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{{#Wiki_filter:AMERICANELECTRlCPGN/ERSERYICECORPORATlGN | |||
,DonaldC.Cook,NuclearPlantRADIOLOGICAL'NVIRONMENTAL MONITORING AnnualReport1981'ubmitted byEBERLINEINSTRUMENT CORPORATION MidwestFaciiityWestChicago,Illinois8204020390 820323PDRADOCK05000315RPDRgg2G' (P/~&>>V-~.'I*II*P45I1'IkCi$I4keICI1C''%1lt(7,%%1K IaMtA.tat~~ | |||
DONALDC.COOKNUCLEARPLANTOPERATIONAL ENVIRONMENTAL RADIOLOGICAL SURVEILLANCE PROGRAMAnnualReportJANUARY1-DECEMBER31,1981PreparedforAMERICANELECTRICPOWERSERVICECORPORATION ByEBERLINEINSTRUMENT CORPORATION NUCLEARSERVICESDIVISION-MIDWESTFACILITIES 245WESTROOSEVELT ROADBLDG.2,SUITE9WESTCHICAGO,IL60185asacontractor toAMERICANELECTRICPOWERSERVICECORPORATION Compiledby:KahrynA.hl,AdminstratorWritten,Adbl7CChung-King Liu,P,ManagerFinalDate:03/10/82 | |||
'II).>ya~+P~: | |||
'Vy~i4QQpgp~iyQ+j'lgg~ihq)jap( | |||
W(~wg | |||
~~~~~~IIIIIIIIIIIIIIIIIIIIIIIIIIIIIIII~~~~e~ | ~~~~~~IIIIIIIIIIIIIIIIIIIIIIIIIIIIIIII~~~~e~ | ||
ilC'FFh>PV+PPataiiFFFCollection'Site: | ilC'FFh>PV+PPataiiFFFCollection'Site: | ||
DONALDC.COOKGAMMAEMITTERSINLAKEWATERSAMPLES( | Collection DateOl/10/8102/07/8103/07/8104/04/8105/02/8106/06/8107/04/8108/01/8109/12/8110/10/81ll/07/8112/05/81DONALDC.COOKRADIONUCLIDES inMILKSAMPLES(MonthlyCollections) | ||
Indicator StationsGalienCs-137Ci/l<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10(.)<10<10<10<10<10<10<10<10<10<10<10BridmanK2Stevensville K1<10<10<10<10<10<10<10<10<1010+3<10<10<10<10<10<10<10<10<10<10(a)(a)<10<10BackroundStationsDoMaiacKlSouthBendKli:~>-'V';FF'FVVF.'p4.PWCZcli:F'ei%5tF.,~~(<,+5-hh.5,,/FFF't.,PiiYFQ~k.OtherGammaEmittersCil<10<10<10<10<10<10<10<10<10<10<10<10<10<lo<lo<10<10<10<10<10<10<10<10<10(a)<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<lO<10<10<10(a)(a)<10<ln(a)SeeListingoEMissingSamples.page.Q<'k5+.j DONALD'".C | |||
.COOK'AMMA ISOTOPICANALYSISOFPRECIPITATTON SAMPLES(MonthlyCollections) | |||
Collection Sites:Collection PeriodIndicator | |||
~Ci/1r01/m*BackroundrCi/1.rCS/r*JanuaryFebruaryMarchAprilMay.~JuneJulyAugustSeptember OctoberNovemberDecember<10<10<10<10<10<10<10<10<10<10<10<10<0.4<0.2<0.3<0.4<0.4<0.3<0.3<0.4<0.5<0.5<0.3<0.2<10<10<10<10<10<10<10<10<10<10<10<10<0.4<0.2(a)<0.3<0.3<0.3<0.2<0.2<0.3<0.3<0.3<0.5<0.2RADIOSTRONTIUM CONCENTRATIONS INPRECIPITATION SAMPLES(Semiannual AnalysisonComposites ofMonthlys) | |||
Indicator Ci/1BackroundCi/lCollection PeriodSr-89Sr-90Sr-89Sr-90January-June July-December | |||
<2<2<1<1<2<24+2<1(a)Ru-103=0.4+0.1nCi/ma.45 ee~e~eejII1CgejiAA')~Ici)Collection Site:Collection Date01/23/8105/06/8109/11/81DONALDC.COOKRADIONUCLIDES INWELLWATERSPPPLES(18-weekIntervalCollections) | |||
BackroundStationsONS1ONS2ONS3ONS4ONS7TritiumCi/ml<10.8+0.408+0.4<1<1<1l.2+0.4<1<1<10'+0.40.6+0.41.5+0.41.2+0.41.2+0.4GammaEmittersCi/1<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10'e~','4'Indicator StationsONS5ONS6peg'.1+0.41.1+0.41.0+0.4<11.4+0.41.2+0.4>,i.eeelV,vs(j<10<10<10<10<10<10'"Q,~;f~ffe-[4,' | |||
DONALDC.COOKGAMMAEMITTERSINLAKEWATERSAMPLES(MonthlyComposites ofIndicator andBackground Stations) | |||
GammaEmittersCi/1/nuclide MonthIndicator ComositeBackroundComositeJanuaryFebruaryMarchApril?fayJuneJulyAugustSeptember OctoberNovemberDecember(a)(a)<10<10<10<10'<10<10<10<10<10<10(a)(a)<10<10<10<10<10<10<10<10<10<10i4Iuarter1st2nd3rd4thIndicator Stations200+100400+110<200500+100BackroundStations200+100'20+200 | |||
<200300+200TRITIUMINLAKEWATERSAMPLES(Quarterly Composites ofMonthlySamples)TritiumCi/1RADIONUCLIDES INAQUATICORGANISMS (Semiannual Collections whenAvailable) | |||
LocationCollection DateSr-89Ci/wet')Sr-90Zr-95OtheryONSSONSNOFSSOFSNONSSONSNOFSSOFSN07/23/8107/23/8107/23/8107/23/8109/15/8109/15/8109/15/8109/15/81<0.05<0.05<0.05<0.05<0.05<0.05<0.05<0.050.013+0.005 0.033+0.028 0.024+0.019 0.017+0.013 | |||
<0.005<0.005<0.005<0,0051+1<11+12il<1<1<1<1<1(b)<1<1<1(c)<1<1<1<1(a)SeeListingofHissingSamplespage.(b)Ce-144,Nb-95=lil;Cr-512~1.(c)Ce-144,Nb-952+1;Ce-1411+1.47l'il+l9'I0.Pan%IgsqqI~Pgll'I~,''~'algal".I'' | |||
''''r'I">Pl'0P~IIIllQR>litsuPI@*v)*,I''Ih~i%i,lIPOe9<<Ii~li'LII RADIONUCLIDES INSEDIMENTSAMPLES(Semiannual Collections) | |||
Slf>>gDONALDC.COOKe9:>>')Collection SiteCollection DateCi/dr)GammaEmittersSr-89S>>-90ONSNONSSOFSViOFSS05/19/8105/19/8105/19/8105/19/81<l<1<l<l<0.05<0.05<0.05<0.05<0.0050.013+0.004 | |||
<0.0050.048+0.009 f"-,'i~>>'>>e>>rONSViONSSOFSNOFSS09/21/8109/21/8109/21/8109/21/81<1<1<1<1RADIONUCLIDES INFISHSAMPLES(Semiannual Collections) | |||
<0.05<0.05<0.05<0.05<0.006(a) | |||
<0.005<0.005<0.005Collection SiteCollection DateCi/wet)Se-89GammaEmittersSe-90ONSiVONSSOFSNOFSSONSNONSSOFSNOFSS05/12/81OS/l2/8l05/12/8105/12/8109/23/8109/23/8109/23/8109/23/81<1<l<l<l<1<1<1<1<0,05<0.05<0.05<0.05<0.05<0.05<a.as<0~050.031+0.005 0.032+0.008 0.053+0,012 0.045+0.007 0.043+0.0080.018+0.009 0.030+0.015 0.051~0.017 RADIONUCLIDES INFOODCROPS(AnnualFallHarvestCollection) | |||
Collection Site:Collection SampleDate~e09/30/81Grapes09/30/81LeavesONSiteOFFSiteCi/(wet)GammaEmitters(a)Lowersensitivity duetolowchemicalyield.448 DONALDC.COOKGANfARADIATION (Quarterly3 (Measured UsingThermoluminiscent Dosimeters3 DateAnnealed: | |||
DateRead:12116/8004/07/811st0tr.)iain'ackupTLDTLD03/18/8107/08/812ndOtr.MainBackupTLDTLD06/18/8110/06/813rdOtr.HainBackupTLDTLD09/17/8112/30/814thOtr.MainBackupTLDTLD'I,'l~<LocationIndicator StationsOn-SitelOn-Site2On-Site3On-Site4On-Site5On-Site6On-Site7On-Site8On-Site90.9+0.2missing0.8+0.10.9+O.l0.8+0.20.7+0.10.9+O.l0.8+0.20.8+O.l0.7+0.1missing0.8+0.20.8+O.l0.7+0.10.7+0.10.7+O.l0.9+0.10.7+0.10.7+O.l0.8+O.l0.7+0.10.9+0.11.0+0.2missing0.9+O.l0.8+0.10.8+O.l0.9+O.l0.9+0.10.8+0.20.9+O.l0.9+O.l1.0+0.10.8+0.10.7+0~21.0+O.l1.3+0.21.4+0.11.2+O.l1.0+0.l1.2+O.l1.2+0.11.3+0.11.3+0.11.20.2MeasuredmR/week1.2+0.11.0+0.11.2+0.1missing1.3+0.21.2+0.11.2+0.21.1+0.11.1+O.l1..5+0.21.6+0.21.5+0.41.4+0.41.8+0.5'.6+0.1 1.8+0.41.5+0.21.5+0.21.5+0.61.7+0.11.6+0.31.4+0.41.8+0.81.5+0.52.1+1.51.6+O.E)2.0+0.3Background StationsNewSouthBendDowagiacColoma0.9+0.21.0+O.l0.7+0.10.7+0.10.8+O.l0.9+0.20.8+O.l0.8+0.20.8+0.10.7+0.20.8+O.l0.7+O.l0.9+O.l1.0+O.l0.9+0.20.9+O.l1.1+0.11.0+O.l1.0+0.11.0+O.l1.2+0.11-3+0.10.9+0.10.9+0.11.5+0.1l.7+0.41.5+0.31.5+0.21.6+O.l1.7+0.31.7+0.41.8+0.6Off-Site-1 Off-Site-2 Off-Site-3 Off-Site-4 Off-Site-5 Off-Site-6 Off-Site-7 Off-Site-8 Off-Site9Off-Site-10 0.8+O.l0.8+O.l0.8+O.l0.7+O.l0.8+0.10.7+O.l0.9+0.20.9+O.l0.9+O.l0.9+0.20.9+O.l0.8+O.l0.8+0.3,0.7+O.lEffective 4thQuarter0.9+0.20.8+0.20.7+0.10.8+0.10.9+0.21.0+0.20.9+O.l0.9+0.10.9+0.10.8+0.10.9+0:10.9+O.l0.8+O.l0.8+0.11.1+0.11.0+0.11.8+O.l1.3+0.11.1+0.11.1+O.l1.0+0.2l.0+0.11.0+O.l1.1+0.21.0+0.10'+0.20.9+0.11.0+O.l1.5+0.21.4+0.11.6+0.51.5~0.21.7+0.41.9+0.31.5+0.41.5+0.31.7~0.31.4+0.11.5+0.41.5+0.51.8+0.71.8+0.71.8+0.42.1~1.21.6+0.61.5+0,41.7+0.21.5+0.4 SECTION6QUALITYASSK4QICE DATA50 ENVIRONMENTAL QUALITYCONTROLANALYSESSUMMARY1981'Ihetablesbelowsummarize resultsofsamplesrunforprocessqualitycontrolpurposesduringthcsubjectmonth.Theselistingsareinadd-itiontosuchm<<asuremcnts nsdutcctorbackgrounds, checksourcevalues,radiometric-gravimetric comparisons, systemcalibrations, etc.Detailedlistingsofeachmeasurement aremaintained atthelaboratory andareavailable forinspection ifrequired. | |||
'BLANKSAMPLES.NuclideAnalzedNumbursof. | |||
Determinations Numburofanalysesexceeding theLLDforthatanalsisGrossbetaGrossalphaStrontium-89 Strontium-90 TritiumGammaemitterIodine-131 Calcium-45 46479595616419131*000]*000SPLITSAMPLESNuclideAnnlvz<<.d GrossbetaGrossalphaGammaemittersIodine-131 Strontium-89 Strontium-90 TritiumCalcium-45 UraniumNumberofDet'ns14239126-146384489871No.agreeingwith'I.n2a13838122146384289871SPIKEDSAMPLESNo.agreeingwithin3a414002000No.differing bv>3a000000000NuclideAnalzed'rossbetaGammaemittersIodine-131 Strontium-89 Strontium-90 TritiumNo.ofDes'es5544ll189445Within2aof'nown534311189344Within3aofknown110011differing fromknownb>3a1*00000*Corrective actionsweretakentoeliminate theproblem.51 EPAINTERCOMPARISON 1981~~~I~hu~~~~~~I1~1~I~I~I~~~2~~~~~!iRESULTSpage1of3'onth/Yea rDecember1980D<<cember1980December1980December1980Decembex'980 D<<cumber1980,1anuary1981January1981January1981January1981January1981January1981January1981January1981January1981January19811'<<brunry1981F<<bruary1981Februax'y 1981February19811:obruary 1981February1981February1981Mareh1981M;ix'c1<1981March1981March1981'larch1981March1981April1981April1981April1981April1981April1981April1981April1981Apx'il1981Hay1981May1981May1981Yiay198lMay1981i~1Qy1981SampleTe1aterWaterAirFilterAizFilterAirFilterAirF11c<<tWaterWaterHaterWaterMilkMilkMilkMilkMilkN.lkWaterWaterWaterWatezWacerWaterWaterHaterWaterAirFilterAirFilterAirFilterAirFilterWaterWaterWaterWaterWaterWaterWaterWaterWaterWaterWaterWaterWater'HaterAnalsisIodine-131 TH.tiumGrossAlphaGrossBetaStrontium-90 C<<siuu<-137 GrossAlphaGrossBetaStrontium-89 Strontium-90 Strontium-89 Strontium-90 Iodine-131 Cesium-137 Barium-140 Potassium TritiumChromium-51 Cobalt<<60Zinc-65Ruthenium-106 Cesium-134 Cesium-137 GrossBetaGrossAlphaGrossAlphaGrossSetaStrontium-90 Cesium-137 TritiumCesium-134 Cesium-137 Strontium-89 Strontium-90 Radium-226 Radium-228 UraniumStrontium-89 Strontium-90 Strontium-89 Strontium-90 Iodine-131 Cesium-137 AgencyValuu22224021190199441634020.225.843.501551176002585036425253050181427101015382815.012.0123622ControlLimitsQ3nn3)66049;18.708.78.78.78.72.902.610.48.7013459008.78.708.78.78.710.4138.72.68.76158.78.78.72.64.03.1108.72.6MWFMeasuredx2oerror*17+22600+30021228~3LT119+210~143+4LT535+4LT214+129+347~5LT251350+1401680170LT10029+592+9LT10029+59327+320+230+366+717+415+23000+3007+213135+724313.2~1.310+26+229+326+3UnicspCi/liter pCi/liter pCi/filter pCi/filter pCi/filter oCi/Cilc<<r pCi/litez pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/literpCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter | |||
