ML20204A251

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Annual Environ Radiological Monitoring Rept for Lapl Waterford Steam Electric Station,Unit 3,1985
ML20204A251
Person / Time
Site: Waterford Entergy icon.png
Issue date: 12/31/1985
From: Iyengar K, Lesan H, Rollins E
LOUISIANA POWER & LIGHT CO.
To: Martin R
NRC OFFICE OF INSPECTION & ENFORCEMENT (IE REGION IV)
References
W3P86-0078, W3P86-78, NUDOCS 8605090529
Download: ML20204A251 (172)


Text

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          . .s.                                                                     ENVIRONMENTAL RADIOLOGICAL MONITORING REPORT FOR THE LOUISIANA POWER AND LIGHT
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WATERFORD STEAM ELECTRIC STATION, UNIT 3 I JANUARY 1 THROUGH DECEMBER 31, 1985 E E E . I

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I I I ENVIRONMENTAL RADIOLOGICAL MONITORING REPORT FOR THE LOUISIANA POWER AND LIGHT WATERFORD STEAM ELECTRIC STATION, UNIT 3 JANUARY 1 THROUGH DECEMBER 31, 1985 I ' I I PREPARED BY: W V 9 YBA H. C. Ihsag '% ' DATE I REVIEWE BY: 24 E. M. Jkfilins ' Radia gon Control Unit Coordinator vbbc

                                                   ' DATE APPROVED BY:
                                                   }}/A .2 Co [f K. R. Iyengar                                    DATE           i Nuclear Support Manager                                         (

l I .

ABSTRACT This report is issued pursuant to Waterford 3 SES Technical Specification 6.9.1.7. Its purpose is to discuss the Waterford 3 SES Radiological Environmental Monitoring Program (REMP), present the results of the program for the year of 1935, and to evaluate the radiological impact on the environment resulting from plant operation. The Waterford 3 SES REMP collected data on environmental radio-activity levels around the Waterford 3 SES nuclear power plant. These levels were determined by analyzing samp1ss of air, water,  ! shoreline soil, fish, vegetation, and milk fron various locations l around the facility. Based on the evaluation of these analyses, the operation of Waterford 3 SES exhibited no discernable < impact on the levels of radioactivity in the environment during 1985. l I l I I / I 3 8 l E

l TABLE OF CONTENTS l 1 PAGE l ABSTRAC,. . . . . . . . . . . . . . . . . . . . . . . . . . 11 TABLE OF CONTENTS . . . . . . . . . . . . . . . . . . . . . iii  ! LIST OF TABLES . . . . . . . . . . . . . . . . . . . . . . . v l LIST OF FIGURES . . . . . . . . . . . . . . . . . . . . . . vii -

1.0 INTRODUCTION

. . . . . . . . . . . . . . . . . . . . . .                                                1 1.1 Program and Report Objectives . . . . . . . . . . .                                               1 1.2 Plant and Site Description . . . . . . . . . . . .                                                1 2.0 PROGRAM DESCRIPTION           . . . . . . . . . . . . . . . . . .                                        3 2.1 History and Development . . . . . . . . . . . . . .                                               3 2.2 Sample Collection and Handling Procedures . . . .                                        .        3 2.2.1 Direct Radiation Exposure Pathway Samples       . . . . . . . . . . . . . . . . . .                                        4 2.2.2 Airborne Exposure Pathway Samples .                                   . . . .             4 2.2.3 Waterborne Exposure Pathway Samples I              2.2.4 Ingestion Exposure Pathway Samples .

2.3 Analytical Procedures . . . . . . . . . . . . . . . 5 6 7 2.4 Laboratory Quality Assurance . . . . . . . . . . . 7 3.0 DISCUSSION OF RESULTS . . . . . . . . . . . . . . . . . 23 3.1 Direct Radiation Exposure Pathway . . . . . . . . . 23 3.2 Airborne Exposure Pathway . . . . . . I 3.2.1 Airborne Particulates 3.2.2 Airborne Iodine . . . 24 24 24 3.3 Waterborne Exposure Pathway . . . . . . . . . . . . 24 3.3.1 Drinking / Surface Water . . . . . . . . . . . 24 3.3.2 Groundwater . . . . . . . . . . . . . . . . 26 3.3.3 Shoreline Soil . . . . . . . . . . . . . . . 26 3.4 Ingestion Exposure Pathway . . . . . . . . . . . . 27  ; 3.4.1 Milk . . . . . . . . . . . . . . . . . . . . 27 1 3.4.2 Fish . . . . . . . . . . . . . . . . . . . . 28 3.4.3 Broad Leaf Vegetation . . . . . . . . . . . 28 3.4.4 Food 29

 -      3.5 Deviations / Garden Crops . . . . . . . . . . . . .

from the REMP . . . . . . . . . . . . . 29 3.5.1 Unavailable Samples 29 I 3.5.2 Missed Lower Limits of Detection . . . . . . 30 3.5.3 Changes to the REMP , . . . . . . . . . . . 30 3.6 Annual Land Use Census Results . . . . . . . . . . 31

4.0 CONCLUSION

S . . . . . . . . . . . . . . . . . . . . . . 34 I . iii

I 1 TABLE OF CONTENTS (CONTINUED) 1 PAGE APPENDIX A REMP DATA

SUMMARY

. ... . . . . . . . . . . . .                      35 APPENDIX B REMP DATA I                             . . . . .............. .

APPENDIX C

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED 41 l i LOWER LIMITS OF DETECTION . .. . . . . . . . . . . . . 138 APPENDIX D

SUMMARY

OF INTERLABORATORY COMPARISONS . . . . . 144 I APPENDIX E SYNOPSES OF ANALYTICAL PROCEDURES . . . . . . . . E-1.0 ANALYSIS OF SAMPLES FOR GROSS BETA ACTIVITY . E-1.1 Air Particulates . . . . . . . . . . . . . . 150 151 151 E-1.1 Water . . . . ... . . . . . . . . . . . . 151 I E-2.0 ANALYSIS OF WATER SAMPLES FOR TRITIUM . E-3.0 ANALYSIS OF SAMPLES FOR IODINE-131 . . . E-3.1 Milk and Water . 151 151

                                          .. . . . . . . . . . . . .               151 E-3.2 Broad Leaf Vegetation . . . . . . . . . . .                 152 E-4.0 GAMMA SPECTROSCOPY ANALYSIS . . . . . . . . . . .                  152 E-4.1 Milk and Water . ............. .                            152 E-4.2 Vegetation, Food and Garden Crops, I                     and Fish . . . ........... . . . .

E-4.3 Soils and Sediment . . . . . . . . . . . . . 152 153 i E-4.4 Charcoal Cartridges (Air Iodine) . . . . . . 153 E-4.5 Air Particulates . ............ . 153 E-4.6 Computer Software . . . . . . . . . . . . . 153 E-5.0 ENVIRONMENTAL DOSIMETRY , . . . . . . . . . . . . 154 , APPENDIX F STATISTICAL ANALYSES ............ . . 155 F-1.0 CALCULATION OF MEAN AND STANDARD DEVIATION . . . 156 F-2.0 COMPARING TWO SAMPLE POPUIATION MEANS . . . . . . 156 F-3.0 TLD MEASUREMENTS . . .............. 158 F-4.0 GROSS BETA ACTIVITY ON AIR PARTICULATE FILTERS . . . . . . ..... . . . . . . . . . 158 F-5.0 GROSS BETA ACTIVITY IN MONTHLY DRINKING , WATER COMPOSITES . . ............. . 158 i I o I J iv l l

I LIST OF TABLES PAGE I TABLE 2.1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP)

SUMMARY

. . . . . . . . . . . . . . . . . . . .                    9 TABLE 

2.2 DESCRIPTION

OF REMP SAMPLING STATION LOCATIONS . . . . . . . . . . . . . . . . . . . . . . . 10 TABLE 2.3 DETECTION CAPABILITIES FOR ENVIRONMENTAL SAMPLE ANALYSIS, LOWER LIMIT OF DETECTION (LLD) . . . . . . . 19 TABLE 3.1 1985 DIRECT RADIATION DATA ORGANIZED BY COMPASS DIRECTION AND DISTANCE FROM WATERFORD 3 SES . . . . . . 32 TABLE 3.2 1985 ANNUAL LAND USE CENSUS RESULTS . . . . . . . 33 TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM

SUMMARY

. . . . . . . . . . . . . . . . . . . .                36 TABLE B-1 QUARTERLY TLD EXPOSURES      . . . . . . . . . . . . . .           42 TABLE B-2 AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES:

GROSS BETA AND IODINE-131 ANALYSES . . . . . . . . . . 44 TABLE B-3 AIR PARTICULATE FILTERS: GAMMA ISOTOPIC ANALYSIS OF QUARTERLY COMPOSITES . . . . . . . . . . . . . . . . 64 TABLE B-4 DRINKING WATER: IODINE-131 ANALYSIS . . . . . . . 69 TABLE B-5 DRINKING WATER: GROSS BETA AND GAMMA ISOTOPIC ANALYSES ON MONTHLY COMPOSITES . . . . . . . . . . . . 71 TABLE B-5 DRINKING WATER: TRITIUM ANALYSIS ON QUARTERLY I COMPOSITES AND GAMMA ISOTOPIC ANALYSIS ON FILTERS .

                                                                        . . 83 TABLE B-7 SURFACE WATER: GAMMA ISOTOPIC ANALYSIS ON MONTHLY COMPOSITES     . . . . . . . . . . . . . . . . . .             86 l

TA'BLE B-8 SURFACE WATER: TRITIUM ANALYSIS ON QUARTERLY l COMPOSITES AND GAMMA ISOTOPIC ANALYSIS ON FILTERS . . . 98 l TABLE B-9 GROUNDWATER: TRITIUM AND GAMMA ISOTOPIC ANALYSES . . . . . . . . . . . . . . . . . . . . . . . 101 TABLE B-10 SHORELINE SOIL: GAMMA ISOTOPIC ANALYSIS . . . . . 102 TABLE B-11 MILK: IODINE-131 AND GAMMA ISOTOPIC ANALYSES . . 104 TABLE B-12 FISH: GAMMA ISOTOPIC ANALYSIS . . . . . . . . . 122 V I

LIST OF TABLES (CONTINUED) PAGE

     ' TABLE B-13 BROAD LEAF VEGETATION: IODINE-131 AND GAMMA ISOTOPIC ANALYSES . . . . . . . . . . . . . . . . . . .                                         126 TABLE B-14 FOOD / GARDEN CROPS: IODINE-131 AND GAMMA ISOTOPIC ANALYSES . . .            . . . . . . . . . . . . .    . .                             137 I      TABLE C-1 

SUMMARY

OF UNAVAIIAELE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF JANUARY l TO MARCH 31, 1986 . . . . . . . . . . . . . . . . . . . . 139 TABLE C-2

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF APRIL 1 TO JUNE 30, 1985 . . . . . . . . . . . . . . . . . . . . . 140 TABLE C-3

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF JULY l TO SEPTEMBER 30, 1985 . . . . . . . . . . . . . . . . . . 141 TABLE C-4

SUMMARY

OF UNAVAILABL3 SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF OCTOBER 1 TO DECEMBER 31, 1985 . . . . . . . . . . . . . . . . . . . 142 TABLE C-5

SUMMARY

OF UNAVAILABLE TLD MEASUREMENTS FOR THE PERIOD OF JANUARY 1 TO DECEMBER 31, 1985 . . . . . 143 TABLE D-1 US EPA CROSS-CHECK PROGRAM RESULTS FOR 1985 . . . 145 1 TABLE D-2 SEVENTH INTERNATIONAL INTERCOMPARISON OF ENVIRON-MENTAL DOSIMETER RESULTS . . . . . . . . . . . . . . . 149 ' TABLE F-1 STATISTICAL COMPARISON OF TLD MEASUREMENTS FROM STATIONS GROUPED BY DISTANCE FROM WATERFORD 3 SES . . . 160 TABLE F-2 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY ON .I AIR PARTICULATE FILTERS FOR 1985 . . . . . . . . . . . 161 i I TABLE F-3 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY IN o MONTHLY DRINKING WATER COMPOSITES FOR 1985 . . . . . . 162 TABLE F-4 STATISTICAL COMPARISON CF GROSS BETA ACTIVITY IN l MONTHLY DRINKING WATER COMPOSITES FOR 1984 AND 1985 . . 163 I  ! vi  ! l f l

LIST OF FIGURES PAGE FIGURE 2.1 REMP SAMPLE LOCATIONS WITHIN 2 MILES OF WATERFORD 3 SES . . . . . . .............. 20 I FIGURE 2.2 REMP SAMPLE LOCATIONS WITHIN 10 MILES OF WATERFORD 3 SES . . . . . .... ..... ... ... 21 FIGURE 2.3 REMP SAMPLE LOCATIONS WITHIN 50 MILES OF WATERFOPD 3 SES . . . . . . ........ ..... . 22 I I I I

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1.0 INTRODUCTION

This report describes the Radiological Environmental Monitoring Program (REMP) for the Waterford 3 SES nuclear power plant and discusses the results obtained during the calendar year 1985. The results discussed within this report were used to evaluate the radiological environmental impact resulting from the. opera-I tion of Waterford 3 SES. The submission of this report to the Nuclear Regulatory Commission fulfills the requirements pursuant to Waterford 3 SES Technical Specification 6.9.1.7. 1.1 Procram and ReDort Obiectives The overall objective of the monitoring program was to evaluate the radiological environmental impact of the plant. The evaluation included an assessment of actual or I potential exposures of humans to radioactive materials or radiation resulting from plant operation. In order to conduct this evaluation, the data analyses and interpreta-I tions contained in this report fulfilled the following specific objectives:

a. identify if any radioactive materials or radiation
  '                       in the environment was associated with plant operations E                b. compare the results obtained during the reporting B                     period-with past operational and preoperational data, when appropriate, to identify any trends or
accumulation of radioactivity in the environment;
c. estimate the maximum exposure to a member of the general public from any environmental data which indicates the presence of plant related radioac-tivity; and i
d. verify compliance, when appropriate, with
relevant federal requirements.

l 1.2 Plant and Site DescriDtion The Louisiana Power and Light company, Waterford Steam Electric Station, Unit No. 3 employs a pressurized water reactor for the production of approximately 1153 gross (1104 net) megawatts of electricity. The station uses a once

E through flow of water obtained from and discharged to the
3 Mississippi River for condenser cooling. During the period covered by this report, on March 4, 1985, the unit achieved initial criticality.

.I 1

Waterford 3 SES is located on the west bank of the Missis-sippi River at River Mile 129.6 between Baton Rouge and New Orleans, Louisiana. The site is in the northwestern section of St. Charles Parish approximately 3 miles southeast of the St. John the Baptist Parish boundary near the towns of Killona and Taft. The Mississippi River is the closest I prominent natural feature while others include Lac des Allemands, about 5.5 miles southwest of the site, and Lake Ponchartrain, about 7 miles northeast of the site. I Most of the man-made features are located on the narrow strip of dry land between the Mississippi River and the wet-lands. Near the Waterford SES site are several large industrial facilities, including Waterford 1 and 2 Steam I Electric Stations (0.4 miles northwest of the site), Little Gypsy Steam Electric Station (0.8 miles north northwest of the site, across the river from Waterford 3 SES), Beker I Industries, a fertilizer manufacturer (0.6 miles east southeast), Occidental Chemical company (0.8 miles east southeast), and Union Carbide, a chemical manufacturer (1.2 I miles east southeast). Louisiana Power and Light Company owns and operates the above mentioned steam electric stations. Major urban centers in the region of the site include New Orleans (approximately 25 miles east of the site) and Baton Rouge (approximately 50 miles west northwest). Communities I in St. Charles Parish near the site include Killona (0.9 miles west northwest), Montz (1.0 miles north), Norco (1.9 miles east), Hahnville (3.7 miles east southeast), and Destrahan (6.3 miles east southeast). Laplace (4.7 miles north) is located in St. John the Baptist Parish. i I  ! I I  : I . l 2 i

I 2.0 PROGRAM DESCRIPTION A general summary of the REMP is given in Table 2.1. Brief descriptions of the sampling stations and their locations are I given in Table 2.2. The locations of the sampling stations with respect to the Waterford 3 SES site are illustrated in Figures 2.1 through 2.3. A more detailed description of the overall REMP is discussed in the following chapter. 2.1 History and Develocuent The Waterford 3 SES REMP was initiated in April of 1983. The program evolved from the Preoperational Environmental Radiological Surveillance (PERS) Program which was conducted from 1978 through 1982. The equipment, procedures, tech-I niques, and many of the same sampling locations used during the preoperational survey were incorporated into the i operational program. The environmental data collected i during the first two years of the REMP (1983 and 1984), when  : Waterford 3 SES had not yet achieved initial critical-ity, were used to supplement the baseline data obtained . during the PERS Program. I I LP&L personnel were responsible for.the proper implementa-tion of the REMP and insuring that the program complied with , I federal regulatory requirements and Technical Specification  ! requirements. Specific responsibilities of LP&L personnel

  • included collecting (with the exception of fish samples), i preparing, and shipping of environmental samples; conducting lI environmental dosimetry measurements; reviewing analytical results reports; and preparing and submitting the annual '

Environmental Radiological Monitoring Report as well as any other relevant report to the Nuclear Regulatory Commission. i The primary contractor, Teledyne Isotopes, Inc., located in I Westwood, New Jersey, was responsibile for performing radiological analyses; conducting the initial data review; preparing quarterly and annual results reports; and over-l seeing laboratory quality assurance and control. A separate l [ contractor, Dancs and Moore, was responsible for the 1 e collection, and delivery to LP&L, of fish samples. II 2.2 Samele collection and Handlina Procedures The types of samples collected, the analyses performed, the sample collection frequencies, and the location of the sampling stations are summarized in Tables 2.1 and 2.2. The information contained in these tables is based on the r 3 'I I

I requirements in Table 3.12-1 of Waterford 3 SES Technical I Specification 3.12.1. The locations of the sampling stations with respect to the Waterford 3 SES site are illustrated in Figures 2.1 through 2.3. I the REMP Any deviations from (i.e., unavailable samples and missed lower limits of detection) observed during 1985 are discussed in Section 3.5. Changes made to the REMP during 1985 as a result of I the 3.5. annual land use census are also discussed in Section The environmental samples collected were classified into I four general categories according to exposure pathways: direct radiation, airborne, waterborne, and ingestion. The l i collection and handling procedures used to obtain these I samples are described in the following sections. The descriptions are intended to provide a concise overview of what was done rather than to be step-by-step procedures. I 2.2.1 Direct Radiation ExDosure Pathway SamDies

 ,I           Integrated external gamma exposures were determined                                 1 using thermoluminescent dosimeters (TLDs). Multi-ele-I          ment TLDs manufactured by Panasonic were placed at thirty-one locations as follows:
a. an inner ring of stations, one in each of the I , sixteen meteorological. sectors in the general area of the site boundary, I b. an outer ring of stations, one in ten of the meteorological sectors in the six to eight kilometer range from the sita, and
c. the balance placed in areas of special interest (e.g., population centers, schools, I etc.) with one area serving as a control.

The TLDs were exchanged and analyzed quarterly by LP&L . personnel. 1 2.2.2 Airborne Ernosure Pathway Sannles Samples of airborne particulates and radiciodines were collected at five locations. The locations included I four indicator stations (APP-1, APQ-1, APG-1, APC-1) and one control station (APE-30). The samples were collected using low-volume air sampling devices. The devices were designed to sample air on a continuous 4 I I

I I basis and record the volume of air sampled. The pump and metering device were housed inside a weatherproof shelter. l Airborne particulate samples were obtained by passing air through a particulate filter using the device described above. The filters were collected weekly by I LP&L personnel and sent to the contract laboratory for gross beta analysis. These filters were composited by the contract laboratory on a quarterly basis for analysis by gamma spectroscopy. Airborne iodine sampling was done in conjunction with I air particulate sampling. After the air passed through the particulate filter, it passed through a charcoal cartridge to collect airborne iodine. The cartridges were collected weekly by LP&L personnel and sent to the I contract laboratory for iodine-131 analysis by gamma spectroscopy. 2.2.3 Waterborne Ernosure Pathway Samoles I The Mississippi River is the major source of drinking water in the vicinity of Waterford 3 SES and it is also i the surface water into which the plant discharges. I Therefore, water samples taken from the Mississippi River were designated as both drinking water and surface water samples. Composite drinking / surface water samples were obtained from the Mississippi River using automatic composite samplers placed at one upstream (DWP-7) and two I downstream (DUG-2, DWE-5) locations from the plant. These composite water samples were collected biweekly by LP&L personnel. LP&L personnel acidified the I samples with hydrochloric acid and added sodium bisulfite (to prevent protein binding of iodine) prior to shipment to the contract laboratory. The contract laboratory analyzed the biweekly samples for iodine-131. The biweekly samples were composited on a monthly basis by the contract laboratory for gross beta and gamma spectroscopy analyses. The samples were I also composited on a quarterly basis for tritium analysis. Due to the high water table resulting from shallow I aquifers in the vicinity of the site, groundwater discharge could be sampled from a drainage canal. Groundwater samples were obtained quarterly by LP&L personnel from one sampling location (GWJ-1) using a 5 I I

'I grab sampling technique. The samples were acidified with hydrochloric acid and had sodium bisulfits added prior to shipment to the contract laboratory for , tritium and gamma spectroscopy analyses.

    ~

' Shoreline soil samples were obtained semi-annually by LP&L personnel from two sampling stations. One station a s located on the shoreline of the Mississippi River (t'iWE-3) and the other was located on the shoreline of the 40-Arpent canal (SHWJ-1) . Station SHWJ-1 was not 'I ad. led to the REMP until the second half of 1985 and therefore only one sample was obtained. The samples collected were shipped to the contract laboratory without further processing. I 2.2.4 Incestion Exnosure Pathwev sammles Milk samples were collected semi-monthly by LP&L I personnel. Control samples were obtained through Louisiana Nuclear Energy Division personnel from the Louisiana State University Department of Agriculture (MKQ-50) located in Baton Rouge, Louisiana. Indicator samples were collected locally from two stations (MKQ-5, MKE-4). All samples had sodium bisulfite added (to inhibit protein binding of iodine) prior to I shipment to the contract laboratory for iodine-131 and gamma spectroscopy analyses.

 'a     Fish samples were collected upstream (FH-1) and
>g      downstream (FH-2) from the plant by a contractor. The fish were obtained by netting. The contractor seg-regated the samples by species and location sampled prior to delivery to LP&L.       The samples were shipped I     frozen to the contract laboratory        for annlysis by gamma spectroscopy.

LP&L personnel collected broad leaf vegetation samples monthly by obtaining cuttings taken at least one inch I

  • above the ground. Samples were collected from two indicator locations (BLB-1, BLQ-1) and from one of two control locations (BLH-10, BLK-15). The samples were shipped to ,.he contract laboratory without further i processing.

l A food / garden crop sample (soybeans) was collected by I LP&L personnel from one location (FPP-1) . The sample was collected by normal harvesting techniques at the time of harvest. The sample was sent to the contract

                                                                         ,i laboratory without further processing for iodine-131             !

l and gamma spectroscopy analyses. , 6 I f 1 I

l I 2.3 Analvtical Procedures Brief synopses of the analytical procedures used by Teledyne I Isotopes and LP&L are given in Appendix E. These synopses are intended to provide an overview of what was done rather than to be step-by-step procedures. The minimum sensitivities for the analytical procedures used in the REMP are reflected by the Lower Limits of Detection (LLD) values presented in Table 2.3. These values are the I same as the ones given in Table 4.12-1 of Waterford 3 SES Technical Specifh ation 4.12.1. The LLD's are a criori estimates based on assumed sample volumes, counting times, I detector efficiencies, etc. These values reflect the lower levels of detection that were to be attained for the majority of the analyses performed. Deviations from the assumptions used in calculating these estimates (i.e., I different sample volumes, counting times, etc.) caused some actual values to be higher than the ones given in Table 2.3. All analyses that could not achieve these lower limits of detection are discussed in Section 3.5. 2.4 Laboratory cuality Assurance Teledyne Isotopes performed a variety of quality assurance I analyses. The types consisted of spiked and blank samples prepared in-house; spiked samples sent by customers or by a second laboratory under contract to a customart and EPA and I NRC samples sent by the originator to customers and then sent to Toledyne Isotopes. Also certain customers have either 5% or 10% of their samples analyzed in duplicate. It has been estimated that at Teledyne Isotopes, 5% of all analyses are for quality assurance purposes. Teledyne Isotopes also participates in the EPA radiological I interlaboratory comparison (cross-check) program. Parti-cipation in this program involves a number of analyses on various sample media as found in most REMP's. As a result of participation in the program an objective measure of t I

  • analytical precision, accuracy,,and an estimation of bias can be obtained. In the event that any results obtained by l

Teledyne Isotopes were not within control limits, as speci-fled by the EPA, an investigation was conducted to determine , the cause and correctiva action was taken to prevent a l recurrence. Appendix D lists the 1985 results of Teledyne Isotopes participation in the crosscheck program. l In 1984 and 1985, LP&L participated in the Seventh and t Eighth International Environmental Dosimeter Intercomparison Project sponsored jointly by the Department of Energy, the , l 7 I

P I  ! I Nuclear Regulatory Commission, and the Environmental Protection Agency. Results of LP&L's participation in this f l comparison program for 1984 are presented in Appendix D.  ; I The results for 1985 will not be available until some time during 1986. These results will be presented and discussed in the 1986 Environmental Radiological Monitoring Report. I I I I I . I. I i I I I . I I I - i 8 l I

E E 4 E E E E E E E E E E E E l TABLE 2.1 .

                                                                                               "                RADIOLOGICAL ENVIRONMENTAL g ITORING PROGRAM (REMP) SIR 9tARY Sample Type                                     Location                       Analysis                    Frequency Direct                                  A-2,  B-1,  C-1, D-2, E-1,             TLD gamma                   Quarterly Radiation                               F-2,  G-2,  H-2, J-2, K-1, L-1,  M-1,  N-1, P-1, Q-1, R-1,  A-5, B-4,  D-5, E-5, F-4, G-4, H-6, P-6, Q-5, R-6, F-9, 3-9, E-15, J-15, E-30 Radiciodine and                          APP-1, APQ-1, APG-1,                   Cross beta, I-131           Weekly Particulates                            APC-1, APE-30                          y isotopic                  Quarterly composite Drinking Water                           DWG-2, DWE-5, DWP-7                    H-3                         Quarterly composite e

Gross beta, y isotopic Monthly composite I-131 Bi-weekly composite Surface Water SWG-2, SWE-5, SWP-7 H-3 Quarterly composite y isotopic Monthly composite Ground Water GWJ-l y isotopic, H-3 Quarterly Shoreline Sediment SKWE-3, SHWJ-l y isotopic Semi-annually Milk MKE-4, MKQ-5, MKQ-50, y isotopic, I-131 Semi-monthly / monthly , MKQ-1 Fish FH-1, FH-2 y isotopic In season or semi-annually Food Products FPP-1 y isotopic At harvest time Broad Leaf BLQ-1, BLB-1, BLH-10, BLK-15 y isotopic, I-131 Monthly When milk samples not collected

4. Based on requirements in Table 3.12-1 of Waterford 3 SES Technical Specification 3.12.1.
b. Drinking and surface water samples are identical.

I i

l TABLE 2.2  ! DESCRIPTION OF REMP SAMPLING STATION LOCATIONS I l I LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION t t Direct Radiation (TLD)  ; A-2 (Eastbank) On fence enclosure 1.1 N I surrounding water tower west of Little Gypsy opposite Etienne St. Access from River Road (LA 628). I The TLD's are located on the (S) I fence opposite the entrance gate to the water tower. l I B-I (Eastbank) On fence enclosing the-transmission tower 0.3 miles west (up-river) from Little Gypsy. 0.8 NNE Access from River Road (LA 628). TLD's are located at SW corner of  ! fence enclosure. , I C-1 (Eastbank) On fence enclosing the Little Gypsy Cooling Water Intake. 0.8 NE I Access is from River Road (LA 628) I across from Little Gypsy Power Station entrance. TLD's are on the south side (inside) of the Cooling i Water Intake fence enclosure, ' directly opposite the entrance gate. D-2 (Eastbank) Located at USGS Witness 1.1 ENE I Post Survey Marker approximately 0.3 miles east of Little Gypsy Power Station. Access from River Road (LA 628) near the west end of the I # Bonne Carre Spillway. TLD's are on the back of the Survey Marker Sign (located on levee). , E-1 (Westbank) Located on utility pole 0.2 E along River Road (LA 18) approxi-I mately 0.3 miles east of Waterford 3 plant entrance. Access from LA

18. TLD's are on the third utility l

I pole east of the construction entrance road.

                                                                                 'e t f,

S 10

TABLE 2.2 (CONTINUED) E LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION F-2 (Westbank) Located on fence 1.1 ESE enclosure surrounding the LP&L substation on LA 3142. Access I from LA 3142 approximately 0.2 miles south of LA 18. TLD's are on the southeast corner of the fence enclosure. G-2 (Westbank) Located on utility pole 1.2 SE on East side of LA 3142 near Witco I entrance gate (Next to Union Carbide Star Plant Gate 3). Access from LA 3142 approximately 0.2 miles north of railroad overpass. H-2 (Westbank) Located on fence enclosure 1.2 SSE to shell road off of LA 3142. Access 'I from LA 3142 south of railroad overpass on east side of LA 3142. TLD's are on the south side of the gate for shell I road. (Just south of Texaco pipeline station) J-2 (Westbank) Located on northeast 1.3 S I corner of fence enclosing Texaco valve station south of LA 3127. Access from LA 3127, approximately I 0.6 miles west of LA 3127/3142 intersection. I K

  , -1      (Westbank) Located behind " Private Road" sign at Gate 8 entrance off of LA 3127. Access from LA 3127, 1.0      SSW        .

approximately 1.3 miles west of I LA 3127/3142 intersection. (Gate 8 is the access to the Waterford 3 switchyard station) L-1 (Westbank) located behind " Private 1.0 SW Road" sign at LP&L Gate 9 entrance I off of LA 3127, approximately 1.6 miles west of LA 3127/3142 inter-section. (Gate 9 is an access road for Waterford 3) 11

TABLE 2.2  : (CONTINUED) I LOCATION LOCATION MILES FROM SECTOR  ; NUMBER DESCRIPTION PLANT DIRECTION I M-1 (Westbank) Located on south gate into the Waterford I and 2 fuel 0.7 WSW t oil storage tank enclosure. I Access is either thru LP&L Gate 8, Gate 9 off of LA 3127, the shell access road from LA 18 between i Waterford 3, or thru the Waterford  ; I and 2 access road. I N-1 (Westbank) Located behind the "No 0.9 W Trespassing" sign off on Short  ! Street, in Killona, just south of  ! the entrance to Killona Elementary [ I P-1 School. (Westbank) Located behind "No 0.8 WNW L Trespassing" sign on Short Street, I in Killona, approximately 0.1 miles south of air sample station. I Q-1 (Westbank) Located on fence 0.8 NW enclosing air sample station i approximately 0.5 miles west of i I Waterford I and 2 on River Road (LA 18). t R-1 (Westbank) Located on fence 0.5 NNW I enclosure for Waterford 1 and 2 Cooling Water Intake Structure. l Access is from River Road (LA 18) I opposite Waterford 1 and 2. l

 '         TLD's are on the southwest corner                         !

of fence. j A-5 (Eastbank) Located on utility 4.5 N j pole just east of the Shady Nook , Trailer Park on Hwy 61 in Laplace. t TLD's are on second utility pole  ; east of trailer park on north side  ; of Hwy 61 (eastern end of La Place). I 12

ll  ! 1 TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR , NUMBER DESCRIPTION PLANT DIRECTION l B-4 (Eastbank) Located on utility pole 3.8 NNE just east of shell access road to South Central Bell transmission tower on south side of Hwy 61. Transmission tower is just east of Weigh Station at St. John /St. Charles Parish line. TLD's are on first utility pole east of access road. D-5 (Eastbank) Located on fence gate 4.2 I ENE on shell access road to Big 3 Chemical Plant. Shell access road is approximately 0.1 miles west of Hwy 61/48 intersection (at black and yellow gate). TLD's are on { fence gate 0.1 miles north on shell access road from Hwy 61. E-5 (Eastbank) Located on the'Norco 4.2 E Substation fence enclosure. Access from River Road (LA 48) onto Wesco St. (adjacent to Norco Shell Chemical Plant), take Wesco St. to the dead end. TLD's are located on sixth fence post south of the north substation gate. F-4 (Westbank) Located on utility pole 3.5 ESE behind blonde brick house on Aquarius St. in Hahnville. Access I , from River Road (LA 18) and turn onto Oak St. Follow Oak St. to Hickory St., turn right on Hickory St. and follow to Aquarius St. and turn left. Blonde brick house is second house on right (west) side of Aquarius St. heading south. G-4 (Westbank) Located on railroad sign 3.2 SE northwest side of LA 3160/ railroad track intersection. Access from either LA 3127 or River Road (LA 18) , onto LA 3160. 13

TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION H-6 (Westbank) Located on a construction 5.7 SSE sign on the southwest side of the second canal bridge east of LA 3160 along LA 3127. P-6 (Westbank) Located on utility pole 5.5 WNW i at southwest corner of LA 640/ railroad track intersection. ' Utility pole is just west of LA 640 and east of radio transmission tower. Q-5 (Westbank) Located on fence post 5.0 NW surrounding (green) river marker on levee just east of Edgard. Fence post is located along River Road (LA 18) across from the Webre's house. R-6 (Eastbank) Located on fence 5.3 NNW enclosing LP&L Laydown Yard on LA 3223 in Laplace. Access from Hwy 61 onto Elm St. (LA 3223), take Elm St. to the northeast corner of LA 3223/ railroad inter-section. TLD's are located on the southeast corner of fence enclosure. F-9 (Eastbank) Located on entrance 8.2 ESE gate to Destrehan Substation Access from River Road (LA 48), I ' approximately 0.3 miles east of Luling-Destrehan Ferry, onto Destrehan Road (west of Bunge Corp. Grain Elevator), and proceed to substation gate. G-9 (Westbank) Located on back fence 8.1 SE l I of LP&L District Office in Luling. Access via Ellingto m . from either River Road (LA 18); or Second or Third St. from Paul Mallard Rd. (LA 52) to Ellington , St. 0 14

I y TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION I E-15 (Eastbank) Located on Kenner Substation fence enclosure. Access from either River Road 11.8 E (LA 48) or Hwy 61, turn onto Alliance Ave. TLD's are located on the north side of the fence enclosure, near a light pole. J-15 (Westbank) Located on fence 12.0 S enclosure surrounding LP&L , switchyard at LA 631/ Hwy 90 - intersection in Des Allemands. TLD's are on the northwest corner of fence. Access from l LA 631 via shell road. E-30* (Westbank) Located on fence at 27.0 E I LP&L General Office on Delaronde St. in Algiers. TLD's are or. the fence, facing the Mississippi River, in the passageway to the transformer shop. -- Airborne APP-1 (Westbank) Located in soybean 0.8 WNW field at northwest corner of Short St. in Killona. APQ-1 (Westbank) Located at northwest 0.8 NW corner of soybean field on east

                 '         side of Killona. Access from River Road (LA 18) approximately 0.6 miles east of LA 18/3141 intersection.

