ML21238A011: Difference between revisions

From kanterella
Jump to navigation Jump to search
(StriderTol Bot insert)
 
(StriderTol Bot change)
 
Line 17: Line 17:
=Text=
=Text=
{{#Wiki_filter:Nuclear Fuel Services, Inc.
{{#Wiki_filter:Nuclear Fuel Services, Inc.
21G-21-0103 Certified Mail                                                                                   GOV-01-55 Return Receipt Requested                                                                       ACF-21-0182 August 16, 2021 Director Office of Nuclear Material Safety & Safeguards U.S. Nuclear Regulatory Commission ATTN: Document Control Desk Washington, DC 20555-0001
21G-21-0103 Certified Mail GOV-01-55 Return Receipt Requested ACF-21-0182 August 16, 2021 Director Office of Nuclear Material Safety & Safeguards U.S. Nuclear Regulatory Commission ATTN: Document Control Desk Washington, DC 20555-0001


==Reference:==
==Reference:==
Line 26: Line 26:


==Dear Director:==
==Dear Director:==
In accordance with the requirements set forth in 10 CFR Part 70.59, Nuclear Fuel Services, Inc. (NFS), submits the attached reports. Attachment 1 reports the Radioactivity in Effluent Liquid for the period January to June 2021. Attachment 2 reports the Radioactivity in Effluent Air for the period January to June 2021. Attachment 3 summarizes an evaluation of the dose and air activity concentrations for the maximally exposed offsite individual due to gaseous effluents during the period January to June 2021.


In accordance with the requirements set forth in 10 CFR Part 70.59, Nuclear Fuel Services, Inc. (NFS), submits the attached reports. Attachment 1 reports the Radioactivity in Effluent Liquid for the period January to June 2021. Attachment 2 reports the Radioactivity in Effluent Air for the period January to June 2021. Attachment 3 summarizes an evaluation of the dose and air activity concentrations for the maximally exposed offsite individual due to gaseous effluents during the period January to June 2021.
If you or your staff have any questions, require additional information, or wish to discuss this, please contact me or Mr. R. Jason Faddis, Environmental Safety Unit Manager, at (423) 735-5438. Please reference our unique document identification number (21G 0103) in any correspondence concerning this letter.
If you or your staff have any questions, require additional information, or wish to discuss this, please contact me or Mr. R. Jason Faddis, Environmental Safety Unit Manager, at (423) 735-5438. Please reference our unique document identification number (21G   0103) in any correspondence concerning this letter.
 
Sincerely, NUCLEAR FUEL SERVICES, INC.
Sincerely,
IE4?
 
                                                                                                        !lflvj552D
NUCLEAR FUEL SERVICES, INC. IE4?
                                                                  ,:J~/~
,:J~/~ !lflvj552D
Tim Knowles Safety & Safeguards Director jl}Jv/55 CJB/pj/smd Attachments
 
Tim Knowles jl}Jv/55 Safety & Safeguards Director CJB/pj/smd Attachments
: 1) Report of Radioactivity in Effluent Liquid for the Period January to June 2021
: 1) Report of Radioactivity in Effluent Liquid for the Period January to June 2021
: 2) Report of Radioactivity in Effluent Air for the Period January to June 2021
: 2) Report of Radioactivity in Effluent Air for the Period January to June 2021
: 3) Report of Gaseous Effluent Dose and Activity Concentrations for the Maximally Exposed Off-Site Individual for the Release Period January to June 2021 Page 1 of 13                      People Strong 1205 Banner Hill Rd, Erwin, TN 37650 t: +1.423.743.9141 f: +1.423.743.0140 www.nuclearfuelservices.com                 INNOVATION DRIVEN         >
: 3) Report of Gaseous Effluent Dose and Activity Concentrations for the Maximally Exposed Off-Site Individual for the Release Period January to June 2021
 
1205 Banner Hill Rd, Erwin, TN 37650 Page 1 of 13 People Strong
 
t: +1.423.743.9141 f: +1.423.743.0140 www.nuclearfuelservices.com INNOVATION DRIVEN >
21G-21-0103 GOV-01-55 ACF-21-0182
 
Copy:


21G-21-0103 GOV-01-55 ACF-21-0182 Copy:
Mr. Joel Rivera-Ortiz
Mr. Joel Rivera-Ortiz
*senior Fuel Facility Inspector U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257 Regional Administrator U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257 Mr. James Downs Fire Protection Engineer Division of Fuel Management Office of Nuclear Material Safety and Safeguards U.S. Nuclear Regulatory Commission Two White Flint North 11555 Rockville Pike Rockville, MD 20852-2738 Dr. Robert Williams Chief, Projects Branch 1 U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257 Mr. Larry Harris Senior Resident Inspector U.S. Nuclear Regulatory Commission Page 2 of 13
*senior Fuel Facility Inspector U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257
 
Regional Administrator U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257
 
Mr. James Downs Fire Protection Engineer Division of Fuel Management Office of Nuclear Material Safety and Safeguards U.S. Nuclear Regulatory Commission Two White Flint North 11555 Rockville Pike Rockville, MD 20852-2738
 
Dr. Robert Williams Chief, Projects Branch 1 U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257
 
Mr. Larry Harris Senior Resident Inspector U.S. Nuclear Regulatory Commission
 
Page 2 of 13 21G-21-0103 GOV-01-55 ACF-21-0182
 
Attachment 1 To Letter Dated August 16, 2021
 
Report of Radioactivity in Effluent Liquid for the Period January to June 2021
 
(2 Pages to Follow)


21G-21-0103 GOV-01-55 ACF-21-0182 Attachment 1 To Letter Dated August 16, 2021 Report of Radioactivity in Effluent Liquid for the Period January to June 2021 (2 Pages to Follow)
Page 3 of 13 21 G-21-01 03 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Liquid January 1, 2021 to June 30, 2021
Page 3 of 13
 
Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of Location (I) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Banner Spring Down Pu-238 472,037,000 0.00E+OO 8.57E-l l 2.28E-10 0.00E+OO O.OOE+OO O.OOE+OO Pu-239/240 472,037,000 O.OOE+OO 9.4JE-l l 2.40E-10 O.OOE+OO O.OOE+OO O.OOE+OO Tc-99 472,037,000 O.OOE+OO 3.44E-08 6.1 OE-08 0.00E+OO O.OOE+OO O.OOE+OO Th-228 472,037,000 1.08E-11 1.43E-IO 2.99E-10 5.IOE-06 6.22E-09 5.40E-05 Th-230 472,037,000 3.59E-l I l.81E-10 3.66E-10 l.70E-05 8.40E-04 3.59E-04 Th-232 472,037,000 O.OOE+OO l.OOE-10 2.67E-10 O.OOE+OO O.OOE+OO O.OOE+OO U-233/234 472,037,000 2.73E-10 2.SIE-10 3.43E-10 1.29E-04 2.07E-02 9.llE-04 U-235/236 472,037,000 1.90E-ll 1.42E-10 2.89E-10 8.96E-06 4.ISE+OO 6.33E-05 U-238 472,037,000 5.64E-l l l.58E-IO 2.82E-10 2.66E-05 7.95E+Ol 1.88E-04
 
Total: 1.58E-03 Sewer Pu-238 25,036,000 O.OOE+OO l.l lE-10 2.41E-10 O.OOE+OO O.OOE+OO O.OOE+OO Pu-239/240 25,036,000 O.OOE+OO 1.22E-10 2.92E-10 O.OOE+OO O.OOE+OO O.OOE+OO Tc-99 25,036,000 3.62E-09 3.74E-08 6.SSE-08 9.05E-05 5.36E-03 6.03E-06 Th-228 25,036,000 l.88E-l l 2.43E-IO 4.88E-10 4.71E-07 5.75E-10 9.41E-06 Th-230 25,036,000 l.58E-10 3.08E-IO 4.97E-10 3.97E-06 l.96E-04 l.58E-04 Th-232 2s,0J6,poo O.OOE+OO l.68E-IO 3.93E-10 O.OOE+OO O.OOE+OO O.OOE+OO U-232 25,036,000 3.03E-ll l.83E-IO 3.74E-10 7.59E-07 3.55E-08 5.0SE-05 U-233/234 25,036,000 l.8 !E-08 1.40E-09 2.9!E-10 4.54E-04 7.27E-02 6.04E-03 U-235/236 25,036,000 7.02E-10 3.03E-10 2.56E-10 l.76E-05 8.14E+OO 2.34E-04 U-238 25,036,000 2.57E-09 5.38E-IO 2.SSE-10 6.44E-05 l.92E+02 8.58E-04
 
Total: 7.36E-03 West Ditch Pu-238 169,304,000 O.OOE+OO l.12E-10 2.79E-10 O.OOE+OO O.OOE+OO O.OOE+OO Pu-239/240 169,304,000 O.OOE+OO l.22E-10 3.45E-10 O.OOE+OO O.OOE+OO O.OOE+OO Tc-99 169,304,000 5.83E-09 3.48E-08 6.06E-08 9.87E-04 5.84E-02 9.72E-05 Th-228 169,304,000 l.17E-ll l.76E-10 3.92E-10 l.98E-06 2.4!E-09 5.84E-05 Th-230 169,304,000 7.71E-ll 2.ISE-10 4.03E-10 l.30E-05 6.46E-04 7.71E-04 Th-232 169,304,000 O.OOE+OO 1.25E-IO 2.76E-10 O.OOE+OO 0.00E+OO O.OOE+OO U-233/234 169,304,000 l.SIE-08 l.40E-09 3.14E-10 2.56E-03 4.l lE-01 5.0SE-02 U-235/236 169,304,000 7.09E-10 3.SIE-10 2.SIE-10 l.20E-04 5.56E+O! 2.36E-03 U-238 169,304,000 l.53E-09 4.SIE-10 2.33E-10 2.59E-04 7.72E+02 5.09E-03
 
Total: 5.89E-02 WWTF Am-241 3,947,307 O.OOE+OO 9.48E-11 2.19E-10 O.OOE+OO O.OOE+OO O.OOE+OO Cs-137 3,947,307 O.OOE+OO l.24E-09 l.43E-09 O.OOE+OO O.OOE+OO O.OOE+OO Na-22 3,947,307 8.95E-11 8.13E-10 l.39E-09 3.53E-07 5.66E-11 l.49E-05 Np-237 3,947,307 2.61E-l l 2.74E-IO 5.62E-IO l.03E-07 1.46E-04 l.3 IE-03 Pb-212 3,947,307 1.20E-09 3.35E-09 3.02E-09 4.72E-06 3.41E-12 5.98E-04 Pu-238 3,947,307 l.33E-l l 5.35E-l l l.07E-10 5.27E-08 3.08E-09 6.67E-04
 
1 ECV: Effluent Concentration Value from 10-CFR-20, Appendix B.
 
Note: A value of "a~ was substituted for negative analytical results.
 