'Ci/liter pCi/lit<<r pCi/filter pCi/filter pCi/filtex pCi/filter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter | |||
*Whenanalysesofaparticular typeresultinconcentrations belowthedetection limits,theterm"LT"isusedtoindicate"LessThan"valuesforthatmeasurement. | |||
basedon3a(99.5%)confidence level.~~~~"ieiqqp e~-EPAINTERCOMPARXSON RESULTS1981Page2"of3.>>.5Month/Year 198119811981198119811981198.1198119811981198119811981198119811981198119811981198119811981198119811981198119811981198119811981MayaMayJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJulyJulyJulyJulyJulylylyulyJulyJulyJulyJulyAugusthu>>ustAugustSeptember September September September September September'eptember September September September September | |||
~1981198119811981198119811981198119811981SampleTeMaterWaterWaterMaterWaterWaterWater'aterWaterWaterMaterAirfilterAirfilterAirfilterAirfilterFoodFoodFoodFoodFoodPoodMilkMilkMilkMilkMilkMilkWaterWaterWaterMaterWaterUrineMaterWater.WaterWaterAirfilterAirfilterAirfilterAirfilterAnalsisBarium-140 Potassium Chromium-51 Cobalt-60 Zinc-65Ruthenium-106 Cesium-134 Cesium-137 TritiumRadium-226 Radium-228 GrossalphaGrossbetaStrontium-90 Cesium-137 Strontium-89 Strontium'-90 Iodine-131 Cesium-137 Barium-140 Potassium Strontium-89 Strontium-90 Iodine-131 Cesium-137 Barium-140 Potassium Iodine-131 TritiumUraniumStrontium-89 Strontium-90 TritiumRadium-226 Radium-228 GrossalphaGrossbetaGrossalphaGrossbetaStrontium-90 Cesium-137 AgencyValue01559017015213119506.78.02854191644318245026402517031016002326302323ll20508.311.7332825521619ControlLimits~3eu)013508.708.78.78.75961.72.1128.72.68.'78.72.8148.702298.72.608.7013913613108.72.65992.23.048.7118.72.68.7MWFMeasured~7oerrorLT20)400+140LT2016+2LT2013+413+225+32300+2005.9~0.410.6i).631674+821+515+238+428+375+840~4<252267i22713+316+3<535+12<161463+30553+11297387814+218+514+22166+6248.4+0.84..6+3a7'"32+1430+625+671+718+220+2UnitspCi/liter mg/literpCi/liter pCi/liter | |||
~pCi/liter | |||
-.pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/filter pCi/filter pCi/filter pCi/filter pCi/kilogram pCi/kilogram pCi/kilogram pCi/kilogra~ | |||
pCi/kilogram mg/kilogram pCi/li.terpCi/liter pCi/literpCi/liter pCi/liter mg/literpCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/~terpCi/liter pCi/liter pCi/filter PCi/filter PCi/filter pCi/filter | |||
;53ps~~~~g<e<<~v<<,was>>q,.-r>>a<>>e<aaea>> | |||
'<<ae<.<<<<We<et<'ee'<<e<V.e EPAINTERCOMPAPiXSON RESULTS1981Month/Year SampleTeAnalsisAgencyValueControlLimits~3eu)MWFMeasured+7oerrorUnitsOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberNovemberNovemberNovemberNovemberNovemberNovemberDecember198119811981193119811981193119811981198119811981198119811981,19811981198119811981198119811981WaterWaterWaterWaterWaterWater'WaterWaterWaterWaterliilkMilkMilkHi,lkMilkMilkFoodFoodFoodFoodFoodPoodWaterGrossalphaGrossbeta.Cobalt-60 Strontium-89 Strontium-90 Cesium-134 Cesium-137 Radium-226 Radium-228 CrossUraniumStrontium-89 Strontium-90 Iodine-131 Cesium-137 Barium-140 Potassium Strontium-89 Strontium-90 Cobalt-60 Cesium-137 Barium-140 Potassium Tritium809602114.4121512.79.215231852250153038233033027302700358.708.72.62.68.73.32.4108.72.6108.701338.72.68.78.7023661591+2611211LT513+614.6+2.014+220+1411.8~3.58.3+5.19+224+814+558ll.29+9LT161700+24041+621+535+832+8LT312700+2702950+127pCi/liter pCi/li,ter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/literoCi/liter pCi/liter pCi/liter pCi/liter mg/literpCi/kilogram pCi/kilogram pCi/kilogram pCi/kilogram pCi/kilogram mg/kilogram pCi/liter 54 EPAINTZRCOMPARLSON RESULTSp$<X<j1981(LabPerformance Evaluation Study-EHSL-LV) | |||
SampleAgencyControlLimits~(3an]MMPMeasured2eerrorUnitsg~:WaterWaterWaterWaterWaterWater,WaterMaterWaterWaterWaterGrossalpha39Grossbeta60Cobalt-60 12Cesium-134 12Cesium-137 20Ruthenium-106 0Zinc-650Strontium-89 6Strontium-90 0Radium-226 12.8Uranium5101.839+470+7LT2011+220+2LT100LT20LT112.6+1.34+2pCi/liter pCi/liter | |||
.,pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/1'[ter pCi/liter 55 1981SampleTe,Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)0.244E+040.117E+030.450E+020.630E+010.122E+030.139E+040.190E+040.223E+Ol0.2470.015E+040.0930.006E+030.5150:087E+02(0.100E+020.8280.048.E+020.1330.006E+040.133+0.007EM40.750+0.053 E+01Be-7Mn-54Sr-89Sr.-90Zr-95Sb-125Cs-134Ur.~I,I'~~r~r.r~USDOEUALITYASSESSMENT PROGRAMMeasuredNuclideKnown~2aerror"lUnitspCi/filter pci/filter pCi/filter pCi/filter pCi/filt'er pCi/filter pci/filter pCi/filter P;'I'trSoil(81-04)Soil(81-04)Soil(81-04)Tissue(81-04)Tissue(81-04)Tissue(81-04)Tissue(81-04)K-40Sr-90Ra-226U0.158E+010.240E+Ol0.450E+000.290E-OLK-400.213E+02Cs<<1370.200E+00Ra-2260.770E+000,290+0,017 K+020.250+0.070 E+000.668+0.057 E+000.433+0.058 E+Ol0.188+0.016 E+010.433+0.058 E+000.850+0.333 E-01pci/gpci/gpCi/gpci/gpci/gpCi/gpCi/g~'I~i~IVegetation (81-04)Vegetation (81-04)Vegetation (81-04)Vegetation (81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)K-40Sr-90Cs-137UH-3Co-57Co-60Sr-90Cs-137Ce-141UU0,224E+030.560E+010.230E+000.310E+000.246E+020.118E+010.129E+010.440E-010.137E+010.527E+010.145E-010.102E-010.277+0.018 E+030.258+0.016 E+Ol0.200+0.058 E+000.133+0.058 E+000.197+0,012 E+020.243+0.018 E+Ol0.133+0.006 E+010.405i0.063 E-010.150+0.012 E+010.193~0.012 E+010.200+0.026 E-Ol0.?50+0.140 E-02pci/gpci/gPCi/gpCi/gpCi/mlpCi/mlpCi/mlpci/mlpCi/mlpCi/mlug/mlpCi/ml TLDIntezcomparison BadgesIrradi.ated byBattelleNorthwest'. | |||
LabsTotalmRlesstransortationcontrol1sttr2ndtr3rdtr4thtrMeasuredIH.O18.54.126.029.1+2'2<).I+6.I 18.017.85aO24.024.5+5.538.034.1+9.057.042.16.059.061.4i6.569.077.612.569.071.219.047.046.85'44.043.2+6.020.025.54.890.086.2-15.5 28.031.4~2.551.053.65.316.017.9+2.7100.093.4~10.1 32.036.5+3.542.041.9~19.7 40.041.24.018.020.1+3.453.055.4~15.2 29.032.0-3.076.065.66.673.074.1~21.6 69.075.1~13.2 34.032.0~3.088.088.6+12.6 79.080,8+17.3 82,080.4+10.7 82.079.0+8.0I00.0I00.0I02+I099+1079.079.9+18.2 99.0100.2i25.4 93.0100.086.1+15.534.038.7~9.3100.4~15.374.069.2~8.857 | |||
'.JJl)."0,g~,lp44',"!'r.3l",j~l(ACliJP,'Il'~%PAL+'th,Wll.JI9(%pfH\8,gW4q".)ApAp~~)t}} | '.JJl)."0,g~,lp44',"!'r.3l",j~l(ACliJP,'Il'~%PAL+'th,Wll.JI9(%pfH\8,gW4q".)ApAp~~)t}} |
Revision as of 10:00, 29 June 2018
ML17319B255 | |
Person / Time | |
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Site: | Cook ![]() |
Issue date: | 12/31/1981 |
From: | KOHL K A, LIU C K INDIANA MICHIGAN POWER CO. (FORMERLY INDIANA & MICHIG |
To: | |
Shared Package | |
ML17319B254 | List: |
References | |
NUDOCS 8204020390 | |
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,DonaldC.Cook,NuclearPlantRADIOLOGICAL'NVIRONMENTAL MONITORING AnnualReport1981'ubmitted byEBERLINEINSTRUMENT CORPORATION MidwestFaciiityWestChicago,Illinois8204020390 820323PDRADOCK05000315RPDRgg2G' (P/~&>>V-~.'I*II*P45I1'IkCi$I4keICI1C%1lt(7,%%1K IaMtA.tat~~
DONALDC.COOKNUCLEARPLANTOPERATIONAL ENVIRONMENTAL RADIOLOGICAL SURVEILLANCE PROGRAMAnnualReportJANUARY1-DECEMBER31,1981PreparedforAMERICANELECTRICPOWERSERVICECORPORATION ByEBERLINEINSTRUMENT CORPORATION NUCLEARSERVICESDIVISION-MIDWESTFACILITIES 245WESTROOSEVELT ROADBLDG.2,SUITE9WESTCHICAGO,IL60185asacontractor toAMERICANELECTRICPOWERSERVICECORPORATION Compiledby:KahrynA.hl,AdminstratorWritten,Adbl7CChung-King Liu,P,ManagerFinalDate:03/10/82
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SECTlON1PREFACE ABSTRACTThisreportpresentsthedataobtainedfromtheanalysesofenvironmental samplescollected fortheAmericanElectricPowerServiceCorporation DonaldC.CookNuclearStationEnvironmental Radiological Surveillance Programfortheperiod01January1981through31December1981.Theactivitypresentabovethedetection limitsintheroutinely collected samplemediawasobservedtobeofnaturalandatmospheric origin.Theresultsshowthattheradiation dosetoamemberofthegeneralpopulation didnotexceedthetechnical specifications of1Xofthe10CFR20limitduring1981.
