IITIP.e.r.:.: !~9~P.P.~ .CP.l"!Q,:. :~.e.Y. !~9. ,i:;:9!W, :l.~Q(.~~Y. g~tj9: .1'?9. !~9/~~.Y.: ..... f ~P.t.Qt'.' ...... : .. !~9;_i:;:9nq, .. : ... f ~P.t.Qt'.' ... .

.. . . LQ~.4?...... :.: .. ~.-.1.;:-R9 .... :.: .. -~' 1~.-:Q~ .... : .. u~~~:-Q~ .... :.... :-.4,e...... : .... i .. ;:;::~:-Q~...... : .... J.. ~~:-Qf.: ..... L?..... ..

. . .. J.Q~.4'?...... :.: .. ?.-~~:-Rl ... :.: .. .1 ,4~.-:QJ. .... : .. }.~~:-Q~ .... : .... :-.:?,9 ...... : .... i ..;:;::~:-R~ ...... : ... J ..P.~:-Q~ .. : .... :-.1. ,9.... ..

.. . . LQ~.47...... :.: . .'~.-~~:-R4.... :.: ...4,9~::Q.1..... :.. ~--~~:-Q~ .... : .... :-.:?,I ..... : .... ~.. ;:;::~:-R~...... : ... -~--~~:-R4 .. :.... :-.4, 1.... ..

. . . . LQ?.!:;i'?, ..... :.: .. ~..,1.~:-R9 .... :.: .. ,1.*e~:-:Q~ .... : .. J.. J~:-Q~.... : .... :-.:?,e...... : .... i .. ;:;::~:-Q~...... : .... 1.. Q~:-Q9 .. : ..... L~..... ..

.. . P.1 :-.1. 9.~7.... : .: .. '?.-R; :-R't. ... : .: .. .4.~~::O .1 .*... : .. '.?.-~~ :-R~.... :.... :-.:? ,9...... :.... ~--~~ :-R~...... : .... !;:i.. Q~ :-Q4 .. :.... :-.1. ,4 .... ..

61-1088 : : 1.E,E-04 :( 1.5E-01 : 1.1E-03 : -3.0 : 2.2E-03 : 3.3E-04 : 2.0

- -- - - - -*- - \.

S l' . . .

s' ............... ..:............... :. .:. ......C9:-........ 60 . . . .A

............... : ............... : .. Y.~t: ~9.~ .. 9ft. !1)9. : .. r;:f!JP.l..!1.~~~9 .. : .I~.'=! .'{f,. 9:a.lP.* .

. :afflP. l.~ .~':IITIP.~r: . : !~9~PP.~ ,,;:Pf!9: : . : l:<.~Y. !~9,. 9?.1'!9, :1.S:Q /.~~Y. g~~i9: .199. !~9 /~~.Y . :..... f ~P.\Qr: ...... : .. !~9,. 9?.l'!'-1, .. : ... f ~P.t.Qr: ... .

.. .. !.Q~.4!?....... : .. '?..J.;:-Q~ .... :.: ...1 .~~.-t:9.1..... : .. J..'.~~:-R9 .... : .... :-.~ .~...... : .... ;i..7~:-Qi;. ....... : .... 9.-~~:-Q4 .. : ..... 'f..~...... .

.. .. !.Q~.49....... : .. ~--~;:-Q~ .... :.: .. .1., 1~.-t:9.4 .... : .. :?.-~;:-Q!:?.... : .... :-.4,7...... : ... ,;i,.~~:-Qi;....... : .... ;i)::\~:-Q4.. : .... :-.4:~.... ..

.. .. LQ~.47....... : .. '?.-~~:-Q4 .... :.: ...~.~~:t:9:4 .... : .. :?.. ~~:-Q9 .... : .... :-.~:9 ...... : .... ;i.. 7~:-Q9 ...... : .... :?.. Q~:-Q~ .. : .....4. !. ..... .

.. .. l.Q;i.~f>....... : .. ~.-H:-Q~ .... :.: .. .1. :~~.-t:9.Q .... : .. JA~:-Q!:?.... : .... :-.4,~...... : .... !?.. ~~:-Q9 ...... : .... "?.. ~~:-Q'9 .. : .... :-.~,'.?.... ..

.. . !=: 1*:-.1. 9.E;I?. .... : .. f>.Q~:-Q4 .... :.: .. .1. ,7~:t:9:4 .... : .. ~.. ~~:-Q9 .... : .... :-.~ ,!:? ...... : .... ;i.. 7~:-Q9 ...... : .... ~.. ~~:-Q4 .. : ..... 1..!;5...... .