APG-1 (Westbank) Located at the north 0.5 SE side of the Secondary Meteorology Tower. 15

TABLE 2.2 (CONTINUED) LOCATION I NUMBER LOCATION DESCRIPTION MILES FROM PLANT SECTOR DIRECTION I APC-1 (Eastbank) Located inside the Little Gypsy Cooling Water Intake Structure fence enclosure. 0.8 NE APE-30* (Westbank) Located on the roof of 27.0 E the LP&L General Office building on Delaronde St. in Algiers. Waterborne DWG-2 (Westbank) Located at the Union - 2.0 ESE SWG-2 Carbide drinking water canal. Access from LA 3142 through Gate 28. DWE-5 (Eastbank) Located at the 4.5 E SWE-5 St. Charles Parish Waterworks I off of River Road (LA 48) near New Sarpy. DWP-7* (Westbank) Located at the St. 6.5 NW SWP-7* John Parish Waterworks off { of LA 18 in Edgard. SHWE-3 (Westbank) Located at the Foot 3.0 ' I Ferry Landing off of LA 18 in Taft. E i SHWJ-1 (Westbank) Located at 40 Arpent 0.3 S . Canal South of the Plant. Access from LA 3127 through LP&L Gate 8. ' The canal is northwest of the '

    '         shell access road / railroad track                                                                       ;

intersection. I GWJ-1 (Westbank) Located at 40 Arpent Canal south of the plant. Access from LA 3127 through LP&L Gate 8. 0.3 S I The canal is northwest of the shell access road / railroad track inter-section. I 16

I TABLE 2.2 (CONTINUED) I LOCATION NUMBER LOCATION DESCRIPTION MILES FROM PLANT SECTOR DIRECTION Ingestion Milk MKE-4 (Westbank) Located .8 miles west 4.0 E of the Time Saver in Hahaville off of River Road. MKQ-1 (Westbank) 1.0 miles west of 1.0 NW Waterford 3 at the corner of River Road and Post Street in Killona. MKQ-5 (Westbank) Located at the Webre's 5.0 NW house, just across LA 18 from river marker, at the eastern end of Edgard. I MKQ-50* (Eastbank) Located at the LSU Dairy in Baton Rouge. 52 NW Fish FH-1* Upstream of the plant intake structure. FH-2 Downstream of the plant intake structure. i Broad Leaf BLQ-1 (Westbank) Located between LA 18 0.8 NW  ! i

                          ,                 and soybean field on eastern edge of Killona, near air sample station                                        !

APQ-1. BLB-1 (Eastbank) Located at wooded ares 0.8 NNE at the southwestern corner of the LP&L Little Gypsy plant along River Road. I I . l 17 l __ _ _. _. - . - . -.

TABLE 2.2 (CONTINUED) l 1 LOCATION LOCATION MILES FROM SECTOR l NUMBER DESCRIPTION PLANT DIRECTION I BLN-10* (Westbank) Located under overhead transmission lines along LA 633. 9.5 SSE BLK-15* (Westbank) Located 3.5 miles SSW 15 SSW of Des Allemands on Hwy. 90. Food Products FPP-1 (Westbank) Located in soybean 0.8 kW ' I field on eastern edge of Killona,- between air sample stations APP-1 and APQ-1. l

  • DENOTES CONTROL LOCATION I ,

I I \ I 18

i 'I TABLE 2.3 ( DETECTION CAPABILITIES FOR ENVIRONMENTAL SAMPLE ANALYSIS LOWER LIMIT OF DETECTION (LLD)(*) WATER FISH MILK FOOD PRODUCTS ( SEDIMENT ANALYSIS (pCi/2) AIRBORNEPARTICp)TE OR GAS (pCi/m (pCi/kg, wet) (pCi/1) (pCi/kg, wet) (pCi/kg dry) gross beta 4 0.01 H-3 2000 Ma-54 15 130 Fe-59 30 260 Co-58,60 15 I 2n-65 30 130 260 Zr-Nb-95 15 d I-131 I 0.07 1 60 Cs-134 15 0.05 130 15 60 150 Cs-137 18 0.06 150 18 80 180 Ba-La-140 15 15 I a. From Table 4.12-1 of Waterford 3 SES Technical Specification 12.4.1.

b. Applicable to broad leaf vegetstion.

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3.0 DISCUSSION OF RESULTS Analytical results for the year 1985 are discussed in this section by exposure pathway, type of sample, and analysis performed. The analytical results of the REMP are summarized in Appendix A and data for the individual analyses are presented in the tables of Appendix B. The radioactivity values summarized in Appendix A do not include any from naturally occurring radioac-tivity. 3.1 Direct Radiation Ernosure Pathway The average exposures on both control and indicator Thermo-luminescent Dosimeters (TLDs) were 16, 19, 16, and 15 mrem per standard quarter (90 days) for the first, second, third, and fourth quarters of 1985, respectively. The average of 112 TLD exposures for all of the indicator locations was 17 mram/ standard quarter compared to 21 aren/ standard quarter for the average of four exposures at the control location. The lowest and highest individual exposures were 13 and 27 mrom per standard quarter for all locations. Note that the exposure for station J-2 during the first quarter of 1985 was 32 mram per standard quarter. Upon investiga-tion it was found that radiography was performed in the vicinity of station J-2 by the company which owns the property on which the TLD is located. The results obtained " from this TLD were deemed to have been affected by the radiography and therefore the datum was not included in the I evaluation. , Table 3.1 compares the TLD results by direction and distance from the facility. The average exposure rate from TLD's

                                                                           )

located within two miles from the plant was statistically lower than the average exposure from stations located more than five miles from the plant using the standard "t" test (see Appendix F). The average exposure rate from TLD's located between two and five miles from the plant was statistically the same as the average exposure rate from stations located more than five miles from the plant. Therefore, Waterford 3 SES operation did not have a detect-able impact on direct radiation exposures from gamma radiation. 23

, 3.2 Airborne ExDosure Pathway 3.2.1 Airborne Particulates Gross beta activity ranged from 0.0034 to 0.083 pC1/ cubic meter with an average of 0.021 pCi/ cubic meter for 253 measurements from all five sampling loca-tions. The average gross beta activity for the control location, APE-30, was 0.022 pCi/ cubic meter compared to 0.021 pCi/ cubic meter for the four indicator locations I (APP-1, APQ-1, APG-1, APC-1). The control station average is statistically the same as the average from each indicator station using the standard statistical "t" test (see Appendix F). The gross beta activity results obtained during 1985 are consistent with those from the preoperational program. During the preoperational survey, in periods not significantly influenced by nuclear weapons , detonations, the gross beta activity ranged between I 0.02 and 0.04 pCi/ cubic meter. During the first two years of the REMP prior to Waterford 3 SES operation, the average gross beta activity for all stations was I 0.021 pCi/ cubic meter with a range of 0.006 to 0.5 pCi/ cubic meter. I Gamma spectroscopy results indicated detectable levels I of cosmogenically produced beryllium-7 and potas-slum-40 in the twenty quarterly composites. No j man-made radionuclides were detected above their respective lower limits of detection. 3.2.2 Airborne Iodine All of the 255 airborne iodine-131 results were below the lower limit of detaction which ranged from 0.01 to 0.6 pCi/ cubic meter. The variability of the lower limit of detection was due primarily to the difference between air sample volumes. 3.3 Waterborne Exnosure Pathway 3.3.1 Drinkina/ Surface Water I As mentioned previously, drinking water is considered synonymous with surface water. Results obtained from samples collected and analyzed as drinking water can be I designated " surface water results". Therefore, the results of the monthly and quarterly gamma spectral

1 I analyses as well as the quarterly tritium analysis reported as drinking water results are the same as for those reported as surface water results. i Seventy-six composite drinking / surface water samples were analyzed by a radiochemical procedure for 'E iodine-131. All measurements were below the lower 'g limits of detection. The samples were composited on,a monthly basis and analyzed by gamma spectroscopy. Only naturally occurring potassium-40 was detected. No I man-made gamma emitters were detected above their respective lower limits of detection. I The monthly composites were then filtered through a Whatman number 54 filter and a gross beta analysis performed on the filtrate. Gross beta activity was detected in all of the thirty-six composites with an average activity of 6.2 pci/ liter. The average activity for the control location was 5.7 pCi/ liter, compared to the averages of 7.9 and 5.0 pCi/ liter for indicator stations DWG-2 and DWE-5, respectively.

 'g The average gross beta activity detected at indicator station DWE-5 is statistically the same as that of the E                             control station DWP-7 using the standard "t" test (see Appendix F). The average gross beta activity at station DWG-2, two miles downstream, is statistically I                             larger than the control station average using the same statistical test. However, the difference between gross beta results for stations DWG-2 and DWP-7 was I                             also   observed prior to Waterford 3 SES operation during 1984. Therefore the difference in measurements between stations DWG-2 and DWP-7 appears to be the result of l

some factor other than Waterford 3 SES operation. In order to test this assumption, the numerical differences between control and indicator station I monthly gross beta results were calculated and compared

                                  * . - the years 1984 and 1985. A detailed discussion of '.his comparison is presented in Appendix F. Based on the results of this comparison, the difference I
  • in gross beta activity between control station DWP-7 and indicator station DWG-2 were deemed to be unrelated to the operation of Waterford 3 SES.

Drinking / surface water samples were also composited quarterly and analyzed for tritium. All measurements were below the respective lower limits of detection. Although not required in the REMP the filters obtained from the gross beta analysis were composited quarterly I and analyzed by gamma spectroscopy. No man-made gamma, 25 e i l

I' emitters were detected above their respective lower limits of detection. 3.3.2 Groundwater Four groundwater samples were collected from one sampling location, GWJ-1, and analyzed for tritium and gamma ray emitters. All measurements were below the lower limits of detection. 3.3.3 Shoreline Soil I Three shoreline soil samples were collected from two sampling locations: two samples from the Mississippi River shoreline downriver of the plant (SHWE-3) and one sample from the shoreline of a drainage canal into which turbine building sumps are discharged (SHWJ-1). The latter location was added to the REMP during the second half of 1985. Naturally occurring potassium-40, radium-226, and thorium-228 were detected in all of the samples. Man-made radioactivity, cesium-137, was detected in the sample obtained from station SHWJ-l at a concentra-tion of 99 pCi/kg(dry). No other man-made radio-nuclides were detected in any of the samples. Radioactive release permits for the year 1985 show that no casium-137 was discharge into the drainage canal from which the sample came. Therefore, the presence of the cesium-137 is most likely attributable to fallout from past nuclear weapons detonations. This assumption is consistent with observations made during the preoperational survey for soil samples collected from the shoreline of the Mississippi River. During the preoperational program, cesium-137 was detected in 13 of 18 soil samples at concentrations ranging between 30

               ,       and 890 TCi/kg(dry) with an average concentration of 138 pC1/ia(dry).

However, conservatively assuming that all of the cesium-137 activity detected in the shoreline soil at station SHWJ-l originated from the plant, the maximum I dose to a member of the general public was calcu-lated. The methodology and assumptions used to calculate the maximum dose were based on the guidance provided in Regulatory Guide 1.109 (10/77). The dose f I 'I

l l I i i to the maximum exposed individual, a teenager, was  ! calculated by the following equation: I i (1) R = (40) (C) (U) (D) where: R is the annual dose to the skin or the total body in aram/ year; 40 is the area-mass conversion factor given in Appendix A of Regulatory Guide 1.109 in . kg/ square meter; l l C is the radionuclide concentration in the l shoreline soil sample in pCi/kg; U is the maximum exposure time given in Table E-5 of Regulatory Guide 1.109; 67 hours for a teenagor; and i D is the external dose conversion factor for I standing on contaminated ground given in Table E-6 of Regulatory Guide 1.109; the i values for exposures resulting from cesium-137 to the skin and total body are 4.9E-09 and 4.2E-09 aren/hr per pCi/ square meter, respectively. Using Equation (1), the maximum annual dose to a teenager spending 67 hours at the shoreline of the I canal was calculated to be approximately 0.001 mram/yr to the skin and to the total body. Therefore, any radiological impacts to the general public resulting I from cesium-137 detected in the shoreline soil are infinitesimal. 3.4 Incestion Ernosure Pathway 3.4.1 H1D; Fifty milk samples were collected from three sampling locations and analyzed by a radiochemical procedure for I iodine-131. All measurements were below the lower limits of detection. The samples were also analyzed by gamma spectroscopy. Naturally occurring potassium-40 was detected in all samples. All man-made gamma 27 )

i I emitters were below their respective lower limits of detection. , i 3.4.2 Fish i Twelve fish samples, five upstream and seven downstream of the plant, were collected and the edible portions i analyzed by gamma spectroscopy. Naturally occurring potassium-40 was detected in all samples. No man-made i gamma emitters were detected above their respective  ; lower limits of detection. j I 3.4.3 Broad Leaf Vecetation i I Waterford 3 3ES Technical Specification 3.12.1 requires broad leaf vegetation to be sampled in the event milk samples are unavailable. Since milk samples could be l collected reliably from only one sampling location l within five miles of Waterford 3 SES, broad leaf I vegetation was sampled monthly at two indicator locations. Broad leaf vegetation was also collected from one of two control locations when milk from a control location was unavailable. l Twenty-seven broad leaf vegetation samples were collected and analyzed by a radiochemical procedure for iodine-131. All measurements were below the lower I limits of detection. The samples were also analyzed by gamma spectroscopy. Naturally occurring radionuclides wei , detected in all of the samples. Cesium-137 was dateted in two of the control samples at an average .I concuntration of 33 pCi/kg(wet). This man-made activity is most likely attributable to fallout from past nuclear weapons detonations. The cesium-137 concentrations detected in the control samples are consistent with preoperational results. t I , During the preoperational program, cesium-137 was occasionally detected at concentration ranging between 27 and 140 pCi/kg(wat) with an average concentratica of 70 pCi/kg. No dose calculations were performed for these results since the activity was detected at a m control location and could not attributed to Waterford 3 SES operation. I , I . 3 I

l 3.4.4 Food / Garden Croos one food / garden crop sample was collected and analyzed I by a radiochemical procedure for iodine-131. Iodine-131 was below the lower limit of detection. The sample was also analyzed by gamma spectroscopy. Naturally occur-ring potassium-40 was the only radionuclide detected. I All man-made gamma emitters were below their respective lower limits of detection. Il < 3.5 Deviations from the REMP I 3.5.1 Unavailable Samoles During 1985 deviations from the REMP sampling schedule occurred. All of the deviations (with the exception 'E of those associated with TLDs) were either the result E of equipment malfunctions or the result of natural events beyond the control of LP&L. With respect to equipment malfunctions, the causes leading to the malfunction were identified and maintenance or replace-ment performed to prevent recurrence of the event. Deviations from the REMP associated with TLDs were beyond the control of LP&L and resulted from theft of a few of the dosimeters placed in the field. When a dosimeter was discovered missing during a monthly inspection, the TLD was replaced and the deviation noted. A listing of all unavailable samples for 1985 along with associated explanations of why the samples were not collected is given in Appendix c. A more detailed explanation for milk and vegetation sample unavailability is discussed below. Milk samples were not available on a regular basis from the animal owner at station MKE-4 due to the small volume of milk produced by the animals. With the absence of milk samples at this station, broad leaf

        ,      vegetation sampling was performed. One control location sampls, MKQ-50, was unavailable from Louisiana Nuclear Energy Division personnel due to participation of the state in the Annual Emergency Planning Exercise conducted in September of 1985. Broad leaf vegetation was sampled at a control location during this month in lieu of the milk sample.

Broad leaf vegetation was not sampled at a control location during the months of January through May, 1985, since milk samples were available from the , 29 t

l control location. However, beginning in June of 1985, broad leaf vegetation was sampled even when control milk samples were available in order to accumulate baseline data for future comparisons. j I 3.5.2 Missed Lower Limits of Detection I A licting of all analyses that could not attain the lower limits of detection specified in Table 4.12-2 of Waterford 3 SES Technical Specification 4.12.1 is presented in Appendix c. With the exception of ons drinking / surface water sample, the LLDs were not attained due to insufficient sample size resulting from equipment malfunction. In all of these cases the equipment was repaired or replaced to prevent recur-rence. I The LLD for barium-140/ lanthanum-140 could not be attained for one drinking / surface water sample. missed LLD resulted from the gamma spectroscopy The analysis being delayed. The delay was caused by the I contract laboratory postponing the analysis while awaiting arrival of a biweekly sample necessary to form a monthly composite. However, the biweekly sample was never collected due to equipment malfunction and miscommunication regarding the unavailable sample delayed analysis. 3.5.3 Chances to the REM? I During 1985, one new milk station, MKQ-1, was added to i the REMP as a result of the 1985 Annual Land Use Census. However, no samples were available from the i new location during 1985 (see Section 3.6). l The location of the control broad leaf vegetation i station was changed during 1985 as a result of re-eval-unting site meteorological data. The location was l changed from BLH-10 to BLK-15 such that the new sampling station was located in the compass sector coinciding with the least prevalent wind direction. Shoreline soil sampling location SHWJ-1 was added to the REMP during the second half of 1985. The new location was added to monitor shoreline soil from a drainage canal into which effluents from the turbine building sumps are discharged. 30 I 1

3.6 Annual Land Use Census Results In compliance with Waterford 3 SES Technical Specification 4.12.2, the Annual Land Use Census was conducted on July 10 and 11, 1985. The nearest residence, garden, and milking animal in each sector within a five mile radius of the plant were found by visual inspection and verbal inquiry. The results of the 1985 census are given in Table 3.2. A new milking cow was found in sector Q at a distance of 1.1 miles from the plant. As a result, a new milk sampling station (MKQ-1) was added to the REMP. The owner of the animal stated that the cow was nursing a calf and would not begin producing milk for human consumption until December 1985. The owner was contacted an a periodic basis to determine the status of obtainibrJ. samples. The owner of milking goats at location MKE-4 has sold all but one of his goats. The remaining goat does not produce enough milk for Waterford 3 SEJ to obtain samples as stated by the owner. However, the sampling. station will remain as part of the REMP and the owner will be contacted period- , ically to determine the status of obtaining samples. i h t P 31 I

TABLE 3.1 1985 DIRECT RADIATION DATA ORGANIZED BY COMPASS DIRECTION I AND DISTANCE FROM WATERFORD 3 SES BY COMPASS DIRECTION l SECTOR COMPASS AVERAGE STANDARD NUMBER DIRECTION EXPOSURE DEVIATION IN (arem/std qtr) (aren/std qtr) GROUP , A N 18 3.6 8 B NNE 16 0.8 8 C NE 13 1.5 3 D ENE 18 3.7 6 E(a) E 16 2.0 12 F ESE 17 I 12 2.8 G SE 17 1.9 11 H SSE 16 4.5 7 J S 17 5.1 7 K SSW 16 1.3 4 L SW 15 0.5 4 i M WSW 17 2.4 4 N W l 21 4.9 2  !

P WNW 19 3.6 8 l Q NW 16 2.O 8 i R NNW 16 2.3 8 CONTROL E 21 4.1 4 i BY DISTANCF - FROM PLANT DISTANCE AVERAGE STANDARD NUMBER FROM PLANT EXPOSURE DEVIATION IN (miles) (ares /std qtr) (aren/std qtr) GROUP O-2 I 2-5
       > 5(a) 16 17 18 1.6 3.0 3.4 58 26 28 CONTROL                21               4.1                             4
a. Does not include control station data 32 l \

TABLE 3.2 1985 ANNUAL LAND USE CENSUS RESULTS SECTOR DIRECTION DISTANCE FROM THE PLANT I (miles) MILK MILK VEGETABLE RESIDENCE COW GOAT GARDEN I A B C N NNE NE 1.1 1.3 1.0 0.8 0.8 0.9 D I ENE - - 0.9 0.9 E E F 3.3(a) 3.2 2.6 ESE - - 2.3 3.4 G SE - - 2.3 3.9 I H J K SSE S SSW 0.9 0.9 - L SW - - 0.9 - M WSW - - 0.9 - N W - - 1.1 1.3 P WNW - - 0.9 0.9 Q NW 1.1(b,c) - 0.9 0.9 R NNW - - 2.9 2.0 Means none found in sector within a 5 mile radius of [ Waterford 3 SES.

a. Goat was not producing enough milk for samples.
b. Milk cow was nursing calf and does not supply milk for human

, consumption. The owner will be contacted on a periodic i basis to determine availability of samples. 1

c. Samples will also continur, to be taken 4.4 miles (MKQ-5).

This is the only reliabir, milk sample within 5 miles of ' Waterford 3 CES. 11 l . Il

4.0 CONCLUSION

S The radiological environmental data collected during 1985 are consistent with the data obtained during the Preoperation Environmental Radiological Surveillance (PERS) Program and during the first two years of the REMP prior to Waterford 3 SES initial criticality. The only man-made radionuclide detected out of all I of the environmental samples analyzed during 1985 was casium-137. Cesium-137 was detected in one shoreline soil sample and two control location broad leaf vegetation samples. The origin of this man-made radioactivity is most likely attributable to fallout from past nuclear weapons detonations and not Water-ford 3 SES operation. I In conclusion, based on the evaluation of the REMP data collected during 1985 the operation of Waterford 3 SES had no observable radiological impact on the environment. II

 .Il 11 I

i P ll  ! t ll t t l 34 ,

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l l I l I ' 1 l l 1 1 i i i* l P f I L I  ! APPENDIX A i REMP DATA

SUMMARY

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i TABLE A-1 SASletACICAL MaynammenstAL Ime1Malus reemest seemRT i Emme of postlity is r-a s aan tschet No._ sa-ses Lacettee of messitty St. h ates. Langelaas j (Parteh. State) Seporties perled 1 - s! neat { ADEsten ra m T -- " " 5"""

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1. street mediaties Tim als 1

! 17(112/112) 5-3e 21(4/4) s-3e (aren/Std. 4tr.) (13-27) 27.e miles I o j t.> (18-27) 21(4/4) . (18-27)

2. Airkerne Perste- Crees 253 le 21 2e8/281) Ar3-Je i mistas Bote W) 27.e allee E 22(51-52)

(10-42) Ars-3e 22(51/52) e (le'3 pct /m3 ) l i Gamma 20 (c) etJa (a/16) HA Ila i APE-30 e (-) <tas (e/4) 1 (-) i

3. Aschere. Iedtee 1-131 255 7e <tas (c/2e3) as na Ars-w (10'3 pct /m3 ) e

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                                  " " ' ' " "                      as,3, upscase sacavesus    tactress viu enemmer assunLsea.                                  i sesosas                                                                                                          esanos.Racarsam
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11. Feed /Carden Crey Cemens 1 (c) cIAS (S/1) E i

(pC1/ka-met) M Bone O O (-) l ? I l 1 - - i

     *lsestaal Immer Limit of Detection (Lla) es defined sa unterford 3 Technical specificatione, b

samen and reage beoed uses detectable meneeramente only. Fraction of detectable naaews at specified lecettene is indicated in perentheste.

     *gmuer Limite of Betection (123) for ladividual radiomec11 des emelysed for by gemene spectreecepy are given in unterford 3 Technical          n.      Sp

! A h mistamm Imune Limit of metection (118) defined se unterford 3 Technical Specificatione. I i l I I.

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                                                                                             ?

l l 1 APPENDIX B REMP DATA l 1 l I 41 m

                                                       - - - - - .,.y p, - ,-- - - , . --- -

E " . s TABLE B-1 Qt!ARTERLY TLD EXPOSURES mRee/ stands 74 90 day quarter STATION FIRST quASTER SECONO QUARTER 59000fB INIRD QUAR 11R FOUNIN quARifR 12/27/04-43/28/05 03/28/85-06/28/45 06/28/05-10/02/85 10/02/85-01/03/46 A-2 18 19 19 15 A-5 17 26 (d) 15 15 s-1 15 16 16 15

  ,         3-4                           17                                              17 w                                                                                                                        16                   15 C-1                           13 (a)                                          14                              11 (b) e-2                           la                                             21                               19 (n) 8-5                          (b)                                             21 (d)                           13                   13

(-1 17 (a) 19 16 15 E-5 14 17 14 13 E-15 17 19 la 15 E-34 27 (c) 20 19 la F-2 15 15 15 14 F-4 13 21 19 15 F-9 17 23 16 15 6-2 It 20 19 16 6-4 17 (b) 14 14 6-9 17 la 17 15 N-2 17 18 17 (b) _. H- 6 13 25 13 12 ( a) T10 Vandaltred; replaced 03/01/85. ' (b) 110 Vandallied (c) 110 Vandal t sed; replaced 01/08/85, (d) ILD VandalI4 :d; replaced 05/03/85, __ _____ _ _ __ - _ - - - -- - - - - - - - - ^ ^ - - - - ^ ~ ^ ^ ^

M ' M TABLE B-1 (Cont.) QUARTERLY TLD EXPOSURES stes/ standard 90 day quarter STAiles FIRST QUAtift SEC058 QUARTER sustetR I2/27/84-83/28/85 IMIRD QUAtlER F00aTN QUARTER 03/28/85-06/28/85 06/28/05-10/02/85 I0/02/85-01/03/s6 J-2 32 (a) In 14 g3 J-15 15 28 16 15 E-1 16 17 16 14 L-1 15 15 16 15

a. m-1 15 w 20 15 16 N-1 (b) 24 (c) 17 (b)

P-1 17 27 (d) 13 15 P-6 19 20 I3 1y 4-1 14 17 15 13 l Q-5 17 19 13 16

;    R-1                      14                       17                                        14                33 R-6                      17                       19                                        la                la i

ll a' f Radiography la area i I h i TLS Vandalsaed ! I c i ILS Vandallaed; replaced 06/08/85. I L dll TLS Vandallaed; replaced 05/01/85. l 1 l 5

M M M TABLE B-2 AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND 10 DINE-131 ANALYSES STATION RUNGE4 APC-1 1955 COLLECTIDs DATE #10 COUni STAsi STOP A P FILTER Mle COUNI CNARCOAL F ILTER IINE GROSS BETA TIME l-131 SATE DATE VOL UNE UNITS DATE (DCS/Co. M.) DATE (pCl/Cu, N.) 12/31 01/07 1.02E 04 CU. FI. 01/15 2.2 a 0.3 E-02 01/11 L.T. 4 E-02 01/07 01/14 1.02E 04 CU. FT. 01/25 2.4 2 0.4 E-02 01/16 L.T. 2. E-02 01/14 01/22 1.17E 04 CU. FI. 01/30 2.1 1 0.3 E-02

                 #                                                                                                                                      01/24       L.I. 3. E-02 01/22         01/28       8.51E 03                            CU. FT. 02/06      1.9 a 0.4 E-02     01/30       L.T. 3. E-02 01/28         02/04       1.0lE 04                            CU. FI. 02/11      1.9 a 0.3 E-02     02/07       L.I. 5. E-02 02/04         02/11      9.94E 03                             CU. FT. 02/21      3.4 2 0.4 i-02     02/13       L.T. 3. E-02 j                                                02/11        02/18       1.02E 04                             CU. FI. 02/26      2.8 2 0.4 E-02     02/21       L.T. 3. E-02 02/18        02/25       1.02E 04                             CU. FT. 03/05      1.5 t 0.3 E-02     02/27       L.T. 3. E-02 02/25        03/04       1.03E 04                             CU. FT. 03/13      1.8 2 0.3 E-02     03/06       L.T. 3. E-02 03/04        03/11       1.03E 04                             CU. FT. 03/20      2.1 1 0.3 E-02     03/13       L.T. 3. E-02 03/11        03/18       1.03E 04                            CU. FT. 03/26      2.0 s 0.3 E-02     03/20       L.T. 3. E-U2 03/18        03/25       1.03E 04                            CU. FI. 03/29      1.3 $ 0.3 E-02     03/28       L.T. 4. E-02 03/25        04/01       6.56E 03                            CU. FT. 04/08      2.4
  • 0.4 E-02 04/03 L.T. 6. E-02 i

1 i

M . M TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STAil0N NUNGER APC-1 lyst COLLECil00 SATE NIO COUNT STASI STOP A P FILTER MID COUNT CNAACOAL FILTER IINE 68055 OETA IINE OATE DATE VOL UNE UNIis DATE (pCl/Cu. M.) l-131 DATE (pCl/Cu. M.) 04/01 04/09 1.16E 04 CU FI. 04/16 2.0 2 0.3 E-02 04/11 L.T. 3. E-02 04/09 04/15 0.73E 03 CU. FT. 04/25 2.1 2 0.4 E-02 04/10 L.I. 4. E-02 04/15 04/22 1.02E 04 05/01 CU. ff. 1.0 s 0.3 E-02 04/24 L.T. 3. E-02 04/22 04/30 1.20E 04 CU FT. 05/24 2.1 a 0.3 E-02 05/01 L.I. 2. E-02 04/30 05/06 (a) 05/06 05/00 3.69E 03 CU. FT. 05/21 3.0 t 0.0 E-02 05/16 L.I. 2. E-ut(b) i 05/40 05/20 (c) 05/20 05/27 1.02E 04 CU. FT. 06/06 2.1 a 0.3 E-02 05/30 L.I. 2. E-02 05/27 06/03 1.00E 04 CU. FT. 06/17 3.0 t 0.3 E-02 06/05 L.T. 3. E-u2 06/03 06/10 1.00E 04 CU. FT. 06/19 2.6 s 0.4 E-02 06/13 L.I. 3. E-02 06/10 06/17 1.0lE 04 CU. FI. 07/02 1.3 2 0.3 E-02 06/19 L.I. 4. E-02 04/17 06/24 1.Olt 04 CU. Fi. 07/10 2.0 s 0.3 E-02 06/26 L.T. 3. E-02 06/24 07/01 1.0lE 04 CU. FT. 07/15 2.7

  • 0.4 E-02 0//03 L.T. 4. E-02 lla Sample not cellected; pump not workine.

I b Required LLO could met be met due to low air volume. Lc Power failure; sample not collected. i I

M TABLE B-2 (Cont.) AIR PARTICUr. ATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND IODINE-131 ANALYSES SIATION NUNGER APC-1 15s3 COLLECTION SATE START MID COUNT A P FILTER MID COUNI CHAACOAL FILIER STOP TIME GROSS SETA TIME l-131 DATE DATE WOL UNE UNITS DATE (pCl/Co. M.) DATE (pCl/Cu. h.) 07/01 07/03 3.95E 03 CU. Fi. 07/17 3.5 t 0.6 E-02 07/11 L.T. I. E-Ol(a) 07/09 07/15 8.80E 03 CU. FT. 07/22 2.3 a 0.4 E-02 07/l? L.T. 3. E-02 07/15 07/23 1.IIE 04 CU. FT. 07/26 I.9

  • 0.3 E-02 07/24 L.T. 3. E-02 07/23 07/29 9.22E 03 CU. FT. 04/07 1.8 1 0.3 E-02 07/31 L.T. 3. E-02 07/29 08/05 1.02E 04 CU. FI. 08/15 2.0 2 0.3 E-02 08/07 L.T. 3. E-02 08/05 08/12 1.01E 04 CU. FT. 08/19 2.2 a 0.3 E-02 08/14 L.T. 3. E-U2 08/12 08/19 1.02E 04 CU. FT. 08/29 1.5 t 0.3 E-02 08/22 L.T. 3. E-02 08/89 08/26 1.04E 04 CU. FT. 08/30 1.9 a 0.3 E-02 08/28 L.I. 3. E-02 08/26 09/03 1.15E 04 CU. FT. 09/09 2.0 t 0.3 E-02 09/04 L.I. 2. E-02 09/03 09/09 9.71E 03 CU. FT. 09/19 1.5 t 0.3 E-02 09/10 L.I. 3. E-02 09/09 09/16 1.02E 04 CU. FT. 09/23 2.1 1 0.3 E-02 09/17 L.I. 4 E-02 09/16 09/23 1.0IE 04 CU. FT. 10/03 1.8 1 0.3 E-02 09/24 L.T. 2. E-02 09/23 0*/30 1.03E 04 CU. FT. 10/07 2.3 1 0.3 E-02 10/01 L.T. 2. E-02

( a) Regulred LLD could act be met due to lou air volume. 4 o y, . ,m _ . , _ _ . - - , _ . - - _ - - - - , . .,,. _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ . _ . _

M - M t

                           ,                      TABLE B-2 (Cont.)

AIR PARTICULATE FILTERS AND CllARCOAL CARTRIDGES:

      "**'                                GROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APC-1 Ivst COLLECTIDs     DATE                                NID COUNI     A P FILTEA                                                MID COUni STAti          510P                                                                                                                      CHARC0AL flLTER TIME       GA055 BETA                                                        TIME        l-131 SATE           SATE       VOLUME        UNIT 5       DATE        (pCl/Cu. M.)                                                     DATE   (pct /Cu. M.).

09/30 10/07 1.0lt 04 CU. fi. 10/11 1.9 a 0.3 E-02 10/Os L.T. 3. E-02 10/07 10/14 1.02E 04 CU. ft. 10/22 2.3 s 0.3 E-02 10/16 L.f. 3. L-02 10/14 10/21 1.02E 04 CU. FT. 10/29 1.3 s 0.3 E-02 10/23 L.T. 2. L-u2 10/21 10/28 1.02E 04 CU. FT. 11/13 2.1 a 0.3 E-02 10/30 L.I. 3. E-02 10/28 11/04 1.01E 04 CU. F1. 11/13 1.5 a 0.3 E-02 11/06 L.T. 3. E-02 11/04 11/11 1.Olt 04 CU. FT. 11/21 3.1 s 0.4 E-02 11/14 L.I. 3. E-02 11/11 11/18 (a) 11/18 11/25 (a) 21/25 12/02 1.00E 04 CU. FT. 12/09 7.2 s 3.3 E-03 12/04 L.T. 3. E-02 12/02 12/09 1.02E 04 CU. Ft. 12/19 3.1 s 0.4 E-02 12/11 L.T. 3. L-02 12/09 12/16 9.61E 03 CU. FT. 12/30 2.1 s 0.3 E-02 12/19 L.I. 3. E-02 12/16 12/23 9.96E 03 CU. FT. 01/03 3.5 s 0.4 E-02 12/27 L.T. 2. E-Uz 12/23 12/30 9.89E 03 CU. FT. 01/07 2.3 s 0.3 E-02 01/02 L.T. 3. E-02 (a) Pump malfunction; no sample available.

   ,.                                                                ~
                                                                            . , , - - , . . _ - - - - - - - - , . - , - - . - ~ , , - .                   -- -        --rvv -- ---- --

M M M t TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES SI Ail 0h NUNSER APG-1 1955 COLLECil0N BATE MID COUNT START STOP A P FILIER Mle COUNT CHARCOAL FILIES TIME GROS $ SET A IINE DATE SATE VOL UME UNITS DATE (pCl/Cu. M.) I-131 OATE (pCi/Cu. M.I 12/31 01/07 9.79E 03 CU. FT. 01/15 2.2 1 0.3 E-02 01/11 4. L.T. E-02 01/07 01/14 9.SSE 03 CU. FT. 01/25 2.6 2 0.4 E-02 01/16 L.I. 2. E-02 01/14 01/22 9.!SE 03 CU. FT. 01/30 2.4 2 0.4 E-02 01/24 L.I. 4. E-02 g 01/22 01/24 8.34E 03 CU. FI. (a) 01/30 L.T. 3. E-02 01/28 02/04 9.89E 03 CU. FT. 02/11 1.9 2 0.3 E-02 02/07 L.T.

5. E-02 02/04 02/11 9.86E 03 CU. FT. 02/21 3.3 2 0.4 E-02 02/13 L.I. 3. E-02 02/11 02/18 9.90E 03 CU. Fi. 02/26 2.6 2 0.4 E-02 02/21 L.T. 3. E-02 02/18 02/25 9.96E 03 CU. Fi. 03/05 1.7 4 0.3 E-02 02/27 L.I. 3. E-02 02/25 03/04 9.97E 03 CU. FT. 03/13 1.5 e 0.3 E-02 03/06 L.T. 3. E-02 03/04 03/11 1.00E 04 CU. FT. 03/20 1.9 2 0.3 E-02 03/13 L.T. 3 E-02 03/11 03/18 9.94E 03 CU. FT. 03/26 1.9 2 0.3 E-02 03/20 L.T. 3. E-02 03/18 03/25 9.98E 03 CU. Fi. 03/29 1.7 2 0.3 E-02 03/28 L.T. 5. E-02 03/25 04/01 1.00E 04 CU. Fi. 04/08 2.2 1 0.3 E-02 04/03 L.I. 3. E-02

( a) Losk filter during collecties. High winds blew filter este puddle of water, s.

M M s TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CilARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STATION NUNSEA APG-1 Iyuz COLLECilee SATE MID COUNT A P FILTER STARI STOP MID COUNI CNARC0AL FILTER TIME GROS 5 SETA IlNE OATE DATE VotumE UnlT5 l-131 DATE (pCl/Cu, N.) DATE (pCl/Cu. M.) 04/01 04/09 1.06E 04 CU. FT. (a) 04/11 L.T. 3. E-02 04/09 04/15 7.93E 03 CU. F1. 04/25 2.4 2 0.4 E-02 04/18 L.T. 4. E-02 04/15 04/22 9.20E 03 CU. FI. 05/01 2.2 2 0.4 E-02 04/24 L.T. 3. E-02 04/22 04/29 9.13E 03 CU. FT. 05/24 2.0 2 0.4 E-02 05/01 L.I. 3. E-02 04/29 05/06 9.22E 03 CU. FI.