INTRODUCTION TheDonaldC.CookNuclearStationofAmericanElectricPowerServiceCorporation consistsoftwoWestinghouse PWRunits(Unit1andUnit2).Eachunitconsistsofapressurized waterreactor(PWR)whichgenerates about3250megawatts (MW)ofheattogenerateabout1100MMofelectricity.
ThestationislocatedinBentonHarbor,Mich-igan.TheD.C.CookPlantutilizesapressurized waterreactorwitharadwastehold-upandtreatment systemthathasbeendesignedtokeepcdradioactive releasestoaslowasispractblelevels.However,smallquantities ofnoblegasesandradioiodine maybereleasedtoLakeMich-igan.Thequantities ofradionuclides releasedtotheenvironment areexpectedtobeminiscule andinsignificant asasourceofpotential exposuretofloraandfaunainthearea.However,directradiation ex-posuretomanandradionuclide accumulations invariouscomponents offoodchainstomanwillbecarefully monitored.
Theenvironmental radiologicaLmanitoring programisintendedtoservethefollowing purposes:
a)Toyield'averagevaluesofradiation levelsandconcentrations ofradioactive materialinvariousmediaoftheenvironment.
b)Toidentifysamplelocations and/ortypesofsamplesthatdeviatefromtheaverages.
c)Todocumentseasonalvariations thatcouldbeerroneously interpreted whenthepowerstationisoperating.
d)Toindicatetherangeofvaluesthatshouldbeconsidered "background" forvarioustypesofsamples.
ThebasicapproachfortheDonaldC.CookNuclearPlantistocon-trolthereleaseofradioactive materialatlevel'sfarbelowthatwhichwouldbeexpectedtocausedetrimental impactontheenvironment.
Theenvironmental radioactivity surveillance programwillbecloselycoord-inatedwithconditions ofplantoperation andsubjecttoperiodicreview.Levelsofenvironmental radioactivity aresubjecttochangeforreasonsinnowayrelatedtotheoperation oftheD.C.CookNuclearPlant.Therefore, theradioactivity surveillance programhasbeende-signedtoincludereference or"background" stationsaswellas"indicator" stations.
Theprogramissunznarired inTableI.Thisreportcontainsacompilation oftheresultsofanalysesofvarioustypesofsamplescollected duringtheperiodJanuary1981throughDecember1981.~'"'
SUMMARYEnvironmental monitoring resultsshowedthattheradiation dosetoamemberofthegeneralpopulation didnotexceedTehcnical Specifications of1Xofthe10CFR20limitduringduring1981.Theactivitypresentabovethedetection limitsintheroutinely collected samplemediawasobservedtobeofnaturalandatmospheric falloutorigin.Table3summarizes therangeandaverageconcentrations formeasurements attheindicator andcontrollocations, andthelocationwiththehighestannualmean.Completeinformation isgivenintheSampleDataTables(Section5).),4I+~O0,9t,low,~W0+,I9%1g'>0't'"(>>'t,.'g1'%'v,,~',s~~""',~~pleC,seg>>s1~'"r<<,(dye SECTION2SPZPLINGPROGRAM Allsamples'are collected byEberlinepersonnel andshippedtotheEberlinelaboratory inWestChicago,Illinois.
Thesamplecollection procedures remainedthesameasthosedetailedinthesemi-annual reportfortheperiod01Januarythrough30June1973.Uponreceiptofthesamples,thelaboratory staffentersthesamplesinalogbookidentifying themastosampletype,collection date,andsamplecodenumberoflocation, thenverifiesthespecificanalysestobeperformed oneachsample.Thesamplesarethenstored,awaitinganalysis, onshelvesexpressly forthispurposetoassureaccountability throughthelaboratory processes.
Table1liststhesamplinglocations andfrequencies.
FiguresI,II,andIIIshowthelocations ofthevarioussamplingenvirons.
Ieat~wTable1liststhesampleanalysisprogram-sampletype,frequency, andthetypeofanalysisrequired.
Table2liststheLLD's(LowerLimitsofDetection) fortheanalytical program.TheseLLD'sarebasedontheRegulatory Guide4.8.ForanalysesnotlistedinRegulatory Guide4.8,FederalEPA,formerrequirements forsimilarprogramsorotherappropriate guidesareused.TheLLD'sarecalculated atthe3o(99/confidence) level.TheGuidespecifically statesthattheLDL'areapriori,notafosterlori (after'he fact)limitforaparticular measurement Whenhowever,RG4.8orotherLLD'shavenotbeenachieved, afootnotegivingabriefexplanation hasbeeninserted.
~4~4~PI(AlltI64IIdLPC~eiCe@gTABLE1ENVIRONMENTAL MONITORING PROGRAMDONALDC.COOKNUCLEARPLANTLCp~SampleTeNo.Station.Ind.-Bk.Collection FreuencAnalysisFreuencTypeAnalsisRemarksJCJ'Cpp'IAirParticulate 64AirborneI-131Precipitation LakeWaterWeeklyWeeklyMonthlyMonthlyWeeklyMonthlyQuarterly WeeklyMonthlySemi-annual MonthlyGrossBetaGammaIsotopicComposite, 2SamplesSr-89,Sr-90GammaIsotopicGaamaIsotopicComposite, 2SamplesSr-89,Sr-90Composite, 2SamplesGammaIsotopicComposite, 2SamplesByindicator andbackground samples.Byindicator andbackground samples.Byindicator andbackground samples.Byindicator andbackground samples.P.LWellWaterQuarterly Every18wks.Every18wks.TritiumComposite, 2SamplesGanmaIsotopicTritiumByindicator andbackground samples.jPQPjrJFish2peryear2peryearGammaIsotopicSr-89,Sr-90Edibleportiononly.
DONALDC.COOKNUCLEARPLANTSampleTeNo.StationsInd.-BkTypeAnalsisAquaticOrganisms 222peryearWhenavailable MilkMonthlySediment2xperyearQuarterly TotalDoseTLDFoodCropsAnnuallyGammaIsotopic~~~TABLEl(Cont'd)ENVIRONMENTAL MONITORING PROGRAMCollection AnalysisRemarksl'-"2peryearGammaIsotopicSr-89,Sr-9032MonthlyGammaIsotopicSr-89,Sr-90I-131222xperyearGammaIsotopic'4ÃSr-89,Sr-90914Quarterly f".",.'c'5-lIAnnuallyg-.'c'~'46ljggf;g(7j4:~';gKt'~t4'~
2ISamoleClassTable2LOWERLIMITSOFDETECTION (LLD's)LEDAnalsisUnitsAirParticulates AirborneIodineMilkWellWaterPrecipitation LakeWaterAquaticOrganisms GrossB'etaGammaIsotopicSr-89Sr-90I-131I-131GammaIsotopicSr-89Sr-90LSTritiumGammaIsotopicGammaIsotopicSr-89Sr-90GammaIsotopicEnrichedTritiumGammaIsotopicSr-89Sr-900.010.010.0020.0010.010.0510511000101021100.210.050.005pci/mspCi/mspCi/mspCi/mspci/mspCi/lpCi/lpCi/1pC1/1pCi/1.pCi/1pCi/1pCi/lpCi/1pCi/lpCi/mlpCi/gwetpCi/gwetpCi/gwetjSedimentFishFoodCropsBackground Radiation (TLD)GammaIsotopicSr-89Sr-90GammaIsotopicSr-89Sr-90GammaIsotopicGammaDose10.050.00510.050.005pCi/gdrypCi/gdrypCi/gdrypCi/gwetpCi/gwetpci/gwetpCi/gwetmR/week TRUEPLANTNORTHNORTHWlMETEOROLOGICAL TOWERPROPERTYLINEL3TO7T2ROADSW2-eR.R.TRACKLlLT08545KVYARDSHORELINE~E-WPLANTQTO94ATQ>765KVMYARDCHESAPEAKE 6OHIOR.R.T6W72,000FOOTRADIUSINTERSTATE 94SCALE0l,0002,0003,0004,000FEETFIGUREILOCATIONS OFINDICATOR AIRSAMPLINGSTATIONSA'ir,Precipitation TTLDStationWWellMaterLLakeWater(takenatshoreline)
A-AIr,Preclpitatlon, TLDStationsL-LakeMaterSampleStationsHNIlkSanyleStations2DMILES~1196MateI94BEHTOHHARBORLST~JOSEPHM51Stevensvk I~DoC.COOKPLAHTBRdna3EauIalreberrlenSpringsM51HewBuffaloHICHIGAHCITTI94MICHIGAN176KQiANeoCarlIsle%IlesUFO8ScaleofHIles102Ol'IGUREIT.OFFSITSLOCATIOXS OFSAIC.IXGSTATIONS13 44IoVI,<varv44~)lzSCO~0/IwI~aarv3~arCao4LCll4090.LEio149I,4q~~LEl545C444llLUCV,a:~I)44a.l~aaccJLUIII.I~'CalvaavLUCra~4ooaaro~l5S0D20'alaIrI~~I~~I~I3892OL~~.YtOQDVa99/209~mr444I-.'4/4r-~-3l3aaocrara242NC".,344444rrVV<<Va235~IN:~alar3oR'0Y3I29AL32LI44928274~,I'Qc(N0N33AHOYI5r?"'33LI644C'4JKRI0~\~\'I\~4rarl)599I0I~9oI2~V~\o559IL+HINCHIciAN 9jjI0II41VI164jfBAROOAisrlaaaLLCvavCP3I.~IgLQlLCVCUII~455l3"IS1194/Ilr0R"0Ni0K:"l7l6gl5o444943vVtt444a)Irav3302I~22I23j2435'aaaaVL~2I~i9elV20!i2Il22)5~zg9,)1vc44'42'86SNO'WIR"Of52~0A.30CVOVdV27I(3rI~442253LIavIItacarv3322536~IVX3I/PaallmraIL3i3834~~Io-i.<<z-'~ICULVO4831'il2.3."5.6;7.'8.9.10.TLDMONITORLOCATIONS LOCATEDONTHEFIVEMILERADIUSFROMTHEPLANTRedArrowHighwayandvicinity'ofI-94overpass.
Stevensville SubStation.Washington AvenuemidwaybetweenBrentwood DriveandKingmanDrive.Washington AvenueandLincoRoad.FIGUREIIICleveland Avenue.andShawneeRoad.Holden'Road andSnowRoad.BridgmanSubStation.California RoadbetweenBrowntown andSnowRoads.RugglesRoadbetweenHinchmanandLemonCreekRoads.Atintersection ofHildebrant RoadandRedArrow.Highway.
14IIC+9<v~/4rl441~.~4LL444w/II'~,roIrrvr44rarrv44I44~%4r.,~444 SECTION3ANALYSISPROGRAM15 Samplesreceivedatthelaboratory areanalyzedforthevariousradio-equalto,andinmostcases,identical with,thoseoftheU.S.D.O.E.
orBriefdescriptions ofanalytical procedures areavailable intheLab-radioanalytical contractor's laboratory.
GrossBeta-Exposedairparticulate filtersarecounted'inlowback-background suppression aftertheshort-lived naturally occurring radonandthorondaughters havedecayed.Filtersarecountedlongenoughto-'"~mc4(>'5p',1~ANALYTICAL PROCEDURES ijCactivecomponents bystandardradiochemical methods.Thesemethodsare'1+thoseoftheFederalE.P.A.oratoryProcedures Manualavailable attheCookNuclearPlantandthe&AIRPARTICULATE FILTERS'groundGeigerorproportional flowbetacountersusinganti-coincidence e'jjfl1tgif1~'nsurethattherequiredsensitivity (LLD)ismet.GammaIsotoic-Monthlycomposites ofairparticulate filtersgroupedbyindicator andbackground stationsintotwosamplesarecountedinhighresolution (GeLi)gammaspectrometers forperiodsoftimelongenoughtoensurethattherequiredprogramsensitivity (LLD)ismet.Strontium-89 andStrontium-90
-Aftercarrierstrontium isaddedtosemiannual composite samplesofairparticulate filters,thestrontium "l\ilI~isthenseparated andpurifiedbyeitherionexchangechromatography (EPAmethod)orstraightwetchemistry (HASLmethod).Thechemical1HASLProcedures Manual,editedbyJohnH.Harley,HealthandSafetyLaboratory, USAtomicEnergyCommission, 1972edition,revisedannually.
