ML20151V858

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Radiological Environ Monitoring Program for 1987
ML20151V858
Person / Time
Site: Shoreham File:Long Island Lighting Company icon.png
Issue date: 12/31/1987
From:
LONG ISLAND LIGHTING CO.
To:
Shared Package
ML20151V855 List:
References
NUDOCS 8805030217
Download: ML20151V858 (133)


Text

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SHOREHAM NUCLEAR POWER STATION l RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM l I

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i JANUARY 1 TO DECEMBER 31, 1987 j l

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SHOREHAM NUCLEAR POWER STATION -

OPERATIONAL RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM 9

l 1987 ANNUAL REPORT JANUARY 1 to DECEMBER 31, 1987  ;

i Prepared by [

E LONG ISLAND LIGHTING COMPANY I I

and TELEDYNE ISOTOPES i I e

i April 15, 1988 l l

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TABLE OF CONTENTS l PAGE i EXECUTIVE

SUMMARY

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! THE PR0 GRAM......................................................... 3 A. Objectives...................................................... 4 B. S am p l e Co l l e c t i o n . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5

1. Aq u a t i c E n v i r o nme n t . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5
2. Atmospheric Environment..................................... 5
3. Terrestrial Environment..................................... 6
4. Direct Radiation............................................ 6 C. Quality Assurance............................................... 6
1. T e l e d yn e i s o t o p e s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 6
2. L o n g I s l a nd L i g h t i n g Co mp a ny . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 7 D. Data Interpretation............................................. 8
1. General..................................................... 8
2. Gamma Isotopic.............................................. 9 E. Dose Assessment................................................ 10 F. P r o g r am S umm a ry . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1 II. R E S U L T S AN D D I S C U S S I O N . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 14 A. Aquatic Environment............................................ 15
1. Su r f a c e W a t e r . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 15
2. Fish....................................................... 15
3. Invertebrates................c............................. 16
4. Aquatic P1 ants............................................. 16
5. Sediment................................................... 16 B. Atmo s ph e r i c E n v i r o nme n t . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 17
1. Ai rborne P a rt icul at e s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 17
2. Airborne lodine............................................,17
3. Noble Gas.................................................. 17

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TABLE OF CONTENTS PAGE C. Terrestrial Environment........................................ 21

1. Milk....................................................... 21

. . 2. Potable Water.............................................. 21

3. Game....................................................... 21
4. Fo od P r o d uc t s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 2
5. Precipitation............................................... 22 D. Direct Radiation............................................... 22 E. Do s e As s e s sme nt . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 4 111. CONCLUS10NS.............. ......................................... 26 IV. REFERENCES......................................................... 28 APPENDIX A - Radiological Environment al Monitoring. . . . . . . . . . . . . . . . . 31 Program Summary - 1987 APPENDIX B - Sample Designation and Sampling Locations. .. ... . . . . .. . 41 AP?ENDIX C - Data Tab 1es........................................... 50 APPENDIX 0 - An alyt ic al Procedures Synopsi s. . . . . . . . . . . . . . . . . . . . . . . . 91 APPENDIX E - Sunmary of EPA Interlaboratory Comparisons. .. . .. . .. . .104
- APPENDIX F - REMP Sampling and An alytical Exceptions. . . . . . . . . . . . . .110 APPENDIX G - SNPS Land Use Surveys...........,.................... 119 APPENDIX H - Species Collect ed in the Radiological . .. . . . . . . . . . . . . .125 Environmental Monitoring Program ii

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D LIST OF TABLES NO. TITLE PAGE

1. Synopsis of the Shoreham Nuclear Power St ation's. . . . . . . . . . . . . . . . . . . . 12 -

Dperational Radioltagical Environmental Monitoring Program for the period January 1 through December 31, 1987

2. Summary of Dose Determination for 1987.............................. 25 Appendix B - Sample Designation and Sampling Locations B-1 S am p l e L o c a t i o n s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 3 Stations Required by SNPS Technical Specifications B-2 Airborne Particulate and Airborne lodine Monitoring Stations........ 45 '

B-3 Waterborne Mo ni tori ng St at i on s. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 5 B-4 Ingestion Moni tori ng St ations. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 45 B-5 Direct Radi ation Monitoring St at ions. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 46 Appendix C - Data Tables Aquatic Environment C-1 Concentrations of Tritium. Strontium-89 and Strontium-90 . .. . . . . .. . . 51 and Gamma Emitters in Surf ace Water Samples C-2 Concentrations of Strontium-89 and Strontium-90 and Gamma. . . . . .. . . . . 52 Emitters in Fish Samples C-3 Concentrations of Strontium-89 and Strontium-90 and Gamma. .. . . . .. .. . 53 1 Emitters in Invertebrate Samples C-4 Concentrations of Strontium-89 and Strontium-90 and Gamma. . . . . .. .. . . 54

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Emitters in Aquatic Plant Samples C-5 Concentrations of Strontium-89 and Strontium-90 and Gamina. .. .. . . . . . . 55 Emitters in Sediment Samples Atmospheric Environment C-6 Concentrations of Gross Beta Emitters in Weekly Airborne. .. . . . . . . . . . 56 Particulate Samples i C-7 Concentrations of Gamma Emitters in Quarterly Composite.. . . . . . . . . . . . 62 of Airborne Particulate Samples

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i LIST OF TABLES (Cont.)

NO. TITLE PAGE AtmospheHcTnvironment (Cont.)

C-8 Concentrations of Strontium-89 and Strontium-90 in Quarterly. . . . . . . . 66 Composites of Airborne Particulate Samples C-9 Concentrations of lodine-131 in Air Cartridge Samples. . . . . . . . . . . . .. . 67 Terrestrial Environment C-10 Concentrations of Tritium, Gross Beta and Gamma Emitters............ 73 in Precipitation C-11 Concentrations of lodine-131 i n Milk SEnples. . . . . . . . . . . . . . . . . . . . . . . . 74 C-12 Concentrations of Strontium-89 and Strontium-90 and Gamma . . . . ... .. . 75 Emitters in Milk Samples C-13 Concentrations of Tritium, lodine-131 and Gamma Emitters in.. . .. . . . . 78 Potaole Water Sampi;s C-14 Concentrations of Gamma Emitters in Game Samples. . . . . . . . . . . . . . . . . . . . 79 C-15 Concentrations of Gamma Emitters and 1-131 in Food Product Samples.. 80 DIRECT RADIATION C-16 Direct Radi ation Measurements - Quarterly TLD Result s. . . . . . . . .. . . . . . 83 C-17 Direct Radi ation Measurements - Monthly TLD Re sult s. . . . . . . . . . . . . . . . . 85 NOBLE GAS C-18 Concentrations of Krypton-85 and Xenon-133.......................... 87 in Air Samples LOWER _ LIMIT OF DE*ECTION (LLD)

C-19 Typical LLDs Achieved for Gamma Spectrometry. . . . . . . . . . . . . . . . . . . . . . . 88 C-20 LLDs and Reporting Action Levels Required by Technical ... . . . . . .. . . . . 89 Specifications and 1987 Contract 10 -

LIST OF FIGURES NO. PAGE

1. Average Weekly Gross Beta Results in Airborne Particulates. . .. . . . . ..18 (January 1 through December 31,1987)'
2. Comparison of Aversge Monthly Gross Beta Resu'its in Airborne........19 Particulates (February 1977 - December 1987)
3. Comparison of Average TLD Results (February 1977 - December 1987)... 23 APPENDIX B - SAMPLE DESIGNATION AND SAMPLING LOCATIONS -

LIST OF MAPS B-1 Sh o r eh am S i t e L o c a t i o n . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 7 B-2 On Si t e Sampl i ng L oc at i on s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 8 B-3 Of f Si te Sampl i ng Loc at io ns . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 9 e

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e EXECUTIVE

SUMMARY

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1 EXECUTIVE

SUMMARY

l l This report samarizes the Shoreham Nuclear Power Station's (SNPS)

Radiological Environmental Monitoring Program (REMP) for 1987. SNPS received i a 5% power license in 1985. During 1987 the plant was shutdown except for a j period between May 26 and June 8, when testing below 5% power resmed.

The objective of the operational REMP is to identify and measure

' plant related radioactivity in the environment and calculate the potential dose to the surrounding pupulation. The operational phase uses the preopera-l

tional baseline data to identify plant contributed radiation and evaluates the possible effects of radioactive plant effluents on the environment.  !

The SNPS REMP is designed to comply with the Plant's Technical Specifications i and NRC Regulatory Guides.  !

i- The REMP data is acquired by sampling various media in the environment  !

which are then analyzed for any radiation present. Media sampled within the i aquatic environment included surf ace water, algae, fish, invertebrates '

(clams, lobsters, etc.) and sediment. The atmospheric environment was i sampled for airborne particulates, airborne iodine and noble gases. Milk, '

l potable water, precipitation, game and food p%1ucts were obtained from the i

terrestrial environment. Direct radiation W measured using thermo-lainescent dosimeters (TLDs).

Radioactivity in environmental media varies from sample to suple as well as geographically; therefore, a number of sampling locations for each -

media were selected using available meteorological, land and water use  !

. data. Sampling locations are designated as either indicator or control locations. The indicator locations are placed close enough to Shoreham so {

', that plant contributed radioactivity will be at its highest concentration. e

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The control sample locations are placed so that they will be beyond measurable  ;

influence of Shoreham and any other nuclear facility. An exception to this i

. occurred at the on shore site for REMP location 13G2, at the entrance to i j Port Jefferson Harbor. During preoperational testing aquatic samples revealed the presence of low levels of iodine-131. An investigation revealed i t

that the iodine-131 was from area hospitals treating patients for thyroid L c arcinoma. Thereaf ter a second onshore aquatic background location was i sampled at the entrance to Mt. Sinai Harbor. T l A number of radioanalyses were performed on each medium s upled. All samples did not undergo all types of radioanalyses; only those analyses i appropriate for the particuler medi a were performed. The analyses included '

l gamma spectrometry, strontium-89 and -90, iodine-131, tritium, gross beta l radiation, direct radiation and noble gases. '

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l Dose calculations for the SNPS environs were perfonned using positive concentrations of radioactivity detected in the samples collected. In all cases the calculated doses were similar to the background doses calculated for the previous years. -

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I. PROGRAM 9

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THE PROGRAM The Shoreham Nuclear Power Station's (SNPS) Radiological Environmental  ;

Monitoring Program (REMP) is conducted in compliance with NRC regulations, licensing comitments, Program technical / legal requirements and the Plant's Technical Specifications. The REMP was developed in general accordance with the NRC Radiological Assessment Branch Technical Position (BTP) Rev.

1, Nov. 1979. LILCO's Updated Safety Analysis Repoit (USAR) 11.6, Environmental Report (ER) 6.1.5 and Technical Specification Section 3/4.12.

All samples were collected by personnel of the Long Island Lighting Company (Environmental Engineering Department) or EA Engineering, Science and Technology Inc. A synopsis of the sampling program can be found in Table 1.

A map and description of sampling locations appear in Appendix B. More detailed information concerning sample locations and collection is available in niMP Procedure 1.0 Radiological Environmental Monitoring Prograt '.REMP)

Program Oescription.

During 1987 sample analyses were performed by Teledyne isotopes (TI) of Westwood, New Jersey (referred to througho'Jt the text as "the laboratory"),

under contract to LILCO. A sunmary of analytical results appears in Appendix A and individual analysis results in Appendix C.

A. Objectives The objectives of the operational radiological environmental monitoring program are:

1. Identify and measure plant related radioactivity in the environment for the calculation of the potential dose to the population.
2. Identify excessive radionuclide concentration of limited duration so that appropriate action may be taken.
3. Determine the long term variation in radionuclide concentrations.

4 Determine the effects of plant effluent on the envirorynent.

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5. Comply with regulatory requirements and specifications and provide j records to document compliance.

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6. Sample Collection
1. Aquatic Environment The aquatic environment at the SNPS site was examined by analyzing samples of surface water, fish, invertebrates, aquatic plants and sediment. Surface water samples were taken at six loca-tions in May and October using a Niskin bottle or by wading into the -

water and filling a new two gallon polyethylene bottle. The samples were placed in new polyethylene bottles following three rinses with the suple medium prior to collection. Samples of Winter Flounder, Pseudopleuronectes americanus, Windowpane, Scophthalmus aquosus, Sea Robin, Prionotus spp, Little Skate, Raja erinacea, and Summer Flounder (Fluke), Paralichthys dentatus were taken by trawl, sealed in plastic bags, frozen, and shipped to the laboratory for analysis, r Invertebrate samples of Merican Lobster, Homarus americanus, Squid, Loligo pealeil and Channeled Whelk, Busycon canaliculata were collectec by trawl. Channeled Whelk were also collected using pots.

These invertebrate samples were sealed in plastic bags, frozen and shipped to the laborato g for analysis. Blue Mussels, Mytilus edulis were collected by hand along jetties. Soft-shell clams, Mya arenaria, and Oysters, Crassostrea virginica, from Wading River were shelled and sealed in plastic bags, frozen ano shipped to the laboratory.

Aquatic plants, Fucus sp., Ulva lactuca, Enteromorpha sp., and Codium sp., among others were collected while trawling for the fish samples and from along the shoreline, then sealed in plastic bags, refrigerated and snipped. Deep water sediment was collected using a Smith-MacIntyre bottom sampler, sealed in plastic bags, frozen and shipped. Beach sediment samples were also collected, sealed in plastic bags, frozen and shipped to the laboratory.

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2. Atmospheric Environment

! The atmospheric environment was examined by analyzing airborne 1

particulates collected on Gelman Type A/E filters using low volume air samplers (approximately 1 cfm). Airborne iodine was collected by absorption on triethylenediamine (TEDA) impregnated charcoal car-tridges which were connected in series behind the airborne partic-ulate filters. The samplers used were equipped with a vacuum recorder for sample volume correction and to ensure sample validity and indicate maintenance problems when they occurred. Should the sampler lose vacuin due to a leak tne vacuum level reading will drop I to zero. Since this may occur without a corresponding loss of electric supply the exact time of the maintenance problem will be evident on the recorder chart.

Sample volumes were measured using dry gas meters and corrected for differences between the actual pressure seen by the volume meter and the average atmospheric pressure. Sample volumes are l corrected to standard pressure using average weekly barometric 1

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A pressure (measured at Environmental Engineering Department, Melville) and air sampler vacuum readings. Time totalizers indicate the duration of time the s uple was taken.

Air samples were collected weekly at St. Joseph's Villa and analyzed for the Noble Gases Krypton-85 and Xenon-133. The samples were collected using a modified low pressure air compressor. Outside air is drawn into an interim holding tank evacuated to 20" Hg and then transferred to a nmple tank for transport to the laboratory for analysis.

3. Terrestrial Environment The terrestrial environment was examined by analyzing samples f of milk, precipitation, potable water, game, food products, and soil.

When available, milk samples were collected from four locations monthly, except during the pasture season (May through October) when the sampling was increased to twice a month. Milk samples were shipped on ice with Sodium Bisulfite (NaHS03) preservative added.

Precipitation was collected at two locations weekly. In order to ensure sufficient sample volume weekly precipitation samples were combined for a monthly sample composite. Potable water was collected quarterly from'three well locations. Game samples (Squirrel, Sciurus carolinensis and Raccoon, Procyon lotor) were obtaintd semi-annually from on site locations, sealed in plastic bags, frozen and then shipped. Food products consisting of vegetables and fruit were collected from area f arm stands and shipped fresh to the laboratory.

4 Direct Radiation Direct radiation levels in the environs were measured with energy compensated Calcitn Sulfate (CaSO4:Dy) TLDs, each contain-ing four separate readout areas. The TLDs are annealed by LILC0 prior to placement in the field. Two TLDs were placed at 36 locations and exchanged on a monthly and quarterly cycle, respectively. The units were then packaged and shipped to the laboratory for analysis.

C. Quality Assurance

1. Teledyne isotopats l i I

Teledyne isotopes (TI) has an extensive quality assurance progra designed to ensure the precision and accuracy of the data generated. An Interlaboratory Comparison Progra is conducted with

( the Environmental Protection Agency (EPA). The results of the Progra analyses are listed in Appendix E. Participation in this l

program permits estimation of bias in Tl results from the deviation [

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e from the "known" value given, or by comparison with means of all participants. The Tl Quality Assurance Program for Radiological i Monitoring is described in various TI publications (references 15, '

16,17).

Approximately 10 percent of TI's total analytical effort is spent on quality control including process quality control, instrument quality control, intra and interlaboratory cross-check, and compre-hensive data review. In addition, LILC0 specifically requires that ten percent of its analyses be duplicated for further quality control cross check.

2. Long Island Lighting Company
a. Nuclear Review Board (NRB) Audit The annual REMP NRB audit was conducted on May 4 8, 1987 As with last year's audit the 1987 NRB audit focused on internal LILC0 ,

REMP activities in the Environmental and Nuclear Engineering, Nuclear ,

Operations Support and Shoreham Operations Departments. The Program areas audited were: procedures, records control, sample collection and documentation, training records, analysis results, land use surveys and interlaboratory comparison progrvns.

Audit report NK 87-01 was issued on June 10 listing one (1) finding and five (5) observations. No SNP5 Technical Specifications Violations were cited. Corrective action on the one finr'ing was completed by April 1, 1988.

b. LILCO Quality Assurance Audits  ;
1. Field Audit  !

/ The REMP sampling effort has been audited by LILCO's QA Department since the beginning of the Program. The 1987 surveillances were conducted on March 12 (Milk), May 27 (Fish and Invertebrates) and July 14 (Noble Gas and Precipitation).

No findings were noted during these surveillances.

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2. Environmtental Radiological Laboratory Audit As with the REMP field sampling the environmental radiological laboratory performing REMP radioanaly,ses has been audited annually since the start of monitoring. Tne laboratory utilized during 1987 was Teledyne Isotopes.

This years' surveillance was performed on December 10, 1987, at Teledyne's laboratory in Westwood, New Jersey. This surveillance sought to verify corrective actions taken in response to the 1986 audit. All findings from the 1986 audit have been addressed by Teledyne and are closed.

D. Data Interpretation

1. General The analytical data generated during the program are routinely evaluated by the TI project leader who is the liason with Long Island Lighting Company's Environmental and Nuclear Engineering Departments.

Several factors are important in the interpretation of the data.

These f actors are discussed here to avoid repetition in sections that follow.

Within the data tables (Appendix C) an approximate 95 percent (12 sigma) confidence interval is supplied for those data points above the lower limit of detection (LLD). These intervals represent the range of values into which 95 percent of repeated analyses of the same sample would f all. Tables C-19 and C-20 present typical and required LLD's, respectively.

Results for each type of sample were grouped according to the analysis performed. Means and standard deviations of these results

. arte calculated when applicable. The calculated standard deviations of grouped data represent sample rather than analytical variability.

For these calculations any values below LLO are considered to be at the LLD. As a result, the means are biased high and the standard deviations are biased low. When a group of data is composed of mainly LLD values (>50%), averages are not calculated.

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e Grab sampling is a useful and acceptable procedure for taking environmental samples of a mediun in which the concentration of radionuclides is expected to vary minimally with time or where inter-mittent sampling is deemed sufficient to establish the radiological characteristics of the medium. This method, however, is only repre-sentative of the supled medium for that specific location and instant of time. As a result, variation of radionuclide concentra-tions in the s uples will normally occur. Since these variations will tend to counterbalance one another, the extraction of averages based upori repetitive grab samples is valid.

2. Gamma Isotopic Analyses SNPS Technical Specifications Table 3.12.1-1 requires that ana'yses be performed on all media for gamma emitting radionuclides which may be attributable to effluents from the plant. These analyses are in addition to requirements for specific game emitters such as I-131, Cs-134, Cs-137 Ba-140, Mn-54, Fe-59 Co-58, Co-60, Zn-65, Zr-95 and Nb-95. Industry experience suggests that these are the most likely radionuclides to find their way into the environment from a BWR nuclear power plant. Gamma spectroscopy is expected to identify most other nuclides which may be discharged when the LLD's for specified gama emitters are met by this technique.

Tables 3.1 and 3.2 of the Shoreham Final Environmental Statement list tne calculated liquid and gaseous effluents by radionuclide in curies per year. These release rates assume normal operation of the plant, including anticipated operational occurrences. Those nuclides listed in Tables 3.1 and 3.2 which are not routinely observable by

  • gbnma spectroscopy and which are not specifically analyzed in other ways fall into two categories:
1. Those radionuclides with half-lives on the order of hours or minutes which cannot accumulate appreciably in the environment (Na-24 Cu-64, Zn-69m 2n-69, Sr-91, Y-91m. Y-92, Y-93, Tc-99m, Rh-10 h , Rh-105, Rh-106, Te-129. Te-131m. Te-131, 1-132, 1-135 Ba-137m Pr-143, Ce-143, Pr-144 and W-187).
2. Those radionuclides with no gamas (P-32, Fe-55), those with a trivial percentage of their transitions going by gamma emission (Y-91), or those with their primary gama occurring at such a low energy and at such low abundance that it is not routinely observable in the presence of other gama activity (Nd-147). With only 10 pCi of hd-147 calculated to be released per year in Shoreham's liquid effluents, the nuclide cannot be an important contributor to dose.

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E. Dose Assessment .

In order to assess the total dose an individual may receive from the Shorehm environment, appropriate environmental suples, located along critical effluent pathways, are analyzed for the presence and total activity of specific radionuclides. The exposure an individual receives may then be approximated by quantitative analysis of these radionuclide concentrations in air, water, milk and food samples as well as due to direct radiation exposure. It is also possible to estimate the dose rate to a particular internal body organ when the average concentrations in a particular environmental medium are known, Radionuclides may enter the body through ingestion of water and milk, inhalation of and imersion in air, submersion in water, or consmption of food. Thas, in order for the REMP to provide an estimate of the total radiation dose, a radionuclide intake is deterTnined for each pathway.

The methodology for determining doses is similar for all path-ways. Laboratory analyses from the REMP for each sample type are compiled. Data from all locations taken on the same date are averaged to obtain the most reliable approximation of the radioactivity concen-tration on that date for that sample type. The averages of all dates are then taken to provide the best approximation of radioactivity concentrations for the year.

When an average value has been obtained which represents a sample medium or an exposure pathway, it can then be used to calculate the i dose for the year. Additional information, such as the quantity of fish, milk, water, meat, vegetables, etc., consumed per year by the maximum individual is also needed to calculate the total dose (13).

'The dose due to direct radiation exposure is monitored by TL0s.

Tne laboratory results for TLD's are expressed in dose units directly and do not require any additional calculations.

The dose to the total body or to a specific organ is then calcu-lated by the product of the radionuclide specific dose conversion f actor for its applicable exposure pathway, the environmental sample

! radionuclide concentration, and the ingestion or inhalation rate of the sample or medium of interest. For example, the following general equation expresses this principle:

Dose = Concentration x Quantity ingested x Dose factor (mrem /yr) per sample per year i

l The sample concentration is typicaly expressed in pCi/l or pCi/kg.

For the ingestion pathway, the quantity ingested or constJned per year is expressed in kg/ year or 1/ year. Finally, the dose conversion factor is expressed in terms of mrem /pCi ingested or innaled.

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F. Program Summary Table 1 sunmarizes information on the REMP as performed i during the period of this report, January 1 through December 31, ',

1987. During this reporting period 3205 analyses were performed on 2479 environmental samples. Appendix A sunmarizes the analytical results obtained from the SNPS REMP. The format used is that recommended in NRC Radiological Assessment Branch Technical Position BTP, Rev. 1 Nov 1979. Appendix B describes the sample coding system, which specifies sample type and relative locations at a glance, in addition, pertinent information on individual sanpling loc.1tions, and maps which show their pographic location, are included. Appendix C presents the analytical results of the Shoreham Nuclear Power Station's Radiological Environmental Monitoring Program for the period January 1 through December 31, 1987. Appendix 0 contains a synopsis of the analytical procedures used in the REMP. Results of the EPA inter-laboratory comparison program can be found in Appendix E. Appendix F lists the program exceptions for 1987, and Appendix G reports the land use surveys performed by LILCO's Environmental Engineering Department during 1987 in the vicinity of the SNPS. Common and scientific nanes of species collected in the program are presented in Appendix H. ,

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lABLE 1 .

Sym0P515 of i;4E SMORtHAM NUCLE AR Powta ST ATI0e*5 OPERAil0eAL R ADIOLOGICAL EnvlR0entmTAL MONI T OR I NG PROGR AM F OR int Pitl00 JANUARY I THROUGH OECEM8ER 31. 1987 ANALYSIS RUMett SAMPLING NURSER PERFORiett SAMPLE COLLECTED ANALY515 F RE QU( NCY FAtQUENCY L3 CATIONS TTPt Aquatic Environment H-3 Scolannual 12 Seelensual 6 12 12 Surface Water Gamma Seelannual Seelannual 12 Sr-89 12 Sr-90 Seelannual Seelannual 26 26 Gamma Fish Scalannual 3 Sr-89 SeeIanneal 26 Sr-90 SeeIannoal 26

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Gamma Seelannual 23 ro Sealannual 6 23 23 Instriebrates Sr-89 Seelannual Sr-90 Seelannual 23 Gamma Seelannual 12 Seelannual 3 12 12 AgustIc Plants $r-89 Seelenaual 5eelannual 12 5r-90 1

Gamma Seelannual 12 l

Seelannual 5 12 I2

! Sedleent -- Seach Sr-89 SeeI amarua1 12 3r-90 Seeltanual l Sealannual a 5 8 Gamma 5edlocat -- Offshore Sealannual Sr-89 Sealannual 8 Sealannual 8 Sr-90 Atmospheric E n.f ronment Gross seta Weekly 196 Weekly 16 196 62 Airborne Particulates Gamma Guarterly Composite

$r-89 Quarterly Ceepestte 62 Sr-90 Quarterly Ceeposite 62 l-131 Weekly 196 Weekly 16 796 Airborne lodine tr-P5 Weekly 52 Weekly I 52 52 Noble Gas Re-133 weekly e

TABLE I (COct.)

STm0P515 0F THE SHOSENAM WUCLE AR P0utR ST ATI0e'$ OPfCAfl0eAL RADIOLOGICAL ENVIRONMENTAL MOWITORING PROGRAM FOR TWE PERIOD JANUART I THROUGH OECEMGER 31. 1987 AaALT515 mWNSER SanPLING suMcER 2

5 AMPLE ANALYSIS FREQUENCY PIRFORMES LOCATIOe5 COLLECTED TfPE FREQUENCY Terrestrial Environment 1-131 Bl ocelly 60 Nilk Slecet ty (1) 7 60 60 Gamea SIweekIy Sr.89 Monthly 46 Sr-90 Monthly 46 Gamma Quarterly 12 Quarterly 3 12 Potable Water 1-131 Quarterly 12 H-3 Qearterly IF Gaema Monthly 24 Monthly 2 24 C Precipitation M-3 Monthly -24 24 Gr-Beta Monthly Seelannual 4 4 4 Gamma Game Seelannual Monthly 66 Annual (2) 6 66 Gamma Food Products I-131 Monthly 66 1

Every Three Years 0 Every Theee Years 10 0 Gamma 0

Soll Sr-90 Every Three Years

)

perect Radiation a

144 Games Dese Quarterly 144 Qvarterly 36 432 TLDs 432 Gamma Dose Monthly Monthly 36 (1) Milt is collected blecekly during the pcsture season and monthly during the songrazin9 season.

(2) When ellh samples are discontinued food product samples are collected monthly during harvest if necessary to comply with SWP5 Technical Specification 3.12.1.

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ya 1 II. RESULTS AND DISCUSSION O

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RESULTS AND O!SCUSSION The analytical results for the reporting period of January 1 through December 31, 1987, have been divided into four categories: aquatic, atmospheric, terrestrial, and direct radiation. The individual senples and analyses within each category display the unique radiological characteristics of that type of environment. Analytical results of the REMP are stsnmarized in Appendix A. The data for individual analyses are presented in Appendix C.

A. Acuatic Environment The aquatic environment in the vicinity of SNPS' consists primarily of Long Island Sound. The radiological characteristics were studied by i analyzing samples of surf ace water, Winter Flounder, Windowpane, Sea Robin,

Little Skate, Summer Flounder, American Lobster, Squid, Channeled Whelk, Blue Mussels, Sof t Shell Clams, aquatic plants and sediment. The samples were collected by LILCO Environmental Engineering Department and EA Engineering Science and Technology Inc. (under contract ,to LILCO). '
1. Surf ace Water (Table C-1)

Semiannual surf a'.t water samples were taken at six locations and I were analyzed for tritium, gama emitters, iodine-131, and strontium-89 -

and strontium-90.