  • 05/14 1.9 a 0.3 E-02 05/08 L.I. 3. E-02 05/06 05/13 9.23E 03 CU. FT. 05/21 2.3 2 0.4 E-02 05/16 L.T. 5. E-02 05/13 05/20 9.96E 03 CU. FT. 05/31 2.3 2 0.3 E-02 05/23 L.I. 4. E-02 05/20 05/27 9.95E 03 CU. FT. 06/06 2.0 2 0.3 E-02 05/30 L.I. 2. E-02 05/27 06/03 9.93E 03 CU. FT. 06/17 2.7 1 0.3 E-02 06/05 L.I. 3. E-02 06/03 06/10 1.IIE 04 CU. FT. 06/19 4.2 2 2.0 E-03 06/13 L.T. 2. E-02 06/11 06/18 9.96E 03 CU. FT. 07/02 1.2 a 0.3 E-02 06/19 L.T. 4. E-02 06/18 06/24 1.14E 04 CU. FT. 07/10 3.4 2 1.9 E-03 06/26 L.T. 3. E-02 06/24 06/27 3.81E 03 CU. F T. 07/15 3.3 a 0.7 E-02 07/03 L.I. 1. E-Ul(b) a Sample not received; lost during collection.

h Pump malfunction; required LLO not met due to lou air valuee. 4 w - , n -+n- , - - --, -- - - . ,, ,.e, . . _ _ . _ . . , , _ _ _ ~ , . - _ _ _ _ _ _ _ _, _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ - _ _ _ _ _ _ _ _

            .M       M s

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETt AND IODINE-131 ANALYSES STAil0N NUMMER APG-1 TYET COLLECIl0N DATE M10 COUNI A P flLTER STASI SIDF Miu COUNI CHAMCOAL FILTLN TIME GROSS BEIA DATE DATE V0tuME UNITS DATE (pCl/Co. M.) ilh[ I-131 DATE (pCl/Cu. M.) 07/01 01/02 1.75E 03 CU. FT. 07/17 5.1 s 1.2 E-02 01/11 L.T. 3. E-Ol(a) 07/08 07/13 7.78E 03 CU. FT. 07/22 2.4 a 0.4 E-02 07/l? L.T. 4. E-02 07/15 07/22 9.70E 03 CU. FT. 07/26 1.7 a 0.3 E-02 07/24 L.T. 3. L-02 o 07/22 07/29 9.40E 03 CU. FT. 08/07 1.9 s 0.3 E-02 07/31 3. L.I. E-02 07/29 08/05 9.81E 03 CU. FT. 08/15 2.0 s 0.3 E-02 08/07 L.T. 3. E-02 08/05 08/12 9.28E 03 CU. FT. 08/19 2.1 s 0.3 E-02 08/14 L.T. 3. E-02 08/13 08/19 8.35E 03 CD. Fi. 08/29 1.4 a 0.4 E-02 08/22 L.T. 4. L-u2 08/19 08/26 9.68E 03 CU. ft. 08/30 1.9 s 0.3 E-02 08/2s L.T. 3. L-02 08/26 09/03 1.13E 04 CU. FT. 09/09 2.0 s 0.3 E-02 09/04 L.T. 2. E-02 09/03 09/09 8.35E 03 CU. FT. 09/19 1.9 s 0.4 E-02 09/10 L.T. 3. E-02 09/09 09/16 9.79E 03 CU. FT. 09/23 2.1 s 0.3 E-02 09/17 L.T. 4. E-02 09/16 09/23 9.971 03 CU. Fi. 10/03 2.1 a 0.3 E-02 09/24 L.I. 2. E-02 09/23 09/30 1.04E 04 CU. Fi. 10/07 1.9 s 0.3 E-02 10/01 L.T. 2. E-02 (a) Required LLO could not be met due to low air volume; pump malfunctiones.

    -.-.-,_.m. _ ,     . - - -   y . -,    , , - . .         _.
                                                                  ~ . .      . _ . - . - - _         _ , _      --   . _ _ _ _ . _ _              _ _ . _ _ _ _ _ _ _ _ _ _ _ _ - _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ . _ _                       __

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND IODINE-131 ANALYSES 51Afton nUMsEn AP6-1 I TM COLLECTIoa SATE MlD COUni START STOP A P FILIER hl0 COUni CHAACOAL FILIER IINE GROSS SETA ilME BATE DATE VOL UME UNITS DATE (pCl/Cu. M.) l-131 DATE (pCi/Cu. M.) 09/30 10/07 9.63E 03 CU. FT. 10/11 1.9 2 0.3 E-02 10/08 L.T. 3. E-02 10/07 10/14 9.96E 03 CU, FI. 10/22 1.8 a 0.3 E-02 10/16 L.T. 3. E-02 10/14 10/21 9.92E 03 CU. Fi. 10/29 9.7 a 2.5 E-03 10/23 L.T. 3. E-U2 10/21 10/28 9.88E 03 CU. FT. 11/13 1.3 1 0.3 E-02 10/30 L.T. 3. E-02 10/30 11/04 6.76E 03 CU. FI. 11/13 2.6

  • 0.5 E-02  !!/06 L.T. 4. E-U2 11/04 11/11 9.88E 03 CU. FI. 11/21 4.1 1 0.5 E-02 11/14 L.I. 3. E-U2 11/11 11/18 9.86E 03 CU. FT. 11/25 1.5 2 0.3 E-02  !!/22 L.I. 3. E-02 11/18 11/25 9.92E 03 CU. Fi. 12/06 2.3 t 0.4 E-02 12/02 L.T. 4. E-02 11/25 12/02 9.88E 03 CU. FT. 12/09 7.6 a 3.3 E-03 12/04 L.T. 3. E-02 12/02 12/09 1.00E 04 CU. FI. 12/18 3.4 a 0.4 E-02 12/11 L.T. 3. E-U2 12/89 12/16 9.30E 03 CU. FT. 12/30 2.4 a 0.3 E-02 12/19 L.I. 3. E-U2 12/16 12/23 9.70E 03 CU. FT. 01/03 3.3 a 0.4 E-02 12/27 L.T. 3. E-02 4

12/23 12/30 9.96E 03 CU. FT. 01/07 2.6 s 0.4 E-02 01/02 L.T. .3. E-02 4

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TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES SI ATION NUMSER APP-1 1955 COLLECTISE DATE START STOP M10 COUNT A P FILTER MID Couti CHARCOAL FILTER TIME sa0$$ SETA OATE DATE VOL UME U41T5 OATE (pCl/Cu. M.) TIME l-131 OATE (pct /Cu, M.) 04/01 04/09 1.18E 04 CU. FT. 04/16 1.8 t 0.3 E-02 04/11 L.T. 3. E-02 04/09 04/15 8.83E 03 CU. Fi. 04/25 I.9 2 0.4 E-02 04/18 L.T. 4. f-02 04/15 04/22 1.02E 04 CU. FT. 05/01 s.n 2.5 1 0.4 E-02 04/24 L.T. 3. E-02 63 04/22 04/29 1.0lE 04 CU. FT. 05/24 2.2 1 0.3 E-02 05/01 L.T. 3. E-02 04/29 05/06 1.0lE 04 CU. FT. 05/14 2.0 1 0.3 E-02 05/08 L.T. 2. E-02 05/06 05/13 1.02E 04 CU. FT. 05/21 2.3 a 0.3 E-02 05/16 L.T. 4. E-02 05/13 05/20 1.03E 04 CU. FT. 05/31 2.1 2 0.3 E-02 05/23 L.T. 3. E-02 05/20 05/27 1.03E 04 CU. FT. 06/06 2.5 1 0.3 E-02 05/30 L.T. 2. E-02 05/27 06/03 1.00E 04 CU. FT. 06/17 2.9 i 0.3 E-02 06/05 L.I. 3. E-02 06/03 06/10 1.04E 04 CU. FI. 06/19 3.1 t 0.4 E-02 06/13 L.T. 2. E-02 06/10 06/I7 9.65E 03 CU. Fi. 07/02 1.1 2 0.3 E-02 06/19 L.I. 5. E-02 06/17 06/24 1.0!E 04 CU. FT. 07/10 2.4

  • 0.3 E-02 06/26 L.T. 3. E-Ut 06/24 07/01 9.94E 03 CU. FT. 07/15 2.7
  • 0.4 E-02 07/03 L.T. 4. E-02

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TABLE B -2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APQ-1 19st COLLECTION 0 ATE STAti STOP Mio COUni A P FILTER MID COUNT itnf S8055 SETA CHARC0AL FILTER DATE SATE VOL U8tf TIME I-131 UNITS DATE (pCl/Co. K.) DATE (pC1/Cu. M.) 12/31 01/07 8.08E 03 CU. FT. 01/15 2.3 2 0.4 E-02 01/11 L.T. 5. E-02 01/07 01/14 4.22E 03 CU. FT. 01/25 2.7 2 0.4 E-02 01/16 L.T. 3. E-02 01/14 01/22 8.90E 03 CU. FT. 01/30 2.4 1 0.4 E-02 01/24 L.I. 5. E-02 01/22 01/28 6.27E 03 CU. FT. 02/06 2.0 t 0.5 E-02 01/30 L.T. 4 E-02 01/28 02/04 7.49E 03 CU. Fi. 02/11 2.2 2 0.4 E-02 02/07 L.T. 6. E-02 02/04 02/11 7.45E 03 CU. FT. 02/21 3.5 a*0.5 E-02 02/13 L.T. 4. E-02 02/11 02/18 7.47E 03 CU. FI. 02/26 2.6 2 0.4 E-02 02/21 L.I. 4. E-02 02/18 02/25 7.47E 03 CU. FT. 03/05 1.7 2 0.4 E-02 02/27 L.I. 4. E-02 02/25 03/04 7.48E 03 CU. FT. 03/13 l 1.8 a 0.4 E-02 03/06 L.I. 4. E-02 03/05 03/11 8. 60E '03 CU. FT. 03/20 2.4 a 0.3 E-02 03/13 L.T. 3. E-02 03/11 03/18 1.01E 04 CU. FT. 03/26 2.0 a 0.2 E-02 03/20 L.T. 3. E-02 03/13 03/25 1.01E 04 CU. FT. 03/29 3.0 t 0.4 E-02 03/2a L.T. 5. E-02 03/25 04/01 1.02E 04 CU. FT. 04/08 2.2 a 0.3 E-02 04/03 L.T. .3. E-02 i I

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND 10 DINE-131 ANALYSES stall 0N NUNSES APQ-1 tyst COLLECil0N OATE START ST SP Mib COUNI A P FILIEN MIO COUNT OATE TIME 6R055 SLIA CNARCOAL FILIEu BAlf VOLUME UNii5 TIME l-131 OATE (SCI /Cw. M.) DATE (sCt/Cu. M.) 04/01 04/09 1.16E 04 CU. FT. 04/16 1.8 2 0.3 E-02 04/11 L.I. 3 E oz 04/09 04/15 0.69E 03 .CU. Fi. 04/25 2.2 t 0.4 E-02 04/1s L.T. 4 L-Oz 04/15 04/22 1.02E 04 CU. FI. 05/01 2.0 a 0.3 E-02 04/24 L.I. 3. E-Uz 04/22 04/29 1.03E 04 CU. FT. 05/24 2.1 1 0.3 E-02 05/01 L.I. 3. E-02 04/29 05/06 1.04E 04 CU. Ft. 05/14 2.0 1 0.3 E-02 05/08 L.T. 2. E-02 05/06 05/13 1.04E 04 CU. FI. 05/21 2.4 2 0.3 E-02 05/lb L.I. 4 E-02 05/13 05/20 1.03E 04 CU. Fi. 05/31 2.3 2 0;3 E-02 05/23 L.T. 3. E-uz 05/20 05/27 1.03E 04 CU. FT. 06/06 2.1 2 0.3 E-02 05/30 L.I. 2. E-02 05/27 06/03 1.00E 04 CU. FT. 06/IP 2.3 2 0.3 E-02 06/05 L.I. 3. E-02 06/03 06/10 1.09E 04 CU. FT. 06/19 2.9 s 0.3 E-02 06/13 L.I. 2. E-u2 06/10 06/l? I.04E 04 CU. FT. 07/02 1.2 2 0.3 E-02 06/19 L.T. 4. L-02 06/17 06/24 1.IIE 04 CU. FI. 07/10 i 2.1 2 0.3 E-02 06/26 L.T. 3. L-02 06/24 OO01 1.04E.04 CU. Fi. 07/15 2.6 1 0.3 E-02 07/03 L.I. 4. E-02

m. _ _ _

m m m M M M M s TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: Ch0SS BETA AND IODINE-131 ANALYSES STAT:0N Nun 8Ea APQ-1 1955 COLLECiles SATE N10 COUNT A P FILTER STASI STOP MID COUNT CHASC0AL FILith OATE Tint G8055 SETA TIME l-131 SATE VOL ucif UNITS DATE (pCl/Cu. M.) DATE (pCl/Cu. M.) 07/01 07/08 1.05E 04 CU. FT. 07/17 1.7 4 0.3 E-02 0?/II L.T. 3. E-02 07/08 07/15 1.03E 04 CU. FT. 07/22 2.4 2 0.3 E-02 07/17 L.T. 2. E-02 07/15 07/22 1.10E 04 CU. FI. 07/26 1.9 2 0.3 E-02 07/24 L.I. 2. E-02

  $                                                                                                     07/22            07/29    1.00E 04       CU. FI.                            08/07               2.0 t 0.3 E-02                                                                      07/31           L.T. 3. E-02 07/29           08/05     1.04E 04       CU. FT.                            08/15               2.1
  • 9.3 E-02 08/07 L.I. 3. E-02 08/05 08/12 1.03E 04 CU. FT. 08/19 2.5 4 0.3 E-02 08/14 L.T. 3. E-02 08/12 08/19 1.04E 04 CU. FT. 08/29 1.5 t 0.3 E-02 08/22 L.I. 3. E-02 08/19 08/26 1.05E 04 CU. FT. 08/30 2.0 2 0.3 E-02 i 08/28 L.T. 3. E-02 08/26 09/03 1.15E 04 CU. FT. 09/09 2.1 a 0.3 E-02 09/04 L.I. 2. E-02 09/03 09/09 8.59E 03 CU. FI. 09/19 1.4 2 0.3 E-02

' 09/10 L.T. J.,E-02 09/09 09/16 1.0lf 04 CU. FT. 09/23 1.7 1 0.3 E-02 09/17 L.I. 4. E-02 09/16 09/23 9.91E 03 'CU. FT. 10/03 1.7 a 0.3 E-02 09/24 L.T. 2. E-02 09/23 09/30 1.02E 04 CU. F T. 10/07 2.0 1 0.3 E-02 10/01 L.T. 2. E-02 1

                                                                                  .9 4
                                                                                                                                                                                                                                                                                                                                      , j

E s TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CAR 11tIDGES-GROSS BETA AND 10 DINE-131 ANALYSES STAilom NUMBER APQ-1 19s5 COLLECilDe SATE MID COUNT A P FILTER MID COUNT CHAAC0AL FILTER START STOP 11NE GA055 SETA TIME l-131 DATE SATE Volp06E UNITS DATE (pCl/Cu. M.) DATE (pCl/Cu. M.! 09/30 10/03 9.47E 03 CU. FT. 10/11 1.7 1 0.3 E-02 10/08 L.T. 3. E-02 10/07 10/14 9.80E 03 CU. FT. 10/22 2.3 a 0.3 E-02 10/16 L.T. 3. E-02 10/14 10/21 9.70E 03 CU. FT. 10/29 1.1 2 0.3 E-02 10/23 L.T. 3. E-02 10/21 10/28 S.SSE 03 CU. FT. 11/13 1.5 1 0.3 E-02 10/30 L.T. 3. E-02 u 10/30 11/04 (a) 11/04 11/11 1.02E 04 CU. FT. 11/21 3.1 2 0.4 E-02  !!/14 L.T. 3. E-02 11/11 11/18 1.00E 04 CU. FT. 11/25 1.4 2 0.3 E-02 11/22 L.T. 3. E-02 11/18 11/25 1.02E 04 CU. FI. 12/06 2.4 1 0.4 E-02 12/02 L.T. 4. E-02 11/25 12/02 9.89E 03 CU. FT. 12/09 7.8 s 3.3 E-03 12/04 L.1, 3. E-02 12/02 12/09 1.04E 04 CU. F i. 12/18 3.4 2 0.4 E-02 12/11 L.T. 3. E-02 12/09 12/16 9.57E 03 CU. FI. 12/30 2.1 1 0.3 E-02 12/19 L.I. 3. E-02 12/16 12/23 9.96E 03 CU. FT. 01/03 3.6 2 0.4 E-02 12/27 L.I. 3. E-02 12/23 12/30 9.97E 03 CU. FT. 01/07 2.2 2 0.3 E-02 01/02 L.T. 3. E-02 (a) No sample available; unit being repaired.

               - - - _ _ _                    - _ - - - - - - _ - _ _            - , - - - - - - - - - - - -             - _ ---- _ _ -- --              -- --    - - - - - - - -            -- .-+

g g g g g m M M M M M M M E E E s TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES stall 04 NUNSER A.7 -30 lyst COLLECil0m SATE Mio COUNT A P FILTER START STOP M10 COUNT CHARCOAL FILTER 11ME GROS 5 SETA DATE SATE VOLUME UNITS DATE (pCl/Ca. M.) TIME l-131 DATE (pCl/Cu. M.) 12/31 01/07 9.77E 03 CU. FT. 01/15 2.4 1 0.3 E-02 01/11 L.T. 2. E-02 01/07 01/14 9.84E 03 CU. FT. 01/25 2.5 t 0.4 E-02 01/16 L.T. 1. E-02 01/14 ,, 01/22 1.12E 04 CU. FT. 01/30 2.0 2 0.3 E-02 01/24 L.T. 2. E-02 b 01/22 01/28 8.21E 03 CU. FT. 02/06 1.9 1 0.4 E-02 01/30 L.T. 3. E-02 01/28 02/04 9.68E 03 CU. Fi. 02/11 2.2 a 0.4 E-02 02/07 L.T. 2. E-02 02/04 02/11 9.6M 03 CU. Fi. 02/21 3.2 2 0.4 E-02 02/13 L.I. 2. E-02 02/11 02/18 9.68E 03 CU. FT. 02/26 2.8 a 0.4 E-02 02/21 L.T. 2. E-02 02/18 02/25 9.65E 03 CU. FT. 03/05 1.7

  • 0.3 E-02 02/27 L.T. 2. E-02 02/25 03/04 9.83E 03 CU. FT. 03/13 1.7 1 0.3 E-02 03/06 L.T. 2. E-02 03/04 03/11 9.80E 03 CU. FI. 03/20 2.0 1 0.3 E-02 03/13 L.T. 2. E-02 03/11 03/18 9.84E 03 CU. FT. 03/26 1.9 2 0.3 E-02 03/20 L.T. 2. E-02 03/18 03/25 9.90E 03 CU. FT. 03/29 1.6 2 0.3 E-02 03/28 L.T. 2. E-02 03/25 03/29 9.8M 03 CU. FT. 04/08 2.2 a 0.3 E-02 04/03 L.T. 2. E-02

M - M s TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CilARCOAL CARTRIDGES: GROSS BETA AND 10 DINE-131 ANALYSES STAil0N NUNSER APE-30 tyst COLLECil04 SAIE Mle COUNT A P FILIER MIU COUNT START STOP CNANC0AL FILTEM IBM GA055 3 ETA IIM l-131 SATE DATE VOL UM UNIIS DATE (pCi/Co. N.I DATE (pCi/Co. M.) 04/01 04/09 1.llt 04 CU. FT. 04/16 2.1

  • 0.3 E-02 04/11 L.T. 2. L-02 04/09 04/15 9.43E 03 CU. Fi. 04/25 2.4 2 0.4 E-02 04/18 L.T. 2. E-02 04/15 04/22 9.87E 03 CU. FT. 05/01 2.3 2 0.3 E-02 04/24 L.T. 2. E-02 04/22 04/29 9.9M 03 CU. ft. 05/24 2.4 1 0.4 E-02 05/01 L.T. 2. E-02 b 04/29 05/06 9.0M 03 CU. ff. 05/14 1.9 2 0.3 E-02 05/00 L.T. 2. E-02 05/06 05/13 9.99E 03 CU. FT. 05/21 2.0 2 0.3 E-02 05/16 2.

L.I. E-02 05/13 05/20 9.95E 03 CU. FI. 05/31 2.0 t 0.3 E-02 05/23 3. L.T. L-02 05/20 05/27 1.00E 04 CU. ft. 06/06 2.5 1 0.3 E-02 05/30 2. L.T. E-02 05/27 06/03 9.9M 03 CU. FT. 06/17 2.2 2 0.3 E-02 04/05 2. L.T. E-02 06/03 06/10 9.02E 03 CU. FT. 06/19 2.6 2 0.4 E-02 06/13 2. L.I. E-U2 06/10 06/17 9.94E 03 CU. FT. 07/02 1.6 r 0.3 E-02 06/19 2. L.I. E-02 06/17 06/24 1.02E 04 CU. FT. 07/10 2.0 1 0.3 E-02 06/26 2. L.T. L-02 06/24 07/01 1.0M 04 07/15 07/15 2.5 1 0.3 E-02 07/03 2. L.I. E-02

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63 I

M M i TABLE B-3 AIR PARTICULATE FILTERS: CADe(A ISO 10PIC ANALYSIS ON QUARTERLY COMPOSITES (pCl/Cu.N.) STATION auMSES APC-1 GA8MBA SPECitDN AGALT515 FIRST QUARTER SECONS QUA8IER THIRD QUAkiER FOURIN QUAkiER 12/31-04/01 04/01-07/01 07/01-09/30 09/30-12/30 SE-7 8.864 0.95E-02 9.03t 1.27E-02 8.04: 0. 80E -02 9.49 0.9hE-02 R-40 L.T. 1. E-02 L.I. 3. E-02 5.22 22.92E-03 1.021 0.3nE-02

     ,   Me-54                       L.T.                7. E-04          L.I.                       1. E-03  L.I.       4. E-04       L.I. 7. E-04 CO-54                       L.I.               8. E-04                                     1. E-03   L.T.

L.I. 5. E-04 L.T. 3. E-04 FE-59 L.I. 2. E-03 L.T. 3. E-03 L.T. 1. E-03 L.T. 2. E-03 C0-60 L.I. 1. E-03 L.I. 1. E-03 L.I. 4. E-04 L.I. 9. E-04 2m-65 L.T. 2. E-03 L.T. 3. E,03 L.T. 1. E-03 L.T. 3. E-03 2R-95/st-95 L.I. 8. E-04 L.I. 1. E-03 L.I. 5. E-04 L.I. 8. E-04 RU-103 L.I. 1. E-03 L.I. 1. E-03 L.I. 6. E-04 L.I. 1. E-03 AU-106 L.T. 6. E-03 L.I. 8. E-03 L.I. 4. E-03~ L.I. 6. E-03 1-131 L.T. 7. E-03 L.7. 7. E-03 L.I. 7 E-03 L.I. 5. E-03 C5-134 L.I. 8. E-04 L.I. 1. E-03 L.T. 5. E-04 L.T. 9. E-04 C5-137 L.I. 7. E-04 L.T. 1. E-04 L.T. 4. E-04 3. L.T. E-04 SA-140/LA-140 L.T. 3. E-03 L.I. 4. E-03 L.T. 1. E-03 L.T. 3. E-u3 CE-141 L.T. 1. E-03 L.T. 2. E-03 L.T. E-03 L.T. 1. l. L-03 CE-144 L.I. 3. E-03 L.I. 5. E-03 L.T. 3. E-03 L.T. 4. L-03 RA-226 L.I. 1. E-02 L.T. 1. E-02 L.I. 9. E-03 L.T. 1. E-02 TH-228 L.T. 1. E-03 L.T. 1. E-03 t.T. 9. f-04 3. L.T. E-03

M TABLE B-3 (Cont.) AIR PARTICULATE FILTERS: GMetA ISOTOPIC ANALYSIS Oli QUARTERLY COMPOSITES (pCl/Cu.N.) STAil0E NUNSER APG-1 GANNA SPECiaun ANALI5Is Flest 00ARTER SECONS QUARTER TNIRO QUARTER FOURTH QUARTER 12/31-04/01 04/0l-07/01 07/01-09/30 09/30-12/30 SE-7 9.61t 1.41E-02 7.314 0.89E-02 8.53 10.79E-02 1.01 to.!!E-01 E-40 1.864 0.92E-82 L.T. 9. E-03 L.T. 9. E-03 3. as L.T. E-02 u Ms-54 L.T. 9. E-04 L.T. 5. E-04 L.T. 4. E-04 L.T. 1. E-03 4 CO-58 L.T. 1. E-03 L.T. 6. E-04 L.I. 6. E-04 L.T. 1. E-03 FE-59 L.T. 3. E-03 L.T. 1. E-03 L.T. 1. E-03 L.T. 3. E-03 CO-60 L.I. 1. E-03 5. E-04 5. E-04 L.T. L.T. L.T. 1. L-03 25-65 L.I. 3. E-03 L.I. 1. E-03 L.T. 1. E-03 L.T.

2. E-03 2R-95/08-95 L.T. 1. E-03 L.T. 6. E-04 L.T. 5. E-04 1.

L.T. E-03 AU-103 L.I. 1. E-03 L.T. 8. E-04 L.I. 7. E-04 L.I. 1. E-03 80-106 L.T. 9. E-03 L.T. 5. E-03 L.T. 4. E-03 8. , L.T. E-03 1-131 L.T. 9. E-03 L.T. 8. E-03 L.T. 3. E-03 L.T. 6. E-03 C5-134 L.T. 1. E-03 L.T. 6 E-04 L.T. 5. E-04 L.I. 1. E-03 C5-137 L.T. 1. E-03 L.T. 5. E-04 L.T. 6. E-04 L.T. 9. E-04 BA-140/LA-140 L.T. 4. E-03 L.T. 4. E-03 L.I. 2. E-03 L.T. 3. E-03 CE-141 L.T. 2. E-03 L.T. 1. E-03 L.I. 1. E-03 2. L.T. E-03 CE-144 L.T. 5. E-03 L.T. 3. E-03 L.T. 3. E-03 L.I. S. E-03 RA-226 L.I. 1. E-02 L.T. 9. E-03 L.I. 1. E-02 L.I. 1. L-02 TH-228 L.I. 1. E-03 L.I. 9. E-04 L.I. 8. E-04 L.I. 1. E-03 i

M TABLE B-3 (Cont.) AIR PARTICULATE FILTERS: GAlen ISOTOPIC ANALYSIS ON QUARTERLY COMPOSITES (pCl/Cu.M.) STATION NUNSER APP-1 GAfstA SPECTRUM ANALV515 FIRST QUARIER SECONO QUARTER 12/31-04/01 THlk0 QUARIER FOURIN QUARTEk 04/01-07/01 07/01-09/30 09/30-12/30 SE-7 9.364 1.16E-02 8.30s 0.70E-02 7.15 t0.72E-02 s.00t 0.10E-02 K-40 3. E-02 L.T. L.T. 1. E-02 5.17 s3.03E-03 3.06 1.Olt-02 g 10a-54 L.T. 9. 4-04 L.T. 4. E-04 L.T. 3. E-04 L.T. 9. E-04 CO-53 L.T. 9. E-04 L.I. 5. E-04 L.T. 4.' E-04 L.I. 1. E-03 FE-59 L.T. 2. E-03 L.T. 1. E-03 L.T. 9. E-04 L.T. 2. E-03 LO-60 L.T. 1. E-03 L.T. 4 E-04 L.T. 4. E-04 L.f. 8 E-03 2N-65 L.I. 2. E-03 L.T. 1. E-03 L.T. 7. E-04 L.I. 2. E-03 ' 28-95/as-95 L.T. 1. E-03 L.T. 5. E-04 L.T. 5. E-04 L.I. 1 E-03 RW-103 1. E-03 L.I. L.T. 5. E-04. L.I. 5. E-04 1. L.I. E-03 AU-106 L.T. 7. E-03 L.T. 4. E-03 L.T. 3. E-03 L.T. S. E-03 1-131 L.T. 8. E-03 L.I. 3. E-03 L.I. 2. E-03 L.I. 5. E-03 C5-134 L.T. 9. E-04 L.T. 5. E-04 L.T. 4. E-04 L.T. 9. E-04 C5-137 L.T. 8. E-04 L.T. 5. E-04 L.T. 4. E-04 L.I. S. E-04 5A-140/LA-140 L.T. 5. E-03 2. E-03 L.I. L.T. 1. E-03 L.T. 4. t-03 CE-141 L.I. 2. E-03 L.T. 1. E-03 L.T. 1. E-03 L.T. 1. L-gj CE-144 L.T. ;4. E-03 L.T. 3. E-03 L.I. 3. E-03 L.T. 4. E-03 RA-226 L.T. 1. E-02 L.T. 9. E-03 L.I. 9. E-03 ! L.I. 1. t-Og TH-228 L.I. 1. E-03 1.I. 9. E-04 L.I. 9. [-04 t.I. 2 g-uJ e,__, _ _ , . - _ -. - _ _ . , , , , ._ _. _ _ _ _ _ _

TABLE B-3 (Cont.) AIR PARTICULATE FILTERS: CAlelA ISOTOPIC ANALYSIS ON QUARTERLT COMPOSITES (pCS/Cu.N.) STAil05 NUNSER APQ-1 6 ANNA SPECTRUN AGALV5I5 FIRST QUARTER SEC0a0 QUARTER INIRO QUARTER 12/31-04/01 04/01-07/01 07/01-09/30 FOURIN QUANTER 09/30-12/30 SE-7 8.624 0.86E-02 8.714 0.97E-02 8.44 sl.50E-02 3.35 0.94E-02 E-40 L.I. 1. E-02 L.T. 3. E-02 1.37 to.55E-02 9. L.I. E-03

  ,                        NN-54                                                  L.T. 5. E-04 u                                                                                                          L.I. 9.                  E-04   L.T. 8. E-04   L.T. 4.              L-04 CO-58                                                  L.I. 6. E-04          L.I. 1.                  E-03  L.T. 3. E-04   L.I. 5.             1-04 FE-59                                                  L.T. 1. E-03          L.T. 3                    E-03  L.T. 2. E-03   L.I. 1.             E-gj CO-60                                                  L.T. 5. E-04         L.T. 8.                   E-04  L.T. 7. E-04   L.T. S.             E-04 2N-65                                                         1. E-03 L.I.                      L.T. 2.                   E-03  L.T. 2. E-03           1.

L.T. E-u3 2R-95/us-95 L.1.' g. E-04 L.T. 1. E-03 L.I. 8 E-04

                                                                               '                                                                                  L.I. 6.              E-04 RU-103                                                  L.T. 6. E-04         L.T.
1. E-03 L.T. 1. E-03

! L.T. 6. L-04 AU-106 L.T. 4. E-03 L.T. 7. E-03 L.I. 7. E-03 L.I. 4 E-03 1-131 5. E-03 s L.I. L.T. 6 E-03 L.I. 5. E-03 1 L.I. 3. E-03 4 C5-134 5. E-04 L.T. L.T. 9. E-04 L.I. 9 E-04 L.I. 5. E-b4 C5-137 L.T. 7. E-04 L.I. 9. E-04 L.I. 8. E-04 L.T. 6 E-04 BA-140)LA-140 x L.T. 2. E-03 L.T. 3. E-03 L.T. 2. E-03 L.I. 2. E-u3 C E - 141 L.I. 1. E-03 L.I. 1. E-03 L.T. 2. E-03 L.I. 1 E-03 CE-144 L.T. 3. E-03 L.I. 4 E-03 L.I. 5. E-03 L.T. 3, E-03

          ,               RA-226                                                 L.I. 9     E-03         L.I. 1.                   E-02  L.I. 2. E-02 TH-228 L.I. 8               1-uJ t.i. 3.    [-0)         L.I. 1.                   E-03  t.I. 2.   [ -;;j (,y,   9,              g,g,

e m M M TABLE B-3 (Cont.) AIR PARTICULATE FILTERS: CJd9fA ISOTOPIC ANALYSIS ON QUARTERLY COMPOSITES (pCl/Cu.M.) STAitou NUNSER APE-30 SANNA SPECiaun ASALV515 FIRST QUARTER SECONO QUARTER INlED QUARIER FOURIN QUANTER 12/31-04/01 04/01-07/01 07/01-09/30 09/30-12/30 SE-7 9.12* 0.9IE-02 8.80s 0.69E-02 ! 8.93 to.92E-02 8.26 0.83t-02

K-43 L.T. 1. E-02 8. E-03 L.T. L.T. 2. E-02 L.T. 1. L-02 Ms-54 L.T. 4. E-04 L.T. 4. E-04 L.T. 7. E-04 L.T. 6. E-04 CO-58 L.T. 6. E-04 L.T. 5. E-04 L.T. 8. E-04 L.T. 5. E-04 FE-59 L.T. 2. E-03 L.T. E-03
1. L.T. 1. E-03 L.T. 2. E-03 CO-60 L.T. 7. E-04 L.T. 4. E-04 L.T. 7. E-04 L.T. 5. E-04 2n-65 L.T. 1. E-03 L.T. 1. E-03 3

s L.I. 2. E-03 L.T. 1. E-03 2R-95/n8-95 L.T. 7. E-04 L.T. 5. E-04 8. E-04 L.T. L.T. 7. L-04 RU-103 L.T. 9. E-04 L.T. 6. E-04 L.T. 1. E-03 L.T. 7. E-04 88-106 L.T. 4. E-03 L.T. 4. E-03 L.T. 7. 1 E-03 L.T. 5. E-03 l g-131 L.T. 5. E-03 , L.T. 4. E-03 L.T. 4. E-03 L.I. 4. E-03 ! C5-134 L.T. 6. E-04 L.T. 4. E-04 L.T. 7. E-04 L.T. 5. E-04 C5-137 L.T. 5. E-04 L.T. 4. E-04 L.T. 7. E-04 L.T. 6. E-04 B A-140/L A-140 L.I. 2. E-03 L.T. 2. E-03 L.T. 3. E-03 , L.T. 2. E-u3 CE-141 L.T. 1. E-03 7. L.T. E-04 L.T. 1. E-03 L.T. 1. L-03 - 1 CE-144 L.T. 3. E-03 L.T. 2. E-03

                                                                    ,                                                               L.T. 3. E-03   L.T. 3    E-03 l                RA-226                                                L.I. 1. E-03                            6. E-03 L.1.                     L.I. 8. E-03   L.T. 9. t-03 TH-228                                                L.I. 9. E-04                    L.T. 6. E-04         L.I. 9. E-04   L.I. 9,   g.u4

o M M M M M M M M

                                                                                                                                                                                                  ~

i

                                                                                         /

s l'ABLE . B-4 DRINKING WATER:

   =
                                                          .i IODINE-131 ANALYSIS

_ (PC1/1) Gaff - STAT 100 OWG-2 _ CWE-5 Oup.7 12/24/84-01/87/05 L.T. 5. E-01 L.I. 5. E-01 L.T. 5. E Oh s 01/07/85-01/22/35 L.I. 5. E-01 (a)' L Y. 4. t.01 01/22/85-02/05/8b L '. i . 4. t-G1 L.T. 5. L-01 L.I. 6. L-01 01/86/85:02/18/85 t,I. 5. -E 01 L.is 4 E-01 L.I. 5. E-01 02413/85'-03/04/is5 L.f. 3. E-01 8 1. .3. E - 01 L.T. 3. E-ul 03/04/85-03/18185 L.T. 3. E-01 . (a) L.T. 2. f-01 g 03/18/85-94/01/45 L.I. 3. E-01 L.I. 4. E-01 L.I. 4. E-01 04/01/85-04/15/85 L.I. 4. E-01 L.I. 4. E-01 L.T. 4. E.01 04/15/85-04/2f/85 L.I. J. E-01 L.I. 3. E-Of L.T. 4. E-01

                                                                                                                                                                                                      ~

04/29/85-Ob/13/85- L.T. 5. E-01 L.I. 5. E-64 L.T. 4. L-01 05/13/85-05/27/85 L.T. 3. E-01 L.I. 4. E-Cl L.I. 3. E-Og 05/27/85-06/10/85 L.I. 3. E-01 L.I. 3. E-01 L.I. 3. E-01 06/10/85-06/24/85 L.T. 3. E-01 L.I. 3. L-01 L.T. 2. L-01 s 06/24/85-07/08/85 L.I. 5. E-01 L.T. 8. E-01 L.T. 4. E.0g ( a) Sample not available due to sampler salfunction; lasufficleat volume. t 1

     , , - - - - - - - - -     .~ -. , ,.                    n - - , . , - - - --- -_.           ,       -            . . - - . . .     . _ _ _ _ _ - _ _ _ _ _ _ _ _ . _ _ _ - _ _ _ - -                  ___       ____-_ __ - - ___ - _____ -_

i M M M M M s TABLE B-4 (Cmt.) DRINKING WATER: 10 DINE-131 ANALYSIS (pct /1) CSLLECile8 SAIE STAilee SWG-2 Suf-5 Dur-7 87/88/85-87/23/85 L.T. 2. E-01 L.T. 2. E-01 1.1 2. E-un 87/23/85-88/85/45 L.T. 5. E-01 L.I. 5. E-01 5. L.I. E.on 88/85/85-88/19/85 L.T. 4. E-81 L.I. 4 E-01 L.I. 4 L-o! 88/19/85-89/43/85 L.I. 3. E-81 L.I. 3. E-01 5. L.I. E-ol 49/83/85-89/16/85 L.I. 4. E-01 L.T. 4 E-01 4. L.I. E-on 89/16/85-89/34/85 L.I. 4. E-81 L.I. 3. E-01 L.T. 5.