Printed: 08/04/2021 NFS-EDMS Page I of2
 
Page 4 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Liquid January 1, 2021 to June 30, 2021
 
Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of 1 Location (I) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV WWTF Pu-239/240 3,947,307 O.OOE+OO 6.32E-l 1 I.57E-IO O.OOE+OO O.OOE+OO O.OOE+OO Pu-241 3,947,307 4.56E-IO I.OIE-08 I. 74E-08 l.SOE-06 1.75E-08 4.56E-04 Ra-224 3,947,307 l.20E-08 6.69E-09 l.20E-08 4.73E-05 2.98E-IO 5.99E-02 Tc-99 3,947,307 4.75E-09 l.30E-07 2.24E-07 1.87E-05 I.I IE-03 7.91E-05 Th-228 3,947,307 O.OOE+OO I.SIE-10 3.74E-IO O.OOE+OO O.OOE+OO O.OOE+OO Th-230 3,947,307 l.16E-10 2.23E-IO 3.87E-10 4.60E-07 2.28E-05 l.16E-03 Th-231 3,947,307 O.OOE+OO 3.98E-08 3.89E-08 O.OOE+OO O.OOE+OO O.OOE+OO Th-232 3,947,307 3.63E-II l.33E-IO 2.37E-IO 1.43E-07 1.3 IE+OO l.21E-03 U-232 3,947,307 O.OOE+OO I.ISE-10 2.45E-IO O.OOE+OO O.OOE+OO O.OOE+OO U-233/234 3,947,307 l.34E-08 9.28E-IO 1.75E-IO 5.30E-05 8.50E-03 4.48E-02 U-235/236 3,947,307 5.96E-IO 2.06E-IO l.06E-IO 2.35E-06 l.09E+OO l.99E-03 U-238 3,947,307 9.75E-l l l.02E-10 l.34E-IO 3.85E-07 I.ISE+OO 3.25E-04
 
Total: 1.IJE-01


21 G-21-01 03 GOV-0 1-55 ACF-21 -0182 Radioactivity in Efflue nt Liquid January 1, 2021 to June 30, 2021 Total                  Activity        Error                Quantity    Quantity          Fraction Volume              Concentration      Estimate        LLD      Released    Released            of Location                                (I)                  (µCi/ml)      (µCi/ml)    (µCi/ml)        (Ci) 1 (g)            ECV Banner Spring Down Pu-238                        472,037,000                        0.00E+OO      8.57E-l l    2.28E-10    0.00E+OO    O.OOE+OO      O.OOE+OO Pu-239/240                    472,037,000                        O.OOE+OO      9.4JE-l l    2.40E-10    O.OOE+OO    O.OOE+OO      O.OOE+OO Tc-99                        472,037,000                        O.OOE+OO      3.44E-08    6.1 OE-08    0.00E+OO    O.OOE+OO      O.OOE+OO Th-228                        472,037,000                        1.08E-11      1.43E-IO    2.99E-10    5.IOE-06    6.22E-09      5.40E-05 Th-230                        472,037,000                        3.59E-l I    l.81E-10    3.66E-10      l.70E-05    8.40E-04      3.59E-04 Th-232                        472,037,000                        O.OOE+OO      l.OOE-10    2.67E-10    O.OOE+OO    O.OOE+OO      O.OOE+OO U-233/234                    472,037,000                        2.73E-10      2.SIE-10      3.43E-10    1.29E-04    2.07E-02      9.llE-04 U-235/236                    472,037,000                        1.90E-ll      1.42E-10    2.89E-10    8.96E-06    4.ISE+OO      6.33E-05 U-238                        472,037,000                        5.64E-l l      l.58E-IO    2.82E-10    2.66E-05    7.95E+Ol      1.88E-04 Total:    1.58E-03 Sewer Pu-238                          25,036,000                      O.OOE+OO        l.l lE-10    2.41E-10    O.OOE+OO    O.OOE+OO      O.OOE+OO Pu-239/240                      25,036,000                      O.OOE+OO      1.22E-10      2.92E-10    O.OOE+OO    O.OOE+OO      O.OOE+OO Tc-99                            25,036,000                      3.62E-09      3.74E-08      6.SSE-08    9.05E-05    5.36E-03      6.03E-06 Th-228                          25,036,000                        l.88E-l l    2.43E-IO    4.88E-10    4.71E-07    5.75E-10      9.41E-06 Th-230                          25,036,000                        l.58E-10      3.08E-IO    4.97E-10    3.97E-06    l.96E-04      l.58E-04 Th-232                          2s,0J6,poo                      O.OOE+OO        l.68E-IO    3.93E-10    O.OOE+OO    O.OOE+OO      O.OOE+OO U-232                          25,036,000                        3.03E-ll      l.83E-IO    3.74E-10    7.59E-07    3.55E-08      5.0SE-05 U-233/234                        25,036,000                        l.8 !E-08    1.40E-09    2.9!E-10    4.54E-04    7.27E-02      6.04E-03 U-235/236                        25,036,000                      7.02E-10      3.03E-10      2.56E-10    l.76E-05    8.14E+OO      2.34E-04 U-238                            25,036,000                      2.57E-09      5.38E-IO      2.SSE-10    6.44E-05    l.92E+02      8.58E-04 Total:    7.36E-03 West Ditch Pu-238                        169,304,000                      O.OOE+OO      l.12E-10      2.79E-10  O.OOE+OO    O.OOE+OO      O.OOE+OO Pu-239/240                    169,304,000                      O.OOE+OO      l.22E-10      3.45E-10  O.OOE+OO    O.OOE+OO      O.OOE+OO Tc-99                          169,304,000                        5.83E-09    3.48E-08      6.06E-08    9.87E-04    5.84E-02      9.72E-05 Th-228                          169,304,000                        l.17E-ll      l.76E-10    3.92E-10      l.98E-06    2.4!E-09      5.84E-05 Th-230                          169,304,000                        7.71E-ll    2.ISE-10      4.03E-10      l.30E-05    6.46E-04      7.71E-04 Th-232                          169,304,000                      O.OOE+OO        1.25E-IO    2.76E-10    O.OOE+OO    0.00E+OO      O.OOE+OO U-233/234                      169,304,000                        l.SIE-08      l.40E-09    3.14E-10    2.56E-03    4.l lE-01    5.0SE-02 U-235/236                      169,304,000                        7.09E-10      3.SIE-10      2.SIE-10    l.20E-04    5.56E+O!      2.36E-03 U-238                          169,304,000                        l.53E-09      4.SIE-10      2.33E-10    2.59E-04    7.72E+02      5.09E-03 Total:  5.89E-02 WWTF Am-241                            3,947,307                    O.OOE+OO      9.48E-11      2.19E-10    O.OOE+OO    O.OOE+OO      O.OOE+OO Cs-137                            3,947,307                    O.OOE+OO      l.24E-09      l.43E-09    O.OOE+OO    O.OOE+OO      O.OOE+OO Na-22                              3,947,307                      8.95E-11      8.13E-10      l.39E-09    3 .53E-07    5.66E-11      l .49E-05 Np-237                            3,947,307                      2.61E-l l    2.74E-IO      5.62E-IO    l.03E-07    1.46E-04      l.3 IE-03 Pb-212                            3,947,307                      1.20E-09      3.35E-09      3.02E-09    4.72E-06    3.41E-12      5.98E-04 Pu-238                            3,947,307                      l.33E-l l    5.35E-l l    l.07E-10    5.27E-08    3.08E-09      6.67E-04 1
ECV: Effluent Concentration Value from 10-CFR-20, Appendix B.
ECV: Effluent Concentration Value from 10-CFR-20, Appendix B.
Note: A value of "a~ was substituted for negative analytical results.
Printed: 08/04/2021                                                                  NFS-EDM S                                            Page I of2 Page 4 of 13


21G-21-0103 GOV-01-55 ACF-21-0182 Radioact ivity in Effluent Liquid January 1, 2021 to June 30, 2021 Total                  Activity      Error                Quantity  Quantity        Fraction Volume              Concentration    Estimate      LLD      Released  Released          of Location                                (I)                                                                                      1
(µCi/ml)    (µCi/ml)  (µCi/ml)        (Ci)        (g)          ECV WWTF Pu-239/240                        3,947,307                    O.OOE+OO    6.32E-l 1    I.57E-IO  O.OOE+OO  O.OOE+OO    O.OOE+OO Pu-241                            3,947,307                    4.56E-IO    I.OIE-08    I. 74E-08  l.SOE-06  1.75E-08    4.56E-04 Ra-224                            3,947,307                      l.20E-08  6.69E-09    l.20E-08    4.73E-05  2.98E-IO    5.99E-02 Tc-99                            3,947,307                    4.75E-09    l.30E-07  2.24E-07    1.87E-05    I.I IE-03  7.91E-05 Th-228                            3,947,307                    O.OOE+OO    I.SIE-10    3.74E-IO    O.OOE+OO  O.OOE+OO    O.OOE+OO Th-230                            3,947,307                      l.16E-10  2.23E-IO    3.87E-10    4.60E-07    2.28E-05    l.16E-03 Th-231                            3,947,307                    O.OOE+OO    3.98E-08    3.89E-08    O.OOE+OO  O.OOE+OO    O.OOE+OO Th-232                            3,947,307                    3.63E-II    l.33E-IO    2.37E-IO    1.43E-07  1.3 IE+OO    l.21E-03 U-232                            3,947,307                    O.OOE+OO    I.ISE-10    2.45E-IO    O.OOE+OO  O.OOE+OO    O.OOE+OO U-233/234                        3,947,307                    l.34E-08    9.28E-IO    1.75E-IO    5.30E-05    8.50E-03    4.48E-02 U-235/236                        3,947,307                    5.96E-IO    2.06E-IO    l.06E-IO    2.35E-06  l.09E+OO      l.99E-03 U-238                            3,947,307                      9.75E-l l  l.02E-10    l.34E-IO    3.85E-07  I.ISE+OO    3.25E-04 Total:  1.IJE-01 ECV: Effluent Concentration Value from 10-CFR-20, Appendix B.
Note: A value of "O" was substituted for negative analytical results.
Note: A value of "O" was substituted for negative analytical results.
Printed: 08/04/2021                                                             NFS-EDMS                                         Page 2 of2 Page 5 of 13
Printed: 08/04/2021 NFS-EDMS Page 2 of2


21G-21-0103 GOV-01-55 ACF-21-0182 Attachment 2 To Letter Dated August 16, 2021 Report of Radioactivity in Effluent Air for the Period January to June 2021 (3 Pages to Follow)
Page 5 of 13 21G-21-0103 GOV-01-55 ACF-21-0182
Page 6 of 13


