ML20107K537

Annual Radiological Environ Operating Rept for 1995

ML20107K537
Person / Time
Site:	Waterford
Issue date:	12/31/1995
From:	James Fisicaro ENTERGY OPERATIONS, INC.
To:	NRC OFFICE OF INFORMATION RESOURCES MANAGEMENT (IRM)
References
W3F1-96-0064, W3F1-96-64, NUDOCS 9604260198
Download: ML20107K537 (81)

Text

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.cs Entergy E;gga-*a= 'ac-Operations x>=< t^ 7ooce, Te 504 739-6650 W3F1-96-0064 A4.05 PR April 24,1996 U.S. Nuclear Regulatory Commission ATTN: Document Control Desk Washington, D.C. 20555

Subject:

Waterford 3 SES Docket No. 50-382 License No. NPF-38 Annual Radiological Environmental Operating Report Gentlemen:

Attached is the subject 1995 annual report on radiological environmental monitoring which covers the period of January 1 through December 31,1995. This report is submitted per Section 6.9.1.7 in the Waterford 3 Technical Specification (NUREG-1117).

If there are any questions, please contact C. Jeff Thomas at (504) 739-6531.

Very truly yours, wo .

J.J. Fisi ro Director Nuclear Safety 3 JJF/CJT/ssf Attachment cc: (w/ Attachment)

L.J. Callan (NRC Region IV), NRC Resident inspectors Office (w/o Attachment).

C.P. Patel (NRC-NRR), R.B. McGehee, N.S. Reynolds 9604260190 951231

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ANNUAL RADIOLOGICAL l

l ENVIRONMENTAL l OPERATING REPORT 1995 Entergy Operations, Inc.

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ANNUAL RADIOLOGICAL ENVIRONMENTAL OPERATING j REPORT

1 i FOR WATERFORD 3 STEAM ELECTRIC STATION t i

4 ,. JANUARY 1 THROUGH DECEMBER 31,1995 l i

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! i i Docket Number: 50-382 i

License Number: NPF-38 i

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ABSTRACT This report is issued pursuant to Waterford 3 Technical Specification 6.9.1.7. Its purpose is to discuss the Waterford 3 Radiological Environmental Monitoring Program (REMP), present the results of the program for the year of 1995, and evaluate the radiological impact on the environment resulting from plant operation.

98 The Waterford 3 REMP collected data on environmental radioactivity levels around the Waterford 3 nuclear power plant. These levels were determined by analyzing samples of air, water, shoreline soil, fish,

- vegetation, and milk from various locations around the facility. Based on the evaluation of the environmental data collected, the operation of )

Waterford 3 exhibited no discernable impact on the levels of radioactivity in the environment during 1995.

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a TABLE OF CONTENTS PAGE ABSTRACT................................................................................................................ i

- TAB L E O F C O N TE NTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. . . . . . . . . . . .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .ii. . . . . . . . . . . . .

iv L I ST O F TA B L E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

L I ST O F F I G U R E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .vi

-1.0- I N TR O D U C TI O N . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

Prog ram a nd Report Objectives .. . .... ...... ...... ................. .. .... ..... ..... ... . . .. 1 1.1~

1 1.2 Pla nt a nd Site Description . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

2.0 P R OG RAM D E S C R I PTI O N . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2. . . . . . . . . . . . . .

2.1 H isto ry a nd Development . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 2.2 Respon sibilities . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .2. . . . . . .

! 2.3 Sample Collection and Handling Procedures ...... ........................... ...... 3 i , 2.3.1 Direct Radiation Exposure Pathway Samples......................... ... 3

' 3 2.3.2 Airborne Exposu re P athway Samples . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

2.3.3 Waterbome Exposure Pathway Samples ................................... 4 2.3.4 I ng e stio n Ex pos u re Pathwa y S a m ples . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 2.4 Ana lytica l Proced u res . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5 ....

2.4.1 Gross Beta Analysis in Air Particulates....................................... 5 2.4.2 G ross Beta An alysis in Water ....... .. . ... ... .... ...... . .. . .. ... . . ... . . ... . .. .. .. 5

- 2.4.3 Tritium Anaiy a!s la Water ... ..... ... . . . ....... . . .. .... . . .. .. ... . . . ... . .... . .... . . .... 6 2.4.4 lodine-131 Analysis in Milk and Water ....................................... 6 2.4.5 Gamma Spectroscopy Analysis .......... ....................................... 6 l

, 2.4.6 E nvironmental Dosimetry .. .. .. . . . .. .. . .. .. . . . .... .. ...... . . .. ..... .. . . .. . .. ... .. . 6 2.4.7 Lowe r Limits of Detectio n . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 7 2.5 La boratory Q u a lity Ass u ra nce . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 7 3.0 D I S C U S S I O N O F R E S U LTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .21 ..........

3.1 Di rect Rad iation Ex pos u re Pathway . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 21 3.2 Airborne Exposu re P athway . . . . . . . . . . . . . . . .. . . . . . . . . . . . . . . . . .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 21

. 3.2.1 Airborne P a rticu lates . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 21 ..

3.2.2 Ai rborne l od ine . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .22 .....

3.2.3 Gamma I sotopic Analysis. . .. ...... .. .. .. . .... . . ....... .. . .. ... . .. .. ... . .. .. . . ... ... . 22 ii

TABLE OF CONTENTS (CONTINUED)

PAGE 3.3 Wate rborne Exposu re Pathway .... . . . ........ . . .. . . . .. .. .. . . . . . .. .. . . ... . . .. . .. . . .. . .. . .. 22 3.3.1 D rin king /Su rface Water ... ... .. . . . . . .... . .. . .. ..... .. .... .. .... .. . .. . . . . .. . . ... . . . 22 3.3.2 G ro u n d wa te r. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .23 ......

j 3.3.3 S h oreline Sed iment . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 23

3.4 I ngestio n Expos u re P athway .... ...... . .... .......... .. . ... . ..... .. .. . . .. . .. ... . ... .. .. . .. ... . 24 3.4.1 Milk........................................................................................... 24 3.4.2 Fish........................................................................................24 3.4.3 B road Le af Vegetatio n . . ..... . .. .. . . . .... ..... ... .. . . . ... .... . .. .. . . .. .. . ....... .. 24 3.4.4 Food P rod u cts . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 3.5 Statistica l An a lyse s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 5 3.5.1 Calculation of the Mean and Standard Deviation............ ... .. . 25 3.5.2 Comparing Two Sample Population Means ....... ... ................. 25 3.5.3 TL D M e a s u reme nts . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .2. 7 3.5.4 Gross Beta on Air Particulate Filtars .... .............. .................... 27 3.5.5 Gross Beta in Monthly Drinking Water Composites .... ....... . .. 27 3.6 Deviation s from the R EM P .. ..... . . ... .. . .. .... .. .. ..... . . . . . .. . . . .. . .... . .. . . . ... . . .. . . .. . . 28 3.6.1 U n available Sa mples . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 28 3.6.2 La ck of Sa m ple Contin uity.. .. . .. .. ... . .. .. . . . . .. . . .... . . . . .. . . ... .. . . . . .. .. . ... . . 28

-1 3.6.3 Missed Lower Limits of Detection............................................. 28 3.7 Annual Land Use Census Results ................ .................................. .. ... 28

4.0 CONCLUSION

S............................................................................................ 35 AP P E N DlX A - R E M P DATA S U M MARY .. .. . .. .... . . . . . . . . . . .. . . . . . . ... .. . . . . . . . . . . .. . . .... . . . . .. .. 39 A P P E N D lX B - R E M P DATA . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4. 5 iii

LIST OF TABLES PAGE ,

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TABLE 2.1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM l

( R E M P) S U M MARY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .8. . . . . . . . . . . . . j l

TABLE

2.2 DESCRIPTION

OF REMP SAMPLING STATION LOCATIONS.......... 9 TABLE 2.3 DETECTION CAPABILITIES FOR ENVIRONMENTAL SAMPLE ANALYSIS, LOWER LIMIT OF DETECTION (LLD)............................. 16 l

l TABLE 2.4 ANALYTICAL 1.ABORATORY EPA CROSS CHECK RESULTS......... 17 TABLE 3.1 1995 DIRECT RADIATION DATA ORGANIZED BY COMPASS  !

DIRECTION AND DISTANCE FROM WATERFORD 3 SES.............. 29 i

1 TABLE 3.2

, STATISTICAL COMPARISON OF 1995 TLD MEASUREMENTS FROM STATIONS GROUPED BY DISTANCE FROM l WATE R FO R D 3 S E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3. .0. . . . . . l TABLE 3.3 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY ON AIR 31 4

i PARTICULATE FILTERS FOR 1 9 9 5 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . l l

TABLE 3.4 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY IN MONTHLY DRINKING WATER COMPOSITES FOR 1995.......... .... 32 1 TABLE 3.5

SUMMARY

OF 1995 REMP DEVIATIONS.... ...... ............................. 33 TABLE 3.6 1995 ANNUAL LAND USE CENSUS RESULTS .. .................... ........ 34 TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

........................................................................................39 TABLE B-1 Q UARTE R LY TLD D O S E RATE S .. .. . . . . . . . . . . . . ... . .. . .. ... ... . ... .. . . . . . . . . . . . . . . . . . 46 TABLE B-2 AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES

, GROSS BETA AND IODINE-131 ANALYSES.................................... 47

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I LIST OF TABLES (CONTINUED) I i PAGE '

, TABLE B-3 AIR PARTICULATE FILTERS: GAMMA ISOTOPIC ANALYSIS ON Q U ARTE RLY C O M POS ITES .. .... . . ... . . .. . . .. ... .. . .. . .... . . ... . . . . . . . . ..... . . ..... . . . . 52 i TABLE B-4 DRINKING WATER: LODINE-131 ANALYSIS.................................... 53 TABLE B-5 DRINKING WATER: GROSS BETA ANALYSES ON MONTHLY -

COMPOSITES AND GAMMA ISOTOPIC ANALYSIS ON MONTHLY C O M P O S I T E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .56 ...........

TABLE B-6 DRINKING WATER: TRITIUM ANALYSIS ON QUARTERLY COMPOS!TES.................................................................................62 TABLE B-7 GROUNDWATER: TRITIUM AND GAMMA ISOTOPIC j A N A LY S E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .6. .3. . . . . . .

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, TABLE B-8 SHORELINE SOIL: GAMMA ISOTOPIC ANALYSES........................ 64

, TABLE B-9 MILK: IODINE-131 AND GAMMA ISOTOPIC ANALYSES ............... 65 t

TABLE B-10 FISH: GAMMA ISOTOPIC ANALYSES ............ ........................... .... 67 TABLE B-11 BROAD LEAF VEGETATION: LODINE-131 AND GAMMA 2

I S OTO P I C AN ALYS E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 6 . 9 TABLE B-12 VEGETATION - FOOD PRODUCTS: IODINE-131 AND GAMMA I S OTO P I C AN A LY S E S . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .7. 2 ...

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l FIGURE 2.1 REMP SAMPLE LOCATIONS WITHIN 2 MILES OF I WAT E R F O R D 3 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 18 1

l FIGURE 2.2 REMP SAMPLE LOCATIONS WITHIN 10 MILES OF WATE R F O R D 3 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 19 FIGURE 2.3 REMP SAMPLE LOCATIONS WITHIN 50 MILES OF l 1

WAT E R F O R D 3 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .2. .0. . . . . . . 1 l

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4 FIGURE 3.1 DIRECT RADIATION DOSE COMPARISON.............. ....................... 36

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l FIGURE 3.2 GROSS BETA - AIR PARTICULATE COMPARISON ........................ 37 FIGURE 3.3 GROSS BETA - DRINKING / SURFACE WATER COMPARISON..... . 38 4

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1.0 INTRODUCTION

This report describes the Radiological Environmental Monitoring Program 2

(REMP) for the Waterford 3 Steam Electric Station and discusses the results obtained during the calendar year 1995. The results discussed in this report t

were used to evaluate the radiological environmental impact from the operation of Waterford 3. The submission of this report to the Nuclear Regulatory Commission (NRC) fulfills the requirements pursuant to Waterford 3 Technical Specification 6.9.1.7.

1.1 Program and Report Objectives The objective of the monitoring program is to evaluate the radiological environmental impact of the plant. In order to conduct this evaluation, the data analyses and interpretations contained in this report fulfill the

following specific objectives:

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a. to identify any radioactive materials or radiation in the environment

associated with plant operation,

b. to compare the results obtained during the reporting period with past operational and pre-operational data and identify any trends associated with accumulation of radioactivity in the environment; and

, 3 c. to verify compliance with federal regulatory requirements.

1.2 Plant and Site Description l 4 Waterford 3 employs a pressurized water reactor for the production of approximately 1153 gross (1104 net) megawatts of electricity. The station uses a flow of water obtained from and discharged to the Mississippi River for condenser cooling. On March 4,1985, the unit achieved initial

cnticality.

The plant is located on the west bank of the Mississippi River at River Mile 129.6 between Baton Rouge and New Orleans, Louisiana. The site is in l the northwestern section of St. Charles Parish approximately 3 miles southeast of the St. John the Baptist Parish boundary between Killona and Taft. The Mississippi River is the closest prominent natural feature; other features include Lac des Allemands, about 5.5 miles southwest of the site, and Lake Ponchartrain, about 7 miles northeast of the site.

Most of the man-made features are located on the narrow strip of land between the Mississippi River and the wetlands. Specifically, several industrial facilities including Waterford 1 and 2 Steam Electric Stations (0.4 miles northwest), Little Gypsy Steam Electric Station (0.8 miles northeast), IMC Agrico, a fertilizer manufacturer (0.6 miles east 1 l

i southeast), Oxychem Chemical Company (0.8 miles east southeast), and Union Carbide, a chemical manufacturer (1.2 miles east southeast) are operating in the area.

l Major urban centers in the region include New Orleans (approximately 25 L miles east) and Baton' Rouge (approximately 50 miles west northwest).-

Communities near the site in St. Charles Parish include Killona (0.9 miles west northwest), Montz (1.0 miles north), Norco (2.5 miles east), Hahnville (3.7 miles east southeast), and Destrehan (6.3 miles east southeast).

Laplace (4.7 miles north) is located in St. John the Baptist Parish.

2.0 PROGRAM DESCRIPTION A general summary of the REMP is given in Table 2.1; brief descriptions and locations of the sampling stations are presented in Table 2.2. In addition, station-locations are illustrated in Figures 2.1 through 2.3 A more detailed description of the REMP is provided below.

2.1 History and Development The Waterford 3 REMP evolved from the Pre-operational Environmental Radiological Surveillance (PERS) program (1978-1982) and was initiated

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in April of 1983. Equipment, procedures, techniques, and sampling locationa used during the pre-operational survey were incorporated into the operational program. Further, the environmental data collected during 3 the first two years of the REMP (1983 and 1984), prior to initial criticality, were used to supplement the baseline established during the PERS Program.

2.2 Responsibilities Waterford 3 personnel are responsible for implementing and ensuring that the REMP complies with federal regulatory, Technical Specification, and Offsite Dose Calculation Manual (ODCM) requirements. Responsibilities ,

of Waterford 3 personnel include collecting (with the exception of fish samples), preparing, and shipping of environmental samples; conducting environmental dosimetry measurements; reviewing analytical results reports; and preparing and submitting the annual Radiological Environmental Operating Report and other relevant reports to the Nuclear Regulatory Commission. i The primary contractor, Entergy Services, Inc. (ESl) System Chemistry located in Little Rock, Arkansas, is responsible for performing radiological analyses; conducting initial data review; preparing results reports; and overseeing laboratory quality assurance and control. Additionally, a separate contractor, the Fisheries Co-operative Extension Service of Louisiana State University, is responsible for the collection of fish samples.