Five surf ace water samples analyzed for tritium showed detectable levels between 170 and 430 pCi/l with an average of 268 pCi/t. The other seven samples were btalow the lower limit of detection. This is consistent with tritium concentrations observed in surface water during 1983 and 1984, 1 the preoperational period, and in 1985 and 1986. ,

! Naturally occurring potassium-40 was measured in eleven of the 1 samples with an average of 309 pC1/f and a range between 54.7 and 1290  :

Gi/1. No other gamma activity above the detectable levels was measured in ,

the twelve surf ace water samples as analyzed by gamma spectroscopy.

Surf ace water samples were also analyzed for iodine-131, strontium-89, and strontium-90. hone of these nuclides were observed within the limits ,

of detection, i

2. Fish (Table C-2) -

i l j Twenty-six fish samples were collected at three locations and the edible portions analyzed for ganrna emitters. Gamma spectrometry showed

! potassium-40 present in all samples with an average concentration of 3456 j pCi/kg wet and a range between 2040 and 4480 pCi/kg wet. Cesium-137 .

i wat detected in seven samples with an average activity of 14.6 pC1/kg wet i and a range between 8.9 and 25.8 pCi/kg wet. These activities are less than those reported in 1983 and 1984 during the preoperational period, and 1 Comperable to those reported in 1985 and 1986. i

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3. Invertebrates (Table C-3) ,

Twenty-three invertebrate samples, comprised of sof t shell clams, oysters, mussels, lobsters, squid, and whelks, were collected at six locations and analyzed for gama emitters, strontim-89 and strontim-90.

Gamma spectrometry showed detectable levels of potassim-40 in all samples, ranging from 1090 to 3870 pC1/kg wet with an average activity of 2391 pCi/kg wet. Naturally occurring beryllim-7 and thorium-228 were each measured one time with acttvities of 73.9 and 101 pCi/kg (wet), respec-tively. Cesium-137, attributed to f allout, was measured in two suples with activities of 34.8 and 36.2 pCi/kg wet. Neither strontium-89 or strontim-90 was detected.

4 Aquatic Plants (Table C-4)

Marine algae, collected at five locations (ten suples) in Long Island Sound and at one location in Wading River Marsh (two suples), were analyzed for gamma emitters and strontium-89 and strontium-90. Gamma spectrometry showed detectable potassium-40 in all samples ranging from 2930 to 36900 pC1/kg dry with an average of 17527 pCi/kg dry. Cosagenically ,

produced beryllium-7 was measured in eight of the s uples ranging from 172 to 3760 pCi/kg dry with an average activity of 1159 pCi/kg dry. Cesim-137 was measured in one sample with an activity of 85.5 pCi/kg dry. Naturally '

occurring thori m-228 was measured in nine samples with an average activity of 361 pCi/kg dry and a range of 111 to 1190 pCi/kg dry. Radium-226 was measured in two s uples with an average activity of 1086 pCi/kg dry and a range of 711 to 1460 pCi/kg dry. Strontim-90 was measured in two samplas with an average activity of 13.2 pCi/kg dry and a range from 8.3 to 18 pCi/kg dry. Strontim-89 was not observed.

The measured activities for Strontium-90 and Cesium-137 are consistent with those reported during the preoperational period of 1983-1984.

5. Sediment (TableC-5)

Eight of fshore sediment samples were collected in May and November at four offshore locations and analyzed for gama emitters and strontium-89 and l strontium-90. For the summation.of samples collected, location 4A3 is grouped with the offshore sites. Gama spectrometry showed detectable levels of potassim-40 in all samples ranging from 1840 to 8310 pCi/kg dry with an average activity of 3996 pCi/kg dry. Naturally occurring radi m-226 was observed in one sample with an activity of 839 pCi/kg dry. Thorium-228, also naturally occurring, was measured in seven samples within the range of 123 to 1080 pCi/kg dry with an average activity of 463 pCi/kg dry.

Cesium-137 was measured in one suple with an activity of 2167 pCi/kg dry.

All other gama emitters, were below the lower. limit of detection. No l strontin-89 or strontim-90 was detected in these samples.

Twelve beach sediment suples were collected and analyzed for strontium-89, strontium-90 and gama enitters. No stronti m was detected.

All suples had measurable activities of naturally occurring potassium-40 with an average activity of 2999 pC1/kg dry and a range of 1490 to 4900 pCi/kg dry. Two smples had measurable radium-226 with an average activity L

M1 , _ _ _ _ _ . _ _ _ _ _ _ _ _ __

of 859 pCi/kg dry and a range of 478 to 1240 pCi/kg dry. Eleven suples had i measurable thorium-228 with an average activity of 198 pCi/kg dry and a range of 74.0 to 741 pCi/kg dry. All other game emitters were below the lower limit of detection.

1 B. Atmospheric invironment The atmospheric environment in the vicinity of the SNPS was examined by analyzing smples of airborne particulates and airborne todine at 16 s upling locations. TEDA-impregnated charcoal cartridges used to collect airborne iodine were collected weekly and analyzed by gama spectrometry for ,

iodine-131. Airborne particulate filters were collected weekly and analyzed for beta emitters. Quarterly composites from each station were analyzed for gama emitters and radiostrontium.

1. Airborne Particulates (Tables C-6, C-7, C 8 and C-9)

Beta-emitter concentrations ranged *from 0.004 to 0.032 pC1/m3 with an annual average for the 16 supling locations of 0.016 pCi/m3 -

(Table C-6). Of the 796 measurements nine were below the detection limit, nominally 0.004 pCi/m3 Figure 1 shows the average weekly gross beta fluctuations in air particulates from all stations for 1987.

Figure 2 represents the avera particulates from January 1, 1977 ge monthly through gross beta Dec eber 31,results 1987. in air Results of gama spectrometry (Table C-7) showed detectable levels of naturally occurring bery111um-7 in all sixty two suples. Due to an i electric cable f ailure no weekly suples were collected at station 652 in the third and fourth quarters. Therefore, there ore only 62 composite ,

suples for the year. The average bery111um-7 activity in the q analyses was 0.084 pCi/mJ with a range of 0.046 to 0.128 pCi/m3.uarterly Naturally occurring potassium-40 was obserted seven times. The potassium-40 had an average of 0.015 pCi/m3 with a range of 0.0089 to 0.028'pCi/m3 All other gamma emitters were below the lower limit of 1 detection.

The radiostrontin analyses on the 62 quarterly composites showed i no detectable levels of strontium-89 or stronti m-90. '

2. Airborne lodine (Table C-9)

Analytical results of airborne iodine-131 were all belgw the lower t limit of detection which ranged between 0.01 and 0.06 pCi/m3 [,

3. Noble Gas (Table C-18)

Air suples were collected weekly at St. Joseph's Villa and ,

! analyzed for Krypton 85 and Xenon-133. Xenon-133 was not found in any sample. All 52 s uples had p ranging from 24 to 45 pC1/m3,ositive concentrations with an average of Krypton-85 concentration of 32

pCi/m3, similar to the average concentrations found during the pre- i operational years.  !
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C. Terrestrial Environment The terrestrial environment in the vicinity of the SNPS was examined by analyzing samples of game (raccoon and squirrel), milk, food products, rainwater and potable water. Gama spectrometry was performed on all s amples , in addition, iodine-131, stronti m-89 and strontium-90 analyses were performed on the milk samples, while tritium and iodine-131 analyses were performed on the potable water samples. Rainwater samples were analyzed for gross beta, tritium and gamma emitters.

1. Milk (Tables C-11 and C-12)

All of the 60 monthly and semimonthly cow and goat milk samples analyzed for iodine were below the LLD which ranged between <0.2 and <0.6 pCi/t. Naturally occurring potassium-40 was oM erved in all the milk samples. The goat milk samples had an average mesurement of 1332 pCi/l and a range of 1190 to 1860 pCi/l. The cow milk samples had an average concen-tration of 1270 pCi/l with a range of 800 to 1880 pCi/l. Cesium-137 was detected in seven of the 31 goat milk samples with in average of 8.7 pCi/l and a range of 7.5 to 10.1 pCi/l. Six of the 27 cow milk sanples had detectable measurements of cesim-137 with an average of 8.4 pCi/l and a range of 5.9 to 11.5 pCi/1.

All other gamma emitters, as well as strontium-89 were below the detection limit. Strontium-90 was observed in all of the cow and goat milk samples. In the 18 cow milk samples, the average strontium-90 concentration was 5.8 with a range from 1.3 to 15.0 pCi/f. For the 22 goat milk samples, the average strontim-90 concentration was 2.4 pCi/f and the range was from 0.61 to 6.3 pC1/l. The activities reported for strontium-90 are consistent with those found in cow and goat milk samples from 1983 to present.

2. Potable Water (Table C-13)

Tritium activity was measured in four of the twelve potabl? water samples collected at three locations. In these four samples, t?' average tritium concentration was 253 pCi/l with a range of 140 to 450 pCi/1. The other tritium results were below the lower limit of detection which varied between 100 and 200 pCi/l. This is consistent with the iesults of the

previous four years. No iodine-131 was measured above the lower limit of detection which was between 0.2 and 0.3 pCi/f. Naturally occurring potassium-40 was observed in one sample with an activity of 60.5 pCi/l. All other gamma emitters were below the lower limit of detection.

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3. Game (Table C-14)

Potassium-40 was observed in the four game samples (two raccoons and two squirrels) with an average activity of 3173 pCf /kg wet and a range from 2370 to 3960 pCi/kg wet. However, cesium-137, the only other observed gamma emitter, was measured over a greater range of activity due presumably to differences in diets and possibly to seasonal effects. For the two raccoon samples the average cesium-137 activity was 277 pCi/kg wet and the two tralues were 35.1 pCi/kg wet and 518 pCi/kg wet. These results are consistent with results of the previous four year;. The average cesium-137 activity in the two squirrel samples was 3321 pCi/kg wet and the range was from 152 to 6490 pCi/kg wet.

21 __ _ _.

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4. Food Droducts (Table C-15)

Sixty-six human food products from local f arms were analyzed, including tomatoes, potatoes, cabbage, lettuce, beets, radishes, spinach, onions, ,

collards, strawberries, carrots, and corn. All samples contained naturally '

occurring potassi m-40 with an average of 2951 pCi/kg wet and a range of 1250 to 7200 pCi/kg wet. Naturally occurring beryllium-7 was measured in i seven samples with an average activity of 171 pCi/kg wet and a range of 91.8 to 250 pCi/kg wet. The seven samples were lettuce and spinach, both being large surf ace leafy vegetables onto which beryllim-7 could deposit from the atmosphere. Cesium-137 with an activity of 86.3 pCi/kg wet was measured in one lettuce sample. Naturally occurring thorim-228 was detected with an activity of 67.9 pCi/kg wet in one spinach sample. All other gamma emitters were below the lower limit of detection. The samples were also analyzed for iodine-131 by a radiochemical procedure. No activity was found. The detection limit varied from 3 to 30 pCi/kg wet.

5. Precipitation (Table C-10)

Twenty-four precipitation samples were collected at two stations during the twelve months and analyzed for gross beta, tritium and gamma emitters.

Gross beta activity was measured in the 24 samples with an average activity of 8.2 and a range of 1.8 to 65 pCi/1.

Tritium was measured in nine of the 24 samples with an average activity of 252 pCi/l and a range of 130 to 370 pCi/1.

Naturally occurring beryllim was observed in five samples from station 12A1 with an average of 72.1 pCi/t and a range of 48.7 to 85.1 pCi/1. All other gamma emitters were below detection limits. .

D. Direct Radiation (Tables C-17 and C-18)

Direct radiation measurements were taken monthly and quarterly at 36 l locations using CaSO4:Dy thermoluminescent dosimeters (T'.Ds). TLDs were

( used to detect radiation levels near ground level in the vicinity of the Shoreham site due to terrestrial and cosmic gama ray emitters and possible SNPS contributed direct radiation. Figure 3 presents a compar ison of average TLD results from 1977 to 1987. All TLD results presented in this report have been normalized to a standard month (30.4 days) to eliminate the apparent differences caused by the variations in exposure period. The average cf the quarterly exposures was 3.7 mR/ standard month and the average of the c.enthly exposures was also 3.7 mR/ standard month. This is less than quarterly and monthly values, respectively, measured during the pre-operational years 1983 and 1984.

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E. Dose Assessment Table 2 summarizes the results of the dose assessment determinations based on 1987 data.

Initially all positive concentrations of radionuclides in indicator samples, as shown in Appendix A, were considered for inclusion in the dose calculation. In an attempt to factor out as much of the contribution due to natural and man-made background radiation as possible, indicator and control sample results were compared. If the control location results were com-parable to or greater than those at the indicator location, then the indicator sunple results were not included in the dose assessment. Surface water, aquatic plants and precipitation were not considered as significant human exposure pathways and, therefore, not considered in the dose assessment.

The dose due to standing on contaminated soil / sediment was not calculated since this is accounted for in the direct radiation dose.

Bery111un-7, potassium-40, radium-226, radium-228 and thorium-228 are all naturally occurring isotopes and not likely to be produced as a result of the operation of Shoreham so they were excluded. Krypton-85 was also excluded as an individual contributor to dose since it is not absorbed or -

ingested and is included in the direct radiation component. The remaining .

positive isotopes, cesium-137, strontium-90 and tritium, could be produced as a result of plant operation so they were included in the dose calculations.

It should be noted that tritium also occurs naturally as a result of cosmic interactions, and cesium-137 and strontium-90 exist in the environment as a result of atmospheric weapons testing and the Chernobyl accident.

Comparison of the results of the dose assessment of 1987 with those of the preoperational years 1983 and 1984, show similar results for all three years. The direct radiation dose in 1987 (Appendix 0) was less than in 1983 and 1984. Doses calculated for 1983 were based on ingestion factors

. f or the averaos individual, whereas the maximun individual ingestion factors were used in 1984 and 1987. This makes exact comparison of the results difficult; however..the dose is directly proportional to the activity in the medium: in all cases considered the concentrations found in 1987 are consistent with those of 1983.

It should be noted that cesium-137 found in game samples was considered as a dose contributor by using ingestion factors for meat. This is highly conservative.

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TABLE 2

SUMMARY

OF DOSE OETERMINATION FOR 1987 PATHWAY / TOTAL BODY CRITICAL ORGAN MOST SEN51TIVE RADIONUCLIDE ACTIVITY QUANITITY OOSE FACTOR DOSE FACTOR BODY DOSE ORGAN DOSE AGE GROUP (5) OR TLD IN MEDIUM INGESTED (1) (den /pCl (dee/pCl (den /yr.) (den /yr.)

INGESTED)(2) INGESTED)(2)

Invertebrates Adult Cs-137 35.5 pCl/kg wet 5.0 kg/yr. 7.14 E-5 1.09 E-4 Ilver 1.27 E-2 1.93 E-2 liver Teen 3.8 kg/yr. 5.19 E-5 1.49 E-4 liver 7.00 E-3 2.01 E-2 liver lN w Fish Mutt Cs-137 16.5 pCl/kg met 21. kg/yr. 7.14 E-5 1.09 E-4 liver 2.47 E-2 3.78 E-2 Ilver Teen 16. kg/yr. 5.19 E-5 1.49 E-4 liver 1.37 E-2 3.93 E-2 liver Game M ult Cs-137 1799 pCl/kg wet 110 kg/yr(3) 7.14 E-5 1.09 E-4 Ilver 1.41 E+1 2.16 E+1 !!ver i Child 41. kg/yr(3) 4.62 E-5 3.27 E-4 bone 3.41 E+0 2.41 E+1 bone 1

-i I.

  • Comparison of the 1987 doses with those of the preoperational years 1983 and 1984 shows no signiflCant differences.

j (1) From Table E-5 maaleum exposed individual. Reg. Guide 1.109.

(2) From Tables E-II. E-12. E-13 and E-14. Reg. Guide 1.109.

! (3) Meat and Poultry pathway, Table E-5. Reg. Guide 1.109. Utilizing 110. Eg/yr. for adults and 41. kg/yr. for

  • Children as the quantity of game Consumed results in a Conservatively high Calculated dose.

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CONCLUSIONS During 1987 the Shoreham Nuclear Power Station conducted tests at power levels below 5% between May 26 and June 8, and was shutdown for the remainder of the year.

The accident at the Chernobyl nuclear reactor in 1986 in Russia contributed measurable amounts of radioactivity to the environment still evidenced in 1987. By comparison of results for indicator and control locations, most of the positive results for possible plant generated radionuclides can be attributed to natural or man-made background radiation and not Shoreham. Otherwise, analyses of the environmental samples show results consistent with those found during the preoperational years 1983 and 1984. Sensitive indicators revealed minute quantities of radioacthe fallout from the October 1980 atmospheric nuclear weapons test by the Peoples Rebuplic of China, in addition to radioactivity remaining from two decades of atmospheric testing.

Along with these anomalies in the environment, expected normal back-ground radioactivity has been measured in REMP samples. Aquatic and terrestrial samples were analyzed and reflected the normal background radiation found in the environment. The atmospheric environment was sampled for airborne particulate matter, iodine, and noble gases. Figure 1 represents the average weekly gross beta results in airborne particulates from January through December 1987. Figure 2 shows the average monthly gross beta results in airborne particulates from February 1977 to December 1987. Direct radiation levels were relatively low and approximately the same at all locations. Figure 3 shows the average quarterly TLD results in mR/ standard month from January 1977 to December 1987.

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4 IV. REFERENCES 1

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0 IV. REFERENCES (1) Long Island Lighting Company. "Shoreham Nuclear Power Station, Environmental Report, Construction Permit Stage", December 1977.

(2) United States Atomic Energy Comission, Directorate of Licensing "Final Environmental Statement Related to Operation of Shoreham Nuclear Power Station", Docket No. 50-322, September 1972.

(3) Long Island Lighting Company. "Shoreham Nuclear Power Station, Updated Safety Analysis Report".

(4) Radiation Management Corporation. "Shoreham Nuclear Power Station Radiological Environmental Monitoring Program - 1977 Annual Report",

March 1978.

(5) Radiation Management Corporation. "Shoreham Nuclear Power Station Radiological Environmentai Monitoring Program - 1978 Annual Report",

April 1979.

(6) Radiation Management Corporation. "Shoreham Nuclear Power Station Radiological Environmental Monitoring Program - 1979 Annual Report",

June 1980.

(7) Radiation Management Corporation. "Shoreham Nuclear Power Station Preoperational Radiological Monitoring Program - 1980 Annual Report", September 1981.

(8) Radiation Management Corporation "Shoreham Nuclear Power Station Preoperational Radiological Monitoring Program - 1981 Annual Report,"

October 1982.

(9) Eisenbud, M., Environmental Radioactivity, 2nd Ed.,1973.

(10) National Academy of Sciences, Radioactivity in the Marine Environment, National Research Council, Washington, D.C., 1971.

(11) Long Island Lighting Company. "Shoreham Nuclear Power Station, Procedure Manual, Radiological Environmental Monitoring Program",

29

IV. REFERENCES (Cont.)

(12) EA Science and Technology Shoreham Project Quality Assurance and Procedures Manaual, March 1985.

(13) U.S. Nuclear Regulatory Commission Regulatory Guide 1.109, Rev. 1-1977.

(14) Health Physics Journal, Vol. 38, No.4, April 1980.

(15) Teledyne isotopes "Nuclear Reactor Environmental Radiation Monitoring Quali cy Control Manual", IWL-0032-361.

(16) Teledyne Isotopes "Quality Control Internal Controls and Audits, Environmental Analysis Department". IWL-0032-365.

(17) Teledyne Isotopes "Quality Assurance Manual, Environmental Analysis Department Compliance with 10CFR50 Appendix B and Reg. Guide 4.15",

IWL-0032-395.

(18) Long Island Lighting Co. and Teledyne isotopes,1982 Radiological Environmental Monitoring Program Annual Report.

(19) long Island Lighting Co. and Teledyne Isotopes,1983 Radiological Environmentai Monitoring Progra Annual Report.

i' f (20) long Island Lighting Co. and Teledyne Isotopes,1984 Radiological Environmental Monitoring Progra Annual Report.

(21) Long Island Lighting Co. and Teledyne Isotopes,1985 Radiological Environmental Monitoring Program Annual Report.

(22) Long Island Lighting Co. and Teledyne Isotopes,1986 Radiological Environmental Monitoring Progra Annual Report.

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4 APPENDIX A RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

31

RADIOLOGICAL ENVIR0f*IECTAL MONITORING PROGtAM StMIARY SHOREHAM NUCLEAR POWER STATION DOCKEi No. 50-322 SUFFOLK COUNTY NEW YORK JANUARY I to DECEMBER 31. 1987 MMBER OF l ANALYSIS AND LOWER LIMIT '

MEDitM OR PATHWAY 10iAL NUMBER OF ALL INDICAIOR LOCATION 5(3) LOCATION WITH HIGHEST MEAN CONTROL LOCATION 5(3) NONROUllNE 5AMPLED OF ARALYSES DETECTION M[AN(2) NAK MEAN(2) KAN(2) REPONTED DISTANCE AND DIRECTION RANGE RANGE MEASURENENTS (UNIT OF ME ASUREMENT) PERf0RMLD (LLD) (1) RANGE 250(3/8) 251 0.1 al NME 295(2/4) 260(1/4) 0 Potable Water H-3 12 100 (pCl/f) (140-450) (140-450) -

I-131 12 0.1 -(0/8) N/A N/A -(0/4) 0 Gamuna 12 K-40 60.5(1/8) 251 0.1 al ImE 60.5(1/4) -(0/4) 0 Th-228 -(0/8) N/A N/A -(0/4) 0 Game Gamma 4 (pCl/kg wet) 0 K-40 300 3173(4/4) 1353 0.3 at W 3173(4/4) -(0/0)

(2370-3960) (2370-3960) -

.1799(4/4) 1353 0.3 at W 1739(4/4) -(0/0) 0 Cs-137 7 (35.1-6490) (35.1-6490) -

Direct Radiation Gamuna 432 (mR/ Standard month) Dose 1.5 3.7(360/360) 6Al 0.7 at ESE 4.9(12/12) . 3.8(72/72) O Montiety (2.8-6.9) (4.3-6.3) (2.8-5.3)

Gamma Dose 144 1.5 3.7(120/120) 6Al 0.7 at ESE 4.8(4/4) 3.8(24/24) 0 Quarterly (2.9-5.0) (4.6-5.0) (3.2-4.6)

(1) The LLDs quoted are the lowest actual LLDs obtained in the various media during the reporting period. Typical LLDs were determined for each nuclide as found on Tables C-19 and C-20. Idhere all nuclides were (tLD for a specific media no LLO was listed.

(2) Means calculated using detectable measurements only. Fractions of detectable measurements in parentheses.

(3) Indicator and control locations are noted in Appendix 8. Table 8-1. ,

I \

RADIOLOGICAL ENVIR0petENTAL MONITORING PROGRAM

SUMMARY

SHOREHMI NUCLEAR POWER STATION DOCKET NO. 50-322 .

1 SUFFOLK COINITY, NEW TORE JANUARY l to DECEMBER 31, 1987 l ANALY515 AND LOWER LINIT Nem8ER OF MDitM OR PATHWAY TOTAL M MBER OF ALL INDICATOR LOCATION 5(3) LOCATION WITH HIGHEST '(AM CONTROL LOCATION 5(3) NONROUTINE SAfeLED OF ANALYSES DETECTION MAN (2 } NAME T AN(2) MEAR(2) REPOR TED (UNIT OF MASUREMENT) PERf0RMED (LLD) (1) RANGE DISTANCE AND DIRECT 104 RANGC RANGE M ASUREM Nis Al rne Particulates Gross Beta 7% 4 16(581/588) 10t1 0.3 al SSW 17(52/52) 16(206/208) 0 (10- pCl/m3) (4-32) (7-30) (4-30)

Sr-89 62 0.3 -(0/46) N/A N/A -(0/16) 0 l

l w Sr-90 62 0.8 -(0/46) N/A N/A -(0/16) 0 w - -

Gasma 62 Be-1 -

86(46/46) 12Al 0.9 at W5W 95(4/4) 79(16/16) 0 (45.7-128) (63.9-126) (50.9-110)

K-40 7 19(5/46) 2A3 0.3 at NME 28(1/4) 7.0(2/16) 0 (9.3-27.5) -

(8.9-5.1)

Air rne dine I-131 1% 10 -(0/588) N/A Nia -(0/208) 0 (10- pCi/ ) -

(1) The LLDs quoted are the lowest actual LLDs obtained in the various media during the reporting period. Typical LLDs were determined for each nuclide as found on fables C-19 and C-20. Where all nuclides uere <LLD for a specific media no LLD was listed.

(2) Means calculated using detectable measurements only. Fractions of detectable measurements in parentheses.

(3) Ind!cator and control locations are noted in Appendix 8. Table 8-1.

RADIOLOGICAL ENVIR0 MENTAL MONITORING PROGRAM StMMARY SHOREHMt NUCLEAR POWER STATION DOCKET No. 50-322 SUFFOLK COUNTY, NEW YORK JANUARY l to DECEMBER 31, 1987 ANALYSIS AND LOWER LIMIT NUMBER OF MEDItM OR PATHWAY TOTAL NtMBER OF -ALL INDICATOR LOCATl0N5(3) LOCATION WITH HIGHEST MEAN CONTROL LOCAT10N5(3) NONROUTINE SAMPLED OF ANALYSES DETECTION m antzt negt MAN (2) MEAN(2) REPORTED (UNIT OF E ASUREMENT) PERf0RMED (LLD) (1) RANGE DISTANCE AND DIRECTION RANGE RANGE MEASUREMENTS 1

Aquatic Plants Sr-89 12 6 -(0/8) NA 0 (pCl/kg-dry) -

-(0/4 )

Sr-90 12 1 -(0/8) 13G2 13 al W 18.0(1/2) 13.2(2/4) 0 (8.3-18.0)

$ Gamma 12 Be-7 200 1533(5/8) 4A3 0.2 at NW 3340(2/2) 537(3/4) 0 (172-3760) (2920-3760) (523-558)

K-40 300 14703(8/8) 16Al 0.4 al NNW 28600(2/2) 23175(4/4) 0 (2930-36900) (20300-36900) (18000-30200)

Cs-137 6 85.5(1/8) 4A3 0.2 at NNW 85.5(1/2) -(0/4) 0 Ra-226 100 1460(1/8) 4A3 0.2 al NW 1460(1/2) 711(1/4) 0 Th-228 10 464(6/8) 4A3 0.2 el NW 1140(2/2) 156(3/4) 0 (111-1190) (1090-1190) (117-220)

(1) The LLDs quoted are the lowst actual LtDs obtained in the various media during the reporting period. Typical LLDs were l determined for each nuclide as found on Tables C-19 and C-20. Eere all nuclides wre <LLO for a specific media no LLD was listed.

(2) Means calculated using detectable measurements only. Fract ions of detectable measurements in parentheses.

(3) Indicator and control locations are noted in Appendia 8. Table B-1.

RADIOLOGICAL ENVIRGIMENTAL MONITORING PROGRAM SUPMARY SHOREHAM NUCLEAR POWER stall 0M DOCKET NO. 50-322 SUFFOLK COUNTY, NEW YORK JANUARY l to DECEMBER 31, 1987 ANALYSIS AND LOWER LIMIT INDISER OF MEDitM OR PATHWAY TOTAL NUMBER OF ALL INDICATOR LOCAT1045(3) LOCATION WITH HIGHEST MEAN C08tTROL LOCATION 5(3) NONROUTINE

$AMPLED OF ANALYSES DETECTION M AN(2) NAME EAfe(2) MAse(2) REPORTED (UNIT OF MEASUREMENT) PERFORMED (LLD) (1) RANGE DISTANCE AleD DIRECTION RANGE RAfeGE E ASUREMENTS Milk I-131 60 0.2 -(0/28) N/A N/A -(0/32) 0 (PC1/2) - -

Sr-89 40 2 -(0/14) N/A N/A -(0/26) 0 w Sr-90 40 1 2.6(14/14) 8G2 10.8 al SSE 8.7(9/9) 4.6(26/26) O m

(0.61-5.7) (2.3-15.0) (0.9-15) i Gamuna 60

-! K-40 100 1594(19/19) 1381 1.9 at W 1850(1/1) 1341(41/41) 0 (1190-1880) -

(800-1860) l Cs-137 4 8.l(5/19) 8G2 10.8 el SSE 9.9(1/14) 8.8(8/41) 0 4' (5.9-11.5) -

(7.5-10.1) t (1) The LLDs quoted are the lowest actual LLDs obtained in the various media during the reporting period. Typical LLDs were determined for each nuclide as found in Tables C-19 and C-20. mere all nuclides were <LLD for a specific media no LLD was listed.

] (2) Means calculated using detectable mPasurements only. Fractions of detectable measurements in parentheses.

(3) Indicator and Control locations are noted in Appendix 8 Table B-1.

l

a, .