     $      49/38/85-18/14/85                                                                             L.T. 4. E-81 L-o!

L.I. 3. E-01 3. 18/14/85-18/28/85 L.I. E-u! L.T. 2. E-41 (a) L.I. 2. E-41 L.T. 2. L-on 18/28/05-11/11/85 L.T. 3. E-01 L.I. 3. E-01 4. L.I. E-ol 11/11/85-11/25/85 L.I. 4. E-01 L.I. 4. E-01 L.I. 4. g-og 11/25/85-12/89/85 L.I. 2. E-01 (b) L.I. 2. E-01 L.I. 4. t-on 12/18/85-12/23/85 L.I. 4. E-01 L.I. 4. E-01 t.T. 5. g-o! a h Collecttoe dates 10/15/85-10/28/85 Collecties dates 11/25/05-12/18/85

 ---   -_        - _ - - - - . - - - - - - - - - - - - - - - - - - - - - - - . , - - - , - - -                ,       _,--wm,-_-.
                                                                                                                             -      - _- . . _ e _ _ - - . - - _  _a---w---.     ,,w-. _. ,.-wn--,., u. -,,,e-,e   -,www,,      w,...,m,.r,     . , , ,m -   --p.

I I .O O O naa w w w _ O O 0 0 0 0 0 O O O O O O O O O O O 0O0 O0 0O0 has has naa w w tea w nas tes w w w w O O O 3 a .4 I m . e . . . . . . . . . . . . . 30 *" M *n M M O M W M M M d M M w

  • W e N N 4 q.
                                   == O,.                         .        .      .      .        .      .       .      .      .       .       .       .       .

3% a= . . . . . a= e= a= e= N M. e=. . e=. . . a=. . a=. . e=. e

                                                                                                                                               . e=. e.
                                                                                                                                                                   >       em om        e-
                                                                                                                                                                                                      >=.

w O e .a .J .a -a -s =s .a .a .a -s .a

                                                                                                                                                                            .a
                                                                                                                     -d                                     -s   . .a               w           a w I                                                 O O          ==. == O O O O O O O .* O O O O O O O O O O O O O O O O O

O O O

                                                                                                                                                                                   .= == O O O O e           w           ins I                                    a.

tea tea tea ina ene ens nas w w w ins tea nas ins nas i.e ins m% gN M. . . . . . . . . . . . . . . . . 40 .e M w M M e M N M w M e M M e e N  % e

                                                                                                                                                                                                         . i 2 e                                                                                                                                                                          ,

WN es M aN . . . . . . . . . . . . . . . . . . e W em em em ao en en e= e= te em >= t/3 ina g .%. N. . . a=. . . . . e=. . e=. e=. . . . . or em t- t

               >                      O          N            -s         a    .a     w        .a        a    os     .a      .a     .a      .a         a            .a      w
                                                                                                                                                                                             .a
                                                                                                                                                                                                .       .      r a                    .a                a         !

M N U W e f M N O Se M 3 . M t/3 O i M O ' in F4 O ' I M O h *"* ^ see g =. O O O O O O O O O O O =* ** O O ==e O ** == O i W U *=* e O O O O O O O O O O O O O p.3 .u.4 3 2 N N i.e i.s i.a w is s w i.a i.s ns w i.s w w i.a i.e i.e w 6.s 64 ee G ,

                   .De3      a   =%

y m e. N. . m. . . . . . p w S 4O O e N M w e M N w in M M w M M

                                                                                                                                                                                            *=.

N U O - .e .e . em (N  ; O 4 "3 % me em

                                                               . en a

em N .s to. e.. em. e= em se en em 2: a

                                                   .                                                 em. a=. em. a=. e=. en.n en.                            .               .

e i

                                     =           ==          a
  • s a . .
           .g                                                                                          a a w                                                                                                   l I                 O a                                          .a     w a               a     .a              s                                    t
            =

S i f./3 US I O M O 1 i I

                                             ..         epg en          .=
               .                            ==

We to. n l

                                            >           .a                                                                                                                                                      I i

a 4 4 3 O 4

                                     .. g e                  S w         a         2                                                                                                        O
                                    >      4           5 W      W           e=                                                                                                        w efe                                           me ind    ==          W                                                           S I

e

                                    .a     E           tea                                                          e                                            4 w      ina         e.                                                          as                                              a O      2           to                                                          a                                             %

W eg  % M to w h O a. e e ao

                                           .G                                w G e O en                            in O                  .mo     M       M       w w e                      N        N ied      =  S           h        O ta en efe                     @     q       S      an.    .O mo     M       sus     amo     se      .e      s=.        N       N a=     O     e           4       w        e      4       e       a      e       e      4      0      .4       e        e       4      4        4         e        a 4      4 I

5 4 eaa e S O taa O E E 3 3 44 th 4 ina 4 2 O m WW e ad E W is. W N ene e a ** W W e e nas W W W >= 71 i i

O 9 O ** O =* OO OO OO OO OO OO OO O == OO ==O0 O OO O OO == O

                                                                                                                                                                                                                                                                         .=O 3 3

N tad W w med tad tad

                                         %                                                                                   had         tea              tad        w w                  tad             tad         w          tas           w w                         w               =s I                                  tea E

ON 9N a are

                                                      =*
                                                       *e
                                                         =

M w M M N M 4 w o= 9 M N 8"I M S W M 30 4 0 . >=. a=. e=. N. >=. ==. e=. >=. e=. a=. e. n= 4 4 4 e e a

                                                                                                                                                           .                                               .        >=. a=. e=. a=. e=.

J d a e e e a a e e a a a

                                                     ==

N O =. O O==O OO OO OO OO OO OO OO== O OO OO OO O O O .=O == O O 0 I N tas tad tas ned has tad

                                        %                                                                                 tea         tad              tas        tad        ned       tas             tee         tad         tad          tas            tad          td              w            I en a= O               N.                .          .         .          .           .         .            .               .

4 e O M en M M @ 8"I E in @ M e M e M M @ N M e N

                                       ==            4e UI                    %                               .          .

I W w a= U3 D O. >=. N. s=. >=. >=. . a=. e=. e=. a=. n=. e=. a=. >=. e=. e=. a=. a=

                                                    ==                                              -a
                 >*                                                -s         .a         =d                    -d            d       -s .4 .d -a .a .a -a .4                                                                                  d           .d           a a

t/3 N O W e M f.e W A. .. m., i.e 3 U W t/3 G C W H I g C ' U V y M ^ tad as O O

                                                                  == == O O O O O O O == =. O O O O .=

I U M e

                         %,e 5 M       .en.*        nee O O O O O O O O O O O O O O O O O OO tad        tas        sad       na/         tad
                                                                                                                                                                                                                                                                    -a                               -

a .ze >.  % had tad nad had tad nad has tad tad nad tad ted a a .a e 4 had

                                 == O                                .          .         .

Ca3 v W me =o w wt M M d O

                             ==
e. W ag ==

e% e as e en M se w e N as M e a3 W'"8 O >=  % es O 'C M @

                                                                    .          .          .         .           .          .           e               .          .          .          .               .           .          .

I

                             ==                                  8=         >=         $=        >=                                a=

O em. I 9= D= t= to

                                                     .              .          .         .          .        >=.          .           .                .                             e=. e=. a=.                            o=

a=. .=. == I N -s -d a .d as a -s d .a

                                                                                                                                                                  .          .                                                 .                                    m.                   .           !

d .d .a .a .d .4 a a a H< rd3 8 tJ3 V3 C og U I a en

                                             ==

en. 3

                                                           =

opt In 9=

                                                           =d ed            EC 4             5
                                      . k              =

tas -a 3

                                   >=       4             e                                                                                                                                                               O b3       tJ            >=

idt e I nas == W s.e

                                   .4       E             tad 96                                                                       e e
                                   -d       tes           a.                                                                                       e                                                                      at O        3             en                                                                                                                                                                 s W         41                                                                                                     a                                                                      %

G  % dut O w N O es e 4 e 6 m O en eft en tas == m N O 4A eft eft O O =e M M w w w N N o= G @ te Gb ao e.e M ano =e N e e e e ame sm. ae N I e e e e e e se 4 8C & 4 tad O

  • e e e e e a e O W WW G e lad O sW W 3 3 e t#t t#9 EC tea *C E e

ad W te. W pe N g a me y u a u u eg ned e-

                                                                                                                                                                                                                                                               #                                      l l

l 72

                                                                                                                                                                                                                                       ,           , -.-             .e.-    -w-           - -

M M M M M M M M TABLE B-5 (Cont.) DRINKING idATER:

                                          \

CROSS BETA AND CA MA ISOTOPIC ANALYSES ON MONTHLY COMPOSITES (pci/1) STATION - OhG-2 JULT AUGUST DATE COLLECTED: 06/24-07/23 SEPTEMBER 07/23-09/01 09/03-09/30 RA010CNENICAL ANALV515: GR-8 7.8 a 1.7 E 00 6.8 s 1.2 E 00 7.2 a 1.5 E 00 CANNA SPECTRUM ANAL V515: B(-7 L.T. 4. E 01 L.T. 3. E 01 L.I. 3. E O! K-40 L.I. 5. E 01 L.T. 5. E 01 L.T. 5. E 01 Ma-54 L.T. 3. E 00 L.T. 3. E 00 L.T. 3. [ 00 CO-58 3. E 00 L.I. L.T. 3. E 80 L.T. 3. E 00 TE-59 L.T. 9. E 00 L.T. 7. E 00 L.T. 6. E 00 C0-60 L.T. 4 E 00 L.T. 3. E 00 L.I. 3. E 00 25-65 L.T. 7. E 00 L.T. 7. E 00 L.I. 6. E 00 i 2R-95/NS-95 4. E 00 L.T. L.T. 4. E 00 L.T. 3. E 00 RU-103 5. E 00 L.I. L.T. 4. E 00 L.T. 4. E 00 20-106 L.I. 3. E 01 L.T. 3. E 01 L.I. 2. E O! I til L.T. 3. E 01 L.I. 2. E 01 L.I. 9. E 00 C5-134 L.T. 4. E 00 L.T. 3. E 00 L.T. 3. E 00 C5-137 L.T. 3. E 00 L.T. 3. E 00 L.T. 3. E 00 SA-140/LA-140 1. E 01 L.I. L.T. 9. E 00 L.T. 6. E 00 CE-141 L.T. 9. E 00 L.T. 7. E 00 L.I. a. E 00 I CE-144 L.T. 2. E 01 L.I. 2. E 01 L.I. 3. E 01

                 ..RA-226                                     L.I. 7    E 01        L.I. 7. E 01     L.T. 6    E 01 IH-228                                     L.I. 7    E 00        L.I. 7. E 00     L.I. 7. t Du 1
  . - -   .   --               . ,   -    --   . . _   ._ ~      _          _-.

I 3N M O O tad

                                                                             ==*

3 O O== O ned tad had OO ins O O ned O O nad O O tad O OO 3O3==O == OoOo3 o3 o o= 3o ted% had had ned and nad W end med had .ma w I I,Ne e e . . . . . . . . ned e *=*

  • T T T O T e Wen T =ft * =* W T 3 8J M 3 3 ned N *e o .g . .e em e-e.=
                                               ..e em         om         en                                            se         om.        >=         e-              >=

ee. >=. em. I

                                                                .               .          .         .           .           .                                                                                                                          om         a=          e=
                                                            **.             w          .d        ad
                                                                                                                                       .                                            .          .           .         .                .      >=.           .          . .

a a .d .A s a .d -d -d -d d .J e e .e I O W O _ _ O O O O O O O O O O O O O O _ _ _ O O . en O O O O O O O O O I e e e at N tad e e has med led tas ts.s nas ned ene % had ted tad tas tad tad tad tas =s .e .e 84 i_se . . . . . . . . . . . . ned e .= 36 am e . . DG N M e N -. == @ N N N - est e == N ON es 3% . . . . t/3 O e >= >= e= >= gal =* * * *

  • e== e- *= *= *= o= e. e- >= p. m. e. a.

I ga e .d a d

                      >                                                                                        e         d           d       .d          d          e          .d             a          a       .d                 s         d        -,                    .4 s

I e u p f

e. ..
a. ee N W N Q e r I

C". Dt] te W y O N O 3 L

              <                      O                    O 3      me p        ^                                           == == 0 O O O O O O O O O O O O O O O O O== O                                                                                                O O O ='. ==
                                                                                                                                                                              .ie O

M e e N tad tas tad ted O O O O ON O O . z **'.=4

                              .u     W  W                                                                 had        tad        tad        had                  tas M

e e-a

                           >  n      O  ta,  %            .

ned tad tea tad nad tea tad tad gas tee f J 5 == e .C. . . . . . . e* Oe . . . . . . M y 4 a-. W W ful w fan . M e T nn M

   .,,3       e.e                    >=

a= O Wm ao M w e ==. m - e

                                                          *e g                we Os                                  .          .         .           .          .                                                                                                                                                         i i
      ]                                      O              .

D=

                                                                            .       >=.       >=
                                                                                                 .        se.

e-ee

                                                                                                                                           >=        p.        em            p.         gm.        em          p.            >=

em e-td'l .4 a e ed .ms ed -d ad ad

                                                                                                                                                                  .              .          .          e          .               .          .          .       ==.             .

ed -d ad .d .d w .# =# s M M I rn I b in O < I e

                   ,                                M e.

to D en

                                                                   ==

en am

                                                                   .d I
                                                    .d             4 4              3 S              4
                                            ..      eg S                       E ens      -w             2
                                           >=       4              m                                                                                                                                                      O W       W              em                                                                                                                                                       W eft I

nas == W se

                                           .d      3                                                                                                Ge                                                                       e tes                                                                                e
                                           .s      tes            a.                                                                                e                                                                     4 O         E             wt                                                                                                                                                           a W        W                                                                                                S                                                                     %

Q 4 W  % M q w N O me e @ W tad == G E N O en G S O tdt eft O O am. #83 fut e w w N N

                                          *=                                                             eft       tdl         @         W          S         s.e           s.e        fut        a.e         me O              5                                                                                                                                                       sue            ano       s          N           N I

e e 9 e e e e e e e sus 4 4 W 4 tes e g O e e e e e e e e O M W W tad O 3 *=dm 3*=d 3 e wt to 4 4 E e ad a W te. W a e == W W e W tea ned W e *= 74 l

em= 0 =* == O O O O O O O == == 0 C O O == == y O 3 O O O O O O O O O O O O O O O O O o

                                     ,            and           tad      w       tad    w w w                      tad     led             w O

ned had ned has ted 4.d w =a me

                                                  =*

3Q g W en M M N M @ M 4A M N M w uo St @t M S 3 "3" %

                                                                                                             . e.

em O w ad me =d =d ad =d ad ad =d =d -d -d

                                                                                                                                                                      =d       me d
                                                                                                                                                                                                 =d
                                                                                                                                                                                                         =d me I                                               O O             == ==* O O O O O O O == O O O O O O O O O O O O O O O O O O O O
                                                                                                                                                                                                == ==

O O 3 O . e tad tad ned nas tad ned tad W tas nas ese tad ted tad e se ted had ned tea tea == gN O. . . . . . . . . . . . . . . . E 4O M w M

                                                                                                                                                                                                   .       .             =            9 a=e                                    M        96       8's      @       M       w M              $        f'l      M        @       N         M      %             %

2e @ a e%d *e W g og . . . . . . . . . . . . . S M tad % @ e= om em e-W w .= . >=. a=. e. . . a=. e=. . a=. e=. . a=. . e=. . De om o=

                                                                                                                                                                                                                                      ,e p                       C           M               ad       ad        d    and      ad       ed       -d      ed      -d      -d      =d        and      d        d       ad
                                                                                                                                                                                               =d      eme           ad              .

s G eo . M 4# 6 e Q ag =A S*G a=e N ' tad 3 O'=" 3 e .. Se N M M "OEO O * *

  • e O e - e.==

IvQ .sg ^ A E3C d a w 3  %=

                                  ===

4 O O

                                                              == =* O O == tp                                    @       O O ==                   N        O O ==                    =e       ==       se           O         .e me  e. es tme                                 O O              O O O               O O O Q O O O O O O O O O O   O              4 e h            w              w w w w w w w                                              w'W                                                                                                   .wn. w    .

m 8 2 e=4 e3 a n= O w w w w w w w w w wdm

                                                                                                                                                                                                                              ..e=

W w m .%

                                               ==

Em1 X 5 4O

                                   =              .              .       .       .      .        .        .        .       .       .       .        .        .        .         .       .        .       .             .         e3 at
                                                                                                                                                                                                                                    ==
                                                                                                                                                                                                                                         ,3
                                               =*            *A        @       M      w       me       w         N       en     on.      M                 w w
   ]   g                  O   2e ame                         N       suo      M       St            e            C=C e g.

at A ** e= 4N C O 4 "A % w

                                                                .                .      .        .        .        .       .       .       .        .        .        .        .        .        .       .             .        OgO es      ese      em        em      >=              em                                                   e=

om W . e=. . e=. . . . . . a=. . a=. em. e=. a=. >=. >=. e= ee g e.e M =* w ad =d -d -d .d .J aJ -e me =d =d .d =d .d .d ad

                                                                                                                                                                                                      -d            d e3 e.2 3es 99D=

M N Gd W g N U == y == o M O-O a m a. es 3m 9

                                                                                                                                                                                                                              %          e OOO Nw%
                                                                                                                                                                                                                              ====M C eo            j 9         i Gw$
  • o%o bo6 i w w ==

I i

                                                         **                                                                                                                                                                         me
                                           **           M                                                                                                                                                                     D eD i

M == ed 4 es i

               /                          ==           M                                                                                                                                                                      ee a =e         i M             3"                                                                                                                                                                    w          w 3=                                                                                                                                                                                                  l
                                          =d           4
                                                        =#
                                                                                                                                                                                                                             .ef= g4.==   e I

4 W . ==== S 4 O o l

                                  *. 4                                                                                                                                                                                    w as u e                      E                                                                                                                                                                           e tae      -d            D                                                                                                                   o                                                 eae
                                                                                                                                                                                                                             == =

i D= 4 5 e W W o= 4A me

                                                                                                                                                                                                                              & es &
                                         ==            u                                                                                                                                                                      EOE I

nas

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e. d W
                                 .d O

tee 3 to e .mo O W S  % O ad O Q %M 99 W N O == w @ W O W .ms E ta == G Pe O e e tAen enO is 4A la en O O sue == #se see e er w N N e.d 43 $ one M se sue ano =e ese N N E e e e e e e o e e e e ese e I e e e e e e 8=.am.=m. 4 4 5 4 tad a j O tad O 3 m 3 3 to M 4 l e e m == u u e u w as 4 Z e led es 48 ta e ad a w w w N N nad 9aw o= ww  ! P 75

1 l I T N 4 O O tad N

                                                           ~ - O O O O nad       tad       tad O o O O O O O O O O O O O O O O O tad        had      tad      ned      tad     tad       tad
                                                                                                                                                         - O ned      had O

had tea O c O O O tad w .ad e o e seg g e o e e e o e e o I e o e . e e . Se T *A M M N M N M N W S et. T in M "* W M N ***

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e e o e o e e m .d .d .d .d .a .d a .J .J .d .a

                                                                                                                                                                                           .         e         e         e         .

I d .d s -d -d d d I m N O O had has O O O O O O O O O O ted nad ted had had tad O O O O O O N Q Q had had had had ned tad had had led

                                 %                                                                                                                                                                                   med       sad I                           3m O 4 e S tn til
                                 -=

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                                            +e e

en e tn e en o s=e e e en e e

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                   %g=

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                                                                                                                                                               . O .

has O nad O had tad O ned e N O O had O tas

                   *       .s.O.                           .         .         .        .         .         .       .

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                                                                                        .         .         .       .        .        e        .        .        e            e        .          .         e         e         .

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                                                                                        .      se. em.            se
                                                                                                                    .      se. >=.           ge.      em. se. am.                    >=

se en

                                                                                                                                                                                                            .      e.        m.
                                                        .d        -d        .a        .a       .4           s     -s       .d         s      -d       -s       .d           .d       -d        .d s      -d        a to in O

N O

                                      ..           e to           em
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                              >=     4            su                                                                                                                                O W      W            >=                                                                                                                                w a=                                                                                   en                                                        ame had ed    S 4.3 tad m                                                          e I

e 4

                               .e    had          e.                                                                      e O      2            to                                                                      a                                                         .d W      W                                                                                                                                              %

O  % M t$ e h O a. W 4 m 4 9 g m O en en O g a. M M g g w N tes D=

                                     ==

O m g Pm O nn in en e e m a. s=e m a. a. a=o a. === N N N e s 0 W e e e e e e e e s't e 4 4 W 4 tad I W O tad O 3 m 3 3 M t e e o e a O M WW e M 4 had had 4 E I G nd E W nam W N N N 5 =* W W e W W m *= 0 I 76

m M M M M M TABLE B-5 (Cont.) DRINKING SLATER: GROSS BETA AND CAletA ISOTOPIC ANALYSES ON HONTHLY COMPOSITES (pCi/1) STATION - DWE-5 JULY AUGUST SEPTENSEE DATE COLLECTES: 04/24-07/23 07/23-09/03 09/03-09/30 RADISCMENICAL AGALYSIS: GR-B 5.1 a 1.4 E 00 6.3 a 1.4 E 00 4.9 a 1.3 0 00 GAlutA SPECiaum ANALYSI5: SE-7 L.T. 4. E 01 L.T. 4. E 01 4. L.T. E 01 E-40 L.T. 5. E 01 L.I. 5. E 01 L.T. 1. E U2 Na-54 L.T. 3. E 00 L.T. 3. E 00 L.T. 4. E 00 C0-58 L.T. 4. E 00 3. E 00 L.T. 4. L.I. E 00 FE-59 L.T. 9. E 00 L.I. 7. E 00 L.T. 1. E 01 C0-60 L.T. 4. E 00 L.T. 3. E 00 L.I. 5. E 00 Zu-65 L.T. 7. E 80 L.I. 6. E 00 L.T. 9. E 00 2R-95/as-95 L.T. 4. E 00 L.T. 4. E 80 L.I. 5. E 00 AU-103 L.T. 6. E 00 L.T. 4. E 00 5. L.T. E 00 30-1 D6 L.T. 3. E 01 L.T. 3. E 01 L.T. 4. E 01 1-131 L.I. 3. E 01 L.T. 2. E 01 L.T. l. E 01 C5-131 L.I. 3. E 00 L.T. 3. E 00 L.I. 5. E UU C5-137 L.T. 4. E 00 L.T. 4. E 00 L.T. 4. E 00 BA-140/LA-140 L.T. 1. E 01 L.T. 9. E 00 L.T. 9. E 00 CE-141 L.T. 1. E 01 L.T. 1. E 01 1. L.T. E 01 CE-144 L.T. 3. E 01 L.T. 3. E 01 4. L.T. E 01

                     ' RA-226                                     L.T.      9. E 01                       L.T. 9.                   E DI              L.I.                 1. L 02 s

TH-228 LA 8. E 00 L.T. 8. E 00 L.I. 9. [ ou

O O O O O O 3N m tad and nad and 3 O O O O 3 3 O O O O 3 3 and med ed .nd ted ted ted% end tad ned ned w ine .no es .a aN

                                                 'n.

I g ,.. . . . . . . . . . te,e e. a e @ m e a m e e . . . . . . . . . WJe to e N w w a .= w .= m me dN

  • 3g . . . . . . . . .
                                    -.           m.             e==        e=       es.       >=            em so               .               .

a= e= e== e= em em >= >= o-

                                                                &          .&       &         ad             &          &
                                                                                                                                                         .e ed S
                                                                                                                                                                                                            .          .                            >=. >=. =. ==.

na ed O $ .l0 I en O Q O _ O O O e O O O O O O O O O O O O O e O O O O =. C o o o o O Q WN and had tad tea tad ned had e e tas I end ime had ted tad tad 6ed tad ens *=d ==. go %. na# e E m. . . . . . . . tad e e m m e -

                                                                                                                                                        -. e e n e De                                                                                                                                                                                      e                       N                                       m.          -

ON es 3% . . . . . . . . . C#3 . . . . . w gn

                                  .O           m.              >=. e=.

p=

                                                                                     .      >=.
                                                                                                           >=

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                                                                                                                                                                                                                                                                                     >=

a=

                                                                                                                                                                                                                                                                                                            ==

m e e

             >                                                                       a           e            e           a       .d        a w a                             .d          .e         a           .d                       .d                                         a           w
 ^

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                 =

ta M e .. a. M e G4 fn e C N O tad Q H 4. IwV p 8

     .q:

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                                                                                                                                                                                                                                                                                       .        N --

med naa N g Q w

                        =O g
                          = e .O.            in.
                                             ==              e N

M m of Wm . m m N m N e e m m n .= N N -. t as g c " 0%

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a= e=

                                                                                                                                                                                           *           *          *                                                                   =           *
  • U O e . a=. a=.= s=.= >=. e=. . e=.

e. a=. e-. os.

                                                                                                                                                                                                   >=. s=. e=.

e- - == a a a e e a a e a e a e a a a a a a to I to ' O { 5 l I

                                         ..            m M              ==
          ,                             -              en
         ,                             M               De 98               e ad             4 4              8 I                              S
                              >=

W ene 4 5 eg

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4#e O w nas == W Ge

                                                                                                                                                                                                              .=.

E I d tad 0 l O e ned e. e n ( ) 2 M -d u u a  % i O w e e e %m it w N O a. e e 03 j W - G mO W d W e e 9 in in e em m e-o m M w w w N N i a= O e a w e e M m m m m m N N I s e e e .mo 4 4 M 4 tad 3 O O a e e e e a e e I e e tad M E 3 3 O E W W W ad S W W e M M ( tad ins ( 2 na. N N N S m. WW W W W M >= I , 78

M M TABLE B-5 (Cont.) DRINKING WATER: GROSS BETA AND C/JelA ISOTOPIC ANALYSES ON N0lf11tLY COMPOSITES (pci/1) i STAT 10N NUMBER - DWP-7 JANUART FESRUARV GATE COLLECTE0: MARCH 12/24-01/22 01/22-02/18 02/18-03/18 RA010CNENICAL ASAlv515: GR-s 5.2 s I.I E 00 6.7 s 1.3 E 00 a.1 a 1.3 E 00 GAsutA SPECTaum AmALV5I5: SE-7 L.T. 4. E 01 L.T. 4. E 01 L.I. 3. E og E-40 L.T. 6. E 01 L.T. 5. E 01 L.I. 4. L 01 NN-54 L.T. 3. E 00 L.I. 4. E 00 L.I. 3. E 00 CO-53 L.T. 4. E 00 L.T. 4. E 00 L.T. 3. E 00 FE-59 L.I. 9. E 00 L.T. 7. E 00 L.T. 6. E 00 Co-60 L.T. 4. E 00 L.T. 4. E 00 L.I. 3. E 00 2s-65 L.I. 7. E 00 ' L.T. 8. E 00 L.T. 6. E 00

2R-95/as-95 L.I. 4. E 00 L.T. 4 E 00 L.I. 3. E 00 au-IO3 L.T. 5. E 00 L.T. 5. E 00 L.T. 3. E 00 RU-106 L.I. 3. E 01 L.T. 3. E 01 L.T. 2. E 01 1 131 L.I. 3. E 01 L.T. 1. E 01 L.I. 5. E 00 C5-134 L.I. 4. E 00 L.T. 4. E 00 L.T. 3. E 00 C5-137 L.T. 4. E 00 L.I. 4 E 00 L.T. 3. E 00 SA-140/LA-140 L.T. 1. E 01 L.T. 8. E 00 L.I. 4. E 00 CE-141 L.T. 1. E 01 L.T. 8. E 00 L.I. 6. L 00
 ,CE-144                              L.T. 3.                  E 01         L.T.       3. E 01  L.T. 2. E 01 RA-226                             L.T. 1.                 E 02          L.T.       8. E of  L.T. 7. L of TH-228                             L.T. 9.                 E 00          L.T.       1    [ 00  L.I. 6. 1 00

I I r I M N O O tad

                                                     = == O O O O O O O O O led    a O O O O O O O O O OO O ned    had     tad   had    ned    had    and
                                                                                                                    -e tad
                                                                                                                           .e led    tad O

tad O O oO O O nad a td e ned 3 3

                                                                                                                                                                                      .ad I

e gad g N e e . e e n e e o . . . e o e e e e o e 3e se 9 to M M N M W ey 9 M N M i SN M W S M 3  %

                         *1 N            *e
  • g * = e o e e e o e e e o e e e . . .

to O e= a= > >= > ein om em e= em e= t= > > e= e= e= [ O e e e o e e . . e e o e e s=. e e . . . e j I

                                                     -d     .4        d     d    .4       a             e    .4     -d                    .e d                          d      d             .d         d     a        a        .d    .

i I O == == O O O O O O O ==e O O O O O == = c O O O O O O O O e O O O O O O O O O O i m < N ted tad had had nad had had tad had led had ted had led had tad

                            %                                                                                                                                     tad      and      tad    i tdt      IA                                                                                                                                                    e 9m c              e           e      e      e      o       e     e      e      e      o      e      o      e        e       a       e       o         e       e 4e           se             M      g      M      M      @      M      e      fut    g             G      M       M        @

E en cut d N e e L

                            ~         ee
           @                %                          o      e      e      e       o     e      e      e      e      e      o      e       e        e       e       e         e       e
                                                                                                                                                                                           ?

M W N e= De > e- > to ema em aus > e= em > e= >= em t m O e o e o e e e e o e e *

  • I.=
  • e e sue e e p e d .d e -e a =4 .d a d .d .d -d -J .a .A .4 d .d e

4 4

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u M N

              $     N e

M N ee ao N d. Q m g  ! agW

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C Fe 8 O -e =e O eg

                 %e e      en O              . O O                 s o. s a a 8 a.                          . .O                  .O s .           . . O O
a. .e O p w "
                                                   * * * * * * "- - " = " = " * * * = =

m e.3 9m I a t

                        .d e        N ld          w      == O             e            e      e      o      e       . e      o             e                             e h4  m m

a ae .e M en M w e w N ,e en f=t a w w e o e e m ~ ~ e3 O g g = es 4 ee no I g o.  % e e o e e e o e e e e e e e e . . . M M M M M M M

                    >=     O                       N.            N.      N.                                                     M       M        $.D     e.D     e.=       e=      I=

M e M. N. e e o e e e e o e o e o e M a a a a a a a a a a a a a a a a a a M m 1 (4 en C 5 I p ee en

                                =*

M en em en De me 4 I E e. 4 S E tas -d 3 a= 4 m O W W em 9 tA as tad me W S

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                          =#    tad           &                                                     e                                           4.d O     3             en                                                    a                                           %

u ed %M w m o O W W D @ tA em e e40 se M M sy

                                                                                                                                                        =e er w w eN en tad   me  a             h       O In          en se e              gg     g             se N

a= ese M ese se e =e me N N S e a W e a e e e e e e m e e e a e a e 4 4 E ted 9 g O ned O E M 3 3 44 M S S @ W G m W tse U 9 4 tad tad 4 E h5 N N M W W E ** W W G W e= l l

                                                                                                                                                                         #                   i I

80

M M TARI.E B-5 (Cont.) DRINKING WATER: GROSS BETA AND CAletA ISOTOPIC ANALYSES ON MONTNLY COMPOSITES (pCi/1) STAil04 - SWP-7 JULY AUGU51 DAlt COLLECTE0: 06/24-07/23 SEPTENBER 07/23-09/03 09/03-09/30 RADISCNENICAL AsALV515: G8-8 6.4 s 1.5 E 00 3.3 s 0.8 E 00 4.2 t 1.3 E 00 GA8utA SPECTRUN AaAL YSI5: SL-7 5. L.I. E 01 L.I. 5. E 01 L.T. 4 E 01 K-40 L.I. 7. E 01 L.T. 7. E 01 l L.T. 6 E 01 Ma-54 4. L.I. E 00 L.T. 4 E 00 L.I. 4 E 00 C0-58 L.T. 5. E 80 L.I. 5. E 00 L.I. 4 E 00 FE-59 L.T. 1. E 01 L.I. 1. E 01 L.I. S. E 00 Co-60 L.T. 5. E 80 L.T. 5. E 00 L.I. 4. E 00 2N-65 L.T. 8. E 80 L.I. 8. E 00 L.I. 8. E 00 23-95/us-95 L.T. 5. E 00 L.T. 5. E 00 L.I. 4. E 00 80-103 L.I. 7. E 00 L.T. 7. E 00 L.I. 5. E 00

 ;                                        30-106                                               L.T.                 4     E 01            L.I.       4. E 01           L.I.      3. E 01 1 131                                                L.T.                 4     E 01            L.I.       3. E 01          L.T.       1. E 01 C5-134                                               L.I.                 5. E 80            L.I.       5. E 00          L.T.      4. E 00
 ;                                       C5-137                                                L.T.                 4     E 00            L.T.       4    E 00          L.I.      5. E 00 SA-140/LA-140                                         L.I.                 1. E 01           L.T.        1. E 01          L.I.      6. E 00 CE-141                                                L.T.                 1. E 01           L.I.        1. E 01          L.I.      9. E 00 CE-144                                                L.T.                4      E 01          L.T.         4. E 01                    3.

L.I. E 01

                                       - RA-226                                               L.I.                 1      E 02          L.T.         1. E 02                           E 0!

L.I. 8.

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I MN tod % M O O O taf tad

                                                                                                                                              .o med O O O O O O O O O O O O O O O O O O 3O O O O and               ted        ted       tee       ted          tea       w           tad        tee          ned       tea       tad O _

O ad a O O 3 ud .a IeN ned e 8e e T

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                                                                                  ..                    e em        em          em         em           em        s=        e=              >=         e=         a=           s=

e o e e e e s s s e e e e o e e e e b ed a.d ed I enO em0 m$ gus em0 ed 4.d ed aid ed em0 .d ed ed ed I et N in O O ted

                                                                                                                                ==

O O == nad O =* OO O e e o

                                                                                                                                                                                          == O O O O a

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O O O tad had and tea tes tad tea nas tad tad ted tad % ted ted tad es and w G ame N 2e e e e e . e e o e e e o e * * . . tad e s.e - - S sue M S N

                                                                                                                                                                                                                                                                                                                                   .                e DG                                                                                                                                          se         N           N         N             N         G         as              M          w          me         c.e g                                                         ON                       m g                                                         as                                                       .          .               .               e          e         *
  • e . * * * *
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ese

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e e O O O O O O O O O N w w tes w w w w w a a O a as s tes w w w een ine w w w t., t.d en g w te. n o. 4 e . e . a g a g Of = O M M e w m e e M

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o e e sue sie e== a= em a= a=e o= t= o= >= e= em o e o s s e e e o e e e a e e e a e a a a e a e e a e e e e e I d a I w a a l M o l I

e. e en ==
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tes I ad 4 3 se 4 es O W W >= e 4A sue had == W 9 me E ane e

                                                                              .*         ten               es e

at O 3 en e .d w w a  % O %M te e mM o me e eN e tad == m w e S O in te e e a=e sue e w w N h O 48 44 nn O 49 S se me M se ese we se N em S e 4 , e e ao N 4 4 e e e e e e se e e e e e e e 5 tee e g O ted O E E 3 3 O es ta 48 e ad a W e 44 44 4 tad ted 4 E tee W N N m a es u u e w w eg o.