'5"52National Environmental ResearchCenter,Environmental Protection Agency;HandbookofRadiochemical Analytical Methods.ProgramElement1HA325.OfficeofResearchandDevelopment, LasVegas,Nevada89114.16~>>\5(III'55IPt~'I'lI,9$59~P\51%hhI~~\I~5t~%5~I11w~e~WI.1II~5,~'~~l wyieldforstrontium isdetermined.
by'atomic, absorbtfan'pectrometry orgravimetric methods.Afterasuitableperiod(usually14days)toallowforingrowthofY-90,thesamplei'scountedinalowbackground betacounter(equilibrium ortotalSrcount).Thestrontium isnextputintosolution, carrieryttriumadded,andthestrontium andyttriumfractions separated.
TheyttriumiscountedandfromtheY-,90(Sr-90daughter) count,theSr-90concentration canbedetermined.
Thedifference betweenthetotalstrontium concentration asdetermined bytheequilibrium countandtheSr-90concentration asdetermined fromtheY-90countistheSr-89concentration.
Equations areavail-abletopermitcalculation ofSr-89andSr-90bycountingthepurifiedstrontium fractionattwopointsduringingrowthoftheSr-90daughterY-90.Whileeithermethodisacceptable, wefindtheformermethodprovidesmoreconsistent results.WATERSAMPLES(Includes Lake,Well,Precipitation)
GammaIsotoic-Ameasuredaliquotofthesampleisevaporated toasmallcontrolled volumeandcountedinastandardgeometryinahighresolution (GeLi)gammaspectrometer longenoughtoensuremeetingthesensitivity requirements oftheprogram.SeealsotheIntro-ductiontoDataTables.Strontium-89 andStrontium-90
-Stablestrontium carrierisaddedtoameasuredaliquotofsample.Thestrontium isthentreatedfromthispointoninthesamemannerasareairparticulate samples.Tritium-Tri.tiumastritiated waterisanalyzedbyliquidscintil-lationcountingafterdistillation.
Ifhighsensitivity isnotrequired(ie.LLD-500pCi/1)thesampleisdistilled, mixedwiththeappropriate countingphosphors andcountedwithnofurther17 treatment.
Ifhighersensitivity isrequired(ie.<-300pCi/1)thesampleisisotopically enrichedintritiumconcentration priortoliquidscintillation counting.
Isotopicenrichment isdonebytheclassical methodofOstlundwhichinvolvesalkalineelectrolysis ofapurifiedaliquotofsampleundercontrolled conditions oftemper-atureandelectrode currentdensity.MILXSAMPLESI-131-Measuredamountsofcarrieriodideareaddedtoaknownvolumeofmilkandtheiodineextracted onanionexchangeresin.Theiodineisrecovered andpurifiedbyclassical iodinechemistry methodswhicharesimilartothosegiveninformerRegulatory Guide4.3.Theyieldorrecoveryofiodineismeasuredgravimetrically andtheprecipitated sampleismountedandcountedinalowlevelbetadetectorforalongenoughperiodtoensurethattherequiredLLDismet.GammaIsotoic-Ameasuredaliquotofsampleisevaporated andoven-driedtoastandardvolumeandcountedinafixedgeometryinahighresolution (GeLi)gammaspectrometer foralongenoughperiodtoensurethattherequiredLLDsarereached(seealsoIntroduction toDataTables).Strontium-89 andStrontium-90
-Stablestrontium carrierisaddedtoanaliquotofthesamplewhichisthendriedandashedathightem-perature()700c).Theashisdissolved andthesolutiontreated0fromthispointoninthesamemannerasareairparticulate samples.ORGANICSPZPLES(AquaticOrganisms, FoodCrops,Fish)asappropriate, placedinacontrolled geometryandcountedinahigh18 resolution (GeLi)gammaspectrometer fora.periodlong-enough-toen-surethattheLLDsoftheprogramwillbeset(seealsoIntroduction toDataTables).Strontium-89 andStrontium-90
-Stablestrontium carrierisaddedtoaweighedaliquotofthesampleandthesampleisashedathightem-perature(>700c).Theashedsampleisthendissolved andprocessed 0inthesamemannerasareairparticulate samples.SEDIMENTSAtiPLESthensievedtoremovepiecesofstoneand/orotherlargepiecesofmaterial.
Anappropriate sized,weighedaliquotofthesampleisthentransferred intoastandardgeometrycontainer andcountedfor'aperiodlongenoughtoensurethattheLLDsoftheprogramwillbe.met.(SeealsoIntroduction toDataTables.)Strontium-89 andStrontium-90
-Asampleisasheduntilfreeofcarbon.Theash,withcarriersadded,isdissolved inhydrochloric acid,thenprocessed inthesame'anner asareairparticulate samples.THERMOLUMINISCENT DOSIMETERS Environmental radiation dosesaremeasuredusingbadgescomprizing fivechipssealedinplasticprotective holdershavingadensityof50mg/cm.TheTLDchipsare1/8"x1/8"x1/32LiE(thallium activated) knowncommercially asHarshaw-100.
Thechipsareallselectedtopro-videuniformresponsetowithin,fivepercentofthemeanforthebatch.jPriortoinstallation, thechipsareannealedbyastandardcycleof60minutesat400candimmediate coolingtoambienttemperature byplac-0ingthetraycontaining theannealedchipsonanaluminumblock19sttI($%tPI\ll~4T'Ilt~~Fv~~rtl 12"x12"x1".AfterexposurethechipsarereadonanEberlineinstrument Corporation ModelTLR-6reader.Thesystememploysapreheatcyclewhichremoveslowtemperature peaksandintegrates anddigitizes onlythelightoutputinaselectedtemperature range.Thedoseiscalculated fromtheaveragelightoutputforthefivechipsandthestatistical uncertainty isthestandarddeviation ofthefivereadings.
Controlbadgesareusedtodetectanyunusualexposuretothebadgewhichmightoccurduringshipment.
20 QUAL'ITYASSURANCE'ROGRAM A.DesignofPlanQualityofproductorservicehasalwaysbeenaprimarykeytoin-creaseissales,customersatisfaction, andprofit.Themanagement ofEberlineInstrument Corporation recognizes theeverincreasing demandforhigherqualityandreliability forservicesrelatedtoprotection ofworkersandtheenvironment.
Itisourfirmbeliefthatinordertojudgetheworthofasupportservice,onemustknowthephilosophy behindit.Eber-linewillprovideonlythoseservicesforwhichitisqualified andthesewillbeprovidedinamannerthatisreliable, withaqualityassurance programthatmaintains ahighdegreeofclientconfidence.
Thisqualityassurance programhasbeenpreparedconsistent withthefollowing specifications, pertheTechnical andQualityAssurance Requirements forSpecialPurposes.
ANSI-N4S.2, AmericanNationalStandards Institute NRCBranchTechnical PositionofNovember1979NRCRegulatory Guide4.15,Revision1ofFebruary1979.B.Intercomparison ProgramResultsofEberline's Midwestern Facilityparticipation intheUSEPA'sCrosscheck Programwillbeincludedinthemonthlyreportsprovidedtotheclient.Otherintercomparisons inwhichweroutinely participate include:Environmental Protection AgencyEnvironmental Measurement LabDOEQualityAssessment ProgramBattelleNorthwest Laboratories IAEAAnalytical QualityControlServiceUSNationalBureauofStandards Eberline's Albuquerque Laboratory.
Eachofthelaboratory managersisresponsible forpreparing spikesandblankstoberunroutinely.
Everytenthsampleisaspike,ablank,orasplitsample.RegularQCreportsarepreparedbythelaborarymanageronamonthly21 scheduleandforwarded toeachclient.Eachreport'outinely includes:
resultsfromEICinterlaboratory comparison, resultsfromEPACrosscheck program,andresultsfromotherintercomparison programs.
Resultsarereviewedbythelaboratory manager.Ifaproblemisin-dicatedbythedata,thenatureoftheproblemisinvestigated andcorrective stepstakenimmediately.
AcopyofeachreportisalsoprovidedtotheQualityAssurance ManageroftheNuclearServicesDivision.
C.QualityAssurance PlanTheQualityAssurance Programfollowstherequirments ofCompanyandDivisionManuals.Thediscussion belo~outlinesQualityAssurance Programsasconducted inthelaboratory andasrequiredinourQAManual.Procedure AroyalEachprocedure goesthroughavigorousevaluation andreviewprocessbeforeitisincorporated intotheEICProcedures Manual.Established pro-ceduresoftheEnvironmental Protection Agency(EPA)ortheEnvironmental Measurements Laboratory oftheUSDepartment ofEnergy(EML)areusedunlessthoroughtestinghasdemonstrated thatanalternate procedure isequaltoorbetterthantheEPAorEHLprocedure.
Uniformprocedures areusedatbothlaboratories tothefullestextentpossible, exceptwhendeviations arenecessary tomeetthespecificrequirements oftheclient.Themanagerofeachlaboratory andthequalityassurance managerreviewandapprovesignif-icantprocedural changesbeforetheyareimplemented.
EuimentCalibration andMaintenance Equipment usedforquhlitative orquantitative measurements iscare-fullycalibrated andmaintained withrecordsofeachcalibration ormain-tenanceactionkeptinappropriate logbooks.
Totheextentpossible, certified standards areusedforallprimarycalibrations.
Thefollowing standards areusedfortheapplication indicated:
22 Measurement GrossBetaTritiumCalibration StandardSolutionofStandardCscertified byNBSor137AmershamSearleSolutionstandardofHcertified byNBS3GammaSpectrometry Strontium-89 and90GrossAlphaRadiation DoseSolutionstandards ofvariousgammaemitterscertified byNBSorAmershamSearle.Standards areusedtocalibrate eachcountinggeometryused.Solutionstandards ofSrcertified byAmersham90SearleorNBSSolutionstandards ofPucertified byNBSor239AmershamSearle.137Csgammasourcecross-referenced withNBSusingR-meters.
Raisusedforsomespecialapplication.
Whensuitablestandards arenotavailable foraspecificgammaemitter,quantitative gammaisotopicanalysisisbasedonanenergycalibration ofthegammaspectrometer andthegammaenergyandabundance information providedinTableofZsotopes, SixthEditionbyLeds'er,Hollander, andPerlman.TheresultsoftheQualityControlProgramsaresummarized inSection6.23 SECTION4RESULTSANDDISCUSSION 24 444IAMiiE~i~iJNmI4<iliii&hCSSTa3Page1of3Environmental RadioloicalMonitorin ProramNameofFacility:
DonaldC.CookNuclearStationDocketNumber:50-315and50-316LocationofFacility:
BerrienCountyMichiganStateReporting Period:January-December1981MediumorPathwaySampled(UnitofMeasurement)
AirParticulates (pCi/m3)TypeandTotalNumberofAnalysesPerformed Gross8509C8-14424Zr-9524Nb-9524Ce-14124RU-10324Othery24Sr-898Sr-90LowerLimitofDetection (LLD)0.010.010.010.010.010.Ol0.010.0020.001AllIndicator Locations Meanl(Rane)0.12(291/301) 0.01-0.96 0.06(9/12)0.01-0.120.03(7/12)0.01-0.06 0.04(7/12)0.01-0.13 0.02(4/12)0.01-0.03 0.02(5/12)0.01-0.02 AllLLD0.002(1/4)0.002AllLLDLocationwithHihestMeanNameMean(Rane)NotApplicable NotApplicable NotApplicable NotApplicable NotApplicable NotApplicable NotApplicable On-Site60.16(52/52)0.02-0.96 NotApplicable ControlLocations Meanl(Rane)0.11(205/208)
Oi01-0.49 0.06(8/12)0.01-0.11 0.02(6/12)0.01-0.04 0.03(8/12)0.01-0.11 0.03(3/12)0.02-0i04 0.02(3/12)0.01-0.03 AllLLDAllLLDAllLLDNumberofNon-routine ReportedMeasurements 0000000AirborneIodine(Ci/m')WellWater(pCi/1)I-131508Tritium21ySpec.210F01100010AllLLD1120(9/12)600-1500AllLLDNotApplicable On-Site51300(3/3)1200-1500 NotApplicable AllLLD933(3/9)800-1200AllLLD0Meanandrangebasedondetectable measurements only.Frac'onsindicated inparentheses.