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2.3 Sample Collection and Handling Procedures Sample types, location, collection frequency, and the analyses performed 1 are summarized in Tables 2.1 and 2.2. The information contained in

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these tables is based on requirements specified in Table 5.8-1 of the . l Waterford 3 ODCM. Location maps of the sampling are illustrated in l Figures 2.1 through 2.3. Any stations deviations (i.e., unavailable .

samples and missed lower limits of detection) or changes made to the REMP during 1995 are discussed in Section 3.6.

The environmental samples collected are classified into four general categories according to exposure pathways: direct radiation, airbome,.

waterbome, and ingestion. Sample collection and handling procedures are described in the following sections. The descriptions are intended to provide a concise procedural overview rather than a step-by-step description.

2.3.1 Direct Radiation Exposure Pathway Samples Integrated external gamma exposure, determined using Panasonic multi-element thermoluminescent dosimeters (TLDs), was measured at thirty-one locations as follows:

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a. an inner ring of stations, one in each of the sixteen meteorological sectors, in the general area of the site

. boundary;

b. an outer ring of stations, one in ten of the sixteen meteorological sectors, in the six to eight kilometer range  :

from the site; and

c. the balance placed in areas of special interest (e.g.,

population centers, schools, etc.) with one area serving as a control.

The TLDs were exchanged and analyzed quarterly by Waterford 3 personnel.

2.3.2 Airborne Exposure Pathway Samples

! Samples of airborne particulates and radiolodines were collected at four indicator stations (APP-1, APQ-1, APG-1, APC-1) and one

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control station (APE-30). Low-volume air pumps and flow totalizers in weather proof shelters provided continuous air sampling.

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i Using the sampling device described above, airborne particulate samples were obtained on a filter and collected weekly by Waterford 3 personnel for shipment to the contract laboratory for

, gross beta analysis. The filters were composited quarterly by the contract laboratory for isotopic analysis by gamma spectroscopy.

Airborne iodine sampling was done in conjunction with air particulate sampling using a charcoal cartridge to collect iodine.

The cartridges were collected weekly by Waterford 3 personnel and sent to the contract laboratory for iodine-131 analysis by gamma spectroscopy.

i. 2.3.3 Waterborne Exposure Pathway Samples

. Because the plant discharges into the Mississippi River, the major source of drinking water in the vicinity of Waterford 3, water samples taken from the Mississippi River were designated as both drinking and surface water samples.

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i Composite drinking / surface water samples were obtained biweekly from the Mississippi River using automatic composite samplers

placed at one upstream (DWP-7/SWP-7) and two downstream (DWG-2/SWG-2, DWE-5/SWE-5) locations. Hydrochloric acid was

added to each sample prior to shipment. The contract laboratory

analyzed the biweekly samples for lodine-131, composited them

- monthly for gross beta and gamma spectroscopy, and composited  ;

them quarterly for tritium analysis. '

! Due to the high water table resulting from shallow aquifers in the i

vicinity of the site, drainage canal sampling represents groundwater discharge. Groundwater was obtained quarterly by grab sampling from one sampling location (GWK-1). Again, hydrochloric acid was

! added to the sample prior to shipment to the contract laboratory for  !

tritium and gamma spectroscopy analyses.

) Shoreline sediment samples were obtained semi-annually from a

, sampling station at each plant discharge point. Station SHWE-3 is i located downstream on the shoreline of the Mississippi River; I

! station SHWK-1 is on the shoreline of the 40-Arpent canal. The i samples were shipped without further processing, 2.3.4 Ingestion Exposure Pathway Samples i

Milk samples were collected semi-monthly from one indicator location (MKQ-5) and one controllocation (MKQ-45). Sampling of the control station was performed by Louisiana Radiation l Protection Division personnel. Although one additionalindicator l location was identified (MKQ-1), no samples were available from 4

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O this location during 1993 (see Section 3.6). Finally, formaldehyde -

was added as a preservative to all samples prior to shipment.

Upon arrival at the laboratory, iodine-131 and gamma spectroscopy analyses were performed.

Fish samples were collected bi-annually from the Mississippi River  ;

upstream (FH-1) and downstream (FH-2) from the plant. A contractor performed the sampling by netting. Subsequently, the fish were segregated by species and location prior to delivery to Waterford 3. The samples were shipped frozen for analysis by  !

gamma spectroscopy.  ;

- The Waterford 3 ODCM, Section 5.8.1, requires broad leaf l vegetation to be sampled from 3 locations within 5 miles of the j plant in the event milk samples are unavailable. Since milk  :

samples were collected from only one sampling location within five I miles of Waterford 3, broad leaf vegetation was sampled monthly at I I

two indicator locations (BLQ-1 and BLB-1) and one control location (BLK-15). The samples were shipped without further processing.

I Food product sampling was not required because no areas surrounding the plant were irrigated with water in which plant wastes are discharged. However, food products grown within the site boundary were collected to demonstrate the absence of radionuclide accumulation.

These food product samples (sugarcane) were collected at the time '

of harvest from two locations (FPG-1 and FPP-1) by normal harvesting techniques and shipped without further processing.

lodine-131 and gamma spectroscopy analyses were performed.

2.4 Analytical Procedures 2.4.1 Gross Beta Analysis in Air Particulates l After allowing for the radon-222 and radon-220 daughter products .

to decay, the particulate filters were counted in a gas-flow I proportional counter.

[

4 2.4.2 Gross Beta Analysis in Water

! A known volume of water, usually 200 milliliters, was reduced by evaporation, transferred to a two inch diameter planchet, and evaporated to dryness. The planchet was counted for 100-200

minutes or until the required LLD is achieved in an automatic l- alpha-beta counter.

1 1

5 l

s,v- - - --, , .,.

2.4.3 Tritium Analysis in Water A known volume of water, 5 milliliters, was added to 15 milliliters of liquid scintillation solution in a 25 milliliter vial. The sample was

counted for 500 minutes in a liquid scintillation counter.

2.4.4 lodine-131 Analysis in Milk and Water

! Approximately four liters of sample were mixed with a stable iodine carrier solution and eluded through an anion exchange resin column to remove iodine from the sample. lodine analysis was i performed using gamma spectroscopy. The time between sample receipt and analysis, sample amount, and count times were ~

adjusted in order to attain the required LLD. The chemical yield was corrected by measuring the stable iodide content of the milk or water with a specific lon electrode.

I 2.4.5 Gamma Spectroscopy Analysis l Air particulate filters and iodine cartridges, water, milk, broadleaf vegetation, sediment, food products and fish samples are prepared

in containers, using the appropriate geometry for its sample type.

4 Secondly, the sample is counted in a shielded high purity l germanium (HPGE) or germanium lithium (GeLi) detector coupled to a computer based data acquisition system that performs pulse height analysis.

~ The computer software program defines peaks by changes in the i

slope of the spectrum, compares each specific peak energy with a library of pes.ks for isotopic identification, and performs the i radioactivity calculation using the apropriate fractional gamma ray 4 abundance, half life, detector efficiency, and net counts in the peak

, region.

lodine analysis was performed using gamma spectroscopy. The i time between sample receipt and analysis, the sample size and count times were adjusted in order to attain the required lower limit of detection.

I 2.4.6 Environmental Dosimetry 4

) Model UD-814 Panasonic thermoluminescent dosimeters (TLDs) that contain one lithium borate and three calcium sulfate phosphor elements were used for environmental dosimetry. However, only i

the calcium sulfate phosphor elements were used for analysis. For i

placement in field, two annealed dosimeters are placed inside a plastic bag and mounted in an aluminum frame. The dosimeters are checked monthly and exchanged for analysis each quarter 6

I

- ._ .- ._. -. - - - -- . _= .. .- -_ . - -

using an automatic TLD reader manufactured by Panasonic (Model l UD-710).

2.4.7 Lower Limits of Detection (LLD)

The minimum sensitivities for the analytical procedures are j

reflected by the Lower Limits of Detection (LLD) values presented  ;

in Table 2.3 from Table 5.8-3 of Waterford 3 ODCM. The LLD's are a priori estimates based on assumed sample volumes, counting times, detector efficiencies, etc. Analyses that could not achieve these lower limits of detection are discussed in Section 3.6.

l 2.5 Laboratory Quality Assurance i During 1995, the ESI System Chemistry laboratory performed between 5% and 10% of all analyses for quality assurance purposes. Spiked and blank samples were prepared in-house. In addition, the laboratory participated in the EPA Radiological Interlaboratory Comparison (cross-check) Program.

j This quality assurance program satisfies the requirements of the Waterford 3 ODCM, Section 5.8.2, for participation in an interlaboratory comparison program. The program involved analyses on various sample media typically found in the REMP. As a result of participation in the program, an objective measure of analytical precision and accuracy was

- obtained. In the event that results obtained by ESI System Chemistry were not within control limits (3 standard deviations), an investigation was l conducted to determine the cause, and corrective action was taken to prevent a recurrence. Table 2.4 lists the 1995 results of the laboratory's i participation in the cross-check program.

2 1

i l

i 7 l

i , .

TABLE 2.1 .

RADIOLOGICAL ENVIRONEMNTAL MONITORING PROGRAM (REMP)

SUMMARY

l l SAMPLE TYPE LOCATION ANALYSIS FREQUENCY DIRECT RADIATION A-2, B-1, C-1, D-2, E-1, F-2, G-2, H-2, J,2, K-1 TLD Gamma - Quarterly L-1, M-1 N-1, P-1, Q-1, R-1 A-5, B-4, D-5, E-5, F-4, G-4, H-6. P-6, Q-5, R-6, G-9, E-15, J-15 E-30 AIR RADIOIODINE AND APP-1, APQ-1. APG-1, APC-1, APE-30 Gross Beta 'lieekly PARTICULATES l-131 Quarterly Composite Gamma Isotopic DRINKING WATER

• DWG-2, DWE-5, DWP-7 H-3 Quarterly Composite Gamma Isotopic Monthly Composite Gross Beta 1-131 Bi-Weekly Composite SURFACE WATER" SWG-2, SWE-5, SWP-7 H-3 Quarterly Composite Gamma Isotopic Monthly Composite Gross Beta 1-131 Bi-Weekly Composite GROUND WATER GWK-1 H-3 Quarterly Gamma Isotopic SHORELINE SEDIMENT SHWE-3, SHWK-1 Gamma isotopic Semi-Annually MILK MKE-4, MKQ-5, MKQ-1, MKO-45 Gamma Isotopic Semi-Monthly 1-131 BROAD LEAF BLQ-1, BLB-1, BLK-15 Gamma Isotopic Monthly l-131 When milk samples are not collected FISH FH-1, FH-2 Gamma Isotopic in season or Semi-Annually FOOD PRODUCTS FPG-1 FPP-1, FPQ-1 Gamma Isotopic At harvest time 1-131 a_ Based on requrernents in Table 5.8-1 of Waterford 3 SES otTsite Dose Calcutational Manual Secten 5.8-1.

b. Dnnking and surfa water samples are identcat.

8

. .- .- - =. - . . .--

TABLE 2.2 .

DESCRIPTION OF REMP SAMPLING LOCATIONS i

LOCATION LOCATION DESCRIPTION DISTANCE METOROLOGICAL FROM DIRECTION PLANT j DIRECT RADIATION (TLD)

A-2 (Eastbank) Located on a utility pole on River Road (LA 628) at the south comer of the Zephrin L 1.1 N Perriloux Fire Station (Station 5)in Montz La.

B-1 (Eastbank) On fence endosing the transmission tower O.3 miles west (up4iver) from Little Gypsy. 0.8 NNE Access from River Road (LA 628). TLDs are located at SW comer of fence enclosure.

I C-1 (Eastbank) On fence endosing the Utile Gypsy Cooling Water intake. Access is from River Road (LA 0.8 NE 628) across from Little Gypsy Steam Electnc Station entrance TLDs are on the south side (inside) of the Coohng Water intake fence endosure, directfy opposite the entrance gate.

D-2 (Eastbank) Located approximately 0.3 miles cast of Little Gypsy Power Station. Access from River 1.1 ENE ,

Road (LA 628). TLDs are attached to a stop sign post located at the peak of the levee on the west entrance road through the Bonne Carre Spillway.

E-1 (Westbank) Located on utility pole along River Road (LA 18) approximately 0.3 miles east of Waterford 0.2 E ,

3 plant entrance. Access from LA 18. TLDs are on the third utility pole east of the construchon entrance road.

F-2 (Westbank) Located on fence endosure surrounding the LP&L 1.1 ESE '

substation on I.A 3142. Access from LA 3142 approximately 0.2 miles south of LA 18. TLDs are on the southeast comer of the fence endosure 9

TABLE 2.2 .

DESCRIPTION OF REMP SAMPLING LOCATIONS LOCATION LOCATION DESCRIPTION DISTANCE METOROLOGICA.L FROM DIRECTION PLANT -

G-2 (Westbank) Located on utility pole on east side of LA 3142 (Next to tinion Carbide Star Plant Gate 3). 1.2 SE Access from LA 3142 approximately 0.2 miles north of railroad overpass.

H-2 (Westbank) Located on fence enclosure to shell road off of LA3142. Access from LA 3142 south of 1.2 SSE i railroad overpass on east side of LA 3142. TLDs are on the south side of the gate for shell road (just south of Texaco pipeline station). -

J-2 (Westbank) located on northeast comer of fence endosing Texaco valve station south of LA 3127. 1.3 S Access from LA 3127, approximately 0.6 miles west of LA 3127/3142 intersechon  !

K-1 (Westbank) Located on fence at Gate 92 entrance off of LA 3127. Access from LA 3127. approximately 1.0 SSW.

1.3 miles west of LA 3127/3142 intersection. (Gate 92 is the access to the Waterford 3 switchyard I station and training center.)

i L-1 (Westbank) Located next to

• Private Road" sign at LP&L Gate 97 entrance off of LA 3127, 1.0 SW approximately 1.6 miles west of LA 3127/3142 intersechon (Gate 97 is an access road for Waterford 3.)

M-1 (Westbank) Located on south gate into the Waterford 1 and 2 SES fuel oil storage tank endosure. 0.7 WSW Access is either thru LP&L Gate 92, Gate 97 off of LA 3127, the shell access road from LA 18 between I Waterford 3, or through the Waterford 1 and 2 SES access road.

N-1 (Westbank) Located behind the "No Tre , passing" sign off of Short Street, in Killona, just south of the 0.9 W l entrance to Killona Elementary School.

P-1 (Westbank) Located, on Short Street, in Killona. TLD is inside fence at air sample station APP-1. 0.8 WNW 10

__ _ _________j

i l

TABLE 2.2 +

i

~

DESCRIPTION OF REMP SAMPLING LOCATIONS i

LOCATION LOCATION DESCRIPTION DISTANCE METOROLOGICAL FROM DIRECTION PLANT Q-1 (Westbank) Located on fence enclosing air sample station approximately 0.5 miles west of Waterford 1 0.8 NW

! and 2 on River Road (LA 18).

R-1 (Westbank) Located on fence enclosure for Waterford 1 and 2 Cooling Water intake Structure. Access 0.5 NNW is from River Road (LA 18) opposite Waterford 1 and 2. TLDs are on the southwest comer of fence.