RADIOLOGICG ENVIR0leqENICl MONITORING PROGRAM SurelARY SHOREHAM NUCLEAR POWER stall 0N DOCKET NO. 50-322

$UFFOLK COUNTY, NEW YORK JANUARY I to DECEMBER 31, 1987 ANALYSIS AND LOWER LINii NLat9ER OF MEDitM OR PATHWAY TOTAL NUM8ER (4 Att INDICATOR LOCATION 5(3) LOCATION WITH HIGHEST MEAN CONTROL LOCATION 5(3) NONR0uilNE i SAMPLED OF ANALYSES DETECTION man (z) RAML F.AN(2) MAN (2) REPORTED l (UNii 0F MASUREMENI) PERIORME D (LLD) (1) RANGE DISTANCE AND DIR'Cil0N RANGE RANGE MEASUREMENTS Iood Product 5 Gamma 66 (pCl/kg-wet)

I-131 4 -(0/44) N/A N/A -(0/22) 0 K-40 300 2815(44/44) 12H2 32.1 at WSW 3521(14/14) 3223(22/22) 0 (1250-6800) (1360-7200) (1360-7200)

Be-7 -

177(4/44) SC2 2.8 at E 184(2/20) 162(3/22) 0 (91.8-250) (156-211) (119-233) i Cs-137 5 -(0/44) 12H2 32.1 at WSW 86.3(1/14)' 86.3(I/22) 0 l

t Th-228 67.9(1/44) SC2 2.8 al E 67.9(I/20) -(0/22) 0 1 - - -

Aquatic Invertebrates Sr-89 23 1 -(0/14) N/A N/A -(0/9) 0 (pCl/kg wet) - -

Sr-90 23 1 -(0/14) N/A N/A -(0/9) 0 Ganna 23 K-40 300 2335(14/14) 14Cl 2.0 at WNW 2728(5/5) 2478(9/9) 0 (l090-3090) (2410-3060) (l390-3870)

Be-7 80 -(0/14) 13FI 9.4 at W 73.9(1/2) 73.9(1/9) O Cs-137 5 35.5(2/14) XI 2.9 al NE 36.2(1/4) -(0/9) 0 (34.8-36.2) - -

Th-228 -

101(1/14) 4A3 0.2 at ENE 101(1/3) -(0/9) 0 (1) The LL0s quoted are the lowest actual LLDs obtained in the various media during the reporting period. TyplCal LLDs were determined for each nucIlde as found on Tables C-19 and C-20. leere all nuclides were (LLD for a specific media no LLD was listed.

(2) Pirans calculated using detectable measurements only. Fracticas of detectable measurements in parentheses.

(3) Ind6cator and control locations are noted in Appendia 8. Table B-1.

o e

- _ _ _ _ _ _ _ .~

RADIOLOGICAL ENVIR0mECIAL MONITORING PROGRAM

SUMMARY

$HOREHAM NUCLEAR POWER STAil0N DOCKET No. 50-322

$UFFOLK COUNTY, NEW YORK JANUARY I to DECEMBER 31, 1987 ANALY515 AND LOWER LIMIT NtMBER OF MEDIUM OR PATHWAY TOTAL NUMBER OF ALL INDICATOR LOCAil0N5(3) LOCATION WITH HIGHEST MEAN CONTROL LOCAT10N5(3) NosNt00 TIME SAMPLED OF ANALYSES DETECTION MEAN(2) NAME FEAN(2) MEAN(2) REPORTED (UNIT OF MEASUREMENT) PE RFORMED (LLD) (I) RANGE DISTANCE AND DIRECil04 RANGE RANGE MEASUREMENTS Sediment (Beach) $r-89 12 2 -(0/8) N/A N/A -(0/4) 0 (pCl/kg dry) ,

Sr-90 12 1 -(0/8) N/A N/A -(0/4) 0 Gama 12 K-40 900 2659(8/8) 4A3 0.2 al ENE 0 (1490-4900) 3775(2/2)

(2650-4900 ) 3680(4/4)

(1500-4600 ) .

Cs-137 8 -(0/8) N/A N/A -(0/4) 0 J

Ra-226 200 4A3 0.2 mi ENE 1240(1/2) -(0/4 ) 0 8592/8)0)

(47 -12 _

Ra-228 200 104(2/8) 3A2 0.7 al lee 137(1/2) -(0/4) 0 (10.2-137) - -

Be-7 -(0/8) NA -(0/4) 0 i Th-228 60 209(8/8) 4A3 0.2 el ENE 165(3/4) 0

(74.0-741) 524(2/2))

(306-741 (95.8-221)

(1) The LLDs quoted are the lowest actual LLDs obtained in the various media during the reporting period. Typical LLDs were determined for each nuclide as found in Tables C-19 and C-20. leiere all nucildes were <tLD for a specific media no LLD was listed.

(2) Mrans calculated using detectable measurements only. Fractions of detectable measurements in parentheses.

(3) Indicator and control locations are noted in Amndix 8, table B-1. ,

4 i

1 4

RADIOLOGICAL ENVIR08 MENTAL MONITORING PROGRAM StMMARY 5HOREHAM NUCLEAR POWER STATION DOCKET NO. 50-322 Suf f 0LK COUNTY, NEW YORK JANUARY l to DECEMBER 31, 1987 ,

ANAlv515 AND LOWER LIMIT NIMBER OF MEDItM OR PATHWAY TOTAL NUMBER OF ALL INDICATOR LOCATION 5(3) LOCATION WITH HIGHEST MAN CONTROL LOCA! ION 5(3) NONROUTINE SAMLED OF ANALV5ES DETECTION M AN(2 ) NARL RLAN(2) MEAN(2) REPORTED l (UNIT OF MEASUREMENT) PERf0RMED (LLD) (1) RANGE DISTANCE ANO DIRECTION RANGE RANGE MEASUREMENTS Sedleent (Of fshore) $r-89 8 2 -(0/6) N/A N/A -(0/2) 0 (PCI/kg dry)

Sr-90 8 2 -(0/6) N/A N/A -(0/2) 0 l

Gamma 8 b K-40 900 4640(6/6) 1681 1.3 al NNW 7765(2/2) 2065(2/2) 0 (1840-8310) (7220-8310) (2000-2130)

Cs-137 10 21.7(1/6) 3C1 2.9 al NE 21.7(1/2) -(0/2) 0 Ra-226 200 839(1/6)) 1681 1.3 el NNW 839(1/2) -(0/2) 0 Ra-228 200 -(0/6) N/A N/A -(0/2) 0 Be-7 366(1/6) 3Cl 2.9 al NE 366(1/2) -(0/2) 0 Th-228 60 520(6/6) 1681 1.3 ml INNd 1045(2/2) 123(1/2) 0 (171-1080) (1010-1080) -

(1) The LLDs quoted are the lowest actual LLDs obtained in the various media during the reporting period. Typical LLDs were determined for each nucIlde as found in Tables C-19 and C-20. Where all nuclides we <LLD for a specific media no LLD was listed.

(2) Means calculated using detectable measurements only. Fractions of detectable measurements in parentheses.

(3) Indicator and control locations are noted in Appendix 8. Table 8-1.

RADIC10GICQ [NVIROIMECTAL MONITORING PROGRAM 5tsenty 5HOREHAM NUCL(AR POWER 5TATION DOCKET NO. 50-322 SUFFOLK COUNTY. NEW YORK JANUARY I to DECEMBER 31. 1987 ANALYS15 AND LOWER LIMIT NtMBER OF MEDILM OR PATHWAY TOTAL NUM81R OF Att INDICATOR LOCATIOW5(3) LOCATION WITH HIGHEST MEAN CONTROL LOCAT1045(3) NONROUTINE SAML E D OF MALY$[$ DETECTION MEAN(2) NAME MEAN(2) MEAN(2) REPORTED (UNIT OF ptASUREMENT) PERf 0RMED (LLD) (1) RANGL DISTANCE AND DIRECTION RANGC RANGC MEASUREMENTS Surf ace Water H-3 12 100 277(3/8) 4A3 0.2 al ENE (pCl/f) 300(2/2) 255(2/4) 0 (170-430) (170-430) (220-290)

Sr-89 12 1 -(0/8) N/A N/A -(0/4) 0

$r-90 12 0.5 -(0/8) N/A N/A -(0/4) 0 W Ganna 12 K-40 50 348(7/8) 3Cl 2.9 al NE 144(2/2) 241(4/4) 0 (54.7-1290) (191-1290) (208-270)

Cs-137 6 -(0/8) N/A N/A -(0/4) 0 Fish Sr-89 26 1 -(0/18) N/A N/A -(0/8) 0 (pCl/kg wet) - -

Sr-90 26 0.5 -(0/18) N/A N/A -(0/8) 0 Ganssa 26 K-40 300 3498(18/18) 14C1 2.1 at WNW 0 (2040-4480) 3533(9/9)

(2240-4480 ) 3360(8/8)

(2400-4290 )

Cs-137 5 16.5(5/18) 14C1 2.1 at WNW 25.8(1/9) 9.6(2/8) 0 (l1.0-25.8) -

(8.88-10.4)

Th-228 -

-(0/18) N/A N/A -(()/8) 0 (1) The tLDs quoted are the l'est actual LLDs obtained in the vartous media during the reporting period. TyplCal LLDs were determined for each auc' de as found on Tables C-19 and C-20. Were all nucIldes were (LLD for a specific media no LLD was listed.

(2) Means calculated using aetectable measureements only. Fractions of detectable measurements in parentheses.

(3) Indicator and control locations are noted in Appendia 8. Table 8-I.

O '

I

t

  • t

{

RADIOLOGICAL ENVIROIMENTAL MONITORING PROGRAM

SUMMARY

SHOREHAM NUCLEAR POWER STAT 104 DOCKEi NO. 50-322 l

SUIf0LK COUNTY, NEW YORE JANUARY I to DECEMBER 31. 1987

' ANALYSIS AND t0W5R LIMIT M 0!tM OR PATHWAY NUMBER OF TOIAL NtMBER Of Att INDICATOR LOCAT10N5(3) LOCATION WilH HIGHEST M[AN SAMPLED OF ANALYSES DETECTION CONTMOL LOCAT10N5(3) NONROUTINE MEAN(2) NAME MAN (2) MEAN(2) REPORTED (UNIT OF MEASUREMENT) PERFORMED (LLD) (I) RANGE DISTANCE AND DIRECTION RANGE RANGE MEASUREMENTS Precipitation Gross Seta 24 (pCl/f) 1 8.2(24/24) 951 0.3 al 5 11.2(12/12) No Control 0 (1.8-65) (2.0-b5) d-3 24 90 268(10/24) 12Al 0.9 at WSW 295(6/12) No Control 0

, (130-410)

@D (160-410)

Gamma 24 Be-1 60 12.l(5/24) 12Al 0.9 el WSW 72.l(5/12) No Control 0 (48.7-85.1) (48.7-85.1)

Noble Qas Kr-85 52 15 32.4(52/52) 1452 0.4 al WNW (pCl/m3) 32.4(52/52) No Control 0 (24-45) (24-45)

Xe-133 52 11 -(0/52) N/A N/A No Control 0 (1) The LLDs quoted are the lowest actual llDs obtained in the various media during the reporting period. Typical LLDs were determined for each nuclide as found on Tables C-19 and C-20. mere all nuclides were (LLD for a specific media no LLD was listed.

Means calculated using detectable measurements only. Fractions of detectable measurements in parentheses.

Indicator and control locations are noted in Appendix 8. Table 8-1.

I e

l l

l APPENDIX 8 SAMPLE DESIGNATION AND LOCATIONS l

41 .

j APPENDIX B i

l Sample Designation LILC0's Radiological Environmental Monitoring Program (REMP) identifies samples by a three , irt code. The first two letters are the power station identification code, ;n this case "SN". The next three letters are for the media sampled.

SWA = Surf ace Water (Long Island Sound) GMK = Goat Milk AQF = Fish (1) PWA = PotableWater(groundwater)

=

AQI = Invertebrates (1) GAX Game (1)

AQP = Aquatic Plants (1) FPV = Food Products (1)

AQS = Sediment FPF = Fruit

=

APT = Airborne Particulates IDM Immersion Dose (TLD)

AIO = Airborne lodine NBG = Noble Gas MLK = Milk RWA = Precipitation (Rain Water)

SOL = Soil The last four synbols are a location code based on direction and distance from the site. Of these, the first two represent each of the sixteen angular sectors of 22 1/2 degrees centered about the reactor site. Sector one is divided evenly by the north axis, and other sectors are numbered in a clock-wise direction, i.e., 2=NNE, 3=NE, 4=ENE, etc. The next digit is a letter which represents the radial distance from the plant:

S = On site location E = 4-5 miles off site A = 0-1 miles off site F = 5-10 miles off site B = 1-2 miles off site G = 10-20 miles off site C = 2-3 miles off site H = >20 miles off site 0 = 3-4 miles off site The last number is the location numerical designation within each sector and zone, e.g.,1,2,3,....For example, the designation SN-SWA-3C1 would indicate a sample in the SNPS program SN, consisting of surface water SWA, which had been collected in the 22-1/2 degree sector centered on the northeast axis (3) between the site boundary and 2-3 miles off site (C). The number 1 indicates that this is sampling station No.1 in the designated area.

Sampling Locations All sampling locations and specific information about the individual locations are given in Table B-1. Tables B-2 through B-5 list the sampling locations and media required by Technical Specifications.

l l

(1) A more specific means of classification will be noted inFor theexample, comment AQI section of each laboratory report for these samples.

l will be designated, n. the sample description, as aquatic invertebrate.

(

However, the coment section will specify the sample type by the generally accepted comon name of the sample involved. In this case, clam, lobster, crab or other aquatic invertebrate would be listed in the coment section.

42

APPENDIX B Sampling Locatior.s Maps B-1, B-2 and B-3 show the locations of 1987 sampling stations with respect to the site. These maps are tracings of portions of larger maps prepared by LILCO's Survey Division after an extensive land survey of REMP monitoring locations. Additional information can be obtained by referring to the Site and Vicinity Map of the Shoreham Nuclear Power Station (Map B-2), the map of Long Island and Connecticut Shore (Map B-3) and by.

contacting either LILCO's Environmental Engineering Department or Survey Division.

LOCATION TABLE S-1 SAMPLE SECTOR CODE LOCATION TYPE N 151 Beach east of intake, 0.3 mi. N IDM(*)

NNE 251 Well, on site, 0.1 mi. NNE PWA(*)

NE 351 Site Boundary. 0.1 mi. NE APT (*),AIO(*),IDM(*)

ENE 451 Site Boundary, 0.1 mi. ENE IDM(*)

E 552 Site Boundary, 0.1 mi E IDM(*)

ESE 652 Site Boundary 0.1 mi. ESE APT (*),AIO(*),IDM(*) ,

S 951 Service Road. 0.2 mi. S APT,AIO,IDM(*), RWA S 952 East Gate SNPS, 0.3 mi. S IDM(*)

W 1352 Well, on site, O.P mi. W PWA(*)

W 1353 Site Boundary, 0.2 mi. W IDM(*),GAX WNW 1452 St. Joseph's Villa, 0.4 mi. WNW IDM(*),GAX,NBG NW 1551 Beach west of intake, 0.3 mi. NW IDM(*)

NNW 1652 Site Boundary, 0.3 mi. NNW IDM(*)

NNE 2A2 West end of Creek Road 0.2 mi. NNE APT (*),AIO(*),IDM(*)

NNE 2A3 Residence. 0.3 mi, NNE APT AIO,lDM(*)

- NNE 2A4 Beach. 0.4 mi. NNE AQS(*)

NE 3A2 Riverhead Town Beach 0.7 mi. NE AQS ENE 4A3 Wading River, Eastern Marsh, 0.2 mi. ENE SWA,AQI,AQP,AQS ESE 6Al Sound Road, 0.7 mi, ESE IDM(*)

SE 7A2 North Country Road, 0.7 mi. SE APT,A!O,IDM(*)

l SSE 8A3 North Country Road. 0.6 mi. SSE APT.AIO,lDM(*)

l SSW 10A1 North Country Road. 0.3 mi SSW APT.AIO,IDM(*)

l SW 11A1 Site Boundary 0.3 mi. SW IDM(*)

WSW 12A1 Meteorological Tower, 0.9 mi. WSW APT , A I O, I DM( * ) , RWA l WNW 14A1 Brookhaven Town Beach, Q.8 mi . WNW AQS

! NNW 16Al Aquatic location, west jetty of intake AQI,AQP canal 0.4 mi. NNW ESE C 681 Remsen Road, Wading River, 1.6 mi. ESE PWA ESE 682 North Country Road,1.4 mi. ESE GMK i

SE 781 Overhill Road, Wading River,1.4 mi. SE APT (*)AIO(*),IDM(*)

l E 783 Farm stand, 1.7 mi, E FPV SSE 881 Farm stand 1.2 mi. SSE FPV(*),FPF l 0 1381 Briarcliff Road,1.9 mi. W GMK NNW 16B1 Long Island Sound,1.3 mi. NNW AQS.SWA

( 43

TABLE B-1 LOCATION LOCATION SAMPLE SECTOR CODE TYPE NE 3C1 Outfall area, aquatic location SWA(*),AQF(*),AQ1(*)

B-5, 2.9 mi. NE AQP,AQS E SC2 Farm 2.8 mi. E FPyFPF(*)

g WSW 12C1 Local Store, McCarricks Dairy, 2.7 mi WSW MLK

  • WNW 14C1 Outfall area, aquatic location SWA(*),AQF(*),AQl(*)

B-4, 2.1 mi. WNW AQP,AQS E 501 Wildwood St ate Park , 3.4 mi . E IDM(*)

E 503 Wildwod State Park, 3.1 mi E APT,IDM(*),A10 WSW 1201 North Shore Beach Substation, APT,A10,IDM(*)

3.7 mi. WSW ESE 6El LILCO R0W, 4.8 mi. ESE IDM(*)

SE 7El Calverton, 4.9 mi. SE IDM(*)

SSE 8E1 Calverton, 4.4 mi. SSE IDM(*)

S 9El Brookhaven National Laboratory IDM(*)

5.0 mi. S SSW 10E1 Ridge Substation IDM(*)

SW 11El LILCOR0W,4.7mI.4.0mi.SSW SW IDM(*)

W 13E1 Longview Ave. and Rocky Point Landing IDM(*)

Rd., 4.5 mi W E C SF2 Farm, 6.1 mi. E FPV E C 5F3 Fam, 7.8 mi . E APT,AIO,lDM(*)

SSE 8F2 Goat Farm, Wading River Rd., 9.5 mi. SSE GMK SSW C 10F1 Goat Farm, 9.2 mi. SSW GMK(*)

W C 13F1 Background aquatic location 9.4 mi. W AQl,AQP,5WA,AQS ESE C 6G1 Hampton Bays Substation, 19.0 mi. ESE IDM(*)

SSE C 8G1 Wading River Rd., 10.1 mi. SSE APT, AIO, l DM( * )

SSE C 8G2 Dairy Farm, Center Moriches,10.8 mi. SSE MLK SW C 11G1 MacArthur Substation, 16.6 mi. SW APT (*),A!O(*),IDM(*)

WSW C 12G1 Central Islip Substation, 19.9 mi. WSW IDM(*)

WSW C 12G2 Flowerfield Substation, 15.4 mi. WSW APT,AIO,IDM(*)

, W C 13G2 Background aquatic location, 13.2 mi. W SWA(*),AQP,AQS I

AQF(*),AQI(*)

i WSW C 12H1 Farm, 25.8 mi. WSW FPV(*),FPF(*)

WSW C 12H2 Farm, 32.1 mi. WSW FPV, FPF C Denotes Control Location

  • Denotes SNPS Technical Specification sampling locations and sample type.
    • Bottled Milk l

44 l __. .. . - ... . - -. - _ .

REMP LOCATIONS REQUIRED BY SNPS TECHNICAL SPECIFICATIONS TABLE B-2 Airborne Particulate and Airborne Iodine Monitoring Stations Location Codes NUREG-0473 Shoreham REMP Location Description A1 652 Site Boundary, 0.1 mi. ESE A2 2A2 West end of Creek Road. 0.2 mi. NNE A3 351 Site Boundary. 0.1 mi., NE A4 781 Overhill Road,1.4 mi. SE A5 11G1 MacArthur Substation, 16.6 mi. SW TAB 6E B-3 WATERBORNE MONITORING STATIONS Location Codes NUREG-0473 Shoreham REMP Location Description WA1 13G2 Surf ace, background trea,13.2 mi. W WA2 14C1 Surface, outfall area, 2.1 mi. WNW WA3 3C1 Surface, outfall area, 2.9 mi. NE Wbl 251 Potable Water, well on site, 0.1 mi. NNE Wb2 1352 Potable Water, well on site, 0.2 mi. W Wdi 2A4 Sediment, Beach 0.4 mi NNE

~

TABLE B-4 INGESTION MONITORING STATIONS Location Codes NUREG-0473 Shoreham REMP Location Description l

Ia1 681 Goat Farm, 1.6 mi. ESE la2 10F1 Goat Farm, 9.2 mi. SSW Ib1 3C1 Fish and Invertebrates, outfall area, 2.9 mi. NE Ib2 14C1 Fish and Invertebrates, outfall l area, 2.1 mi. WNW l Ib3 13G2 Fish and Invertebrates, background, 13.2 mi. W Ic1 881 Local Farm, 1.2 mi. SSE Ic2 SC2 Local Farm, 2.8 mi. E Ic3 12H1 Background Farm. 25.8 mi. WSW

REMP LOCATIONS REQUIRED BY SNPS TECHNICAL SPECIFICATIONS TABLE B-5 Direct Radiation Monitoring Stations Location Codes NUREG-0473 Shorel.am REMP -

Location Description DR1 151 Beach east of intake 0.3 mi. N DR2 2A2 West end of Creek Road. 0.2 mi. NNE DR3 351 Site Boundary 0.1 mi. NE DR4 451 Site Boundary. 0.1 mi. ENE DRS 552 Site Boundary. 0.1 mi. E DR6 652 Site Boundary, 0.1 mi. ESE DR7 7A2 North Country Road 0.7 mi. SE DR8 8A2 North Country Road. 0.6 mi. SSE DR9 951 Service Road SNPS, 0.2 mi. 5 DR10 10A1 North Cou.1try Road, 0.3 mi. SSW DR11 11A1 Site Boundary, 0.3 mi. SW DR12 12A1 Meteorological Tower, 0.9 mi. WSW DR13 1353 Site Boundary, 0.2 mi. W DR14 1452 St. Joseph's Villa, 0.4 mi. WNW DR15 1551 Beach west of intake, 0.3 mi. NW DR16 1652 Site Boundary, 0.3 mi. NNW DR17 503 Wildwood State Park, 3.1 mi. E OR18 6El LILCO RDW, 4.8 mi ESE DR19 7El Calverton, 4.9 mi. SE DR20 8E1 Calverton, 4.4 mi. SSE DR21 9El Brookhaven National Laboratory, 5.0 mi. 5

~

DR22 10E1 Ridge Substation, 4.0 mi. SSW DR23 11El LILCO R0W, 4.7 mi. SW DR24 1201 North Shore Beach Substation, 3.7 mi. WSW DR25 13E1 Longview Ave, and Rocky Point Landing Rd. 4.5 mi. W DR26 501 Wildwood State Park, 3.4 mi. E DR27 SF3 Dairy Farm, 7.8 mi. E DR28 781 Overhill Road,1.4 mi. SE DR29 12G2 Flowerfield Substation.

15.4 mi. WSW DR30 12G1 Central Islip Substation, 19.9 mi. WSW l

DR31 11G1 MacArthur Substation, 16.6 mi. SW DR32 8G1 Wading River Road,10.1 mi. SSE DR33 6G1 Hampton Bays Substation, 19.0 mi. ESE

( 6Al Sound Road. 0.7 mi. ESE DR34 DR35 2A3 Nearest Residence 0.3 mi. NNE DR36 952 East Gate SNPS, 0.3 mi. S l

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APPENDIX C DATA TABLES 50

= a TAgtE C-1 CONCENTRATIONS OF TRITIUM, STRONiluM-89* and -90 AND GAMMA EMITTER 5**

IN SUNFACE WATER SAMPLES Results in Units of pCl/l i 2 sigma LOCATION CODE COLLECTION DAT[ H-3 I-131*** Sr-89* Sr-90 K-40 Cs-137 54-5WA-4A3 05/06/87 170 t 100 <0.2 <2 <1 <80 (6 10/01/87 430 t 1 00 <0.2 <4 <1 54.7 1 29.7 (4 SN-5WA-3Cl 05/18/87 (100 <0.4 <2 <0.9 197 2 39 (4 11/02/87 <100 <0.4 <2 <0.3 1290 t 130 <3 aa

"" 253 e 49 <5 5N-5WA-13G2 (cI) 05/29/87 <200 <0.5 <2 <0.8 10/30/87 290 t 110 <0.3 <4 <1 270 t 43 <4 t

l l

l 54-5WA-13F1 (cl) 05/21/87 <100 <0.5 <4 <1 208 1 47 <3 l 10/29/87 220 t 90 (0.3 <3 <1 233 1 52 <4 l

SN-5WA-14Cl 05/18/87 <100 (0.5 <3 El 275 a 42 <4 11/02/87 230 t 100 <0.4 <1 <0.3 230 2 37 <3 SN-5WA-1681 05/18/87 (200 <0.4 <3 <1 136 t 66 <7 11/02/87 (200 <0.4 <2 <0.3 251 1 43 <3

  • Sr-89 results are corrected for decay to the sample stop date.
    • All other gamma emitters not listed were <LLD; typical LLO's are given in Tables C-!9 and C-20.
      • l-13] results determined by radiochemical analysis.

(cI) Denotes Control Location l

TABLE C-2 CONCENTRAil045 0F STROMilDM-89* AND -90 AND GAMMA EMITTER 5** IN FISH SAMPLES Results in Units of pCl/kg (WE T) t 2 sigma LOCATION COLLECTION DESCRIPTION CODE Sr-89 $r-90 E-40 Cs-137 DATE Th-228

$N-AQF-3CI 05/27/87 Winter Flounder <2 <2 4030 t 400 15.6 1 5.4 05/27/87 Sea Robin <1 (10 05/27/87 Little Skate

<1 3900 t 390 ~ (9 <10

<1 <1 2090 2 210 05/27/87 Windowpane <l <0.9 12.3 2 5.9 <10 10/20/87 Little Skate 3320 t 330 <9 (20

<3 <1 2040 1 200 10/20/87 Sea Robin (4 11.0 t 5.2 <10 10/20/87 Svaner Flounder (2

<3 3840 t 380 <10 (30

<0.8 4110 t 410 10/20/87 Windompane (4 (8 (10 10/20/.87 Winter Flounder

<3 3720 1 370 (10 <20 (5 <2 4120 1 410 17.9 1 7.5 <20 g 52-AQF-13G2 (c t ) 05/29/87 Sea Robin <2 <1 4150 t 410 05/29/87 <8 <10 Winttr Flounder <I <0.6 4050 2 400 05/29/87 Windowpane (2 (9 (10 05/29/87 Little Skate

<1 3300 a 330 8.88 1 5.04 <10

<4 <3 2410 a 240 10/30/87 Little Skate <5 <9

<2 <0.9 2400 2 240 10/30/87 Sea Rnbin <3 10.4 1 4.4 <10 10/30/87 Windowpane

<1 3460 t 350 <9 (10 (2 <0.9 4290 t 430 10/30/87 Winter Flounder <9 <10 (2 (0.6 2820 t 280 (7 (10 53-AQF-14Cl 05/28/87 Sea Robin <l 05/28/87 Little Skate

<0.8 3820 1 380 (10 (10 (2 <1 2340 t 230 05/28/87 <9 (20 Winter Flounder <l <l 4070 1 410 05/28/87 Windowpane <l <0.7 3370 1 340 (9 (10 10/21/87 Fluke <8 (10 10/21/87 (2 <0.7 3750 t 380 (7 <10 Little Skate <3 <2 2240 t 220 10/21/87 Sea Robin <3 <l (8 <10 10/21/87 Windowpane 4020 t 400 <10 (20

<2 <1 3710 t 370 10/21/87 Winter Fjounder (4 25.8 2 4.9 <8

<2 4480 2 450 (10 (20

    • Sr-89 results are corrected for decay to the sample stop date.

All other gamma emit ters not ilsted were <LLO; typical LLDs are given in Tables C-19 and C-20.