21G-21-0103 GOV-01-55 ACF-21-0182 Radioa ctivity in Efflue nt Air Janua ry 1, 2021 to June 30, 2021 Total                   Activity                       Error                                         Quantity                   Quantity             Fraction Volume             Concentration                   Estimate                       LLD               Released                   Released                 of Location                               (mJ)                   (µCi/ml)                   (µCi/ml)                                                                                                 1
Attachment 2 To Letter Dated August 16, 2021
(µCi/ml)                   (Ci)                         (g)               ECV Main Stack 416                                                         1070.66 m3/min                   17.84 m3tsec Th-228                         282,139,411                       6.58E-16                   l.50E-16                   8.16E-I 7               I.86E-07                   2.27E-10         3.29£-02 Th-230                         282,139,411                       6.58E-16                   l.50E-16                   8. 16E-l 7             l.86E-07                   9.19E-06         3.29E-02 Th-232                         282,139,411                       4.94E-16                 1.13E-16                     6.12E-17               l.39E-07                   l.28E+00           l.23E-0l U-234                           282,139,411                       l.55E-13                 3.54E-14                     l.92E-l 4             4.38E-05                     7.02E-03       3.I0E+00 U-235                           282,139,411                       5.92E-15                 l.35E-15                     7.35E-16               I.67E-06                     7.74E-0l         9.87E-02 U-238                           282,139,411                       l.65E-15                 3.76E-16                     2.04E-16               4.64E-07                   l.39E+00         2.74E-02 Total:     3.42E+00 Stack 185 Bldg. 131                                                     112.74 m /min 3 1.88 m3tsec Pu-241                           29,384,273                       4.92E-16                 9.20E-16                     l.62E-15               l.45E-08                   l.40E-10         6.!6E-04 Tc-99                             29,384,273                       l.59E-14                 2.98E-14                     5.23E-14               4.68E-07                     2.77E-05         1.77£-05 U-234                             29,384,273                     2.42E-16                 7.61E-15                     l.93E-14               7.12E-09                     l.14E-06         4.85E-03 U-235                             29,384,273                     7.50E-18                 2.36E-16                     5.98E-16               2.20E-I0                     l.02E-04         l.25E-04 Total:     5.61E-03 Stack 234 Bldg. 234                                                     328.49 m3/min                   5.47 m3tsec Am-241                           85,678,107                     5.83E-l 7                 2.63E-17                     4.34E-l 7             5.00E-09                     I .46E-09       2.92E-03 Pu-238                           85,678,107                     7.13E-l 7                 3.22E-l7                     5.30E-17               6.I IE-09                   3.57E-10         3.56E-03 Pu-239/240                       85,678,107                     2.53E-16                 l.14E-16                     l.88E-l6               2.16E-08                   3.48E-07         l.26E-02 Pu-241                           85,678,107                     4.78E-15                 4.34E-15                     7.l3E-15               4.09E-07                   3.98E-09         5.97E-03 Th-228                           85,678,107                     3.89E-l 7                 l.75E-l 7                   2.89E-17               3.33E-09                   4.07E-12         l.94E-03 Th-230                           85,678,107                     4.86E-16                 2.19E-16                     3.62E-l6               4.16E-08                     2.06E-06         2.43E-02 Th-232                           85,678,107                     6.15E-l6                 2.78E-16                     4.58E-16               5.27E-08                     4.84E-0I         1.54E-0l U-234                           85,678,107                       l.33E-15                 5.99E-l6                     9.89E-l6               l.14E-07                   1.82E-05         2.66E-02 U-238                             85,678,107                     3.89E-16                 l.75E-16                     2.89E-l6               3.33E-08                     9.94E-02         6.48E-03 Total:     2.38E-0l Stack 327 Bldg. 330                                                     1036.36 m3/min                 17.27 m3tsec Pu-241                         270,157,102                       2.50E-15                 5.19E-l6                     7.28E-16               6.75E-07                     6.55E-09         3.12E-03 Tc-99                           270,157,102                       8.08E-14                 l.68E-14                     2.35E-l4               2.18E-05                     l.29E-03         8.98E-05 U-234                         270,157,102                       1.40E-13                 l.3 IE-14                   8.78E-15               3.77£-05                     6.05E-03       2.79E+00 U-235                         270,157,102                       4.32E-15                 4.05E-16                     2.71E-l6               l.l 7E-06                   5.40E-01         7.20E-02 Total:     2.87E+00 Stack 421 Bldg. 100                                                       32.96 m 3/min                 0.55 m3tsec Pu-241                             8,590,906                     3.61E-l5                 l.28E-15                     l.95E-15             3. I0E-08                   3.0IE-10         4.51E-03 Tc-99                               8,590,906                     1.17E-13                 4.15E-14                     6.30E-14               I.00E-06                   5.93E-05         l.30E-04 U-234                             8,590,906                     1.26E-l4                 1.29E-14                     2.12E-14               1.08E-07                   l.74E-05         2.52E-0l U-235                               8,590,906                     3.90E-16                 3.98£-16                     6.55E-16               3.35E-09                     l.55E-03         6.50E-03 Total:     2.63E-0l Stack 424 Bldg. 100                                                       32.62 m 3/min                 0.54 m3/sec Pu-241                             8,502,340                     1.29E-15                 l.02E-15                     1.57E-l 5             l.09E-08                     l.06E-10         l.6 IE-03 Tc-99                               8,502,340                   4.16E-14                 3.31E-14                     5.0SE-14               3.54E-07                   2.09E-05         4.62E-05 ECV: Effluent Concentralion Value from 10-CFR-20, Appendix B. Fraction o*f ECV at the stack is provided for rererence only. Concentrations at off-site locations significantly less than those reported here (at stack) due to the atmospheric dispersion                                                                               are that occurs before the effluent exits the site.
 
Report of Radioactivity in Effluent Air for the Period January to June 2021
 
(3 Pages to Follow)
 
Page 6 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Air January 1, 2021 to June 30, 2021
 
Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of Location (mJ) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Main Stack 416 1070.66 m 3/min 17.84 m3tsec Th-228 282,139,411 6.58E-16 l.50E-16 8.16E-I 7 I.86E-07 2.27E-10 3.29£-02 Th-230 282,139,411 6.58E-16 l.50E-16 8. 16E-l 7 l.86E-07 9.19E-06 3.29E-02 Th-232 282,139,411 4.94E-16 1.13E-16 6.12E-17 l.39E-07 l.28E+00 l.23E-0l U-234 282,139,411 l.55E-13 3.54E-14 l.92E-l 4 4.38E-05 7.02E-03 3.I0E+00 U-235 282,139,411 5.92E-15 l.35E-15 7.35E-16 I.67E-06 7.74E-0l 9.87E-02 U-238 282,139,411 l.65E-15 3.76E-16 2.04E-16 4.64E-07 l.39E+00 2.74E-02
 
Total: 3.42E+00 Stack 185 Bldg. 131 112.74 m 3/min 1.88 m3tsec Pu-241 29,384,273 4.92E-16 9.20E-16 l.62E-15 l.45E-08 l.40E-10 6.!6E-04 Tc-99 29,384,273 l.59E-14 2.98E-14 5.23E-14 4.68E-07 2.77E-05 1.77£-05 U-234 29,384,273 2.42E-16 7.61E-15 l.93E-14 7.12E-09 l.14E-06 4.85E-03 U-235 29,384,273 7.50E-18 2.36E-16 5.98E-16 2.20E-I0 l.02E-04 l.25E-04
 
Total: 5.61E-03 Stack 234 Bldg. 234 328.49 m 3/min 5.47 m3tsec Am-241 85,678,107 5.83E-l 7 2.63E-17 4.34E-l 7 5.00E-09 I.46E-09 2.92E-03 Pu-238 85,678,107 7.13E-l 7 3.22E-l7 5.30E-17 6.I IE-09 3.57E-10 3.56E-03 Pu-239/240 85,678,107 2.53E-16 l.14E-16 l.88E-l6 2.16E-08 3.48E-07 l.26E-02 Pu-241 85,678,107 4.78E-15 4.34E-15 7.l3E-15 4.09E-07 3.98E-09 5.97E-03 Th-228 85,678,107 3.89E-l 7 l.75E-l 7 2.89E-17 3.33E-09 4.07E-12 l.94E-03 Th-230 85,678,107 4.86E-16 2.19E-16 3.62E-l6 4.16E-08 2.06E-06 2.43E-02 Th-232 85,678,107 6.15E-l6 2.78E-16 4.58E-16 5.27E-08 4.84E-0I 1.54E-0l U-234 85,678,107 l.33E-15 5.99E-l6 9.89E-l6 l.14E-07 1.82E-05 2.66E-02 U-238 85,678,107 3.89E-16 l.75E-16 2.89E-l6 3.33E-08 9.94E-02 6.48E-03
 
Total: 2.38E-0l Stack 327 Bldg. 330 1036.36 m 3/min 17.27 m3tsec Pu-241 270,157,102 2.50E-15 5.19E-l6 7.28E-16 6.75E-07 6.55E-09 3.12E-03 Tc-99 270,157,102 8.08E-14 l.68E-14 2.35E-l4 2.18E-05 l.29E-03 8.98E-05 U-234 270,157,102 1.40E-13 l.3 IE-14 8.78E-15 3.77£-05 6.05E-03 2.79E+00 U-235 270,157,102 4.32E-15 4.05E-16 2.71E-l6 l.l 7E-06 5.40E-01 7.20E-02
 
Total: 2.87E+00 Stack 421 Bldg. 100 32.96 m 3/min 0.55 m3tsec Pu-241 8,590,906 3.61E-l5 l.28E-15 l.95E-15 3. I0E-08 3.0IE-10 4.51E-03 Tc-99 8,590,906 1.17E-13 4.15E-14 6.30E-14 I.00E-06 5.93E-05 l.30E-04 U-234 8,590,906 1.26E-l4 1.29E-14 2.12E-14 1.08E-07 l.74E-05 2.52E-0l U-235 8,590,906 3.90E-16 3.98£-16 6.55E-16 3.35E-09 l.55E-03 6.50E-03
 
Total: 2.63E-0l Stack 424 Bldg. 100 32.62 m 3/min 0.54 m 3/sec Pu-241 8,502,340 1.29E-15 l.02E-15 1.57E-l 5 l.09E-08 l.06E-10 l.6 IE-03 Tc-99 8,502,340 4.16E-14 3.31E-14 5.0SE-14 3.54E-07 2.09E-05 4.62E-05
 
ECV: Effluent Concentralion Value from 10-CFR-20, Appendix B. Fraction o*f ECV at the stack is provided for rererence only. Concentrations at off-site significantly less than those reported here (at stack) due to the atmospheric dispersion that occurs before the effluent locations are exits the site.
Note: A value of "O~ was substituted for negative analytical results.
Note: A value of "O~ was substituted for negative analytical results.
Printed: 08/04/2021                                                                               NFS-EDM S                                                                                Page 1 of3 Page 7 of 13
Printed: 08/04/2021 NFS-EDMS Page 1 of3
 
Page 7 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Air January 1, 2021 to June 30, 2021
 
Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of Location (m3) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Stack 424 Bldg. 100 32.62 m 3/min 0.54 m3/sec U-234 8,502,340 8.14E-15 l.09E-14 1.88E-14 6.92E-08 l.llE-05 l.63E-01 U-235 8,502,340 2.52E-16 3.38E-16 5.SIE-16 2.14E-09 9.91E-04 4.20E-03
 
Total: l.69E-0l Stack 573 Bldg 306-W 120.88 m 3/min 2.01 m3/sec Pu-241 31,507,371 3.97E-16 8.ISE-16 l.49E-15 l.25E-08 l.21E-10 4.96E-04 Tc-99 31,507,371 1.28E-14 2.64E-14 4.SIE-14 4.04E-07 2.39E-05 l.43E-05 U-234 31,507,371 1.78E-16 6.65E-15 1.SOE-14 5.60E-09 8.98E-07 3.56E-03 U-235 31,507,371 5.SOE-18 2.06E-16 5.57E-16 l.73E-10 8.02E-05 9.16E-05
 
Total: 4.16E-03 Stack 600 Bldg. 110 319.61 m 3/min 5.33 m 3/sec Pu-241 83,303,746 1.23E-15 5.93E-16 9.73E-16 l.03E-07 9.99E-IO 1.54E-03 Tc-99 83,303,746 3.99E-14 l.92E-14 3.ISE-14 3.33E-06 l.97E-04 4.44E-05 U-234 83,303,746 2.46E-14 8.07E-15 1.22E-14 2.0SE-06 3.29E-04 4.92E-01 U-235 83,303,746 7.61E-16 2.SOE-16 3.78E-16 6.34E-08 2.94E-02 l.27E-02
 
Total: 5.06E-01 Stack 615 Bldg. 306-W 48.41 m 3/min 0.81 m 3/sec Pu-241 12,618,460 3.07E-16 8.62E-16 l.57E-15 3.88E-09 3.77E-ll 3.84E-04 Tc-99 12,618,460 9.94E-15 2.79E-14 5.0SE-14 1.25E-07 7.42E-06 l.lOE-05 U-234 12,618,460 3.02E-16 7.32E-15 1.88E-14 3.SIE-09 6.IOE-07 6.03E-03 U-235 12,618,460 9.33E-18 2.26E-16 5.SIE-16 l.lSE-10 5.45E-05 l.55E-04
 
Total: 6.58E-03 Stack 646 Bldg. 110 37.49 m 3/min 0.62 m 3/sec Pu-241 9,771,787 5.32E-16 9.0IE-16 l.57E-15 5.20E-09 5.0SE-ll 6.65E-04 Tc-99 9,771,787 l.72E-14 2.91E-14 5.07E-14 l.68E-07 9.94E-06 l.91E-05 U-234 9,771,787 9.59E-16 7.68E-15 l.88E-14 9.38E-09 l.SOE-06 l.92E-02 U-235 9,771,787 2.97E-17 2.38E-16 5.SOE-16 2.90E-10 l.34E-04 4.95E-04
 
Total: 2.04E-02 Stack 701 Bldg. 307 119.13 m 3/min 1.99 m 3/sec Pu-241 31,049,779 3.58E-!6 9.91E-16 I.SOE-IS l.llE-08 I.OSE-10 4.47E-04 Tc-99 31,049,779 l.16E-14 3.20E-14 5.84E-14 3.59E-07 2.13E-05 l.29E-05 U-234 31,049,779 2.60E-15 9.65E-15 2.16E-14 8.07E-08 l.29E-05 5.20E-02 U-235 31,049,779 8.04E-17 2.99E-16 6.67E-16 2.SOE-09 l.16E-03 l.34E-03
 
Total: 5.38E-02 Stack 702 Bldg. 307 158.63 m 3/min 2.64 m 3/sec Pu-241 41,345,582 3.63E-16 8.72E-16 l.57E-15 l.SOE-08 l.46E-IO 4.53E-04 Tc-99 41,345,582 I.I 7E-14 2.82E-14 5.0SE-14 4.85E-07 2.87E-05 1.30E-05 U-234 41,345,582 2.35E-15 8.30E-15 l.88E-14 9.7IE-08 l.56E-05 4.70E-02
 
ECV: Effluent Concentration Value from 10-CFR-20, Appendix B. Fraction of ECV at the stack Is provided for reference only. Concentrations at off-site locations are significantly less than those reported here (at stack) due to the atmospheric dispersion that occurs before the effluent exits the Site.