Table3(continued)
Facility:
DnaI0Page2of316MediumorPathwaySampled(UnitofMeasurement Milk(pCi/l)Precipitation (pCi/l)LakeWater(pCi/l)AquaticOrganisms (pCi/gwet)TypeandTotalNumberofAnalysesPerformed I-13157Sr-8957Sr-9057ySpec.57ySpec.24Sr-894Sr-904ySpec.20Tritium8Ce-1448Nb-958Zr-958Cr-518Ce-1418Othery8LowerLimitofDetection LLD0.051010'0200AllIndicator Locations MeanlRane)AllLLDAllLLD3.1(34/35)1.0-8.0AllLLDAllLLDAllLLDAllLLDAllLLD367(3/4)200-5001(1/4)11(1/4)1(1/4)12(1/4)2AllLLDAllLLDLocationwithHihestMeanNameMeanRaneNotApplicable LNotApplicable Galien3.3(11/11)1.0-7.0NotApplicable PNotApplicable NotApolicable NotApplicable NotApplicable NotApplicable South2On-Site2(1/4)NotApplicable NotApplicable South1(1/2)On-Site1South1(1/2)On-Site1South1(1/2)On-Site1ControlLocations Meanl(RaneAllLLDAllLID5.2(22/22)2.0-14.0AllLLDAllLLDAllLLD4(1/2)4AllLLD273(3/4)200-3202(1/4)22(1/4)21.5(2/4)1.0-2.0AllLLD(1/4)1AllI.I.DNumberofNon-routine ReportedMeasurements 0000000000000jgQg)1Meanandrangebasedondetectable measurements only.Fractions indicated inparentheses.
Table3(continued)
Facility:
DonaldC.CookNuclearStationPage3of3MediumorPathwaySampled(UnitofMeasurement AquaticOrganisms (pCi/gwet)TypeandTotalNumberofAnalysesPerformed Sr-898LowerLimitofDetection LLD)0.05AllIndicator Locations MeanlRaneAllLLDLocationwithHihestMeanNameMean(Rane)NotApplicable ControlLocations Meanl(Rane)AllLLDNumberofNon-routine ReportedMeasurements 00.021(2/4)0.017-0.024 Sr-9080'23(2.4)0.013-0.033 North0.033(1/2)On-Site0.0330.0050NotApplicable AllLLD0.05AllLLDNotApplicable South0.013(1/2)On-Site0.013Sr-908AllLLDySpec.4FoodCrops(Ci/wet)0AllLLDNotApplicable 7rSedimentySpec.81AllLLD(pCi/gdry)Sr-898AllLLD00.0050.013(1/4)0.048(1/4)00.0130.0481Fish(pCi/gwet)Background Radiation (TLD)(mR/week) ySpec8Sr-898Sr-908yDose820.050.005AllLLDAllLLD0.031(4/4)0.018-0.043 l.1(35/35)0.7-1.8NotApplicable NotApplicable North0.037(2/2)On-Site0.031-0.043 On-Site71.2(4/4)0.9-1.8AllLLDAllLLD0.045(4/4)0.030-0.053 1.1(47/47)0.7-1.90001Meanandrangebasedondetectable measurements only.Frationsindicated inparentheses.
7lJWd6
~r>>>>t>>~'>>,J>>>>>>ResultsofalltheanalysesforJanuarythroughDecember1981arepresented infullinSection5,DataTablespages38through49.Table3summarizes therangeandaverageconcentrations formeas-urementsattheindicator andcontrollocations withthehighestannual>>>>'!)>>rmean.Environmental monitoring resultsshowedthattheradiation dosetoamemberofthegeneralpopulation didnotexceedTechnical Specifi-cationsof1percentofthe10CFR20limitduring1981.Specificfindingforthevariousenvironmental mediaarediscussed below:'!>>>>>>>>AIRPARTICULATE SAMPLESAtmospheric particulate matteratafieldlocationisaccumulated foraone-weekonaglassfiberfilterusingalow-volume airsampleratacollection rateofonecubicfootperminute.Thisparticulate mattercontained onthefilteriscountedforbetaactivityinalowbackground countingsystemaftertheshort-lived naturally-occurring radonandthorondaughters havedecayed.Thegrossbetaparticulate dataobtainedduringthefirstsix-month 1t>>Aperiodof1981arehigherthanthedataobtainedduringthelatterhalf.According toP.K.Kurodaetal1,concentrations ofSr-89andSr-90inrainandsnowatPayetteville,
- Arkansas, showedaspectacular increaseduringthespringmonthsof1981duetothe25thChinesenucleartestexplosion ofOctober1980.Itistherefore suggested thatthesehigherP.K.Kuroda,"RecentAtmospheric ln)ections ofNuclearDebris:Palloutfromthe16October1980NuclearExplosion",
unpublished manuscript, 1981.28P>>>>'Y~>>~~8<<'>>>>>>)>>>>>>1>>>>>>>>>>hVlf\IVWWV~>>~f>>>>-~8>>Y>>V>>'w>>">>>>tl~>>>>'-
~'>>%*
levelsareattributable tothestratospheric falloutfromthistest.Theaveragegrossbetaconcentration fortheyearforallindicator stationswas0.12pCi/m,andwas0.11pCi/mforthebackground stations.
Dataforanalysesofindividual filtersaregivenonpages38through41in.Section5.Thefollowing tablesummarizes theaveragegrossbetaconcentrations forbothindicator andbackground stationsforeachyearfrom1973through1981.Thepreoperational datawerecollected in1973and1974;operational datawerecollected from1975throughthepresent.Indicator
~BackroundCi/m3+2crPreoperational 19731974Operational 19751976197719781979198019810.04+0.04 0.16+0.24 0.08+0.18 0.09+0.22 0.22+0.63 0.12+0.40 0.04+0.16 0.04+0.16 0.12+0.40 0.04+0.04 0.16+0.29 0.09+0.17 0.08+0.19 0.22+0.53 0.11+0.30 0.04+0.16 0.04+0.16 0.11+0.30 Theelevatedlevelsofgrossbetaactivityatbothindicator andbackground locations duringpreoperational andoperational phasesfrom1974through1981weremainlytheresultofnucleartestexplosions intheatmosphere bythePeople'sRepublicofChina.Suchteststookplaceon27June1973,17June1974,23January1976,26September 1976,17November1976,17September 1977,13March1978,14December1978,andSeeAnnualEnvironmental..Monitoring Reportsfor,D..C.CookPlantfrompreviousyearsfordetails.29 October1980.Thedataindicatethatthereis,significantly nodifference betweenthelevelsofgrossbetaactivitymeasuredattheindicator andback-groundlocations fortheoperational andpreoperational phasesoftheprogram.Theactivitydetectedarenotattributable totheoperation oftheCookplant.AirborneI-131concentration waslessthan0.1pCi/mforallsamplesreceived.
Thegammaspectrometry dataformonthlycomposites ofairparticulate filesbeginsonpage42.TracesofCe-144,Zr-95,Cs-137,Ru-103,Ru-106,"Nb-95,andCe-141weredetectedatbothindicator andbackground stationsduringthefirstsix-month periodof1981andareattributable tothestratospheric falloutfromthe25thChinesenucleartest.Be-7,anatu-rallyoccurring nuclideformedbythecosmicrayinteraction withnucleiintheupperatmosphere, wasalsodetectedinthecomposites.
Theseweregenerally intherangetobeexpectedfrommeasurement ofthisnuclideinthismedium.Quarterly composites ofairparticulate filterswereanalyzedforSr-89andSr-90.Sr-89concentrations wereatorbelowthedetection limitof0.002pCi/m,andSr-90werealsoatorbelowthedetection limitof0.001pCi/mforbothindicator andbackground locations.
Theseweregenerally intherangetobeexpectedfrommeasurements ofthesenuclidesinthismedium.MILKSAMPLESMilksampleswerecollected monthlyandwereanalyzedforI-131,Sr-89,Sr-90,andgammaemitters.
Sr-89concentrations measuredbelowthedetection limitof5pCi/l30+qr,.7~1~/4etit;':er'gi~'~P;h<<7,5r".Sar.,,,re
..Cs<ECPf..7.0>:V,5.9'"J~.'Ve*0~'.W'~
inallsamplescollected during"the year.:Si-90.:concentrations continued todisplayconsiderable variation, whichistypicalforthistypeofsam-pie.Thisnuclideisattributable toworldwide falloutfrombothrecentandoldernucleartestprograms.
Dataaregivenonpage43.I-131concentrations werebelowthedetection limitsof,theprogram.Date.arepresented onpage43.Gammaemittersotherthanthosewhichoccurinnaturewerenotde-tectedinmostsamplesatameasurement sensitivity of10pCi/1.TraceCs-137wasdetectedinonesamplefromDowagiacandwasduetoworldwide falloutfromrecentnucleartests.Dataaregivenonpage44.PRECIPITATION SAMPLESGammaisotopicanalysesofmonthlyprecipitation samplesfromindica-torandbackground locations indicatethepresenceofnogammaemittersinconcentrations exceeding 10pCi/1(<3000pCi/m2),.
Sr-89concentrations werelessthanthedetection limitof2pCi/l.TracesofSr-90werede-tectedinonebackground sampleandareattributable totherecentChinesebombtest.Dataarepresented onpage45.WELLWATERSAMPLESMellwateriscollected fromsevenlocations at18-weekintervals duringtheyearand.analyzed for.tr5.tium.and.-gamma emitters..
Low-concen-trationsoftritiumweredetectedinsamplesfrombothindicator stationsandbackground stationsthroughout 1981.Itispossiblethatthetritiumfoundisthesesamplesisaresultofplantoperations.
Gammaemitterswerebelowthedetection limitinallsamplesanalyzed.
Dataarepresent-4edonpage46.31 SamplesofwaterfromLakeMichiganarecomposited byindicator andbackground locations andanalyzedforgammaemittersonamonthlybasis.Quarterly composites ofthemonthlycomposites areanalyzedfortritium.Thegammaemittersinthemonthlycomposites weremeasuredtobelessthanthedetection limitof10pCi/1pernuclideforallsamples.Thetritiumconcentrations inthequarterly composites wereintherangeof200to500pCi/lforinindicator locations and200to320pCi/lforthebackground locations.
Theseconcentrations areintherangetobeexpectedfrommeasurements ofthisnuclideinthismedium.AVATICORGANISMS~LESAquaticorganisms werecollected twiceduringtheyearfromareasnorthandsouthoftheplant,aton-siteandoff-sitelocations.
Thesampleswereanalyzedforgammaemitters, Sr-89,andSr-90.TracesofCe-144,Nb-95,Ce-141,andZr-95werepresentinseveralsamples.Longandshorttermworldwide falloutdepositsareprobablythereasonfortheseactivities.
Sr-89wasnotdetectedinanyofthesamples;thedetection limitof0.05pCi/g(wet)wasachieved.
Sr-90weredetectedattracelevel(0.03pCi/gwet)infoursamplesandwereattributable torecentfallout.Dataarepresented onpage47.SEDIMENTSAMPLESSedimentsampleswerecollected twiceduringtheyearfromareasnorthandsouthoftheplant,aton-siteandoff-sitelocations.
Thesampleswereanalyzedforgammaemitters, Sr-89,andSr-90.Thegammaemitterswerebelowthedetection limitof1pCi/g(dry)32
~'na11thesamples;,
Sr.-89wasialsobelow.thedetection.
lirait-,0;.05-pCi/g(dry).TraceSr-90wasevidentintwosamplesandisduetorecentstratospheric fallout.Datearegivenonpage48,FISHSAMPLESFishsamplescollected fromareasnorthandsouthoftheplant,bothon-siteandoff-sitelocations, wereanalyzedforgammaemitters, Sr-89,andSr-.90.Forallsamples,gammaemitterswerebelowthedetection limitof11pCi/g(wet),andSr-89wasbelowthedetection limitof0.05pCi/g(wet).Sr-90rangedinconcentration from0.018to0.053pCi/g(wet).Theconcentrations observedwereattributable toworldwide falloutandweregenerally intherangetobeexpectedfrommeasurements ofthisnuclideinthismedium.Dataaregivenonpage48.FOODCROPSAMPLESGrapesandgrapeleaveswerecollected duringthefallharvestperiodfromon-siteandoff-sitelocations andwereanalyzedforgammaemitters.
Theywerefoundtobebelowthedetection limitof1pCi/g(wet)atbothon-andoff-sitelocations.