(ct) Denotes Control Location

TA8tt C-3 CONCENTRATiens OF Simonfilm-89* Ano -90 Ano GAfeen EMilTER5** IN InutRIESRATE SerLES Results in Units of pCl/kg (WET) t 2 slyne COLLECYl0N DATE DESCalriloM Sr-89 Sr-90 K-40 Cs-137 Th-228 Se-/

LOCATION C00E Oysters <5 C 1870 t 190 <5 * <8 (40 58-AQl-4A3 05/06/87 CO <10 10/01/87 Oysters <3 <2 1410 t 140 <8 Sof t 5ftell Class O G 2170 1 220 <10 101 1 15 (100 10/01/87

<2 1990 t 110 <4 0 <40 ui Sa-AQl-16Al 05/18/87 Slue faussels <5 '

fesssels C (1 1780 t ISO 34.8 1 9.1 CO <90 w 10/13/87 CO <80 l 05/27/87 Lobster <2 <2 2430 t 240 (8 55-AQl-X1 2650 1 270 <10 C0 <100 I 10/20/87 Lobster (2 <2 10/20/87 $guld C C 3090 2 310 36.2 1 7.5 (10 <10 l o o 2560 2 260 <5 <s <40 10/20/87 isielk ,

05/28/87 Lobster G C 2610 2 260 (9 C0 <80 Su-AQl-14Cl <10 (20 <90 06/23/87 isselk O <2 2410 2 240 Lobster C <1 2850 t 290 (10 <20 <100 10/21/87 (10 <10 10/21/87 5gul4 C <1 3060 1 310 <1 isselk <2 (0.4 2710 t 270 (6 (10 (50 10/29/S7 l

05/21/87 Mussels <5 <1 1750 t 180 <5 <9 73.9 1 36.8 Sa-A41-13F1 (ci) <4 2130 2 210 <5 <9 <50 10/29/87 flussels <1 O

TA8t[ C-4 COnCENTRAilows CT STRONiluM-89* Ano -90 Ano GAsset (MITIER 5** 13 AQUATIC PLAmi 5AMPtts Results in Units of pCl/kg (DAT) t 2 signia

! LOCATION COLLECTION Sr-89 Sr-90 Se-1 E-40 l 1-131 Cs-131 Ra-226 Th-228 C00t DATE 5N-AQP-4A3 05/06/87 <30 <10 3760 2 380 17900 a 1800 00 <30 (500 1190 t 120 Ulva hus l

Su-AQP-4A3 10/01/87 (20 <10 2920 t 290 16900 t 1700 (50 85.5 t 24.5 1460 t 390 1090 1 110 Ulva Codium 54-AQP-13FI (c1) 05/21/87 <9 8.3 a 3.8 529 t 239 -

30200 t 3000 (to <30 <500 117 1 40 Ascophyllum, Sp.

l SN-A0P-13FI (ct) 10/29/87 CO (6 523 t 179 20600 1 2I00 <60 00 711 2 363 220 t 22 Fucus Into . ,,ta

, SN-AQP-13G2 (cI) 05/18/87 (9 18 t 4 <400 23900 t 2400 <100 <30 (100 (60 m Ulva A ThC .

i 54-AQP-13G2 (c1) 11/03/87 (20 (7 558 t 215 18000 t 1800 <90 <30 <400 130 t 36

! CodIum 54-AQP-16A1 05/18/87 <9 <5 <500 20300 2 2000 <100 <50 <900 <90 Chrondus Su-AQP-16Al 10/13/87 <10 <5 571 1 274 36900 t 3700 (300 <30 <100 111 2 48 Codlism Focus 06/10/87 (30 SN-AQP-14Cl <10 0 00 12000 t 1200 <60 <20 Ulva <300 158 t 28 To3 Time SM-AQP-14Cl 10/29/87 (20 <10 240 t 98 5??O t 520 <30 (10 <300 114 t 13 Ulva, Sp.

SM-AQP-3Cl 06/10/87 <30 <20 172 1 96 5470 2 550 <40 (10 (300 <30 Ulva Cod 6een SN-AQP-3Cl 10/29/87 <30 <6 <100 2930 3 290 <30 <10 <300 118 t 13 Codless

, Sr-89 results are corrected for decay to the sample stop date.

1 AII other gauna custtlers not IIsted escre <tLD; typical itDs are found in Tables C-19 and C-20.

(ct) Denotes Control Location a

~ , ,

t TA8tt C-5 CONCETPATIONS or STRONTItal-89* AND -90 ANO GAfetA (MITTE15M 13 5(DIME T SAfetti Results in Units of PCl/kg (DRT) t 2 sigma l

LOCATION C00E 5AmrtE Cott f CTION Sr-89 3r-90 E-40 Ra-226 Th-228 Cs-137 10 CATION DAT[

l SP-AQS-2A4 8each 06/01/87 C <1 1940 1 230 <300 5N-AQS-2A4 8each 11/04/87 121 2 17 CO (I <0.8 3800 t 380 (300 119 1 15 Co SM-AQS-3A2 8each 06/01/87 C (3 5N-AQS-3A2 Beach 2850 2 280 <300 (a) 109 e 13 C0 11/04/87 C (I 1490 t 160 0 00 100 1 17 (10 54 AQS-3Cl of fshore (b) 05/18/87 <5 C SN-AOS-3Cl 3620 2 360 <500 227 2 24 (30

, Offshore 11/02/87 <3 <2 4510 2 450 <300 330 a 33 21.7210.8 1

1

! $N-AQS-4A 3 tsading River 05/06/87 (4 0 4900 t 490 l SN-AQS-4A3 Idading River 1240 2 430 741 2 74 (30 10/01/87 <4 C 2650 1 270 <400 306 2 31

, 00

'm

  • 54-AQS-lyl (cI) 8each 05/21/87 <3 <3 4550 t 460 SN-AQS-ly l (cI) Beach <400 177 2 22 (30 10/29/87 <3 <1 4600 1 460 (400 221 2 30 C0 Su-AQS-13Q (ct) 8each 05/18/87 <4 C 4070 t 410 <300 SN-AQS-13G2 (ct) Offshore 05/29/87 (30 C0 C C 2000 t 290 (400 123 2 19 54-AQS-13G2 (cI) Offshore 10/30/87 <3 CO

<1 2130 1 210 <400 <40 00 54-AQS-13Q (ct) Beech 11/03/87 <3 C 1500 t 150 0 00 95.8 a 11.3 <10 SM-AQS-l4Al acach 06/01/87 C C i

54-AQS-14Al Beach 1770 t 180 4781 179 (c) 74.0 t 10.8 <10 11/04/87 <2 <0.9 1870 2 190 0 00 103 2 12 (10 54-AQS-14Cl Offshore 05/18/87 <2 <1 2340 1 230 (400 299 1 30 00 5N-AQS-14C l Offshore 11/02/87 C (1 1840 t 180 0 00 171 i 17 (10 54-AQS-1681 Offshore 05/18/87 C <2 1220 t 120 SM-AQS-1681 Offshore 0 00 1080 t 110 <50 11/02/87 <3 C 8310 t 830 839

  • 252 1910 t 100 (20 Average t 2 s .d . 3398 1 3783 852 2 762 300 2 624 21.7 t 10.8
  • a Sr-89 results are corrected for decay to the sample stop date.

All other gamma emitters were (LLD; typical LLDs are found in Tables C-19 and C-20.

(ct) Denotes Control location (a) Ra-228 = 137 2 59 (b) Se-T = 366 a 189 (c) Ra-228 - 70.2 2 45.9

TABLE C-6 CONCENTRATIONS OF GROSS SETA EMITTERS IN wtEKLY AIRBORNE PARTICULATES Results in Units of 10-3 pCl/m3 1 2 sigma .

LOCATION CODES COLLECTION DATES $4-APT-2A2 Su-APT-2A3 54-APT-351 SM-APT-503 Su-APT-5F3 Su-APT-652 Su-APT-7A2 Su-APT-701

, _ (ct)

JANUARY 87 12/30/86-01/06/87 15 2 3 13 a 3 <4 (a) 15 t 3 14 1 3 13 t 5 15 t 3 15 t 4 01/06/87 01/13/87 15 t 3 17 2 3 15 1 3 14 2 3 18 1 3 15 1 4 1713 14 1 3 01/13/87-01/20/87 15 2 3 18 e 3 15 2 3 14 1 3 13 2 3 15 1 3 14 2 3 13 2 3 01/20/87-01/21/87 17 2 3 18 1 3 14 2 3 17 2 3 16 a 3 15 2 3 17 1 3 13 i 3 FEBRUARY C1/27/87-02/03/87 25 a 4 25 1 4 22 e 4 23 1 4 24 i 4 22 t 4 24 1 4 24 t 4 02/03/87-02/10/87 18 2 3 19 2 4 18 2 4 20 2 3 22 2 4 18 1 4 17 1 3 17 2 3 I

02/10/87-02/11/87 16 a 3 18 2 3 15 t 3 15 a 3 16 1 3 14 2 3 15 t 3 15 1 3

$ G2/17/87-02/24/87 16 2 3 16 1 3 5t 3 16 a 3 1723 17 2 4 18 1 3 ~16 1 3 NARCH C2/24/87-03/03/87 11 2 3 15 t 3 10 t 3 82 3 913 713 9t 3 63 3 03/03/E7-03/10/87 26 i 4 21 1 4 25 t 4 23 i 3 20 t 3 26 1 4 2514 26 1 4 03/10/87-03/17/87 19 a 3 18 a 3 19 2 3 21 1 3 22 1 3 18 a 3 20 t 3 20 1 3 03/17/87-03/24/87 82 3 11 2 3 81 3 9t 3 10 2 3 Si3 92 3 82 3 03/24/87-03/31/87 17 2 3 19 1 3 18 t 3 16 2 3 18 1 3 18 2 3 19 1 3 16 a 3 APRIL 03/31/87-04/07/87 10 2 3 10 t 3 11 2 3 11 2 3 14 1 3 11 2 3 12 1 3 91 3 2

04/07/87-04/14/87 <4 (b) 72 3 12 a 3 63 3 92 3 11 2 3 (4 (b) 11 2 3 04/14/87-04/21/87 5t 3 42 3 8t 3 42 3 8a3 61 3 71 3 422 04/21/87-04/28/87 10 2 3 92 3 10 t 3 8a3 72 3 92 3 91 3 9a3 I

2 (ct) Denotes Control Location (a) Sample light in deposition of particulate matter.

(b) Coaf irmed try a secord count.

)

TABLE C-6 (Coct.)

CONCENTRAil0NS OF GROSS BETA [MITTER5 IN WEEKLY AIRBORNC PARTICULATES Results in Units of 10-3 pCS/m3 2 2 sigma LOCAtl0N CODES COLLECil0N DATES SN-APT-2A2 Su-APT-2A3 5N-APT-351 SN-APT-5D3 SM-APT-5F3 SN-APT-652 SN APT-7A2 $N-APT-781 (ct)

"Al E4/28/87-05/05/87 16 2 3 15 1 3 14 1 3 13 1 3 15 t 3 to a 3 16 t 3 14 2 3 C5/05/87-05/12/87 17 a 3 18 a 3 17 a 3 17 1 3 7a3 17 t 3 16 1 3 20 1 3 C5/12/87-05/19/87 13 a 3 11 1 3 12 t 3 15 2 3 14 2 3 13 2 3 15 t 3 13 a 3 05/19/87-05/26/87 82 3 8t 3 (900 (a) 10 t 3 10 2 3 (900 (a) 11 2 3 9a3 05/26/87-06/02/87 23 t 4 22 2 4 (c) 23 1 4 21 2 4 (b) 28 1 5 1714 JUNE 06/02/87-06/09/87 15 a 3 15 t 3 b 15 t 3 16 1 3 lb 14 2 3 11 1 3 C 6/09/8 7-06/16 /8 7 18 i 3 20 2 3 cl 21 2 4 2424 Lb 20 1 3 19 a 3 on

'd 06/16/87-06/23/87 15 a 3 16 2 3 bl 16 2 3 15 t 3 I b 16 1 3 15 1 3 C6/23/87-06/30/87 14 a 3 14 2 3 15 2 3 11 2 3 12 1 3 16 2 4 12 e 3 11 1 3 JULY 06/30/87-07/07/87 19 i 4 18 2 4 15 2 3 15 a 3 16 1 4 <4000 (a) 14 1 3 18 2 4 07/07/87-07/14/87 21 a 4 24 t 4 24 1 4 18 1 4 30 1 4 (bl 23 1 4 19 1 4 C1/14/87-07/21/87 18 2 3 17 t 3 20 2 3 20 2 4 20 1 4 (bj 15 1 3 15 t 3 07/21/87-07/28/87 21 2 3 18 t 3 23 a 4 25 t 4 26 2 4 (bj 22 1 4 22 a 4 CUGUST 07/28/87-08/04/87 12 2 3 11 i 3 13 1 3 12 a 3 13 1 3 (bl 10 2 3 9t 3 08/04/87-08/11/87 16 t 3 13 1 3 81 3 14 1 3 16 2 3 (bh 12 2 3 17 a 3 C8/II/87-08/18/87 14 a3 13 i 3 12 2 3 15 1 3 15 2 3 Lbl 15 t 3 14 a 3 C8/18/87-08/25/87 14 2 3 11 2 3 14 2 3 15 1 3 11 2 3 Lbj 16 1 3 18 2 3 08/25/87-09/01/87 13 2 3 11 2 3 12 i 3 12 t 3 7a3 lb) 11 2 3 13 1 3 (c1) Denotes Centrol Location (a) Power outage; result in total PCI.

(b) Power outage; no semple collected.

(c) Sampler malfunction; no sample collected.

(d) Results are in total pCl.

TABLE C-6 (Cost.)

CONCENTRATIONS OF GROSS BETA EMITTERS IN WEEKLY AIRBORNE PARTICULATES Results in Units of 10-3 pCl/m3 1 2 sigma LOCATION CODES COLLECil0N DATES SN-APT-2A2 54-A P T -2A 3 SM-APT-351 5N-APT-5D3 j

SN- AP T-5F 3 54-APT-652 SM-APT-TA2 SN-APT-7BI (ct)

SEPTEM8ER C9/01/87-09/08/87 14 1 3 16 2 3 17 1 3 16 2 3 09/08/87-09/15/87 18 2 3 (al 14 2 3 19 2 4 09/15/87-09/22/87 12 1 3 14 1 3 13 1 3 12 t 3 14 1 3 (aj 11 2 3 15 t 3 16

  • 4 14 1 3 13 2 3 13 2 3 14 2 4 (a? 10 1 3 18 1 4 09/22/87-09/29/87 25 t 4 (b) 25 2 4 26 2 4 25 2 4 (a? 22 1 4 24 1 4 OCTOBER C9/29/8 7-10/06/8 7 15 t 3 11 2 5 (c) 15 a 3 18 2 3 17 2 3 10/06/87-10/13/87 15 2 3 13 i 3 (a) 1713 on 10/13/87-10/20/87 (b) 13 t 3 14 1 3 12 1 3 s a) 16 1 3 1323 27 2 4 (b) 26 2 3 28 2 4 29 2 4 La) 27 2 4 14 1 3 00 10/20/87-10/27/87 24 1 4 17 2 5 17 1 3 20 t 4 21 1 4 ta) 11 t 3 21 1 4 IG/27/87-II/03/87 21 2 3 18 1 3 19 1 3 19 2 3 23 1 3 La) 12 1 3 21 1 3 l

NOVEnBER 11/03/87-11/10/87 28 1 4 27 2 4 22 1 3 25 t 4 29 2 4 al 22 2 3 11/10/87-11/17/87 18 2 3 19 i 3 18 i 3 20 1 3 18 2 3 a? 92 3 13 1 3 11/17/87-11/24/87 13 1 3 14 2 3 92 2 15 t 3 17 1 3 14 2 3 a? 13 1 3 91 3 11/24/87-12/01/87 17 i 3 17 2 3 17 2 3 20 t 3 17 2 3 (a) 21 1 4 16 1 3 DECEMBER 12/01/87-12/08/87 15 2 3 11 2 3* 91 3 12 1 3 13 t 3 (a) 10 1 3 12/08/87-12/15/87 10 t 3 19 t 3 19 i 4 18 2 3 24 t 5 (b) 19 2 4 (a) 27 i 5 (b) 18 e 4 12/15/87-12/22/87 18 i 3 19 2 3 15 1 3 16 t 3 15 1 3 (a 15 9 3 12/22/87-12/29/87 30 t 4 24 2 3 26 2 4 30 t 4 27 2 4 (a)) 21 1 3 15 1 3 25 1 4 cuerage 17 t to 16 i 9 16 a 10 17 t 11 1 2 s .d .

17 i 12 14 t 10 16 1 10 15 t 10 (cI) Denotes Contro s Locat ion (a) Power outage; no sample Collected.

(b) Pump malfwn(tlon; low volume.

(c) Pump ran 3.5 days.

v - , y

TIBL E C-6 (Cont.)

CONCENT2ATIONS OF GROSS BETA EMITTERS IN WEEKLY AIRBORNE PARTICULAT[5 Results in Units of 10-3 pC1/m3 1 2 sigma l

COLLECTION DATE5 S u-AP T-8A 3 LOCATION CODES SM-APT-8GI SN-APT-951 54-APT-10Al WEEELF (ct)

SM-APT-IIGl $N-APT-12Al SN-APT-1201 SW-APT-12G2 (ct) (c1)

AVERAGE e 2 s.d.

JANUARY 12/30/86-01/06/87 15 t 3 16 i 4 13 2 3 EI/06/87-01/13/87 17 1 3 16 1 3 15 t 3 16 2 3 16 1 3 14 1 3 17 a 3 16 2 3 1614 15 1 2 01/13/87-01/20/87 14 1 3 16 1 3 18 t 3 15 t 3 15 t 3 15 t 3 16 1 3 01/20/87-01/21/87 13 i 3 16 2 3 13 a 3 16 1 3 17 i 3 92 3 17 a 3 18 a 3 11 1 3 15 i 3 15 2 3 15 t 3 15 2 3 10 1 3 21 1 3 15 t 6

[E8RUAR1 01/27/87-02/03/87 24 2 4 22 t 4 20 t 4 02/03/87-02/10/87 18 t 3 <4 ( a) 15 a 3 27 i 4 21 1 4 26 1 4 22 2 4 20 t 4 C2/10/87-02/17/87 16 1 3 19 2 4 10 t 3 18 t 3 17 1 3 2314 11 2 3 14 a 3 18 1 3 21 2 4 18 2 6 (n

to C2/17/87-02/24/87 16 1 3 7i3 14 1 3 91 3 16 1 3 12 t 3 12 e 3 15 t 5 14 i 3 16 t 3 13 1 3 MARCH 16 2 3 14 1 3 14 2 7 02/24/87-03/03/87 7i3 71 3 72 3 03/03/87-03/10/87 2624 26 1 4 25 1 4 10 t 3 11 2 3 623 81 3 713 03/10/87-03/17/87 22 1 3 23 1 4 22 1 4 23 e 4 14 2 3 915 23 1 4 22 2 3 20 t 3 2214 23 2 6 03/17/87-03/24/87 81 3 72 3 92 3 20 t 3 24 2 4 17 2 3 20 t 4 03/24/87-03/31/87 17 2 3 71 3 62 3 - 10 2 3 82 3 20 2 4 21 1 3 18 a 3 21 2 3 18

  • 3 20 t 3 71 3 82 3 APalt 15 t 3 17 1 3 18 1 3 03/31/87-04/07/87 11 t 3 13 1 3 11 1 3 10 1 3 C4/07/87-04/14/87 11 t 3 12 1 3 10 t 3 12 2 3 10 t 3 11 2 3 10 t 3 11 2 3 11 2 2 04/14/87-04/21/87 14 1 3 7i3 10 t 3 11 2 3 72 3 61 3 72 3 81 3 10 1 4 C4/21/87-04/28/87 82 3 10 t 3 91 3 81 3 4 2 3 72 3 6a3 (4 (b) 62 3 62 3 10 1 3 <3 10 m 3 912 (ct) Denotes Control Location (a) Sample light in deposition of particsaate matter.

(b) Confirmed by a second count.

TCBLE C-6 (Cost.)

EONCENTRATIONS OF GROSS BETA EMITIERS IN WEEKLY AIRBORNE PARTICULATES Results in Units of 10-3 pCl/m3 1 2 sl 9ea WLLKLY LULATIUM LU DL ) AVERAGE "

SN-APT-8GI Su-APT-951 SM-APT-10A1 SM-APT-IIGI SN-APT-12AI SM-APT-1201 (ct) $N-APT-12G2 2 s.d. {

COLLECTION CATES $N-APT-8A3 (ct) (ct) I l

Ea1 13 2 3 14 1 3 14 1 3 )

15 t 3 15 t 3 16 1 3 1313 16 1 6 13 2 3 12 a 3 1713 IT t 3 17 2 3 1313 i

C4/28/87-05/05/87 13 t 3 13 1 3 16 2 3 18 1 3 13 2 3 10 2 3 15 2 3 l' C5/05/87-05/12/87 17 a 3 13 2 3 13 2 3 13 a 3 10 2 3 11 2 3 91 3 13 1 3 13 2 3 81 3 82 3 22 1 10 05/12/87-05/19/87 8e3 11 2 3 81 3 2324 2724 22 a 4 05/19/87-05/26/87 81 3 20 1 4 24 14 72 3 25 a 4 25 t 4 05/26/87-06/02/87 14 1 3 g JUNE 14 1 3 14 2 3 16 t 3 15 t 3 13 2 3 15 t 3 2023 20 t 4 06/02/87-06/09/87 14 a 3 15 i 3 19 1 3 20 t 3 21 2 3 20 t 3 14 2 3 15 t 2 16 2 3 21 2 4 17 2 3 15 2 3 06/09/87-06/16/87 19 t 3 15 t 3 16 2 3 15 t 3 11 2 3 1313 13 1 4 l 06/16/87-06/23/87 12 1 3 14 i 3 13 t 3 12 2 3 15 i 1 12 1 3 82 3 14 t 3 06/23/87-06/30/87 l

JULY 16 2 4 16 1 3 16 1 3 17 1 4 18 1 3 17 1 4 25 2 4 23 1 6 14 1 3 17 1 4 16 2 4 24 a 4 19 i 4 06/30/87-07/07/87 23 1 4 26 2 4 25 t 4 20 2 4 20 1 3 17 2 3 19 a 4 07/07/87-CF/14/87 22 2 4 20 t 4 11 2 3 19 t 3 19 2 3 23 1 4 2113 22 1 4 19 1 3 22 2 4 21 2 3 24 t 4 07/14/87-07/21/87 22 1 4 2r i 3 2314 22 t 4 07/21/87-07/28/87 AUGUST 13 2 3 11 2 3 12 1 5 14 2 3 11 2 3 15 t 3 14 2 5 13 1 3 7i3 1623 15 t 3 9A 3 15 2 3 15 2 3 14 a 6 07/28/87-08/04/87 17 a 3 15 t 3 15 t 3 14 2 3 18 2 3 16 1 3 08/04/87-08/11/87 I4 t 3 13 2 3 15 2 3 15 1 3 15 t 3 16 2 5 13 2 3 52 2 17 2 3 11 e 3 15

  • 3 12 1 3 08/11/87-08/18/87 15 2 3 19 2 3 19 1 3 11 2 3 12 2 3 14 2 3 08/18/87-08/25/87 17 t 3 12 a 3 13 2 3 13 2 3 12 i 3 13 1 3 08/25/87-09/01/87 (ct) Denotes Control Location C

1ABLE C-6 (Cont.)

CONCENTRATIONS OF GROS 5 BETA EMITTERS IN WEEKLY AIR 80RME PARTICUL ATES Results in Units of 10-3 pCl/ml i 2 sigma LOCATION CODES WEEKLY l COLLECTION DATES $N-API-8A3 $N-APT-8G1 5N-APT-951 Su-APT-lCA1 Su-APT-IIG1 Su-APT-12Al SN-APT-1201 Su-APT-12G2 AVERAGE l (cI) (ct) (ct) t 2 s.d.

1 SEPTEm8ER C9/01/87-09/08/87 16 2 3 16 1 3 16 1 3 16 t 3 14 2 3 18 a 3 18 a 3 17 a 3 16 1 3 C9/08/87-09/15/87 11 2 3 II 1 3 12 i 3 14 1 3 15 t 3 10 t 3 12 1 3 14 1 3 13 1 3 09/15/87-09/22/87 15 1 4 14 24 19 2 4 13 2 3 14 t 3 12 e 3 16 a 4 11 t 3 14 a 5 C9/22/87-09/29/87 21 1 3 21 2 3 25 t 4 23 1 4 22 i 3 24 1 4 26 2 4 2414 24 1 3

, OCTOBER w

C9/29/87-10/06/87 14 2 3 17 a 3 14 i 3 16 t 3 12 2 3 17 1 3 15 t 3 16 1 3 15 t 4 10/06/87-10/13/87 14 2 3 15 1 3 14 1 3 13 1 3 17 2 3 13 1 3 17 2 4 1513 14 1 3 10/13/87-10/20/87 30 t 4 27 t 4 32 2 4 29 1 4 27 1 4 30 t 4 30 1 4 2724 27 a 8 10/20/87-10/21/87 2214 23 2 4 22 1 4 23 1 4 24 i 4 24 1 4 26 2 4 20 1 3 21 e 7 10/21/87-11/03/87 19 1 3 14 2 3 21 1 3 20 t 3 21 2 3 21 2 3 20 2 3 22 1 3 19 2 6 NOVEMBER 11/03/87-11/10'87 29 2 4 15 t 3 27 2 4 30 t 4 2824 2824 32 i 4 29 i 4 26 1 11 11/10/87-11/11/87 17 2 3 9t 3 19 a 3 18 2 3 22 2 3 20 t 3 20 1 3 18 2 3 17 a 9 II/17/87-11/2G/87 16 1 3 10 2 3 15 t 3 17 t 3 14 1 3 15 t 3 16 1 3 13 a 3 14 15 11/24/87-12/01/87 22 1 3 15 2 3 19 2 3 21 2 3 20 t 3 22 2 3 20 2 3 18 2 3 19 2 4 9ECEMBER 12/01/87-12/08/87 12 1 3 91 3 11 t 3 10 1 3 9t 3 8t 3 11 t 3 12 1 3 11 2 4 12/08/87-12/15/87 18 t 3 18 2 3 15 t 3 16 2 3 19 2 3 18 t 3 20 t 4 20 a 3 19 a 6 12/15/87-12/22/87 17 1 3 16 2 3 18 2 3 16 1 3 16 1 3 15 2 3 19 2 3 16 2 3 16 a 3 12/22/87-12/29/87 26 1 4 24 1 3 21 2 3 24 2 4 26 ? 4 26 2 4 28 t 4 26 2 4 26 1 5 Averare 16 t il 15 t 11 16 2 11 17 2 11 16 i 11 17 t 11 17 1 12 17 1 10 16 2 2 t 2 s.J.

(ct) Denotes Control Location

l I .- i taste C-7 .

I l CONCENTRAil0NS OF GA8M94 EnliitR5* lu QUARTERLY COMPOSITE OF AIRBORNE PARTICUL ATE SA99PLES Results is Units of 10-3 pCl/m3 1 2 sigma FOURTH QUARTER AVERAGE FIR $T QUARTER SECONO QUARTER THIRO QUARTER LOCATION NUCLIDES 09/29/87-12/29/97 t 2.s.d.

CODES 12/30/86-03/31/87 03/31/87-06/30/87 06/30/87-09/29/87 62.7 e 1.8 88.3 e 44.5 5N-APT-2A2 se-7 86.8 2 8.7 117 e 12 86.8 a 8.7 (20 -

<6 <1 <1 K-40 (0.4 <0.4 <0.7 -

Cs-134 (0.4

<0.4 <0.7 -

Cs-137 <0.4 <0.3 73.9 i 9.0 92.2140.0 5N-APT-2A3 Be-7 103 1 11 115 t 12 77.0 e 7.7 (20 27.5 1 7.0 (8 <8 K-40 27.5 1 7.0 (0.9 -

$ Cs-134 (0.8 <0.4 <0.5 (0.4 (0.9 - -

Cs-137 (0.8 <0.4 91.4 t 10.6 a5.7 1 8.4 84.8 1 60.5 Su-APT-351 Be-7 82.9 2 11.8 119 2 17 15.9 1 7.1 K-40 (10 (30 15.9 1 7.1 (20 (0.8 <0.9 Cs-134 <0.7 (I

<0.8 -

<0.9 <2 <0.9 Cs-137 122 a 12 94.2 t 9.5 61.6 2 6.6 91.6 2 49.5 SN-APT-5D3 Be-7 88.7 a 13.4 <10 (9 -

K-40 (20 <10 -

<0.7 <0.6 (0.5 Cs-134 <1 (0.6 -

<0.9 <0.9 <0.9 Cs-137

  • All other gamma emitters not listed were <tLD; typical LLDs are found in Tabies C-19 and C-20.

O

i l

TASLt C-7 (Cont.)

C0ectnTRAT1045 0F GasweA (MITTER5* IN QUARTERLY C0f0F05tTE OF AIRBORNE PARTICULATE SAf0PLES Results in Units of 10*3 pCl/e3 e 2 sigma LOCATION NUCL I DE S FIRST QUARTER SECOND QUARTER CODES THIRO QUARTER FOURTH QUARTER AVERAGC 12/30/86-03/31/87 03/31/87-06/30/87 06/30/87-09/29/87 09/29/87-12/29/87 1 2.5.4.