21G-21-0103 GOV-01-55 ACF-21-0182 Radioa ctivity in Effluen t Air Januar y 1, 2021 to June 30, 2021 Total                  Activity                    Error                                          Quantity                    Quantity            Fraction Volume              Concentration                    Estimate                      LLD                  Released                    Released                of Location                                (m3)                  (µCi/ml)                  (µCi/ml)                  (µCi/ml)                                                                        1 (Ci)                        (g)                ECV Stack 424 Bldg. 100                                                      32.62 m3/min                  0.54 m3/sec U-234                              8,502,340                      8.14E-15                l.09E-14                    1.88E-14                6.92E-08                    l.llE-05        l.63E-01 U-235                              8,502,340                      2.52E-16                3.38E-16                      5.SIE-16                2.14E-09                    9.91E-04        4.20E-03 Total:      l.69E-0l Stack 573 Bldg 306-W                                                    120.88 m3/min                  2.01 m3/sec Pu-241                          31,507,371                      3.97E-16                8.ISE-16                      l.49E-15                l.25E-08                    l.21E-10        4.96E-04 Tc-99                            31,507,371                      1.28E-14                2.64E-14                    4.SIE-14                4.04E-07                    2.39E-05          l.43E-05 U-234                            31,507,371                      1.78E-16                6.65E-15                    1.SOE-14                5.60E-09                    8.98E-07        3.56E-03 U-235                            31,507,371                      5.SOE-18                2.06E-16                    5.57E-16                l.73E-10                    8.02E-05        9.16E-05 Total:      4.16E-03 Stack 600 Bldg. 110                                                      319.61 m3/min                  5.33 m3/sec Pu-241                          83,303,746                      1.23E-15                5.93E-16                    9.73E-16                l.03E-07                    9.99E-IO        1.54E-03 Tc-99                            83,303,746                      3.99E-14                l.92E-14                    3.ISE-14                3.33E-06                    l.97E-04        4.44E-05 U-234                            83,303,746                      2.46E-14                8.07E-15                      1.22E-14                2.0SE-06                    3.29E-04          4.92E-01 U-235                            83,303,746                      7.61E-16                2.SOE-16                    3.78E-16                6.34E-08                    2.94E-02          l.27E-02 Total:      5.06E-01 Stack 615 Bldg. 306-W                                                    48.41 m3/min                  0.81 m3/sec Pu-241                            12,618,460                      3.07E-16                8.62E-16                      l.57E-15                3.88E-09                    3.77E-ll        3.84E-04 Tc-99                            12,618,460                      9.94E-15                2.79E-14                    5.0SE-14                1.25E-07                    7.42E-06          l.lOE-05 U-234                            12,618,460                      3.02E-16                7.32E-15                    1.88E-14                3.SIE-09                    6.IOE-07        6.03E-03 U-235                            12,618,460                      9.33E-18                2.26E-16                    5.SIE-16                l.lSE-10                    5.45E-05          l.55E-04 Total:      6.58E-03 Stack 646 Bldg. 110                                                        37.49 m3/min                  0.62 m3/sec Pu-241                            9,771,787                      5.32E-16                9.0IE-16                    l.57E-15                5.20E-09                    5.0SE-ll        6.65E-04 Tc-99                              9,771,787                      l.72E-14                2.91E-14                      5.07E-14                l.68E-07                  9.94E-06          l.91E-05 U-234                              9,771,787                      9.59E-16                7.68E-15                    l.88E-14                9.38E-09                    l.SOE-06        l.92E-02 U-235                              9,771,787                    2.97E-17                2.38E-16                    5.SOE-16                2.90E-10                    l.34E-04        4.95E-04 Total:    2.04E-02 Stack 701 Bldg. 307                                                      119.13 m3/min                  1.99 m3/sec Pu-241                          31,049,779                      3.58E-!6                9.91E-16                      I.SOE-IS                l.llE-08                    I.OSE-10        4.47E-04 Tc-99                            31,049,779                      l.16E-14                3.20E-14                    5.84E-14                3.59E-07                    2.13E-05          l.29E-05 U-234                            31,049,779                      2.60E-15                9.65E-15                    2.16E-14                8.07E-08                    l.29E-05        5.20E-02 U-235                            31,049,779                      8.04E-17                2.99E-16                    6.67E-16                2.SOE-09                    l.16E-03          l.34E-03 Total:    5.38E-02 Stack 702 Bldg. 307                                                      158.63 m3/min                  2.64 m3/sec Pu-241                            41,345,582                      3.63E-16                8.72E-16                    l.57E-15                l.SOE-08                    l.46E-IO        4.53E-04 Tc-99                            41,345,582                      I.I 7E-14                2.82E-14                    5.0SE-14                4.85E-07                    2.87E-05          1.30E-05 U-234                            41,345,582                      2.35E-15                8.30E-15                    l.88E-14                9.7IE-08                    l.56E-05        4.70E-02 ECV: Effluent Concentration Value from 10-CFR-20, Appendix B. Fraction of ECV at the stack Is provided for reference only. Concentrations at off-site locations are significantly less than those reported here (at stack) due to the atmospheric dispersion that occurs before the effluent exits the Site.
Note: A value of "O" was substituted for negative analytical results.
Note: A value of "O" was substituted for negative analytical results.
Printed: 08/04/2021                                                                             NFS-EDMS                                                                                   Page 2 of3 Page 8 of 13
Printed: 08/04/2021 NFS-EDMS Page 2 of3
 
Page 8 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Air January 1, 2021 to June 30, 2021
 
Total Activity Error Quantity Quantity Fraction Volume Coucentratiou Estimate LLD Released Released of Location (ml) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Stack 702 Bldg. 307 158.63 ml/min 2.64 m3tsec U-235 41,345,582 7.27E-l 7 2.57E-16 5.81E-!6 3.00E-09 l.39E-03 l.21E-03
 
Total: 4.87E-02 Stack 703 Exhaust Room Air 776.96 ml/min 12.95 m3tsec Pu-241 202,506,263 9.09E-15 2.57E-14 4.69E-14 l.84E-06 l.79E-08 l.14E-02 Th-228 202,506,263 l.76E-16 7.41E-16 1.72E-15 3.56E-08 4.35E-ll 8.S0E-03 Th-230 202,506,263 l.0!E-16 4.26E-16 9.SSE-16 2.05E-08 l.02E-06 5.06E-03 Th-232 202,506,263 1.44E-16 6.06E-16 1.40E-15 2.91E-08 2.67E-0l 3.60E-02 U-234 202,506,263 1.!0E-15 4.64E-15 1.07E-14 2.23E-07 3.58E-05 2.20E-02 U-235 202,506,263 l.14E-16 4.79E-!6 1.l lE-15 2.30E-08 l.07E-02 l.90E-03 U-238 202,506,263 l.39E-16 5.84E-16 l.35E-15 2.SIE-08 8.38E-02 2.3 !E-03
 
Total: 8.74E-02 Stack 773 Bldg. 440 166.92 ml/min 2.78 m3tsec Pu-241 43,576,819 2.!0E-14 3.53E-14 6. !SE-14 9. l 7E-07 8.90E-09 2.63E-02 Th-228 43,576,819 1.98E-16 1.31E-15 3.23E-15 8.61E-09 l.05E-ll 9.88E-03 Th-230 43,576,819 2.54E-!6 l.68E-!5 4.15E-15 1.llE-08 5.48E-07 l.27E-02 Th-232 43,576,819 1.69E-16 l.12E-15 2.76E-15 7.38E-09 6.77E-02 4.23E-02 U-234 43,576,819 5.22E-16 3.46E-15 8.52E-15 2.28E-08 3.65E-06 1.04E-02 U-235 43,576,819 9.18E-17 6.07E-!6 1.50E-15 4.00E-09 l.85E-03 l.53E-03 U-238 43,576,819 !.84E-16 l.21E-15 2.99E-15 8.00E-09 2.39E-02 3.06E-03
 
Total: l.06E-0l Stack 774 Bldg. 301 319.16 ml/min 5.32 m3tsec Th-228 83,185,658 5.43E-18 1.71E-!6 4.29E-16 4.52E-10 5.5!E-13 2.71E-04 Th-230 83,185,658 1.85E-l 7 5.SIE-16 1.46E-15 l.54E-09 7.62E-08 9.25E-04 Th-232 83,185,658 l.l0E-17 3.45E-16 8.67E-16 9.12E-10 8.37E-03 2.74E-03 U-234 83,185,658 4.94E-l 7 l.55E-15 3.91E-15 4. llE-09 6.59E-07 9.SSE-04 U-235 83,185,658 3.21E-18 1.0IE-16 2.54E-!6 2.67E-10 l.24E-04 5.35E-05 U-238 83,185,658 2.33E-l 7 7.31E-!6 1.84E-15 l.94E-09 5.78E-03 3.SSE-04
 
Total: 5.37E-03 Stack 796 Bldg. 100 19.37 ml/min 0.32 m3tsec Pu-241 5,048,265 8.86E-16 9.59E-!6 l.57E-15 4.47E-09 4.34E-11 l.l lE-03 Tc-99 5,048,265 2.87E-14 3.I0E-14 5.0SE-14 1.45E-07 8.56E-06 3.ISE-05 U-234 5,048,265 0.00E+00 7.14E-15 l.88E-14 0.00E+00 0.00E+00 0.00E+00 U-235 5,048,265 0.00E+00 2.21E-16 5.SIE-16 0.00E+00 0.00E+00 0.00E+00
 
Total: l.14E-03
 
ECV: Effluent concentration Value from 10-CFR-20, Appendix B. Fraction of ECV at the stack is provided for reference only. Concentrations at off-site locations are significantly less than those reported here (al stack) due to the atmospheric dispersion that occurs before the effluent exits the site.