Dataaregivenonpage48.G~fA-DOSEGammaradiation dosewasmeasuredwithThermoluminiscent Dosimeters (TLDs)onaquarterly schedule.
Atotalof20fieldlocations (9indicator and11background) weremonitored duringthefirst,second,andthirdquartersoftheyear.Threeadditional background locations wereaddedinthefourthquarter.Throughout theyear,therewasnostatistically significant dif-33 ferenceindoseratesbetweenindicator andbackground locations, nordo.theydiffersignificantly fromdoseratesmeasuredinpreviousyears.Dataarepresented onpage49.34 SECTION5DATATABLES35 INTRODUCTION TOTHEDATATABLESThefollowing information willbehelpfulinunderstanding thepresentation ofthedatainthetablesinthissection.WetWeightareporting unitusedwithorganictissuesamplessuchasvegetation andanimalsamplesinwhichtheamountofsampleistakentobetheweightasreceivedfromthefieldwithnomoistureremoved.DryWeightareporting unitusedforsoilandsedimentinwhichtheamountofsampleistakentobetheweightofthesampleafterremovalofmoisturebydryinginanovenatabout110forabout15hours.pCi/msareporting unitusedwithairparticulate andradioiodine datawhichreferstotheradioactivity
.contentexpressed inpicocuries ofthevolumeofairexpressed incubicmeterspassedthroughthefilterand/orthecharcoaltrap.Notethatthevolumesarenotcorrected tostandardconditions.
GammaEmittersorGammaIsotopicsampleswereanalyzedbyhighresolution (GeLi)gammaspectrometry.
Theresulting spectrumisanalyzedbyacomputerprogramwhichscansfromabout50to2000kevandliststheenergypeakofanynuclidespresentinconcentra-tionsexceeding thesensitivity limitssetforthatparticular experiment.
NA,NS,NRusedinplaceofaconcentration whenasamplewasnotavailable (NS),orwhenasamplewasnotanalyzedforsomespecificmeasurement (NA),orwhenananalysisisnotrequired(NR).ErrorTermsfiguresfollowing "i"areerrortermsbasedoncountinguncertainties atthe2a(95Zconfidence) level.Valuespre-cededbythe"<"symbolwere.belowthestatedconcentration atthe3a(99Zconfidence) level.Exponents Exponents necessary topreventdatatablesfrombeingcumbersome arehandledintheconventional mannerofincluding theminthecolumnheadings.
Sensitivity Ingeneral,allanalysesmeetthesensitivity requirements oftheprogramasgiveninTable3.Forthefewsamplesthatdonot(becauseofinadequate samplequantities, analytical interferences, etc.)thesensitivity actuallyobtainedintheanalysisisgiven.Commentwhenallanalysesofaparticular typeduringtheperiodresultedinconcentrations belowthesensitivity limits,astatement ismadeontheappropriate tableratherthanpresenting awholepageof"<"data.Ifallbutoneortwodatapointsarebelowthesensitivity limits,thepreviously mentioned convention isfollowedandthefinitedataaregivenasfootnotes.
36 L'ISTINGOFMISSEDSAMPLES1981SamleneLocationExpectedCollection DateReasonLakeWaterAllJanuaryFebruaryLakefrozenatallpoints.AirParticulates ONS201/05-27Exposedpartoffiltermissingduetoapparentvandalism.
MilkGalienAirParticulates ONS4AirParticulates ONS4January02/1005/1906/19-3007/07Nomilkleft.Roadclosedduetosnow.Areaflooded.MilkSBN09/1210/10Nomilkavailable.
IodineCartridge COLAirParticulates ONS209/2612/14Lostinprocessing.
Nopowertounit.37 Collection Date01/05/8101/12/8101/19/8101/27/8102/03/8102/10/8102/17/8102/24/8103/03/81~03/10/8103/17/Sl03/24/8103/31/8104/07/8104/14/8104/21/8104/28/8105/05/8105/12/8105/19/8105/26/8106/02/8106/09/8106/16/8106/23/8106/30/81AIRBORNEIODINE-131*
andGROSSBETAinAIRPARTICULATE FILTERS(MeeklyCollections)
ON-SITE1ON-SITE3ON-SITE4Volume~msVolumeGrossGrossGrosstt9+112+114+120+213+1ll+118+210+1ll+112+126+317+243+166+718+126+334+231+223+241+434+317+235+318+218+221+25+13+18+17+13+12+16+13+13+16+14+15+18+113+16+110+15+11+1ll+115+212+16+112+12+13+14+1335335330360390(a)710375380380385385395355340355380375510lnoo420(a)(a)(a)(a)10+1ll+114+118+212+112+116+29+1ll+113+130+319+237+442+412+129+323+229+221+238+437+416+219+216+219+220+239539039536542037036535519028095(b)190405335330355350360350345235280265270250250DONALDC.COOKGrossB~ta10aCi/m"-ON-SITE2ON"SITE5VolumeVolumeVolumej~ra~~GrossGrossB~m>8355(a)4258+14653602+143514+146035040016+2460395(a)47046+53803758+146037-+33553553+14503303456+145015+23353551+143510+13653555il41010+12753556+140013+133036016+341529+33253504+141015+232532011+141040+431534516+239537+4110(c)g>-~~g+33510+1.40522+160(d)33010+139528+332029016+260(e)37+232035012+124523+13554857+128521+234529526+335035034022i236033+33003808+1385ll+131533542+4415295~,A$-.3556+13902803408+136032036516+2395315w,gP*Iodinecartidges aresampledweekly.Concentrations are<OslOpCi/munlessotherwise noted.(a)SeeListingofMissingSamplespage.(b)Lowvolumeduetobrokenmeter.'(c)Nopowor-(d)Lowvolumeduetopoweroffage.(e)Lowvolume:calculation basedonaveragevolume.-0
)<<4~~)m<<mm)seedwmauwwme
'ssmo,sef'vDONALDC.COOKAIRBORNEIODINE-131>>
andGROSSBETAinAIRPARTICULATE FILTERS(WeeklyCollections)
GrossBeta10Ci/m')S,=ON-SITE1ON-SITE2ON-SITE3ON-SITE4ON-SITE5Collection DateVolume~ms~GrossVolumeVolume~msGross0~msGrossVolume~msGross8VolumeGross807/07/Sl07/14/8107/21/8107/28/8108/04/8108/10/8108/17/8108/24/8108/31/8109(07/8109/14/8109/21/8109/28/8110/05/8110/12/8110/19/8110/26/8111/02/8111/09/8111/16/8111/23/81ll/30/8112/07/8112/14/8112/21/8112/28/81325305.3603352653302353803654253753753754054154153852504304353303503402152153455+14+13+110+12+1<11+11+12+1<11+1<1<11+1<1<11+11+11+11+11+11+11+15+11+11+1265255300320290305350390400350350340320425430445365195375420395390330(a)2252904+16+14+13+16+16+12+14+15+11+13+11+1<13+1<12+11+12+11+12+11+11+11+11+1<135541043046536537041539044540034034034533535536536036037036538038039536035035017+216+2ll+110+110+16+17+18+17+14+17+13+14+13+11+15+13+18+15+16+15+14+16+13+15+17+11140305210265270305335385320300295305300290285320325350420450410430405355360(a)13+110+114+1ll+16+16+18+16+13+16+12+13+16+12+14+13+17+15+15+1<15+15+14+14+16+132531532034030532034036539029028535035537037037536536040538540043036038035536516+216+212+110+112+16+18+110+17+13+17+13+14+13+12+16+1"3+18+12+17+15+15+16+17+16+18+1l)eee",.*Iodinecartidges aresampledweekly.Concentrations are<0.10(a)SeeListingofMissingSamplespage.pCi/msunlessotherwise noted.
ermmmq~im'sl>w~~~Ia<~wm~.t~~qCV't~.1,'IgmmIi(AIRBORNEIODINE-131" andGROSSBETAinAIRPARTICULATE FILTERS(WeeklyCollections) nci/m3Nr.vlBUFFALODOWAGIACCollection DateVolume(m3)Volume(m~)Volume(m3)GrossBetaVolume(m')'Ol/05/81 01/12/8101/19/8101/27/8102/03/8102/10/8102/17/8102/24/8103/03/8103/10/8103/17/8103/24/8103/31/8104/07/8104/14/8104/21/8104/28/8105/05/8105/12/8105/19/8105/26/8106/02/8106/09/8106/16/8106/23/8106/30/81355370355410445400420470425410430430465155(a).85(b)385360405415440440420430435425405410405405405395395375395365345350395425435445370425400440375400415415395400425460415350330325350340350305300270270265310315415415405395415415435420445375375365405380375380375365355310310310320345330330430435390405400395415390380375375365410350355355355370355310300305305340325310510460470520515380(a)Nopower.(b)Lowvolumeduetopoweroffage."Iodinecartridges aresampledweekly;Concentrations are<Om10DONALDC.COOKlk;<GrossBeta102ON-STTE6SOUTHBENDCOLCMAGrossCollection GrossVolumeGrossGrossBetaDateBeta(m3)BetaBeta12+101/03/&17+16+112+15+19+101/10/8115+1ll+113+12+117+201/17/8110+18+18+18+124+2Ol/24/8118+22+119+2ll+18+101/31/815+113+114+1ll+115+202/07/817+1.1+112+112+121+202/14/8110+1(110+14+16+102/21/8118+213+113+118+212+102/28/811+18+15+17+125+303/07/8114+15+114+14+12&i303/14/8118+230+319+218+217+203/21/8119+25+118+2-17+242+403/28/8117+220+223+29+196+1004/04/8145+542+449+522+222+104/11/8124+12&+225+114+148528+304/18/8127+327+324+29+139+104/25/8122+17+17+114+133+105/02/8130+28+135+29+125+305/09/8123+2ll+126~36+148543+405/16/8132+3ll+133+321+233+305/23/8133+37+140+433+313+105/30/8124+28+123+217+219+206/06/Sl'2+1 29+214+16+139516+206/13/8124+28+114+112+136017+206/20/8110+17+114+112+137519+206/27/8115+19+112+112+1pCi/munlessotherwise noted.3~~
.~ePtee'retteeDONALDC.COOKAIRBORNEIODINE-13l" andGROSSBETAinAIRPARTICULATE FILTERS(WeeklyCollections) ah~a~~),GrossBetalO2Ci/m~ON-SITE6NEWBUFFALOSOUTHBENDDOWAGIACCOLOMAe'I.";I~\4e~)Collection Date07/07/8107/14/8107/21/8107/28/8108/04/8108/10/8108/17/8108/24/8108/31/8109/07/8109/14/8109/21/8109/28/8110/05/&110/12/8110/19/8110/26/8111/02/8111/09/8111/16/8111/23/8111/30/8112/07/8112/14/8112/21/8112/28/81Volume(m~)350340365385320325355340365315295285290300295290320325315320300320310375355355GrossBeta15+216+211+111+112+16+17+110+17+14+17+14+14+16+12+15+14+17+17+17+18+16+15+15+15+17+1Collection Date07/04/&l07/11/8107/18/8107/25/8108/01/8108/08/8108/15/810&/22/8108/29/8109/05/8109/12/8109/19/8109/26/8110/03/8110/10/8110/17/8110/24/8110/31/8111/07/8111/14/8111/21/8111/28/8112/05/8112/12/8112/19/8112/26/81Volume(me)475425360400345350395410320290305335315335325340365340340360385360355370375365GrossBeta17+215+213+113+17+17+18+18+17+15+16+13+14+14+13+14+13+18+15+1'+12+14+15+15+14+14+1Volume(m~)355270315380330315350370'20305335320370375345325320355365380380365355340350330GrossBeta8+1,4+13+18+15+12+16+11+15+12+11+1<12+13+1<12+13+11+13+14+14+12+14+14+13+13+1Volume(n?~)330360350425350425425415325285300295280395310310325335325335330320355360370350GrossBeta21+211+111+112+17+17+18+1,6+17+15+14+14+14+13+13+14+15+18+15+16+15+14+15+14+13+14+1Volume(me)325335325350305340370430400430425390320(a)275295305295295290295285305330330325335GrossBeta19+2ll+15+113+14~17+11+16+17+14+14+13+14+14+12+15+12+16+14+12+15+16+14+14~14+131~'"'1(a)SeeListingofHissedSainplespage."Iodinecartridges aresainpledsleekly.Concentrations are<Oe10pCi/munlessotherwise noted.