A-5 (Eastbank) Located on utility pole just east of the Shady Nook Trailer Park on Hwy 61 in Laplace. TLDs 4.5 N are on second utility pole east of trailer park on north side of Hwy 61 (eastem end of Laplace).

B-4 (Eastbank) located on utility pole just east of shell access road to South Central Beu transmission 3.8 NNE tower on south side of Hwy 61. Transmission tower is just east of weigh station at St. John /St. Charles Parish line. TLDs are on the first utility pole east of access road.

D-5 (Eastbank) Located on fence gate on shell access road to Big 3 Chemical Plant. Shell access road is 4.2 ENE approximately 0.1 miles west of Hwy 61/48 intersechon (at black and yellow gate). TLD's are on fence gate 0.1 miles north on shell access road from Hwy 61.

E-5 (Eastbank) Located on the Norco Substation fence enclosure. Access from River Road (LA 48) onto 4.2 E Wesco St. (adjacent to Norco Shell Chemical Plant), take Wesco St. to the dead end. TLDs are located on sixth fence post south of the north substation gate.

F-4 (Westbank) Located on utility pole behind blonde brick house on Aquarius St. in Hahnville. Access 3.5 ESE from River Road (LA 18) and tum onto Oak St. Follow Oak St to Hickory St., tum right on Hickory St.

and follow to Aquarius St d tum left Blonde brick house is second house on right (west) side of Aquarius St. heading south.

11

TABLE 2.2 .

DESCRIPTION OF REMP SAMPLING LOCATIONS LOCATION . LOCATION DESCRIPTION DISTANCE METOROLOGICAL FROM DIRECTION PLANT G-4 (Westbank) Located on railroad sign northwest side of LA 3160/ railroad track intersechon Access from 3.2 SE either LA 3127 or River Road (LA 18) onto LA 3160.

H-6 (Westbank) Located on a road sign on the northwest side of the second canal bndge east of LA 3160 5.7 SSE along LA 3127.

P-6 (Westbank) Located on a fence surrounding the Union Pacific communications tower at the LA 5.5 WNW 640/ railroad intersechon approximately 500 ft from LA 640.

Q-5 (Westbank) Located on fence post surrounding (green) river marker on levee just east of Edgard. 5.0 NW I

Fence post is located along River Road (LA 18) across from the Webre's house.

R-6 (Eastbank) Located on fence enclosing LP&L laydown yard on LA 3223 in Laplace. Access from Hwy 5.3 NNW 61 onto Elm St. (LA 3223), take Elm St. to the northeast comer of LA 3223/ railroad intersechon TLDs are located on the southeast comer of fence enclosure.

i F-9 (Eastbank) Located on entrance gate to Destrehan Substation. Access from River Road (LA 48), 8.2 ESE l approximately 1.5 miles east of Luling-Destrehan Ferry, onto Jonathan Street (west of Bunge Corp.

Grain Elevator), and proceed to substation gate.

l G-9 (Westbank) Located on back fence of LP&L District Office in Luling. Access via Ellington St. imm either 8.1 SE River Road (LA 18); or Second or Third St. from Paul Maltaird Rd- (LA 52) to Ellington St.

E-15 (Eastbank) Located on Kenner Substation fence enclosure. Access from either River Road (LA 48) or 11.8 E Hwy 61, tum onto Alliance Ave. TLDs are located on the north side of the fence enclosure, near a light j pole.

i 12

TABLE 2.2 ,

DESCRIPTION OF REMP SAMPLING LOCATIONS LOCATION LOCATION DESCRIPTION DISTANCE METOROLOGICAL FROM DIRECTION PLANT J-15 (Westbank) Located on fence enclosure surrounding LP&L switchyard at LA 631/ Hwy 90 intersechon in 12.0 S Des Allemands. TLDs are on the northwest corner of fence. Access from LA 631 via shen road.

t E-30" (Westbank) at LP&L General Office on Delaronde St in AJgiers. TLDs are in the courtyard at the south 27.0 E entrance to the building.

AIRBORNE APP-1 (Westbank) Located in soybean / sugarcane field ai northwest comer of Short SL in K Nona 0.8 WNW i APQ-1 (Westbank) Located at northwest comer of soybean / sugarcane field on east side of KiBona Access 0.8 NWO from River Road (LA 18) approximately 0.6 miles east of LA 18/3141 intersechon.

APG-1 (Westbank) Located at the north side of the Secondary Meteorological Tower. 0.5 SE 1

APC-1 (Eastbank) Located inside the Little Gypsy Cooling Water intake Structure fence enclosure. 0.8 NE APE-30" (Westbank) Located on the roof of the LP&L General Office building on Delaronde St. in Algiers. 27.0 E WATERBORNE DWG-2 (Westbank) Located at the Union Cartade drinking water canal. Access from LA 3142 through Gate 28. 2.0 SE SWG-2 DWE-5 (Eastbank) Located at the St Charles Parish Waterworks off of River Road (LA 48) near New Sarpy. 4.5 E SWE-5 13

TABLE 2.2 .

l DESCRIPTION OF REMP SAMPLING LOCATIONS -

! LOCATION LOCATION DESCRIPTION DISTANCE METOROLOGICAL-i FROM DIRECTION

PLANT DWP-7** (Westbank) Located at the St. John Parish Waterworks off of LA 18 in Edgard. 6.5 WNW SWP-7**

SHWE-3 (Westbank) Located at the Foot Ferry Landing off of LA 18 in Taft. 3.0 E SHWK-1 (Westbank) Located at the 40 Arpent Canal south of the Plant. Access from LA 3127 through Gate 92 0.5 SSW G W K ,1 (Westbank) Located at 40 Arpent Canal south of the plant. Access from LA 3127 through LP&L Gate 0.5 SSW 92 which is at the Waterford 3 Training Center. The canalis northwest of the shell access road / railroad track intersection.

INGESTION (MILK)

MKQ-1 (Westbank) 1.0 miles west of Waterford 3 SES at the comer of River Road and Post Street in Killona. 1.0 NW i MKQ-5 (Westbank) Located at the Webre's house, just across LA 18 from river marker, at the eastem end of 4.9 NW Edgard.

MKQ-45** (Eastbank) Located off of I-12 in Denham Springs, take LA 3002 south to LA 1034 then right to LA 42 NW 1032 then left. Farm is 1 mile on the right.

INGESTION (BROAD LEAF VEGETATION)

BLQ-1 (Westbank) Located between LA 18 and soybean field on eastem edge of Killona, near air sample 0.8 NW station APQ-1.

BLB-1 (Eastbank) Located at wooded area at the southwestem comer of the LP&L Little Gypsy plant along 0.8 NNE River Road.

BLK-15** (Westbank) Located 3.5 miles SSW of Des Allemands on Hwy. 90. 15 SSW 14

-- -- --.-. - - - - . . . - ~ . - ...- - .-_- . -. . - -

TABLE 2.2 DESCRIPTION OF REMP SAMPLING LOCATIONS LOCATION LOCATION DESCRIPTION DISTANCE METOROLOGICAL FROM DIRECTION PLANT-INGESTION (FOOD PRODUCTS ***)

FPP-1 (Westbank) Located in sugarcane / soybean field on eastem edge of KiHona, between air sample 0.8 WNW stations APP-1 and APO-1.

FPG-1 (Westbank) Located in a sugarcar:e/ soybean field east of Waterford 3 near the back-up meteorological 0.4 SE tower and air sample station APG-1.

INGESTION (FISH)

FH-1

• Upstream of the plant intake structure. NA* NA*

l FH-2 Downstream of the plant discharge structure. NA* NA*

NA- NOT APPLICABLE  !

" Control Location

• 3 Food products are not required since no areas surrounding the plant are irrigated with water into which plant wastes are discharged. Food products grown within the site boundary were collected however, in order to dernonstrate the absena of marwnade radionuchdes 15  :

4 TABLE 2.3 DETECTION CAPABILITIES FOR ENVIRONMENTAL SAMPLE ANALYSIS LOWER LIMIT OF DETECTION (LLD)(')

WATER AIRBORNE FISH MILK FOOD SEDIMENT ANALYSIS (pCill) PARTICULATE (pCilkg-wet) (pCill) PRODUCTSN foCilka-drv)

OR GAS (pCI/m') (pCilkg-wet) gross beta 4 0.01 H-3 2000 ,

1 Mn-54 15 130 Fe-59 30 260 Co-58, 60 15 130 Zn-65 30 260 ,

Zr-95 30 Nb-95 15 .

1-131 1 0.07 1 60 Cs-134 15 0.05 130 15 60 150 Cs-137 18 0.06 150 18 80 180 ,

Ba-140 60 60 La-140 15 15

a. From Table 5.8-3 of Waterford 3 SES Offsite Dose Calculation Manual.

b. Applicable to broad leaf vegetation.

16

1 o

i TABLE 2.4 l ANALYTICAL LABORATORY EPA CROSS CHECK RESULTS MEDIA NUCLIDE EPA ESI, SYSTEM NORM DEV.

EPA PREP DATE DATE RESULTS RESULTS CHEMISTRY KNOWN ISSUED RESULTS 75.0 71.67 -0.72 09/30/94 02/06/95 MILK 1-131 59.0 62.67 1.27 GAMMA Cs-137 1715.0 1653.33 -1.24 I (pCUL) K (Total) 4 Gross Beta 23.0 19.00 -1.39 l 10/28/94 02/13/95 WATER (pCi/L)

Co-60 59.0 69.33 3.58' 11/04/94 02/14/95 WATER

• Zn-65 100.0 128.33 4.91*

.I (pCi/L)

Cs 134 24.0 27.33 1.15 Cs-137 49.0 60.33 3.93**

Ba-133 73.0 97.00 5.94 I131 100.0 100.00 0.00 02/03/95 04/21/95 WATER (pCi/L)

Tritium 7435.00 7030.00 0.94 03/10/95 05/18/95 WATER

~

(pCi/L)

Co-60 29.0 29.33 0.12 04/18/95 08/16/95 BLIND B Cs-134 20.0 18.67 -0.46 (pCi/L)

Cs-137 11.0 11.00 0.00 Beta 86.8 77.93 -1.50 Co-60 40.0 39.66 -0.12 06/09/95 Unofficial WATER 76.0 80.00 0.87 (pCi/L) Zn-65 Cs-134 50.0 45.00 -1.73 Cs 137 35.0 35.66 0.23 79.0 76.66 -0.51 Ba-133 19.4 23.4 1.37 07/21/95 10/31/95 WATER Gross Beta (pCi/L) 4872.0 4823.33 -0.17 08/04/95 10/02/95 WATER Tritium (pCi/L)

-u 6_ .

• Each isotope measured by ESI was 14-33% higher than values reported by the U.S. EPA. When EPA published the results on 2/14/95, the ESI cross check sample had been disposed of. Because the EPA sample was inadvertently disposed, no follow-up action could be taken on that particulate sample. Since all measurements made by ESI were higher than the EPA values, it appears that a dilution error when preparing the sample was the cause for the discrepancy between ESI values and the EPA values. A new liquid standard was purchased from Analytics, Inc. in March 1995 and new efficiency curves were calculated using a 3.5 liter Marinelli geometry. There were no appreciative differences between the efficiency curves calculated before and after the Nov 4,1994 cross-check sample was analyzed. A 3.5L resin standard prepared by Analytics, Inc. was analyzed, resulting in efficiency curves which were approximately 90 percent as efficient as deiomzed water. 7hese results are theoreucally in agreement since the Analytics, Inc. resin standard has a density of 1.15 kg/L. No data from gamma wa%

would be affected by this apparent dilution error.

17 l

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3.0 DISCUSSION OF RESULTS i

Analytical results for the year 1995 are discassed in this section by exposure pathway, sample type, and analysis performed. Further, analytical results

focusing only on man-made radioactivity are summarized in Appendix A; data for the individual analyses are presented in the tables of Appendix B.

i j 3.1 Direct Radiation Exposure Pathway The average exposure rates measured by thermoluminscent dosimeters (TLDs) at both control and indicator stations were 13,12,13, and 12

mrem / standard quarter for the first, second, third, and fourth quarters of

- 1995, respectively. The average exposure rate of the 120 indicator TLD l locations was 13 mrem / standard quarter compared to 11 mrem / standard quarter average exposure rate at the control location. The lowest and highest individual exposure rates were 8 mrem / standard quarter (C-1,2nd and 3rd quarters) and 19 mrem / standard quarter (P-8,1st quarter) for all locations. Table 3.1 compares the indicator TLD results by directional sector and distance from the facility. A comparison of directional sectors

! Indicates the highest average exposure rate in 1995 to be 14 mrem / standard quarter in Sectors D, Q, and R.

The average exposure rates during 1995 are consistent with those from

! the pre-operational program and the previous five years of operation j i, (Figure 3.1). In particular, the pre-operational survey indicates that ,

exposure rates ranged between 11 and 33 mrem / standard quarter with an l average of 20 mrem / standard quarter. Similarly, the range indicated l during the previous five years of operation was from 7 to 23 j 1 mrem / standard quarter with an average exposure rate of 13 mrem / standard quarter.

l 3.2 Airborne Exposure Pathway 3.2.1 Airborne Porticulates to i

Gross beta activity ranged from 0.004 pCl/m (APG-1,7/11-7/18)for 0.035 pCl/m (APQ-1,4/25-5/2) with an average of 0.017 pCi/m 258 measurements from all five locations. The average gross beta

! activity for the indicator (APG-1, APQ-1 APP-1, APC-1) locations was 0.017 pCl/m compared to 0.016 pCi/m at the control (APE-j 30) location.

The gross beta activity results obtained during 1995 are consistent l with those from the pre-operational program and the previous five

years of operation (Figure 3.2). Specifically, the pre-operational i l

i l

I 21 4

, . - - . . . . . -- _ - - - - ~ - - - -- .. - . - - . .

1 L i

survey indicates that in periods not significantly influenced by 4

nuclear weapons testing the gross beta activity ranged between  !

0.007 and 0.48 pCi/m with an average of .08 pCi/m'. Similarly, the i range indicated during theprevious five years of operation was i from 0.004 to 0.039 pCi/m with an average activity of 0.017 ,

j pCi/m'. l l 3.2.2 Airbome lodine l 3

l All of the 258 airbome iodine-131 results were below the calculated 2 lower limit of detection (LLD). The sample LLD variability (0.012 to O.032 pCi/m8 ) was due primarily to the difference in air sample i 4 volumes. i f 3.2.3 Gamma Isotopic Analysis i

f Gamma spectroscopy results of the twenty air sample quarterly i

composites indicate that no man-made radionuclides were i

detected above their respective lower limits of detection. )

3.3 Waterborne Exposure Pathway 3.3.1 Drinking / Surface Water l

^

As mentioned previously, drinking water samples also serve as surface water samples for Waterford 3. Therefore, monthly and quarterly gamma spectroscopy analyses of drinking water and quarterly tritium analyses also satisfy the surface water sampling requirement.

! Seventy-eight composite drinking / surface water samples were l analyzed by gamma spectroscopy for iodine-131 (Table B-4). All of 4

the 78 composite sample iodine-131 results were below the  !

calculated lower limit of detection (LLD). j j

~

Gross beta activity was detected in thirty-six of the forty-two composites with a range of 1.3 (DWE-5,2/21-3/21) to 12.1 (DWG-

2,1/24-2/21) pCi/l and an average activity of 3.9 pCi/l. The average <

E activity for the control location, DWP-7, was 3.7 pCi/i compared to i

the averages of 4.9 and 3.2 pCi/l for indicator stations DWG-2 and i DWE-5, respectively. 1 Analyses for gross beta in drinking / surface water were not 1 performed during the pre-operational survey. However, in order to '

fulfill comparison requirements,1995 data will be compared to data from the 1983 report and the previous five years of operation.