54- AP T-5F 3 Se-1 90.7 t 9.1 110 t 11 91.5 t 9.2 (c t) R-40 (7 66.2 a 6.8 89.6 1 35.9

<8 <10 <9 Cs-134 <0.4 (0.6 <0.4 Cs-137 <0.4 -

(0.4 <0.6 <0.5 <0.5 -

SM-APT-652 Se-7 81.6 2 8.2 106 e 14 h K-40 Cs-134 (7 <40 (a) (a) 93.8 2 34.5

<0.4 <1 Cs-137 <0.5 <1 SN-APT-FA2 8e-7 15.1 1 11.3 79.8 t 8.0 K-40 (10 (20 90.7 i 9.1 52.5 t 7.2 74.5 1 32.1 25.0 1 7.7 (10 25.0 1 7.7 Cs-134 (0.6 <0.6 (0.8 (0.7 -

Cs-137 <0.9 <0.6 <0.8 <0.6 -

54-APT-781 Se-7 87.2 i 8.7 128 e 13 62.5 t 6.3 E-40 (8 52.1 2 5.8 82.5 i 67.5 9.27 2 3.86 15.7 1 6.4 (20 12.5 1 9.1 Cs-134 (0.5 (0.5 <0.6 Cs-137 <0.6 <0.6 -

<0.6 <0.7 <0.6 -

All other gamma celtters not listed were (LLO; typical LL0s are found in Tables C-19 and C-20.

(ct) Denotes Control Location (a) Sample not collected.

l l

l

TABLE C-7 (Cont.)

CONCENTRATIONS OF GAMMA EMITTER $* IN QUARTERLV COMP 051TE OF AIRBORNE PARTICULATE SAMPLES Results in Units of 10-3 pCl/m3 1 2 sigma LOCAfl0N NUCLIDES FIRST QUARTER SECOND QUARTER THIRD QUARTER FOURTM QUARTER AVERAGE CODES 12/30/86-03/31/87 03/31/87-06/30/87 06/30/87-09/29/87 09/29/87-12/29/87 1 2.s.d.

50-APT-8A3 Se-7 99.1 1 10.1 100 t 10 95.9 t 9.6 57.0 t 6.9 88.0 1 41.5 K-40 (20 <8 (10 (8 -

Cs-134 <0.7 <0.5 <0.5 <0.3 -

Cs-137 <0.7 <0.4 <0.5 <0.4 -

Su-APT-BG1 Be-7 67.2 1 7.0 81.5 i 8.2 61.8 t 6.2 52.0 t 9.5 65.6 1 24.6 (ct) E-40 (8 <1 (9 (20 -

Cs-134 <0.4 <0.4 <0.4 <0.8 -

T Cs-137 <0.5 (0.4 <0.4 <0.7 -

$N-APT-951 Se-7 91.4 i 13.0 107 i 11 81.0 t 8.1 69.2 2 6.9 87.2 1 32.1 K-40 (20 <6 <F (8 -

CS-134 <0.9 <0.4 <0.4 <0.4 -

Cs-137 <0.8 (0.4 <0.4 <0.5 -

Su-APT-10Al Be-7 63.1 1 7.9 102 e 10 17.4 1 7.7 49.3 2 8.9 73.1 2 44.8 K-40 (20 (9 <? (20 -

Cs-134 <0.6 <0.5 <0.4 <0.8 -

Cs-137 <0.6 <0.5 <0.4 <0.7 -

All other genea celtters not listed were <LLD; typical LLDs are found In Tables C-19 and C-20.

(ct) Denotes Control Location l

l l

l l

c

T ABL E C-7 (Cont. )

CONC [NTRATIONS OF GAMMA (MITTER5* 14 QUARTERLY COMPOSITE OF AIRBORNE PARTICULATE SAMPLES Results in Units of 10-3 pCl/m3 1 2 sigma (0 CATION NUCL I DE S FIRST QUARTER SECOND QUARTER THIRD QUARTER FOURTM QUARTER AVERAGE CODE 5 12/30/86-03/31/87 03/31/87-06/30/87 06/30/87-09/29/87 09/29/87-12/29/87 a 2.s.d.

5N-APT-IlGI Se-1 71.4 e 8.9 94.8 i 1 0 87.3 i 8.7 58.6 i 6.4 (ct) K-40 78.0 t 32.4 8.89 2 4.20 (30 <8 <8 8.89 2 4.20 Cs-134 <0.5 (I <0.3 <0.4 -

Cs-137 (0.5 <0.9 <0.8 <0.4 -

SN-APT-12AI Se-7 95.5 e 10.1 126 t 13 93.9 e 14.4 63.9 i 6.4 E-40 94.8 a 50.7 (20 (20 (20 <0 -

Cs-134 (0.7 (0.8 (0.7 <0.4 -

cn Cs-137 <0.7 <0.8 vs <0.8 (0.4 -

SN-APT-12DI Be-7 65.1 2 7.8 105 a 11 90.3 2 10.4 59.5 t 5.9 80.0 2 42.8 K-40 <9 (9 (10 (9 -

Cs-134 <0.5 <0.5 <0.7 (0.4 -

Cs-131 <0.4 <0.5 (0.9 <0.4 -

SN-APT-12G2 Be-7 89.9 t 10.0 102 a 10 86.6 i 9.0 50.9 1 8.3 E-40 82.4 i 44.0 (ct) <20 5.11 2 2.85 (10 <30 5.11 a 2.85 Cs-134 (0.7 <0.4 <0.5 <0.9 -

Cs-127 (0.7 (0.4 (0.6 (0.8 -

All other gemea emitters not listed were (LLD; typical LLDs are found in Tables C-19 and C-20.

(ct) Denotes Control Location e

TC8Lf C-8 CONCENTRAT1045 0F STR(,eTIUM-89* Am0 -90 In QUARTERLY C08tP051TE5 0F AIR 80RNE PARTICULATE SAMPLES Results in Units of 10-4 pCl/m3 2 2 sl 9ea FIRST QUARTER SECOct QUARTER THIRO-0UARTER F09ETH QUARTER LOCATl04 12/30/86-03/31/87 03/31/87-06/30/87 06/30/87-09/29/87 09/29/87-12/29/87 CODES Sr-89 Sr-90 $r-89 Sr-90 Sr-89 Sr-90 5r-89 sr-90 l 55-APT-2A2 <5 <1 <4 <0.8 <5 <l (2 <0.9 54-APT-2A3 (4 (0.9 (4 <0.8 <5 <1 <4 <1 Su-APT-351 <3 <1 <9 <1 <3 <0.9 <2 <0.9 58-APT-503 (3

, <0.6 (4 <0.7 <5 <l <3 <1 5#- APT-5F 3 (c t) <4 <1 <5 <0.9 (10 <1 <3 <0.9 5N-APT-652 <4 (0.9 <10 <1 (a) (a) l$ 54-APT-1A2 <1 <1 <8 <1 <6 <1 <3 (1 SW! APT-781 (4 <0.9 <4 <1 (6 <1 (3 (0.8 SN-APT-8A3 <3 (0.9 (4 <0.6 (10 <1 <3 <0.8 Su-APT-8G1 (ct) <6 <1 (4 <0.7 <5 (0.8 <2 (0.8

$N-APT-951 <5 <0.8 <5 <0.8 <7 <1 <3 <0.8 Su-APT-10A1 <5 <0.8 <6 <0.8 <6 <1 <3 <0.7 Sa-APT-llG1 (ct) <3 <0.9 <8 <1 (6 (1 (4 <0.7 Su-APT-IZA1 (7 <0.8 (7 <1 (7 <1 <4 (1 Su-APT-1201 <1 <1 <6 (0.9 (7 <1 (4 <1 Su-APT-12G2 (ct) <5 <0.8 <6 <1 (9 <1 <3 .<0.7

  • Sr-89 results are corrected f or decay to sample step date.

(a) Sample not collected.

(ct) Denstes Control location a

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. N == og em en eea .

O a e e a e a e e a e e e e a e e e e g 3g a se end hhhh A >= pm een h g >mAhh km A hn h y

  • = 3 gg3 g eeee a eeeee , ens eeee ind eeee e h h as w J

W m  %%%% w  %%%%% e  %%% e W  %%%%

ned ese

>=

se e en N e @ eS m O N $ mONw E ** @ en N t j

ed O O ** N O N O ** N N end O se se N w O O og N mm  ;

-.d &  %%%% o= %%%%% as  %%%% w  %%%% e===========

O and SS9P w eO O em me ** ** w NNNN WeAwD w e OOOO Oi OeOOO e a= == 3 em se se em O ee == em en w ww w P

P 69

2 m

im ,

em 99999 9999 9999

=w 9999 Nmme amNN tw mnem vvvy NNmmm vvyvv vyvv vvvv 1 e

5 e

I, m-e N

m 9 I O 9999 9999 l

= 0999 99998 NNNN 4 Nmme NmNNN NNNN vvvy e vvvy vvvvv vvvv 5

8 m

4  !

N m

e +

O 9998 OOOO I

= 9990 99909 Nemm s 4 Nome memmm mmmN vvvv e vvvv vvvvy vvvv i s'

e W

  • w m

5 e m

+ m -

em i w

4 Om 9999 OOOO e = = w OOOO 99990 mmmm m + sw Nome memmm vvvvy mmmN vvvv vvyv a e vvvy ,

m N a w +

4 m a W e m a w 8 m E m  % e4 e 4 =

G we Om

  • W w 5 & O*

= WO OOOO OOOO P = OOOO 99990 mmmm s m m. g4 Nome memmm mmmN vvvv vvvy W mmO es vvvy vvvvv J a ms [

w a me w w A 4 S 5 m 9 u k 4 3 n 9 m W l O W m i

= = e E O

g. 3 e O 9999 OOOO s = OOOO OOOOO mmmN Nmmm de. e 4 meme vvvy memNm vvvvy vvvy vvyv o

E m

+ 5 A

o m =

4 3 5 e e t 8 m

  • i

- W O Om

.m

=w OOOO OOOOO C000 0000 w NmNmN NNmN mNNN r (w e mNNN vvvy vvyvv vvvv vvvv i 5

M [

t m 3 a q O ,

e o p

e O

OOOOO 0000 0000 "e

m OOOO mNmm NNmm u r 4 Nmme eemNN vvvy o e vvvy vvvvy vvvv a E

H = t 0 i b )

hhhhh hhhh hhhh a e

Nhhh emme mamme emme meme W a

w  %%%% chem home m emOh mehem OmNN

  • l 4 OmNN Om=NO mmNm  %%%% e O  %%%%

mumm NNNNm mmmm wwww e 99909 e s Oe O. O. O. O. O. O. O. 9. c. 0 0 e 1

! O > hhhhh hhhh Ahhh w m

m ehhh mese e mamme emme emme e i e  %%%%%  %%%%

w a  %%%N mmche z mohe a whom w e Geme 3 W Om=N m mo=N a w 3 me=N a No==N  %%%% u  %%%% = i s 3  %%%% e  %%%%% e mmmm a move w O e twmma w =NNNN 4 w 7 mOOO w 99900 S OOOO 4 0000 p W s

?

I 70 t

I TA8LE C-9 (Cent.)

C00CENTRATI0e5 0F IODim(-131 IN AIR CARTRIOGE 5AftPLES Results In Units of 10-3 pCI/m3 e 2 sigma COLitCil0# DATES 54-A10-843 L9CATIDs C00E5 55-A10-8G1 5t-A!0-951 SW-AIO-10Al $N-4IO-IIG1 (ct) 55-AIO-12Al Sa-Alt-1201 Se-AIO-1767 (ct) (ct)

E 04/28/87-05/05/87 (40 (20 (40 (40 05/05/87-05/12/87 (20 (40 <40 <30 <40 (10 <40 (40 (40 C5/12/87-95/19/87 (30 <20 <30 <30 <30 (40 (20 (40 C5/19/87-05/26/87 (30 (20 (40 (40

<20 (20 <30 C5/26/87-06/02/87 (30 (40 <30 <30 (20

<30 (30 (20 (30 (20 (20 <20 U Just 06/02/87-06/09/87 <40 <40 <40 (20 06/09/87-06/16/87 (20 <30 <30 (30 <30 (10 <30 <30 (30 06/36/87-06/23/87 (60 (60 (60 (20 (30 (30 (20 06/23/87-06/30/87 (40 (20 <30 <30 (20 (20 (20 (20 (30 (30 (30 <10 JULY 06/30/07-07/07/87 <40 (20 <40 (40 (40 07/07/87-07/14/87 (30 <30 <40 (4P <30

<30 <30 (30 <30 C7/14/87-07/21/87 (30 (30 <30 (30

<30 (20 07/21/87-07/28/87 <40 (40 (20 (30 <30 <30 (30

<30 <30 <30 <30 <30 AUGUST C7/28/87-08/04/07 430 (30 <20 <30 <30 C8/04/87-08/II/87 (30 (30 (20 (30 , <30 (20

<30 (30 <30 00/11/87-08/18/87 <30 (30 <30 <30 <30 (30 (20 0G/18/87-08/25/87 (30 <30 <30 (30 <20 (20 (20 (20 CC/25/87-09/01/87 <50 (50 <30 <30 <30 (20 (20 (20

<30 <30 <20 (cI) Denotes Centrol Locatten

.,..,-_m..._,-.-m---.-,.yy-_ -,_- - -- - - _ . - , - , , - - - - ~ , - . - _ . ,-e , , - , . ---r -

.r- . >..e--.. _ .,

-.7-._3-- -

r -, - - - . - - - _ __  %.- ,-_. - . - - - . . _

u N

N en eA O e= 00000 0000 0000

== w OOOO NNwwN NNNN NNNN 4w NNNN vyvvv vvvv vvvv e vvvv a

e me o

N es e

O 00000 0000 0000

== 0000 mmwwm mNmN mNNm eg m ew m e vvvv vvvv e vvvv vvvvv s

e

==

4 N

==

e O C0000 0000 0000

== OOOO mNmN mNNm 4 N ew M w mNmNm vvvv a vvvv vvvvv vvvv E

e e

==9 w

E **

4 @

e ==

n on w 5 ea o e O == 00000 0000 0000 O = == u C000 MNmN MNNN 4w NNmw mNwNm vvvv

== em vvvv vvvvv vvvv a e

> N E m e 4 es em W e m en m E en U ==  % e4

() 4 = wO W W D **

w E & O e

WO COOO C0000 OOcc OC00 P m

mmNmm mNmN feNNm

== E4 NNmw vvvv vvvv W

e mO e

O e vvvv vvvvv

== == == a n, s == e e=6 em 4 m a O u 4 == 0

> O en se O =* ==

= A e e w D e Q O .30000 0000 0000 C == C000 = == N N N ew ==

e = are N N N N N m == N vvvv at vvvv vvvvv vvvv a e O em a

== es e

> ==

4 3 m ea E Es ==

J

. ==e, s e E t @

O O s= C0000 0000 0000 W == u OOOO NNNN NNNN at w NmmN mmmhN vvvv e vvvv vvvvv vvvv E

e m a 4 O ED

  • e ed O 0000 0000 e

== C000 00000 NNNN W er NmNN mmmNN NNNN vvvv 0 e vvvv vvvvv vvvv =6 m ,

e O

b en Ahhh hah % g Nhhhh whhh ED e e are m e e e 50 e ED # EB e e 50 G ED #

%%%%%  %%%%  %%%% w w  %%%% O h w e= meNe

> meNP emOhm O == N N en O == N N O == == N O 4 O == N N  %%%%%  %%%%  %%%% @

Q  %%%% *****=N NNNN =*

peep O O O O == ***esa == ==*===== 0 N OOOO s***====== e e e s a e e e e e a e e e e e e e C a en h h h h g Ahhh g hhhh &

== w hhhh #WWG == ED#SW Q

> en WWWW W GWWWW w

%%%% ac  %%%%

%%%%% as W E  %%%% e.,

eemON E mOhw E == E e N ew w == m e N an w O O ** N a O O == ew O N O == N N =s O == == N ==

%%%%% 3= N%%% w  %%%%

=.e

=* h  %%%%

meep

==

u eOOOO O ======== ==, NNNN W O ew 5 ======== O > ea == == =.*

W e OOOO O O========

72

t L

. r r

i O

N e

W T

E o

S e O De N. m. he m. ee

== hO m% e e e= N en m NN m W 4 e OOOOOOOOOOOO O O OOOOO o= es emeeewwww@ww es es e et es e es e @ w w e to

== 4 yvvvvvvvvvvv v v vvvvv e

==

.h. h. ee. O. N. e. a W ee == e N e w ee N a= N o.

e h a e

a

= 4 3 5 6 e e a e e

e ** e P w

e- N w

    • b

- es e E

w b .= = n t o at .e

  • ** 4 w e. p .==. m. e. O

%. O. d w.m .= P. O. e. O. e.%.80 >. d. e. ==eN. w I

em O =e-

= ==# C == 0 == N w C == 0 ** O O O O O O ac es se O O == O O w l

=  % e s

o ed e es es es es es es es et es es et es es es es et se es es es es . es es W W e e l O & W v w 3 O Oe w. m. se N dM N @ N.N.d.ee . . @ h. e. %. N. O. d. w ee w. d. d. e. *=. =

w e

. 5 ~m~ c.wwm~ .e ~ ~ w e a.eceme .

4 4 es ,

e= em en w - ..

e - O w

+

O

& w .

v F O . ,

3- 4 O O g t ,

a 3 fs COO e

a "

888888.8...g

.= .e . ee .e e .We

.e

~

v ~~

e 8.88.8.88....

e

. =~

C. e..

OCO

~

1

m. vvvvvvOvCOO a=

m NNA vO e vvO e v v v 0cCN O e% O.

e

b. == N N tw N == mNme **

O O C

e e 5 em O b .

== @ es

> w EN

< es a e - O.

n= Eo

. R (r &4 w bN g w

  • a gea O g w e p e% >= e% % e >= em N em om os e% e. % es es e% e% e. p. % % ,. em ens 80 e e e e e e e e e eD se 80e e e e e80e # # ace PAB e  %%%%%%%%%%%%  %%%%%%%%%%%% 3 4  % e == m e e we e O h == O h w == # e p == m O ** == 0 h90 O NNmNNNmNmNOm NNmNNNmNmNOm 4 &W

%%%%%%%%%%%% s=  %%%%%%%%%%%% A3 m == ==Nmve@*=meONN 4 ** N m w e e >= e e O N N == b g 6 e O O O O O O O O O *e s= == O O O O O O O O O == ** ** O=8 c e e i e e a e e e 4 e e .N. e a e e e e e e e e i e == e

.

e ese sm N em A % em h am em *= o% a= em em % A og h on A em N a= sY W 3 m e e s e e m eD e s e e 5 eMesseeme0eme ** Ob  !

w O  %%%%%%%%%%%% O  %%%%%%%%%%%% 4we 6 w == N N N N e e == w == c m e == N m N m e w me w meem m e l

}, w > OOOOOOOOOOaC > C000000000=O O q  %%%%%%%%%%%% 4 ===*=.

w >= == N m e e e % e e O == N e- = N m e en e h e e O == N e eA ww l

e' O O O O O O O O O *e *= == e O O O O O O O O O ****==  :

I i

i

(

i 73 . ,

e t

en K

8 W N.

5

  • e 8

e 5

m e.

W N

  • e e e. e. M. N.

W O O O O g v v v v e

E e

N 6

e e e.d e Mw w so. N. M. M. M. M. M. , . m. N. m. N. N. N.

se O O O O O O O O O O O O O O

, w v v v v v v v v v v v v v v i 9 .

e e a O e W =

e ed on me K N E ee i-em se ee e me  %. eos O se m = & se

  • e *e W C ea w w w w w w o e a. w se m. . . N. . en. M. m. M. . . m. m. N. . m. e. m.

W end w O O O O O O O O O O Ce o O O O O O O

  • i a e. S w v v v v v v v v v v v v v v v v v v 6 '

and e= g O e , se W O =S e &

8 O d we a i 4 == es ( .s 4

  • "
  • V w em 4 8 O 9 G S =# * ==

m O e a= eb W N em 6 es G 4) 9 == S

  • e e8 W &O e= ee am 4aw i 4 *= W= w en4 a 3 yw m. @ . N. m. w. . m. m. m. m. N. N. N. N. a es h  !

os sa aw O O O O O O O O O O O O O O 4 en ,

E 6

  • v v v v v v v v v v v v v v w he w a a & ee == i

%d e d6e t 1

S &S '

, 6 %3W W be "I , =* b i

s es e 4

=Om i 36 -

N h e F 9 8=

4 E=b e w w w *9@

m. e. m. m. e. M.

g . . m . k es i E O O 9 O O O O O O O 3 ee b I J v v w v v v v v v v 9be e &S S S&SF A G a* 9

&Og 9 se .6 w=bw e e a= 6 e ** O ed aa

mO == * * * *

  • O at N *= *= 0 \
  • mh es se e 9m*w 5 e a en O se O e e,' b == 9 h O N @ O@ e O ==**=*a O OO e e se se se a e 8 5 4 ** ,

e o e N 4 y se e e 4e

  • i w e w em e m .Ne O so O e

e e =o 4* me w en65 E = ==

em q

@O e e en N N en e O o =

O se N O p e o e se O E4sa ** 9 O e N m o e o se me w O e en D @

  • 4 e en se == e e O m N O se m o e e e em 4 ** O == ,

e O m h se N N , e se eO es e 9 p en e, 8

O e e se N w h m a s == # 3 ** 8 ** i

) ee > Q N e e e O en e., eos ee# MM 9499999

  • se W

% g se se Ne Ie OeNN eO em N e8 e e e* gggaw w S a a W N and ens f

@W5mSEG ,

f w 4 3 3 ed se N e.,

en 3 4 w me een ee# > > 3 3 en en e= O ees one W *"*

ed 8 O E 5 > > 3 3 d ed J d b, b e= > W ed Y ** #"

7 O 4 w 4 A G 6 3 3 3 3 3 3 &.,

. e w w O tes = % w "se "9 A" -

V *) to. E g6 3 3 *g 9 *3 *% ( ( eeeO S O E5wwww '

t I

i o

30

TA8tt C-12 COWC(NTR ATIO45 0F Sta0eTIU4-09 .990 -90 Amp GAMMA EMIffER5* 15 MIit SAMPt*5 Results in Units of PCS/f a 2 sI9ea l

! CotitCTIce DATES NUCLIDE se.GNE-602 5m.mtt-8G2 5m.ntz-8F2 l

Sw.snt-ler l 54.Gma-12Cl(s)

(ct) , (ct) (ct) l l

JA#UARV 05. 06. 07. OS Sr-89 <5 (4 <3

, $r-90 2.5 e 1.0 8.7 a 1.1 2.6 3 0.7 i

E-40 1860 t 190 975 e 98 (b) 1630 2 160 Cs-137 <5 <6 9.61 a 4.98 ff88UART 01, 04, 08. 09 Sr-89 (4 44 <4 t 5r-90 1.2 a 0.6 6.9 t 0.9 2.5 a 0.8 K-40 1570 e 160 1080 e 110 1670 e 178 Cs-137 (5 9.88 e 4.09 9.61 2 3.60 u

C" MARCH 10 I? Sr-89 <2 <4 Sr-90 0.88 a 0.52 1.8 i 8.8 E-40 1350 e 140 1230 a 120 Cs-137 7.78 1 3.87 <5 APRIL 12. 13 Sr-89 (c) <4 <4 <4 Sr-90 4.3 e 2.1 2.2 a 1.1 1.6 t 0.6 E-40 876 a 88 1630 a 160 1270 t 130 Cs-137 <8 <5 <5 MAT 12. 13. 14 Sr-89 (d) (d) (d) (d) 5r-90 (d) (d) (d) (d)

E-40 1430 e 140 987 e 99 1630 t 160 1440 t 140 Cs-137 C.02 e 3.84 (8 9.44 a 3.93 (6 MAY 26. 27. 28 $r-89 <2 <4 <3 <3 <3 Sr-90 5.1 a 0.6 13 e 1 2.9 a 0.7 1.8 e 0.6 3.1 a 0.8 K-40 1990 a 150 880 t 88 1600 t 160 1500 t 150 7350 e 130 Cs 137 <F <6 <8 (7 <5 tote: See festeetes at end of t ab l e .

-_e,s ,.- ,,,,=s, . _ _ . - - -,.----w,-.---., - - - . _ , -_r .,,,.,,,,%,1, -- - - . - ,n- , - - . , -, , , . , , , - - , _ - - ,- - --- - - y, .,- _ , -- ,

n e, j TA8tE C-12 (Cset.)

CONCENTRATIONS OF STRONTIUM-89 ANO Se APO GAMMA EMITTER 5* IN MILK SAMPLES Results in Units of pt'.. t 2 sigma COLLECTIGN OATES NUCLIDE SN-GMK-G82 $N MLK-8G2 SN-MLK-8F2 SN-GMK-10F1 'SN-GMK-12Cl(a)

I (cl) (cl) (ct) e""'" 5;::: 1:1 1:1 1:1 1:1

! K-40 1230 t 120 947 t 95 1600 t 160 1750 t 170 i Cs-137 <6 <4 11.5 t 3.7 <6 i

q JUNE 22, 23, 24, 25 -

Sr-89 <4 <3 <3

Sr-90 2.3 2 0.6 5.7 2 0.8 2.1 1 0.7 i K-40 1720 t 170 1500 t 150 1430 1 140 Cs-137 <1 <F <8 y JULY 08 Sr-89 (d) (d) (d) cn Sr-90 (d) (d) (d)

K-40 1770 t 180 912 2 91 1710 t 170 Cs-137 <5 <7 10.1 1 4.1 JULY 21, 22 Sr-89 (2 <4 <2 <4 Sr-90 6.3 2 0.5 15 t 1 1.7 2 0.3 2.5 t 0.7 l K-40 1820 t 180 800 t 80 1810 t 180 1610 t 160

Cs-137 8.14 1 4.46 <5 5.92 1 3.48 <4

^ " " " " " "

l K-40 1:1 1480 t 150 1:1 866 1 87 1:1 1480 t 150 1:1 1523 1 150 Cs-137 7.49 2 4.00 <7 <6 <6 AUGUST 19, 20 SR-69 (4 <3 <3 SR-90 13 t 1 (f) 2.6 t 0.5 1.5 1 0.5 K-40 (e) 804 t 80 1720 t 170 1640 t 160 Cs-137 <5 6.48 2 3.26 <4 i

i Note: See footnotes- at end of table.

}

9 4

TABLE C-12 (Cest.)

CONCENTRATI0M5 0F STRONTIUM-89 AND -90 AND GAMMA EMITTER 5* IN MILK SAMPLES Results in Units of PCl/l i 2 sigma COLLECTION DATES NUCLIDE SM-GMK-682 $N-MLK-8G2 54-MLK-8F2 $N-GMK-10F1 SM-GMK-12Cl(a) SN-GMK-1381(g)

(c1) (ct)

SEPTEM8ER 02, 03 Sr-89 (e) (d) (d) (d)

Sr-90 (d) (d) (d)

K-40 1020 t 100 1880 2 190 1600 ! 160 Cs-137 (4 <5 <1 SEPTEMBER 14, 16, 17 Sr-89 <2 <3 '<2 Sr-90 3.5 t 0.7 2.3 1 0.6 2.0 1 0.5

, K-40 1840 t 180 1590 t 160 1360 t 140 j Cs-137 <4 (4 (6 1 SEPTEMBER 30, Sr-89 (d) (d)

OCTOBtR 1 Sr-90 (d) (d) .

'd

'd K-40 1500 t 150 1580 t 160 Cs-177 <7 <5 OCTOBER 1.' , 14, 15 Sr-89 <4 <3 <3 Sr-90 9.6 1 0.8 1.8 t 0.5 2.7 1 0.5 K-40 897 t 90 1520 t 150 1670 t 170 Cs-137 <4 <5 <6 NovtMBER 8, 9, 11, 12 $r-89 <2 <3 <2 Sr-90 5.1 1 0.6 3.9 1 0.4 2.9 t.0.5 K-40 936 2 94 1800 t 180 1530 t 150 Cs-137 <6 7.28 2 3.55 <5 DECEMBER 5, 8, 9, 10 Sr-89 <2 <3 <2 <2 <3 Sr-90 2.3 1 0.4 1.3 1 0.4 1.0 t 0.2 3.0 2 0.5 0.61 2 0.3 K-40 894 t 89 1800 1 180 1510 t 150 1190 2 120 1850 t 180 Cs-137 (4 <5 (6 <6 <4

  • All other gamma esitters not listed were <LLD; typical LLD's are given in Tables C-19 and C-20.

GMK Goat's Milk MLK Cow's Mllk j (a) Bottled Mllk J

(b) No goat milk avaltehle during the winter due to kidding.

(c) No sample available, owners did not supply sample.