61-1088 : 1.6E-04 : : 3.2E+01 : 5.0E-06 : -5.3 : 5.2E-06 : 1.7E-04 : 1.0

- -. - - - - - - - - - - - ---*- - Pu-242 (Np-237) in Primary (Key Isotope : Ce-144)

. . . . C 144 . . .A S 1' .

. . . . . . . . . . . * . * . . . : . : .........*..... : . : ....* ,.-. ..*.**.. : *.............. : .........*..... : .. Y~I'.' f9.E! .. 9'1. )(19. : **Cf!JP.41.~~"~* . : .lf.C! x,:. Cfl.lP.*.

$i1.rriP.l.E! N\Jro~.E!I'.':.: !~9~f.'P.~ .Cf.l.l"!Q::. :l.<.E!Y. !~9... CP.l"!Q, :l.~Q l.~,Y. R~~j,;,: .1Qg: !~9/~,.Y.: ..... f ~P.t.C?I'.' ...... : .* !~9... CP.l'!Q: .. : ... f ~P.t.QI'.' ..*.

.. .. !.Q~.4!;i...... :~: .. ~.-~~:-!F.... :.: ...1$:1 ~.-.o~ .... :.. 1...1.~:-Q!;i.... :.... :-4.~...... :.... ~..~~:-Q!;i ...... : .... i .. ~~:-Q9.. :.... :I.7..... ..

.. .. !.Q~.49...... :.: .. J..~~:-R9.... :.: ..."? :?~.-.9.1..... : .. , .. ~~:-P9.... :.... :-.4,7...... :.... ~.. ~~:-P9...... : .... ~.. Q~:-P9.. :..... ?. ~..... ..

.. .. J.Q~.47...... \.: .. J..~~:-R!;i.... :.: .. ,4,Q~.-:Q.1 ..... : .. ~.. ~~:-Q!;i .... : .... :-4,? ...... : .... ~..~~:-P9 .. : ... : .... ~.. ~~:-Q9 .. :.... :-.1. ,4.... ..

.: .. !.Q!;i.!!;i9, ..... :.: .. !;i.. J.;:-R?.... :.: .. .1. :E;:i~.-.Q~ .... : .. i .. ~~:-Q~.... : .... :-:4:i$ ...... :.... ~.. ~~:-Q~...... : .... 7.. J'.~:-Q?.. :..... L?..... ..

.. .~1 :-.1.9.~7.... :~: .. *t~~:-R!;i .... :.: .. :4:~~.-.0.1..... : .. :?.-.1.~:-Q4 .... : .. :. :-~ :? ...... :.... f-~~:-Q~ ...... : .... ~..~~:-Q9 .. :.... :-.~, 1..... .

61-1088 :<: 1.1E-05 :<: 1.SE-01 : 7.3E-05 * : -4.1 : 4.2E-05 : 6.3E-06 : -1.8

- -. - - - ---i--- - - - -*- - Pu-242 (Np-237) in Prima in (Key l:s:o~ope. : Co-60)

\.

. . . . . . . . . . . . . . . . . :. . :. ............... :. . :. .....C!='.'": 144 ........ :' ............... :. ............... : .A.Y~t:{19.~ .~9,rt,lj,:-.g: ..Cl'l.lP.41.-!!~~~ .. : .1!>.C? ."<?: .C,rt.lP.*.

$l'lfflP.1~ .~':IITi~.~I'.':.: !~9~P.P.~ .CP.rll?::.: l<.~Y. !~9... CP.F'!Q: :I.S:'? f.~'?'Y. g{l~ja;i: .1'?9. !~9/~!='.Y.: ..... f {IP.t.C?I'.' ...... : .. !~9... CPf!Q: .. : ... f {IP.t.C?I'.' ... .

.. .. !.Q~~~...... : ~: ..

.. l*~:.447'?...... :.: .. 'L.;!:~:-R!:?

?.*~~:-!'.H........ ::.:.:......1.:1 :~~.-t:9.1 ~ ~~ ~

..... : .. .. :-R~ .... : .... -:-~ :O ...... : .... .. ~~:-Re ...... : .... 1.. ?i~:-Ra$ .. :.... , .o :!:? .... ..

1~.-t:9.=? .... :.. J.. ~~:-Q?.... : ... .":-.Et:~...... :.... ~/:~~:-Re...... :.... J..Q~:-Q!:?.. :.... :-.1. :?.... ..