1 b

4 22

p i- '

The gross beta activity results obtained during 1995 are consistent 4

with those from the 1983 reporting period and the previous five years of operation (Figure 3.3). In particular, the 1983 survey indicates that in peilods not significantly influenced by nuclear weapons testing the gross beta activity ranged between 2.9 and 14.0 pCill with an average of 7.0 pCl/l. Similarly, the range indicated during the previous five years of operation was from 1.1 l to 12.4 pCi/l with an average activity of 4.4 pCi/l.

Tritium analysis of drinking / surface water samples indicate that all t

of the twelve measurements were below the calculated LLD.

3.3.2 Groundwater

- Four groundwater samples were collected from one sampling

location, GWK-1, and analyzed for tritium and gamma emitters.

Results from all gamma and tritium analyses indicate that all

measurements were below the calculated LLDs.

a The tritium concentrations detected in 1995 are consistent with those from the pre-operational program and the previous five years of operation. In particular, the pre-operational survey indicates that

!- tritium concentrations in groundwater samples ranged between 50

and 180 pCl/l with an average of 121 pCi/l. Similarly, the range indicated in the previous five years of operation was from 270 to j 650 pCl/l.

3.3.3 Shoreline Sediment Four shoreline soil samples were collected from the following i sampling locations: two samples from the Mississippi River shoreline downriver of the plant (SHWE-3) and two samples from j the shoreline of a drainage canal (SHWK-1).

i

! Naturally occurring radionuclides including potassium-40, radium-226, and actinium-228 were detected in all of the samples.

1 Cesium-137, a man-made nuclide was detected in samples from i station SHWK-1 at concentrations of 31 and 34 pCi/kg (dry) and

from SHWE-3 at concentrations of 44 and 45 pCi/kg (dry). No l other man-made radionuclides were detected in any of the samples. ].

The cesium-137 results obtained during 1995 are consistent with

.those from the pre-operational program and the previous five years  ;

i of operation, in particular, the pre-operational survey indicates that i

cesium-137 was detected in 9 of 14 soil samples at concentrations 23

- - - _ . - . - -.--= . . _ - - . . . -- .

l

. ranging between 30 and 890 pCi/kg(dry) with an average concentration of 164 pCi/kg (dry). Similarly, the range indicated

~

during the previous five years of operation was from 18 to 66 i pCi/kg (dry) with an average activity of 45 pCi/kg (dry). Further, i studies in Louisiana indicate that cesium-137 is commonly found in

, soils and sediments as a result of atmospheric weapon testing.

! Because the cesium-137 levels are consistent with pre-operational -  ;

l values, the cesium-137 levels detected in 1995 are more than likely

! attributable to weapon testing fallout.

1 2 3.4 Ingestion Exposure Pathway 3.4.1 Milk Forty-eight milk samples were collected from two sampling locations and j analyzad by gamma spectroscopy and a radiochemical procedure for j iodine-131. Naturally occurring potassium-40 was detected in all i samples. Results from iodine-131 analyses indicate thaf. all i measurements were below the calculated LLD. Further, cesium-137 was i detected in two control samples (MKQ-45,7/18 and 10/17) at l concentrations of 2.0 and 3.0 +/- 2.0 pCi/l. However, the levels of cesium-j in these control samples are below both the reporting levels and the LLD j- required by the Waterford 3 ODCM and have a high level of statistical

uncertainty associated with them.

3.4.2 Fish

! Sixteen fish samples, eight upstream and eight downstream of the j

plant were collected and the edible portions analyzed by gamma l l spectroscopy. Only naturally occurring potassium-40 was detected

above the lower limits of detection in any samples.

i 3.4.3 Broad Leaf Vegetation l

Thirty-six broad leaf vegetation samples were collected and l analyzed by gamma spectroscopy and a radiochemical procedure j for iodine-131. Naturally occurring radionuclides were detected in

! all of the samples; however, no man-made radionuclides were j detected above their calculated LLDs.

I

3.4.4 Food Products

) Two food products samples were collected and analyzed by

gamma spectroscopy and a radiochemical procedure for iodine-131. Naturally occurring potassium-40 was detected in all the l samples; however, no man-made radionulides were detected i above their calculated LLDs.

24

. .__ ._ _ . ~. ___ _ -

4 4

f 3.5 Statistical Analyses 3.5.1 Calculation of the Mean and Standard Deviation The mean and standard deviation for different groups of analyses are calculated using the following equations:

i (F-1) <

2=f5 s. n (F-2) f o, 8 03

[ (X, - XJ' s- ~

i (n-1) i where:

x = mean of sample population, s = standard deviation of sample population, n = number of samples in sample population, and  :

x i = value of the i'th sample.

3.5.2 Comparing Two Sample Population Means

, The means of two sample populations are compared for statistical )

difference using the standard "t" test. The use of the test requires i the assumption that the data within the populations are normally I distributed and that the true standard deviations of the mean are i equal for both populations. The standard "t" test tests the hypothesis that the true means of both populations are equal. The "t" value can be calculated from the equation below (obtained from the CRC Standard Mathematical Tables,26th Edition (1981)). <

l (F-3) l T - T' t=

,- I)S, + h,- I , 1

n. + n, - 2 , < n. n,,

8

)

25 l 1

Q where:

t = calculated "t".value, -

x = mean of first data set, -

y = mean of second data set, n , = number of variables in first data set, s , = standard deviation of first data set, .

n y= number of variables in second data set, and j s y= standard deviation of second data set.

1 The calculated "t" value is used to test the hypothesis that the true mean of the first population (m ,) is equal to the true mean of the

second population (m y) assuming that the true standard deviations

. _of both populations are equal (m , = my ). The calculated "t" value is compared to a tabular "t" value such that:

a. if t > t p,n then reject the hypothesis when m y > m y,

b. if t < -t p,n then reject the hypothesis when m , < my,

c. if t > t pa,n then reject the hypothesis when m , = my ,

where t pa,n and t p,n are the tabular "t" values, with a

preselected error (5%), confidence level (1 - p) or (1 -

p/2), and degrees of freedom n (n=n ,+ny-2 for '

Equation F-3 and n=N-1 for F-4, respectively). I Tabular values of the "t" were obtained from the CBC Standard Mathematical Tables. 26th Edition (1981).

3.5.3 TLD Measurements i TLD stations were categorized by distance into three groups: 0-2 i miles,2-5 miles, and >5 miles from the plant. A statistical analysis 4 using the standard "t" test (described above) was performed comparing average exposure rates from 0-2 miles and 2-5 miles to

! the average exposure rate at >5 miles. In short, results indicate l that the average exposure rates at 0-2 miles and 2-5 miles are statistically the same as the rates at >5 miles. Table 3.2 summarizes the results of this ant!ysis.

3.5.4 Gross Beta Activity on Air Particulate Filters Additionally, the standard "t" test was used to compare average

, gross beta activity from each indicator station to the average gross beta activity at the control station. The results from this test show average activity detected at all indicator stations (APG-1, APQ-1, APC-1, and APP-1) to be statistically the same as the activity l 26

1 detected at the control station. Table 3.3 summarizes the results of-this analysis.

j 3.5.5 Gross Beta Activity in Monthly Drinking Water Composites Finally, t'he standard "t" test was used to compare average gross beta activity from the two indicator stations to the average gross beta activity from the control station. The results from this test

- show average activity at indicator stations (DWG-2 and DWE-5) are statistically the same as the average activity detected at the control station. Table 3.4 summarizes the results of this analysis.

3.6 Deviations from the REMP

3.6.1 Unavailable Samples Two air samples were missed during the 1995 reporting period.

One of the air samples was unavailable because the air sample

heads were inadvertantly switched, while the other sample was missed due to a disconnection in the sample line.

'- Milk samples were not available during 1995 from the animal owners at station MKQ-1 since the cows are not currently  ;

4 producing milk for human consumption. With the absence of milk  !

samples at these stations, broad leaf vegetation sampling was P performed. These results are summarized on Table 3.5.

3.6.2 Lack of Sample Continuity Two air samples failed to meet the requirement for sample continuity as a result of air sample pump failures, l i 3.6.3 Missed Lower Limits of Detection All lower limit of detection requirements were met for 1995.

3.7- Annual Land Use Census 1

)

In compliance with Waterford 3 ODCM, the annual land use census was conducted on August 23,24, and 25,1995. The nearest residence,

. garden, and milking animalin each sector within a five mile radius of the plant were located by visual inspection and verbal inquiry.

I While residence locations remained unchanged for 1995, minor changes in garden locations were observed as recorded on Table 3.6. Additionally, large tracts of sugar cane are still being cultivated near the plant and remain classified as food products.

27 l

4  !

One new location for milk cows and one new location for goats was identified; however, in all cases it was determined that the animals are not currently producing milk for human consumption. This information was ascertained by verbalinquiry with the owners of the animals. As a result of the interviews, Waterford 3 personnel obtained a verbal agreement that the animal owners will sell milk samples to Waterford 3 in the event of a radiological emergency to provide additional data for analysis of environmentalimpact i

1 1

l 28

i

. l l

. TABLE 3.1

! 1995 DIRECT RADIATION DATA -  !

ORGANIZED BY COMPASS DIRECTION i

AND DISTANCE FROM WATERFORD 3 SES i BY COMPASS DIRECTION 1

SECTOR COMPASS AVERAGE STANDARD NUMBER i DIRECTION DOSE RATE - DEVIATION IN (mrem /std qtr) (mrem /std qtr) GROUP A N 13 1.00 8

) B NNE 13 0.99 8 i C NE 9 0.83 4

! D ENE 14 2.44 8 i E* E 12 0.86 12

F ESE 13 1.37 12 l G SE 12 1.93 12 i

H SSE 13 1.39 8

J S 13 1.62 8 K SSW 12 2.28 4 L SW 12 1.92 4

! M WSW 12 0.83 4

, N W 13 2.12 4 l P WNW 12 2.82 8

Q NW 14 1.56 8 R NNW 14 3.08 8 i CONTROL E 11 1.12 4 j BY DISTANCE FROM PLANT 1

' DISTANCE AVERAGE STANDARD NUMBER FROM PLANT DOSE RATE DEVIATION IN (MILES) (mrem /std qtr) (mrem /std qtr) GROUP  ;

0-2 12 2.14 64 f 2-5 13 1.52 28 5* 13 2.28 28 CONTROL 11 1.12 4

• Does not include control station data.

]

i 29

TABLE 3.2 -

STATISTICAL COMPARISON OF 1995 TLD MEASUREMENTS FROM STATIONS GROUPED BY DISTANCE FROM WATERFORD 3 SES Stations Located 0-2 Stations Located 2-5 Stations Located more than 5 Miles from the Plant Miles from the Plant Miles from the Plant Mean 12.44(12) 12.89(13) 12.82(13)

(mrem /std.qtr.)

Standard Deviation 2.14 1.5229 2.28 (mrem /std. qtr.)

Number in Sample 64 28 28 Calculated "t" Value to 0.78 0.14 NA*

Comparisons with Stations Located more than 5 miles from the Plant Tabular "t" Value at 1.986(a) 2.006(a) NA*

95% Confidence (to.o2s.n) ,

a. Results indicate that the means for stations located 0-2 miles and 2-5 miles from the plant means are statistically identical  ;

to the mean for stations located more than 5 miles from the plant.

• Not Applicable 30

TABLE 3.3 STATISTICAL COMPARISON OF 1995 GROSS BETA ACTIVITY MEASUREMENTS ON AIR PARTICULATE FILTERS FROM WATERFORD 3 SES SAMPLE STATION APC-1 APG-1 APP-1 APQ-1 APE-30 Mean 17.1 16.6 15.0 17.9 16.4 (10pCi/m8)

Standard Deviation 5.33 5.87 4.82 5.87 5.42 (104pCi/m')

Number in Sample 52 50 52 52 52 Calculated "t" Value 0.67 0.20 1.38 1.41 NA*

Comparing Control Station ,

(APE-30) to Indicator l Station Tabular "t" Value at 1.986(a) 1.987(a) 1.986(a) 1.986(a) A'fl 95% Confidence (to.o2s,n)

a. Results indicate that the means for indicator stations APC-1, APG-1, , APP-1, and APQ-1 are statisF.; ally identical to mean for the control location APE-30.

• Not Applicable 31

_ _ _ . _ _ _ _ . . . .. _ _ _.___._ ._._ _ . _ _ - =

l TABLE 3.4 STATISTICAL COMPARISON OF 1995 GROSS BETA ACTIVITY MEASUREMENTS IN DRINKINGISURFACE WATER SAMPLES FROM WATERFORD 3 SES DWG-2 DWE-5 ' DWP-7 l

Mean 4.9 3.2 3.7 (pCilliter)

Standard Deviation 3.7 1.3 1.3 (pCilliter)

Number in Sample 12 11 12 Calculated "t" Value to 1.01 1.03 NA*

Comparing Control Station DWP-7 to Indicator Station Tabular "t" Value at 2.074(a) 2.080(a) NA*

95% Confidence (to.o2s.n)

a. Results indicate that the means for indicator stations DWG-2 and DWE-5 are statistically identical to mean for the control location DWP-7.

• Not Applicable 32

i TABLE 3.5

SUMMARY

OF 1992 REMP DEVIATIONS SAMPLE TYPE ANALYSIS LOCATION DATE - EXPLANATION OF DEVIATION -

MISSED SAMPLES l

l 1. Air Gross Beta & I-131 APG-1 04/18/95 - 04/25/95 Sample head switched.

2. Gross Beta & I-131 APG-1 06/13/95 - 06/20!95 Sample line disconnected.

LACK OF SAMPLE CONTINUITY

1. Air Gross Beta & l-131 APQ-1 05/02/95- 05/10/95 Sample pump failure - replaced.

i 2. Gross Beta & 1-131 APE-30 06/13/95 - 06/20/95 Sample pump failure - replaced.

MISSED LLDs NONE N/A* N/A* N/A* N/A*

• Not Applicable 33

\

l l

TABLE 3.6 1995 ANNUAL LAND USE CENSUS RESULTS SECTOR DIRECTION DISTANCE FROM PLANT IN MILES BEEF MILK MILK FOOD COW COW GOAT GARDEN RESIDENCE PRODUCTS ;

) A N - - -

1.7 1.3 4.1 B NNE - - -

1.3 1.1 -

C NE - - -

0.9 0.9 -

D ENE - - -

0.9 0.9 -

l E E 2.3 3.2* 2.3* 2.2 2.2 0.3 F ESE 2.3 3.5 -

2.2 3.1 0.3

G SE 2.4 - -

4.1 4.0 0.3 H SSE - - - - -

0.3 J S - - - - -

0.5 K SSW - - - - -

0.5 L SW - - - - -

0.5 ,

M WSW 1.0 - -

1.4 -

0.5 j N W - - -

1.1 1.0 0.6 I i-P WNW 0.9 -

0.9 0.9 0.9 0.5 O NW 0.9 4.9'* -

0.9 0.9 0.5 R NNW 4.9 - -

3.0 3.0 2.6 l

None found in sector within five mile radius of the plant.

a Samples are being taken at 4.9 miles (MKQ-5) for the Waterford 3 REMP. -

l i b Cows at Location MKQ-1 are currently not producing milk for human consumption. The l owner will be contacted on a periodic basis to determine if milk will be used for human consumption and for the availability of samples. .

l 1

i e Milk animals at these locations are not currently producing milk for human consumption.