                                                                                                                                                                                                                                                                                                                        .J 82

m tas M e- m o =* o O ** o o o o o O o OO O o O o == o o=*oOO Oo OO OO OO == O m I GN 4% SN

                                          @e, 3e e

nas o. N nas tad ned w tas M w N tas tad w w w tad w

                                                                                                                                                                                                                        =ad tad ud naa o
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s.

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e- .- a a a a a a a a a a a a a a a a a a a . . . I He e t.13 O A M rat n3 se 1 g tee Q m o o o o e 'o o e o o e o e o e o eo oo e oo .eo O e m o O

               ,,3       y w
                                        ===               ins o

w w w one o o m mN tas w w w tas tas w w w w w w w w M N 4% 4 H H H e z o. . . . . . e o. e ^ N N .a N se e N w n m N m n N ee m

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                             .-e o m

se.e . . . ta a o g

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um . e-

m. a.
                                                                                                         ==

m. a. s m. e. e-go w y w w g .a .s -d -d a .a a .s a a a a a

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               >        VJ I

3 M Y m 4 *e e o e o e o o m end e em -. o w o o e o e o o o o o o oO Oo o eo oo O - O O O tas had tas nas nas one taa nas nas ens 4% tas tas les had tad has one ins ee em p g me o. . . . . . .

              ,                        @e               N                           N              e     me       N        .mo                     .e w                                                                                        s.e                     .mo       en            en ..              ao        N          M         es        mm
                                       >= N en %                .            e               e          .       .         .        .          .            .         e        .             .        .          e          e EN               D.            D.           em                                      p.        m.
                                       ====                                                      se. e.           go.                                        -                       p.                                      De        en        e.        p.

ns. .a

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                                                     ..          3
                                            ..      M.

4 A vs 3 ins a= 3

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S == tas u e e

                                           .e       4           tad a.

e et o s 3 M e -d u 3 S  % e oene en o en  % m t$ e h a me w e e e een m o ==e me 4 se m w w w ene e.= N o en m me .M me me == N N N s= =. M w =e N 4 as e 4 e nas a e e g a nas e a og 3 3 e e e e e s == s e e e o e e e e= 3 e e e en M 4 ene w .C . E ad a u tem u N N su as a. u u e u u es* s= 83

a nas M =* == 0 O

                                >= m                   O               O O O O O O 3O O O O OO OO O.-.                                                                                        O                   O c s a .= c I                             WN 4%

23 N.s 3g e tad N O. ned se se ned led me ned ame tad fue ted me tad N had me tad O O had las n.s o e o o o o tad ned tad d i.a w em .st ame @ N m as @ N id's N N I g; OS

                                                      .4 e

a= auf ad ad and ed ed

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                                                                                                                                                             -d
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                                                                                                                                                                                                                -d ad ed ed ed d

I as tad O

                               *= m W%

4 56 30 CF e m O tad O.

                                                                      ==

tad

                                                                                =e had O O O O O O O O O O tbO OO OO ==*

ted tad ted led tad ned had O O ** O O had O O O OO ted taf had tad O = = c ted O had O ted O tad w

  • I N N T N N w me 8"a N N == N N QN N a9 w = m m 5%

am @ . . . . . . . . . . . . . . . . 3 e= em m. e. >= e=

e. O . e=. . em. e=. ==. >=. e. >=. e=.

e= s= M (/) and auf ed 8 ad

                                                                                                                                          .                    .          .                                                    .       e=.            .        .=.            .

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             !a l _.

ed c H M M H MN 4%

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                                                                                                    >=. e=.                 em       em.                             em                e-         >=                                             >. ==

M 4 E M E taf O ef ed

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D't k C 0. tA and af ad em$ ed ed ed ed ad one ad ad ad ad ed ed ad M z w o 8 O 4 M H m M M Q ~ Q M W g *

             >*  N       em m                                      O                                O as                    O               O O O                                                   O                                                                                O                        O _ _ C ins e                                                                                                                                  O O                                     O                        O          O           O            O e= O                  taf             tad        nad        led       had          tad        tee      tad 5%                                                                                                                tad        tad       tad                nad       had        ted        ted           had        tme         tad M                                                                                                                                                                                                                                                           had I

4m I"8 30 O. . . . 8"8 . . . . . . . 4F e N N 4A N N afe N w M e 8"o N N N N e tre e-o m e't  ! e* N i tA % . . . . . . . . . . . e . . . . D* W= e= De E N. mo m . e en.* >=. e De. em. em. ee. >=. em. pm en em p=

                             -                     ed              ed         d em0       ed           and        ed
                                                                                                                                       .                                                            .      e=. em.                     .           .           .        >=.

em0 end and d ad ad and ed ed ed and ed i r I ..

                                                              ==

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                                                                                                                                                                                                                      -d W           3                                                                                                 %M em.                                          W                                                                                                      e          N          O             an         e e eB W S S en                                    tA         G                                      M          M          W I

ima >= N O en tA sus W W N N em .= M e w e e we e e S se s=e M se as se ** == N N ' e e e e e e se 4 as e e e 4 EuO wta.e eu as e e e # a and e a ada e w a < .e e- a sa e as 4

                                                                                                                                                                                                                                                                       -z in.

me as a -. u u a u u as i i t i I i 84

5 as M -. -. O O

                                                              -m                                                                                           O .= 3 O O O ~ O O                                                                                  O I

O O O O O O 3 EE N O O O O O O O O O O e O O O O O tas had ned tad tad 4 3 .% ted ted nad tes les tes tad w tad w tad w a w

                                                              @..                                   O.

e . . . . . . . 3O N .= me N N e- m N O ~ e m a N N I $h OO s,,

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                                                                        .                        ~                               a                      M            . ~                         ==          .e                                                         N o N

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                                                                                                     .              .        .       .      s=.            .         .          . a=.            .      e=.            .                . *=.             .             .      ==. .=.

e=

                                                                                                                 .4          #   .d         -s          .d       .a         .4           d       .a          .o        .a               .d       .d         .a           .4         .4         w          w m

I O H M E. N En3 N 1 e.e 5 u a Q

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o m . 1 m m ~ - O ta. t= . O tad O O ned tee nas 888O 388O tad O O O O O O O O ~ ~ O O O O O O s tas ese tee nas tas nas nas nas tes ned gas nas 4.s =ne i

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                                                                        .                 m.

3

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8. .. ~- .O ~ ~

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M M M M M M M TABLE B-7

                                   .        SURFACE WATER:

CAlttA ISOTOPIC ANALYSIS i ON MON 11tLY COMPOSITES (pci/1) STAil0N NUNSER - 5U6-2 JANUARY FE8NuARY SATE COLLECTES: MARCH 12/24-01/22 01/22-02/18 02/18-03/18 GANNA SPECTRUM AuALv585: t SE-7 L.I. 4 E 01 L.T. 3. E ul L.T. 3. E O! E-40 9.171 2. 78E 01 L.T. 4. E 01 L.T. 5. E 01 me-54 L.I. 3. E 00 L.T. 3. E 00 L.I. 3. E 00 Co-5e L.I. 4. E 00 m 6.1. 3. E 00 L.I. J. E 00 os TE-59 L.I. 9. E 00 L.'. 6. E 00 L.T. 6. E 0u CO-60 L.1, 3. E 03 L.T. 3. E 00 L.T. 3. E 00 2m-65 L.T. 7. E 00 L.T. 7. E 00 L.I. 6. E 00 28-95/NS-95 L.T. 4. E 00 L.T. 3. L 00 L.T. 3. E 00 i EU-103 L.I. 5. E 00 L.T. 4. E 00 L.I. 3. L ou -j 30-106 L.T. 3. E 01 L.T. 3. E 01 L.T. 3. L ul j I-131 L.I. 3. E 01 L.T. 9. E 00 i L.I. 5. E 00 i C5-13a L.I. 4. E CO L.T. 3. E 00 L.T. 3. L 00 C5-137 L.I. 3. E 00 L.I. 3. E 00 L.I. 3. E 00 l SA-140/L A-140 L.I. 1. E 01 L.T. 6. E 00 L.I. 4 E 00 CE-141 L.T. 9. E 04 L.I. 6. E 00 L.T. 5. E 00 CE-144 L.I. 3. E 01 L.I. 2. E 01 L.I. 2. E ut RA-226 1. L.1. E 01 L.I. 1 L ul 1. L.I. E un TH-228 7. E 00 L.T. L.T. 6. t 00 L.I. 6. L 0u

M M M M M M M M M TABLE B-7 (Cont.) SURFACE WATER: CAttlA ISOTOPIC ANALYSIS ON HONTHLY COMPOSITES (pci/1) STATION huMSEB - SWG-2 APRIL MAT DATE COLLECTES: 03/18 04/15 JohE 04/15-05/27 05/27-06/24 EA8eIA SPECTRUM ANAL VSIS: i SE-7 L.T. 4. E 01 L.I. 3. E O! L.T. J. E O! K-40 5. E 01 L.T. L.T. 5. E 01 L.T. 4. E O! Ne-54 L.T. 3. E 00 co L.T. 3. [ 00 L.T. 3. L 00 CO-54 3. E 00 L.I. L.T. 3. E 00 L.I. 3. L 00 FE-59 L.T. 7. E 00 L.I. 6. E 00 L.T. 7. E 00 CO-60 4. E 60 L.T. L.T. 3. E 00 L.T. 3. E 00 2n-65 8. E 60 L.I. L.T. 6. E 00 L.T. 6. E 00 2R-95/tt-95 L.I. 4. E 00 L.T. 3. E 00 L.I. 4. L 00 ku-103 L.I. 5. E 00 L.I. 4. E 00 L.T. 4. E 00 au-IS6 L.I. 3. E 01 L.T. 3. E 01 L.T. 3. L 01 1-131 1. E 01 L.I. L.T. 9. E 00 L.T. 2. E O! C5-134 L.I. 4. E 00 L.I. 3. E 00 L.T. 3. E 00 C5-137 L.I. 4. E 00 L.T. 3. E 00 L.I. 3. L 00 S A-140/L A-140 7. E 00 i L.I. L.T. 6. [ 00 L.T. 3. L 00 CE-141 L.T. E 00

8. L.T. 7. E 40 L.T. s. t 00 CE-144 L.T. 3. E 01 L.T. 3. [ 01 L.T. 3. L 01
  • RA-226 L.I. 9. E 01 L.T. B. t 01 L.T. a. t 01

{ TH.228 L.T. 8. [ 00 L.I. 7. [ 00 L.I. D. L 00

                                                              ==

O* oO oO oO o3 o O e O 3 o == o o3 o3 oO oO o 3 o o o3 e O I es m tad **8 tad ta8 tad *me had W nne w and % nad tea had nad w tas w w GS go . . . . . . . . . . . we M tal M M @ M @ M w N 2 eu m M M @ W M se N G. O I ud % . . . . . . . . . . . . . . . . 44 St >* De >= >= >= tm. 0- 3- pm pus. g-o . . . . . . . . . >=. . km em >= B=. em .-

                                                             .a        .a        .d        .a          .a        .a        .a                    .a                      a w
                                                                                                                                      .d                   .4                               4       .a          .a         .4            d             a I

I O O O O O O O O O O O O . . . . . m O o O Q Q o tad ted tad had tad tee tad nad em.%O had tad had nad ted had ned had .m# e.s tM O 3o . . . . . . . . . . . . . . M . . 69 e til M M N M N w w M N M M A 3M St N I ft. N (N N . . . em se em to se g= se c >=. . . to. to. . . . . gm to. em tem e-

                                                                                                                                                                                                                 .        >=.

pm. em, a .4 .d .d .4 -d .d .d .a e .d -d s .a e .4 .4 .d I ^ e M pe M b g b N N e 4.8 .e f/) e I M C 3 _q as ws b) b A

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u. *g , . . .o . .o o.=o =oo I a U N G
                      -                       ~            W        t         t         .          t.,        t.,       t.,        te.        te,       40
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w at

                      ==

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em em. om a.a .d .d .d and

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I O

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e 4 O to se .d be E  % at e g %M t@ W h 9 ** W @ W Se g gn tag g g on M M g g w N tes E  % O est in to to te St .mo ==. M s=. as == me N a= 2 e 9 e o e e e e e e aus

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e  := - .. . I e . . W th 1* .. . . a w a o . . . . . . . . .

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                                             .h.e t=

W

                                                       .S
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s W . I

                                             .d          d 9
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  • m q W . W pa. .% W W .
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i

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                                                                                                                                                                                                           =. .=. .=. N e

e e. .e .e a. .e .e .e o e m.e e e e e N.

                                             .         W    . ad E W                                      .a.        W          N        N                               . W W e              e. .e              =

W W . s= O I 89

                    - - - - - - -    -        -                                  -.-. -                              ,-                                                              -.-                    e     .- -

g M M M M M M M M M M M TABLE B-7 (Cont.) SURFACE WATER: CAle(A ISOTOPIC ANALYSIS 018 HDIITHLY COMPOSITES (pci/1) STAil04 NUNSER - SWE-5 Janvany DATE COLLECTES: easuumaT 12/24-01/07 01/22-02/18 nasLn 4 02/18-03/04 GANNA SPECTRUM AaALV585: I' BE-7 L.T. 5. E 01 L.I. 3. E 01 L.T. 4 E 01 E-40 L.I. 6. E 01 L.T. 4. E 01 Na-54 L.I. h. L of L.T. 3. E 00 L.I. 3. E 00 CO-58 L.I. 3. E 00 L.T. 4 E 00 L.I. 3. E 00

   $                    FE-59                                                                              L.I. 3. L 00 L.I. 1. E 01      L.I. 6. E 00 CO-60                                                                               L.I. 7. E 00 l                                                           L.T. 4     E 80      L.T. 3. E 00 25-65                                                                               L.I. 3. L 00 l                                                          L.I.     /. E 00         L.T. 6. E 00 28-95/58-95                                                                         L.T. 6. L 00 L.T. 5. E 00     L.T. 3. E 00 AU-143 L.T. 3. E og 1.1. 7     E 80     L.T. 4     E 00 Au-306 L.T. 5. L 00 L.I. 3. E 01     L.I. 3     E 01 I-131                                                                              L.T. 3 .- L 01 L.T. 1. E 02      L.T. 9     E 00 C5-134 L.I. 2. L 01 L.T. 4     E 00      L.I. 3    E 00 C5-137                                                                              L.I. 3. L 00 L.T. 4     E 00      L.T. 3    E 00 SA-140/LA-140 L.I. 4. E 00 L.I. 2. E 01     L.T. 6     E 00 CE-141 L.T. 9. E og L.T. 1. E 01     L.T. 7     E 00 CE-144                                                                             L.I. 9. E ou L.I. 3. E 01     L.T. 3 RA-226 t 01      L.T. 3. E of L.T. 9. E 01     L.I. 7     E of
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                                             -         m        o                   = = . . .

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m M M M TABLE B-7 (Cont.) l s SURFACE niATER: CAIG(A ISOTOPIC ANALYSIS 001 M00f7HLT COMPOSITES (pC1/1) STATION NunSta - SbP-7

l APRIL MAV JUNE BATE COLLECTE8
03/18-04/15 04/15-05/27 05/27-06/24 y

GAMMA SPEClauN ANALV515: BE-7 L.I. 3. E 01 L.T. 3. E 01 L.T. 4. L ut K-40 L.I. 5. E 01 L.I. 4. E 01 L.T. 5. E of NN-54 L.T. 3. E 00 L.I. 3. E 00 L.T. 3. E 00

C0-50 L.I. 4. E 00 e L.I. 3. E 00 L.T. 3. E 00 FE-59 L.T. G. E DO L.T. 6. E 00 L.T. 7. L 00 CO.60 -

L.T. E' 00

4. L.I. 3. E 00 L.I. 3. E 00 Z3-65 7. E 04 L.I. L.T. 6. E OD  ; L.T. 4. E 00 ZR-95/Na-95 L.T. 4 E 00 3.

L.I. E 00: L.I. 4. L 00 30-103 L.I. 5 .' E 00 L.T. 4. E 00 , L.T. 4. L 00 A8-106 L.T. 3. E 01 L.T. 3. E ' 01 L.I. 3. E 01 1-131 'L.I. '$. E 04 L.I. 8. E 00 L.I. 2. L 01 C5-134 L.I. 4. E 00 3. E 00 i L.T. L.T. 3. L 00 C5-137 L . I . ' 4. E 00 L.T. 3. E GO L.T. 3. E 00 BA-140/LA-140 L.I. 7. E 00 L.I. 6. E 00 L.I. a. E og CE-141 L.T. 7. E 00 L.I. 6. E 00 L.T. 9. E 00 ! CE-144 L.I. 3. E 01 L.T. 2. E 01 L.I. 3. L og RA-226 L.I. 7 E 01 L.I. 6. t 01 L.I. 8. L 01

IH-228 ~. L.I. E 00 7 L.T. 6. E up L.I. 7 L ou

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                                                                   - - O . . O . . O O O O O O O O O O O O. .O. OO O OO - O tad         ted         .ad               had         tad         tad           ned         tad         led       tad        tad         had         had        tad         nad         nad O O had O

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pm om e= >= em - I A & & & & & & &

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                                           ==

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til se a= == M e W e e se 889 se .e se .e .o N N e s e o e .e 4 5 0 4 tad W G e e e e e ei= 3 e e mg 3 u e tad O E E 3 3 e 44 44 4 e e 4 e e te. *J pd ed Lad nad 3 a 5 ** W tad a W W W o= l 8 l 1 I i g .

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                                                       ==   ==.h.

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                                                                               .                        .                   .                                        .          .       a=. a=. a=. a=. e=. a=. a=. >=. o=.                                                              :

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                                                          >=         O    M         $     e        e 1A e

4A tot @ @ m =e =e m a.9e =e =e =e N 4 4 as e e o e e e e == e e e e e e N. S e et R e g O tes O E NE 3N 3 e t#9 t#9 4 tas tad E et X ta ad a W te. W W 5 *= W W G W W EC at > t 101 l

l t l l I o l I s l N w a=e == aus me me me aus N N ==e me N O O O se N est #=e O O O O O O O O O O O O I 5e OO e- % e nas % 3g w w O tad e ese. ge ted tad T tea and and S had 4A tes to had e ** to tes tad ned e == W ned e and o O O O t.d M C e di a w a r= o WO se O.e I O ne ed a=. e. me me em. ed en ad em ed e e e=.

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                             ==

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4 9 se e . a=. . >=. a=. . . . . . e-

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T W a=e 4 S O tA 4A O O me M w w  ! I N O N N tas tA tA 4A f's T t$ 49 9 ** se M me suo se me 0- e W e e e e e e e e se e.

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e end ( 3 l I > i l l 102

M M TABLE B-10 (Cont.) SHORELINE SOIL: CAben ISOTOPIC ANALYSES (pts /kg Day) STATI0s muMBER - SNWJ-1 OCTOSER SATE EOLLECTES: 10/04 GANNA SPECTRUN ANALV515: SE-F 1.74 30.33E 03 E-40 4 1.88 so.19E 04 g Ne-54 L.I. 4. E 01 w C0-58 L.I. 5. E 01 FE-59 L.I. 1. E 02 C0-60 4. L.I. E 01 25-65 L.I. 1. d 02 22-95/as-95 L.T. 5. E 01 au-303 L.I. 5. E 01 1 AU-106 L.I. 4 E 02 1-131 L.I. 2. E 02 C5-134 5. L.I. E 01 C5-137 9.93 23.o1E 01 SA-140/LA-140 L.T. 8. E 01

                                                                                                                                                                                                                                                                        ~

J CE-14! L.I. 7. E 01

                                                                      .,                         CE-144                                                                                   L.f.                   2.            E 02 RA-226                                                                                   3.44 20.63E 03
IH-228 1.26 so.13E 03

\ i

m M TABLE B-11 HIIX: IODINE-131 AND CAletA ISOTOPIC ANALYSES (pC1/1) stall 0N NUMBER MKQ-5 JANUART JANUART DATE COLLECTE0: 01/88 FESRUART 01/23 02/05 RADISCNENICAL AEAL V5I5: 1-131 L.T. 2. E-01 L.I. 4. E-01 L.I. 2. E-01 GANNA SPECTRUN ANALTSI5: SE-7 L.T. 4. E 01 L.T. 3 E 01 L.T. 3. E 01 K-40 1.35 to.14E 03 1.18 10.12E 03 1.06 20.!!E 03 5 Ma-54 L.I. 3. E 00 s~ L.I. 3. E 00 L.I. 4 E 00 CO-58 4. L.T. E 00 L.I. 3. E 00 L.T. 4 E 00 FE.59 L.T. 9. E 00 L.I. 7. E 00 L.I. O. E 00 CO-60 L.I. 4. E 00 L.I. 4 E 04 L.T. 4. E 00 Zu-65 L.T. 1. E 01 '.I. L 8. E 00 L.I. 9. E 00 ZA-95/as-95 L.I. 4. E 00 L.T. 3. t 00 L.I. 4. E 00 RU-103 L.T. 4. E 00 L.T. 4 E 00 L.I. 4. E 00 20-106 L.I. 3. E 01 , L.I. 3. E 01 L.I. 3. E 01 1 331 L.T. 7. E 00 L.T. 4 E 00 L.T. 5. E 00 C5-134 L.T. 4 E 00 L.I. 4. E 00 L.T. 4 E 00 CS-137 L.T. 4 E 00 L.T. 4. E 00 L.I. 4 E 00 SA-140/LA-140 L.T. 5. E 00 L.T. 4. E 00 L.T. t CE-141 4 E 00 L.T. 7. E 00 L.T. 5. E 00 L.T. 7. E 00 j . CE-144 L.T. 3. L 01 L.T. 2. E 01 3. L.I. L 01 i RA-226 L.T. 8 [ 01 L.I. 7. L 01 L.I. 1. L 02 TH-228 L.I. 8 E 00 L.I. 7. t 00 i L.I. v. t 00 l

TABLE B-11 (Cont.)

                                                                                       ..                                          MIIK:

IODINE-131 AND cat 04A ISOTOPIC ANALYSES (pC1/1) stall 0N NUN 8ER NEQ-5 FE8EUARf NARCH DATE COLLECTES: 02/19(a) MARCH 03/05 03/19 RABIOCNENICAL ASALTSIS: 1-131 L.T. 3. E-01 L.T. 2. E-01 L '. I . 2. E-01 GA8MtA SPECTRUN ANAL V515: SE-7 L.I. 4 E 01 L.T. 4. E of L.T. 4. E 01 E-40 1.24 20.12E 03 1.33 20.13E 03 1.18 10.12E 03 NN-54 L.T. g 4 E 00 L.I. 4. E 00 o u L.T. 4. E 00 C0-58 L.T. 4. E 00 L.T. 4. E 00 L.I. 4. E 00 TE-59 L.T. 1. E 01 L.T. 9. E 00 L.I. 7. t 00 C0-60 L.T. 5. E 00 L.T. 4. E 00 L.I. 4. g 00 ZN-65 L.T. 9. E 00 ..L.T. 9. E 00 L.I. 9. t 00 2R-95/NS-95 L.T. 4. E 00 L.I. 4. E 00 L.T. 4. E 00 au-103 L.T. 5. E 00 L.I. 5. E 00 L.I. 5. E 00 AU-106 L.T. 3. E 01 L.T. 4. E 01 L.I. 4. E 01 1-131 L.I. 4. E 00 L.I. S. E 00 L.I. 4. E 00 C5-134 L.I. 4. E 00 L.I. 4. E 00 L.T. 4. g 00 C5-137 L.T. 4. E 00 L.I. 4 E 00 L .,I . 5. E 00 SA-140/LA-140 L.T. 6. E 00 L.T. 5 E 00 4. L.T. E 00 CE-141 L.I. 9. E 00 L.T. I. E 01 L.T. 9. L 00 CE-144 L.I. 3. [ 01 L.T. 4 E DI L.T. 4. E 01 RA-226 1. L.I. E 02 L.T. 1. E 02 L.I. 1. E U2 TH-228 9. E 00 L.I. L.T. 9 E 00 L.I. 9, i og ( a) Shipped late; 5 days old.

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e. U e w g I

   **%      b                                                                                                                                                                                                                       '

W e = I v M g o O M set M W E z a S O O e tad m. O tad M tad M O O O O O O O O O O ned tad tad tad e.e tad o O O O O O O O O O O O O tad had nad tad e O O O ned ted tad tad w

                                                                                                                                                                                                                 ~ O med nad
                      ==       ==           .              . se.        .

I U . . . . . . . E NN N . . . . . . . E e s T O T T O T We T 4A T .Ee T t@ @ an Q .= @ M e.c. nn se 44 0 . . N

   *3                                    a=
                                                                            .        .         .       .       .        e        .        .         .         .         .          .          .         .              . .

i en en a=

                                           .             e.      N.       e=. e=. e=.                  .       . e=. e=. e=.                    .

es. e e= em

p. n=
                                                                                                                                                                                                                             ==

M M M M M M M ed M N M M M M M M ed M I

                                                                                                                                                                                                     .ul         .m0          .'O M

M i i M E w I 8 w i I.. tA

                                    <=

en LA me sn I

                                     .d             4 4               3 S               4
                               .. as S                     E tad   .e              D                                                                                                                         o e=    4               m W      W               e=                                                                                                                        w 4A                                                        ==

tas = u S

                              .4    5               w                                                                 e                                                       4 e

a en e e. m O 3 4A 3 a W u %M

                                                                                                                                                                              'a%                                                 !

O .* 4 W te W N O me e @ W M N G S O GA 4A O O as M M 9 W w N N tad == O 4A 4A 4A @ W m m. m. M ene ame me am. == N N a= 0 ** e 9 e e e e o e me

                             =      <               =   w                                                                      e        e                   9         9         e           s         e           o            e  i O      m e
                                        - w             e as e

EOu ind te. O a a a m u N ~ m = - u u a u u = - 9 a w = w ind < z  ; Y L I '

E E 1 0 1 0 0 3 0 0 0 0 1 0 0 1 0 0 0 0 0 3 1 0 E

                                           -                              0 0 6 0 0 0 0 0 0                                                                      0 0 0                          0          0         0 0 E        E          E       E        E        E         E        E         E 2                                                                            E         E         E          E          E        E          t         E         E T6                                  1 S0 M                        U/

68 3 4 0 1 4 4 S 4 1 4 4 4 7 4 4 5 8 3 9 8 U0 A .

                                                        . 2                 .       .        .        .          .       .          .         .

I. . L I. 2 I. I. T. I. T. T. T. I

                                                                                                                                              .      T.        T.        T.         T.        T.

T. T. T. L 1 L L L L M L L L L L L L L L L L L M 1 0 1 0 0 3 0 0 4 0 0 0 0 0 0 0 0 0 0 0 000 00 1 0 0 1 0 0 0 1 0 0 0 2 0 E E E E E E E E E E E 5 E E E E E E E [ 6 1 TI . . . . . . . . . . . . S L/ U7 2 3 os 4 4 9 5 1 4 4 4 7 4 4 6 8 3 1 8 E J0 S . . 0 . . . . . . . . . . . . . Y L T. L T. L 5 1 I. L T. L T. T. T. T. T. T. T. T. T. T. T. T. T. T. A L L L L L L L L L L L L L L N M A

   )         C I      5 P        -

t n D 1 Q K o 0 N C S ) (  : I 1 R E l K I A

                 /

i B M 1 I I t e cp U 0 1 3 0 0 0 4 0 0 0 1 0 4 0 0 0 M B

    -   M M    (

N E E 0 E0 0 E 0 E 0 0 0 0 0 0 8 E 0 0 0 0 C 0 00 1 1 E E E E E E C t o 3 E E E E E E E E 1 L D t 2 . . . . . . . . . B N i A Y0 3 4 0 4 4 9 4 9 4 5 4 7 4 4 A A T L/ U7 a 4 7 3 8 8 T S J0 . . 6 . . . 1 . . . . . . . . . . . . 2 . 3 T. T. T. 1 L L 1 L T. L T. L T. L T. L T. L T. L T. L T. L T. L I. L I. L T. I. T. I

             -                                                                                                                                                                              L         L         L         L E

N I D O I

5 5 1 I 5 S v Y l L A A N a S E
A L

E A N U T A R 0 C C T 4 E I C 5 1 9 g L L O N E N E P S 8 5

                                                                                                                    -                                                           A L

C C / 3

                                                                                                                                                                                /

O 1 A 4 6 4 7 0 1 4 6 8 E I 3 N 7 0 5 0 95 0 5 5 0 0 5 1 3 3 4 4 4 2 2 T S N - - 6 6 9 1 1 3 1 1 1 1 1 2 2 1 4 - - - - - - - 1 - - - - - A A - A E - I - - g S A I G B E N OC I E F S 5 8 C 7 2 U 0 A 3 I

                                                                                                                                                   -       5 C C 5          A S

E C E C A R H T _ g g "o.

a'* M M O O = O -e 3 O -. C =e Q O O e O O O O O O O O O O O O O O o O

                                                                                                                                                                                                                                          --          N o o              l tad              tad      had        W          tad        had         tad       ted         med       had        tad        tad i

W had tad tad and .ad and ' I

                                                                                                                                                                                                                                                                .d sad m                                      N.ne                                                                                                                                                                                           I e .e            O.                  .        .          .         .           .          .          .          .          .          .

g% ** 4A O 4A 4A tad S e @ me en h en me @ @ h e. T m == 98 8", e O .

                                                                   . N                .          .          .           .          .          .         .          .          .          .

t= . . t.d n= e.= > s= s= wt . N. e. s=. a=. a= > om d & M &

                                                                                      .                     .          .                                .      a=. >=. .=.                           .       e=.             .             .        ==.

4 d 4 4 4 4 4 4 4 & d d d e a l l l l I l l

                                             ==               == m O O                                 =e O                O O                                                  O == O O == O O O                                                                        O           -e            .=          N M

e O O O O O O O O O O O O O O O o had had led tee ted and had had tad had tad tad tad had ned tad i N had and ime e ST me 30 I tad % N 4A O 4A nn me @ me en 8= 9 es @ 4A N @ @ @ m. T m. e

e. O tad i
                                               .                .      N            .          .          .

W D'. $= f#$. p . 3

                                                                .      N.                   De.

O'- De 8= $= 0 t= > to g= t= 0. > d .d == a

                                                                                                          .          .          .          .          .          .          .         .        en.            .           .

I I d d . .

                                                                                                                  .d         &           .d           d       -d            d         d        .d          &           &             .d          .d          _.

Q 4A I a 4 l

     .       Se        #'                                                                                                                                                                                                                                               '

I U k a a es G

   %u#

n led

         ..       s.4 S 5        3 E I
                                           .e g-g                      O                O O O mO 38O O                            -e O O - O O O O                                                                  O - -                                 O a=             .
                      -   >O
41. 4.d g 4.d 48 n., led O O O O O O O O n.d ted L.d 48 led 4.d 48 tad O

e.d O e O d O 94 *= to ce . . . . . . I 4 3% P'l T O W W I a= @g G T me W W W N w to nO og T 4A N m e e ' i 4 . . @ . . . . l g . . . . d M

m. > > > > > > > > > > > > = = =, =.
                                                                                 .          .           .          .         .           .          .         .          .          e

( d d & & & & 4 & & I d d e e a w as 5 8 N i I . I 8 to

                                     .e en 3"
                                     .4 en
                                                     ==

en. 3

                                                     .d 4

i I S 4 S E tad

                                    .a 4

a O S 4 4.d W to IA T I led .* W me d E tes S e i e e ned e. e 4 O 2 to d SJ W S  % O  % M e O W 1 m W O S O 4A tA O mm ri. a. @ e ' ted == mO tA e tA @ @ S se aus 9 W T N N i 9= O 8e 0 W .e #=e se .* .= == N N D 9 0 0 0 4 4 4 0 0 e me 9 I 8 tad 9 9 0 O 5 = @ 8 5 O tad O E E 3 3 0 4A to 4 led t 4 t 2 t

  • G ad E W te. W N N eB eB == W W G W had LJ ct p.

8

                                                                                                                                                                                                                                 ',                                  i 4

I '

m =e =* M O O O OO O O O O OO OO OO OO O =oO O O O O O .= =* 3 ud e O O O O O O 3 tes w I nas tes les tad m M tes tes nas nas tes tad tes w =s a n.d =* ted@ s'* to

 '                                 %             09              M                                                                       .         .                   .

tas sm. O*e w w e 9 m w w w tes v w w a a . . . . .

                              ===                                                                                                                                                                                            M 00 O 0                     .               . g                 .        .          .        .

I 3 e= . . . . . . . . . . . .

                                                   .            e=. N.              e=. em. e=. e=. e.                                a=        p.        em        e.                   s.          e=                               == -
                                                -e              -s       .*         -a        -d        -s        &
                                                                                                                                         .        .          .         .      en.            .          .        >=.           . . .
                                                                                                                            .d        ad        .s        .a        .a        =a         -a          -s          .d            s      -d        a I                                              -.

0 e tes

                                                              =.

O O OO O tes M tad tad O .=* ted O O OO =* tne ins O OO OO == O O 0 OO O O O

                                                                                                                                                                                                               =. =. N ==

O O O O M and tad tas nas nas tes ned ted tad =* I had in. as M.s est t . . . . . . . . . O am. M . . . . O% en O @ en =* 4 =* @ @ tA P.

                                                                        *e                                                                                                  to         @          @           ==e         tre =* **
                          *= O 14          ue                     .               . w                .         .

aut O . . . . . . . . . .

                                              >=.             e=. M.
                                                                                                                                                                                                                  .         . . .                 )
                                                                                 ==. >=. ese. e=. >=. o=.                                    em                            e=

I C4 s=. e=. em e= e. .=

              >*                              -d              .a       ==        -s        -s        -d        .d        -d        .a
                                                                                                                                                .                             .        n=. e=.                    .         . . .
                                                                                                                                             -d        =s        .d        -d          .4         .d          .s          .d        -s      -d    )

1 I e u C t3

             . .e m

E er 1

                  ^  U I   %s' M

g 1 E hd J.e p M M w W S 3 E E O a O e tad

                                                            ==

las M O O O O O O O e tes w O O O O O tad nas ned tad nas O OO == had las O OOO OO O and tas tes O O nas sad O =* =* O O med O O O ted tad had

                     ==

a= tad =e 3g

                                               .               e        e.        .         .         .         .         e M                 <   0%

N q g g g g gg g g g g pg g eJ >= *= g g g m g g

                     @   u .O=                .               . en                .

O W= t= t= e= t=

                                              .               .       M.                                     em       >=         t.                  p.        su.       em A               &        Y          &
                                                                                            .         .         .        .          .      >=.          .         .         .       e=. e=. e.                         >= ==
                                                                                                                                                                                                                           . .             >=.

M & & & & & e.d ed & O & M 1 E 8 I ~ I y @ em 44 m m 44 3

                                      >               -s I                            S tad
                            *=       4 ad 48 S

eg

                                      .a 5
                                                      #T
                                                      .4 4

5 O O W w I tad (mJ.

                                     =

U nn == s 3 tas O e w tes & e 4 O 2 to e .d w w E  % O =*  % M @ w s=. tas m. M w e & O 4A ede O O == O == w @ cD P. O 4A 4A tA 94 @ M e w =ew N N I s= g =e a w $ =e ese M =e M.