(d) Strontium analysis performed once a month.

(c) Supplier moved; milk will no longer be collected at this site.

(f)

Lg i Result confirmed by recount.

New location added to the program December 1987.

Lcl) Denotes Control Location

TABLE C-13 CONCENTRATIONS OF TRITIUM. 100lNE-131 AND GAMMA EMITTERS ** IN POTABLE WATER Results in Units of pCl/ liter i 2 sigma LOCATION COLLECTION H-3 I - 13.l *

CODE DATE K-40 Cs-137 Th-228 4

PWA-25! 03/18/87 140 t 70  ? <90 <6 <10 06/17/87 (100 <o <200 (6 <10 09/09/87 (200 <0.. <100 (6 <10 12/16/87 450 t 140 <0.2 60.5.2 30.9 (a) <3 <6 sa PWA-681 03/19/87 (200 (0.2 <200-

,m <6 <10 (ci) 06/17/87 <100 <0.3 <60 <3 <8 09/09/87 <200 (0.3 <50 <3 <1 12/16/87 260 1 90 <0.2 <10 <4 <9 '

i

PWA-1352 03/18/87 <100 <0.2 <200 <6 <10 i

06/17/87 <100 <0.3 <80 <5 <10 l 09/09/87 (100 <0.3 <60 <4 <8

! 12/16/87 160 t 100 (0.3 <100 <4 (7 i AVERAGE i 253 r 283 60.5 1 30.9 2 s.d.

I 1

lodine-131 results are corrected for decay to sample stop date. Determined by radiochemic.1 analysis.

i Gamma emitters not listed were <tLO; typical LLDs are found in Tables C-19 and C-20.

(a) Sample had rusty appearance. That may explain the K-40 result.

{ct) Denotes Control Locat ion 1

j I

  • j 4

I

TABLE C-14 CONCENTRAT10NS OF GAMMA EMITTER $* IN GAME SAMPLES Results in Units of pCl/kg (wet) i 2 sigma LOCATION CODE COLLECTICM DATE SAMPLE TYPE K-40 Cs-137 SN-GAX-1353 03/03/87 Raccoon 2850 t 290 35.1 t 6.8 SN-GAX-1353 04/08/87 Squirrel 3510 t 480 152 t 36 SM-GAX-14SI 06/10/87 Rabbit (a)

SM-GAX-1353 10/27/87 Raccoon 2370

  • 240 518 i 52 SN-GAX-1353 11/19/87 Sqstrrel 3960 2 400 6490 t 650 Average t 2 s.d. 3173 1 1406 1799 2 6268 1 All other (a) Sample gamma celtters Unavailable not listed were <LLD: typical LLDs are found in Tables C-19 and C-20.

C

TABLE C-15 CONCENTRATIONS OF GAMMA EMITTER 5* ANO l-131 IN F000 PRODUCT SAMPLES Results in Units of pCl/kg (wet) 1 2 sigma SAMPLE TYPE COLLECTION DATE K-40 I-131** Cs-137 Be-7 LOCATION CODE CABBAGE 08/20/87 2120 1 2I0 <4 <10 (100 SM-F PL-78 3 <20 <100 S M -F P L- 18 3 LETTUCE 08/20/87 3400 1 340 <4 1350 t 130 <7 <10 <100 SM-FPF-881 STRANBERRIES 06/10/87 <10 <100 SM-FPL-881 CAB 8 AGE 07/15/87 2520 t 250 <10 01/15/87 2670 t 270 <10 <20 250 1 139 SM-FPL-881 LETTUCE

<10 <100 03 S M -F P V-8B I BEETS 07/15/87 2980 1 300 <10 O 07/15/87 3440 2 340 <20 <9 <80 SM-FPV-881 CARROTS ,

ONIONS 07/15/87 1760 t 180 <20 (9 <90 SM-FPV-881 <20 SM-FPL-8BI CA88 AGE OR/13/87 2210 1 220 (7 (200 COLLAR 05 08/13/87 4180 1 420 <10 <10 <100 S N-F P L -881 <80 SM-FPV-881 8EETS 08/13/87 2270 1 230 <10 (8 CARROTS 08/13/87 3390 1 340 <9 <10 <100 S M -F P V- 881 <80 08/27/87 2740 1 270 <7 <9 SN-FPV-881 BEETS

<10 <90 SM-FPV-88? CARROTS - 08/27/87 2660 1 270 (7 08/27/87 2570 t 260 <5 <7 <50 SM-FPL-Stt CORN

<5 (20 <100 SM-FPL-881 (ABBAGE 08/27/87 1580 t 160

<7 <10 (A88 AGE 09/16/87 1820 t 180 <5 SM-FPL-881 <4 <8 91.8 i 41.1 SM-FPL-8BI LETTUCE 09/16/87 2380 1 240 09/16/87 2480 1 250 <10 <10 <100 S M -F P V -881 IEETS <10 <100 SM-FPV-881 (ARROTS 09/16/87 3360 t 340 <8 09/16/87 2860 1 290 <7 (10 <l00 SM-F PV-881 10MATOES 10/22/87 3200 1 320 <6 <10 (1 00 SM-F PL -8B I LETTUCE <100 POTATOES 10/22/87 4080 t 410 <6 <10 SN.FPV-881 <1 <8 <80 SM-IPV-881 CARROTS 10/22/87 2400 t 240

  • All other gamma emitters not ilsted were <LLO; typical LLO's are given in Tables C-19 and C-20.

" I-131 by Radlochemistry

TABLE C-15 (Cont.)

CONCENTRATIONS OF GAMMA EMITTER $* ANO I-131 IN FOOD PRODUCT SAMPLES Results in Units of pCl/kg (wet) i 2 sigma LOCATION CODE SAMPLE TYPE COLLECTION DATE K-40 I-131** CS-137 Se-7 SN-FPL-5F2 (cI) $PINACH 06/17/87 3840 1 380 <30 <10 <100 SN-FPL-5F2 CA88 AGE 08/20/87 2250 1 220 <4 <10 S N-F PL-5F 2 <80 LETTUCE 08/20/87 1730 t 170 <6 <9 5N-FPV-5F2 (80 1

BEETS 08/20/87 3500 1 350 <4 (10 <100 SN-FPL-12H1 (ci) 8EETS 07/15/87 2940 1 290 <20 (10 <100 SN-FPL-12H1 RADISHES 07/15/87 2480 1 250 <10 l co $ N-F P V-12H 1 (20 (200 i ~

BEETS 09/16/87 3060 1 310 <7 (7 <10 SM-FPL-12H1 TDMATOES 09/16/87 1800 t 180 <7 (7 <70 1

SN-FPF-12H2 (cl) STRAW 8ERRIES 06/10/87 1360 t 150 <6 <10 (90 SM-FPL-12H2 LETTUCE 08/13/87 1360 1 140 (20 <10

! <90 S N-F P L-12H 2 SPINACH 08/13/87 5450 t $50 (10

! <6 119 i 43 S M-F P V- 12H 2 CARROTS 08/13/87 2610 1 260 (7 <8 <70 1

SM-FPL-12H2 LETTUCE 08/20/87 1710 t 170 SN-FPL-12H2

<4 (10 <100

, SPINACH 08/20/87 5360 2 540 <3 (20 (200 4

SM-FPV-12H2 CARROTS 08/20/87 2160 1 220 <4 <10 <100 1

5N-FPL-12H2 CORN 08/27/87 3070 1 310 <6 SM-FPL-12H2 (8 <60 LETTUCE 08/27/87 2480 t 250 (6 (20 (200 j SN-FPL-12H2 SPINACH 08/27/87 5850 t 590 <S SN-FPL-12H2 <6 (50

, LETTUCE 09/16/87 1880 t 190 <7 (9 <90 4

S M-F PL - 12 H2 SPINACH 09/16/87 5030 t 500 <7 5 N-F PL -12H2

<20 <200 LETTUCE 10/22/87 3780 1 380 <8 86.3 1 13,9 233 i 116 SR-FPL-12H2 SPINACH 10/22/87 7200 1 720 <6 <9 135 t 56 I

    • All other gamma emitters not ilsted were <tLO; typical LLD's are given in Tables C-19 and,C-20.

l-131 by Radlochemistry (c1) Denotes Control Location i

e

T ABL E C-15 (Cont. )

CONCENTRATIONS OF GAMMA EMITTER $* AND I-131 IN F000 PRODUCT SAMPLES Results in Units of pCl/kg (wet) i 2 sigma LOCATION CODE SAMPLE TYPE COLLECTION DATE K-40 1-131** Cs-137 Be-7 SM-FPF-5C2 STRAW 8ERRIES 06/10/87 1250 t 140 <4 <10 <100 SN-FPL-5C2 CABBAGE 07/15/87 2000 2 200 <4 <10 <100

$ N-F PL -5C 2 LETTUCE 07/15/87 2060 2 210 (6 <20 <100

$N-FPL-5C2 SPINACH 07/15/87 5130 t 510 <6 <20 <200 SM-FPV-5C2 BEETS 07/15/87 3190 1 320 (10 <10 <100 SM-FPL-5C2 CABBAGE 08/13/87 1530 t 180 <1 <20 (200 SN-FPL-5C2 LETTUCE 08/13/87 1620 1 170 <10 <10 <90 SM-FPL-5C2 SPINACH 08/13/87 5550 1 550 <10

$N-FPV-5C2 8EETS 08/13/87 (7 211 1 56 (a)

CD 4470 t 450 <20 (10 <90

" $N-FPV-5C2 CARROTS 08/I3/87 3110 t 370 (10 <10 <100 -

5N-FPV-5C2 RADISH 08/27/87 2l00 t 210 (7 <8 (60 SM-FPL-502 CORN 08/27/87 2680 1 270 <5 <7 <60 SM-FPL-5C2 CABBAGE 08/27/87 2109 1 210 (6 (10 <90 SM;FPL-5C2 SPINACH 08/27/87 4040 2 400 (6 <6 <50 SM-FPL-5C2 CABBAGE 09/16/87 1890 t 190 (7 <9 <80 SM-FPV-5C2 RADISH 09/16/87 1780 t 180 <7 <10 (90 SM-FPL-$C2 CABBAGE 10/22/87 2010 t 200 <6 <9 (80 SM-F PL -5C 2 SPINACH 10/22/87 SM-FPV-5C2 6800 t 680 <6 <9 156 t 60 POTATOES 10/22/87 3250 t 320 <10 <10 <100 SN-FPV-5C2 RA015HE5 10/22/87 2290 1 230 <10 (10 <100 All other gamma emitters not listed were <LLO; typical LLO's are given in Tables C-19 and C-20.

I-131 by Radiochemistry (a) Thorium-228 was measured at 6 7.9 2 7.1.

e

TABLE C-16 DIRECT RADIATION MEASUREMENTS - QUARTERLY TLD RESULTS mR/ standard month

  • A LOCATION
  • FIRST QUARTER SECOND QUARTER THIRD QUARTER FOURTH QUARTER ANNUAL AVERAGE CODES 01/07/87-04/02/87 04/02/87-07/08/87 07/08/87-10/01/87 10/01/87-01/06/88 1 2 s.d.

SN-IDM-151 3.6 2 0.5 4.4 1 0.4 3.3 t 0.1 3.1 t 0.0 3.6 1 1.1 l

i SN-IDM-351 3.4 1 0.1 3.4 1 0.2 3.3 1 0.2 3.3 1 0.2 3.4 1 0.1

$N-IDM-451 3.6 1 0.3 3.6 t 0.2 3.4 2 0.3 3.5 t 0.1 3.5 t 0.2 SM-IDM-552 3.8 1 0.2 3.6 t 0.1 3.5 1 0.1 3.7 1 0.2 3.7 1 0.3 SN-IDH-652 3.4 1 0.3 3.3 1 0.1 3.5 t 0.1 3.4

  • 0.2 3.4 1 0.2 4

SN-IDM-951 3.8 t 0.1 3.8 2 0.2 3.6 t 0.1 3.8 2 0.1 3.8 t 0.2 SN-IDM-952 3.8 1 0.2 3.7 i 0.2 3.6 t 0.1 3.6 t 0.3 3.7 1 0.2

$ SM-IDM-1353 4.0 t 0.5 3.7

  • 0.4 3.4 2 0.1 3.5 t 0.1 3.7't 0.5 SM-IDK-1452 3.3 1 0.2 3.1 1 0.1 3.1 t 0.2 2.9 t 0.2 3.1 1 0.3

$N-IDM-1551 3.2 t 0.1 3.0 1 0.1 2.9 t 0.2 3.0 1 0.2 3.0 1 0.3

$N-IDM-1652 3.7 1 0.1 3.5

  • 0.3 3.2 i 0.2 4.0 t 0.3 3.6 1 0.7 SM-IDM-2A2 3.6 1 0.4 4.0 t 0.2 3.4 t 0.1 3.2 i 0.3 3.6 1 0.7

) 54-IDM-2A3 3.5 1 0.1 3.2 i 0.1 3.2 2 0.3 3.2 2 0.2 3.3 1 0.3 SN-IDM-6Al 5.010.3 4.9 t 0.2 4.7 1 0.2 4.6 1 0.4 4.8 t 0.4  :

1

$N-IDM-7A2 3.5 t 0.0 3.5 1 0.1 3.4 2 0.2 3.5 t 0.4 3.5 t 0.1 SM-IDM-8A3 3.6 1 0.2 3.6

  • 0.1 3.3 2 0.2 3.5 t 0.1 3.5 t 0.3

$N-IDM-10Al 3.6 t 0.1 3.7 t 0.1 3.4 s 0.1 3.4 1 0.1 3.5 t 0.3 SN-IDM-IIAl 3.5 t 0.1 3.6 1 0.2 3.71 0.2 3.4 1 0.2 3.6 t u.3 SM-IDM-12Al 4.2 1 0.2 4.0 t 0.3 3.9 1 0.2 3.8 1 0.3 4.0 1 0.3 SM-IDM-7BI 3.6 t 0.1 3.5 t 0.1 3.4 1 0.1 3.6 i 0.2 3.5 t 0.2

, The standard month = 30.4 days.

4

TABLE C-16 (Cont.)

DIRECT RADIATION MEASUREMENTS - QUARTERLY TLD RESULTS mR/ standard month * .

LOCATION IIRST QUARTER SECOND QUARTER THIRD QUARTER FOURTH QUARTER ANNUAL AVERAGE CODES 01/07/87-04/02/87 04/02/87-07/08/87 07/08/87-10/01/87 10/01/87-01/06/88 1 2 s.d.

$N-IDM-SDI 4.7 1 0.7 4.6 1 0.2 4.4 t 0.2 4.6 1,0.4 4.6 i 0.3

$N-IDM-5D3 4.2 1 0.1 4.2 1 0.1 4.2 1 0.2 4.1 i 0.3 4.2 1 0.1

$N-IDM-1201 4.1 1 0.1 4.1 1 0.2 3.9 1 0.3 3.9 1 0.3 4.0 1 0.2 l SM-IDM-6El 3.9 1 0.1 3.6 1 0.1 3.4 t 0.1 3.5 2 0.1 3.6 i 0.4 j SM-IDM-7El 3.5 t 0.2 3.7 2 0.1 3.3 t 0.1 3.5 1 0.2 3.5 t 0.3

! SM-IDM-8El 4.0 t 0.1 4.0 t 0.4 3.8 1 0.1 3.6 2 0.3 3.9 2 0.4 i

co SM-IDM-9El 3.7 1 0.2 3.9 1 0.3 3.5 1 0.2 3.6 t 0.4 3.7 1 0.3

.b SM-IDM-10EI 3.8 1 0.3 3.8 1 0.2 3.7 2 0.1 4.0 1 0.3 3.8 1 0.3 SN-IDM-llEl 3.5 1 0.7 3.2 1 0.3 3.2 i 0.4 3.0 1 0.2 3.2 1 0.4 SM-IDM-13El 4.0 1 0.1 4.0 t 0.2 3.8 1 0.1 3.7 1 0.2 3.9 2 0.3 SM-IDM-5F3 (ct) 4.6 2 0.2 4.5 t 0.0 4.3 1 0.2 4.5 2 0.4 4.5 i 0.3 SM-IDH-6GI (ct) 3.4 1 0.1 3.3 i 0.3 3.2 1 0.1 3.2 1 0.2 3.3 2 0.2

$N-IDM-8Gl (ct) 3.8 1 0.1 3.8 1 0.1 3.6 2 0.1 3.8 2 0.2 3.8 2 0.2

SN-IDM-IIGl (c t) 3.8 2 0.1 3.7 1 0.2 3.5 t 0.1 3.4 2 0.3 3.6 2 0.*

SM-IDM-12GI (ct) 3.1 1 0.1 3.5 1 0.2 3.4 1 0.2 3.2 1 0.2 3.5 1 0.4 SM-IDM-12G2 (ct) 4.5 t 0.1 4.3 t 0.2 4.3 1 0.1 4.0 t 0.4 4.3 2 0.4

Average t 2 s.d. 3.8 i 0.8 3.8 i 0.9 3.6 1 0.8 3.6 2 0.8 3.7 1 0.2 The standard month = 30.4 days.

(ct) Denotes Control tocation e

TABLE C-11 DIRECT RADIAil0N MEASUREMENTS - MONTHLY TLD RESULTS mR/ standard month

  • LOCATION JANUARY FECRUARY MARCH APRIL MAY JUNE CODE 1987 01/07-02/05 02/05-03/05 03/05-04/02 04/02-05/07 05/07-06/03 06/03-07/08 SN-IDH-151 3.6 1 0.4 3.0 t 0.2 3.7 2 0.3 3. 7 t 0.4 SM-IDH-351 3.5 t 0.5 3.4 t 0.8 3.4 1 0.4 3.1 2 0.1 3.8 1 1.0 3.5 t 0.3 3.4 1 0.2 3.6 1 1.1 SM-IDM-451 3.8 2 0.4 3.4 1 0.5 3.8 2 0.3 3.5 t 0.1 SM-IDM-552 3.7 t 0.3 3.8 1 0.9 3.8 1 0.9 3.5 t 0.3 4.0 t 0.7 3.8 1 0.2 4.0 1 0.0

$N-IDM-652 3.8 1 0.8 3.5 t 0.2 3.1 1 0.2 3.6 1 0.2 4.0 t 1.3 3.6 1 0.1 3.2 1 0.4 SM-IDM-951 3.7 1 0.2 3.5 t 0.2 3.9 t 0.7 3.7 2 0.1 3.7 1 0.3 SM-IDM-952 3.7 1 0.2 3.4 2 0.1 3.5 2 0.2 4.1 1 0.4 3.8 1 0.1 3.9 i ..! 4.0 1 0.4 SM-IDM-1353 4.5 1 0.6 4.1 t 0.4 4.0 1 0.5 3.8 1 0.1 3.7 1 0.2

$N-IDM-1452 3.3 1 0.1 3.7 t 0.4 3.4 2 0.8 3.6 t 1.1 3.2 t 0.2 3.5 2 0.1 3.2 t 0.6

$N-IDM-1551 4.3 1 0.3 3.1 1 0.5 3.3 1 0.2 3.3 2 0.2 3.1 1 0.1 SM-IDM-1652 2.8 2 0.3 3.7 2 0.2 3.4 1 0.5 4.4 1 2.9 3.9 2 0.1 3.7 i 0.3 3.3 1 0.1 SM-IDM-2A2 3.5 1 0.3 3.2 1 0.6 3.8 t 0.6 3.6 1 0.2 3.7 1 0.2 SM-IDM-2A3 3.3 1 0.5 3.8 t 0.8 3.5 t 0.6 3.7 1 1.2 3.6 1 0.2 3.5 1 0.1 3.5 t 0.7 SM-IDH-6Al 4.7 1 0.4 8.4 1 0.3 6.9 1 3.4 5.0 t 0.2 4.7 2 0.3 S t:- I DM- 7 A 2 4.9 2 1.1 g 3.9 t 0.3 3.4 1 0.6 3.7 i 0.3 3.6 i 0.3 3.8 2 0.3 3.4 1 0.3 u, SM-IDM-8A3 3.7 1 0.2 3.2 1 0.3 3.6 1 0.3 3.4 1 0.2 3.6 2 0.2 SM-IDM-10Al 3.7 1 0.5 3.7 t 0.6 3.2 t 0.1 3.6 2 0.1 3.8 2 0.3 3.7 t 0.2 3.5 t 0.1 SM-IDM-IIAI 3.7 t 0.2 3.6 1 0.7 3.1 10.3 3.4 1 0.2 3.9 1 0.1 3.3 1 0.2

$N-IDM-12Al 4.0 1 0.5 3.9 1 0.6 4.1 1 0.4 4.1 1 0.1 3.9 t 0.4 3.8 1 0.7

$N-IDM-181 3.6 1 0.2 3.3 2 0.2 3.1 1 0.3 3.7 1 0.1 3.7 2 0.1 SM-IDH-5DI 3.2 1 0.1 4.6 1 0.2 4.3 1 0.4 5. 3 t 1.2 4.6 t 0.6 4.5 2 0.1 4.4 1 0.4 SM-IDM-5D3 4.3 1 0.4 4.1 1 0.8 4.3 1 0.2 4.4 1 0,3 4.3 1 0.1 3.9 2 0.4 SM-IDM-12DI 4.3 t 0.2 4.0 t 0.3 4.6 1 0.7 4.2 1 0.1 4.0 i 0.3 SM-IDM-6El 3.8 2 0.6 3.8 t 0.3 3.4 1 0.4 4.1 1 0.4 3.8 1 0.2 4.0 1 0.2 3.6 1 0.4 SN-IDM-7El 3.6 2 0.1 3.0 t 0.3 3.7 t 0.6 3.6 1 0.3 3.6 1 0.2 SM-IDM-8E1 3.2 2 0.3 4.0 t 0.3 3.6 1 0.5 4.3 1 0.5 4.0 1 0.3 4.3 2 0.3 SM-IDM-9El 3.6 i 0.2 4.0 1 0.2 3.4 t 0.3 4.2 1 0.4 3.8 1 0.4 4.0 1 0.1 SM-IDM-10El 3.8 1 0.3 3.6 1 0.2 3.6 1 0.2

- 3.9 1 0.2 3.7 1 0.1 4.4 1 0.3 3.6 t 0.1 SM-IDH-llEl 3.5 1 0.5 3.5 1 0.5 3.9 t 1.1 3.6 t 0.3 3.5 t 0.2 SM-IDW-13El 4.72 0.4 3.1 1 0.3 3.8 t 0.3 4.1 t 0.2 4.1 t 0.2 3.8 1 0.2 4.0 1 0.5 SM-IDM-5f3 (cI) 4.6 1 0.1 4.1 1 0.1 4.7 t 0.4 4.8 1 0.3 4.8 2 0.4 SM-IDM-6el (ct) 4.6 t 0.4 3.7 2 0.7 3.1 1 0.2 3.5 t 0.2 3.3 1 0.2 3.3 t 0.1 SN-IDM-8G1 3.7 1 0.4 2.9 1 0.1 cI) 3.4 2 0.3 4.0 1 0.6 3.9 t 0.1 3.8 1 0.3 SN-IDM-IIGI ((ct) 3.9 t 0.4 3.5 1 0.3 3.6 2 0.8 4.0 t 0.9 3.7 t 0.1 3.4 1 0.5 3.5 1 0.2 SM-IDM-12G1 (cI) 3.8 2 0.6 3.4 1 0.5 3.8 1 0.3 3.7 1 0.1 3.4 2 0.3 3.3 t 0.3 SM-IDM-12G2 (ct) 4.2 1 0.2 4.1 1 0.2 4.4 1 0.3 4.5 t 0.0 4.1 t 0.7 4.3 t 0.2 Average 1 2 3.9 t 0.7 3.5 1 0.7 4.1 t 1.2 3.8 1 0.8 3.8 1 0.8 3.6 t 0.9 s.d.

The standard month = 30.4 days.

{cl) Denotes Control location

TABLE C-17 (Coat.)

DIRECT RADIATIO 3 MEASUREMENis - MONTHLY TLD RESULTS mR/ standard month

  • AWNUAL LOCATION JULY AUGUST SEPTEMBER OCTOBER NOVEMBER DECEMBER AVERAGE CODE (1987) 07/08-08/05 08/05-09/03 09/03-10/01 10/01-11/05 11/05-12/03 12/03-01/06/88 t 2 s.d.

$N-IDM-151 3.1 1 0.2 3.3 1 0.1 3.4 1 0.4 3.1 1 0.6 2.9 i 0.2 3.5 t 0.3 3.4 1 0.5

$N-IDM-351 3.1 i u.3 3.7 1 0.6 3.2 1 0.2 2.9 1 0.2 3.0 2 0.2 3.4 1 0.3 3.3 1 0.6

$N-IDM-451 3.2 1 0.3 4.0 1 0.2 3.5 t 0.1 3.4 1 0.1 3.2 1 0.3 3.6 1 0.3 3.6 2 0.5 SN-IDM-552 3.4 1 0.2 4.3 1 0.4 3.8 1 0.5 3.4 1 0.2 3.1 i 0.2 3.8 1 0.3 3.7 1 0.7

$N-IDM-652 3.1 1 0.3 4.0 1 0.6 3.3 1 0.2 3.0 1 0.3 3.0 1 0.1 3.8 1 0.4 3.4 1 0.7 SM-IDM-951 3.4 1 0.1 3.7 1 0.3 3.5 t 0.1 3.4 1 0.4 3.1 t 0.1 3.7 1 0.5 3.6 1 0.4 SN-IDM-952 3.4 1 0.2 3.8 1 0.4 3.6 1 0.1 3.4 1 0.4 3.2 1 0.2 3.8 1 0.3 3.1 1 0.5 SM-IDH-1353 3.5 1 0.2 3.5 t 0.3 4.8 1 0.5 3.5 t 0.5 3.9 1 0.3 3.7 1 0.2 3.9 t 0.9

$N-IDM-1452 3.0 1 0.2 3.2 1 0.4 3.2 t 0.2 3.1 2 0.2 3.2 2 0.6 3.1 2 0.2 3.3 t 0.4 SM-IDM-1551 2.8 t 0.1 3.1 1 0.3 3.4 1 0.6 3.0 1 0.3 3.0 1 0.2 3.2 1 0.2 3.2 1 0.8 SM-IDM-1652 3.0 1 0.4 3.6 1 0.2 4.3 1 0.8 3.4 1 0.5 4.0 1 0.8 3.6 1 0.1 3.7 1 0.8 SM-IDH-2A2 3.2 1 0.2 4.0 1 0.6 3.5 1 0.6 3.3 1 0.3 3.3 1 0.4 3.6 1 0.3 3.5 t 0.5

$N-IDM-2A3 3.1 2 0.3 3.9 t 0.8 3.5 t 0.1 3.2 1 0.4 2.9 2 0.3 3.6 1 0.4 3.5 1 0.6 SM-IDM-6Al 4.3 2 0.6 5.4 t 0.2 4.9 t 0.5 4.4 1 0.4 4.4

  • 0.3 4.7 1 0.6 4.9 2 1.4

$N-IDM-1A2 3.2 2 0.3 4.1 1 0.2 3.4 1 0.4 3.1 1 0.2 3.0 t 0.4 3.7 1 0.4 3.5 2 0.7 SM-IDM-8A3 3.2 2 0.4 3.6 1 0.5 3.2 1 0.2 3.2 1 0.3 3.0 t 0.2 3.5 1 0.1 3.4 t 0.5

$N-IDM-IDAl 3.4 2 0.2 3.7 1 0.2 4.0 1 0.8 3.7 1 0.3 3.3 1 0.2 3.7 1 0.5 3.6 t 0.4 "cn SM-IDM-IIAI 3.3 1 0.4 3.5 1 0.3 3.3 1 0.1 3.5 1 0.2 3.4 t 0.4 3.9 1 0.3 3.5 t'O.4

$N-IDM-12Al 3.7 1 0.3 4.1 1 0.4 4.8 1 0.7 4.1 1 0.1 3.9 t 0.5 4.4 t 0.5 4.2 t 0.8 SM-IDM-781 3.2 1 0.2 4.0 1 0.2 3.4 1 0.2 3.1 1 0.1 3.1 t 0.3 3.6 2 0.3 3.5 1 0.6 SM-IDM-501 4.2 1 0.9 4.8 1 0.2 4.7 1 0.3 4.2 t 0.3 4.1 t 0.4 4.6 2 0.3 4.5 2 0.7

$N-IDM-503 3.8 t 0.2 4.7 2 0.4 3.8 2 0.2 3.7 1 0.2 3.8 1 0.2 4.5 1 0.9 4.1 1 0.7 SN-IDM-1201 3.1 1 0.2 4.2 1 0.7 4.8 2 0.6 3.9 i 0.1 4.4 10.3 4.1 1 0.3 4.2 i 0.6 S M-I DM-6E l 3.3 2 0.4 3.9 t 0.4 3.5 t 0.1 3.5 t 0.3 3.2 2 0.2 3.9 t 0.4 3.7 2 0.6

$N-IDM-7El 3.3 1 0.2 3.4 1 0.1 3.4 1 0.2 2.9 1 0.2 2.8 1 0.2 3.6 1 0.6 3.3 2 0.6 5M-IDM-8El 3.4 1 0.4 3.8 1 0.3 3.9 t 0.2 3.7 1 0.2 3.4 1 0.2 3.8 2 0.7 3.8 1 0.6

$N-IDM-9El 3.6 1 0.2 4.2 t 0.8 3.6 1 0.3 3.4 t 0.1 3.2 i O.2 4.0 t 0.4 3.8 1 0.7 SM-ICM-10El 3.4 1 0.3 3.9 t 0.4 3.7 1 0.1 3.3 1 0.0 3.5 1 0.2 3.7 1 0.1 3.7 2 0.6 SN-IDM-llEl 3.2 1 0.3 3.3 1 0.3 3.1 1 0.2 3.5 1 0.3 3.5 1 0.4 3.6 1 0.1 3.4 2 0.5

$N-IDM-13El 3.6 1 1.0 4.2 2 0.5 4.5 t 0.8 4.3 t 0.3 3.8 1 0.1 4.1 t 0.5 4.1 t 0.6

$ N-I DM- 5F 3 (ct) 3.9 1 0.3 5.3 1 0.5 4.5 1 0.3 4.04 0.2 3.9 1 0.3 4.5 1 0.8 4.5 t 0.9

$N-IDM-6GI (ct) 2.9 1 0.2 3. 5 t 0.5 3.3 s 0.3 3.01 0.3 2.8 1 0.2 3.5 1 0.1 3.2 1 0.6

$N-IDM-8GI (ct) 3.5 1 0.4 3.7 1 0.7 3.7 1 0.3 3.3 1 0.2 3.4 2 0.3 3.6 1 0.2 3.6 1 0.4 SN-IDM-IIGl (ct) 3.5 t 0.3 3.4 1 0.2 3.9 t 0.6 3.4 1 0.1 3.1 t 0.6 3.7 1 0.2 3.6 1 0.4 SN-IDM-12G1 (ct) 3.1 t 0.1 3.6 1 0.4 3.5 1 0.3 3.5 t 0.3 3.8 1 0.4 3.6 1 0.3 3.5 1 0.4 SM-IDM-12G2 (cl) 4.1 1 0.3 4.5 1 0.4 4.4 1 0.2 4.3 1 0.2 4.4 2 0.6 4.5 2 0.5 4.3 t 0.3 Avera9e 1 3.4 1 0.7 3.9 t 1.1 3.8 t 1.1 3.5 t 0.8 3.4 2 0.9 3.8 1 0.8 3.7 t 0.4 2 s.d.