. The owners will be contacted on a periodic basis to determine if milk will be used for l human consumption and for the availability of samples.

i l

34

1

4.0 CONCLUSION

S

) The radiological environmental data collected during 1995 are consistent with the data

, obtained during the previous five years of plant operation (1990-94), the first two years of the REMP prior to Waterford 3 initial criticality (1983-84), and the Pre-operational Environmental Radiological Surveillance (PERS) Program (1978-82). The only man-made radionuclide detected in the environmental samples analyzed during 1995 was cesium-137, i Cesium-137 was detected in four shoreline soil samples. Studies in Louisiana indicate

that cesium-137 is commonly found in soils and sediments as a result of fallout from 3

nuclear weapons testing, in addition, the detected concentrations were consistent with j pre-operational levels and the levels detected in the previous five years of operation.

Further, the concentrations detected in both instances were lower than the required LLD and well below levels requiring notification.

l Analyses of milk samples indicated cesium-137 in two samples collected from the

control location in July and October of 1995. The activity detected in both instances

! was at levels below the required LLD and well below reporting levels defined in the i Waterford 3 ODCM. In addition, cesium-137 concentrations detected in 1995 milk samples are consistent with the levels indicated in the pre-operational program and the levels detected in the previous five years of operation. Further, statistical errors l- associated with the indicated concentrations are higher than would be expected with j true activity and may be artifacts of counting statistics.

i~ In conclusion, based on the evaluation of the REMP data collected during 1995 the

operation of Waterford 3 had no discernable radiological impact on the environment.

1 J

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e b

TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

Name of Facility Waterford 3 SES Docket No. 50-382 January 1 to Location of Facility St Charles. Louisiana Reporting Penod December 31.1995 (Parish, State)

MEDIUM OR PATHWAY ANALYSIS AND LOWER LIMIT ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL MEAN CONTROL NUMBER OF SAMPLED TOTAL NUMBER OF MEAN" NAME MEAN" LOCATION NONROUTINE (UNIT OF OF ANALYSES DETECTION * (RANGEf DISTANCE AND DIRECTION (RANGE)* MEAN* REPORTED MEASUREMENT) PERFORMED (LLD) (RANGEf MEASUREMENTS

1. Dired Radiation TLD 120 (c) 12(11G/116) P-6 19(4/4) E-30 0 (mrem /Std. qtr.) (8-19) 5.5 miles WNW (11-19) 11(4/4)

(9-12)

2. Airbome Gross 258 10 17(206/206) APQ-1 18(52/52) APE-30 0 Particulates Beta (4-35) 0.5 miles SE (8-35) 16(52/52)

(10*pCi/m*) (6-33)

Gamma 20 (d) <LLD (0/16) N/A t&A APE-30 0

(-) <LLD (0/4)

(-)

3. Airbome I-131 258 70 <LLD (0/206) N/A N/A APE-30 0 lodine (-) <LLD (0/52)

(10*pCi/m') (-)

NOTE- Footnotes at end of table.

39

TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

Name of Facirrty Waterford 3 SES Docket No. 50-382 January 1 to Location of Facility St. Charles. Louisiana Reporting Penod December 31.1995 (Parish, State)

MEDIUM OR PATHWAY ANALYSTS AND LOWER LIMIT ALL IPOCATOR LOCATIONS LOCATK)N W TH HIGHEST ANNUAL MEAN CONTROL NUMBER OF SAMPLED TOTAL NUMBER OF MEAN* NAME MEAN" LOCATK)N NONROUTirE (UNIT OF OF ANALYSES DETECTION * (RANGEf DISTANCE AND DIRECTION (RANGEf MEAN* REPORTED MEASUREMENT) PERFORMED (LLD) (RANGEf MEASUREMENT S

4. Drinnung/ Surface Gross 42 4 4.0(23/28) DWG-2 4.9(12/14) DWP-7 0 Water (pCin) Beta (1.3-12.1) 2.0 miles SE (1.8-12.1) 3.7(12/14)

(1.8-5.5) 1-131 78 1 <tLD (0/52) N/A N/A DWP-7 0

(-) <LLD(0/26)

(-)

Gamma 42 (d) <tLD (0/28) N/A N/A DWP-7 0

(-) <LLD (0/14)

(-)

Tritium 12 2000 <tLD (0/8) N/A N/A DWP-7 0

(-) <LLD (0/4)

(-)

NOIE: Footnotes at end of table.

40

TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

Name of Facility Waterford 3 SES Docket No. 50-382 January 1 to Location of Facility St Charles. Louisiana Reporting Period December 31.1995 (Parish, State)

MEDfuM OR PATHWAY ANALYSIS AND LOWER LIMIT ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL MEAN CONTROL NUMBER OF SAMPLED TOTAL NUMBER OF MEAN* NAME MEAN* LOCATION NONROUTINE (UNIT OF OF ANALYSES DETECTION * (RANGE)* DISTANCE AND DIRECTION (RANGE)* MEAN* REPORTED MEASUREMENT) PERFORMED (LLD) (RANGE)* MEASUREMENTS

5. Groundwater lamma 4 (d) <LLD (0/4) N/A N/A NONE O (pCin) (-)

Tritium 4 2000 <LLD (0/4) N/A N/A NONE O

(-)

6. ShorelineWater Gamma 4 180 38(4/4) SHWE-3 45(2/2) NONE O Sedment Cs-137 (31-45) 3.0 miles E (44-45)

(pCiAg--dry)

NOTE: Footnotes at end of table.

41

_ _ _ ._. ._ _ . ._ _ _ . __ ._ _.m .

TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM SutMRARY Name of Facility Waterford 3 SES Docket No. 50-382 January 1 to Location of Facility St.Chartes Louisiana Reporting Period December 31.1995 (Parish, State)

MEDIUM OR PATHWAY ANALYSIS AND LOWER UMIT ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL MEAN CONTROL NUMBER OF SAMPLED TOTAL NUMBER OF MEAN" NAME MEAN* LOCATION NONROUTINE (UNIT OF OF ANALYSES DETECTION" (RANGE)* OtSTANCE AND DIRECTION (RANGE)* MEAN* REPORTED MEASUREMENT) PERFORMED (LLD) (RANGE)* MEASUREMENTS

7. Milk l-131 48 1 <LLD (0/24) N/A N/A MKO-45 0 (pCill) (-) <LLD (0/24)

(-)

Gamma 48 18 <LLD (0/24) MKO-45 N/A MKO-45 0 Cs-137 (-) 42.0 miles NW 3.0(2/24)

(2.0-3.0)

8. Fish Gamma 16 (d) <LLD (0/8) N/A N/A FH-1 0 (pCilkg-wet) (-) <LLD (0/8)

. (-)

NOTE: Footnotes at end of table.

42

'D i.

TABLE A-1 j RADIOLOGICAL ENVIRONARENTAL MONITORING PROGRAM SURRAARY Name of Facihty Waterford 3 SES Docket No. 50-382 January 1 to l Location of Facility St. Chartes. Louisiana Reportmg Period December 31.1995 (Parish, State)

MEDIUM OR PATHWAY ANALYSIS AND LOWER LIMIT ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST APNUAL MEAN CONTROL NUMBER OF SAMPLED TOTAL NUMBER OF MEAN* NAME MEAN* LOCATION NONROUTDE (UNIT OF OF ANALYSES DETECTION" (RANGE)* DISTANCE AND DIRECTION (RANGE)* MEAN* REPORTED MEASUREMENT) PERFORMED (LLD) (RANGE)* MEASUREnENTS

9. Broad Leaf I-131 36 60 <LLD (0/24) N/A N/A BLK-15 0

. Vegetabon (-) <LLD (0/12)

. (pCWg-wet) (-)

Gamma 36 (d) <LLD (0/24) N/A N/A BLK-15 0

(-) <LLD (0/12)

(-)

9. Food / Garden Crop Gamma 2 (d) <tLD (0/2) N/A N/A NONE O (pCWg- wet) (-)

NOTE- Footnotes at end of table.

i i

43

l TABLE A-1 (Cont.)

RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

FOOTNOTES aNominal Lower Limit of Detection (LLD) as defined in the Waterford 3 Offsite Dose Calculation Manual.

b Mean and range based upon detectable measurements only. Fraction of detectable measurements at specified locations is indicated in parenthesis.

c Lower Limit of Detection (LLD) not defined in Waterford 3 Offsite Dose Calculation Manual.

d Lower Limit of Detection (LLD) for individual radionuclides using gamma spectroscopy are given in Waterford 3 Offsite Dose Calculation Manual.

44

l l

't 1

4 4

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I I

I i

i J

e, 1

i APPENDIX B

!' REMP DATA I

e 4

f 1

A t

.f 4

4

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4 4

4

- 45 I

TABLE B-1 QUARTERLY TLD DOSE RATES LOCATION 1ST 2ND 3RD 4TH AVERAGE QUARTER QUARTER QUARTER QUARTER DOSE RATE DOSE RATE DOSE RATE DOSE RATE DOSE RATE (mrem /std qtr) 4 (mrem /std qtr) (mrom/std qtr) (mrom/std qtr) (mrem /std qtr)

A-2 13 12 15 13 13 A-5 13 12 14 12 13 B-1 14 13 14 12 13 B-4 15 12 14 13 14 C-1 10 8 8 9 9 D-2 12 19 15 13 15 D-5 14 14 13 10 13 E-1 13 10 12 11 12 i E-5 12 12 12 12 12 E-15 12 10 11 12 11 E-30 12 11 10 9 12 F-2 14 11 15 10 13 F-4 13 13 14 13 13 l, F-9 13 12 13 11 12 G-2 16 14 16 13 15

G4 12 11 11 10 11

,' G-9 11 11 11 12 11 H-2 14 14 13 14 14 l H-6 13 11 13 10 12 i J-2 13 11 16 12 13 l J-15 14 14 14 11 13

! K-1 16 10 12 11 12

! L-1 11 10 13 15 12

, M-1 12 11 13 11 12 N-1 15 10 15 12 13 P-1 11 10 12 10 11 P-6 19 11 14 11 14 Q-1 12 12 13 13 13 Q-5 15 13 16 16 15 R-1 14 9 11 10 11 R-6 15 17 18 15 16 Average 13 12 13 12 13 46

TABLE B-2 l AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES GROSS BETA AND IODINE-131 ANALYSES SAMPLE LOCATION: APC-1 UNITS: pCi/ CUBIC METER LAB NO. BEGIN DATE END DATE GROSS BETA l-131 LAB NO. BEGIN DATE END DATE GROSS BETA l-131 9500069 12/27/94 01/03/95 0 022 +/-0.002 < 0.024 9513914 06/27S 5 07/03/95 0.011 +/-0.002 <0.028 9500670 01/03SS 01/10/95 0.027 +/-0 003 < 0.032 9514347 07/03/95 07/11/95 0.017 +/-0.002 < 0.019 9500912 01/10/95 01/17/95 0 024 +/-0.002 < 0.021 9514968 07/11/95 07/18/95 0.014 +/-0.002 < 0.014 9501383 01/17/95 01/24/95 0.022 +/-0.002 <0.027 9515403 07/18/95 07/25/95 0.012 +/-0.002 < 0.020 9501722 01/24/95 01/3165 0.016 +/-0 002 < 0.018 9516253 07/25S 5 08S1/95 0.006 +/-0.002 < 0.016 9502204 01/31/95 02/07 S 5 0.017 +/-0.002 < 0.024 9516679 08/01/95 08/08/95 0 012 +/-0.002 < 0.018 9502898 02!O7/95 02/14/95 0.015 +/-0.002 < 0.021 9517614 08/08/95 08/15/95 0.012 +/-0.002 < 0.023 9503381 02/14/95 02/21/95 0.012 +/-0.002 < 0.023 9518264 08/15 S 5 08/22 S 5 0.017 +/-0.002 <0.023 9503702 02/21/95 02/27/95 0.014 +/-0.002 < 0.030 9518863 08/22/95 08/29/95 0.020 +/-0.002 <0.017 9504190 02/27S 5 03/07/95 0.021 +/-0 002 <0.019 9519476 08/29/95 09/05/95 0.022 +/-0.003 < 0.025 9504612 03/07SS 03/14/95 0.018 +/-0.002 < 0.024 9520279 09/05/95 09/12/95 0.024 +/-0.003 < 0.023 9505239 03/14/95 03/21/95 0.014 +/-0.002 < 0.021 9520491 09/12/95 09/19/95 0.013 +/-0.002 <0.022 9505673 03/21/95 03/28/95 0.019 +/-0.003 < 0.023 9520896 09/19/95 09/26/95 0.022 +/-0.002 < 0.014 9506221 03/28/95 04/04SS 0 023 +/-0 002 < 0.021 9521414 09/26 S 5 10/03/95 0.030 +/-0.003 < 0.021 9506945 04/04/95 04/11/95 0 019 +/-0.002 < 0.025 9522110 10/03/95 10/10/95 0.019 +/-0.002 < 0.024 9507520 04/11/95 04/1835 0 020 +/-0.002 <0.022 9522653 10t10/95 10/17S5 0.020 +/-0.002 < 0.024 9508232 04/1845 04/25/95 0.017 +/-0.002 < 0.023 9522996 10/17S 5 10/24/95 0.012 +/-0.002 < 0.023 9523473 10/24/95 10/31/95 0.012 +/-0.002 < 0 026 9508692 04/25/95 05/02/95 0.014 +/-0.002 < 0.020 9509382 05/02/95 05/10/95 0 012 +/-0.002 < 0.024 9523888 10/31 S 5 11/07/95 0.012 +/-0.002 <0.027 9509674 05/10/95 05/16/95 0.011 +/-0.002 < 0.031 9524375 11/07/95 11/13/95 0.015 +/-0.002 < 0.030 9510361 05/16/95 05/23/95 0.010 +/-0.002 < 0.021 9525015 11/13/95 11/20/95 0.022 +/-0 002 < 0.029 9510734 05/23SS 05/30/95 0.014 +/-0.002 < 0.012 9525281 11/20/95 11/27/95 0.024 +/-0.003 < 0.025 9511399 05/30 S5 06/06/95 0.012 +/-0.002 <0019 9525655 11/27S 5 12/04/95 0.018 +/-0.002 <0.024 9512035 06/06/95 06/13/95 0.012 +/-0.002 < 0.032 9525818 12/04/95 12/11/95 0.029 +/-0.003 <0023 9512685 06/13/95 06/20/95 0.016 +/-0.002 < 0.018 9526532 12/11/95 12/18/95 0.008 +/-0.002 < 0.019 9513235 06/20/95 06/27/95 0.020 +/-0.002 < 0.019 9526792 12/18/95 12/27/95 0.024 +/-0.002 < 0.017 47

I O

TABLE B-2 AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES GROSS BETA AND IODINE-131 ANALYSES i