                                                                                                                                                                                  ==                                                       N 4                                                   e         e         e         e        e          e         e                  =e s-.                    =. N 44     e        4                                                                                                e O        E     .= W tas        e        WO                 led        O E E                         3 3 a

14 e 44 e e e o e G ad E W ta. W N N M S e

                                                                                                                                                              == W W 4

G tad nad 4 O W WE * e I 110

M M M TABLE B-11 (Cont.) s MILK: 10 DINE-131 AND CAlefA ISOTOPIC ANALYSES (pCi/1) STATION auMSER MKQ-5 i NOVENGER DECENGER DATE COLLECTES: 11/19 DECEM8ER 12/03 12/16 SADIOCNENICAL AEALV515: 1-131 L.T. 2. E-01 L.T. 3. E-01 L.T. 2. E-01 GANNA SPECIAoM ANALYSIS: SE-F 4. E 01 L.T. L.T. 3. E 01 L.I. 3. E 01 K-40 1.25 10.13E 03 1.21 so.12E 03 1.21 so.12E 03 na-54 L.I. 4. E 00 L.I. 4 E 00 L.T. 4. E 00 p CO-53 L.T. 4. E 00 4. E 00 w L.I. L.T. 4. E 00 FE-59 L.T. 9. E 00 L.I. 9. E 00 L.T. a. E 00 CO-60 L . I'. 4. E 00 L.T. 5. E 00 L.f. 4. E 00 2m-65 L.T. 4. E 04 L .'i . 1. E 01 L.T. 1. E O! 23-95/98-95 L.T. 4. E 00 L.T. 4. E 00 L.I. 4. E 00 89-103 L.T. 5. E So L.T. 4. E 00 L.T. 4. E 00 88-106 L.I. 3. E 01 L.T. 3. E 01 L.I. 3. E 01 I-131 L.I. 8. E 00 L.I. 5. E 00 L.T. 6. E ou C5-134 L.T. 4. E 00 L.T. 4. E 00 L.T. 4. E 00 C5-137 L.T. 4. E 00 4. L.T. E 00 L.T. 4. E 00 SA-140/LA-140 L.I. 6. E 00 L.I. 4 E 00 L.I. 5. E 00 i CE-141 L.I. 1. E 01 L.I. 7. E 00 L.T. 7. E 00

                          .LE-144                                L.I.            4. E 01           L.T.      3. E 01        L.T. 3. E 01 RA-226                               L.I.            1. E 02           L.I.      1. E o?        L.I. 1. t 02 TH-228                               L.I.            9. E 00           L.I.      9. E 00        L.I. 9. I ou

M M TABLE B-11 (Cont.) ' MILK: IODINE-131 AND CADGE ISOTOPIC ANALYSES (pC1/1) STATION NUNSER NKE-4 (a) NASCN (b) NAACH DATE COLLECTES: 03/04 03/19 8ABIOCNENICAL AaALV515: I-131 2. k-01 L.I. L.T. 3. E-01 GAIW8A SPECTRUM ANALV5IS: SE-7 4. E 01 L.I. L.1. 4. E 01 K-40 1.27 so.13E 03 1.35 to.let 03 NN-54 L.T. 4. E 00 L.I. 4. E 00 CO-58 L.T. 4 E 00 L.I. 4. E 00 FE-59 L.T. 9. E 00 L.I. 9. E 00 C0 60 L.T. 4. E 00 L.T. 4 E 00 ZN-65 L.I. 9 E 00 L.T. 9. E 00 2R-95/NS-95 L.T. 4. E 00 L.T. 4. E 00 RU-103 L.T. 4. E 00 L.T. 4. E 00 RU-106 L.I. 4. E 01 L.T. 3. E 01 1-131 L.I. 8. E 00 L.T. 8. E 00 C5-134 L.I. 4. E 00 L.I. 4. E 00 C5-137 L.I. 4 E 00 L.T. 4. E 00 SA-140/LA-140 L.T. 6. E 04 L.T. 6. E 00 CE-141 L.I. 9. E 00 L.T. 9. E 00 CE-144 L.T. 3. E 01 L.T. 3. E O! RA-226 L.I. 1. E 02 L.T. 1. E 02 TH-228 L.T. 9. E 00 L.I. 9. E 00 ( a) New st at ion added to program. (b) No saeples were available prior to March since goats were not lactating.

M . M TABLE B-ll (Cont.) MllK: IODINE-131 AND CAltl& ISOTOPIC ANALYSES (pC1/1) STATION NUNSEE NKE-4 NAT SATE COLLECTED: 05/07 SA010CNENICAL ANAlv515: 1-131 L.T. 3. E-01 GANNA SPECTRUN ANALVSIS: SE 7 L.T. 4 E 01 E-40 1.23 10.12E 03 NN-54 L.I. 5. E 00 C0-58 L.T. 4. E 00 w [ FE-59 L.T. 1. E 01 C0-60 L.T. 5. E 00 Za-65 L.I. 1. E 01 2A-95/st-95 L.T. 5. E 00 8U-103 L.T. 5. E 00 au-106 L.I. 4. E 01 1-131 L.I. 6. E 00 C5-134 L.I. 5. E 00 C5-137 L.T. 5. E 00 SA-140/LA-140 L.T. 5. E 00 CE-141 8. L.I. E 00 i CE-144 L.I. 4. E O! j RA.226 L.T. 1. E 02 4 IH-228 L.I. 1. L On 4

                                                 **              *e        M O                                  O O O O O O O                                                             -s les e             O wO O O O O O O O O OO OOO O tad                ins O

3 O 3 O O o 3 les tea w w I 8= tea tes e.g

  • tes ses tag t., t, i., w w m e **

(3 . . . . . . . 3% w M O T w e e m e w SN ** M e w w e N M e % e., i O . . N . . . . . . .

                                                ==             > w                                                                                             .        .

I in. . . . . . . .

                                                                                                                   >=                  0
                                                   .               .        . a=. a=. a=.                         .      >=.                  >=. e=. ==. ==.                        e=

e=. e- e- *=

                                                .a              .a       ==       .J       .a             a        .a           e      .#
                                                                                                                                                                                             .                      .      ==.            . .
                                                                                                                                                  .d        .a       as          a        .4         .d          .a            a        -s      .a I                                              =.

O e tad

                                                              =e tes M

O O O OO OO O O OO OO OO O O O tea M nas nas tea tea ens les one ee tes nas o O O O O O O nas had O w O ted

                                                                                                                                                                                                                          *e O

ind

                                                                                                                                                                                                                                      == 3 O O tes      ma N

I f45 D's mN 4N 3% E == 40

                           *3 M

w O ge

                                                                . e
                                                                        *e.

w w m 4de e to tre w N w 4A e e M e e

                                                                                 >=. s=. >.

e=. e=. N. a=. >=. >=. a=. e=. e=. em. p= a= > I as >=. >=. >=.

                                             -d                         me                                                                                                                .                                             . .

a .d .d .d . . w .d .a .d -d s .a a me .d .d a U e.e O A b in I U V N a o 8 8 n e=e u b n tea

                  %e g   e e=4    hd        L3  S                     ==                         M e-o I     a.e a

3, w W 3 O e a'* O O O O O O OO OO OO OO OO** O OO OO OO OO O O == O N == O O g g nas O N sad g ned nad las les nas nas led tea nas tad nad ted tea =ma n.d ena

                      =

es O . . I 4O N T O T T m 4 e-3 a .%. es te St w en w e T W e O w == == w en 40 . . M . . . . gag *1 . . . s= . . . . . . . . .

            ,q                                e             >=.       te.      a=. >=. >=. ==. a=. a=. e.                                               >=.

a= e- e= e-g ad .e se .d .d me -e ed e n=. e=. . >=. .=. . .

                                                                                                                                             .d                   as I

a ed W ad s ed .d =a -s as E e4 8 I e e o e. tM tM 3* 4A eo en. 8 a I

                                      .d              4

( 3 S 4

                               .. eg S                        3 tea     .a               3
                             *=      4               e                                                                                                                                         O W        W               e=                                                                                                                                        w I

tea *= W en e

                                #    E               tes                                                                          96                                                            e O
                             .a      las E

e, e a ( to e W e.t a N O == T O Sb O eft

                                                                                                                                  %         M          e                  w         N          O =* w e e 4A        O                    as
                                                                                                                                                       .O. M == se .= w                              w w tes      ==   M               N                                                                                                               M         M e wO to                 ene       in          e e am ==                                                                                                              N         N e=       S                                                                                                                                                         == ==

I s=8 e e N N 4 4 e 4 tad e e a e ao e e e G a 5 O ted O E 5 3 3 44 e e o EB == ed e 4d S W te. M N N g g e as y u e w to 4 led 4.e s 4 E W as >= 4 11k

I '

                                                  'ma               ==        M         Q O =* O O O O O O O O OO OO ==O ==O cOO O                                                                                       -e                                                                                O                   == ==                    N         -me o                                                                                                                                                        3             O                    O          Q             3 m had              med        tad       tad        tad           .6         tea           had          had       tes        ned                             ted

' 9 ned med tad led has .a ed Eg =s une o e e e e o e e e e e 3% M T 3 @ @ se @ e o e e e . e e 4 #et aus @ @ tA sue d @ St ese en se == ce EO e o m e e e e e o e e o e e em >= M o e o e e o e to o em >= >= p= em em e= p. em e= em >= e- se > e n e e e e o e e ed == o e o e e e e

                                                                   .d                  -d                                                                                                                                                                                 .
                                                                                                  .A              d        .J            .d           .J        -e         -d       .d          .J         -d          -d                      .4        .md            -d        .4 I                                             am O

e amo O O O M O (*. C.d se O O O O O O O O O O O se O O me ame O O =e =e O

                                                                                                                                                                                                                                                        ==

O N == O O tad tad tad had 13 4 tad had tad tee had led had tad ted 3g W had ted had had nee se WO e

  • e e *
  • e e o e e
  • W% N @ O q q se e sue q
                                                                                                                                                                                                 *          =
  • e e o e WM *e h in se d q suo se in me me C/3 EG 1al e e et * *
  • e o e e *
  • e t/3, a= e= M a= em em s=

o . . . e e p e e o e e e e *>=e t== >= >= 0= em a== t= se >= se p. e e o e o e e e om3 .a .ud == .a e . .

                                                                                                .d           -s         .ma           .4           -d         .md        .a        .J         .J         .d         .ma                      .J         .a           .d o

I O n M

  • e m 4 Y

o S X Q o tn a u I w e. M M t.s

                      %  G w                w  E                   ==                -e         M O O OO OO **                              O OO O                 =* OO OO O                          == O=*O OO OOO **O =*

w w 3 O N ** I E E e O O O fill V a >= tes tad tad had had tad ted tad tad tad tad

                                                                         .had e                                                                                                                tad        ted        tad                      tad        tad           has        ted O     E d5                                       se h3                 ==    4=                 o
     ,m3                                                          e         e          e         e            o            e            e e=    3O             M                                                                                                       e          e         e         e          e          o           e 4    SN                                e O                  N         ene                    m              N            N          g e                             %          pte        g o          e             e          e
                                                                          +0                                                                                                                                                                          tre          N e==  G%

p to had Ene o e N e e o e e o g tem O >= e o e e e o e tuo me em >= em em p= e =

  • t= p. km se em a=

o e e e e >= s-. >= >= em I o e e o e o e e ed ed e's e e o e e o and -d .md .mo ad .ma auf .d

                  ,                                                                                                                                                              .d         .md        ad         .md                      ame        and          .me        .md tea 1

2; w l C < o I '"' e

                                                                                                                                                                                                                                                                                                    \

l t I O

e. de 8 ee M m 44 == g
                                        ==              m                                                                                                                                                                                                                                    13 M

I 3=

                                        >               ad                                                                                                                                                                                                                                  d's
                                        -d              4 4               5                                                                                                                                                                                                                                      ==

S 4 Se

                                   *e   4                                                                                                                                                                                                                                                   aus S                     E                                                                                                                                                                                                                                     g tes   .d              2                                                                                                                                                                                                                                  ==

I to aC g O W Ed e* 4A g ql3 nas == 44 sue to ed E tad 96 9 s 41

                                 .4    tad             en                                                                                                                                                        et                                                                           dlk O     3               40                                                                                       G                                                                .a                                                                          ==

W t.7 a  % c

                                                                                                                                                %          M          99                                         O
  • O **

M W O e O 4A eft ** 9 M Ptn me W w W e as to tes ame N O tA 4A 4A ee e e .O. .O. M .M. N N e= O ** 8 T e e e e e e me a== == =me N N 4 e e 4 8 4 tad 5 O e e e a e e a=e O e e* e 0 E ted O E 5 O 3 8 to t#9 4 tad 3 9 ta W W nas ene N N e m == W W e had W aC be m > === I 115

m TABLE B-11 (Cont.)

                             .                              M11K:

IODINE-131 AND CAlelA ISOTOPIC ANALYSES (pCi/1) STATION NUNSER NKQ-50 SATE COLLEtift. APRIL APRIL 04/01 NAT 04/l5 05/06 BASIOCNENICAL ASALV$l5: 1-131 L.T. 1. E-01 L.T. 3. E-01 L.I. 2. E-01 6 ANNA SPECTRINI ANALYSIS: SE.7 L.T. 4. E 01 L.T. 5. E 01 L.T. 4. E 01 K-40 1.26 10.13E 03 1.30 10.13E 03 Ita-54 1.42 so.14E 03 L.T. 4. E 00 L.I. 5. E 00 L.I. 4 E 00 h C0-50 E.T. 4. E 00 L.T. 5. E 00 L.T. 4 E 00 FE-59 L.T. 1. E 01 L.I. 1. E 01 L.T. 9. E 00 Co-60 5. L.I. E 00 L.T. 6. E 01 L.T. 5. E 00 2N-65 L.I. 1. E 01 L.T. 1. E 01 L.I. 1. E 01 2A-95/58-95 L.I. 4 E 00 L.T. 5 E 00 L.I. 4. E 00 AU-103 5. L.I. E 00 L.T. 6. E 00 L.T. 4. E 00 80-106 L.I. 4 E 01 L.T. 5. E 01 L.I. 4. E 01 1-131 L.T. 9. E 00 L.T. 8. E 00 L.I. 5. E 00 C5-134 L.I. 4 E 00 L.T. 5 E 00 L.T. 4. E 00 C5-137 L.T. 5 E 00 L.T. 6 E 00 L.T. 5. L 00 SA-140/LA-140 L.T. 6 E 00 L.T. 6. E 00 L.T. 5. E 00 CE-141 1. L.I. E 01 L.T. 9. E 00 L.T. 8. L 00 CE-144 L.T. 4 E 01 L.I. 4. E 01 L.I. 3. E 01

 '*RA-226                             L.I.      1.      [ 02                   L.T. 1. E 02                             L.T. 9. t 01 TH-228                            l .' I . 9        E 00                   L.I. 1. t 01                             L.I. 9. t oo

I I . e med led had nad tad had tad tes had led had tad lef tad

                                                                                                                                                                              . . . . =

tad had tas

                                                                                                                                                                                                                                         ~ .

nas .d

                                                                 ~
                            ,,,~.
                            ,.,          n
3. **
                           'O                .             . g              .       .                    .      .       .      .       .       .
                                         .d             .d               a a a                                .A        ,    _d     _.      .d      _.     .A       a a                                 e               .d
                                                       . .              3.3o.                              .                       . .

tad had tad 440 had tel tal tad had tad ted

                                                              ,                                                                    med                    ned     had       had               ted                      ta$                e    t.d I

M t, %. ~ ~ ~ m

                                                               .e sta          2 m            =s e            .             . m              .       .                     .      .       .      .       .      .       .      .        .        .                     .                    .

p em te m to t= 0 p. t= 0 t= W. - e. a a e _A

                                                                               .e
                                                                                  .                     .           to.

_A

                                                                                                                                   .A
                                                                                                                                          .d
                                                                                                                                             . to.

a a to. . D

                                                                                                                                                                           .d               _d                         .6 I   ^

k U N m a.3 o I u w 8 5 s e m as a M i N z  % E= V had tes nas 3 led nas nas 3 and 88_. ned ned ned

                                                                                                                                                  . 3                 ..-~

W med nas led had ted med 44 te.s

                                                             .les a                -
                                       ~
                                                                                                            ~
                      .   .- ~s                              .,,              4                                                  ~ to                                                                                               - -
                      .-  =.
              .n                       .d             _d a

_d

                                                                                                                  .d

_. a

                                                                                                                                                                 .d
                                                                                                                                                                          .4 f                                                                                                                                                                                                      .d                      .d but I            =

M n o w I f

                                   -             a S           *E
                                . eg tas
                                                =

4 3 . u o - . 4.

                                  -            o                                                                          .                                                .

_. = 4., 4

                             .-   3 S

o u 3 .~.%

                                                                                                                                                                                                                                  ~ ~

n -

                                      -             ~ .               4.                                                  .        .             -                       -                                             . ~ ~
p. g . e e e e s .m. e e e e e e 88 *
  • t 9 g tes .e W .e 3 3 i
                             .                                                                                                                   .e. la        to at                                                 4s                      3 I
                                      .S*                                                                                                                                              ned                                        aC
                                  .E           .E . .ad      ad a             W              ta.           W      N       N      gg      g              u u .                         y                              u eg >.

E 117

   "                                                                                                                                                                              e,,                                        ,-.._w.,                ., -,_

I I ae O e

                                                    == m O O O O O O O O O O O O O O O O O OO OOO O
                                                                                                                                                                      =e                          O O == .=

O O O O 0 o l nas tas tad N med tad ned tad tes tad w w tas nas nas nas w w w w s= en ** vg g . . . . . . . . . . . . . . . 3% M T O 9 e e e S e m . . . . O M 9 m e e e e m e e I

                                                   -        .m.                                                      - -                       - -
                                    .4              -a      .u.                      .4                      .J      .md      .J      .a       .a       os         -s           .a       .4       .a       os a        d       -s       a l

t I =e O e nas me M O O O O O O O O O O O O O O O O nas e.s O O O O == O O == O O O O nas tad has tad O == == O O O l e and taa nas tas ens ned tas tea taa tea tad w I E M tn p m mo

                     .a %

DN

                     '9 0 en M

e w

                                                     . m en O

ee T T e m e == w e 4A e T e S e tA en e N e W M e m

                                                                                                                                                                                                                                         .       e
                                                                                                                                                                                                                                                     )

J 0- t= t- 0= t= t= >= Im De

                                                                                                                                                                                                                     .        .         .        . i I
                                     .                     M.                                                                        to.                                                                 t=       t-       tu.       t=        p-
                                                     .                                  .                     .        .       .                .      to.             .         .      De.        .        .        .        .
                                                                                                                                     =a' _'a
                                  -d              .J       =e                    -d                         -e      =e         e                       ed      =d              .J       =d       d       a        .J       .d        .d        .a
                                                                                                                                                                                                                                                 . i I

O O n w e l b e I 4J (J w .. M

             ^

N N tes G l l s=4 W j g E g . _* ., 9 O O g O O O O O O O O O $OO - O O O O O 0 0

                                                                                                                                                                              .e       O O               _e      _. _ ~ .*

O O w me om w tas nas and w w w taa w tas w w w w w w w w  ;

                                                          .N.                                                                                                                                                                                        4 I

4 N . . . . . . . . . 5

                 *=                                                                                                                                     .           .                    .        .
                     >O          M               N        O                   h                            h       N       N        N       N                 h 1A  me %                                  en St                      N S S                      se      me       e         N         ==

[ g Sh a g 90 . . g . . . . . . . . . . . .

                                 >=              p=                                                                                                                                                                 .        .         .        .

g == >= a= >= t= p= se a=

                                    .               .       .                        .                     e=.       . to.        .        .      s=.          .          e=. to.         .        . e.       >=.          .

n-9 ed ed M =$ ed M ed ed .$ J ed ed eO M M ed .m0 .m0 es E w > O . O I w

                                                                                                                                                                                                                                                     ?

F 7 a

                             *.             to
       .*                   tA              me                                                                                                                                                                                                       r en              en en              >
                             >              ad 4

e 4 i e s 1

                       =                    3                                                                                                                                                                                                        :

D= 4 W O , W W I W D= idt == taf *= W & ,

                       .a   E               w                                                                                                e                                                          4 8
                        .e  en e              as                                                                                             e O    2               W9                                                                                                                                                          -n W    y                                                                                                              3                                                            %

w =* 9  % M te w N O ao e e e

                            ==                                                                          W S O                      4A      tfe       O                       se      su        fut      @       W        W         N         N
                                                                                                                                                                                                                                                     ~

tas 8't N G tA en en e e S ==e .O

                                                                                                                                                              = M                    e.le == == == .=                              N to   S   sue              a       9                    e                            e       a        e       e        a        e       e              se        e        e        e        e                  6       N.

4 4 8 4 had 0 E O tad O 5 5 3 3 44 m 4 t G W =* 48 S 9 tad had 4 E nd E w te. W N N e 5 == W W G WW EE >= I , 118 t

1 l1 E 1 0 1 3 0 0 1 0 1 0 0 1 E k E

                                               -            0 0 0 0 0 0 0 0 0 0 00 00 E        E         E        E         E         E 0 0 0 0 0                 0            o o ou g           g S6                                      3                                               E         E         E         E        E         E         E         E         E            g N1                                      1                                                                                                                                                      1           I E                             E/

I9 P0 2 4 o 4 s 4 1 4 1 4 4 4 4 4 4 5 a 3 E 9 8 S .

                                                              . 0                .        .         .         .        .         .        .

3 . . . . T. L T. T. I. T. I. T. I. T. T. T. T. T. T. I I I I E L 1 L L L L L L L L L L L L L L L L M R 1 0 0 30 0 3 0 4 0 t 0 0 4 0 8 e 4 0 0 0 1 04 0 0 0 0 0 1 2 0 E E E 0 0 0 0 0 0 84 E E E E E E E 1 E E E E E E N0 . E E 1 S E/ . T9 2 . 0 . . . . . . E . M S Y P0 E S . 4 1 4 3 8 4 9 4 4 3 5 4 4 4 7 3 1 8 L . 4 . . . . . . . I. 3 N A T. I. T. I. T. T. T. I. T. I. T. A L L 1 L L L L i L L L L L T. L T. T. T. I. I M ) C I 0 L L L L L 5 t P - n O Q o T K C O N M ( S I

                   )

1 R E l l K # S L I A t i N ~ Cp U B M e l k 1 1 3 e 0 A ( 1 0 M E L C N O E 0 0 E0 Es 0 0 E 0 1 0 0 0 4 0 0 1 00 0 0 00 0 00 0 1 0 2 0 0 0 B I E E E D l E E E E E E E E A N T A T9 E E E E T A T S1 U/

                                           .              . l.           .        .         .         .

S 3 4 0 4 G8 4 m 1 4 1 . . . . 1 2 4 5 4 9 4 4 U0 6 9 4 1 9 3 A .

                                                          . 4                .        .

1 . . . . . . . E

               -                        T.             T.

1 I. T. T. I. I. T. T. T. I. I. I. N L L 1 L L L L L L L L L T. L L T. L L T. I. I L e I L L D O I e

5 _

s 5 1 - 1 5 5 V V L L A A m 0 E G A A 5 N L U T A R 0 C C T 4 E I C 5 1 L N E 9 - L E P - A O N S 0 L C C 4 / O 1 A 4 / 3 6 4 7 0 E I 3 N F 0 5 0 9 50 5 5 5 0 0 1 3 3 4 1 4 4 4 6 8 T S 1 N - 4 - - 6 6 9 1 1 3 1 1 2 2 g - 1 1 A A - A E - - - - 1 - - - 1 2 7 D - o O E - - - B 1 E S K n C F C O 52 R 2U U - 5 5 A E E A H R B 1 C C S C C. R T g g g

M

                                                                                                                                                           ~

m TABLE B-11 (Cont.) MIIX: 10 DINE-131 AND CAMMA ISOTOPIC ANALYSES (pCi/1) STAil0N NUNSER NKQ-50 0CTOGER OC100ER DAYE COLLECTE9: 10/01 sevfMSER 10/14 11/04 SA910CNENICAL A0ALYSIS: 1-131 (a) L.T. 2. E-01 L.T. 3. E-ci GANIBA SPECTRUN ANALYSIS: SE-7 L.T. 5. E 01 L.I. 4 E 01 K-40 1.24 20.12E 03 1.27 20. lJE 03 Ne-54 L.T. 5. E 00 L.I. 4 [ 00

                                                    >.                           C0-58 w                                                                                                                                    L.T. 5. E 00                                    L.I.       4. E 00 FE-59 L.I. 1. E 01                                    L.T.       9. E 00 CO-60 L.I. 7. E 00                                     L.T.       4. E 00 2N-65 L.T. 1. E 01                                     L.I.       9. E 00 22-95/s8-95                                                                                             L.I. 6. E 00                                    L.T.       4. E 00 AU-103 L.T. 6. E 00                                    L.I.       5. E 00 au-106 L.I. 4     E 01                                     L.T.       4. E 01 l-131                                                                                                  L.T. 7. E 00                                    L.T.        6. E 00 C5-134 L.I. 6. E 00                                    L.T.        4. E 00 CS-137 L.I.      6. E 00                                    L.T.        5. E 00 SA-140/L4-140                                                                                          L.T.      6. E 00                                    L.I.        5. E 00 j                                                                               CE-141 L.T.       9. E 00                                     L.T.        9. E 00 CE-144

, L.T. 4. E 01 L.T. 4. E 01 RA-226 L.I. 1. E 02 L.T. 1. E U2 TH.228 L.T. 9. E 00 L.T. 9. E 00 i ( a) No sample available: emergency drill.

I

                                                  ==              =*       M O O OO O                                 O O       O 3O OO OO OOO OO OO OO O O 1

O 3 o -. o e O o a o med had tad les tes had tee had .ns les I y had the had had N had had tad ted of tas .A t% . e

      .                                           N               M                                                                                                                                                  .         .              .          .                                            .

O w w & in S g w w te ese e in e M e e and N *e Mme tes . . efe e . e . . . . . S ene se em to e= >= es

                                                  >=.                .        e                .                  . e=.

een e e . to. e=. . ese em e to e== km em >=

                                                                                                                                                                                                        .                     .               e         e                                  a         e end             M       8's          end                    =s           d          d     .ma        .m0       and          .md        .us         .ud        .ad           s         and             a                               .md          d I                              M a=*

O e had O O O haf M had 9 O g g O O O O tad O O O O O O O O O O O tied has had led isd had a.e the O O O O tes had las had O == == c O O tad tee O had O ene tee I gn Q EM sad % WN O tas se O N

                                                >=.

M De e se. O e W ee T T De S sus T he S T eo T e

                                                                                                                                                                            #8e e=

e T T T 0-T pun M WW

                                                                                                                                                                                                                                                                                                             ]

I

                                                                   .        .            .                     .         .           .        .         .      e=.              .      e=.         De.            .         .

een e pm. >=. >=. a d == a .d d e d .O d d .d .d a .O .d M a .d U m M ,O, e as , l M C cv C Pe w O O E U E4 ^ w .. w as I s-4 e=4 U S l X b 3 == .mo cut g O e g e g m amo se v O O O O O e O O O O O O OO OOO O O eme O .-e me N == E e O O g M tas O .Omo tag nas nad cut nas and . tes nas nas nas nas ans tad has las nas tad w tas ina 4 e= E == . . m. . . . . . . . ins % M in O en am en

                                                                                                                                                                              .          .           .          .          .            .            e                                            e en   a me                                     me amo                 amo        em e w == q en                                                     ce         .-s            w                                            ==

M O ne m E . . ee e e . . . e e . . g e= em

                                                                                                                                                                                                    .           .         .            .             .                                 e         e
                    ,                          e=.            e=.                                                                                             no                                 a-         >=

M. . >=. . se. e=. e=. . >=. e=. p. e=. e=. e.

                                                                                                                                                                                                                                                                                              >=

g =a e == a s .d a a .d d a a d a a a .d e lE a w O O M

                                           ..           en g                            en            ==
                                          ==            tM 4A            no am             .ms and           4 8

4 O E taa .e D em 4 S G W W em idt 9 tid == W se a E ene S e e s one a. e 4 O 2 to O  % a W ed G ** W G S

                                                                                                                                                   *==.      M           q                      w          ram         O == w                                           @                     e tes    ==   M                                                                                O en                tA        O e                     se         sue        M           9         W              W                      N                      N
                                                             *mn       O efe                             tA         em te e                        S*        en                      M          see        es          me e=     S    ==*                      e                                                                                                same                                                     se             amo                    N                      N I

e o e e e e a e e a=* e 4 set e 4 tad e 3 O e e e e e e O 5 "" ed S M E W tad ts. W O N Net 3 3W g e en en 4 tad and aC E j N == W u e W W es >= i 4 i 121

3 M 3 3 3 4 3 0 3 - 12 4 3 M M M g 3 e u o o o a a 3

                                             'sas n.s        .            e . .                            e       d            d                 .          .a.                               e, e*                      &

Nat . N e . . e e e e e 3w 4

  • N N N e== N N W o e o e e e . .
                                         %                           3                                                                                    @          N         N         N          ==         ese         A          me         ==

en tae *e 33 * * * * * * * * * * * *

  • s e= ae == s= e == e= e p. == e. > e= m-e.

3 e e e . *

  • e . . e e e e e e a N 4 4 4 4 4 4 4 4 4 4 e e 4 4 4 d d e I '

N N M M M M So M M N We M M M me N N me Q 3 O O O O O O O 3 O O O O O 3 3 s I A Og

                                       %3 are S 04 w

N e tea M M O m e tas N e N nas tas w e 9 e N e tae T e N and e tes N e tea e=e e les nas one o d N N e e ned M e M ens e tes em tea M to M e o men e o e o e e p.e e o e e e . .

                                                        >=         N                    em        s.=       >          to         sus       em         te
                                                                                                                                                                                                                                       .         e e         e            e       o          e         e een        e-        >=         tem       a=          em         s.m        >m      I o          e         e           e         o          e         e         o           e          e          e e.$      N         e.d         ed        ed        e.d        ad         M          ed        e.$        M a

e.$ ed ed d ad ed M and N < M I e \ 3 i

                       *%  te.

N t= M w a I .* Oa one M 3: M t/ %e h3 e2e m J  %  %.

            #          e W

z e M O ene e.e . M .e O O 4 m O O O O ame -e N I"* M w& e=

                                          -                                                                           O
  • O O O O O O O O O tad nas tee tas tee las tse ned
                            .             n.n
                                            .                    l,es                                                                                 tes tas les tea                           tea        tes         naa        mas        tea 4          N4                         M em en Ow                  e         e          o         e          e        e           .          .         e          .          .         e         e          e tan 3 e e 4ee                         N        N         N           N N                  N          e N w                          N          ==        me e           o een == ==

e e 09, m e o e e e e o e e e a= w se . e . . e e d a= >= em em se em e= tas e e e e e. . e e e o e o o e e e-e

                                                                                                                                                                                                          > >= >=                            em De           ed        M         e4          ed       eO         e.$        ed
                                                                                                                                                                                                              .           .          e         e ens       me         ed         e.s       ed        ad         ed        e.f         ad          ed         ed 1

l l i se

                                                  ==
       #                                          Y be ed e            E                                                                                                                                                                                                    i tas          3 e=            a                                                                                                                                           O W            t=                                                                            4A e

w w S see . 4 w e l ens en e e = O M S ed W  %

                                                                                                                                *%        M                               W         N         O          ao          e e                    g w           S S S
  • 61 O se M I

tad A O M g w w N N tA 4A 4A @ tap A ese ame M as se se se

                                   >                   e        9          e           e         e         s          e          e         e                    aus ame        N           N e                    e          e 4                 has                                                                                                                                       e          e           e          e          e e i e              a w e

IOw w w tad O S S N N a 3 3 e

                                                                                                                                                                - u u GA        M         4          tad u w . -

nad ( 3 I 122

t 1 i i l 1 l l l I l i i i gaggO o - e e ge - - e e 3ee -.o e o e ~ e_ _e

                                  $       *** *             **8      hd          4*8      the     ta8     w w          tas    the                           nas nas tes    tea                            w          , w e te.                   ->

e> e e . . . .

  • E N m f f**N e k m W
  • C * * * * . . e e . . . . ,
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                                 =        -* a -.                   -4           -.       &       &       &      &            &      J j j j _; ;

M N U3 m >e =e

       . e.3        e a                   x        x        .o     n e o                          me        e - e e C            a    te.                                                                                                    .e     e e                   =e       =e      -e      ~ -

9 w a= M e tad N. tem O e e e e e e e had led had led lef tad Gef taf e e e e e e e e e e a > en tai ted had had lee V ** U e e4 M had had had ted tad

         *E*
         .. M    e 3       ou             e          e      e M   Se  m 3        %            tA     ees
                                                                     .            .        .       e       o      e            .       .      .              .        .

Ne e s=e O  % = -3 tA e N te ne ~ ~ tA tA en N == se

                                                                                                                                                                                          ==

g b @ ** E u e *e .e, . e e e . . . w

                  & O tas e
                                                .e   *     > > de>& > > > >>>>> > > > > >
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N & a e o e e e i hPI N N en Y t e e a tes $ W g o has u g se

                          -a        les
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l 123

                                                 -_-                     __ _ , . . _                       _ _                              _ _ _ - _ . . _ - - . , . ...____..-.l

1 I k I A to 4 N nad 3 O O O O O O O O O tea 4 M tes tad tad .es ned ted a - ~ tad ind 3 and a.e O o ies

                                                                                                                                                                                         -e td 3 3 = c s
                                                                                                                                                                                                     .4

_e tea

                                                                                                                                                                                                                           .s w

se

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e I No . m e . . . . . . j O N e N N g N 9 N N N g e e e . . e e .

                                  %@                             O                                                                                                            N          N          M          g          aus        er e
                                  @ tad                           **                                                                                                                                                                                         l es   ..             e-e       e
                                                                 =0         a=

e a= e e o e e e e e e e o e o e e a= em s= s= a= a= e= a= e= e= g e *

  • e e e e e a= e- == e=

e e e e e

                                                      .a                                                                                                                                                         e I

M e e

                                       >                                    -d        .4         .0         .a        =a         .ma       .d          -d         .A          and e           e 6

in .md .J .J .d .J -d s I - . O .* O O O O O O O O O O O O O O O . . O O O

                                                                                                                                                                                                            .e        .e           N O O E

I tee nas ina tes tad tas had les 3 nee tad tad tas nas nas ned tad ted tid j hq m > OS

  • N e * * * * * * *
  • e *
                                 %                   en           e       en en                 me         e         me
                                                                                                                                                                                                    *          *
  • e .

tp tad O 4 4 w one ers e N e=e w me en O e= es l

                                      ==
  • 4 e e e o e o e e I

e e . e e E tas e a= em me >= a= s= a= e e e 2 e o e

  • e o e e e e- >= > >= se >= t= e= e-e * * * *
                                                    -d         N          -s        =0          .0        .0         -0        -a        .0          .d                    .e         ad
                                                                                                                                                                                                    *
  • e e 6
                                                                                                                                                                .ma                              -d         .d            d       .d         w             l l

I ' I 4 M N @ h M h M h h h 4 O O O O O O O e O O O Oh h O O O O ON O 3 M M M M We N en g M

   ^

u esa aan e-2 w e Nw

                                    =

te. ww w wwwwwwwwwwwwwwww j l Og a m . . e C O g 'W N ted

                                **                 S O
  • 4 Pin N W N S S N N m G me e

N N se U e o les ce ' V ** U S 3 3 e e e e e e e e e e de 3 e o e e o  !

n ee .a a= m e= a= e= a=

e e e N N

                  %    a            e                e          e          e                  e=.                  a=.                  em. e=. me.

em a= > e. == b ** . . e . >=. a=. e e I

                                                   .d        M                    ed          ad                                                                                                                                   .           .

a=* eme O W = ase and auf ame as and ad ed ed ed eme ame .d -f l b Ese

                  .&., O g                   =e p=
   =J                  we S

I 4 l H< O We M @ $ I 3 ese $ See

                                                                                                                            $ $                  We          sue        Q $                   em         me en
                                   =

O O O O O O O O O O O O tad led led ned tes had gad O O O O ON O sue ame tad led dee tad tad led na. @ lef tad ned les tad ' eID s'I i pim et e e o e e e e e e e e I OW @ O 44 e N N ao e e e e e e e e

                               %                                                                                                       N en N te te                                           se         se        nn I
                                                             *e           e                                                                                                                                                    me         me               '

an a ee e e e e e e e e e . . e e e e

                                   .#            >=         ta         e=        e-         >=          e=       e=                                                                                                   o           e          e e                                                                       s=         to        >=          o=        e=          e=         we         n=        >=          e=
                                  .d                          o           e         e          e          e         e         e          e          e          e                                                                          o=

the N e o e e e e e and ed and and em$ ed -d ed

                                  >                                                                                                              am8         and       and         and        ad         and       ame         -d         and            a I          .