21G-21-0103 GOV-01-55 ACF-21-0182 Radioac tivity in Effluen t Air January 1, 2021 to June 30, 2021 Total                  Activity                    Error                                            Quantity                    Quantity              Fraction Volume              Coucentratiou                    Estimate                      LLD                  Released                    Released                  of Location                                (ml)                  (µCi/ml)                  (µCi/ml)                                                                                                    1
(µCi/ml)                    (Ci)                          (g)                ECV Stack 702 Bldg. 307                                                      158.63 ml/min                  2.64 m3tsec U-235                            41,345,582                      7.27E-l 7                2.57E-16                    5.81E-!6                3.00E-09                    l.39E-03          l.21E-03 Total:      4.87E-02 Stack 703 Exhaust Room Air                                              776.96 ml/min                  12.95 m3tsec Pu-241                          202,506,263                      9.09E-15                  2.57E-14                    4.69E-14                l.84E-06                    l.79E-08            l.14E-02 Th-228                          202,506,263                      l.76E-16                7.41E-16                      1.72E-15              3.56E-08                    4.35E-ll          8.S0E-03 Th-230                          202,506,263                      l.0!E-16                4.26E-16                    9.SSE-16                2.05E-08                    l.02E-06          5.06E-03 Th-232                          202,506,263                      1.44E-16                6.06E-16                    1.40E-15                2.91E-08                    2.67E-0l          3.60E-02 U-234                          202,506,263                      1.!0E-15                4.64E-15                    1.07E-14                2.23E-07                    3.58E-05          2.20E-02 U-235                          202,506,263                      l.14E-16                4.79E-!6                      1.l lE-15              2.30E-08                    l.07E-02          l.90E-03 U-238                          202,506,263                      l.39E-16                5.84E-16                    l.35E-15                2.SIE-08                    8.38E-02          2.3 !E-03 Total:      8.74E-02 Stack 773 Bldg. 440                                                      166.92 ml/min                  2.78 m3tsec Pu-241                            43,576,819                      2.!0E-14                3.53E-14                      6. !SE-14              9. l 7E-07                  8.90E-09          2.63E-02 Th-228                            43,576,819                      1.98E-16                  1.31E-15                    3.23E-15                8.61E-09                    l.05E-ll          9.88E-03 Th-230                            43,576,819                      2.54E-!6                  l.68E-!5                    4.15E-15                1.llE-08                    5.48E-07            l.27E-02 Th-232                            43,576,819                      1.69E-16                  l.12E-15                    2.76E-15                7.38E-09                    6.77E-02          4.23E-02 U-234                            43,576,819                      5.22E-16                3.46E-15                    8.52E-15                2.28E-08                    3.65E-06            1.04E-02 U-235                            43,576,819                      9.18E-17                6.07E-!6                      1.50E-15              4.00E-09                    l.85E-03          l.53E-03 U-238                            43,576,819                      !.84E-16                  l.21E-15                    2.99E-15                8.00E-09                    2.39E-02          3.06E-03 Total:      l.06E-0l Stack 774 Bldg. 301                                                      319.16 ml/min                    5.32 m3tsec Th-228                            83,185,658                      5.43E-18                1.71E-!6                    4.29E-16                4.52E-10                    5.5!E-13          2.71E-04 Th-230                            83,185,658                      1.85E-l 7                5.SIE-16                    1.46E-15                l.54E-09                    7.62E-08          9.25E-04 Th-232                            83,185,658                      l.l0E-17                3.45E-16                    8.67E-16                9.12E-10                    8.37E-03          2.74E-03 U-234                            83,185,658                    4.94E-l 7                l.55E-15                    3.91E-15                4. llE-09                    6.59E-07          9.SSE-04 U-235                            83,185,658                    3.21E-18                  1.0IE-16                    2.54E-!6                2.67E-10                    l.24E-04          5.35E-05 U-238                            83,185,658                    2.33E-l 7                7.31E-!6                      1.84E-15                l.94E-09                    5.78E-03          3.SSE-04 Total:      5.37E-03 Stack 796 Bldg. 100                                                      19.37 ml/min                  0.32 m3tsec Pu-241                              5,048,265                    8.86E-16                9.59E-!6                      l.57E-15              4.47E-09                    4.34E-11            l.l lE-03 Tc-99                              5,048,265                    2.87E-14                3.I0E-14                      5.0SE-14                1.45E-07                    8.56E-06          3.ISE-05 U-234                              5,048,265                    0.00E+00                  7.14E-15                      l.88E-14              0.00E+00                    0.00E+00          0.00E+00 U-235                              5,048,265                    0.00E+00                  2.21E-16                    5.SIE-16              0.00E+00                    0.00E+00          0.00E+00 Total:      l.14E-03 ECV: Effluent concentration Value from 10-CFR-20, Appendix B. Fraction of ECV at the stack is provided for reference only. Concentrations at off-site locations are significantly less than those reported here (al stack) due to the atmospheric dispersion that occurs before the effluent exits the site.
Note: A value of "O" was substituted for negative analytical results.
Note: A value of "O" was substituted for negative analytical results.
Printed: 08/04/2021                                                                             NFS-EDMS                                                                                   Page 3 of3 Page 9 of 13
Printed: 08/04/2021 NFS-EDMS Page 3 of3
 
Page 9 of 13 21G-21-0103 GOV-01-55 ACF-21-0182
 
Attachment 3 To Letter Dated August 16, 2021
 
Report of Gaseous Effluent Dose and Activity Concentrations for the Maximally Exposed Off-Site Individual for the Release Period January to June 2021
 
(3 Pages to Follow)


21G-21-0103 GOV-01-55 ACF-21-0182 Attachment 3 To Letter Dated August 16, 2021 Report of Gaseous Effluent Dose and Activity Concentrations for the Maximally Exposed Off-Site Individual for the Release Period January to June 2021 (3 Pages to Follow)
Page 10 of 13 21G-21-0103 GOV-01-55 ACF-21-0182
Page 10 of 13
 
Report of Potential Gaseous Effluent Dose to the Maximally Exposed Offsite Individual and on the Maximum Radionuclide Concentrations for the Period:
January to June 2021
 
Introduction During this biannual period, NRC License SNM-124, Section 9.1.1.3, required NFS to assess the total effective dose equivalent (TEDE) to the maximally exposed offsite receptor and the maximum radioactive air concentrations at the site boundary attributable to NFS' air effluents. The required biannual assessment has been completed and the details of the assessment are provided in the subsequent sections.


21G-21-0103 GOV-01-55 ACF-21-0182 Report of Potential Gaseous Effluent Dose to the Maximally Exposed Offsite Individual and on the Maximum Radionuclide Concentrations for the Period:
January to June 2021 Introduction During this biannual period, NRC License SNM-124, Section 9.1.1.3, required NFS to assess the total effective dose equivalent (TEDE) to the maximally exposed offsite receptor and the maximum radioactive air concentrations at the site boundary attributable to NFS' air effluents. The required biannual assessment has been completed and the details of the assessment are provided in the subsequent sections.
Summary of Methods In accordance with SNM-124, Section 9.1.1.4, and internal procedure NFS-HS-A-27, the U.S. Department of Energy's CAP88-PC computer program was used to estimate off-site doses and activity concentrations for gaseous effluents. NFS operated sixteen (16) radiological stacks during the first half of 2021. Based on effluent types and stack physical characteristics, releases from these stacks were grouped into effective stacks for modeling purposes. To accommodate the co-location limitation of the model, the effective stacks were taken to be at the approximate center of the plant site. The distance to the site boundary (nearest model receptor distance) was conservatively taken to be 150 meters for all sectors.
Summary of Methods In accordance with SNM-124, Section 9.1.1.4, and internal procedure NFS-HS-A-27, the U.S. Department of Energy's CAP88-PC computer program was used to estimate off-site doses and activity concentrations for gaseous effluents. NFS operated sixteen (16) radiological stacks during the first half of 2021. Based on effluent types and stack physical characteristics, releases from these stacks were grouped into effective stacks for modeling purposes. To accommodate the co-location limitation of the model, the effective stacks were taken to be at the approximate center of the plant site. The distance to the site boundary (nearest model receptor distance) was conservatively taken to be 150 meters for all sectors.
Meteorological data was based on the average wind speed and direction frequencies from the onsite meteorological tower covering the time period for this report.
Meteorological data was based on the average wind speed and direction frequencies from the onsite meteorological tower covering the time period for this report.
Atmospheric stability class D (neutral atmosphere) was used for all releases (default value recommended by the U.S. Environmental Protection Agency in "User's Guide for COMPLY"). The most conservative inhalation class was assumed for each radionuclide released. A particle size (activity median aerodynamic diameter or AMAD) of 1.0 micron was assumed for modeling purposes since no information on actual particle sizes exists.
Atmospheric stability class D (neutral atmosphere) was used for all releases (default value recommended by the U.S. Environmental Protection Agency in "User's Guide for COMPLY"). The most conservative inhalation class was assumed for each radionuclide released. A particle size (activity median aerodynamic diameter or AMAD) of 1.0 micron was assumed for modeling purposes since no information on actual particle sizes exists.
Because CAP88-PC models releases over an entire year, the six-month source term (i.e., total curies of each radionuclide released over the period, given in Attachment 2) was annualized (i.e., transformed into a 12-month release) so that airborne activity concentrations would not be under-estimated during the release period.
Because CAP88-PC models releases over an entire year, the six-month source term (i.e., total curies of each radionuclide released over the period, given in Attachment 2) was annualized (i.e., transformed into a 12-month release) so that airborne activity concentrations would not be under-estimated during the release period.
Summary of Results Doses are reported in Table 1 below and are derived from the CAP88-PC "Synopsis Report." These doses are at the location of the maximally exposed (off-site) individual (MEI). The results include an adjustment (using the normalization factor mentioned above) to convert the "annualized" doses back to those doses that were actually received in the six-month release period. Activity concentrations reported in Table 2 come directly from the CAP88-PC "Concentration Tables" report; no adjustments are needed for these concentrations. The CAP88-PC output reports are available for review at NFS.
Summary of Results Doses are reported in Table 1 below and are derived from the CAP88-PC "Synopsis Report." These doses are at the location of the maximally exposed (off-site) individual (MEI). The results include an adjustment (using the normalization factor mentioned above) to convert the "annualized" doses back to those doses that were actually received in the six-month release period. Activity concentrations reported in Table 2 come directly from the CAP88-PC "Concentration Tables" report; no adjustments are needed for these concentrations. The CAP88-PC output reports are available for review at NFS.
Page 11 of 13


21G-21-0103 GOV-01-55 ACF-21-0182 Table 1 summarizes the six-month dose to a hypothetical individual at the MEI location, which was determined to be approximately 550 meters North-Northeast from the center of the plant site. The TEDE to the MEI was estimated to be 3.2E-03 mrem for gaseous effluents released during the first half of 2021. The highest organ committed dose equivalent (COE) to the MEI was estimated to be 1.7E-02 mrem to the lungs. These MEI doses are well below the Environmental Radiological Monitoring Program action levels and applicable regulatory limits/ALARA constraints.
Page 11 of 13 21G-21-0103 GOV-01-55 ACF-21-0182
Table 1. Organ Doses and Total Effective Dose Equivalent at the MEI Location Organ                                       Committed Dose Equivalent (mrem per first half of 2021)
 
Adrenals                                   2.2E-04 Urinary Bladder Wall                       2.6E-04 Bone Surface                               9.2E-03 Brain                                     2.2E-04 Breasts                                   2.3E-04 Stomach Wall                               3.7E-03 Small Intestine                             2.5E-04 Upper Large Intestine Wall                 1.1 E-03 Lower Large Intestine Wall                 2.SE-03 Kidneys                                     2.SE-03 Liver                                       8.0E-04 Muscle                                     2.3E-04 Ovaries                                     2.4E-04 Pancreas                                   2.2E-04 Red Bone Marrow                             1.2E-03 Skin                                       4.5E-04 Spleen                                     2.2E-04 Testes                                     2.5E-04 Thymus                                     2.2E-04 Thyroid                                     1.9E-03 Gall Bladder Wall                           2.2E-04 Heart Wall                                 2.2E-04 Uterus                                     2.2E-04 Extra-thoracic                             1.5E-02 Lungs                                       1.7E-02 Total Effective Dose Equivalent             3.2E-03 mrem Location of MEI:                           550 meters North-Northeast Page 12 of 13
Table 1 summarizes the six-month dose to a hypothetical individual at the MEI location, which was determined to be approximately 550 meters North-Northeast from the center of the plant site. The TEDE to the MEI was estimated to be 3.2E-03 mrem for gaseous effluents released during the first half of 2021. The highest organ committed dose equivalent (COE) to the MEI was estimated to be 1.7E-02 mrem to the lungs. These MEI doses are well below the Environmental Radiological Monitoring Program action levels and applicable regulatory limits/ALARA constraints.
 