SAMPLE LOCATION: APG-1 UNITS: pCi/ CUBIC METER LAB NO. BEGIN DATE END DATE GROSS BETA l-131 LAB NO. BEGIN DATE END DATE GROSS BETA I-131 9500066 12/27 S 4 01/03/95 0.020 +/-0.002 < 0.024 9513911 06/27SS 07/03/95 0.010 +/-0.002 <0.028 4 9500667 01/03/95 01/10/95 0.025 +/-0 002 <0032 9514344 07/03/95 07/1185 0.015 +/-0.002 < 0.019 9500909 01/10/95 01/17S 5 0.020 +/-0 002 < 0.021 9514965 07/11/95 07/18/95 0.004 +/-0.002 <0.014 9501380 01/17/95 01/24/95 0.019 +/-0.002 < 0.027 9515400 07/18/95 07!25/95 0.011 +/-0.002 < 0.020 9501719 01/24 S 5 01/31/95 0 018 +/-0.002 < 0.018 9516250 07/25/95 08/01S5 0.006 +/4 002 <0016 9502201 01/31/95 02/07 S 5 0.028 +/-0.003 < 0.024 9516676 08/01/95 08/08SS 0.013 +/-0.002 <0.018 9502895 02/07/95 02/14/95 0.015 +/-0.002 < 0.021 9517611 08/08SS 08/15/95 0.011 +/-0.002 < 0.023 9503378 02/14/95 02/21/95 0.012 +/-0 002 < 0.023 9518261 08/15/95 08/22/95 0.016 +/-0.002 < 0.023 9503699 02/21 S 5 02/27/95 0.014 +/-0.002 < 0.030 9518860 08/22 S 5 08/29/95 0.019 +/-0.002 < 0. 017 9504187 02/27/95 03/07/95 0.019 +/-0.002 < 0.013 9519473 08/29/95 09/05/95 0.024 +/-0.003 < 0.025 9504609 03/07/95 03/14/95 0.019 +/-0.002 < 0.024 9520276 09/05/95 09/12/95 0.025 +/-0.003 < 0.023 9505236 03/14/95 03/21 S 5 0.016 +/-0.002 < 0.021 9520488 09/12/95 09/19/95 0.013 +/-0.002 <0.022 9505670 03/21/95 03/28/95 0.016 +/-0.003 < 0.023 9520893 09/19/95 09/26/95 0.022 +/-0.002 < 0.014 9506218 03/28/95 04/04/95 0.020 +/-0 002 < 0.021 9521411 09/26/95 10/03/95 0 028 +/-0.003 < 0.021 9506942 04/04/95 04/11 S 5 0.016 +/-0.002 < 0.025 9522107 10/03/95 10/10 S 5 0.019 +/-0.002 <0.024 9507517 04/11/95 04/18!95 0.020 +/-0.002 < 0.022 9522650 10/10/95 10/17/95 0.016 +/-0.002 < 0.024 9508229 04/18/95 04/25/95 N/A N/A 9522993 10/17/95 10/24/95 0.013 +/-0.002 < 0.023 9523470 *0/24/95 10/31 S 5 0.013 +/-0.002 < 0.026 9508689 04/25/95 05/02 S 5 0 020 +/-0.003 < 0.020 9509379 05/02/95 05/10/95 0.010 +/-0.002 < 0.024 9523885 10/31/95 11/07/95 0.012 +/-0.002 < 0.027 9509671 05/10/95 05/16/95 0.011 +/-0 002 < 0.031 9524372 11/07/95 11/13/95 0.020 +/-0.002 < 0.030 9510358 05/16/95 05/23/95 0 010 +/-0.002 < 0.021 9525012 11/13/95 11/20/95 0.020 +/-0.002 < 0.029 9510731 05/23/95 05/30/95 0.014 +/-0.002 < 0.012 9525278 11/20/95 11/27!95 0 021 +/-0.002 < 0.025 9511396 05/30/95 06/06/95 0.011 +/-0.002 < 0.019 9525652 11/27/95 12/04SS 0.017 +/-0.002 <0.024 9512032 06/06/95 06/13/95 0.014 +/-0.002 < 0.032 9525815 12/04SS 12/11/95 0.024 +/-0.003 <0.023 9512682 06/13/95 06/20/95 N/A N/A 9526529 12/1185 12/18/95 0.010 +/-0.002 < 0.019 9513232 06/20/95 06/27/95 0.020 +/-0.002 <0019 9526789 12/18/95 12/27S 5 0 020 +/-0.002 <0017 48

TABLE B-2 (continued)

AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES GROSS BETA AND IODINE-131 ANALYSES SAMPLE LOCATION: APP-1 UNITS: pCi/ CUBIC METER LAB NO. BEGIN END DATE GROSS BETA l-131 LAB NO. BEGIN END DATE GROSS BETA I-131 DATE DATE 9500068 12/27/94 01/03 S 5 0 017 +/-O 002 < 0.024 9513913 06/27 S 5 07/03S5 0.010 +/-0.002 < 0.028 9500669 01/03/95 01/10 S 5 0.022 +/-0.002 < 0.032 9514346 07/03SS 07/11/95 0.014 +/-0 002 <0019 9500911 01/10/95 01/17 S 5 0 018 +/-0 002 < 0.021 9514967 07/11/95 07/1&95 0.013 +/-0 002 < 0 014 9501382 01/17/95 01/24SS 0 015 +/-0.002 <0027 9515402 07/1&95 07/25/95 0.009 +/-0.002 <0020 9501721 01/24SS 01/31 S 5 0.016 +/-0 002 < 0.018 9516252 07/25SS 08/01/95 0 005 +/-O 002 <0016 9502203 01/31/95 02/07S 5 0.018 +/-0.002 < 0.024 9516678 08/01 S 5 O&O8/95 0.009 +/-0.002 < 0.018 9502897 02/07/95 02/14SS 0 015 +/-0 002 <0021 9517613 08/08S 5 08/15/95 0 011 +/-C 002 < 0.023 9503380 02/14/95 02/21/95 0.011 +/-0.002 <0023 9518263 08/15/95 08/22/95 0.013 +/-0.002 < 0.023 9503701 02/21/95 02/27/95 0.014 +/-0 002 < 0 030 9518862 08/22/95 0&'29S5 0.019 +/-0.002 < 0. 017 9504189 02/27/95 03 S 7/95 0.016 +/-0.002 < 0.019 9519475 06/29/95 09/0595 0.021 +/-0.003 < 0.025 9504611 03/07/95 03/14/95 0.018 +/-O 002 < 0.024 9520278 09/0595 09/12/95 0.023 +/-0.003 <0.023 9505238 03/14/95 03/21/95 0.015 +/-0.002 < 0.021 9520490 09/12/95 09/19/95 0.012 +/-0.002 < 0.022 9505672 03/21/95 03/28S5 0 016 +10 002 <0023 9520895 09/19/95 09/26/95 0.021 +/-0.002 < 0.014 9506220 03/2&95 04/04SS 0.019 +/-0.002 < 0.021 9521413 09/26/95 10/03/95 0.024 +/-0.002 < 0.021 9506944 04/04/95 04/11 S 5 0 018 +/-0 002 <0025 9522109 10/03/95 10/10/95 0.020 +/-0.002 < 0.024 9507519 04f11S5 04/1&95 0.017 +/-0.002 < 0.022 9522652 10/10/95 10/17/95 0.013 +/-0.002 < 0.024 9508231 04/18/95 04/2595 0 014 +/-0 002 < 0.023 9522995 10/17/95 10r24/95 0.011 +/-0.002 <0023 9523472 10/24/95 10/31/95 0.010 +/-0.002 <0026 9508691 04/25/95 05/02 S 5 0 010 +/-0.002 < 0.020 9509381 05/02/95 05/10/95 0.010 +/-0 002 < 0.024 9523887 10/3185 11/07/95 0.012 +/-0.002 < 0.027 9509673 05/10/95 05/1695 0.009 +/-0.002 < 0.031 9524374 11/07/95 11/13/95 0.015 +/-0.002 < 0.030 9510360 05/1695 05/23/95 0.010 +/-0 002 < 0.021 9525014 11/13/95 11/2a95 0.021 +/-0.002 <0029 9510733 05/23/95 05/30/95 0.011 +/-0.002 <0012 9525280 11/20/95 11/27SS 0.020 +/-0.003 < 0.025 9511398 05/30/95 06/06/95 0.011 +/-0 002 < 0.019 9525654 11/27/95 12/04/95 0 016 +/-0.002 < 0.024 9512034 06/0695 06/13/95 0 009 +/-0.002 <0032 9525817 12/04/95 12/11/95 0 030 +/-0.003 < 0.023 9512684 06/13/95 06/20/95 0.012 +/-0.002 <0018 9526531 12/11 S 5 12/18/95 0.010 +/-0.002 < 0.019 9513234 06/20/95 06/27/95 0 015 +/-0.002 < 0.019 9526791 12/18/95 12/27/95 0 021 +/-0.002 < 0.017 49

TABLE B-I ! continued)

AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES GROSS BETA AND IODINE-131 ANALYSES SAMPLE LOCATION: APQ-1 UNITS: pCi/ CUBIC METER LAB NO. BEGIN END DATE GROSS BETA l-131 LAB NO. BEGIN END DATE GROSS BETA 1-131 DATE DATE 9500067 12/27 S 4 01/03/95 0 020 +/-0.002 < 0.024 9513912 06/27/95 07/03/95 0.011 +/4 002 < 0.028 9500668 01/03/95 01/1065 0.027 +/-0.003 < 0.032 9514345 07/03/95 07/11/95 0.019 +/-0 002 < 0.019 9500910 01/10/95 01/17/95 0.022 +/-0.002 < 0.021 9514966 07/11/95 07/18SS 0.013 +/-0.002 < 0.014

, 9501381 01/17/95 01/24/95 0.020 +/-0.002 < 0.027 9515401 07/18/95 07/25/95 0.012 +/-0.002 <0.020 1

9501720 01/24/35 01/31/95 0.018 +/-0.003 <0018 9516251 07/25/95 08/01 S 5 0.008 +/-0.002 <0.016 9502202 01/31/95 02/07/95 0.022 +/-0.003 < 0.024 9516677 08/01 S 5 08/08 S 5 0.015 +/-0.002 < 0.018 9502896 02/07/95 02/14/95 0 016 +/-0.002 < 0.021 9517612 08/08/95 08/15/95 0 012 +/-0.002 < 0.023 9503379 02/14/95 02/21/95 0.012 +/-0.002 < 0.023 9518262 08/15/95 08/22/95 0.016 +/-0.002 <0.023 337t10 02/21/95 02/27/95 0.015 +/-0.002 < 0.030 9518861 08/22 S 5 08/29/95 0.018 +/-0.002 < 0. 017 9504188 02/27/95 03/07/95 0.019 +/-0.002 < 0.019 9519474 08/29/95 09/05/95 0.025 +/-0.003 <0.025 9504610 03/07 S 5 03/14/95 0 019 +/-0 002 < 0.024 9520277 09/05/95 09/12 S 5 0 023 +/-0.003 < 0.023 9505237 03/14/95 03/21/95 0.019 +/-0.002 < 0.021 95204ts9 09/12/95 09/19/95 0.014 +/-0.002 < 0.022 9505671 03/21/95 03/28/95 0.020 +/-0.003- < 0.023 9520894 09/19/95 09/26/95 0.024 +/-0.003 < 0.014 9506219 03/28/95 04/04/95 0.022 +/-0.002 < 0.021 9521412 09/26 S 5 10/03/95 0.030 +/-0.003 < 0.021 9506943 04/04/95 04/11/95 0.018 +/-0.002 < 0.025 9522108 10/03/95 10/10/95 0.022 +/-0.002 < 0.024 1 l

9507518 04/11/95 04/18/95 0 022 +/-0.003 < 0.022 9522651 10/10/95 10/17/95 0.017 +/-0.002 < 0.024 9508230 04/18/95 04/25/95 0.016 +/-0.002 < 0.023 9522994 10/17/95 10/24/95 0.014 +/-0.002 < 0.023 9523471 10/24 S 5 10/31/95 0.012 +/-0.002 < 0.026 9508690 04/25/95 05/02/95 0.035 +/-0.003 < 0.020 9509380 05/02/95 05/10/95 0.013 +/-0.002 < 0.024 9523883 10/31/95 11/07/95 0.013 +/-0.002 <0.027 9509672 05/10/95 05/16/95 0.013 +/-0.002 < 0.031 9524370 11/07/95 11/13/95 0.015 +/-0.002 < 0.030 9510359 05/16/95 05/23/95 0.010 +/-0.002 < 0.021 952501'4 11/13/95 11/20/95 0.021 +/-0.002 < 0.029 I l 9510732 05/23/95 05/30/95 0.014 +/-0.002 < 0.012 95252b *1/20/95 11/27/95 0.023 +/-0.003 <0.025 J l

95;1397 05/30/95 06/06/95 0.010 +/-0.002 < 0.019 9525653 11/27/95 12/04/95 0.017 +/-0.002 <0.024 9512033 05/06/95 06/13/95 0.011 +/-0 002 < 0.032 9525816 12/04/95 12/11/95 0.033 +/-0.003 < 0.023 9512683 06/13/95 06/20/95 0.014 +/-0.002 < 0.018 9526530 12/11/95 12/18/95 0.010 +/-0.002 < 0.019 9513233 06/20/95 06/27/95 0.024 +/-0.002 < 0.019 9526790 12/18/95 12/27/95 0 024 +/-0.002 < 0.017 l 50 1

- . _ _ _ . ~ _ _ _ _ _ _ - _ _ - - . _ _ _ . _ . - . .

. . \

TABLE B-2 (continued)

AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES GROSS BETA AND IODINE-131 ANALYSES SAMPLE LOCATION: APE-30 UNITS: pCitCUBIC METER LAB NO. BEGIN END DATE GROSS BETA l-131 LAB NO. BEGIN END DATE GROSS BETA l-131 9500070 12/27/94 01/03/95 0.019 +/-0.002 <0.024 S513915 06/27/95 07/03/95 0.009 +/-0.002 <0028 9500671 01/03/95 01/10/95 0.025 +/-0.002 < 0.032 9514348 07/03/95 07/11/95 0.020 +/-0.002 <0019 9500913 01/10/95 01/17/95 0.020 +/-0.002 <0.021 9514969 07/11/95 07/18/95 0.015 +/-0.002 < 0.014 9501384 01/17/95 01/24/95 0.021 +/-0.002 < 0.027 9515404 07/18/95 07/25/95 0.012 +/4002 < 0.020 9501723 01/24/95 01/31/95 0.019 +/-0.002 <0.018 9516254 07/25/95 08/01/95 0.009 +/-0.002 < 0.016 9502205 01/31/95 02/07/95 0.018 +/4002 <0.024 9516680 08/01/95 08/08/95 0.014 +/-0 002 < 0.018 9502899 02/07/95 02/14/95 0.017 +/-0.002 < 0.021 9517615 08/08/95 08/15/95 0.014 +/-0.002 < 0.023 9503382 02/14/95 02/21/95 0.012 +/-0.002 < 0.023 9518265 08/15/95 08/22/95 0.018 +/-0.002 < 0.023 9503703 02/21/95 02/27/95 0.015 +/-0.002 < 0.030 9518864 08/22/95 08/29/95 0.020 +/-0.002 < 0.017 9504191 02/27/95 03/07895 0.020 +/-0.002 < 0.019 9519477 08/29/95 09/05/95 0.023 +/-0.003 <0025 9504613 03/07/95 03/, * *.5 0.018 +/-0.002 < 0.024 9520280 09/05/95 09/12/95 0.021 +/-0.003 < 0.023 9505240 03/14/95 03/21/95 0.015 +/-0.002 < 0.021 9520492 09/12/95 09/19/95 0.014 +/-0.002 < 0.022 9505674 03/21/95 03/28/95 0.017 +/-0.003 < 0.023 9520897 09/19/95 09/26/95 0.021 +/-0.002 < 0.014 9506222 03/28/95 04/04/95 0.006 +/-0.002 < 0.021 9521415 09/26/95 10/03/95 0.025 +/-0.002 < 0.021 9506946 04/04/95 04/11/95 0.019 +/-0.002 < 0.025 9522111 10/03/95 10/10/95 0.023 +/-0.002 < 0.024 9507621 04/11/95 04/18/95 0.020 +/-0.002 < 0.022 9522654 10/10/95 10/17/95 0.021 +/-0.002 < 0.024 9508233 04/18/95 04/25/95 0.018 +/-0.002 < 0.023 9522997 10/17/95 10/24/95 0.013 +/-0.002 < 0.023 9523474 10/24/95 10/31/95 0.010 +/-0.002 < 0 026 9508693 04/25/95 05/02/95 0.013 +/-0.002 <0020 9509383 05/02/95 05/10/95 0.011 +/-0.002 < 0.024 9523889 10/31/95 11/07/95 0.012 +/-0.002 < 0.027 9509675 05'10/95 05/16/95 0.011 +/-0.002 < 0.031 9524376 11/07i95 11/13/95 0.018 +/-0.002 < 0.030 9510362 05/16/95 05/23/95 0.010 +/-0.002 < 0.021 9525016 11/13/95 11/20/95 0 009 +/-0.002 < 0.029 9510735 05/23/95 05/30/95 0.014 +/-0.002 < 0012 9525282 11/20/95 11/27/95 0.033 +/-0.003 <0.025 9511400 05/30/95 06/06/95 0.008 +/-0.002 < 0.019 9525656 11/27/95 12/04/95 0.016 +/-0.002 < 0.024 9512036 06/06/95 06/13/95 0.012 +/-0.003 <0.032 9525819 12/04/95 12/11/95 0.025 +/-0.003 < 0.023 l 9512686 06/13/95 06/20/95 0.011 +/-0.002 <0.018 9526533 12/11/95 12/18/95 0.009 +/-0.002 < 0.019 l