I se 40 Y I I I

                                           -d 4

3

                              .e 4                                                                                                                                                                                                                ?

O E tad 3 a= a O I W >= 4A e tad qua ** w w S e e

                             -e           e.                                                                               G 4                                                               !

O 44 E -s t 4.5  % i

                                                                                                                           %          M 49                             W          N          O 4                           W         W          St          O        tA         4A         O O                   me        8"o se         w e W                                      l tad e=

E Pts O LA in tA te te S se me ese me 8't suo 9 se 9 me T 8%e N ' E e w e e a o o e e a se eso N N I 4 4 tad a 5 O O E e e e e e e e O e lad W 3 3 e wt M 4 tad E ta ad E W wW me sie e S == WW tad 4 GWW W e= i l l 124

i

  • N *e =us me =o ame me P om. me o @ O O O Q 3 O O ame N se .e .m. N ei, .
m. 3 o O 3 C. O o Q 3
                                                  .              w w                i.a          d       w         i.a       na          w w                                       6.s g                        de                                                                                   a       e4                     w w                   jd          i.s         .a           w e-I*                               ,'

gg ou g

                                                                 == O ==

M. ee

                                                                                               =e M
                                                                                                                   =s N **

N

                                                                                                                                                      .         e st == == =*

e . . ar. M

                                                                                                                                                                                                                                ==

N N g.s - 3 o . 4 . . . e e e I e a *= w e= e= ** e- .= >= >= a= a . . . . . a=. ==. em a= a=- a=

                                                                 .4       M         .4         .a       .4         .d       .d          .d
                                                                                                                                                   .d
                                                                                                                                                     .         .         e          e            e         .           .           .        ==. ==.                   ;
                                                                                                                                                             .4        -d         .A          ed         .d         -d         W            .4           ed           l E

e .= G o o m ooo oo o= 3 c = o o= o= o=e oo o o = = = N = w 3 o o o e wa w w w w a I

                                               . s=                                                                                                                 .                      w w w                             w            w           w ab g ou                  .      m.         .          e         .         .         .          .          .         .
                                              %                e Q               N          4         N         WN                   m
                                             == 3                        e ao        e        N          N           N           N          N          e == ==

ao

                                                 .d w

I e . . . om = w . es. a=. ==. >=. e. >=. . >=. s=. e e= e m. em e s= a= .= om

m. .s M .d e o e
                                                                                            .d        .d      . .a        .4        .a           me       .d        ad         .d          =s          .d        .d         .4           .4          .s t/I M

I N (th e ~

            ^            >e           3
                .             a w

ed g w W 4 2 a.d O e v .* U mm s de 5

C M  % a N  %

t,th me o oo=eo o ==oo o==e== o =* o oo==

                              =                                                                                                                                                                                                                                      t
                                                             =e
            .-e gg I

N b Q M W

                               " O
                                - =

s e= o w w o ins w w w 6.s w w oo o oooo

                                                                                                                                                                                                                =e         ==           N ==

I C en ins n.s e.a n.s w w w # M M W M w. og . N. . e e e %3 3 o N N

                                                                                                                 .         .          .          .         e         e          .           .          .. .                   .

R~ , =8 M N W N m a e N N W, m N e = = p =. o e e e e . . e o e a= w em he I De De >= e- >= tm. p= l e e e e o De. a= >= em

                                                             .8        N       =s         .d         ad e

ed .4

                                                                                                                                      .          .         .        e           .          .         a=. >=.                 e            e            .

ed ad .e .d -s .d .d -s ad .d w 4 i

                                                                                                                                                                          >s e

I sA. e 0 i x I 4 . G E t.s 3

                                         >=           es                                                                                                                                            e W           >=                                                                         nn e

w W m we

  • w a I
                                         .d           sh.

e eb o to S

                                                                                                                                                                                                    .d i

I u  % ( e e Vs, C.

                                                                                                                                 %           #=9       te                  w          N             o w==w w eN mN
  • r nas N o JD en re @

ad in m me o ome == m =e M w o= e e #=e se me =e me N N 4 a.a e e e o e e Te e se o e o t S e p o . ned o 3 m 3 3 e to to < t.ed e e e GA S W R WwW N w a 5 =* W W S W 4.s W 4 eg >= 2 5 1 1 I 125

I l l I I I O N m O O O O O O _ O N _ O O O O O O O O O O O O O O O O O tas nas ins m m has tas nas tes nas nas nas taf W tes nas tes w tas w =s Ee um . e. en. . . . . . . . . . . m% M O O e m . . . . e e e =* =* == m . . I 4m N ** N N m N N EO .e *e p.

                                                    .         m e              .             .         .       .       .            .              .       e       .       .       .       .       .          .         .

e= a= p. >

                                                    .         m. N.        e=.               .         . a=. a=.              em
                                                                                                                                    .              .       . e=. e=. o=. s=.                            e-
                                                                                                                                                                                                                     ==.

g,r3 .4 m to . . . a .4 .a .a .a & =a W a =# .a a .a .a e w f.f3 e1 I M Q E M F* O

               #4 O.e a   e e

e a O N s-4 8'= 0 m O O == O O O ca .=* O O == == == N O O O O O O O O O O O = I w a O O O O O O O g g 3 nas ins ses ins e ans ins ins ans ins ins nas ans

         >            e        ze                            N w                                                                                               ins    ses     ins     nas w w w w W                                                       m ER*

an B uO 5%

                                                  .             . a.        .              .        .       .       .            .              .       .       .       .
                     ,%                        en            O O          N             W         N       N N W e te == e d           v =       =O N       ==                 w =               ='s I     y            6 O                                     . .

w ==

                                                  .          O O             .              e        .       .       .            .              .       e g                                >=                                       a=                >=                                          e=

e- . m. e. >=. . a=. . >=. e.

                                                                                                                                 .            >=.       . a=. e=. a=. >=. .=.                        e=        n=      .=
                                               .8           O     Y       A             &         &       &       &          &                &       &               &
                                                                                                                                                              .e              &       &          O          6      &       &

a - - I

         &    M s=e E

W 2 se O I C M

                                           ..          e tA           -

ee M en. 3 3" -a

                                          .4          4 4             8
                                    . k            =

mas .,a m

           .                     e=      4            5                                                                                                                              O W       W            >=                                                                   en                                                        w las     **                                                                                                                                          .-e s    E
                                                      %J ins m                                                          o
                                 .=us tes I

e

e. e 4 O 3 en a W 44 a  %
                                                                                                                           %                M        99              e       N G    =*

M w W S O 4A en M se m M w w w O .=. W @ O tes == N O 4A tA tA te @ m O.e

                                                                                                                                            .        se      m       ao N       N e=      O    me             a w          e             e         e       e       e          e                e me      ao      se        ao        N        N 4       4                                                                                                            e      see      e       e O       5 4      4    tes     s     WO                     tas      O 3 m                              3 3               e      en      4A      4 e       e          e 4

e e

                                              == te        e ad M W                                      u       N        pe                g                                                nas       tes                2 tem                                                  g       me w w a u u a                                          m.

k I I 126

M TABLE B-13 (Cont.) BROAD LEAF VECETATION: IODINE-131 AND CADGIA IS01DPIC ANALYSES (pCl/kg UE T) SIAil0N NUNSER BLS-1 NAV MAT DATE COLLECTED: 05/01 JUSE 05/28 06/26 BAOIGCNENICAL ANALVS15: 1-131 L.T. 4. E 00 L.T. 1. E O! L.T. 1. E 01 GA8MIA SPECitum ANALVSIS: SE-7 1.222 0.15E 03 8.574 1.75E 02 5.964 0.71E 02 E-40 7.38t 0.73E 03 8.51 0.85E 03 8.32 0.83E 03 Me-54 1. E 01 L.T. L.T. 1. E 01 L.I. 7 E 00 C0-58 L.T. 2. E 01 L.T. 1. E 01 L.T. 7 E 00 FE-59 L.T. 3. E 01 L.T. 4. E 01 L.I. 2. E 01 CO.60 L.T. 1. E 01 1 L.T. 2. E 01 L.I. S. E 00 23 65 3. E 01 L.I. L.T. 4. [ 01 L.T. 2. E 01 2R-95/NS-95 2. E 01 L.I. L.T. 3. E 01 L.I. S. E 00 AU-103 L.T. 2. E 01 L.T. 2. E 01 L.T. S'. L 00 RU-106 L.T. 1. E 02 L.T. 1. E 02 L.T. 7. E 01 1-131 L.T. 5. E 01 L.I. 4. E 01 L.I. 2. E 01 C5-134 L.I. 2. E 01 L.T. 1. E 01 L.T. a. E 00 C5-137 L.T. E 01 I. L.I. 2. E 01 L.T. 7. E 00 SA-140/LA-140 L.T. 3. E 01 L.T. 2. E 01 L.I. 1. E 01 CE-141 L.T. 3. E 01 L.T. 3. E 01 L.T. 2. E 01 CE-144 9. E 01

                      ~~

L.I. L.T. I. E 02 L.I. 6. E 01 RA-226 L.T. 3. [ 02 L.T. 3. E 02 L.I. 2. L 02 TH-228 L.I. 3. E 01 L.I. 3. E 01 2. L.I. E 01

m O N M I C O _ O .e O O O O O O O O O O O O=. OOO O O O O _ N = O : m tes has tea nas nas tas W tad w sea w tes ** O and ins nas nas tas tea w a w tN tes % tA O O S S w e . . N e me e . . . . . . . . . . . e N @ W I a.e N St S == e= m *e *e N N N N

4. 0 ene e e o e e e + e e o e e e e to be e se >= De t- em em > em a= t=
                                                                                                                                                                                                                    >=

e= e e .

                                                            .               e     S.         .        e        e            o          e       e          e       e=.           e        e         .

e-e e o a= a= e.a Y & & & & & & & & e e

                                                                                                                                                                              &       &         &        aa         &          .&        mO         e$

I . f i-O M M =e == == se a=* ==o a.e N === === === == == i O N N -= O O O O O O O O O O O O O O O O O O ins w ins nas nea nas w w nas ned nas nas nas ime

                                 >= S                                ede        Q                                                                                                                       ens        ind        tea       ==a       i.a en N                                en g             3%                       e               . e.         .        .         .          e           e        e          e g             WG                   w              O O                ==o      **       M         s.*           M == ** **
                                                                                                                                                                    .          .        .         .        .           .         e         e         e 3O                                   es M         **       s=o       N M                   **       M M             4 to                                                                                                                                                              d=e
                   >e                                                m I
                                                          .                     M          .        .        .          e            .       .           .          .          .        .         .

em) W . . . . e

e. Das D= e.m em >=
                                                                         .      O.      e.m.        . Du.m          .            .   - em.                   e.

to t= een p= em. em ed =4 @ a e.s ma & & e4 a es

                                                                                                                                                                               .        .         .       .           .                    . e.=.             ,

e4 & s a.a s .S en es 2 n Q Oe p I w u e 3 e e e.e lhe em

                            =*

S e e t i h3 m e t M *l> as O M M == e-e  % E ==e == ==e == == e N == == == == .= , O O O O O N N == i g I sne - O u - O O O O O O O O O O O O O O y

                        &   e=

tas sea nea ama nas ins ins sea nas nas nas ene ens esa w W M ned sea nas e.a ==s M 4 s.e M > hm g I d e N. O 88 -a % N e . . . . . . . . . . n x am O O N N en N in M M N w M M w in . N e . is's =A q 70 .e a 3< . ~ e . . . . . . . . . 1 g N e.= em

                                                                                                                                                                                      .         .        .          .          .         .          e             .

g g a=. e N. e em. . e=. h=

                                                                                                                                          >=.

em e=

e. > e= em e= e= s=

g s N w a .4 a =a &

                                                                                                                                   .                   .          .                   .         .        e          .          .      =.           .

a a a .a a =a e .4 .4 a e { 8 I  ! l I e. . en e. em to Se t.o ga 3*

                                                                                                                                                                                                                                                                  ]

i

                                               >              as 4                                                                                                                                                                                                   f 4              E                                                                                                                                                                                                   .

E 4 , e* 4 , e., E i i .a a O e= = a e  ; W W I De nA i tas == W se t w I S e ene a see a. e g O x en e 4 w W a w l O *=e W W G S O 4A

                                                                                                                                         % M e en                                        e m MO -. . e e ans       ==    M          g   h           O       4A S         me         M                  W        W            W        N          N we wt e e e                                         .G.

I

                                  >=        S      **         a               9
                                                                                                                                                              =e        M          se       se                 .e           .=       N          N 4         4 e                  e        e        e         e             e*       e          e          e       se          e        e         a         e EuO e        4   tea                                                                                                                                                        a        e          e O         =     - u            = w e                        tes O                   E        E          O O                   e        W        40        W        las          nas      4          2 te.       w             M        p.
                                                                                                                                                   = = - u u a w w a -                                                                                            :

e l I d 4 t l 128

                                                                                                                                                 - - . . . . - _ . _ - _ _ - , _ _                              .~_., ._.                           . . - , - . ,

I g tad me O O tad e N O O O ted e 8"t tad N w O ==. O O end W

                                                                                                             =e           amo ned me O O O O O O O O O O and      w se         me tad me tee         w w e

tad e se w w me me O O O ena N w e. e EM% . . . . . I

,                                                                                                                                       .          .          e           e         o           e          e 9                O O                  O           ao         N            ==*                   as         ao
                                                                                                                                                                                                                       .           e          .         .         e tes h                               es         ce 8't                             e N                     ==* =* ==                          N          e         N         N Mme ins O                  t=

e m e e e . . . . . . . . e e N aus a= a= se se >= s= e= pe e e . . e e . e e e e >=. em >= e- >= e- >= a= e e e e . e

                                               &               & Y                   &           &          &            &           &

e . e e .

                                                                                                                                               &          &          &           &           &         &            &          &           O         O I

M O O O O O O _ O O O O O O O O O O I O O O e w tes nad tad w tas tad W had W e= w tas med ned w tad ned w tad and and c/) EG IN t=*=* idt edt

                                                                            .         .           .          .             .          .          .          e          e          e           .          .

M O N N te M . . . . e M >== @ M M N @ M M M e N @ p O ist I E g O a e=. ed e-and

                                                                        .=

O.

                                                                                   >=.

and t= ed e t= ed sm. ed

                                                                                                                                   >=

ed e a=. ed t= to end e s= ed e

                                                                                                                                                                                          >=. >=.

and ed to and e em. ed o= and o= ud e >=. W e

m. o 9-4 m

Se U h O en c 4 Fe e r O H O >= a ' u M c4 w ed g 3 e I i m  := = '

    *            %     W O                M         M            e       =. =.                   .e                         e       .e         N           .e f                                      O                                                                                                                                                       - - - ~ ~ _

m Sh* 4

                 == O u     =e                   w O O wO O O O O O O O O O O                                                                                                                        O O O                              O O M         & ==                                       and e.e       E                     t.s         w w w w                                        i.s       w            i,a        w w w w                                       me,        .e,       w Ca3 e.2      w     4  E                                           w I

g o= ens O e M. a

  • Sa *
                                                                         .          .          e           e            .           .         .          .          .           .           .          .            .          e 4

H - *m =

                                                                      * ~ ~ " ~ " - ~ ~ a ~ ~ ~ a - a                                                                                                                                   .         .         . i W _O                .             ~ e d   8 O                 >=

e n"4 . O. Pa.

                                                                         .       to.

t= to

                                                                                                          . .      >=.

g= to. >=. em >= > om om a= e= em. I M

                                                                                                                                   .                                e f

ed M e .4 ed ed ed ed ed e.s ed .d

                                                                                                                                                                                .           .                      .          e          e          .         .

d ed ed e .d .a M X w t 8 > I f ** en

                                      ==

M

                                                       .e en i

l t#9 > I

                                      >                                                                                                                                                                                                                             l ad
                                                                                                                                                                                                                                                                    )

r E 3 * > O E i tan ed 3 .

                            >=       4               e                                                                                                                                                        O I                         W tas ed ed O

W W

                                     ==

3 ted E W t= W tes to tdt e G E e

                                                                                                                                          % M e                                       w e

ame 4 ed e

                                                                                                                                                                                                              **un I

O *e w WG G ndt 4dt 8=. O me e te e > t O O m ee=ew se w I

                                     ==                                                                                                                                     ese       #89 had           889             Fem        O          edt       tdt         tdt        te O m                                         =e          M N         N         '

to O ** 0 e e e e o e e ame me me me N N 4 4 8 4 e e sus e e e O S " @ tad 0 WG tad O E 5 3 3 9 t#t 4 6 e e a S 'W E W te. W N N e W =* W QW9 W tad had 4 3 i S W W M >= ' I $ 129

l l I I . O w N - . . O O O O w g w w w w w w w w w w w w w w w w O O O O O O O O O o o o o a

                                                                                                                                                                                    . . .                                                              N ze                               ,

I wN . a. . . . . . . . .  ! m% M O O O e N (m .* N e a en me a e e N N N N EO *e ce

                                          .          e ega                                 .       .         .       .      .         .         .                    .        .       .       .            .                        .             .       .       .
e. p.
e. o. e. a=. e=. a=.

e.

e. em. e=.

e.

                                                                                                                                                                                            >=. e.                                                     e-      e gp3                                      es e
                                                                                                             .       .                .                                               .                             >=.                           .

W a -s .a .4 .a .a w .a .d .a -s a -s .a .a a e til 3 I ^ u e Q N

s g.s u

N b se e cr 5 l i i C a

                 = a                  o             N     e.t                   O O
                 *=                  O                                                                            O               O O .=                                           o o                                                                N w as 3                   tad O O O O O                  ta8            ted       tid O led O       Oled O                      O       O        O       O          O            O                          O        o       C                           4 i

Gad las tad tad m > z. . , led had had ted tad taf tee I b I w. . . . . . )

                 %   E   5%          edt g             =.      4m                        O O G W N
  • N 9 m N N tot e .=* .=* trl N a

W E EO 4e de g g w a o*= . e e . . . . . . . . . . O **

e. em.

s.* em om e 4 .d 4 , N. . n=. to. a=. om. a=. . . em. se. em

                                                                                                                                                                                                         .        a=. *=. ==.

n=

                                                                              -d                 e      .d         a    .a       .s       .a                    .d       .a      .4       .a         .a e                                                                                                                                                                                                                                         .4 a                                a       a I
                                                                                                                                                                                                                                                                                         )

A M . M 1 W X w 8 t#t e. m

                                .=           44 Sm 4M.

3 .#

                                 =a          4 I

S 4

        #                   las .d           3
                           >    4           m                                                                                                                                                      O W    W           em                                                                                 til W

las em W .e

                            .a  E           tas e                                                                     e e

et N N h w tes w W m. N O W eft W eft 9 til O tM s M 4d% S O a.e

                                                                                                                                                            .O.

a e.t N.t e Ne O e w w . . . e%# e%e D= 3 .M. e ey e e t s.s se m. N e e o e e%e I e er g e 4 tes e g O e a e e e e e e e O e == ta e ad a W tas te. O W es 3 W 3 e en to et tea tea et E N N g a m. W W st W W es *= I  % l l I 130

l i I s'. 3 N W OOO me M tad S QQ W OW sue OO tad O W W W ame OOOOOOOOO g ame led sie W ame W Q g 140 W me tad 400

                                                                                                                                                                                                                                 ,,e 3

had eg, O tad o tad a

                                                                       *==
                                                          .              .      M.          .         e         .        .        .        .        .

e a G N 9 N 9 m N N m WN 3 9 N e N N S% #8 *8 sq

  • O M . . . . . . . .

i

                                     =3 O              >                                                     a=       om i
e. S. e=. e=.= e. >= >= p. m.

ed M M

                                                                                                                .        . s=.         .        .      e=. e=. s=.                       e            .

e- = ad e$ qul m$ ed M ed ed ed .O M ed ed ami and ad I S see O tad N tas e M W eA amo O O O O O O O O O O O O O O W eo tas me med ame ted amo has ame had ame med has N ao nas ame tas ame tad

                                                                                                                                                                                                     =s tad
                                                                                                                                                                                                                 ==

O O tad N sad N O O w

                                                                                                                                                                                                                                                     -me
                                                                                                                                                                                                                                                     ==s I

t= N . M. Fmm. . . . . C/) 4% . . . . . me O . . . . W Em sme se se er 0%f gy se N me er me N N

                                                                                                                                                                                                                                .         .              e M           .e          mm m                   O                             *
  • p=
                                                        .            O        e           .         .         .        .        e        .        .         .         .         .

J w. w a= t= t- p= p= pun a

                                                        .                       .         .      De.          .        .        .      suo. em. >=. a=.                         .      >=.                      e.          >=. >=.

em I e m a a a a a a a a a a a a a . . a a a 2 y **

      ^       O    M d
         . M    Ao a       >    O
                              ,d e

I C 4 E*

  • O H O >= m u ha to w tan v M a e n > <  ; !

I I == W g ~ M , O .e O O. m E bI u O

                          & =

a= bad G O O O O O O O O O O OO O O O O O-. tes had e ~ O O a.] me en g had had tee les has tne had tas had tee tai tad nas had w tas

     .mJ c,           4        ==

g M - >= mO a. e.

     <       q   q            e

{% en . . . I H O O O *=. e N es N e e M e e .m N e N e

                                                                                                                                                                                                                                                  -=

08 M O , . E O . N emi . . . . . . .

                                                   >                                 t=                                                                             .         .          .            .           .          .          .             .

c=1 t

                                                      .            8".5     e.          .      to.       >=. . >=. to.               to.

t= pi t= se. p= em. e== >= e= a= bI

                                                   =e              e e               me        -d         me      .4        .a         a      .d       .d        .d
                                                                                                                                                                           .A
                                                                                                                                                                                                 =a
                                                                                                                                                                                                                 .           e          .             .
                                                                                                                                                                                     .d                       ma          .d          -s          .4 7.

M Q O M I l

                                              .e en een in en m

4M

                                                             .d ed              4 I                                 e tae a=

ena g as

                                            -d 4

4J 4 E S S as

                                                            >=

O e tas == W 4A ame . I .4 E tad D e e

                                     -d     tee             &                                                                                                                                   4 O      2               to                                                                      e                                                           -d 4J      W                                                                                       a                 q                                         %

O me  % M w pm. O am. w e e e g 3 O gm gp S O tas == M Pan O 4A tA en eg 49 9 ee aus M M er er w N N se S ame g ey e e g ese M amo suo amo suo sue N N g g 3 3 ese 4 4 9 4 e 0 0 S e == e e ad tad e E OW ens E te. e a e 3 3 W N e to to 4 0 and g ned 4 e Z e N g g == u u a w W eg = I l ,m 131 !g r i t

1 l O N N O _ O .e .e O O O O O O O O O .e .= N , g w O O O O O O O O O 3 I w tas

                                                             @      N med     w w w w w                                    tea      w w w                           tea          w w w                          t.a        w                    .

N N @ I,N e e o e e e e e e o e o e e e

                                                                                                                                                                                                                          ,                    {

1 t,% N Oee O == 4 N e N m ==e o e e e o= m ce a N m ==e sie N N == N Ge 9 gas es e N N e e e o e o e e M De 8'l Pte to >= >= e- Bus B- Be to e e o a= e e e a e e e e o e o amo em B= t= em N s-e e e e o e e o e e e

                                             -d             W       N        -d      ed        ad                ad e            o     j
                                                                                                       .d                ad        -d       ed       -a           ed           ed        -f        ad         ed         N           me s

I O O 8"9 889 ==e *=8 O O O O O O O O O O O O O O O O ON

                                                                                              ** ==                     me           e     N        .e           me           ==e       == ==                           N            me O

tes tea nas las w w I ted nas tad les BG N en nas led tad ens tad w tad tes med M tM N N **9 N 3% e e e e o e M Wq egg O O me ao f"I se e det o me e one o se e e e e o e o e o 3e ce ce fut se am N fut me seg set M 4

               ,,s                             e          .=       N          .       .         .        .        e        o        e        .         e            e           .         .

be one W >= ene se >= emo . B= to >= *=

                                                                                                                                                                                                    .          .          e            e e             o       e        e       o         e       o         e        e        e Bue o

De se pm Bee >= a= e e e o e o ed b N and ed ed ed ed w auf euO end auf e e se em0 and em' EuS eu0 ed e e o M w b N I M C .e ene e M 8" @ g * . w n =0 . e I m g M g e.2 b a=3 O a

                   = O u

w W

                        =o B=

4 == O O tad N eet O O O e O e O .= med 6 & one and o q tas tad

                                                                                             ,e tad q

tea O OO0 O O O and tas and

                                                                                                                                         .e tas       w e        .= q tas G

tee tea e O O O O n.# e tes e N

                                                                                                                                                                                                                      =ma
                                                                                                                                                                                                                                   -e O

tad e. ti#9 s a9 . e se. . e e . e . . . ed % W O O 4 h N W N W

                                                                                                                                                     .            .            .         .         e          e          e            .

DN W @ an am W me N @ N N 7O *e ce g e W e o e e o e e o g g *= W* W e Be >= to B= pe e= e= e-e

                                                                                                                                                   >=

o em e p. e o= o e

                                                                                                                                                                                                *= >.

e e= e e= e e o e e o e e o end Y M e o e e e e e e and auf et0 eu0 eu0 gm0 ed ed ed ed euf and ed one ed M and 8 w t e I e e e. tR me GM e= ga em en Em ad ad 4 I S e. tas 0= 4 4 8 g

                                      .d m

8 4 E 3 0 W u *=e W las a= W en se e.s 3 tas S e e tan a. e e 4 O 3 to a .,d W y  % G am W W S O

                                                                                                                      ==.      #80      40                   e            N          O         se        w       eN e
                                     ==                 N                                                    GA       eft      O G                eme        889          8st        9         W         W tas       889                    O       eft      IA       GA       @        WS                ase      se        est        me           ao N

0- O se e e me see se N N I e e e , 4 4 4 e e a e se e e O e e

                                          =e       e tas       e      WG                tad      O 3 g                      3 3                 e         t#9          t#9        4 e         e         e          e            e e ad E u                           tee      u        N        N        e e == u u e u u a4 >=E                                         tad       taa e

I 132

I I O N M O O O _ O _ O O O O O _ N _ 3 O O O O 3 O O O O O 3 O O m tas tad w tad ted les ned tes nas nee ned tes w tag N e one tes nas tad tea w S M E.e pue e e o . . e e e e e e e taa % W O O O S N m N e =.o e N me e . N

                                                                                                                                                                                                                                 .             .              e      e uN                                   ge      es                                                                                                                                    == .*=                         2              N N ned s=e O                       e          w o                           e               o        e      e        e             o                e                o          e       o        e       e        e p=                                                                                                                                                                                               e              .       e tre      O               e=             a=          e-      >= >=                 e.             e=                e=                  e=               e=

e e o e e e

o. s= o= >= s= ==

e e o e o e o e o e e e e ed $ M & & & & & & & & & & & & & en$ ed and I O N M _ _ _ N O N e O O O O O O O O O O O O O O O O O O ned d and tad est tas and tes nas noe tas nas tad ted IN% ens ans tad tad ned tad

                                                           @        G                                                                                                                                                                                            ens M        in tes aus                e               o       e                e                e       e       e        o             e               o                 e          a        e       e Q            D_                 d              M        O              M            M             M       N w                    N N                             M             M      M o        e             e              e      e   <

M N M M M M  ! E a m I e - O e o e . e

                                           >=                                                                                     o.                           .                 e           .       .        e       e        o             e             e N        O              e=           e=            a=        =      a=~           >=            a=               e=             e=     e=       >= >=           om            >=            e=

e e e e o e o e o e e o e o= N o e o e e e se em0 N ed and =0 ed end and ed ed em0 and muO & ed eu$ ed ens i 3 0 i n e o w w < she I U l"a i

                .=. e                                                                                                                                                                                                                                                t
                >=   @                                                                                                                                                                                                                                                  <
 %s'    C.S 04  tes  -d g       3 e I

s M Ele e e i M m ' I b O 8"o M ==* ==e == a.

                %    e                     O                                                                                  === == == s%e                                               e-o    me       a=      ==      ao             N             N         ==

SR 4 M

                ==

u == 0 O O O O O O O O O O O O O O O O O O i M ,J & e= W nas nne nas taa nas tes les tas saa nas and and ans nas nas tes =s l N N i.e ta a g a w 4 em iO em. M i { M 4=D e e e o e ee e e e o e e 4  % w O O N N M N w N N N w N e e e e o e e H e= O f%s N w =* w w w .e es i

                        $me                  e            M        we                 .              .          .       e I

M e= N amo e= e- e=

                                                                                                                                 .             e              e                e            e       e        .       e       e             e              o        e    I m                                o                                                                       >=,                    en           em                e.             e-     >= >=            e=      om           em             >=        a=

o e e De. e e e e o e g =d a.e M .d as =s =a e e e e e e

                                                                                                             .a                             .4            .d               .4             .a     .a .a            -e      .d            =a            e.d        .a 8

w I  ; m M se

                                      ==

e es in

                                      >            es ums          4 5

ee 4 tad -d 3 em 4 5 O tie 4me om g 18 m. tad == u 9

                           .d        3             ene                                                                                       e e

ed ees e. e 4 O 3 we S e W tup  % O == w S S O

                                                                                                                                            %           M                 99                    w        h       S =* w                              W          e 4A             4A          O e                              sus    fu       M       w w w                               N          N I

tad == 88e h O tA tA tA @ q S a. sus sus a.e as ame me N N

                          >=

4 0 4 as e e e e e e e e e e se o e e amo e e e 4 tad e g O ned O 3 a 3 3 e e e e ** 48 e ed a u nas u N e we to 4 tad ned 4 E pe e e *= u u e u u 35 >= 133  ! l 1

  -          -                  - ..                   ,             - - . - - _ _ , _ . , -                                                       ... . - - . . - - - , . . - . . . , .                                           , . - - . ~ . . . - , - ,

TABLE B-13 (Cont.) BROAD LEAF VECETATION: IODINE-131 AND CAPSIA ISOTOPIC ANALYSES (pCl/kg WE T) STATION NUNSEE BLN-10 i JUNE l OATE C0ttECTES: 06/26 - RABIOCNENICAL ANALVSIS: 1-131 L.I. 1. E 01 GANNA SPECTRUM ANAL YSIS: SE-7 7.20s 0.72E 02 K-40 5.032 0.50E 03 NN-54 L.T. 6. E 00 C s- C0-58 L.T. 6. E 00 FE-59 L.I. 2. E 01 C0-60 L.I. 7. E 00 Zu-65 1. L.I, E 01 28-95/us-95 L.I. 6. E 80

RU-103 7.

L.I. E 00 l RU-106 L.T. 5. E 01 1-131 L.T. 1. E 01 C5-134 6. L.T. E 00 C5-137 1.352 0.50( 01 i i SA-140/LA-140 L.T. S. E 00 4 CE-141 L.T. 1. E 01 ', CE-144 L.I. 4. E O! l ' RA-226 1. i L.f. E 02 TH-228 L.I. l. E 01 i

t l l I i M N M M M M M sue W I O M N M M == N O O O .mo N tee tes W O O O O O O O O O O O O O w w O O

                                                                                                                                                                                                                                                                               .e
                                         .a.s                                  w ned                                         tad      W          Ies             w           tad                             w e                                              #                                                                                                      and        nad                 tes          tad         had        w         ==a INw tea %              N e

8=s e O O N e o N e o e e e e e e e e e o e e e

                                         >= m                                                                                9         N w N N                                        see        M          N         N          N           M            s's ee            ce                                                                                                                                                                     M         M ee O M

tad e= e e e o e e e e e e e e o e e e N s% > e== em > s= ee > e o e o e e o e e e ems to e= e= s= a= e= a= e= e o e o e e

                                                            &                M           $            &          &           &        &

o e o e e s ed & & & & & & & ed & .4 eu6 O M M a=e ==o ==* === me 0 e=o aus N a=e a=e == === === N N O O O O O O O O O O O O O O O O O

                                                                                                                                                                                                                                                                             ==

Q inn ena ina w tad tea w w w w les w a= G @ P i.a ina i.s ted w ina w

                                       @N                                   *e        en'e

(/) 3% e o e e e e M ta G W O O =e N w N e w e N o e o e e e e e e e e m 3O es es N ** w N N N M se #s's M

                   >                                         e              e        M                  e         o           e        o        e          e I

a= o e e e e e e M N ese aim em e= >= a= e e e e o e e o e== a= a= to em em emo e= a= p.o e e e e o e e

                                                          &                 M                                                                                                                                e         o         e           o            e
                                                                                     $              &          &          &         &                                                                                                                               e         e
                                                                                                                                             &         &               &            &         &          &          &         &           &            ad ee                                                                                                                                                                                                                                                 e6         &

E O m O m e 0-0 b I M 94 O ao C a== a o >= z Q go, t.s s 3 e O B M as e O M M se ese sus =e me

   '"I'                 %    B                           C                                                                                            ao             ame           N         amo        me         s=e       ==          ==e          N          N m

lhe

            <t
                        == O u -                              i.e O O i.eO O O O O O O O O O O O O w

O O O em M & t= w 8't i.e i, i.e i.e i., ins ins ins w w ina w ,, w M y ==p 4 == i.s a e- >m . em. N. I e . g M .J % IA 3P O O se se M N w N N se M N N "10's ene M me w M es et e me one e o e e e e o e e e e DE O N b om M em e= sus W e= e e e e e e e o e e M eme >= M PSe ad =* N =a =d ad o

                                                                                                                                  =a e
                                                                                                                                           .d o          e               o           e          e       suo. e=,                e           e emo e          o M

e t -d .d ed .d =# ad =d =# -d .d -a M 5 8 I

  • e ee t#l
                                                   =e t#s 3

en are en wig

                                                                   =#

I ed 4 S ee 4 G S t.s .4 3 em 4 5 O W W > w I les == W 4A me ed E ins e e e

                                        .4        ese             e.                                                                                e                                                                      4 O         3               @                                                                                                                                                        .d W         4.p                                                                                               S                                                                      %
                                                                                                                                                    %M                           q                    w                    O e w w e                         eN e O                                                                                                                                                                                   se e.#

a=

                                                  ==

S a=e M N O w eta eeseee en tA e m en e e me me s=e M M sus see M se == == == N e N N I e e e e 4 4 0 4 e e e e e e's e e e e

  • e*ad* Ea* e t S 5 == EA W taaW
  • N* *N
  • W= ' ** *
  • te. *a* te* * *a=

W *= W W e W W , er 135

M M TABLE B-13 (Cont.) BROAD LEAF VEGETATICW: 10 DINE-131 AND CAMtA ISOTOPIC ANALYSES (pCl/kg WET) stall 0N NUNSER SLK-15 NOVENSER DATE COLLEC1ED: 11/26 BASISCNENICAL ANALV515: l l-131 L.T. 6. E 00 i GANNA SPECTRUN ABALVSI5: SE-7 2.154 0.24E 03 ra K-40 7.41t 0.74E 03 Ne-54 L.T. 2. E 01 CO-58 L.T. 2. E 01 l FE-59 L.T. 5. E 01 C0-60 L . T . ' 2. E O! Zu-65 L.T. 5. E 01 j 2R-95/ut-95 L.T. 2. E 01 AU-103 L.T. 3. E 01 R U- 106 L.I. 2. E 02 I 1-131 L.T. 6. E O! C5-134 L.f. 2. E O! C5-137 5.33t 2.14E 01 BA-140/LA-140 L.T. 3. E 00

    , ,     CE-141                                      L.T.      5. E 01 CE*l44                                      L.T.      2. E u2 NA-226                                      L.I.      6   E Ut lu-??8                                      L.I.      S. I ut

M M i l s TABLE B-14 FOOD /CARDEN CROPS: IODINE-131 AND CA)MA ISO 10PIC ANALYSES (pct /kg met) 3 51 ATION - FPP 50V SEAh5 SEP1 enter SATE COLLECTED: i i 09/17 SANNA SPECTREN ANALVSIS: BE-7 L.T. 1. E 02 1 E-40 9.33 s0.93E 03 mm-54 L.I. 1. E 01

p. C0-58 L.T.

ca 1. E 01

   'd FE-59                                                                                                                   '

L.T. 3. E 01 i C0-60 L.I. 1. E 01 25-65 3. L.T. E 01 ' 28-95/m8-95 L.I. 1. E 01 8U-103 L.I. 1. E 01 ' j RU-106 L.I. 1. E 02 I I-131 2. L.I. E 01 f C5-134 i L.T. 1. E 01 ' i C5-137 , L.I. 1. E 01 SA-140/LA-140 L.I. 1. E 01 CE-141 L.I. 2. E 01 CE-144 i L.I. 9. E 01 RA-226 3. L.T. E 02 TH-228 L.T. 2.