10556 ...... :.: .. J..~~-:-Q~ .... :.: ...~,~~.-+:9.~ .... : .. ...1.~:-Re.... : .... -:-l,9 ... : .. 9.9E-08

. . 5 E 07 * * * ~ * : 3.9E-05 :

. . . . . ............................................... . 3.2

...s, ..fr;s ..... :.: ..... .1 *. :-....... : . : .. .,. ~

~~.-t:P.o .... :.. i.JJ:-R? .... : .... :-~ :9...... :.... .. :5!~:-Q~...... : .... J..:5!~:-Q?.. : .... -:-.'4:7..... .

- - 61 =*iciai ***} **f-:f~::g;* *** 1:1~*:gf *** }!~:§~* *** =!t ***** *;*:;~:ge. ***** }~~:§~* * :f;* *****

1* 1*

1* 1* * *

1* *

1* *

1* * *

No ou~ of spec. nonoonserv .ative oorrel.ations: .are observed

- -. - - - - - - - - -* - -*- - - - Cm-243 (Cm-244) ;n Pdma ;n (Key Isotope : Ce-1 44)

,. \.

................. : . : ........... .'... :.: ....C,~ M4 .... : ............... : ............... : *"Y~t:{l9.~ .E!9jlJjr;i9.:. ,<;jl,lp,41_~,~~ .. : .1~.C! .~,...G:aJP.*.

~:af!'l.P.1.~ N':lroP.~t::.: 1~9~!>P.~ .C!>.f'!Q::.: K~Y.1~9 ... C~>nQ: :l.~C? /.IStY. ,l?{l~j9: .1<?9. !~9/~,.Y.: ..... f ~P.t.qr: ...... : .. !~9; .C!>.l'!Q: .. : ... f ~P.t,qr: ... .

.... !.Q~.4!;>...... :.: .. 7.. rt*Q~ .... :.: .. ,q= 1~.":O~ .... : .. , .. ~~:-Q~ .... : .... :-.4:~ ...... : .... f.~~:-Q't ...... :.... i ..~~:-R~ .. :.... :-.4 .~ ..... .

.. .. !.Q~.49...... :.: .. 9.,l~:-Q't. ... :.: ..."? :4~."":9.1..... :.. '?'.. ~~:-P.f ... :.... :-.~:9...... :.... ~.. ~~:-Q~...... :.... ~.. ~~:-Q'f .. :.... :-.4:9.... ..

.. .. J.Q~.47...... :.: .. iA~:-Q4.... :.: ...~.Q~."":0.1 ..... : .. J.. ~~:-Q~ .... : .... :-.4 .~...... :.... ~..~~:-P.~ ...... :.... '?'..~~:-P.~ .. :.... :-~.?..... .

.. .. !.Q~.~9...... :.: .. i ..l~:-R~.... :.: .. .1.*e~:-:o~ .... :.. U=i~:-P.~.... : .... :-.4,e...... :.... ~.. ~~:-P.4...... :.... ~.. ~~:-P.9.. :.... :-.~.~..... .

. . . ~1 :-.1.9.En ... :.: .. 7.. Q~:-Q~ .... :.: ...4,~~:-:0.1..... : .. ~.. Q~:-Q4 .... : .... :-~:9...... : .... ~.. ~~:-P.~ ...... :.... J...1.~:-Q't .. :..... 1,.!;), *.*...

61-1088 :<: 2.4E-06 :<: 1.5E-01 : 1.6E-05 -4.8 4.6E-04 6.9E-05 : 28.9 No out of spec. nonconserv atin oorre lat ions are observed

- - - - - -*- -*- - - - - Cm-243 (Cm-244) in Primar n (Key Isotope : Co-60)

\.

................. : .: ............... : .: .... .G9:-~9..... : ............... :............... : l~Y.E:17 ~9.E: .~9~.1ja:i9. : . J;~.lP.41.~~~~ .. : .l!>.C! :~~,. .C~.lP.*.

$~.'TlP.1.e: N':lro!:>.e:r::.: !~9~P.P.~ .(;Pf!Q,:. :l:<.E:Y. !~9... CPM, :1.~q l.~~Y. g~~j9: .1<?9. !~9/'.~!?.Y.: ..... f ~P.t.q17 ...... : .. !~9... CP.l'!Q, .. : ... f ~P.t.q17 ... .

10445

- - - - : : 7.1E-05 : : ............

.......... ******** 7.3E+01 ************** : -6.0 :

9.7E-07 .......................................................................

1.9E-06 : 1.4E-04 : 1.9 .