9513236 06/20/95 06/27/95 0.014 +/-0.002 < 0.019 9526793 12/18/95 12/27/95 0.024 +/-0.002 < 0.017 l

l t

l l

51

TABLE B-3 AIR PARTICULATE FILTERS GAMMA ISOTOPIC ANALYSIS ON QUARTERLY COMPOSITES i SAMPLE LOCATIG!h ALL SAMPLE SITES UNITS: pCi/ CUBIC METER LOCATION LAB NO. SEGIN END DATE Cs-134 Cs-137 DFTE i APG-1 9506197 12/27/94 04/04SS < 0.0012 < 0.0003 l APG-1 9513535 04/04/95 07/03/95 < 0.0014 < 0.0017 APG-i 9522002 07/03/95 10/03/95 < 0.0016 < 0.0011 APG-1 9600215 10/03/95 01/02/06 < 0.0010 < 0.0008 APQ-1 9506198 12/27/94 04/04/95 < 0.0014 < 0.0011 APQ-1 9513536 04/04/95 07/03/95 < 0.0018 < 0.0013  !

APQ-1 9522003 07/03/95 10m3SS < 0.0012 < 0.0010 I APQ-1 9600216 10/03/95 01/02/06 <0.0009 <0.0007

)

1 APP-1 9506199 12/27/94 04/04/95 < 0.0014 < 0 0010 APP-1 9513537 04/04SS 07/03/95 <0.0015 < 0.0010 APP-1 9522004 07/03/95 10/03/95 < 0.0008 < 0.0007 APP-1 9600217 10/03/95 01/02/06 < 0.0009 < 0.0010 APC-1 9506200 12/27 S 4 04/04/95 < 0.0011 < 0.0008 APC-1 9513538 04/04/95 07/03/95 <0.0015 <00015 APC-1 9522005 07/03/95 10/03/95 < 0.0012 <0.0011 APC-1 9600218 10/03/95 01/02/06 < 0.0011 < 0.0013 APE-30 9506201 12/27/94 04/04/95 < 0.0013 < 0.0011 APE-30 9513539 04/04/95 07/03/95 <00015 < 0.0011 APE-30 9522006 07/03/95 10/03SS <0.0007 < 0.0005 APE-30 9600219 10/03/95 01/02/06 < 0.0013 < 0.0009 52

v . .

TABLE B-4 DRINKING / SURFACE WATER IODINE-131 ' ANALYSIS SAMPLE LOCATION: DWGISWG-2 UNITS: pCi/ LITER LAB NO. BEGIN DATE END DATE l-131 9500672 12/27S4 01/10/95 < 0.7 9501385 01110/95 01/24/95 < 0.7 9502209 01/24/95 02/07/95 < 0.7 9503383 02/07S 5 02121/95 < 0.9 9504192 02/21/95 03/07S 5 <08 9505241 03/07/95 03/21195 < 0.8 9506223 03/21/95 04,C4SS < 0.9 9507525 04/04/95 04/18t95 < 0.5 9508694 04/18SS 05/02/95 < 0.9 9509697 05/02/95 05/16/95 < 0.5 9510737 05/16/95 05/3G95 < 0.5 9512037 05/3055 06/13/95 < 0.6 9513237 06/13/95 06/27 S 5 < 15 9514349 06/27/95 07/11 S 5 < 0.5 9515406 07/11/95 07/25/95 < 0.6 9516681 07/25/95 06/08/95 < 0.5 9518266 08/08SS 08/22/95 < 0.7 9519504 08/22/95 0905/95 -05 9520493 0905/95 09/19I95 < 0.9 9521416 09/19/95 10/03/95 < 0.9 9522655 10/03SS 10/17/95 < 0.7 9523475 10/17195 10/31195 <06 9524377 10/3185 11/1495 < 0.7 9525283 11/1495 11/27S 5 < 0.6 9525820 11/27 S 5 12/11/95 < 0.6 9526794 12/11/95 12/27!95 < 0.6 l

l

! 53

m _ .. ,

Ca TABLE B-4 (continued)

DRINKING / SURFACE WATER IODINE-131 ANALYSIS .

SAMPLE LOCATION: DWEISWE-5 UNITS: pCi/ LITER

~

LAB NO. BEGIN DATE END DATE l-131 9500673 12/27/94 01/10/95 < 0.7 9501386 01/10/95 01/24/95 < 0.5 9502210 01/24/95 02/07/95 < 0.5 9503384 02/07/95 02/21/95 < 0.7 9504193 02/21/95 03/07/95 < 0.7 9505242 03/07/95 03/21/95 < 0.9 9506224 03/21/95 04/04/95 < 0.6 9507526 04/04/95 04/18/95 < 0.5 9508695 04/18/95 0502,95 < 0.7 9509698 05/02/95 05/16/95 < 0.7 9510738 05/16/95 05/30/95 < 0.5 9512038 05/30/95 06/13/95 < 0.6 9513238 06/13/95 06/27/95 < 0.6 9514350 06/27/95 07/11/95 < 0.4 9515407 07/11/95 07/25/95 < 0.5 9516682 07/25/95 08/08/95 < 0.7 9518267 08/08/95 08/22/95 < 0.7 9519505 08/22/95 09/05/95 < 0.6 9520494 09/05/95 09/19,95 < 0.9 9521417 09/19/95 1(4,T95 < 0.6 9522656 10/03/95 10/17. % < 0.9 9523476 10/17/95 10/31/95 < 0.7 9524378 10/31/95 11/14/95 < 0.6 9525284 11/14/95 11/27/95 < 0.8 9525821 11/27/95 12/11/95 < 0.9 9526795 12/11/95 12/27/95 < 0.6 54

- - _ _ - _ - _ _ - _ _ _ - _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ - _ - _ _ - _ _ _ _ - _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ - _ _ _ = _ - _ .

TABLE B-4 (continued)

DRINKING / SURFACE WATER IODINE-131 ANALYSIS SAMPLE LOCATION: DWP/SWP-7 UNITS: pCi/ LITER LAB NO. BEGIN DATE END DATE l-131 9500674 12/2754 01/10/95 < 0.7 9501387 01/10/95 01/24/95 < 0.7 9502211 01/24/95 02/07/95 < 0.5 9503385 02/07/95 02/21/95 < 0.7 9504194 02/21/95 03/07/95 < 0.7 9505243 03/07/95 03/21/95 < 0.9 9506225 03/21/95 04/04/95 <C8 9507527 04/04/95 04/18/95 < 0.6 9508696 04/18/95 05/02/05 < 0.5 9509699 05m2/95 05/16/95 < 0.4 9510739 05/16/95 05/30/95 < 0.4 9512039 05/30/95 06/13/95 < 0.5 9513239 06/1385 06/27!95 < 0.8 9514351 06/27/95 07/11/95 < 0.7 9515408 07/11/95 07/25/95 < 0.5 9516683 07/25/95 08/08/95 < 0.S 9518268 08/08SS 08/22/95 < 0.8 9519506 08/22 S 5 09/05/95 < 0.4  !

9520495 09/05/95 09/19/95 < 0.8 9521418 09/19/95 10/03/95 < 0.9 9522657 10/03/95 10/17/95 < 0.8 9523477 10/17/95 10/3I/95 < 0.9 9524379 10/31/95 11/14/95 < 0.6 9525285 11/14/95 11/27/95 < 0.9 9525822 11/27/95 12/11/95 < 0.7 9526796 12/11/95 12/27 S 5 < 0.6 55

TABLE B-5 DRINKINGISURFACE WATER GROSS BETA ANALYSIS ,

ON MONTHLY COMPOSTES SAMPLE LOCATION: DWG/SWG-2 UNITS: pCi/ LITER LAB NO. BEGIN DATE END DATE BETA 9501388 12/27/94 01/24/95 2.6 +/- 1.4 9503386 01/24!95 02/21 S 5 12.1 +/- 1.9 9505258 02/21/95 03/21/95 < 1.8 9507528 03/21/95 04/18/95 < 2.3 9509700 04/18/95 05/16/95 1.9 +/- 1.4 9512040 05/16/95 06/13/95 2.8 +/- 1.6 9513240 06/13/95 06/27/95 12.0 +/- 2.2 9515411 06/27/95 07/25/95 3.9 +/- 1.8 9518269 07/25/95 08/22/95 1.8 +/- 1.7 i 9520496 08/22/95 09/19/95 1.8 +/- 1.3 9521419 09/19/95 10/03/95 3.9 +/- 1.7 9523478 10/03/95 10/31 S 5 2.4 +/- 1.7 9525286 10/31/95 11/27/95 8.9 +/- 2.0 9526797 11/27/95 12/27SS 4.1 +/- 1.6 56

TABLE B-5 (continued)

DRINKINGISURFACE WATER GROSS BETA ANALYSIS ON MONTHLY COMPOSITES SAMPLE LOCATION: DWEISWE-5 UNITS: pCi/ LITER LAB NO. BEGIN DATE END DATE BETA l

9501389 12/27 S 4 01/24/95 5.1 +/- 14 9503387 01/24/95 02/21/95 2.2 +/- 1.3 9505259 02/21 S 5 03/21S 5 1.3 +/- 1.3 9507529 03/21/95 04/18/95 < 2.8 9509701 04/18/95 05/1GS5 4.5 +/- 1.6 9512041 05/16/95 06/13/95 5.9 +/- 1.6 9513241 06/13/95 06/27/95 < 2.8 9515412 06/27S 5 07/25/95 2.6 +/- 1.7 9518270 07/25/95 08/22/95 < 2.7 9520497 08/22/95 09/19/95 2.6 +/- 1.6 9521420 09/1955 10/03/95 2.7 +/- 1.6 9523479 10/03/95 10/31/95 3.1 +/- 1.7 9525287 10/31 S 5 11/27/95 2.5 +/- 1.5 9526798 11/27/95 12/27S 5 2.3 +/- 1.3 57

TABLE B-5 (continued)

DRINKINGISURFACE WATER GROSS BETA ANALYSIS ON MONTHLY COMPOSITES SAMPLE LOCATION: DWP/SWP-7 UNITS: pCi/ LITER t.AE NO. BEGIN DATE END DATE BETA

'1501390 12/27ne. 01/24/95 5.3 +/- 1.5 9503388 01/24/95 Gb2iG5 3.9 +/- 1.4 l l

9505260 02/21/95 03/21,95 1.9 +/- 1.3 9507530 03/21/95 04/18/95 < 2.8 95097C2 04/18,TS 05/16/95 5 5 +/- 1.6 9512042 05/16/95 OS/t3/95 4.3 +/- 1.6 9513242 06/13/95 06/27/95 4.5 +/- 1.9 9515413 06/27/95 07/25/95 1.8 +/- 1.7 9518271 07/25/95 08/22/95 2.5 +/- 1.7 9520498 08/22/95 09/19/95 2.9 +/- 1.6 9521421 09/19/95 10/03/95 3.8 +/- 1.7 9523480 10/03/95 10/31/95 < 2.6 9525288 10/31/95 11/27/95 5.3 +/- 1.6 9526799 11/27/95 12/27/95 2.8 +/- 1.4 l

l 56

TABLE B-5 (continued) 1 DRINKINGISURFACE WATER GAMMA ISOTOPIC ANALYSIS ON MONTHLY COMPOSITES 1

UNITS: pCi/ LITER SAMPLE LOCATION: DWGISWG-2 I

f LAB NO. BEGIN DATE END DATE Mn-54 Fe-59 Co-58 Co-60 Zn-65 Zr-95 Nb-95 Cs-134 Cs-137 Ba-140 La-140 9501388 12/27/94 01/24/95 <2 <3 <2 <2 <5 <5 <3 <3 <3 < 12 <3 9503386 01/24/95 02/21/95 <2 <3 <2 <2 <5 <5 <2 <3 <2 <9 <3 9505258 02/21/95 03/21/95 <2 <3 <2 <3 <5 <5 <2 <3 <3 <6 <2 9507528 03/21/95 04/18/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 <8 <2 9509700 04/18/95 05/16/95 <2 <3 <2 <2 <4 <4 <2 <2 <2 <7 <2 9512040 05/16/95 06/13/95 <2 <3 <2 <2 <4 <5 <2 <3 <2 < 10 <2 9513240 06/13/95 06/27/95 <1 <1 <1 <1 <2 <3 <1 <1 <1 <4 <1 9515411 06/27/95 07/25/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <8 <2 9518269 07/25/95 08/22/95 <2 <3 <2 <3 <4 <5 <2 <2 <2 < 10 <3 9520496 08/22/95 09/19/95 <3 <4 <3 <3 <6 <6 <3 <3 <3 < 12 <3 9521419 09/19/95 10/03/95 <2 <3 <2 <3 <5 <5 <2 <3 <2 <9 <3 9523478 10/03/95 10/31/95 <2 <2 <2 <2 <3 <4 <2 <2 <2 <7 <2 9525286 10/31/95 11/27/95 <2 <2 <2 <2 <3 <4 <2 <2 <2 <7 <2 9526797 11/27/95 12/27/95 <2 <4 <2 <2 <4 <3 <2 <2 <2 <9 <3 59

TABLE B-5 (continued)