Table 1. Organ Doses and Total Effective Dose Equivalent at the MEI Location
 
Organ Committed Dose Equivalent (mrem per first half of 2021)
Adrenals 2.2E-04 Urinary Bladder Wall 2.6E-04 Bone Surface 9.2E-03 Brain 2.2E-04 Breasts 2.3E-04 Stomach Wall 3.7E-03 Small Intestine 2.5E-04 Upper Large Intestine Wall 1.1 E-03 Lower Large Intestine Wall 2.SE-03 Kidneys 2.SE-03 Liver 8.0E-04 Muscle 2.3E-04 Ovaries 2.4E-04 Pancreas 2.2E-04 Red Bone Marrow 1.2E-03 Skin 4.5E-04 Spleen 2.2E-04 Testes 2.5E-04 Thymus 2.2E-04 Thyroid 1.9E-03 Gall Bladder Wall 2.2E-04 Heart Wall 2.2E-04 Uterus 2.2E-04 Extra-thoracic 1.5E-02 Lungs 1.7E-02
 
Total Effective Dose Equivalent 3.2E-03 mrem Location of MEI: 550 meters North-Northeast
 
Page 12 of 13 21G-21-0103 GOV-01-55 ACF-21-0182
 
Table 2 summarizes the maximum radioactive air concentrations at or beyond the site boundary, as determined by CAP88-PC, for the radionuclides released. The total sum of fractions was estimated to be 5.SE-04 and indicates that exposures to the offsite public from gaseous effluents were much less than 1 % of the 10 CFR 20, Appendix B, Table 2, Col. 1 values for all offsite receptors including the site boundary. It is noted that the location of the maximum airborne concentration for a given radionuclide does not necessarily correspond to the MEI location. This is due primarily to the fact that the maximum concentrations for individual nuclides can vary due to differences in values input into the dispersion model for each of the effective stacks - such inputs include stack height, stack diameter, flow rate, and total radionuclide activities released per stack. Another reason for the disparity is the fact that the MEI dose includes both inhalation and ingestion pathways.


21G-21-0103 GOV-01-55 ACF-21-0182 Table 2 summarizes the maximum radioactive air concentrations at or beyond the site boundary, as determined by CAP88-PC, for the radionuclides released. The total sum of fractions was estimated to be 5.SE-04 and indicates that exposures to the offsite public from gaseous effluents were much less than 1% of the 10 CFR 20, Appendix B, Table 2, Col. 1 values for all offsite receptors including the site boundary. It is noted that the location of the maximum airborne concentration for a given radionuclide does not necessarily correspond to the MEI location. This is due primarily to the fact that the maximum concentrations for individual nuclides can vary due to differences in values input into the dispersion model for each of the effective stacks - such inputs include stack height, stack diameter, flow rate, and total radionuclide activities released per stack. Another reason for the disparity is the fact that the MEI dose includes both inhalation and ingestion pathways.
Table 2. Maximum Predicted Airborne Concentrations at or Beyond the Site Boundary
Table 2. Maximum Predicted Airborne Concentrations at or Beyond the Site Boundary
                                                                                                ~
 
Maximum Predicted Airbome Concentrations at or Beyond the Site: Boundary l\1aximum       Concenµ-~tion   10 CFR 20, App. B,       Ratio of Maximum
~
  ,* Nuclide   Concentration       Location     Table 2, Col. 1 Value     Concentration to .
Maximum Predicted Airbome Concentrations at
(l,ICi/mL)   Sector     Dist(m)     .(IJCi/mL)           10 CFR20 Value 99Tc       l.5E-17     NNE         450         9.E-10                   l.6E-08 22sTh 5.5E-20     NNE         650         2.E-14                   2.8E-06 230Th 8.lE-20     NNE         400         2.E-14                   4.0E-06 232Th       9.3E-20     NNE         300         4.E-15                   2.3E-05 234u 2.6E-17     NNE         550         5.E-14               . 5.3E-04 23s 0     8.7E-19     NNE         550         6.E-14                   l.5E-05 23su l.2E-19     NNE         650         6.E-14                 2.0E-06 23sPu 9.0E-21     NNE         250         2.E-14                 4.5E-07 239Pu 3.2E-20     NNE         250         2.E-14                   l.6E-06 241Pu 2.5E-18     NNE         400         8.E-13                 3.2E-06 241Am       7.4E-21     NNE         250         2.E-14                 3.7E-07 Sum of Fractions:             5.8Fr04 Page 13 of 13}}
 
'. or Beyond the Site: Boundary '. ' '
l\\1aximum Concenµ-~tion 10 CFR 20, App. B, Ratio of Maximum
,* Nuclide Concentration Location Table 2, Col. 1 Value Concentration to.
(l,ICi/mL) Sector Dist(m). (IJCi/mL) 10 CFR20 Value
 
99Tc l.5E-17 NNE 450 9.E-10 l.6E-08 22sTh 5.5E-20 NNE 650 2.E-14 2.8E-06 230Th 8.lE-20 NNE 400 2.E-14 4.0E-06 -*
 
232Th 9.3E-20 NNE 300 4.E-15 2.3E-05 234u 2.6E-17 NNE 550 5.E-14. 5.3E-04 23s 0 8.7E-19 NNE 550 6.E-14 l.5E-05
 
23su l.2E-19 NNE 650 6.E-14 2.0E-06
 
23sPu 9.0E-21 NNE 250 2.E-14 4.5E-07 239Pu 3.2E-20 NNE 250 2.E-14 l.6E-06
 
241Pu 2.5E-18 NNE 400 8.E-13 3.2E-06 241Am 7.4E-21 NNE 250 2.E-14 3.7E-07
 
Sum of Fractions: 5.8Fr04
 
Page 13 of 13}}

Latest revision as of 23:38, 19 November 2024

Nuclear Fuel Services, Inc - Biannual Effluent Monitoring Report January to June 2021
ML21238A011
Person / Time
Site: Erwin
Issue date: 08/16/2021
From: Knowles T
Nuclear Fuel Services
To:
Document Control Desk, Office of Nuclear Material Safety and Safeguards
References
21G-21-0103, ACF-21-0182, GOV-01-55
Download: ML21238A011 (13)


Text

Nuclear Fuel Services, Inc.

21G-21-0103 Certified Mail GOV-01-55 Return Receipt Requested ACF-21-0182 August 16, 2021 Director Office of Nuclear Material Safety & Safeguards U.S. Nuclear Regulatory Commission ATTN: Document Control Desk Washington, DC 20555-0001

Reference:

Docket No.70-143; SNM License 124

Subject:

Biannual Effluent Monitoring Report January to June 2021

Dear Director:

In accordance with the requirements set forth in 10 CFR Part 70.59, Nuclear Fuel Services, Inc. (NFS), submits the attached reports. Attachment 1 reports the Radioactivity in Effluent Liquid for the period January to June 2021. Attachment 2 reports the Radioactivity in Effluent Air for the period January to June 2021. Attachment 3 summarizes an evaluation of the dose and air activity concentrations for the maximally exposed offsite individual due to gaseous effluents during the period January to June 2021.

If you or your staff have any questions, require additional information, or wish to discuss this, please contact me or Mr. R. Jason Faddis, Environmental Safety Unit Manager, at (423) 735-5438. Please reference our unique document identification number (21G 0103) in any correspondence concerning this letter.

Sincerely,

NUCLEAR FUEL SERVICES, INC. IE4?

,:J~/~ !lflvj552D

Tim Knowles jl}Jv/55 Safety & Safeguards Director CJB/pj/smd Attachments

1) Report of Radioactivity in Effluent Liquid for the Period January to June 2021
2) Report of Radioactivity in Effluent Air for the Period January to June 2021
3) Report of Gaseous Effluent Dose and Activity Concentrations for the Maximally Exposed Off-Site Individual for the Release Period January to June 2021

1205 Banner Hill Rd, Erwin, TN 37650 Page 1 of 13 People Strong

t: +1.423.743.9141 f: +1.423.743.0140 www.nuclearfuelservices.com INNOVATION DRIVEN >

21G-21-0103 GOV-01-55 ACF-21-0182

Copy:

Mr. Joel Rivera-Ortiz

  • senior Fuel Facility Inspector U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257

Regional Administrator U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257

Mr. James Downs Fire Protection Engineer Division of Fuel Management Office of Nuclear Material Safety and Safeguards U.S. Nuclear Regulatory Commission Two White Flint North 11555 Rockville Pike Rockville, MD 20852-2738

Dr. Robert Williams Chief, Projects Branch 1 U.S. Nuclear Regulatory Commission Region II 245 Peachtree Center Ave., NE Suite 1200 Atlanta, GA 30303-1257

Mr. Larry Harris Senior Resident Inspector U.S. Nuclear Regulatory Commission

Page 2 of 13 21G-21-0103 GOV-01-55 ACF-21-0182

Attachment 1 To Letter Dated August 16, 2021

Report of Radioactivity in Effluent Liquid for the Period January to June 2021

(2 Pages to Follow)

Page 3 of 13 21 G-21-01 03 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Liquid January 1, 2021 to June 30, 2021

Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of Location (I) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Banner Spring Down Pu-238 472,037,000 0.00E+OO 8.57E-l l 2.28E-10 0.00E+OO O.OOE+OO O.OOE+OO Pu-239/240 472,037,000 O.OOE+OO 9.4JE-l l 2.40E-10 O.OOE+OO O.OOE+OO O.OOE+OO Tc-99 472,037,000 O.OOE+OO 3.44E-08 6.1 OE-08 0.00E+OO O.OOE+OO O.OOE+OO Th-228 472,037,000 1.08E-11 1.43E-IO 2.99E-10 5.IOE-06 6.22E-09 5.40E-05 Th-230 472,037,000 3.59E-l I l.81E-10 3.66E-10 l.70E-05 8.40E-04 3.59E-04 Th-232 472,037,000 O.OOE+OO l.OOE-10 2.67E-10 O.OOE+OO O.OOE+OO O.OOE+OO U-233/234 472,037,000 2.73E-10 2.SIE-10 3.43E-10 1.29E-04 2.07E-02 9.llE-04 U-235/236 472,037,000 1.90E-ll 1.42E-10 2.89E-10 8.96E-06 4.ISE+OO 6.33E-05 U-238 472,037,000 5.64E-l l l.58E-IO 2.82E-10 2.66E-05 7.95E+Ol 1.88E-04

Total: 1.58E-03 Sewer Pu-238 25,036,000 O.OOE+OO l.l lE-10 2.41E-10 O.OOE+OO O.OOE+OO O.OOE+OO Pu-239/240 25,036,000 O.OOE+OO 1.22E-10 2.92E-10 O.OOE+OO O.OOE+OO O.OOE+OO Tc-99 25,036,000 3.62E-09 3.74E-08 6.SSE-08 9.05E-05 5.36E-03 6.03E-06 Th-228 25,036,000 l.88E-l l 2.43E-IO 4.88E-10 4.71E-07 5.75E-10 9.41E-06 Th-230 25,036,000 l.58E-10 3.08E-IO 4.97E-10 3.97E-06 l.96E-04 l.58E-04 Th-232 2s,0J6,poo O.OOE+OO l.68E-IO 3.93E-10 O.OOE+OO O.OOE+OO O.OOE+OO U-232 25,036,000 3.03E-ll l.83E-IO 3.74E-10 7.59E-07 3.55E-08 5.0SE-05 U-233/234 25,036,000 l.8 !E-08 1.40E-09 2.9!E-10 4.54E-04 7.27E-02 6.04E-03 U-235/236 25,036,000 7.02E-10 3.03E-10 2.56E-10 l.76E-05 8.14E+OO 2.34E-04 U-238 25,036,000 2.57E-09 5.38E-IO 2.SSE-10 6.44E-05 l.92E+02 8.58E-04

Total: 7.36E-03 West Ditch Pu-238 169,304,000 O.OOE+OO l.12E-10 2.79E-10 O.OOE+OO O.OOE+OO O.OOE+OO Pu-239/240 169,304,000 O.OOE+OO l.22E-10 3.45E-10 O.OOE+OO O.OOE+OO O.OOE+OO Tc-99 169,304,000 5.83E-09 3.48E-08 6.06E-08 9.87E-04 5.84E-02 9.72E-05 Th-228 169,304,000 l.17E-ll l.76E-10 3.92E-10 l.98E-06 2.4!E-09 5.84E-05 Th-230 169,304,000 7.71E-ll 2.ISE-10 4.03E-10 l.30E-05 6.46E-04 7.71E-04 Th-232 169,304,000 O.OOE+OO 1.25E-IO 2.76E-10 O.OOE+OO 0.00E+OO O.OOE+OO U-233/234 169,304,000 l.SIE-08 l.40E-09 3.14E-10 2.56E-03 4.l lE-01 5.0SE-02 U-235/236 169,304,000 7.09E-10 3.SIE-10 2.SIE-10 l.20E-04 5.56E+O! 2.36E-03 U-238 169,304,000 l.53E-09 4.SIE-10 2.33E-10 2.59E-04 7.72E+02 5.09E-03

Total: 5.89E-02 WWTF Am-241 3,947,307 O.OOE+OO 9.48E-11 2.19E-10 O.OOE+OO O.OOE+OO O.OOE+OO Cs-137 3,947,307 O.OOE+OO l.24E-09 l.43E-09 O.OOE+OO O.OOE+OO O.OOE+OO Na-22 3,947,307 8.95E-11 8.13E-10 l.39E-09 3.53E-07 5.66E-11 l.49E-05 Np-237 3,947,307 2.61E-l l 2.74E-IO 5.62E-IO l.03E-07 1.46E-04 l.3 IE-03 Pb-212 3,947,307 1.20E-09 3.35E-09 3.02E-09 4.72E-06 3.41E-12 5.98E-04 Pu-238 3,947,307 l.33E-l l 5.35E-l l l.07E-10 5.27E-08 3.08E-09 6.67E-04

1 ECV: Effluent Concentration Value from 10-CFR-20, Appendix B.

Note: A value of "a~ was substituted for negative analytical results.