The standard month = 30.4 days.

(ct) Denotes Control Location

TABLE C-18 COBLE GAS CO2CEOTRATIO35 0F KRYPTON-85 A D XEC03-133 l'% AIR SAMPLES Results in units of (pCl/m3)

LOCATION CODE - 1452 COLLECTION DATES Kr-d5 Xe-133 COLLECTION DATES Kr-85 Xe-133 12/30/86-01/06/87 30 2 1 <l20 06/30/87-07/07/87 29 2 7 <64 01/06/87-01/13/87 33 1 7 <84 07/07/87-07/14/87 33 t 7 (65 01/13/87-01/20/87 29 1 7 <95 01/14/87-07/21/87 36 1 7 <95 01/20/87-01/27/87 37 t 7 <94 07/21/87-07/28/87 30 1 7 <110 01/27/87-02/03/87 29 1 7 <85 07/28/87-08/04/87 32 1 7 <14 02/03/87-02/10/87 32 2 7 <71 08/04/87-08/11/87 34 1 7 <l10 02/10/87-02/17/87 31 2 7 <96 08/11/87-08/18/87 32 1 7 <78 02/17/87-02/24/87 31 2 7 <94 08/18/87-08/25/87 41 1 7 <79 02/24/87-03/03/87 36 1 7 <94 08/25/87-09/01/87 28 1 7 (64 03/03/87-03/10/87 31 1 7 <94 09/01/87-09/08/87 32 1 7

<p T85 03/10/87-03/17/87 33 2 7 <64 09/08/87-09/15/87 25 1 7 <74 03/17/87-03/24/87 32 2 7 <64 09/15/87-09/22/87 37 1 7 <85 03/24/87-03/31/87' 30 t 7 (87 09/22/87-09/29/87 33 1 7 <97 03/31/87-04/07/87 24 1 7 (95 09/29/87-10/06/87 38 1 7 <60 04/07/87-04/14/87 34 2 7 (110 10/06/87-10/13/87 39 1 7 <65 04/14/87-04/21/87 36 1 7 <!!O 10/13/87-10/20/87 26 1 7 <!!O 04/21/87-04/28/87 35 1 7 (86 10/20/87-10/27/87 35 t 7 <85 04/28/87-05/05/87 35 1 7 <100 10/27/87-11/03/87 34 1 7 <100 05/05/87-05/12/87 31 2 7 <86 11/03/87-11/10/87 29 1 7 <100 05/12/87-05/19/87 30 t 7 <!20 11/10/87-11/17/87 31 1 7 <100 05/19/87-05/26/87' 29 2 1 <!!O 11/17/87-11/24/87 45 2 7 <85 05/26/87-06/02/87 36 1 7 <64 11/24/87-12/01/87 33 2 7 <85 06/02/87-06/09/87 33 2 7 <57 12/01/87-12/08/87 30 1 7 <65 06/09/87-06/16/87 28 1 7 <65 12/08/87-12/15/87 30 1 7 <72 06/16/87-06/23/47 35 t 7 (95 12/15/87-12/22/87 32 1 7 <85 06/23/87-06/30/87 28 1 7 <95 12/22/87-12/29/87 34 1 7 (C5 Average t 32 t 7.8 2 sigma

TABLE C-19 TYPICAL LLDs ACHIEVED FOR GAMMA SPECTROMETRY MILE AND FISH. GAME AND AQUATIC Soll AND AIR WATER AQUATIC INVERTEBRATES PLANTS AQUATIC SEDIMENT PARTICULATES MUCLIOES (pCl/f) (pCS/kg wet) (pCl/kg dry) (pCS/kg dry) (10-3pCl/m3)

Be-7 60 80 80 200 20 Na-22 7 8 10 30 2 E-40 100 300 300 900 20 Cr-51 50 100 70 200 10 Mn-54 5 7 9 30 2 Co-58 5 8 8 20 2

Fe-59 15 20 15 50 2 0o-60 5 8 9 20 2 Zn-65 10 20 20 60 2 i Zr-95 30 10 to 40 2 i Rb-95 15 (a) (a) (a) (a) 1 Mo-99 10 10 10 20 5

)g Ru-103 7 to 10 30 2 i Ru-106 50 60 80 200 10

( Agallom 7 10 10 40 2 Sb-125 15 20 25 80 4 Te-129m 6 10 10 30 2 I-131 10 10 10 30 10 Te-132 to 6 6 25 2

. I-133 10 10 10 40 15 Cs-134 6 7 10 30 2 1 Cs-136 10 10 10 30 2 j Cs-137 6 7 10 30 2 sa-140 60 10 10 5 5 1 La-140 15 (a) (a) (a) (a)

] Ce-141 10 10 15 30 3 i Ce-144 30 40 60 150 7 Ra-226 90 100 150 400 20 Th-228 to 10 25 60 3 (a) No Tech. Spec. Requirements

TI.BLE C-20 LLD's a D REPORTI G ACil0N LEVELS - 1981 REQ 3RRED BY TEC3. SPEC 5. AID C0 TRACT SAMPLE Gross TYPE Requirements UNITS Beta H-3 Mn-54 Co-58 Fe-59 Co-60 Zn-65 Kr-85 Sr-89 ATMOSPHERIC AIRBORNE Air 5 ample LLD* Tech 5. pCl/m3 0.01 - - - - - - - -

LLD Contract 0.01 - - - - - - - .0001 RAL** Tech 5. - - - - - - - - -

RAL Contract 1 - - - - - - - 0.1 AQUATIC Fish Invertebrate LLD Tech 5. pCl/kg - - 130 130 26) 130 260 - -

Algae / LLD Contract - - 130 130 2E a 130 260 - 5 RAL Tech 5. - - 30,000 30,000 10,000 10,000 20,000 - -

RAL Contract - - 30,000 30,000 10,000 10,000 20,000 -

20 WATERBORNE Potable LLD Tech 5. pCl/f 4 3,000 15 15 30 15 30 - -

Surface LLD Contract 4 200 15 15 30 15 30 - 10 Precip. RAL Tech 5. - 30,000 1,000 1,000 400 300 300 - -

l 0$ RAL Contract 50 30,000 1,000 1,000 '400 300 300 - 20-TERRESTRIAL Food LLD Tech 5. pCl/kg - - - - - - - - -

Products LLD Contract (wet) - -- - - - - - - -

RAL Tech ". - - - - - - - -

RAL fcatract - - - - - - - - -

MILE Milk LLD Tech 5. pCl/l - - - - - - - - -

LLD Contract - - - - - - - - 5 RAL Tech 5. - - - - - - - - -

RAL Contract - - - - - - - -

20 i Sediments LLD Tech 5. pCl/kg - - - - - - - -

Solls LLD Contract (dry) - - - - - - - - 5

, RAL Tech 5. - - - - - - - - -

RAL Contract - - - - - - - -

80 NOBLE GAS LLD Tech 5. pC1/m3 - - - - - - - - -

LLD Contract - - - - - - -

25 -

RAL Tech 5. - - - - - - - - -

j RAL Contract - - - - - - - - -

I --

DIRECT LLD Tech 5. - - - - - - - -

l F35TKTlom LLO contract 1.5 mR/sto. month - - - - - - - -

I ILU

  • Lower limit of detection
    • Reporting action level

TA8tE C-20 (Cs t.)

LLD's CCD REPORTI:3 ACTICQ LEVELS - 1987 REQUIRED BY TECH. SPECS. A'ZO C0;TR ACT SAMPLE TYPE UNITS Sr-90 Zr-95 Mb-95 I-131 xe-133 Cs-134 Cs-137 Ba-140 La-140 WATER a

Potable LLD* Tech 5. pCl/t -

30 15 1.0 - 15 18 60 15 Surface LLD Contract 2 30 15 0.5 - 15 18 60 15 Precip. RAL** Tech 5. -

400 400 2 - 30 50 200 200 RAL Contract 20 400 400 2 -

30 50 200 200 AIR ITr Sample LLD Tech 5. pCl/m3 - - -

.07 -

.05 .06 - -

LLD Contract .0001 - - .07 -

.05 .06 - -

RAL Tech 5. - - -

0.9 - 10 20 - -

RAL Contract 0.1 - -

0.9 - 10 20 - -

MILE Milk LLD Tech 5. pCl/l - - -

1.0 -

15 18 60 15 LLD Contract 1 - -

0.5 -

15 18 60 15 RAL Tech 5. - - -

3 -

60 70 300 300 1

to RAL Contract 8 - -

3 -

60 70 300 300 l AQUATIC (1)

Fish Invertebrate LLO Tech 5. pCl/kg - - - - -

130 150 - -

Aquatic Plants /LLD Contract 5 - - - - 130 150 - -

3 Game RAL Tech 5. - - - - -

1.000 2.000 - -

i RAL Contract 20 - - - -

1.000 2.000 - -

FOOD Food LLD Tech 5. pCl/kg - - - 60 - 60 80 - -

Products LLD Contract (wet) - - - 60 - 60 80 - -

RAL Tech 5. - - - 100 -

1.000 2.000 - -

RAL Contract - - -

100 -

1.000 2.000 - -

SE DIME NTS/ SOIL S Sediments LLD Tech 5. pCl/kg - - - -

150 180 - -

Solls LLD Contract (dry) 5 - - - -

150 180 - -

RAL Tech 5. - - - - - - - - -

RAL Contract 80 - - - -

1.000 2,000 - -

NOBLE GAS LLO Tech 5. pCl/m3 - - - - - - - - -

LLD Contract - - - -

100 - - - -

RAL Tech 5. - - - -

100 - - - -

RAL Contract - - - - - - - - -

j

  • tower llelt of detection
    • Reporting action level (1) There are no Technical Specification requirements for game or aquatic plants. Aquatic contract LLD's and RAL's for gamma spectrometry apply to game and aquatic plants. Sr-89/90 LLD's and R AL's for aquatic plants are 30 pCl/kg (dry) "

and 45 pCl/kg (dry), respectively.

e t

APPENDIX 0 ANALYTICAL PROCEDURES SYNOPSIS 91 ,

ANALYTICAL PROCEDURES SYNOPSIS Appendix D is a snyopsis of the analytical procedures performed on samples collected for the Shoreham Nuclear Power Station's Radiological Environmental Monitoring Program. All analyses have been mutually agreed upon by Long Island Lighting Company and Teledyne Isotopes and include those requested by the USNRC Regulatory Guide 4.8, BTP, Rev.1, November 1979.

ANALYSIS TITLE PAGE G r o s s B e t a An a l y s i s o f S am p l e s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 9 3 Precipitation........................................................ 93 A i r bo r n e P a r t i c u l a t e s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 9 5 An a l y s i s o f S am p l e s fo r Tr i t i um . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 9 6 Water................................................................ 96 An alysi s of Sampl es for St ront i um-89 and -90. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 97 Total Water.......................................................... 97 Milk................................................................. 97 So i l a n d S e d i m e n t . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 9 7 Grganic Solids....................................................... 98 Air Particulates..................................................... 98 Analysis of Samples for Iodine-131....................................... 100 Milk or Water....................................................... 100 Gamma Spectrometry of Samples............................................ 101 M i l k a nd W a t e r . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 101 Dried Sol ids other th an So ils and Sediment. . . . . . . . . . . . . . . . . . . . . . . . . . 101 Fish................................................................ 101 So i l s a n d S e d i m e n t s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 101 Ch arco a l Ca r t r i d g e s ( Ai r lo d i n e) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 101 A i r b o r n e P a r t i c u l a t e s . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 101 En v i ro nme n t al 0o s ime t ry. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 103 92

l l

i DETERMINATION OF GROSS BETA ACTIVITY IN WATER SAMPLES

1.0 INTRODUCTION

The procedures described in this section are used to measure the

~

overall radioactivity of water samples without identifying the radioactive species present. No chemical separation techniques are involved.

One liter of the sample is evaporated on a hot plate. A smaller volume may be used if the sample has a significant salt content as measured by a conductivity meter. If requested by the customer, the sample is filtered through No. 54 filter paper before evaporation, removing particles greater than 30 microns in size.

After evaporating to a small volume in a beaker, the sample is rinsed into a 2-inch diameter stainless steel planchet which is stamped with a concentric ring pattern to distribute residue evenly. Final evaporation to dryness takes place under heat lamps.

Residue mass is determined by weighing the planchet before and after mounting the sample. The planchet is counted for beta activity on an automatic proportional counter. Results are calculated using empirical self-absorption curves which allow for the change in effective counting efficiency caused by the residue mass.

t 93

v .

2.0 DETECTION CAPABILITY Detection capability depends upon the sample volume actually represented on the planchet, the background and the efficiency of the counting instrument, and upon self-absorption of beta particles by the mounted sample. Because the radioactive species are not identified, no decay corrections are made and the reported activity refers to the counting time.

The minimum detectable level (MDL) for water samples is nominally 1.6 picocuries per liter for gross beta at the 4.66 sigma level (1.0 pCi/l at the 2.83 sigma level), asstning that i liter of sample is used and that 1/2 gram of sample residue is mounted on the planchet. These figures are based upon a counting time of 50 minutes and upon representative values of counting efficiency and background of 0.2 and 1.2 cpm, respectively. These figures are based upon a 200 minute counting time and upon a representative efficiency of 0.02 and a background of 0.1 cpm.

The MDL becomes significantly lower as the mount weight decreases because of reduced self-absorption. At a zero mount weight, the 4.66 sigma MOL for gross beta is 0.9 picoeuries per liter. These values reflect a beta counting efficiency of 0.38 and an alpha counting efficiency of 0.18.

I t

94

GROSS BETA ANALYSIS OF SAMPLES Air Particulates After a delay of five or more days, allowing for the radon-222 and radon-220 (thoron) daughter products to decay, the filters are counted'in a gas-flow proportional counter. An unused air particulate filter, supplied by LILCO, is counted as the blank.

Calculations of the results, the two sigma error and the lower limit of detection (LLD):

RESULT (pCi/m3 )

= ((S/T) - (8/t))/(2.22 V E) 3 2 2 TWO SIGMA ERROR (pCi/m )

= 2((S/T ) + (8/t ))l/2 (2.22

/ V E)

LLD (pCi/m3 )

= 4.66 (81/2)/(2.22 V E t) where:

S = Gross counts of sample including blank B = Counts of blank E = Counting efficiency T = Number of minutes sample was counted

  • t = Number of minutes blank was counted V = Sample aliquot size (cubic meters)

I l

95

ANALYSIS OF SAMPLES FOR TRITIUM Water Approximately 2 ml of water are converted to hydrogen by passing the t:ater, heated to its vapor state, over a granular zine conversion column heated to 400* C. The. hydrogen is loaded into a one liter proportional detector and the vol me is determined by recording the pressure.

The proportional detector is passively shielded by lead and steel and an electronic, anticoincidence system provides additional shielding from cosmic rays.

Calculation of the results, the two sigma error and the lower limit detec-tion (LLD) in pCi/f:

RESULT

= 3.234 TgV g(CG - B)/(CN Y)

S TWO SIGMA ERROR = 2((Cg + B)At)1/2 3 .234 T Y /((C Y )(Cg-B))

N N NS LLD = 4.66 (3.234)T N NYg(C )1/ /(At C g V) 3 where: T N

= triti s units of the standard 3.234 = conversion factor changing tritium units to pCi/l V

N

= volme of the standard used to calibrate the efficiency of the detector in psia V

3

= volme of the sample loaded into the detector in psia C

N

= the cpm activity of the standard of volse VN C

G

= the gross activity in epm of the sample of volme V3 and the detector volume B = the background of the detector in cpm At = counting time for the sample

' e- --- - -----4 ,. ._ _ym. _ , , . , . , , . _ . _ - . , ._

l l 1

l l

i i

ANALYSIS OF SAMPLES.FCR STRONTIUM-89 AND -90 l Water )

l Stable strontiun carrier is added to 1 liter of sample and the volume is reduced by evaporation. Strontium is precipitated as Sr(NO3 )2 using nitric acid. A barium scavenge and an iron (ferric hydroxide) scavenge are performed followed by addition of stable yttrium carrier and a 5 to 7 day period for yttrium ingrowth. Yttriun is then precipitated as hydroxide, is dissolved and re-precipitated as oxalate. The yttriun oxalate is mounted on a nylon planchet and is counted in a low level beta counter to infer Sr-90 activity. Strontium-89 activity is determined by precipitating SrC03 from the sample af ter yttriun separation. This precipitate is mounted on a nylon planchet and is covered with an 80 mg/cm2 aluminum absorber for low level beta counting.

Milk Stable strontium carrier is added to 1 liter of sample and trichlor-acetic acid (TCA) is added to produce a curd. The curd is separated by filtration and is discarded. An oxalate precipitation is performed on the filtrate and the precipitate is ashed in a muffle furnace. The ash is dissolved and strontium is precipitated as SrN03 using funing (90%) nitric acid. A barium chromate scavenge and an iron (ferric hydroxide) scavenge are then performed. Stable yttrium carrier is added and the sznple is allowed to stand for 7 to 10 days for yttrium ingrowth. Yttriun is then precipitated as hydroxide, is dissolved and re-precipitated as oxalate. The yttrium oxalate is mounted on a nylon planchet and is counted in a low level beta counter to infer Sr-90 activity. Strontium-89 is determined by precipitating SrC03 from the sample af ter yttriun separation. This precipitate is mounted on a nylon planchet and is covered with an 80 mg/cm2 aluminum absorber for low level beta counting.

Soil and Sediment The sample is first dried under heat lamps and a 10 gram aliquot is t ak en . Stable strontiun carrier is added and the sample is leached in nitric acid. The mixture is filtered and the liquid portion is reduced in volune by evaporation. Strontium is precipitated as Sr(NO )2 3 using fuming (90%)

nitric acid. A barium chromate scavenge and an iron (ferric hydroxide) scavenge are then performed. Stable yttrium carrier is added and the sample is allowed to stand for 7 to 10 days for yttrium ingrowth. Yttriun is then precipitated as hydroxide, is dissolved and re-precipitated as oxalate. The yttrium oxalate is mounted on a nylon planchet and is counted in a low level beta counter to infer S -90 activity. Strontium-89 activity is determined by precipitating SrC03 from the sample af ter yttriun separation. This precip-itate is mounted on a nylon planchet and is covered with an 80 mg/cm2 aluminum absorber for low level beta counting.

97 .

Organic Solids A 200g wet portion of the sample is dried and then ashed in a muffle furnace.

Stable strontium carrier is added and the ash is leached in nitric acid. The sample is filtered and the volume is reduced by evaporation. Strontium is precipitated as Sr(NO 3 )2 using ftening (90%) nitric acid. An iron (ferric hydroxide) scavenge is performed, followed by addition of stable yttrium carrier and a 7 to 10 day period for yttrium ingrowth. Yttrium is then precipitatd as hydroxide, dissolved and re-precipitated as oxalate. The yttrium oxalate is mounted on a nylon planchet and is counted in a low level beta counter to infer strontium-90 activity. Strontium-89 activity is deter-mined by precipitating SrC03 from the sample after yttrium separation. This precipitate is mounted on a nylon planchet and is covered with an 80 mg/cm2 aluminum absorber for low level beta counting.

Air Particulates .

Stable strontium carrier is added to the sample and it is leached in nitric acid to bring deposits into solution. The mixture is then filtered and the filtrate is reduced in volume by evaporation. Strontium is precipitated as Sr(h03 )2 using ftsning (90%) nitric acid. An iron (ferric hydroxide) scavenge is performed, followed by addition of stable yttrium carrier and a 7 to 10 day period for yttrium ingrowth. Yttrium is then precipitated as hydroxide, is dissolved and re-precipitated as oxalate. The yttrium oxalate is mounted on a nylon planchet and is counted in a low level beta counter to infer strontium-90 activity. Strontium-89 activity is detennined by precipi-tating SrC03 from the sample af ter yttrium separation.

mountedonanylonplanchetandiscoveredwith80mg/cm{hisprecipitateis altaninum absorber for level beta counting.

Calculations of the results, two sigma errors and lower limits of detection (LLD) are expressed in activity of pCi/ volume or pCi/ mass:

RESULT Sr-89 = (N/At-BC"0A )/I2'22 Y YSOF SR-89 ESR-89)

TWO SIGMA ERROR Sr-89 = 2((N/At+8 CA +0 )/At)1/2

/ (2.22 3 Y SR-89 Y 0F ESR-89)

LLD Sr-89 = 4.66((BC+0A )/At)1/2/(2.22 V Y3 0F SR-89 ESR-89)

RESULT Sr-90 = (N/At - B)/(2.22 V YiY2DF IF E)

TWO SIGMA ERROR Sr-90 = 2((N/At+B)/At)1/2 / (2.22 1 YV2 0F Y E IF))

LLD Sr-90 = 4.66(8/At)1/2/(2.22 Y Y i Y2 IF DF E) 4 98

where: N = total counts from sample (counts)

At = counting time for sample (min)

B C

= background rate of counter (cpm) using absorber configuration 2.22 = dpm/pCi V = volune or weight of sample 6nalyzed B

A

= background addition from Sr-90 and ingrowth of Y-90 B

A = 0.016 (X) + (K) EY/ abs)(IGY-90)

Y 3

= chemical yield of strontiun DF SR-89 = decay factor from the mid collection date to the counting date for SR-89 E

SR-89

= efficiency of the counter for SR-89 with the 80 mg/cm.sq.

aluninum absorber K / IF Y

= (N/At - B )Y-90 C (EY-90 Y-90 0FY-901) 0F Y-90

= the decay factor fo- Y-90 from the "milk" time to the mid count time E

Y-90

= efficiency of the counter for Y-90 IF Y-90 = ingrowth f actor for Y-90 from scavenge time to milking time IG V-90

= the ingrowth factor for Y-90 into the strontium mount from

, the = milk" time to the mid count time.

0.016 = the efficiency of measuring SR-90 through a No. 6 absorber E

Y/ abs

= the efficiency of counting Y-90 through a No. 6 absorber B = background rate of counter (cpm) l Y

y = chenical yield of yttriun l

Y 2

= chemical yield of strontiun DF = decay factor of yttritn from the milking time to the mid count time E = efficiency of the counter for Y-90 l

IF = ingrowth f actor for Y-90 from scavenge time to milking time 99

e ANALYSIS OF SAMPLES FOR 10 DINE-131 t Milk or Water Two liters of sample are first equilibrated with stable iodide carrier.

A batch treatment with anion exchange resin is used to remove iodine from the sample. The iodine is then stripped from the resin with sodium hypochlorite solution, is reduced with hydroxylamine hydrochloride and is extracted into carbon tetrachloride as free iodine, it is then back-extracted as iodide The into sodium bisulfite solution and is precipitated as palladium iodide.

precipitate is weighed for chemical yield and is mounted on a nylon planchet for low level beta counting. The chemical yield is corrected by measuring the stable iodide content of the milk or the water with a specific ion electrode.

Calculations of results, two sigma error and the lower limit of detection (LLD) in pCi/t:

RESULT

=

(N/6t-8)/(2.22 E V Y DF)

TWO SIGMA ERROR

=

2((N/6t+B)/6t)1/2(2.22 E V Y DF)

LLD

= 4.66(B/6t)1/2 /(2.22 E V Y OF) where: N = total counts from sample (counts)

At = counting time for sample (min)

- B

= background rate of counter (cpm) 2.22 = dpm/pCi V = volume or weight of sample analyzed Y

= chemical yield of the mount or sample counted DF = decay factor from the collection to the counting date E

= efficiency of the counter for 1-131, corrected for self absorption effects by the formula E

= E (exp-0.0061M)/(exp-0.0061M3 )

3 E = efficiency of the counter determined from an 3

I-131 standard mount M = mass of Pd! on the standard mount, mg 3 2

=

M mass of Pdl2 on the sample mount, mg

- -_ w.t_

GAMMA SPECTROMETRY OF SAMPLES Milk and Water A 1.0 liter Marinelli beaker is filled with a representative aliquot of the sample. The seple is then counted for approximately 1000 minutes with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performs pulse height analysis.

Dried Solids Other Than Soils and Sediments A large quantity of the sample is dried at a low temperature, less than 100*C. As much as possible (up to the total sample) is loaded into a tared 1-liter Marinelli and weighed. The sample is then counted for approximately 1000 minutes with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performs pulse height analysis.

Fish As much as possible (up to the total sample) of the edible portion of the sample is loaded into a tared Marinelli and weighed. The sample is then counted for approximately 1000 minutes with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performs pulse height analysis.

Soils cnd Sediments Soils and sediments are dried at a low temperature, less than 100*C.

The soil or sediment is loaded fully into a tared, standard 3')0 cc container and weighed. The sample is then counted for approximately six hours with a

' shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performs pulse height analysis, Charcoal Cartridges ( Air Iodine)

Charcoal cartridges are counted up to five at a time, with one positioned on the face of a Ge(Li) detector and up to four on the side of the Ge(Li) detector. Each Ge(Li) detector is calibrated for both positions.

The detection limit for I-131 of each charcoal cartridge can be determined (assuming no positive 1-131) uniquely from the volume of air which passed through it. In the event 1-131 is observed in the initial counting of a set, each charcoal cartridge is then counted separately, positioned on the face of the detector.

Air Particulate The thirteen airborne particulate filters for a quarterly composite for each field station are aligned one in front of another and then counted for at least six hours with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performs pulse height analysis.

101

0-A mini-computer sof tware program defines peaks by certain changes in the slope of the spectrum. The program also compares the energy of each peak '

with a library of peaks for isotope identification and then performs the radioactivity calculation using the appropriate fractional gamma ray abundance, half life, detector efficiency, and net counts in the peak region. The calculation of results, two sigma error and the lower 'imit of detection (LLD) in pCi/ volume or pCi/ mass:

RESULT = (S-B)/(2.22 t E V F)

TWO SIGMA ERROR = 2(S+B)1/2/ (2.22 t E V F) ,

LLO = 4.66(B)1/2/ (2.22 t E V F) .

l where: S = Area, in counts, of sample peak and background (region of spectrum of interest) i B = Background area, in counts, under sample peak, deter-mined by a linear interpolation of the representative backgrounds on either side of the peak .

t = length of time in minutes the sample was counted 2.22 = dpm/pCi E = detector ef ficiency for energy of interest and geometry of sample V = sample aliquot size (liters, cubic meters, kilograms, or gr ams)

F = Fractional gamma abundance (specific for each emitted g amma) b a

k 102

ENVIRONMENTAL 00SIMETRY Teledyne Isotopes uses a CaSO4 :Dy thertnoluminescent dosimeter (TLD) which the company manufactures. This material has a high light output, negligible thermally induced signal loss (f ading), and negligible self dosing. The energy response curve (as well as all other features) satisfies NRC Reg. Guide 4.13. Transit doses are accounted for by use of separate '

TLDs.