etfOrfehtRRDONALDC.COOK"GAMP%ISOTOPICANALYSISofMONTHLYAIRPARTICULATE COMPOSITES MonthCe-144orroCi.mZr-95Ce-Re-0~OtherJanuaryFebruary~RfarchAprilMayJuneJulyAugustSeptember OctoberNovemberDecember<0.010.03~0.01 0.05+0.02 0.04+0.02 0.11+0.01 0.05+0.010.10+0.02 0.10+0.01 0.06+0.01 0.07+0.01 0.06+0.01 0.09+0.01 0.01+0.01 0.0l+0.01 0.07+0.01 0.10+0.01 0.12+0.01 0.07+0.01 0.060.010.05+0.01 0.05+0.01
<0.01<0,01<0.010.03~0.01 0.01+0.01 0.03+0F010.06+0.01 0.04+0.01 0.01+0.01 0.01+0.01
<0.01<0.01<0.01<0.01<0.010.010.010.01~0.01 0'4+0.010.060.010.13+0.01 0.020.010.02+0.01
<0.01<0.01<0.01<0.01<0.010.01+0.01<0.010.03+0.01 0.02+0.01 0.03+0.01
<0.01<0.01<0.01<0.01<0.01<0.01<0.01<O.01<0.010.02+0.01 0.02+0.01 0.02+0.01 0.01+0.01 0.01+0.01
<0,01<0.01<0.01<0.01<0.01<0.01<0.01<0.01<0.01(a)<0.01<0.01<0.Ol<0.01<0.01<0.01<0.01<0.013Jtt4MonthJanuaryFebruaryMarchAprilMayJuneJulyAugustSeptember OctoberNovemberDecemberBe-70.06+0.01 0.020.010.04+0.02 0.14+0.02 0.12+0.03 0.08+0.01 0.08+0.02 0.09+0.01 O.ll+0.02 0.08+0.01 0.13+0.02 0.06+0.01 Ce-144<0.010.01+0.01 0.02+0.01 0.11+0.02 0.11+0.02 0.05+0.01 0.09+0.01 0.020.010.04+0.02
<0.02<0.01<0.01<0.010.01+0.01 0.02+0.01 0.04+0.01 0.04+0.01 0.01+0.01 0.02+0.01
<0.01<0.01<0.01<0.01<0.01<0.010.01+0.01 0.02+0.01 0.07+0.01 0.11+0010.020.010.010.010.010.010.01+0.01
<0.01<0.01<0.01<0.01<0.010.04~0.01 0.040,010.02+0.01
<0.01<0.01<0.01<0.01<0.01<0.01<0.01BackroundStationsCi/msZr-95Nb-95Ce-141RU-103<0.01<0.010.02+0.01 0.020.010.03+0.01
<0.01<0.01<0.01<0.01<0.01<0.01<0.01OtherY<0.01<0.01<0.01<0.01<0.01<0.01(b)<0.01<0.01<0.01<0.01<0.01<0.01STRONTIUM-89/90 hNALYSISofQUhRTERLY hIRPARTICULATE COMPOSITES Indicator StationsBackroundStationsCollection PeriodSr-89Ci/msSr<<90Sr-89oCi/msSr-90~~1stquarter2ndquarter3rdquarter4thquarter<0.0020.002+0.001
<0.002<0.002<0.0010.001+0.001
<0.001<0.001<0.002<0.002<0.002<0.002<0.001<0.001<0.001<0.001(a)Cs-137.0.01+0.01 (b).Ru-106~0.01+0.01 42
~~~~~~IIIIIIIIIIIIIIIIIIIIIIIIIIIIIIII~~~~e~
ilC'FFh>PV+PPataiiFFFCollection'Site:
Collection DateOl/10/8102/07/8103/07/8104/04/8105/02/8106/06/8107/04/8108/01/8109/12/8110/10/81ll/07/8112/05/81DONALDC.COOKRADIONUCLIDES inMILKSAMPLES(MonthlyCollections)
Indicator StationsGalienCs-137Ci/l<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10(.)<10<10<10<10<10<10<10<10<10<10<10BridmanK2Stevensville K1<10<10<10<10<10<10<10<10<1010+3<10<10<10<10<10<10<10<10<10<10(a)(a)<10<10BackroundStationsDoMaiacKlSouthBendKli:~>-'V';FF'FVVF.'p4.PWCZcli:F'ei%5tF.,~~(<,+5-hh.5,,/FFF't.,PiiYFQ~k.OtherGammaEmittersCil<10<10<10<10<10<10<10<10<10<10<10<10<10<lo<lo<10<10<10<10<10<10<10<10<10(a)<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10<lO<10<10<10(a)(a)<10<ln(a)SeeListingoEMissingSamples.page.Q<'k5+.j DONALD'".C
.COOK'AMMA ISOTOPICANALYSISOFPRECIPITATTON SAMPLES(MonthlyCollections)
Collection Sites:Collection PeriodIndicator
~Ci/1r01/m*BackroundrCi/1.rCS/r*JanuaryFebruaryMarchAprilMay.~JuneJulyAugustSeptember OctoberNovemberDecember<10<10<10<10<10<10<10<10<10<10<10<10<0.4<0.2<0.3<0.4<0.4<0.3<0.3<0.4<0.5<0.5<0.3<0.2<10<10<10<10<10<10<10<10<10<10<10<10<0.4<0.2(a)<0.3<0.3<0.3<0.2<0.2<0.3<0.3<0.3<0.5<0.2RADIOSTRONTIUM CONCENTRATIONS INPRECIPITATION SAMPLES(Semiannual AnalysisonComposites ofMonthlys)
Indicator Ci/1BackroundCi/lCollection PeriodSr-89Sr-90Sr-89Sr-90January-June July-December
<2<2<1<1<2<24+2<1(a)Ru-103=0.4+0.1nCi/ma.45 ee~e~eejII1CgejiAA')~Ici)Collection Site:Collection Date01/23/8105/06/8109/11/81DONALDC.COOKRADIONUCLIDES INWELLWATERSPPPLES(18-weekIntervalCollections)
BackroundStationsONS1ONS2ONS3ONS4ONS7TritiumCi/ml<10.8+0.408+0.4<1<1<1l.2+0.4<1<1<10'+0.40.6+0.41.5+0.41.2+0.41.2+0.4GammaEmittersCi/1<10<10<10<10<10<10<10<10<10<10<10<10<10<10<10'e~','4'Indicator StationsONS5ONS6peg'.1+0.41.1+0.41.0+0.4<11.4+0.41.2+0.4>,i.eeelV,vs(j<10<10<10<10<10<10'"Q,~;f~ffe-[4,'
DONALDC.COOKGAMMAEMITTERSINLAKEWATERSAMPLES(MonthlyComposites ofIndicator andBackground Stations)
GammaEmittersCi/1/nuclide MonthIndicator ComositeBackroundComositeJanuaryFebruaryMarchApril?fayJuneJulyAugustSeptember OctoberNovemberDecember(a)(a)<10<10<10<10'<10<10<10<10<10<10(a)(a)<10<10<10<10<10<10<10<10<10<10i4Iuarter1st2nd3rd4thIndicator Stations200+100400+110<200500+100BackroundStations200+100'20+200
<200300+200TRITIUMINLAKEWATERSAMPLES(Quarterly Composites ofMonthlySamples)TritiumCi/1RADIONUCLIDES INAQUATICORGANISMS (Semiannual Collections whenAvailable)
LocationCollection DateSr-89Ci/wet')Sr-90Zr-95OtheryONSSONSNOFSSOFSNONSSONSNOFSSOFSN07/23/8107/23/8107/23/8107/23/8109/15/8109/15/8109/15/8109/15/81<0.05<0.05<0.05<0.05<0.05<0.05<0.05<0.050.013+0.005 0.033+0.028 0.024+0.019 0.017+0.013
<0.005<0.005<0.005<0,0051+1<11+12il<1<1<1<1<1(b)<1<1<1(c)<1<1<1<1(a)SeeListingofHissingSamplespage.(b)Ce-144,Nb-95=lil;Cr-512~1.(c)Ce-144,Nb-952+1;Ce-1411+1.47l'il+l9'I0.Pan%IgsqqI~Pgll'I~,~'algal".I
''r'I">Pl'0P~IIIllQR>litsuPI@*v)*,IIh~i%i,lIPOe9<<Ii~li'LII RADIONUCLIDES INSEDIMENTSAMPLES(Semiannual Collections)
Slf>>gDONALDC.COOKe9:>>')Collection SiteCollection DateCi/dr)GammaEmittersSr-89S>>-90ONSNONSSOFSViOFSS05/19/8105/19/8105/19/8105/19/81<l<1<l<l<0.05<0.05<0.05<0.05<0.0050.013+0.004
<0.0050.048+0.009 f"-,'i~>>'>>e>>rONSViONSSOFSNOFSS09/21/8109/21/8109/21/8109/21/81<1<1<1<1RADIONUCLIDES INFISHSAMPLES(Semiannual Collections)
<0.05<0.05<0.05<0.05<0.006(a)
<0.005<0.005<0.005Collection SiteCollection DateCi/wet)Se-89GammaEmittersSe-90ONSiVONSSOFSNOFSSONSNONSSOFSNOFSS05/12/81OS/l2/8l05/12/8105/12/8109/23/8109/23/8109/23/8109/23/81<1<l<l<l<1<1<1<1<0,05<0.05<0.05<0.05<0.05<0.05<a.as<0~050.031+0.005 0.032+0.008 0.053+0,012 0.045+0.007 0.043+0.0080.018+0.009 0.030+0.015 0.051~0.017 RADIONUCLIDES INFOODCROPS(AnnualFallHarvestCollection)
Collection Site:Collection SampleDate~e09/30/81Grapes09/30/81LeavesONSiteOFFSiteCi/(wet)GammaEmitters(a)Lowersensitivity duetolowchemicalyield.448 DONALDC.COOKGANfARADIATION (Quarterly3 (Measured UsingThermoluminiscent Dosimeters3 DateAnnealed:
DateRead:12116/8004/07/811st0tr.)iain'ackupTLDTLD03/18/8107/08/812ndOtr.MainBackupTLDTLD06/18/8110/06/813rdOtr.HainBackupTLDTLD09/17/8112/30/814thOtr.MainBackupTLDTLD'I,'l~<LocationIndicator StationsOn-SitelOn-Site2On-Site3On-Site4On-Site5On-Site6On-Site7On-Site8On-Site90.9+0.2missing0.8+0.10.9+O.l0.8+0.20.7+0.10.9+O.l0.8+0.20.8+O.l0.7+0.1missing0.8+0.20.8+O.l0.7+0.10.7+0.10.7+O.l0.9+0.10.7+0.10.7+O.l0.8+O.l0.7+0.10.9+0.11.0+0.2missing0.9+O.l0.8+0.10.8+O.l0.9+O.l0.9+0.10.8+0.20.9+O.l0.9+O.l1.0+0.10.8+0.10.7+0~21.0+O.l1.3+0.21.4+0.11.2+O.l1.0+0.l1.2+O.l1.2+0.11.3+0.11.3+0.11.20.2MeasuredmR/week1.2+0.11.0+0.11.2+0.1missing1.3+0.21.2+0.11.2+0.21.1+0.11.1+O.l1..5+0.21.6+0.21.5+0.41.4+0.41.8+0.5'.6+0.1 1.8+0.41.5+0.21.5+0.21.5+0.61.7+0.11.6+0.31.4+0.41.8+0.81.5+0.52.1+1.51.6+O.E)2.0+0.3Background StationsNewSouthBendDowagiacColoma0.9+0.21.0+O.l0.7+0.10.7+0.10.8+O.l0.9+0.20.8+O.l0.8+0.20.8+0.10.7+0.20.8+O.l0.7+O.l0.9+O.l1.0+O.l0.9+0.20.9+O.l1.1+0.11.0+O.l1.0+0.11.0+O.l1.2+0.11-3+0.10.9+0.10.9+0.11.5+0.1l.7+0.41.5+0.31.5+0.21.6+O.l1.7+0.31.7+0.41.8+0.6Off-Site-1 Off-Site-2 Off-Site-3 Off-Site-4 Off-Site-5 Off-Site-6 Off-Site-7 Off-Site-8 Off-Site9Off-Site-10 0.8+O.l0.8+O.l0.8+O.l0.7+O.l0.8+0.10.7+O.l0.9+0.20.9+O.l0.9+O.l0.9+0.20.9+O.l0.8+O.l0.8+0.3,0.7+O.lEffective 4thQuarter0.9+0.20.8+0.20.7+0.10.8+0.10.9+0.21.0+0.20.9+O.l0.9+0.10.9+0.10.8+0.10.9+0:10.9+O.l0.8+O.l0.8+0.11.1+0.11.0+0.11.8+O.l1.3+0.11.1+0.11.1+O.l1.0+0.2l.0+0.11.0+O.l1.1+0.21.0+0.10'+0.20.9+0.11.0+O.l1.5+0.21.4+0.11.6+0.51.5~0.21.7+0.41.9+0.31.5+0.41.5+0.31.7~0.31.4+0.11.5+0.41.5+0.51.8+0.71.8+0.71.8+0.42.1~1.21.6+0.61.5+0,41.7+0.21.5+0.4 SECTION6QUALITYASSK4QICE DATA50 ENVIRONMENTAL QUALITYCONTROLANALYSESSUMMARY1981'Ihetablesbelowsummarize resultsofsamplesrunforprocessqualitycontrolpurposesduringthcsubjectmonth.Theselistingsareinadd-itiontosuchm<<asuremcnts nsdutcctorbackgrounds, checksourcevalues,radiometric-gravimetric comparisons, systemcalibrations, etc.Detailedlistingsofeachmeasurement aremaintained atthelaboratory andareavailable forinspection ifrequired.