DRINKINGISURFACE WATER GAMMA ISOTOPIC ANALYSIS ON MONTHLY COMPOSITES SAMPLE LOCATION: DWEISWE-5 UNITS: pCi/ LITER LAB NO. BEGIN DATE END DATE Mn-54 Fe-59 Co-58 Co-60 Zn-65 Zr-95 Nb-95 Cs-134 Cs-137 Bs-140 La-140 9501389 12/27/94 01/24/95 <3 <4 <3 <3 <6 <6 <3 <3 <3 < 12 <4 9503387 01/24/95 02/21/95 <2 <3 <2 <3 <5 <5 <2 <3 <2 < 10 <3 9505259 02/21/95 03/21/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 <9 <2 9507529 03/21/95 04/18/95 <2 <3 <2 <2 <5 <5 <2 <2 <2 < 10 <3 9509701 04/18/95 05/16/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 < 11 <2 9512041 05/16/95 06/13/95 <2 <3 <2 <2 <5 <5 <2 <3 <2 <9 <3 9513241 06/13/95 06/27/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <8 <2 9515412 06/27/95 07/25/95 <1 <1 <1 <1 <2 <2 <1 <1 <1 <4 <2 9518270 07/25/95 08/22/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <7 <2 9520497 08/22/95 09/19/95 <1 <1 <1 <1 <2 <3 <1 <1 <1 <4 <1 9521420 09/19/95 10/03/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <7 <2 9523479 10/03/95 10/31/95 <2 <5 <3 <3 <6 <5 <3 <3 <3 < 13 <3 9525287 10/31/95 11/27/95 <2 <4 <2 <2 <5 <4 <2 <2 <2 < 12 <3 9526798 11/27/95 12/27/95 <2 <3 <2 <2 <4 <5 <2 <3 <2 <8 <3 60

TABL E 8-5 (Continued)

DRINKINGISURFACE WATER GAMMA ISOTOPIC ANALYSIS ON MONT3LY COMPOSITES SAMPLE LOCATION: DWP/SWP-7 UNITS: pCi/ LITER LAB NO. BEGIN DATE END DATE Mn-54 Fe-59 Co-58 Co-60 Zn-65 Zr-95 Nb-95 Cs-134 Cs-137 Ba-140 La-140 9501390 12/27/94 01/24/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 < 10 <2 9503388 01/24/95 02/21/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 <8 <2 9505250 02/21/95 03/21/95 <2 <3 <2 <2 <5 <5 <2 <3 <2 < 10 <2 9507530 03/21/95 04/18/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 <9 <2 9509702 04/18/95 05/16/95 <2 <2 <2 <2 <3 <4 <2 <2 <r <7 <2 9512042 05/16/95 06/13/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <7 <2 9513242 06/13/95 06/27/95 <3 <3 <3 <3 <5 <6 <3 <3 <3 < 10 <3 9515413 06/27/95 07/25/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <8 <2 9518271 07/25/95 08/22/95 <2 <2 <2 <2 <4 <4 <2 <2 <2 <8 <2 9520498 08/22/95 09/19/95 <2 <3 <2 <2 <4 <5 <2 <2 <2 <9 <3 9521421 09/19/95 10/03/95 <2 <2 <2 <2 <3 <4 <1 <2 <1 <5 <2 9523480 10/03/95 10/31/95 <2 <5 <2 <3 <5 <4 <2 <2 <2 < 12 <4 9525288 10/31/95 11/27/95 <2 <4 <2 <2 <5 <4 <2 <2 <2 < 11 <3 9526799 11/27/95 12/27/95 <3 <5 <3 <3 <6 <5 <3 <3 <3 < 13 <3 61

- . . _ ~

TABLE B-6 DRINKING / SURFACE WATER TRITIUM ANALYSIS ON QUARTERLY COMPOSITES

SAMPLE LOCATION: ALL SAMPLE SITES UNITS: pCi/ LITER LOCATION LAB NO. BEGIN DATE END DATE H-3 DWGISWG - 2 9505266 12/27S 4 03/21 S 5 < 300 DWGISWG - 2 9513243 03/21 S 5 06/27/95 < 320 DWGISWG - 2 9521422 06/27S 5 1003/95 < 290 DWGISWG - 2 9526800 10/03S5 12/27S 5 < 290 DWEISWE - 5 9505267 12/27S 4 03/21 S 5 < 300 DWEISWE - 5 9513244 03/21/95 06/27/95 < 320 DWEISWE - 5 9521423 06/27/95 10/03/95 <290 DWEISWE - 5 9526801 10/03/95 12/27/95 < 290 DWP/SWP - 7 9505268 12/27S 4 03/21/95 < 300 DWPISWP -7 9513245 03/21S 5 06/27/95 < 320 DWP/SWP -7 9521424 06/27/95 1003/95 < 290 DWP/SWP - 7 9526802 10/03/95 12/27 S 5 < 290

'f 62

O TABLE B-7 GROUNDWATER TRITIUM AND GAMMA ISOTOPIC ANALYSES i

SAMPLE LOCATION: GWJ-1 UNITS: pCi/ LITER LAB NO. COLLECTION H-3 Mn-54 Fe-59 Co-58 Co-60 Zn-65 Zr-95 Nb-95 Cs-134 Cs-137 Ba-140 La-140 DATE l

9500306 01AW95 < 310 <2 <3 <2 <2 <5 <5 <3 <3 <2 < 13 <3 j 9506226 04/04/95 < 310 <2 <3 <2 <3 <5 <5 <2 <2 <2 <9 <3 9513918 07/03/95 < 320 <2 <3 <2 <2 <4 <5 <2 <2 <2 < 10 <3 9521425 10/03/95 < 290 <2 <2 <2 <2 <3 <4 <2 <2 <2 <6 <2 63' i

TABLE B-8 SHORELINE SOIL GAMMA ISOTOPIC ANALYSIS l

SAMPLE LOCATIONS: ALL SAMPLE SITES UNITS: pCi/Kg j LOCATION LAB NO. COLLECTION Mn-54 Co-58 Co-60 Cs-134 Cs-137 DATE SHVWK-1 9506227 04.04/95 <7 < 11 < 10 < 13 31 +/- 8 SHWWK-1 9521427 10/03/95 <9 < 11 < 12 < 15 34 +/- 9 SHWWE-3 9506228 04/04/95 < 13 < 13 < 11 < 16 44 +/- 9 SHVWE-3 9521426 10/03/95 < 10 < 10 < 10 < 13 45 +/- 8 64

o i

l TABLE B-9 MILK -IODINE-131 AND GAMMA ISOTOPIC ANALYSES SAMPLE LOCATION: MKQ-5 UNITS: pCi/ LITER

LAB NO. COLLECTION l-131 Cs-134 Cs-137 Ba-140 La-140 DATE 9500304 01/04/95 < 0.5 <4 <3 < 15 <4 9501023 01/18/95 < 0.5 <3 <3 < 12 <2 9501754 02/01/95 < 0.8 <4 <3 < 13 <3 9503033 02/16/95 < 0.8 <3 <3 <9 <3 9503917 03/01/95 < 0.9 <4 <3 < 13 <3 l

9504713 03/15/95 < 0.6 <3 <2 <9 <3 l 9506229 04/05/95 < 0.7 <3 <3 < 10 <3 9507594 04/19/95 < 0.6 <1 <2 <8 <2 9508796 05/03/95 < 0.9 <4 <3 < 14 <4 9509669 05/17/95 <06 <3 <3 < 10 <3 9511114 06/07/95 < 0.4 <2 <2 <7 <2 9512690 06/21/95 < 0.5 <1 <1 <4 <1 S513916 07/05/95 < 0.5 <2 <2 <8 <2 9514836 07/19/95 < 0.4 <2 <2 <8 <2 9516101 08/02/95 < 0.5 <2 <2 <9 <2 I

9517546 08/16/95 < 0.6 <2 <2 <6 <2 9519562 09/06/95 <06 <4 <3 < 13 <3 9520499 09/20/95 < 0.6 <2 <2 <8 <2 9521650 10/04/95 < 0.5 <4 <3 < 13 <3 9522659 10/18/95 < 0.6 <2 <1 <6 <2 9523642 11/01/95 < 0.8 <3 <3 <9 <3 9524370 11/14/95 < 0.6 <4 <4 < 13 <4 9525608 12/05/95 < 0.7 <2 <2 < 11 <2 9526537 12/1 % 5 < 0.6 <2 <2 <9 <3 65

G-TABLE B-9 (continued)

MILK -IODINE-131 AND GAMMA ISOTOPIC ANALYSES -

SAMPLE LOCATION: MKQ-45 UNITS: pCi/ LITER LAB NO. COLLECTION 1-131 Cs-134 Cs-137 Ba-140 La-140 DATE 9500305 01/03/95 < 0.5 <3 <2 < 13 <3 9501043 01/17/95 < 0.5 <3 <3 < 11 <3 9501758 01/30/95 < 0.9 <3 <3 < 11 <2 9503034 02/14/95 < 0.8 <2 <2 <9 <2 9503918 02/27/95 < 0.9 <3 <3 < 13 <4 9504714 03/13/95 < 0.7 <2 <2 <9 <2 9506230 04/04/95 < 0.6 <3 <2 <9 <2 9507595 04/18/95 < 0.6 <3 <3 < 11 <3 9508797 05/02/95 < 0.9 <3 <2 < 10 <3 9509670 05/16/95 < 0.9 <3 <3 < 11 <2 9511115 06/06/95 <06 <2 <1 <5 <2 9512691 06/20/95 < 0.7 <2 <2 <7 <2 >

9513917 07/03/95 < 0.7 <2 <1 <5 <1 9514838 07/18/95 < 0.5 <3 2 +/- 2 <8 <2 9516102 08/01/95 < 0.6 <2 <2 <8 <2 9517547 08/15/95 < 0.6 <2 <2 <6 <2 9519563 09/05/95 < 0.4 <2 <2 <8 <2 9520500 09/19/95 <07 <2 <2 <8 <2 9521651 10/02/95 < 0.6 <2 <2 <7 <2 9522660 10/17/95 < 0.7 <3 3 +/- 2 <9 <3 9523643 10/31/95 <08 <2 <3 < 12 <3 9524371 11/13/95 < 0.7 <3 -3 < 11 <3 9525609 12/04/95 < 0.6 <3 <3 .< 14 - <3 9526538 12/18/95 < 0.6 <2 <3 < 14 <3 66

TABLE B-10 FISH GAMMA ISOTOPIC ANALYSIS SAMPLE LOCATION: FH-1 ' UNITS: pCi/Kg LAB NO. COLLECTION SPECIES Mn-54 Fe-59 Co-58 Co40 Zn45 Cs-134 Cs-137 DATE 9512214 05/30/95 CATFISH < 16 < 29 < 20 < 15 < 37 < 17 < 12 9512215 05/30/95 MULLET <9 < 14 < 11 < 10 < 21 < 10 <9 9512216 05/30/95 CARP < 17 < 31 < 20 < 18 < 37 < 19 < 14 9512217 05/30/95 BUFFALO <8 < 12 <8 <7 < 17 <7 <7 9525933 12/06/95 CATFISH <9 < 15 <9 < 10 < 25 < 11 <i 9525934 12/06/95 MULLET <7 < 19 <7 <9 < 20 <7 <8 9525935 12/06/95 SHAD < 10 < 17 < 10 < 'O < 24 < 11 <9 9525936 12/06/95 STRIPED BASS <7 < 14 <8 < 10 < 24 <9 <9 67

TABLE B-10 (continued)-

FISH GAMMA ISOTOPIC ANALYSIS SAMPLE LOCATION: FH-2 UNITS: pCi/Kg LAB NO. COLLECTION SPECIES Mn-54 Fe-59 Co-58 Co40 Zn45 Cs-134 Cs-137 DATE 9512218 05/30/95 CATFISH < 16 < 32 < 17 < 17 < 41 < 19 < 15 9512219 05/30/95 MULLET < 12 < 19 < 12 < 11 < 24 < 14 < 12 9512220 05/30/95 CARP < 22 < 34 < 21 < 18 < 40 < 21 < 17 9512221 05/30/95 BUFFALO <9 < 16 <9 < 11 < 21 < 10 <8 9525937 12/06/95 CATFISH < 10 < 26 < 12 < 12 < 29 < 10 < 12 9525938 12/06/95 MULLET <7 < 11 <9 <7 < 19 < 10 <7 9525939 12/06/95 SHAD <8 < 21 <9 <9 < 22 <8 <8 9525940 12/06/95 STRIPED BASS <8 < 11 <8 <8 < 18 <9 <6 l

I I

l l

l l

l 68 l

l l

- o TABLE B-11 BROAD LEAF VEGETATION IODINE-131 AND GAMMA ISOTOPIC ANALYSES SAMPLE LOCATION: BLQ-1 UNITS: pCi/Kg LAB NO. COLLECTION 3-131 Cs-134 Cs-137 -

DATE  !

9501377 1/25/95 < 24 < 28 < 24 9503374 02/21 S 5 < 29 < 26 < 22 9505233 03/21/95 < 31 < 25 < 24 9508509 04/25/95 < 18 < 12 <9 9510221 05r23/D5 < 28 < 23 < 22 9512687 06/21/95 < 14 < 15 < 13 9515415 07/25/95 < 23 < 23 < 21 9518272 08l22/95 < 25 < 27 < 20 9520898 09/26/95 < 20 < 17 < 15 9522998 10/24/95 < 14 < 13 < 12 Z25017 11/20/95 < 24 < 29 < 24 9526534 12/18/95 < 14 < 10 < 11 69

4 TABLE B-11 (Continued)

BROAD LEAF VEGETATION IODINE-131 AND GAMMA ISOTOPIC ANALYSES SAMPLE LOCATION: BLB-1 UNITS: pCi/Kg i

LAB NO. COLLECTION 3-131 Cs-134 Cs-137 DATE 9501378 1/25/95 < 26 < 33 < 29 9503375 02/21/95 < 19 < 23 < 19 9505234 03/21/95 < 28 < 30 < 27 9508510 04/25/95 < 18 < 14 < 12 9510222 05/23/95 < 23 < 18 < 20 9512688 06/21/95 < 10 < 11 <9 9515416 07/25/95 < 27 < 27 < 22 9518273 08/22/95 < 23 < 21 < 21 9520899 09/26 S5 < 32 < 24 < 28 9522999 10/24/95 < 19 < 24 < 18 9525018 11/20/95 < 25 < 30 < 26 9526535 12/18/95 < 19 < 18 < 15 70

4

- TABLE B-11 (Continued)

BROAD LEAF VEGETATION IODINE-131 AND GAMMA ISOTOPIC ANALYSES SAMPLE LOCATION: BLK-15 UNITS: pCi/Kg LAB NO. COLLECTION l-131 Cs-134 Cs-137 DATE 9501379 1125/95 < 20 < 22 - < 20 9503376 02/21/95 < 24 < 21 < 19 9505235 03/21/95 < 27 < 28 < 25 9508511 04/25/95 < 19 < 12 < 10 9510223 05/23/95 < 20 < 23 < 21 9512689 06/21/95 < 20 < 18 < 15 9515417 07/25/95 < 24 < 20 < 21 9518274 08/22/95 < 21 < 24 < 21 9520900 09/26/95 < 23 < 20 < 16 9523000 10/24/95 < 26 < 24 < 20

. 9525019 11/20/95 < 23 < 18 < 16 9526536 12/18/95 < 14 <9 < 11 71

TABLE B-12 VEGETATION - FOOD PRODUCTS IODINE-131 AND GAMMA ISOTOPIC ANALYSES SAMPLE LOCATION: ALL SAMPLE SITES UNITS: pCi/Kg LAB NO. LOCATION COLLECTION 1-131 Cs-134 Cs-137 DATE ,

9522661 FPG-1 10/17/95 < 11 < 10 <8 9522662 FPP-1 10/17195 < 13 < 15 < 13 72

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