Following the field exposure period the TLDs are placed in a Teledyne '

Isotopes Model 8300. One fourth of the rectan and the measured light emission (luminescence) gular TLDThe is recorded. is heated at a time TLD is then annealed and exposed to a knowr, Cs-137 doss; each area is then read again.

This provides a calibration ut each area of each TLD after every field use.

The transit controls are read in the same manner.

Calculations of results and the two sigma error in net milliroentgen (mR):

RESULT = 0 = (D g+D2 +D 3 4 +D )/4 l  :

TWO SIGMA ERROR =g 2((D -D)2+(D 2 -D)2+(0 3 -0)2+(0 4 -0)2)/3) where D i = the net mR of area 1 of the TLD, arid similarly for D2, D 3, and D4 D

i =1 1 K/Rg-A ,

I t

= the instrument reading of the field dose in area 1

~

K = the known exposure by the Cs-137 source R

g

= the instrument reading due to the Cs-137 dose on area 1 A = average dose in mR calculated in similar manner as above, of the transit control TLDs I

l l

9 103

4 4

e APPENDIX E

SUMMARY

OF EPA INTERLABORATORY COMPARISONS l

104

US EPA CROSS-CHECK PROGRAM 1987 Collection Teledyne Date Medio Nuclide EPA-Results(a) Isotopes Re3ults(b) 01/09/87 Water Sr-89 25.00

  • 5.00 22.66
  • 0.58 Sr-90 25.00 t 1.50 26.00 t 0.00 01/16/87 Water Pu-239 16.70 t 1.67 14.93 1 0.42 01/23/87 Water Gross Alpha 11.00
  • 5.00 18.33 i 1.15(d)

Gross 8 eta 10.00 t 5.00 11.66 t 0.58 01/30/87 Food Sr-90 49.00

  • 10.00 50.00 2.83 (c) 1-131 78.00 t 8.00 74.00 t 1.41 Cs-137 84.00 t 5.00 91.00 t 5.66 K-40 980.00 t 49.00 984.00 t 67.10 02/06/87 Water Co-60 50.00 i 5.00 50.33 t 1.52 Zn-65 91.00 t 5.00 108.33 t 2.51(e)

Ru-106 100.00

  • 5.00 100.33 1 11.15 Cs-134 59.00 t 5.00 62.00 t 5.57 Cs-137 87.00 t 5.00 92.00 t 3.60 02/13/87 Water H-3 4209.00 2421.00 4100.00 2200.00

, 02/27/87 Milk I-131 9.00 t 0.90 8.67 t 0.58

! 03/13/87 Water Ra-226 7.30 t 1.10 7.50 2 0.10 i Ra-228 7.50 i 1.13 5.87 0.60(f) 03/20/87 Water Gross Alpha 3.00 t 5.00 3.33 t 0.58 l Gross Beta 13.00 t 5.00 14.33 2 0.58 04/03/87 Water I-131 7.00 t 0.70 6.67

  • 0.58 04/10/87 Air Filter Gross Alpha 14.00 i 5.00 18.33 t 1.15 f Gross Beta 43.00 t 5.00 42.00 t 2.64 Sr-90 17.00 t l'.50 15.66 t 0.58 Cs-137 8.00 t 5.00 8.00 t 1.00

_105, _ _ _ _ _ _ __ _ _ _ _ _ _ _ . , _ _ _ _ __

O US EPA CROSS-CHECK PROGRAM 1987 (Cont.)

Collection Teledyne Date Media Nuclide EPA-Results(a) Isotopes Results(b) 04/27/87 Lab Perf. Gross Alpha 30.00 t 8.00 36.33 t 1.52 Ra-226 3.90

  • 0.60 3.80 t 0.10 Ra-228 4.00 0.60 3.86
  • 0.25 U 5.00 t 6.00 5.00 t 0.00 Gr-Beta 66.00 5.00 56.00 t 1,73(g)

Sr-89 19.00 t 5.00 16.33 0.58 Sr-90 10.00 t 1.50 9.33 t 0.58 Co-60 8.00

  • 5.00 8.00 t 1.00 Cs-134 20.00 i 5.00 15.33 t 1.52 Cs-137 15.00
  • 5.00 12.33 t 1.15 05/08/87 Water Sr-89 41.00
  • 5.00 40.33 t 2.31 Sr-90 20.00 t 1.50 21.33 t 0.58 05/22/87 Water Gross Alpha 11.00 t 5.00 9.67 t 0.58 Gross Beta 7.00 t 5.00 8.33 i 0.58 06/05/87 Water Cr-51 41.00 t 5.00 <53.33 Co-60 64.00 t 5.00 63.00 t 4.36 Zn-65 10.00 t 5.00 <9.67 Ru-106 75.00
  • 5.00 72.00 t 11.79 Cs-134 40.00
  • 5.00 34.66 1 1.52 Cs-137 80.00
  • 5.00 79.00 t 4.36 06/12/87 Water H-3 2895.00 i357.00 2800.00 t100.00 06/19/87 Water Ra-226 7.30
  • 1.10 7.30 i 0.17 Ra-228 15.20
  • 2.28 17.23 i 0.70 06/26/87 Milk Sr-89 69.00
  • 5.00 63.67 2.51 Sr-90 35.0,0 t 1.50 39.66 t 1.15(h) 1-131 59.00 t 6.00 49.33 t 3.21(i)

Cs-137 74.00 t 5.00 77.00 t 5.20 K 1525.00 t 76.00 1533.33 i 98.15 07/24/87 Water Gross Alpha 5.00 t 5.00 6.33 1 0.58 Gross Beta 5.00 t 5.00 6.33 0.58 07/31/87 Food Sr-89 20.00

  • 5.00 18.67 i 1.15 (c)' Sr-90 30.00 t 1.50 31.00 t 1.00 1-131 80.00 t 8.00 88.00 1 10.58 Cs-137 50.00 i 5.00 57.33 2 5.51(j)

K 1680.00 t 84.00 1603.33 201.08 106 _ _ _ _ .

US EPA CROSS-CHECK PROGRAM 1987 (Cont.)

Collection Teledyne Date Media Nuclide EPA-Results(a') Isotopes Results(b) 08/07/87 Water I-131 48.00 t 6.00 58.67 t 0.58(k) 08/28/87 Air Filter Gross Alpha 10.00 t 5.00 11.00 1 1.00 Gross Beta 30.00 t 5.00 26.33 2.89 Sr-90 10.00 t 1.50 9.33 2 0.58 Cs-137 10.00

  • 5.00 9.00 t 1.00 09/11/87 Water Ra-226 9.70 t 1.46 9.70 i 0.17 Ra-228 6.30 t 0.95 7.97 1 0.29 (1) 09/18/87 Watcr Gross Alpha 4.00 t 5.00 2.67 0.58 Gross Beta 12.00 t 5.00 13.00 t 1.00 10/09/87 Water Cr-51 70.00 t 5.00 90.67 t 11.59 (m)

Co-60 15.00 t 5.00 16.33 t 0.58 Zn-65 46.00 t 5.00 50.67

  • 0.58 Ru-106 61.00 2 5.00 55.67 4.04 Cs-134 25.00 t 5.00 25.67 0.58 Cs-137 51.00 t 5.00 54.67 t 2.08 10/16/87 Water H-3 4492.00 t449.20 4: 4.00 t100.00

-10/21/87 Lab Perf. Gross Alpha 28.00 t 7.00 40.67 2 2.08 (n)

Ra-226 4.80 t 0.72 4.77 2 0.15 Ra-228 3.60 t 0.54 3.30 t 0.30 U 3.00 t 6.00 3.00 t 0.00 Gross Beta 72.00 5.00 72.67 t 1.53 Sr-89 16.00 1 5.00 14.67 t 0.58 Sr-90 10.00 t 1.50 9.67 t 0.58 Co-60 16.00 2 5.00 19.32 1 2.52 Cs-134 16.00 t 5.00 14.33 i 2.52 Cs-137 24.00 t 5.00 25.00 t 3.61 11/20/87 Water Gross Alpha 7.00 t 5.00 <1.0 (o)

Gross Beta 19.00 2 5.00 <1.0 (o) 12/04/87 Water 1-131 26.00 t 6.00 26.33 t 1.53 107

US EPA CROSS-CHECK PROGRAM 1987 (Cont.)

Collection Teledyne Date Media Nuclide EPA-Results(a) Isotopes Results(b)

Notes:

(a) EPA Results-Expected laboratory precision (1 sigma). Units are pCi/t for water, and milk except K is in mg/t. Units are total pCi for air particulate filters.

l l (b) Teledyne Results - Average i one sigma. Units are pC1/2 for water and l milk except K is in mg/l. Units are total pCi for air particulate filters.

(c) Units for food analysis are pCi/kg except K-40 which is mg/kg.

(d) No aerosol solution was added to the planchets in the final stages of preparation in order to create a more efficient counting geometry. The technicians in the alpha beta laboratory have been instructed to add the aerosol in accordance with Procedure PRO-031-1.

(e) No reason could be ascertained for the high result for Zn-65. Previous results had a normalized deviation from the known of -0.34 (10/10/86) and 0.58 (06/06/86). Therefore this does not appear to be a trend.

Further cross-checks will be studied for any problems.

(f) A new radiochemical method is being developed for this analysis which should give more accurate results.

(g) The previous two EPA beta results are 6 percent low, and our in-house beta spikes are low by about the s ue percentage. Dr. H. Jeter will re-train the analysts in transferring all sample residue into the planchets.

(h) The reported high result was due to small aliquot available for the Sr-90 analysis. Inadvertently a larger aliquot was used for another analysis leaving 40% of the nortnal volume for Sr-90. Additionally, the narrow acceptance limits defined by EPA is particularly difficult to meet. For this analysis 63% of the participants were beyond the t 3 sigma limit. -

(i) The low result is attributed to the application of the resin method rather than the hydroxide method to this analysis. The resin method is inefficient at absorbing protten-bound iodine thus leading to low results. The results obtained by GeLi were higher.

(j) The Cs-137 results in EPA Foods have typically been biased high. We are in the process of performing our annual calibrations. We are using a new Amersham mixed gamma standard rather than the most recently prepared NBS standard which is now several years old. Based on preliminary results the three Cs-137 values would be 52.1, 50.3, and 50.9, which average 51.1.

108 _ , _ , . _ _ __ __

e US EPA CROSS-CHECK PROGRAM 1987 (Cont.)

Collection Teledyne Date Media Nuclide EPA-Results(a) Isotopes Results(b)

Notes: ( Co nt. )

(k) Erroneously high electrode reading of stable iodide in sample (possibly because of interfering species such as S--) leading to erroneously low chemical yields. Af ter repeating the electrode reading, the calculated average 1-131 is 49.6 pCi/t. Technicians have been made aware to be suspicious of high electrode readings. When unusually high readings occur samples will be diluted and/or oxidized and remeasured.

(1) A new Ra-228 analytical procedure is being evaluated as a corrective action to the variability of results with current method. Tl No. 12115 and Tl No.12116 (there was not sufficient sample for a third analysis) were also analyzed by the new procedure with results of 5.9 to 7.0 pCi/l. The new method will be used for the next Radium in Water Cross- '

check samples.

(m) The data for the Cr-51 results were reviewed. The detector efficiencies appear to be correct. The other five isotopes measured in this sample were within two standard deviations indicating there is no systematic error. Chromitsn-51 is difficult to measure at this activity level because of the low branching intensity of the gamma ray and being in the high background region of the spectrum since Cr-51 has a low energy ray, (n) The reason for deviation is due to uneven distribution of residue on planchet, resulting probably because of the omission of aerosol applica-tion. The residue from the original planchets was dissolved, evaporated

. and remounted using aerosol. The counting results then became accurate (2913, 30t3, 26t3). The analysts have been reminded to use aerosol when mounting evaporated liquids.

(o) The EPA sample was not analyzed. A newly trained technician misinter-

! preted the Sample Receipt Form and proceeded to dilute and analyze instead an in-house blank of deionized water. In the future, all dilutions will be performed by the laboratory supervisor or the laboratory manager to ensure accuracy.

109

O 4

e 9

4 APPENDIX F REMP SAMPLING AND ANALYTICAL EXCEPTIONS i

110 _ _.

4 TABLE F-1 REMP EXCEPTIONS FOR SCHEDULE 0 FISH SAMPLING AND ANALYSIS DURING 1987 >

1 Date of Reason (s) for loss /  !

Location Description Sampling Exception  !

3C1 Fish 10/20/87 Samples collected did not I meet specified amount; however, all required

, analyses were performed.

Sea Robin Collected: 0.4 Kg; Required: 1.2 Kg <

l Winter Flounder Collected: 0.4 Kg; {

Required: 1.2 Kg i 13G2 Winter Flounder 10/30/37 Collected: 0.9 Kg; 7 Required: 1.2 Kg l

l i

i 111

TABLE F-2 REMP EXCEPTIONS FOR SCHEDULED INVERTEBRATE SAMPLING AND ANALYSIS DURING 1987 Date of Reason (s) for Loss /

Location Description Sampling Exception 3C1 Wheik 06/23/87 None available Various Invertebrates Samples collected did not meet specified enount; however, all required analyses were performed.

13G2 Whelk 06/24/87 Collected: 0.5 Kg Required: 1.2 Kg 14C1 Whelk 06/23/87 Collected: 0.45 Kg Required: 1.2 Kg 301 Squid 10/20/87 Collected: 0.7 Kg Required: 1.2 Kg 13G2 Squid 10/30/87 Collected: 0.5 Kg Required: 1.2 Kg 13G2 Lobster 10/30/87 Collected: 0.5 Kg Required: 1.2 Kg 13G2 Whelk 11/09/87 Collected: 0.5 Kg Required: 1.2 Kg 14C1 Squid 10/21/87 Collected: 0.8 Kg Required: 1.2 Kg 4A3 Sof t-Shell Clams 10/01/87 Collected: 0.3 Kg Required: 1.2 Kg 112

TABLE F-3 REMP EXCEPTIONS FOR SCHEDULED AIRBORNE PARTICULATE SAMPLING AND ANALYSIS OURING 1987 Date of Reason (s) for Loss /

Location Description Sampling Exception 652 Particulate Filter 12/30/86- Low voltage supply caused 01/06/87 lower than normal volume.

351 05/19/87- Power failure 06/23/87 652 05/19/87- Power failure 06/23/87 652 06/30/87- Power f ailure 12/29/87 2A3 09/22/29 Power failure; however 09/29/87 filter was collected.

Sample volume was low.

2A3 09/29/87- Power f ailure however

. 10/06/87 filterwascollected.

Sample volume was low.

2A3 10/06/87- Power f ailure l 10/20/87 l

l l 2A3 10/20/87- Power failure; however, i 10/27/87 filter was collected.

Sample volume was low.

503 12/08/87- Vacuun pump vanes broke 12/15/87 causing sampler to shut down . Filter was collected but sample volume was low.

7A2 12/08/87- Vacuum pump vanes broke 12/15/87 causing sampler to shut down. Filter was collected but sample volume was low.

113

TABLE F-4 REMP EXCEPTIONS FOR SCHEDULE 0 AIRBORNE IODINE SAMPLING AND ANALYSIS DURING 1987 Date of Reason (s) for Loss / '

Location Description Sampling Exception 652 Canister 12/30/86- Low voltage supply caused 01/06/87 lower than normal volume.

351 05/19/87- Power failure 06/23/87 6S2 05/19/87- Power failure 06/23/87 652 06/30/87- Power failure 12/29/87 1

2A3 09/22/87- Power failure; however, ,

09/29/87 canister was collected.

Sample volme was low.

2A3 09/29/87- Power failure; however, 10/06/87 canister was collected.

Sample volme was low.

l. 2A3 10/06/87- Power failure l

10/20/87 1

2A3 10/20/87- Power f ailure; however, 10/27/87 canister was collected.

Sample volume was low.

503 . 12/08/87- Vacu n p ep vanes broke 12/15/87 causing s upler to shut down. Canister was collected but sample volume was low.

7A2 12/08/87- Vacutn p a p vanes broke E!n}N$r'w#!!olkecNNbb$"'

a s u ple volume was low.

114 [

TABLE F-5

. REMP EXCEPTIONS FOR SCHEDULED MILK SAMPLING AND ANALYSIS DURING 1987 Date of Reason (s) for Loss /

Location Description Sampling Exception 681 Goat Milk 01/08/87- Goats dried up so that 12/10/87 owners could travel.

8F2 Goat Milk 01/,08/87 Goats dried up for kidding.

8F2 Goat Milk 02/09/87 Goats dried up for kidding.

8G2 Cow Milk 03/12/87 No milk available; insufficient supply.

8F2 Goat Milk 03/12/87 Goats dried up for kidding.

6B2 Goat Milk 04/13/87 No milk available.-

8F2 Goat Milk 07/09/87 No milk available, supplier forgot to prepare sample.

682 Goat Milk 08/20/87- Sampling discontinued i 12/10/87 because supplier moved out '

of area. l I

8G2 Cow Milk 09/15/87 No milk available; insufficient supply.

8G2 Cow Milk 10/01/87 No milk available; insufficient supply.

115 .

TABLE F-6 ,

REMP EXCEPTIONS FOR SCHEDULED FOOD PRODUCTS SAMPLING AND ANALYSIS DURING 1987 ,

Date of Reason (s) for Loss /

Location Description Sampling Exception B81 Lettuce, Cabbage, 06/12/87 Not available, too early Carrots, Spinach, in the season. ,

Radishes, Beets &

Onions 5C2 Lettuce, Cabbage, 06/12/87 Not available, too early

. Carrots, Spinach, in the season. ,

Radishes, Beets &

Onions 5F2 Lettuce, Cabbage, 06/17/87 Not available, too early Carrots, Spinach, in the season. >

Radishes, Beets &

Onions 783 Lettuce, Cabbage, 06/17/87 Not available, too early Carrots, Spinach, in the season.

Radishes, Beets & l Onions ,

12H1 Lettuca, Cabbage, 06/12/87 Not available, too early Carrots, Spinach, in the season. 1 Radishes, Beets &

Oniona l

12H2 Lettuce, Cabbage, 06/17/87 Not available, too early Carrots, Spinach, in the season.

Radishes, Beets & r Onions 5C2 Carrots & Radishes 07/15/87 Not available f 5F2 Lettuce, Cabbage. 07/15/87 Not available. I Carrots, Spinach, l Radishes, Beets & l Onions l 116

TABLE F-6 (Cont.)

REMP EXCEPTIONS FOR SCHEDULED FOOD l PRODUCTS SAMPLING ANC ANALYSIS DURING 1987 Date of Reason (s) for Loss /

Location Description Sampling Exception 783 Lettuce, Cabbage, 07/15/87 Farm stand closed. ,

Carrots, Spinach, Radishes, Beets & ,

Onions 12H1 Radishes, Beets, 07/15/87 Not available Lettuce & Cabbage

. I 12H2 Lettuce, Cabbage, 07/15/87 Farm stand closed.

Carrots, Spinach, [

Radishes, Beets &

Onions t 881 Lettuce & Radishes 08/13/87 Not available ,

12H1 Lettuce, Cabbage, 08/13/87 Not available Spinach, Carrots, Radishes & 8eets 12H2 Cabbage, Beets & 08/13/87 Not available Radishes L

i 5F2 Spinach, Radishes 08/20/87 Not grown locally. ,.

& Carrots F l 783 Spinach, Carrots, 08/20/87 Not grown locally.

l Radishes & Jeets 12H2 Cabbage, Radishes 08/20/87 Not grown locally. '

& Beets 5C2 Lettuce, Carrots 08/27/87 Not available [

& Beets 881 Lettuce, Spinach 08/27/87 Not available f

& Radishes ,

117 _._ __ __

TABLE F-6 (Cont.)

REMP EXCEPTIONS FOR SCHEDULED F000 PR000 CTS SAMPLING AND ANALYSIS DURING 1987 Date of Reason (s) for Loss /

Location Description Sampling Exception 12H1 Lettuce, Cabbage, 08/27/87 Farm stand closed.

Spinach, Carrots, Radishes & Beets 12H2 Cabbage, Carrots, 08/27/87 Not grown locally.

Radishes & Beets 5C2 Lettuce, Spinach, 09/16/87 Not grown locally.

Carrots & Beets 881 Spinach & Radishes 09/16/87 Not grown locally.

12H1 Lettuce, Cabbage, 09/16/87 Not grown locally.

Spinach, Carrots,

& Radishes SC2 Lettue' terrots 10/22/87 Not grown locally.

881 Cabbage, Spinach 10/22/87 Not grown locally.

& Radishes 12H1 Lettuce, Cabbage, 10/22/87 Not grown locally.

Spinach, Carrots, Radishes & Potatoes 12H2 Cabbage, Carrots, 10/22/87 Not grown locally.

Radishes, Potatoes .

& Spinach 5C2 Lettuce & Cabbage 11/30/87 Farm stand closed.

B81 Lettuce & Cabbage 11/30/87 Farm stand closed.

12H1 Lettuce & Cabbage 11/30/87 Farm stand closed.

118

4 9

APPENDIX G SNPS LAND USE SURVEYS 119

SNPS LAND USE CENSUS t

OPERATIONAL The operational program is required to comply with Section 3/4.12.2 of SNPS Technical Specifications. The technical specifications require a survey of all milk animals and gardens greater than 50m2 (500 ft2 )

producing broad leaf vegetation within a radial distance of 8 Km (5 miles).

LIL m is also required to identify the nearest milk animal, residence and garoen in each of the 16 meteorological sectors.

Environmental Engineering Department conducted the 1987 dairy animal census, during April through June. This survey was done by Environmental Technicians driving through each neighborhood within the 5 mile radial distance and visually checking for dairy animals. hhen a dairy animal was observed the technicians requested information from the owner concerning the amount of milk produced, feed, number of animals and grazing methods.

The 1987 census results indicated that there are no milk producing cows within a 5 mile radial distance from the site; however, the survey did locate the following milk, producing goats:

1. Sector 6,1.55 miles east-southeast of SNPS

. Mr. Frank Pitti Remsen Road Wcding River, New York 11792 REMP Monitoring Location - 681 (milk not being sampled; goats temporarily dried up (July 86)).

Inventory: 0 milking goats 3 non-milking goats Inventory Date: May 4, 1987

2. Sector 13,1.9 miles west of SNPS Poole Briarcliff Road Shoreham, New York 11786 REMP Monitoring Location 13B1 Inventory: 2 milking goats 6 non-milking goats Inventory Date: December 10, 1987 120
3. Sector 11, 2.40 miles southwest of SNPS '

Shoreham-Wading River School District Middle School Randall Road Shoreham, New York 11786 REMP Monitoring Location -11C1 (Milk not being sanpled due to owners decision not to participate).

Inventory: 3 milking goats 4 non-milking goats Inventory Date: May 6, 1986 t

Table G-1 lists the nearest milk animal in the sixteen meteorological sectors. Additional field survey data are filed in the Shoreham Record Retrieval System (SR2 A39.104) "Animal Census."

The Garden Census was also conducted by Environmental Engineering Technicians visually noting each garden of 50m2 (500 f tz) or greater.

The 1987 census was performed during July, August, September and October locating a total of 343 gardens. Table G-2 lists the nearest garden in the sixteen meteorological sectors. The field survey sheets and maps are filed i at Environmental Engineering Melville while a computer print listing each location is filed in SR2/A39.104 "Shoreham REMP Garden Survey 1987."

e Environmental Engineering identifies nearest residences by utilizing -

both aerial photography and visual confirmation. This years census was conducted in December. Table G-3 lists the nearest residence in ,

each meteorological sector.

(

l 121

, , , , , r- ._- ,- ,.- -._-~ , ~.e -____y. c - . - . _- - - , . _ . - . - , _ ,--- - _ -_-, -

Table G-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP) 1987 Land use Census Nearest Milk Animal (within 8 km)*

Sector Direction Location 1 N Area within sector is Long Island Sound 2 NNE None 3 NE N'ne o

4 ENE None 5 E None .

6 ESE None 7 SE None 8 SSE None 9 5 None 10 SSW None

, 11 SW Shoreham - Wading River Middle School Randall Road, Shoreham - 2.4 mi. from SNPS 12 WSW None 13 W Poole, Briarcliff Road, Shoreham - 1.9 mi.

from SNPS la WNW None l

15 NW Area within sector is Long Island Sound 16 NNW Area within sector is Long Island Sound I

  • SNPS Technical Specification 3/4 12.2 122

o Table G-2 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP) 1987 Land us Census NearestGarden(>50mgwithin8km)*

Sector Direction Location 1 N Area within sector is Long island Sound 2 NNE None 3 NE None 4 ENE Lapham, Central Rd. Wading River, N.Y.-4150' ENE of SNPS.

5 E Loggia Little Bay Rd' Wading River, N.Y.-4177' E. of SNPS.

6 ESE Rhodes Overlook Dr. Wading River, N.Y.-6477' ESE pf SNPS.

7 SE Groffman, Randall Rd./No. Country Rd.

Wading River, N.Y.-4133' SE of SNPS.

8 SSE Gracia, 9 Zophar Mill Rd., Wading River, N.Y.-5249' SSE of SNPS.

9 5 Smith, Randall Rd., Wading River, N.Y.-5965' of SNPS.

  • 10 SSW Fo11mann - 16 Defense Hill Rd., Shoreham, N.Y.-7510' SW of SNPS.

11 SW Schmidt, 25 Jomar Rd. Shoreham, N.Y.-7510' SW of SNPS.

12 WSW Mensnak - 9 Royal Way, Shoreham, N.Y.-6124' WSW of SNPS.

13 W Jehle, 2 Fordham Rd. Shoreham, N.Y. - 6127' W of SNPS.

14 WNW None 15 NW Area within sector is Long Island Sound 16 NNW Area within sector is Long Island Sound SNPS Technical Specification 3/4 12.2 123

Table G-3 RADIOLOGICAL ENVIROW4 ENTAL MONITORING PROGRAM (REMP) 1987 Land use Census Nearest Residence (within 8 km)*

Sector Direction Location / Distance from SNPS 1 N Area within sector is Long Island Sound 2 NNE Thurber-Creek Road, Wading River, 1503' from SNPS 3 NE Creek Road, Wading River,1922' from SNPS (tenth house east of 2A3) 4 ENE Creek Road, Wading River, 3444' from SNPS (fifth house west of Riverhead Town Beach) 5 E Sound Road, Wading River, 3598' from SNPS 6 ESE Bartow - Sound R6ad Wading River, 2917' from SNPS 7 SE North Country Road, Wading River, 3509' from SNPS (at REMP location 7A2) 8 SSE North Country Road, 2nd house west of Pheasant Run, Wading River, 2649' from SNPS i 9 S #20 Long Bow, Wading River, 3839' from SNPS 10 SSW Fo11mann-f16 Defense Hill Road, Wading River, 4877' from SNPS 11 SW #170 North Country Road, Wading River, 1632' from SNPS 12 WSW Gildea-Valentine Road, Shoreham, 5557' from SNPS 13 W Brice - 55 Valentine Road, Shoreham, 4620' from SNPS 14 WNW St. Joseph's Villa, Wading River, 2178' from SNPS 15 NW Area within sector is Long Island Sound 16 NNW Area within sector is Long Island Sound

  • SNPS Technical Specification 3/4 12.2

__12 4__ _ ______

1 APPENDIX H

! COMMON AND SCIENTIFIC NAMES OF SPECIES COLLECTED IN THE REMP G

125

l Table H-1 <

COMMON AND SCIENTIFIC NAMES OF SPECIES COLLECTED IN THE RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM Comon Name Scientific Name Fish Winter Flounder , Pseudopleuronectes americanus  !

Windowpane Scophthalmus aquosus Summer Flounder Paralichthys dentatus Sea Robin Prionotus spp.

Little Skate RJaerinacea invertebrates American Lobster Homarus americanus  ;

4 Squid Loligo pealeii Blue Mussel Mytilus edulis Channeled Whelk Busycon canaliculata Soft-Shell Clam Mya arenaria Oysters Crassostrea virginica Algae l Fucus sp.

Ulva lactuca e

Enteromorpha sp.

Polysiphonia sp.

Chondrus >;rispus Scytosiphon lomentaria

. Codium sp.  !

Ascophy11um sp. ,

Game i

Raccoon Procyon lotor Eastern Gray Squirrel Sciurus carolinensis l l

126 l