Printed: 08/04/2021 NFS-EDMS Page I of2

Page 4 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Liquid January 1, 2021 to June 30, 2021

Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of 1 Location (I) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV WWTF Pu-239/240 3,947,307 O.OOE+OO 6.32E-l 1 I.57E-IO O.OOE+OO O.OOE+OO O.OOE+OO Pu-241 3,947,307 4.56E-IO I.OIE-08 I. 74E-08 l.SOE-06 1.75E-08 4.56E-04 Ra-224 3,947,307 l.20E-08 6.69E-09 l.20E-08 4.73E-05 2.98E-IO 5.99E-02 Tc-99 3,947,307 4.75E-09 l.30E-07 2.24E-07 1.87E-05 I.I IE-03 7.91E-05 Th-228 3,947,307 O.OOE+OO I.SIE-10 3.74E-IO O.OOE+OO O.OOE+OO O.OOE+OO Th-230 3,947,307 l.16E-10 2.23E-IO 3.87E-10 4.60E-07 2.28E-05 l.16E-03 Th-231 3,947,307 O.OOE+OO 3.98E-08 3.89E-08 O.OOE+OO O.OOE+OO O.OOE+OO Th-232 3,947,307 3.63E-II l.33E-IO 2.37E-IO 1.43E-07 1.3 IE+OO l.21E-03 U-232 3,947,307 O.OOE+OO I.ISE-10 2.45E-IO O.OOE+OO O.OOE+OO O.OOE+OO U-233/234 3,947,307 l.34E-08 9.28E-IO 1.75E-IO 5.30E-05 8.50E-03 4.48E-02 U-235/236 3,947,307 5.96E-IO 2.06E-IO l.06E-IO 2.35E-06 l.09E+OO l.99E-03 U-238 3,947,307 9.75E-l l l.02E-10 l.34E-IO 3.85E-07 I.ISE+OO 3.25E-04

Total: 1.IJE-01

ECV: Effluent Concentration Value from 10-CFR-20, Appendix B.

Note: A value of "O" was substituted for negative analytical results.

Printed: 08/04/2021 NFS-EDMS Page 2 of2

Page 5 of 13 21G-21-0103 GOV-01-55 ACF-21-0182

Attachment 2 To Letter Dated August 16, 2021

Report of Radioactivity in Effluent Air for the Period January to June 2021

(3 Pages to Follow)

Page 6 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Air January 1, 2021 to June 30, 2021

Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of Location (mJ) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Main Stack 416 1070.66 m 3/min 17.84 m3tsec Th-228 282,139,411 6.58E-16 l.50E-16 8.16E-I 7 I.86E-07 2.27E-10 3.29£-02 Th-230 282,139,411 6.58E-16 l.50E-16 8. 16E-l 7 l.86E-07 9.19E-06 3.29E-02 Th-232 282,139,411 4.94E-16 1.13E-16 6.12E-17 l.39E-07 l.28E+00 l.23E-0l U-234 282,139,411 l.55E-13 3.54E-14 l.92E-l 4 4.38E-05 7.02E-03 3.I0E+00 U-235 282,139,411 5.92E-15 l.35E-15 7.35E-16 I.67E-06 7.74E-0l 9.87E-02 U-238 282,139,411 l.65E-15 3.76E-16 2.04E-16 4.64E-07 l.39E+00 2.74E-02

Total: 3.42E+00 Stack 185 Bldg. 131 112.74 m 3/min 1.88 m3tsec Pu-241 29,384,273 4.92E-16 9.20E-16 l.62E-15 l.45E-08 l.40E-10 6.!6E-04 Tc-99 29,384,273 l.59E-14 2.98E-14 5.23E-14 4.68E-07 2.77E-05 1.77£-05 U-234 29,384,273 2.42E-16 7.61E-15 l.93E-14 7.12E-09 l.14E-06 4.85E-03 U-235 29,384,273 7.50E-18 2.36E-16 5.98E-16 2.20E-I0 l.02E-04 l.25E-04

Total: 5.61E-03 Stack 234 Bldg. 234 328.49 m 3/min 5.47 m3tsec Am-241 85,678,107 5.83E-l 7 2.63E-17 4.34E-l 7 5.00E-09 I.46E-09 2.92E-03 Pu-238 85,678,107 7.13E-l 7 3.22E-l7 5.30E-17 6.I IE-09 3.57E-10 3.56E-03 Pu-239/240 85,678,107 2.53E-16 l.14E-16 l.88E-l6 2.16E-08 3.48E-07 l.26E-02 Pu-241 85,678,107 4.78E-15 4.34E-15 7.l3E-15 4.09E-07 3.98E-09 5.97E-03 Th-228 85,678,107 3.89E-l 7 l.75E-l 7 2.89E-17 3.33E-09 4.07E-12 l.94E-03 Th-230 85,678,107 4.86E-16 2.19E-16 3.62E-l6 4.16E-08 2.06E-06 2.43E-02 Th-232 85,678,107 6.15E-l6 2.78E-16 4.58E-16 5.27E-08 4.84E-0I 1.54E-0l U-234 85,678,107 l.33E-15 5.99E-l6 9.89E-l6 l.14E-07 1.82E-05 2.66E-02 U-238 85,678,107 3.89E-16 l.75E-16 2.89E-l6 3.33E-08 9.94E-02 6.48E-03

Total: 2.38E-0l Stack 327 Bldg. 330 1036.36 m 3/min 17.27 m3tsec Pu-241 270,157,102 2.50E-15 5.19E-l6 7.28E-16 6.75E-07 6.55E-09 3.12E-03 Tc-99 270,157,102 8.08E-14 l.68E-14 2.35E-l4 2.18E-05 l.29E-03 8.98E-05 U-234 270,157,102 1.40E-13 l.3 IE-14 8.78E-15 3.77£-05 6.05E-03 2.79E+00 U-235 270,157,102 4.32E-15 4.05E-16 2.71E-l6 l.l 7E-06 5.40E-01 7.20E-02

Total: 2.87E+00 Stack 421 Bldg. 100 32.96 m 3/min 0.55 m3tsec Pu-241 8,590,906 3.61E-l5 l.28E-15 l.95E-15 3. I0E-08 3.0IE-10 4.51E-03 Tc-99 8,590,906 1.17E-13 4.15E-14 6.30E-14 I.00E-06 5.93E-05 l.30E-04 U-234 8,590,906 1.26E-l4 1.29E-14 2.12E-14 1.08E-07 l.74E-05 2.52E-0l U-235 8,590,906 3.90E-16 3.98£-16 6.55E-16 3.35E-09 l.55E-03 6.50E-03

Total: 2.63E-0l Stack 424 Bldg. 100 32.62 m 3/min 0.54 m 3/sec Pu-241 8,502,340 1.29E-15 l.02E-15 1.57E-l 5 l.09E-08 l.06E-10 l.6 IE-03 Tc-99 8,502,340 4.16E-14 3.31E-14 5.0SE-14 3.54E-07 2.09E-05 4.62E-05

ECV: Effluent Concentralion Value from 10-CFR-20, Appendix B. Fraction o*f ECV at the stack is provided for rererence only. Concentrations at off-site significantly less than those reported here (at stack) due to the atmospheric dispersion that occurs before the effluent locations are exits the site.

Note: A value of "O~ was substituted for negative analytical results.

Printed: 08/04/2021 NFS-EDMS Page 1 of3

Page 7 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Air January 1, 2021 to June 30, 2021

Total Activity Error Quantity Quantity Fraction Volume Concentration Estimate LLD Released Released of Location (m3) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Stack 424 Bldg. 100 32.62 m 3/min 0.54 m3/sec U-234 8,502,340 8.14E-15 l.09E-14 1.88E-14 6.92E-08 l.llE-05 l.63E-01 U-235 8,502,340 2.52E-16 3.38E-16 5.SIE-16 2.14E-09 9.91E-04 4.20E-03

Total: l.69E-0l Stack 573 Bldg 306-W 120.88 m 3/min 2.01 m3/sec Pu-241 31,507,371 3.97E-16 8.ISE-16 l.49E-15 l.25E-08 l.21E-10 4.96E-04 Tc-99 31,507,371 1.28E-14 2.64E-14 4.SIE-14 4.04E-07 2.39E-05 l.43E-05 U-234 31,507,371 1.78E-16 6.65E-15 1.SOE-14 5.60E-09 8.98E-07 3.56E-03 U-235 31,507,371 5.SOE-18 2.06E-16 5.57E-16 l.73E-10 8.02E-05 9.16E-05

Total: 4.16E-03 Stack 600 Bldg. 110 319.61 m 3/min 5.33 m 3/sec Pu-241 83,303,746 1.23E-15 5.93E-16 9.73E-16 l.03E-07 9.99E-IO 1.54E-03 Tc-99 83,303,746 3.99E-14 l.92E-14 3.ISE-14 3.33E-06 l.97E-04 4.44E-05 U-234 83,303,746 2.46E-14 8.07E-15 1.22E-14 2.0SE-06 3.29E-04 4.92E-01 U-235 83,303,746 7.61E-16 2.SOE-16 3.78E-16 6.34E-08 2.94E-02 l.27E-02

Total: 5.06E-01 Stack 615 Bldg. 306-W 48.41 m 3/min 0.81 m 3/sec Pu-241 12,618,460 3.07E-16 8.62E-16 l.57E-15 3.88E-09 3.77E-ll 3.84E-04 Tc-99 12,618,460 9.94E-15 2.79E-14 5.0SE-14 1.25E-07 7.42E-06 l.lOE-05 U-234 12,618,460 3.02E-16 7.32E-15 1.88E-14 3.SIE-09 6.IOE-07 6.03E-03 U-235 12,618,460 9.33E-18 2.26E-16 5.SIE-16 l.lSE-10 5.45E-05 l.55E-04

Total: 6.58E-03 Stack 646 Bldg. 110 37.49 m 3/min 0.62 m 3/sec Pu-241 9,771,787 5.32E-16 9.0IE-16 l.57E-15 5.20E-09 5.0SE-ll 6.65E-04 Tc-99 9,771,787 l.72E-14 2.91E-14 5.07E-14 l.68E-07 9.94E-06 l.91E-05 U-234 9,771,787 9.59E-16 7.68E-15 l.88E-14 9.38E-09 l.SOE-06 l.92E-02 U-235 9,771,787 2.97E-17 2.38E-16 5.SOE-16 2.90E-10 l.34E-04 4.95E-04

Total: 2.04E-02 Stack 701 Bldg. 307 119.13 m 3/min 1.99 m 3/sec Pu-241 31,049,779 3.58E-!6 9.91E-16 I.SOE-IS l.llE-08 I.OSE-10 4.47E-04 Tc-99 31,049,779 l.16E-14 3.20E-14 5.84E-14 3.59E-07 2.13E-05 l.29E-05 U-234 31,049,779 2.60E-15 9.65E-15 2.16E-14 8.07E-08 l.29E-05 5.20E-02 U-235 31,049,779 8.04E-17 2.99E-16 6.67E-16 2.SOE-09 l.16E-03 l.34E-03

Total: 5.38E-02 Stack 702 Bldg. 307 158.63 m 3/min 2.64 m 3/sec Pu-241 41,345,582 3.63E-16 8.72E-16 l.57E-15 l.SOE-08 l.46E-IO 4.53E-04 Tc-99 41,345,582 I.I 7E-14 2.82E-14 5.0SE-14 4.85E-07 2.87E-05 1.30E-05 U-234 41,345,582 2.35E-15 8.30E-15 l.88E-14 9.7IE-08 l.56E-05 4.70E-02

ECV: Effluent Concentration Value from 10-CFR-20, Appendix B. Fraction of ECV at the stack Is provided for reference only. Concentrations at off-site locations are significantly less than those reported here (at stack) due to the atmospheric dispersion that occurs before the effluent exits the Site.