.. .. !.Q,.4'?...... :.: .. '?.*t~:-R4 .... :.:.: .1., 1~.:t:9:4 .... : .. '?.-~~ :-Q~* .... : .... :-.!:? ,:? ...... : .... J.. ~~:-R9 ...... : .... i .. Q~:-Qf.: .... :-.~,4..... .

.. .. J.Q~.47...... :.: .. i .. ~~:-Qf ... : .: ...~.~~.-+:9.~ .... : .. '?.-~~:-Q7.... : .... :-.~,:?...... :.... J.. ?!~:-Q~...... : .... 7.-~~:-Rf.: .....~ .. ?...... .

.. .. l.Q?.~'?.. : ... :.: .. f .. t~:-Q9 .... :.: .. .1.*~~.-+:9.Q .... : .. J.. ~~:-Q~ .... : .... :-.4.~ .. ~ ... : .... J.. ?!~:-Q9...... : .... ~.-~~:-R9.. : .... :-.1 ,9.... ..

61-1087 : : 7 .OE-05 : : 1 .7E+02 : 4.1 E-07 : -6.4 : 1 .9E-06 : 3.2E-04 : 4.6

- - 61 ~-,ass****:<:** 2*.4E:i:ii. ***: *: **i :~i+o"1 ****: **Eii~-i~-~i~d* *: *****rii:;..: *****: ****1*.9E:oi* *****: ****6*.oi:05* *: ****2*5: 1******

See attach.ed explanation

- - ------- ------ - - Cm-:-243 (Cm-244) in Primary Resin ( +.ope : Co-60)-Unmodified Scaling Factor

\

................. : . . .............. : . : .... ~9:-~9..... : ............... : ............... : lw.e.r. ~9.e. .~9i:1.lii:r9. : ..(;ifl.lP.41.~\,,;t .. : .li>.C! X~, .G:,:iJP.*.

$:affl.P. l.e. N':IITIP.e.t:: . !~9tP.P.'? ,<;p.119,: . :l<,e,y. !~9... GPf!<1, :1.:5:'? /.~~Y. -~~ti9: .1'?9. !~9/'>!?.Y. : ..... f 9P.t.C?r: ...... : .. !~9 ... Gpnq, .. : ... f 99.t.C!t: ... .

.. .. J.Q~.4!;5...... : ... 7.-.1k*Qey, ... :.: .. ."? .~~.+.9.1..... : .. ~.. l~:-Q7.... :.... :-~. ,Q ...... : ... .J ...1.~:-Qi;,...... : .... ~...1.~:-Q!;i .. :..... 1..1. .... ..

.. .. LQ1.4'?...... : ... '?.-l~:-R4 .... :.: .. .1. ,1 ~.+.9.4 .... : .. '?.j~:-Q~* .... :.... :-.~,?...... : .... J...1.~:-Qi;,...... : .... J..~~:-Q4.. : .... :-.~,$.... ..

.. .. J.Q~.4?...... : ... ~.-!=:~:-R4 .... :.: .. ~'~~.+.9.4 .... : .. '?.. !=:~:-Q7.... :.... :-~,?...... :... .1...1.~:-Qi;, ...... : .... ":l.. ~~:-Q4 .. : ..... L?..... ..

.. .. J.Q!;:i.q'?...... : ... ~.. lf:*Rey.... :.: .. .1. ,~~.+.9.Q .... : .. , .. ~~:-Q!:;i .... :.... :-.4,e...... :... J .. .1J:-!'.:!9...... :.... ~...1.~-:-!'.:!9 .. :...."'.1 ~--~ ... ..

.. . !=: 1:-.1. 9iF.... : ... 7.-R~-:-Rey .... :.. : ...1. ,7~.+.P.~ ... :: .. 1.. .1.~:-Q7 .... : .... :-~,4 ...... : ... .1 .. .1.~-:-!'.:!9 ...... : ... .1 .. ~~-:-Q4 .. : .....'4 . 7..... ..

61-1088 :< 2.4E-06 3.2E+01 : 7.5E-08 : -7.1 : 1.1E-06 : 3.5E-05 : 14.7

- - - -*- - - - - -*- - - - - - (

Ca-213 CCa-Zffl m P,:iaa.ry Resin fley Isatoge : Co-601 The unmodified S.F. was l.lE-06; however. this resulted in a nonconservative calculated isotopic concentration for samples 10+t6, and 10556; of which only 10556 except 61-1088, the only.sample containing a <LLD value for the isotope, to provide a conservative factor of l.9E-06. *

ML18149A105

Text

* *

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