'                                                                                               E 01 i

i i

I APPENDIX C

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION l i i 138

g g M M E E 1 i i TABLE C-1 Samee4AY or talAVAllAaLE SApWLas Asse Missen LOWER LIMITS OF DETSCTI(NI B55841C lut PERIOD OF JAleutRY I 10 setaCE 31. 1945 Se89 LE I S IA dEALYSIE tac & TIS EERJIt4 TIS er 5489LE M hvatteSELITT RATE

  • M Istage IJa
1. Atmospheric Groes Sete APC-1 01/22/85-41/28/05 se sample ovellebte. particulate filter use teet duries collecties by strees wiede blantes filter este ground.
2. Driektes/ Surface I-131 BME-5/ 01/97/45-41/12/05 Unter 315- 5 se sample eve 11able, due to sampler malfuncties.
3. Drienties/ surface I-131 en-5/ 43/93/05-43/15/05 as sample eve 11eble, due to sampler amtfuncties.

unter sME-5

4. Drieking/Serface Game EME-5/

tinter Jammary 25-5 Lim est met for Be-144/14-140 due to delayed Campeette emetyste resulttog from missed samyte.

5. Italk 1-131. Comme 15 5-4 Jammary me samples evettable, goeta est lectetteg.
6. Nilk 1-131. Game IEE-4 February No emples evellebte goats not lectaties.
7. Breed Emot vegetettee I-131. Samma M4-1 Jemmary He sample ovellable due to freeee.
4. Breed Leef vegatetten I-131. Came 383-1 Jemmary me sampletevettable due to freeee.
9. Sreed Leaf vegetectee I-131. Samma Sta-10  % Re sample ovellable due to freene.
10. Breed Leaf vegesetten 1-131. Comme sta-10 Pobruary no sample cellected elece milk eamplee were ovellable et centrol necettee.
11. Broad Emot vegotetten 1-131. Came sta-14 teerch me sample collected stece milk semyles were ovellable et control 1ecettee.
    -_____-- - _- __ --                   __a -_------ _ _ _ _ _ - - _ _ _ _ - _ - -                                            - - - -         -- ._   _ _ _ _ _ _ _ -                 _ _ -                           _ _ _ _ _ _ _ _ _ _ . _ _ _ . _ _

I l i i  % TABLE C-2 i SUlsARY OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF ' t i APRIL 1 to J1BIE 30. 1985 i ) , SeeWLR M IA AAALYSIS 1aC& TIS MW NTim er Atena WavallASILITT M M8EM EA8 ) 1. At @ ric Grose Sete l AN-1 M /01/85-M /99/SS se sample ovellable. particolate filter une teet j dortag semple cettection by otrong wiede blowing filter emey.

2. Ae + ric Groes mete. 1-131 AK-1 M/30/85-GS/M/05 se semple ovellable due to pump fettere.
3. Atmospheric 1-131 AFC-1 DS/M/85-GS/GS/85 tAa set met due to law samyte solume. Sample peep faued est running.

4 Atmospheric Groes Bete. 1-131 7 AFC-1 05/08/05-45/28/05 ne semyle eve 11eblo due to peser fattere et I etettee. , S. Ateespberie 1-131 AfG-1 46/24/05-06/27/05 Ea3 est met due to law eseple volemme, ample remy femme met rumstag. } 6 Nath 1-131. Gemme M S-4 i Apell Be semples ovellableg geste met tactatteg.

7. Wilk 1-131. Gamme ms-4 95/30/85

< De semple ovellable from emner. S. Milk 1-131. Gamme MS-4 June !' se semples evettable from aumer. i 9. Breed Leaf vegetation 1-131. Gemme Sta-18 Aprit l no semple collected elece milk semples were ovettable et centrel lacettee.

13. Breed Leaf vegetetten 1-131. Gemme 313-10 nmy 4

no sample collected state etik samples were i postlebte et centrol lecettee. l I I I l i l 1

1 l **

TABLE C-1 i

Sl99tARY OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS

!                                                       OF DETECTION DURING THE PERIOD OF JULY 1 to SEPTEMBER 30. 1985 SAMLE IMIA                                                                                                                                                             stPIAnarles er atWla untava11AalLITT AEALTSIS                                                           1AC& TIS                                          R&Ts                                                         e enemma gas i

l 1. Atmosyberic 1-131 AFC-1 SF/01/05-47/93/85 118 could est be met. Resefficient semple vot es cellected. l 2. Atmospheric 1-131 APG-1 07/91/85-47/s2/05

'                                                                                                                                                                                     123 could met be met. Inomfficient semple 1

weline collected.

3. Nilk 1-131. Gemme 355-4 July as emples eve 11eble from aumer.
4. Nilk 1-131. Geene 155-4 August se semples evettable freus emner.
5. Milk 1-131. Samme 15 5-4 September se semples eve 11eble from aumer.

i

     ~

! fa, , s .* !l I i l 1 1 j .- I i i

   ,                        _    _        _ - . . - - . - - . _ . - . - - . _ - . - . - - - _ - - - - . _ - - . _ _ _ - . _ . . - - . , - . . . ,                               _ . .      -___..__.-....___-.-_.___m                  _ _ _ _ _ - _ . -_ . _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ -

g g M M M i TABLE C-4 l SINGIARY OF UNAVAILABLE SAMPLES AND MISSED IhWER LIMITS OF DETECTION DURING THE PERIOD OF OCTOBER 1 to DECEMBER 31, 1985 8488LE M BA AAALYSIS laE1 TIM EEPMAAften er 843555 W hvalLASILITT BAM e stages las i, 1. Atmospheric Green Bete. 1-131 A59-1 14/30/05-11/04/85 No sample evettables pump betes repetred.

2. Atmospheric crese Bete. 1-131

' Arc-1 11/11/05-11/18/05 ue sample evettable due to ymp malfuncties.

3. Atasophoric Grece Bete. 1-131 AfC-1 11/18/85-11/25/85 us sample ovellahte. Feuer to esmple peep wee diec-ted due to work at discharge etetten.
4. Atmospherie 1-131 APS-30 12/92/85-12/99/85 las could est be met due to imenfficient samyte volesme. Pump found not reates.
5. Milk 1-131. Comme M S-4 October No sample eve 11eble free aumer.
;        6. Milk            1-131. Comme             15 5.-4            Bevember           Es semple ovellebte fame aumer.

r" 7. Milk

!                            3-131. Comme             IEE-4 1

December no sample sea 11able free eumor.

8. Milk 1-131. Game 354-54 10/91/95 se sample collected by state due to amargency Flamelag Emercise.
9. Wegetatise 1-131. C m 5 5-10 10/30/05 no esmyle'esellable due to fleedies fran Surriemme Jues.
13. Veestation g.131. Comme 385-15 12/31/85 Re esmple ereitable due to lack of essetecten, i

I

I TABLE C-5 SU W ARY OF UNAVAILABLE TLD IGASUREMENTS DURING THE PERIOD OF JANUARY 1 70 DECEMBER 31, 1985

I 1

LOCATION QUARTER EEFLAMATION C-1 First TLD stolen: Replaced 3/1/85 D-5 First TLD stolen E-1 First TLD stolen: Replaced 3/1/85 E-30 First TLD stolen: Replaced 3/8/85 I J-2 First TLD results affected by radiography in area; TLD results not included in Data Evaluation. N-1 First TLD stolen A-5 Second TLD stolen: Replaced 5/3/85 I D-5 G-4 Second Second TLD stolen TLD stolen Replaced 5/3/85 N-1 Second TLD stolen: Replaced 6/8/86 F-1 Second TLD stolen: Replaced 5/1/85 l C-1 Fourth TLD stolen D-2 Fourth TLD stolen H-2 Fourth TLD stolen N-1 Fourth TLD stolen I l 143

I I  ; I I I . I APPENDIX D

SUMMARY

OF INTERLABORATORY COMPARISONS i i I 3 . g l I 144 I

M M M M M ' W TABLE D-1 US EPA CROSS-CHECK PROGRAM 1985 trA pate si nailes caLe trA PREPARAil04 trA Il Nore Dev. == Warning Results Issued Results Media nuclide Results(8) Results(h) (Known)(d) *** Action 01/04 02/01/85 04/04/85 Water Sr-89 3.0 1 8.7 L.T. 3. -- Sr-90 30. 1 2.6 29.0 1 12. -0.8 01/11 02/15/85 03/15/85 Water Pu-239 15.7 a 2.8 19. t 3. 3.6 ***(a) 01/18 02/15/85 03/15/85 Water Gross Alpha 5.0 t 8.7 5. t O. 0. 0 Gross Seta 15.0 t 8.7 15.0 t 3. 0.1 01/25 03/08/85 04/15/85 Food Sr-89 34.0 t 8.7 17.0 t O. (c) Sr-90 26.0 1 2.6 22.0 t 6.

                                                                                                                                                          -5.89      ***(e) a.,

1-131 35.0 t 10.4 26.3 2 6.2

                                                                                                                                                          -4.62      ***(e)
                                                                                                                                                          -2.50 Cs-137          29.0 t     8.7       31.0            t 10.4                                 0.69 K             1382.0 2207.9       1393.0 2 96.4                                             0.16 02/02        03/12/85         04/08/85       Water       H-3           3796. 1634.      3933.                  1174.                             0.6

) "" 02/08 03/11/85 04/08/85 Water Cr-51 48. 8.7 L.T.

  $                                                             Co-60           20.

t t 8.7 19.0 t 6.

57. --

2n-65 -0.6

55. t 8.7 57. t 6. 0.7 j

Ru-106 25. t 8.7 L.T. 40. -- ' Cs-134 35. t 8.7 37.0 t 12. CS-137 0.8

25. t 8.7 31.0 a 6. 2.0 02/22 04/04/85 04/15/85 Water Ur an ius 12.0 t 10.4 12.0 t 3. 0.3 03/01 03/20/85 06/10/85 Milk I-131 9. 1.6 t 8.0 a 3. -1.9 03/15 05/09/85 06/07/85 Water Ra-226 1.3 5.0 t 5.9 a 2.1 2.0 **

Ra-228 9.0 2 2.3 5.1 2 1.8 -5.0 ***(f) 4 03/29 05/13/85 07/02/85' Air Filter Gross Alpha 10.0 2 8.7 1 10.33 2 1.7 0.11 Gross Seta 36.0 t 8.7 36.66 t 7.5 0.23 Sr-90 15.0 2 2.6 14.66 1 1.7 Cs-137 -0.38 6.0 t 8.7 6.0 2 0.0 0.00 04/05 ,. 04/23/85 06/10/85 Water I-131 7.5 t 1.4 6.67 a 1.7 -1.80 04/12 05/09/85 06/10/85 Water H-3 3559. 1630 3367. 1963. -0.9

E E E .mme E TABLE D-1 US EPA CROSS-CHECK PROGRAM 1985 EPA Date il 88atted Sate EPA [PA it here Dev. ** Warning PREPARATION Results issued Results Media Nuclide Results(a) Results{b) (Kacwa )( d) *** Action 04/19 04/28/85 08/15/85 Water Gross Alpha t 8.7 25.33 2 1.7 (Sample A) Ra-226 32.0 -2.31 ** 4.1 1 1.0 3.66 2 0.9 -1.25 Ra-228 6.2 1 1.6 6.13 2 0.7 .12 U 7.0 t 10.4 6.67 2 1.7 -0.10 1 04/19 e6/28/85 08/15/85 Water Gross Seta 72.0 t 8.7 92.33 2 (Sample 8) 9.6 7.04 ***(9) Sr-89 10.0 t 8.7 10.0 t 0.0 0.00 Sr-90 15.0 1 2.6 13.33 4 3.5 -1.92 Co-60 15.0 2 8.7 20.0 a 5.2 1.73 Cs-134 15.0 t 8.7 14.66 2 3.5 -0.!! Cs-137 12.0 t 8.7 16.33 1 9.6 1.50 04/26 05/13/85 06/13/85 Urlae H-3 3056. 1622. 2833. 2345. -1.1 05/10 07/05/85 08/05/85 Water Sr-89 39.0 t 8.7 35.66

  • Sr-90 9.2 -1.15 15.0 2 2.6 12.66 a 1.7 -2.69 **

05/24 06/18/85 08/09/85 Water Gross Alpha 12.0 t 8.7 12.00 t 5.2 0.00 Gross Seta 11.0 t 8.7 12.66 2 1.7 0.58 i 06/07 07/15/85 08/12/85 Water Cr-51 44.0 2 8.7 L.T. 53.3 -- Co-60 14.0 t 8.7 15.66 t 3.5 0.58 2n-65 47.0 1 8.7 48.33

  • 7.5 0.46 Ru-106 62.0 t 8.7 53.67 a 9.6 -2.83 e.

Cs-134 35.0 t 8.7 33.0 2 13.1 -0.69 Cs-137 20.0 1 8.7 23.33 2 6.2 1.15 j 06/14 07/12/85 04/06/85 Water H-3 2416.0 2608.0 2366.66 2346.4 -0.24 06/21 08/16/85 09/19/85 Water Ra-226 3.1 2 3.86 2 Ra-228 0.7 0.18 2.82 ** 4.2 2 1.0 3.66 2 2.0 -1.46 4 ' 06/28 09/06/85 10/10/85 Milk $r-89 11.00 t 8.7 11.66 a 3.5 0.23

                                                               $r-90           11.00 1     2.6    10.00 1    0.0    -1.15 l-131          11.00 a 10.4        9.00 2    3.0    -0.5u i

C5-137  !!.00 2 8.7 11.00 t 7.9 0.00 K 1525.0 2131.6 1540.0 s!03.9 0.34 l

g g g g g g E E E E E E E TABLE D-1 US EPA CROSS-CHECK PROGRAM 1985 EPA Date TI Malled '0* ate EPA PREPARATION Results EPA TI Issued Results Media Nora Dev. ** Warning Nuclide Results(a) Results(b) (Known)(d) *** Action 07/05 07/30/85 08/19/85 Urine H-3 2444.0 2610.0 2066.66 1624.5 -1.85 07/13 09/06/85 09/30/85 Water Pu-239 10.6 2 1.9 8.20 2 2.2 -3.78 ***(h) 07/19 08/16/85 09/19/85 Water Gross Alpha 11.0 t 8.7 5.67 a 1.7 -1.84 scoss Seta 4.0 t 8.7 4.33 a 1.7 -1.27 07/26 10/04/85 12/09/85 food Sr-89 33.0 t 8.7 25.33 a 6.2 <2.65 ** (c) Sr-90 26.0 t 2.6 28.33 2 4.6 2.69 ** l-131 35.0 t 10.4 37.33 a 4.6 0.67 Cs-137 29.0 t 8.7 31.00 2 3.0 1 0.69 1514.0 2131.6 1633.33 4154.0 2.72 ** 08/09 09/19/85 10/10/85 Water 1-131 33.0 a 10.4 36.66 2 4.6 1.05 08/16 09/13/85 10/07/85 Water N-3 4480.0 1776.0 4433.3 3458.3 -0.18 3 l 08/23 09/19/85 11/34/85 Water U 4.0 t 10.4 4.33 a 1.7 0.10 08/30 10/30/85 12/30/85 Air Filter Gross Alpha 13.0 2 8.7 12.66 t 1.7 -0.!! Gross Seta 44.0 2 8.7 43.00 1 9.0 Sr-90 -0.34 18.0 t 2.6 20.00 2 3.0 2.31 ** Cs-137 8.0.2 8.7 10.00 2 3.0 0.69 09/06 10/10/85 12/24/85 Water Sr-89 20.0 t 8.7 18.33 a 4.6 -0.58 3r-90 7.0

  • 2.6 6.00 2 0.00 -1.15 09/13 11/06/85 12/16/85 Water Ra-226 8.9 2 2.3 9.23 1 1.5 0.43 Ra-228 4.6 1 1.2 4.03 2 0.6 -1.42 09/20 10/07/85 12/16/85 Water Gross Alpha 8.0 t 8.7 3.33 1 1.7 -1.61 Gross Seta 8.0 2 8.7 4.00 t 0.00 -1.38 10/04 11/14/85 01/08/86 Water Cr-51 21.001 8.7 L.T. 63. --

Co-60 20.00t 8.7 17.66 1 2n-65 9.6 -0.81 19.00t 8.7 25.33

  • 7.5 2.19 **

Ru-106 20.002 8.7 L.T. 37. -- Cs-134 20.002 8. 7 18.33 1 9.2 Cs-137 -0.58 20.00 8.7 22.33 a 3.5 0.81 10/11 11/05/85 12/24/85 Water- H-3 1974.0 1598.  ?!33.33 1624.5 0.8u

I TABLE D-1 I US EPA CROSS-CHECK PROGRAM 1985 Collectica Teledyne Date Media Nuclide EPA-Results(a) Isotopes Results(b) NOTES: (a) EPA %!sults-Expected laboratory precision (3 sigma). Units are pCi/A for water, urine, and milk except K is in og/A. Units are total pCi for air particulate filters. I (b) Teledyne Results - Average t three sigma. urine, and milk except K is in og/A. particulate filters. Units are pC1/A for water, Units are total pCi for air (c) Units for food analysis are pC1/kg. I (d) The history of this analysis indicates no problem with the chenistry. The high result is possibly technician related and sources of error have been discussed with the technician. I (e) The results from the EPA were received on August 09, 1985 for the analysis completed in April. The EPA had difficulty determining the correct results for this sample. It was difficult to scavenge and the  ; results were reported as a courtesy although they were considered ) suspect because of the difficulty of analyzing a synthetic food sampie. (f) A new chemistry wgs tried but did not give good results. A further refinement of the chemistry is planned. (g) The proportional counters are calibrated for beta efficiency with Cs.137. The efficiency correction applied for the low energy beta 'l emitters overcompensated because the amount of the low energy emitters I was small compared with the high energy emitters. (h) A new Pu-239 standard solution was prepared and a new Pu disc was ordered from NBS to check the efficiency calibration of the counters. I , 148

m m m m m W W M M M M M M i l *. l i TABLE D-2 5598575 191E*aATIODAL INTBBCONFABISON OF EMTIRONMENTAL DOSIMBTER RESULTS SEITERS M700W58 (aB) ALL PARTICIPANTS REMETS (air) (a) LPM.'S RESIETS (eA) (b) Estimate emeertainty tenea 2 (c) 2 SS Ng Espequee Gacertalate 2 Error (e) m (f) Laboraterr Eaeseuree Free Coetuse-137 (g) 75.0 3.8 73.0 11.1 13.2 185 75.0 12.0 0.0 0.20 Free Cabelt-40 (b) 73.9 4.0 77.3 13.3 17.7 184 64.0 7.3 13.3 1.0 Field

  • _ _ m (b) 75.8 s.e 73.1 14.9 19.s 144 70.0 a.g 7.6 -0.3 e

ie

e '

l (c) Results of all participante in the Intercomparison Study. (b) Results beoed os using Feassonic UD-814 AQ T1.Ds. (c) SD stands for Standard Deviation. (d) N stande for Number of results. (s) I Error le a asseure of how much LF6L's reeutta differed from the estimated delivered esposures I Error = (LP&L's Exposure - Delivered Esposure) x 10_0 Delivered Esposure (f) MD stande for "Isormalised Deviation". It le a measure of hose many standard deviations LF&L results were from all participants' results. Im = All participants' Boemite esas - LP6L Exposure All Participants' SD (g) Results of all doetmeter types for all participants' results. (::) Raoults of all doelmeter types for all participants' results with one outliner excluded. I l 1 i

i I

I I

I I I ' APPENDIX E I SYNOPSES OF ANALYITICAL PROCEDURES I

I  ;

i

I il l

1 f

    ,                                                                                        150 lI

I E-1.0 ANALYSIS OF SAMPLES FOR GROSS BETA ACTIVITY E-1.1 Air Particulates After a delay of three or more days, allowing for the I radon-222 a.ad radon-220 daughter products to decay, the particulats filters were counted in a gas-flow proportional Counter. I E-1.1 Water I A known volume (usually one liter) of water is evaporated to near dryness, transferred to a two inch diameter ringed planchet, and then evaporated to dryness. The planchet was then counted for 50 minutes in an automatici alpha-beta l counter. I E-2.0 ANALYSIS OF WATER SAMPLES FOR TRITIUM One milliliter of water was added to 20 milliliters of liquid scintillation solution in a 25 milliliter vial. The sample was then counted for 100 minutes in a liquid scintillation counter. E-3.0 ANALYSIS OF SAMPLES FOR IODINE-131 E-3.1 Milk and Watgx Two liters of sample were first eqcilibrated with stable iodide carrier. A batch treatment with anion exchange resin was u. sed.to remove . iodine from the sample. The iodine was then stripped from the resin with soda.ca hypochlorite l3 solution, reduced with hydroxylamine hydrochloride, and then g " extracted into carbon tetrachloride as free iodine. It was then tack-extracted as iodide into sodium bisulfite solution and precipitated as palladium iodide. The precipitate was ll weighed for chemical yield and mounted on a nylon planchet for low level beta counting. The chemical yield was i corrected by measuring the stable iodide content 4of the milk < or the water with a specific ion electrode. 1 I

I E-3.2' Broad Leaf Vecetation I Stable iodide carrier was first added to a measured weight of chopped sample. The sample was then leached with sodium hydroxide solution, evaporated to dryness, and fused in a muffle furnace. The aclt was dissolved in water, filtered, and treated with sodium hypochlorite. The iodine was then reduced with hydroxylamine hydrochloride and extracted into chloroform. It was then back-extracted as iodide into I sodium bisulfite solution and precipitated as palladium iodide. The precipitate was weighed for chemical yield and mounted on a nylon planchet for low level beta counting. The chemical yield was corrected for the natural, stable iodide content of the sample by use of a specific ion electrode or, a separate aliquot (without carrier added) of the sample. E-4.0 GAMMA SPECTROSCOPY ANALYSIS E-4.1 Milk and Water I A one liter Marinelli beaker was filled with a representa-tive aliquot of the sample. The sample was then counted for 1000 minutes with a shielded Ge(Li) detector coupled to a 3 mini-computer-based data acquisition system which performed

'g                                       pulse height analysis.

I E-4.2 Vecetation. Food and Garden Crocs, and Fish ' As much as possible (without drying) of a vegetation, food, or garden crop sample was loaded into a tared one liter Marinelli beaker and weighed. The sample was then counted i for 1000 minutes with a shielded Ge(Li) detector coupled to -I a mini-computer-based data acquisition system which per-formed pulse height analysis. I As much as possible (up to the total sample) of the edible portion of a fish was loaded into a tared Marinelli beaker and weighed. 1 The sample was then counted for 1000 minutes < with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performed pulse height analysis.

   .                                                                 152 I

'I I E-4.3 Soils and Sediment I Soils and sediments were dried at low temperatures, less than 100 degrees Centigrade. The soil or sediment was loaded into a tared, standard 300 ml container and weighed. I The sampic was then counted for at least six hours with a sh.ielded Ga(L1) detector coupled to a mini-computer-based data acquisition system which performed pulse height analy-l ais. I E-4.4 Charcoal Cartrideas (Air Iodine) Charcoal cartridges. ware counted up.to five at a time, with ) one positioned on the face of a Ge(Li) detector and up to I four on the side of the Ge(Li) detector. detector was calibrated for both positions. Each Ge(L1) The detection l limit for iodine-131 of each charcoal cartridge was deter-  ; mined (assuming no positive iodine-131) uniquely from the volume of air which passed through it. In the event l l iodine-131 was observed in the initial counting of a set, I I each charcoal cartridge was then counted separately, positioned on the face of the detector. I E-4.5 Air Particulates I The weekly air particulate filters for a quarterly composite from each field station were aligned one in front of another and then counted for at least six hours with a shielded Ge(Li) detector coupled to a mini-computer-based data I acquisition system which performed pulse height analysis. I E-4.6 fonnuter Software

   ' A mini-computer software program defined peaks by certain changes in the slope of the spectrum. The program also compared the energy of each peak with a library of peaks f6r

'I isotope identification and then performed the radioactivity cticulation using the appropriate fractional gamma ray abundance, half life, detector efficiency, and not counts in the peak region. 1 l I 1

I I E-5.0 ENVIRONMENTAL DOSIMETRY g Thermoluminescent Dosimeters (TLDs) manufactured by Panasonic 3 (model UD-814AQ) were used for environmental dosimetry. The Panasonic TLDs contained elements. one lithium borate and three calcium I sulfate phosphor However, only the calcium sulfate phosphor elements were used. An annealed dosimeter was placed inside a plastic bag and mounted in an aluminum frame prior to placement in the field. The dosimeters were exchanged every I quarter. The exposures of the collected dosimeters were read using an automatic TLD reader manufactured by Panasonic (Model UD-710). I I l I l I I lI . I I lI I I

   ,_a   _ _ _ ,     a - - - - - - - s -a -.a- -  -

I i I I , l I  ! I APPENDIX F STATISTICAL ANALYSES I l I  ! i r

                                                                          +

I I . I I I . I

I ,l F-1.0 CALCUIATION OF MEAN AND STANDARD DEVIATION The mean and standard deviation for different groups of analyses were calculated using the following equations:

                           * "      "x           *i (F-1)                    E i-1           nx I         (F-2)
                                /

f ax I xt2- (n )x (R)2 i=1 0.5 k (nx - 1) ) I where: I Tc s n,

                             = mean of sample population,
                             = standard deviation of sample population,
                             = number of samples in sample population, and x1     = value of the ith sample.

F-2.0 COMPARING TWO SAMPLE POPUIATION MEANS The means of two sample populations can be compared for a statisical difference using the standard "t" test. The use of I the test requires the assumption that the data within the populations are normally distributed and that the true standard deviations of the mean are equal for both populations. The I standard "t" test tests the hypothesis that the true means of both populations are equal. The "t" value can be calculated from the equation below (obtained from the CRC Standard Mathematical Tables, 26th Edition (1981))* I

                                                   ~

(F-3) t= 1 I f(nx- o.,2 + cn,- n.,2 ) f 1 1 f < ^ R x + Dy -2 f (nx "y I 13e

where: t = calculated "t" value, I Tc = mean of first data set, y = mean of second data set, nx = number of variables in first data set, sx = standard deviation of first data set, I = number of variables in second data set, and

                             = standard deviation of second data set.

If the data from both sample populations are treated as cor-related pairs, the difference between individual measurements can I be examined using the statistical "t" test. the true means and true standard deviations for the sample In this case, if populations are equal, the difference between the correlated data points should be normally distributed about a mean of zero. The I "t" value can then be calculated from the following equation (obtained from the CRC Standard Mathematical Tables, 26th Edition (1981)): I (F-4) C = I (n) where: I E= the average of the difference between the cor-related data points from the two sample popula-tions: I d = N E i=1 (xi-yi)/N x= the ith data point from population x, I t yt= N= the ith data point from population y, the number of correlated pairs of data points, and a= d the standard deviation of the difference between the correlated data points. . The calculated "t" value in both cases is used to test the I hypothesis that the true mean of the first population (u x) is equal to the true mean of the second population (uv) assuming that the true standard deviations of both populatibns are equal (or"Oy) . The calculated I value such that "t" value is compared to a tabular "t" a. if t>t ,n then reject the hypothesis when u x>uy, ,I b. i if t<-t ,na then reject the hypothesis when u x<uy, c. if ltl> tan,n then reject the hypothesis when u xyfuy, 157 'I ~ _ . _ . _.

I I where t a/2 n and to,n are the tabular "t" values, with a pre-l selected eferor (5 percent in this case), confidence level (1 a) ! or (1 a/2), and degrees of freedon n (n=n x+ny-2 and n=N-1 for Equations F-3 and F-4, respectively). Tabular values of "t" were i obtained from the CRC Standard Mathematical Tableg, 26th Edition l (1981). F-3.0 TLD MEASUREMENTS The TLD measurements made during 1985 were grouped into cate-gories based on distance from the plant. The means and standard I deviations obtained for each category are given in Table F-1. The mean dose from the stations located more than five miles away from the plant were compared to the mean dose from stations I located within two miles from the plant and to the mean dose from stations located between two and five miles from the plant using the standard "t" test. The "t" values were calculated using Equation F-3 and are given in Table F-1. I Comparing the calcula-ted and tabular "t" values show that the mean dose for stations within two miles from the plant is statistically lower than the mean dose from stations located grsater than five miles from the I plant. The mean dose for stations located between two and five miles from the plant is statistically the same as the mean dose for stations located more than five miles from the plant. I F-4.0 GROSS BETA ACTIVITY ON AIR PARTICUIATE FILTERS The means and standard deviations for airborne gross beta results I obtained during 1985 from the control and indicator stations are given in Table F-2. The mean from each indicator station was compared to the mean from the control station using the standard "t" test to determine if there was a statistical difference. I calculated (using Equation F-3) and tabular "t" values for each indicator / control station comparison are given in Table F-2. The comparing the calculated and tabular values indicate that there is no statistical difference between the means from each indicator location and the mean from the control location. F-5.0 GROSS BETA ACTIVITY IN MONTHLY DRINKING WATER COMPOSITES The means and standard deviations for gross beta activity detected in the monthly drinking water composites obtained during 1985 from the control and indicator stations are given in Table F-3. The mean from each indicator station was ccapared to the mean from the control station using the standard "t" test to determine if there was a statistical difference. The calculated 158

I (using Equation F-3) and tabular "t" values for each indicator / control station comparison are given in Table F-3. Comparing I the calculated and tabular values indicate that there is no statistical difference between indicator station DWE-5 and control station DWP-7 means. However, there is a statistical I difference between the means from indicator station DWG-2 and control station DWP-7. In order to determine if this difference resulted from the I operation of Waterford 3 SES, data obtained in 1985 were compared to data obtained in 1984. Monthly gross beta activity data from each indicator and control location were treated as correlated I pairs. The differences between monthly measurements obtained from each indicator and control station samples were calculated and averaged for 1984 and 1985. The results of these calcula-tions are presented in Table F-4. I The "t" values for each indicator / control station difference were calculated using Equation F-4 and are given in Table F-4. Comparing the calcula-tad "t" values to the tabular "t" values show that the means for I data from station DWC-2 were statistically larger than the means from control station DNP-7 during both 1984 and 1985. The means for data from indicator location DWE-5 and control station DWP-7 were statistically the same during 1984 and 1985. As further comparison, the average of the indicator / control station differences obtained during 1984 and 1985 were compared I to each other using the standard "t" test. The "t" values were calculated using Equation F-3. The calculated and tabular "t" values are presented in Table F-4. Comparing these values I indicate that there was no statistical difference between the results observed during 1984 prior to Waterford 3 SES initial criticality and the results obtained during 1985. Thus the I difference between indicator station DWG-2 and control station DWP-7 gross beta results were deemed to be unrelated to Waterford 3 SES operation. I I I I lI , 159

m M M M M 4 m W W M M M M M M M M TABLE F-1 STATISTICAL COMPARIS0010F 1LD MEASURDtENTS FROM STATICIBS CROUPED BT DISTANCE FRGt WATERFORD 3 SES 0-2 Miles Stations located 2-5 Stations Located from the Flaat Miles from the Flaat more than 5 Miles from the Plant Mean (aren/std. ger.) 16 17 18 Standard Deviation (ares /std. gtr.) 1.6 3.0 3.4 5 o thenber la Sample 58 26 32 Calculated "t" Value to Camparisons with Statione Iacated more then 5 miles from the plant -3.794 -1.153 NA Tabular "t" Value at 951 Confe h e o.025.aI (t * * *

a. Used value for 8 0.025.n, ameults indicate that the mean for station located 0-2 miles from the plant to statistically lower than statimaa located more thaa 5 miles from the plaat.

HA Means not applicable .i e

I . N

                                      ,      =      ,         n i

l l 1 9 N $ I a o . 4 k e . :4 , , = , , I 2 2 o a * - 9 T 4 I .

                 ~

N d 5 H O g N O I 4 . c I. g g a a  : (

                                                             ~

lI I - ya e=1 y

                      -      a 2
a n E

8 I .  !.! aa4 a 4.3 .  ! 4- 1 s-I . 3 3 2* _ 3 s 1 la . . .18 1

                            ?            'S
                                          ~

2 R uo a  ? 2

                             ~

5 Ano . E d II I

                                                          ~

l 161

M 4 W M M M M M M M TASLE F-3 STATISTICAL CobrARISON OF CROSS SETA ACTIVITY IN NOIMILT DEIIEING MATER C009081758 POR 1985 ST& TION EWC-2 DWE-5 4 Dur-7 Sleas (yC1/1) 7.9 5.0 5.7 i i - Standard noviettom

         $                 (yC1/1)                                 1.7                             1.0                              1.2 Ilueber in Sample                             12                              12                               12 Calculated "t" Value Comparing Control Station                       3.506                        -1.486 (Ete-7) to Indicator Station                                                                                        ish Tabular "t" Value at
951 Confidence 2.074 (a) 2.074 mA "0.025.eI i
a. Results from station DWG-2 are statistically larSer than results from station DWP-7 NA Means not applicable 1

E E E E E E E E TABLE F-4 STATISTICAL CO W ARISON OF CROSS BETA ACTIVITT IN NOImILY DRIM ING M TER CCW OSITES FOR 1984 and 1985 Difference of Monthly Resulte Difference of Monthly Results from Statione DMG-2 and DWP-7 from statione DUE-5 and Bur-7 for 1984 for 1985 for 1964 for 1985 Mesa l (pC1/1) 1.9 2.3 -0.1 0.7 l Standard Deviation (pci/1) 1.5 1.8 1.7 1.9 5 w Number in semple 12 12 12 12 i Calculated "t" Value Comparing i Control / Indicator Station Difference 4.388 4.426 -0.204 1.276 Tabular "t" Value Campering Coatrol/ Indicator Station Difference 2.201 2.201 2.201 2.201 at 95I Confidence (t0.025.a) i calculated "t" Value

comparing 1964 amoulte -0.566 MA -1.041 NA to 1945 Beaults Tabular "t" Value Comparing -

l 1984 ameults to 1985 amoulta 2.074 at 952 Confidence MA 2.074 NA i (t0.025.a) i NA MeaAs not applicable i i, 4

p. O. Box e0340 LO U I &SLIGHT POWER IAN A /NEW 317 eAnoNNE ORLEANS, LOUISlANASTaeEr 70160 *

(504)595-3100 NUSNIYS EM April 30, 1986 W3P86-0078 A4.05 QA Mr. Robert D. Martin Regional Administrator, Region IV 1 gg%%- U.S. Nuclear Regulatory Commission ) 611 Ryan Plaza Drive, Suite 1000 Arlington, TX'76011 g , l @ ;l

                                                                         *     ~

Subject:

Waterford 3 SES -- Docket No. 50-382 ,, License No. NPF-38 , Radiological Environmental Monitoring Report

Dear Mr. Martin:

Enclosed is the subject 1985 annual report on radiological environmental monitoring which covers the period of January 1 through December 31, 1985. This report is submitted per Section 6.9.1.7 in the Waterford 3 Technical Specifications (NUREG-lll7) of Appendix A to Facility Operating License No. NPF-38. V ly yours, K.W. Cook Nuclear Support & Licensing Manager KWC:GEW:ssf l Enclosure cc (w/ enclosure): NRC, Director, Office of I&E ) NRC, Document Control Desk, Washington, D.C. l l cc (w/o enclosure): G.W. Knighton, NRC-NRR J.H. Wilson, NRC-NRR NRC Resident Inspectors Office B.W. Churchill W.M. Stevenson ' I I

                                                                                                              /     l y}9 g-439                      -. mu.to ,oorunnry... tov .-

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