Note: A value of "O" was substituted for negative analytical results.

Printed: 08/04/2021 NFS-EDMS Page 2 of3

Page 8 of 13 21G-21-0103 GOV-01-55 ACF-21-0182 Radioactivity in Effluent Air January 1, 2021 to June 30, 2021

Total Activity Error Quantity Quantity Fraction Volume Coucentratiou Estimate LLD Released Released of Location (ml) (µCi/ml) (µCi/ml) (µCi/ml) (Ci) (g) ECV1 Stack 702 Bldg. 307 158.63 ml/min 2.64 m3tsec U-235 41,345,582 7.27E-l 7 2.57E-16 5.81E-!6 3.00E-09 l.39E-03 l.21E-03

Total: 4.87E-02 Stack 703 Exhaust Room Air 776.96 ml/min 12.95 m3tsec Pu-241 202,506,263 9.09E-15 2.57E-14 4.69E-14 l.84E-06 l.79E-08 l.14E-02 Th-228 202,506,263 l.76E-16 7.41E-16 1.72E-15 3.56E-08 4.35E-ll 8.S0E-03 Th-230 202,506,263 l.0!E-16 4.26E-16 9.SSE-16 2.05E-08 l.02E-06 5.06E-03 Th-232 202,506,263 1.44E-16 6.06E-16 1.40E-15 2.91E-08 2.67E-0l 3.60E-02 U-234 202,506,263 1.!0E-15 4.64E-15 1.07E-14 2.23E-07 3.58E-05 2.20E-02 U-235 202,506,263 l.14E-16 4.79E-!6 1.l lE-15 2.30E-08 l.07E-02 l.90E-03 U-238 202,506,263 l.39E-16 5.84E-16 l.35E-15 2.SIE-08 8.38E-02 2.3 !E-03

Total: 8.74E-02 Stack 773 Bldg. 440 166.92 ml/min 2.78 m3tsec Pu-241 43,576,819 2.!0E-14 3.53E-14 6. !SE-14 9. l 7E-07 8.90E-09 2.63E-02 Th-228 43,576,819 1.98E-16 1.31E-15 3.23E-15 8.61E-09 l.05E-ll 9.88E-03 Th-230 43,576,819 2.54E-!6 l.68E-!5 4.15E-15 1.llE-08 5.48E-07 l.27E-02 Th-232 43,576,819 1.69E-16 l.12E-15 2.76E-15 7.38E-09 6.77E-02 4.23E-02 U-234 43,576,819 5.22E-16 3.46E-15 8.52E-15 2.28E-08 3.65E-06 1.04E-02 U-235 43,576,819 9.18E-17 6.07E-!6 1.50E-15 4.00E-09 l.85E-03 l.53E-03 U-238 43,576,819 !.84E-16 l.21E-15 2.99E-15 8.00E-09 2.39E-02 3.06E-03

Total: l.06E-0l Stack 774 Bldg. 301 319.16 ml/min 5.32 m3tsec Th-228 83,185,658 5.43E-18 1.71E-!6 4.29E-16 4.52E-10 5.5!E-13 2.71E-04 Th-230 83,185,658 1.85E-l 7 5.SIE-16 1.46E-15 l.54E-09 7.62E-08 9.25E-04 Th-232 83,185,658 l.l0E-17 3.45E-16 8.67E-16 9.12E-10 8.37E-03 2.74E-03 U-234 83,185,658 4.94E-l 7 l.55E-15 3.91E-15 4. llE-09 6.59E-07 9.SSE-04 U-235 83,185,658 3.21E-18 1.0IE-16 2.54E-!6 2.67E-10 l.24E-04 5.35E-05 U-238 83,185,658 2.33E-l 7 7.31E-!6 1.84E-15 l.94E-09 5.78E-03 3.SSE-04

Total: 5.37E-03 Stack 796 Bldg. 100 19.37 ml/min 0.32 m3tsec Pu-241 5,048,265 8.86E-16 9.59E-!6 l.57E-15 4.47E-09 4.34E-11 l.l lE-03 Tc-99 5,048,265 2.87E-14 3.I0E-14 5.0SE-14 1.45E-07 8.56E-06 3.ISE-05 U-234 5,048,265 0.00E+00 7.14E-15 l.88E-14 0.00E+00 0.00E+00 0.00E+00 U-235 5,048,265 0.00E+00 2.21E-16 5.SIE-16 0.00E+00 0.00E+00 0.00E+00

Total: l.14E-03

ECV: Effluent concentration Value from 10-CFR-20, Appendix B. Fraction of ECV at the stack is provided for reference only. Concentrations at off-site locations are significantly less than those reported here (al stack) due to the atmospheric dispersion that occurs before the effluent exits the site.

Note: A value of "O" was substituted for negative analytical results.

Printed: 08/04/2021 NFS-EDMS Page 3 of3

Page 9 of 13 21G-21-0103 GOV-01-55 ACF-21-0182

Attachment 3 To Letter Dated August 16, 2021

Report of Gaseous Effluent Dose and Activity Concentrations for the Maximally Exposed Off-Site Individual for the Release Period January to June 2021

(3 Pages to Follow)

Page 10 of 13 21G-21-0103 GOV-01-55 ACF-21-0182

Report of Potential Gaseous Effluent Dose to the Maximally Exposed Offsite Individual and on the Maximum Radionuclide Concentrations for the Period:

January to June 2021

Introduction During this biannual period, NRC License SNM-124, Section 9.1.1.3, required NFS to assess the total effective dose equivalent (TEDE) to the maximally exposed offsite receptor and the maximum radioactive air concentrations at the site boundary attributable to NFS' air effluents. The required biannual assessment has been completed and the details of the assessment are provided in the subsequent sections.

Summary of Methods In accordance with SNM-124, Section 9.1.1.4, and internal procedure NFS-HS-A-27, the U.S. Department of Energy's CAP88-PC computer program was used to estimate off-site doses and activity concentrations for gaseous effluents. NFS operated sixteen (16) radiological stacks during the first half of 2021. Based on effluent types and stack physical characteristics, releases from these stacks were grouped into effective stacks for modeling purposes. To accommodate the co-location limitation of the model, the effective stacks were taken to be at the approximate center of the plant site. The distance to the site boundary (nearest model receptor distance) was conservatively taken to be 150 meters for all sectors.

Meteorological data was based on the average wind speed and direction frequencies from the onsite meteorological tower covering the time period for this report.

Atmospheric stability class D (neutral atmosphere) was used for all releases (default value recommended by the U.S. Environmental Protection Agency in "User's Guide for COMPLY"). The most conservative inhalation class was assumed for each radionuclide released. A particle size (activity median aerodynamic diameter or AMAD) of 1.0 micron was assumed for modeling purposes since no information on actual particle sizes exists.

Because CAP88-PC models releases over an entire year, the six-month source term (i.e., total curies of each radionuclide released over the period, given in Attachment 2) was annualized (i.e., transformed into a 12-month release) so that airborne activity concentrations would not be under-estimated during the release period.

Summary of Results Doses are reported in Table 1 below and are derived from the CAP88-PC "Synopsis Report." These doses are at the location of the maximally exposed (off-site) individual (MEI). The results include an adjustment (using the normalization factor mentioned above) to convert the "annualized" doses back to those doses that were actually received in the six-month release period. Activity concentrations reported in Table 2 come directly from the CAP88-PC "Concentration Tables" report; no adjustments are needed for these concentrations. The CAP88-PC output reports are available for review at NFS.

Page 11 of 13 21G-21-0103 GOV-01-55 ACF-21-0182

Table 1 summarizes the six-month dose to a hypothetical individual at the MEI location, which was determined to be approximately 550 meters North-Northeast from the center of the plant site. The TEDE to the MEI was estimated to be 3.2E-03 mrem for gaseous effluents released during the first half of 2021. The highest organ committed dose equivalent (COE) to the MEI was estimated to be 1.7E-02 mrem to the lungs. These MEI doses are well below the Environmental Radiological Monitoring Program action levels and applicable regulatory limits/ALARA constraints.

Table 1. Organ Doses and Total Effective Dose Equivalent at the MEI Location

Organ Committed Dose Equivalent (mrem per first half of 2021)

Adrenals 2.2E-04 Urinary Bladder Wall 2.6E-04 Bone Surface 9.2E-03 Brain 2.2E-04 Breasts 2.3E-04 Stomach Wall 3.7E-03 Small Intestine 2.5E-04 Upper Large Intestine Wall 1.1 E-03 Lower Large Intestine Wall 2.SE-03 Kidneys 2.SE-03 Liver 8.0E-04 Muscle 2.3E-04 Ovaries 2.4E-04 Pancreas 2.2E-04 Red Bone Marrow 1.2E-03 Skin 4.5E-04 Spleen 2.2E-04 Testes 2.5E-04 Thymus 2.2E-04 Thyroid 1.9E-03 Gall Bladder Wall 2.2E-04 Heart Wall 2.2E-04 Uterus 2.2E-04 Extra-thoracic 1.5E-02 Lungs 1.7E-02

Total Effective Dose Equivalent 3.2E-03 mrem Location of MEI: 550 meters North-Northeast

Page 12 of 13 21G-21-0103 GOV-01-55 ACF-21-0182

Table 2 summarizes the maximum radioactive air concentrations at or beyond the site boundary, as determined by CAP88-PC, for the radionuclides released. The total sum of fractions was estimated to be 5.SE-04 and indicates that exposures to the offsite public from gaseous effluents were much less than 1 % of the 10 CFR 20, Appendix B, Table 2, Col. 1 values for all offsite receptors including the site boundary. It is noted that the location of the maximum airborne concentration for a given radionuclide does not necessarily correspond to the MEI location. This is due primarily to the fact that the maximum concentrations for individual nuclides can vary due to differences in values input into the dispersion model for each of the effective stacks - such inputs include stack height, stack diameter, flow rate, and total radionuclide activities released per stack. Another reason for the disparity is the fact that the MEI dose includes both inhalation and ingestion pathways.

Table 2. Maximum Predicted Airborne Concentrations at or Beyond the Site Boundary

~

Maximum Predicted Airbome Concentrations at

'. or Beyond the Site: Boundary '. ' '

l\\1aximum Concenµ-~tion 10 CFR 20, App. B, Ratio of Maximum

,* Nuclide Concentration Location Table 2, Col. 1 Value Concentration to.

(l,ICi/mL) Sector Dist(m). (IJCi/mL) 10 CFR20 Value

99Tc l.5E-17 NNE 450 9.E-10 l.6E-08 22sTh 5.5E-20 NNE 650 2.E-14 2.8E-06 230Th 8.lE-20 NNE 400 2.E-14 4.0E-06 -*

232Th 9.3E-20 NNE 300 4.E-15 2.3E-05 234u 2.6E-17 NNE 550 5.E-14. 5.3E-04 23s 0 8.7E-19 NNE 550 6.E-14 l.5E-05

23su l.2E-19 NNE 650 6.E-14 2.0E-06

23sPu 9.0E-21 NNE 250 2.E-14 4.5E-07 239Pu 3.2E-20 NNE 250 2.E-14 l.6E-06

241Pu 2.5E-18 NNE 400 8.E-13 3.2E-06 241Am 7.4E-21 NNE 250 2.E-14 3.7E-07

Sum of Fractions: 5.8Fr04

Page 13 of 13