'BLANKSAMPLES.NuclideAnalzedNumbursof.
Determinations Numburofanalysesexceeding theLLDforthatanalsisGrossbetaGrossalphaStrontium-89 Strontium-90 TritiumGammaemitterIodine-131 Calcium-45 46479595616419131*000]*000SPLITSAMPLESNuclideAnnlvz<<.d GrossbetaGrossalphaGammaemittersIodine-131 Strontium-89 Strontium-90 TritiumCalcium-45 UraniumNumberofDet'ns14239126-146384489871No.agreeingwith'I.n2a13838122146384289871SPIKEDSAMPLESNo.agreeingwithin3a414002000No.differing bv>3a000000000NuclideAnalzed'rossbetaGammaemittersIodine-131 Strontium-89 Strontium-90 TritiumNo.ofDes'es5544ll189445Within2aof'nown534311189344Within3aofknown110011differing fromknownb>3a1*00000*Corrective actionsweretakentoeliminate theproblem.51 EPAINTERCOMPARISON 1981~~~I~hu~~~~~~I1~1~I~I~I~~~2~~~~~!iRESULTSpage1of3'onth/Yea rDecember1980D<<cember1980December1980December1980Decembex'980 D<<cumber1980,1anuary1981January1981January1981January1981January1981January1981January1981January1981January1981January19811'<<brunry1981F<<bruary1981Februax'y 1981February19811:obruary 1981February1981February1981Mareh1981M;ix'c1<1981March1981March1981'larch1981March1981April1981April1981April1981April1981April1981April1981April1981Apx'il1981Hay1981May1981May1981Yiay198lMay1981i~1Qy1981SampleTe1aterWaterAirFilterAizFilterAirFilterAirF11c<<tWaterWaterHaterWaterMilkMilkMilkMilkMilkN.lkWaterWaterWaterWatezWacerWaterWaterHaterWaterAirFilterAirFilterAirFilterAirFilterWaterWaterWaterWaterWaterWaterWaterWaterWaterWaterWaterWaterWater'HaterAnalsisIodine-131 TH.tiumGrossAlphaGrossBetaStrontium-90 C<<siuu<-137 GrossAlphaGrossBetaStrontium-89 Strontium-90 Strontium-89 Strontium-90 Iodine-131 Cesium-137 Barium-140 Potassium TritiumChromium-51 Cobalt<<60Zinc-65Ruthenium-106 Cesium-134 Cesium-137 GrossBetaGrossAlphaGrossAlphaGrossSetaStrontium-90 Cesium-137 TritiumCesium-134 Cesium-137 Strontium-89 Strontium-90 Radium-226 Radium-228 UraniumStrontium-89 Strontium-90 Strontium-89 Strontium-90 Iodine-131 Cesium-137 AgencyValuu22224021190199441634020.225.843.501551176002585036425253050181427101015382815.012.0123622ControlLimitsQ3nn3)66049;18.708.78.78.78.72.902.610.48.7013459008.78.708.78.78.710.4138.72.68.76158.78.78.72.64.03.1108.72.6MWFMeasuredx2oerror*17+22600+30021228~3LT119+210~143+4LT535+4LT214+129+347~5LT251350+1401680170LT10029+592+9LT10029+59327+320+230+366+717+415+23000+3007+213135+724313.2~1.310+26+229+326+3UnicspCi/liter pCi/liter pCi/filter pCi/filter pCi/filter oCi/Cilc<<r pCi/litez pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/literpCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter
'Ci/liter pCi/lit<<r pCi/filter pCi/filter pCi/filtex pCi/filter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter
- Whenanalysesofaparticular typeresultinconcentrations belowthedetection limits,theterm"LT"isusedtoindicate"LessThan"valuesforthatmeasurement.
basedon3a(99.5%)confidence level.~~~~"ieiqqp e~-EPAINTERCOMPARXSON RESULTS1981Page2"of3.>>.5Month/Year 198119811981198119811981198.1198119811981198119811981198119811981198119811981198119811981198119811981198119811981198119811981MayaMayJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJuneJulyJulyJulyJulyJulylylyulyJulyJulyJulyJulyAugusthu>>ustAugustSeptember September September September September September'eptember September September September September
~1981198119811981198119811981198119811981SampleTeMaterWaterWaterMaterWaterWaterWater'aterWaterWaterMaterAirfilterAirfilterAirfilterAirfilterFoodFoodFoodFoodFoodPoodMilkMilkMilkMilkMilkMilkWaterWaterWaterMaterWaterUrineMaterWater.WaterWaterAirfilterAirfilterAirfilterAirfilterAnalsisBarium-140 Potassium Chromium-51 Cobalt-60 Zinc-65Ruthenium-106 Cesium-134 Cesium-137 TritiumRadium-226 Radium-228 GrossalphaGrossbetaStrontium-90 Cesium-137 Strontium-89 Strontium'-90 Iodine-131 Cesium-137 Barium-140 Potassium Strontium-89 Strontium-90 Iodine-131 Cesium-137 Barium-140 Potassium Iodine-131 TritiumUraniumStrontium-89 Strontium-90 TritiumRadium-226 Radium-228 GrossalphaGrossbetaGrossalphaGrossbetaStrontium-90 Cesium-137 AgencyValue01559017015213119506.78.02854191644318245026402517031016002326302323ll20508.311.7332825521619ControlLimits~3eu)013508.708.78.78.75961.72.1128.72.68.'78.72.8148.702298.72.608.7013913613108.72.65992.23.048.7118.72.68.7MWFMeasured~7oerrorLT20)400+140LT2016+2LT2013+413+225+32300+2005.9~0.410.6i).631674+821+515+238+428+375+840~4<252267i22713+316+3<535+12<161463+30553+11297387814+218+514+22166+6248.4+0.84..6+3a7'"32+1430+625+671+718+220+2UnitspCi/liter mg/literpCi/liter pCi/liter
~pCi/liter
-.pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/filter pCi/filter pCi/filter pCi/filter pCi/kilogram pCi/kilogram pCi/kilogram pCi/kilogra~
pCi/kilogram mg/kilogram pCi/li.terpCi/liter pCi/literpCi/liter pCi/liter mg/literpCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/~terpCi/liter pCi/liter pCi/filter PCi/filter PCi/filter pCi/filter
- 53ps~~~~g<e<<~v<<,was>>q,.-r>>a<>>e<aaea>>
'<<ae<.<<<<We<et<'ee'<<e<V.e EPAINTERCOMPAPiXSON RESULTS1981Month/Year SampleTeAnalsisAgencyValueControlLimits~3eu)MWFMeasured+7oerrorUnitsOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberOctoberNovemberNovemberNovemberNovemberNovemberNovemberDecember198119811981193119811981193119811981198119811981198119811981,19811981198119811981198119811981WaterWaterWaterWaterWaterWater'WaterWaterWaterWaterliilkMilkMilkHi,lkMilkMilkFoodFoodFoodFoodFoodPoodWaterGrossalphaGrossbeta.Cobalt-60 Strontium-89 Strontium-90 Cesium-134 Cesium-137 Radium-226 Radium-228 CrossUraniumStrontium-89 Strontium-90 Iodine-131 Cesium-137 Barium-140 Potassium Strontium-89 Strontium-90 Cobalt-60 Cesium-137 Barium-140 Potassium Tritium809602114.4121512.79.215231852250153038233033027302700358.708.72.62.68.73.32.4108.72.6108.701338.72.68.78.7023661591+2611211LT513+614.6+2.014+220+1411.8~3.58.3+5.19+224+814+558ll.29+9LT161700+24041+621+535+832+8LT312700+2702950+127pCi/liter pCi/li,ter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/literoCi/liter pCi/liter pCi/liter pCi/liter mg/literpCi/kilogram pCi/kilogram pCi/kilogram pCi/kilogram pCi/kilogram mg/kilogram pCi/liter 54 EPAINTZRCOMPARLSON RESULTSp$<X<j1981(LabPerformance Evaluation Study-EHSL-LV)
SampleAgencyControlLimits~(3an]MMPMeasured2eerrorUnitsg~:WaterWaterWaterWaterWaterWater,WaterMaterWaterWaterWaterGrossalpha39Grossbeta60Cobalt-60 12Cesium-134 12Cesium-137 20Ruthenium-106 0Zinc-650Strontium-89 6Strontium-90 0Radium-226 12.8Uranium5101.839+470+7LT2011+220+2LT100LT20LT112.6+1.34+2pCi/liter pCi/liter
.,pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/liter pCi/1'[ter pCi/liter 55 1981SampleTe,Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)Air(81-04)0.244E+040.117E+030.450E+020.630E+010.122E+030.139E+040.190E+040.223E+Ol0.2470.015E+040.0930.006E+030.5150:087E+02(0.100E+020.8280.048.E+020.1330.006E+040.133+0.007EM40.750+0.053 E+01Be-7Mn-54Sr-89Sr.-90Zr-95Sb-125Cs-134Ur.~I,I'~~r~r.r~USDOEUALITYASSESSMENT PROGRAMMeasuredNuclideKnown~2aerror"lUnitspCi/filter pci/filter pCi/filter pCi/filter pCi/filt'er pCi/filter pci/filter pCi/filter P;'I'trSoil(81-04)Soil(81-04)Soil(81-04)Tissue(81-04)Tissue(81-04)Tissue(81-04)Tissue(81-04)K-40Sr-90Ra-226U0.158E+010.240E+Ol0.450E+000.290E-OLK-400.213E+02Cs<<1370.200E+00Ra-2260.770E+000,290+0,017 K+020.250+0.070 E+000.668+0.057 E+000.433+0.058 E+Ol0.188+0.016 E+010.433+0.058 E+000.850+0.333 E-01pci/gpci/gpCi/gpci/gpci/gpCi/gpCi/g~'I~i~IVegetation (81-04)Vegetation (81-04)Vegetation (81-04)Vegetation (81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)Water(81-04)K-40Sr-90Cs-137UH-3Co-57Co-60Sr-90Cs-137Ce-141UU0,224E+030.560E+010.230E+000.310E+000.246E+020.118E+010.129E+010.440E-010.137E+010.527E+010.145E-010.102E-010.277+0.018 E+030.258+0.016 E+Ol0.200+0.058 E+000.133+0.058 E+000.197+0,012 E+020.243+0.018 E+Ol0.133+0.006 E+010.405i0.063 E-010.150+0.012 E+010.193~0.012 E+010.200+0.026 E-Ol0.?50+0.140 E-02pci/gpci/gPCi/gpCi/gpCi/mlpCi/mlpCi/mlpci/mlpCi/mlpCi/mlug/mlpCi/ml TLDIntezcomparison BadgesIrradi.ated byBattelleNorthwest'.
LabsTotalmRlesstransortationcontrol1sttr2ndtr3rdtr4thtrMeasuredIH.O18.54.126.029.1+2'2<).I+6.I 18.017.85aO24.024.5+5.538.034.1+9.057.042.16.059.061.4i6.569.077.612.569.071.219.047.046.85'44.043.2+6.020.025.54.890.086.2-15.5 28.031.4~2.551.053.65.316.017.9+2.7100.093.4~10.1 32.036.5+3.542.041.9~19.7 40.041.24.018.020.1+3.453.055.4~15.2 29.032.0-3.076.065.66.673.074.1~21.6 69.075.1~13.2 34.032.0~3.088.088.6+12.6 79.080,8+17.3 82,080.4+10.7 82.079.0+8.0I00.0I00.0I02+I099+1079.079.9+18.2 99.0100.2i25.4 93.0100.086.1+15.534.038.7~9.3100.4~15.374.069.2~8.857
'.JJl)."0,g~,lp44',"!'r.3l",j~l(ACliJP,'Il'~%PAL+'th,Wll.JI9(%pfH\8,gW4q".)ApAp~~)t