ML20244D843

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Forwards Request for Addl Info Re 860127 Guidelines for Permanent BWR Water Chemistry Installations & 851001 Rev 1 to Air Products Liquid Hydrogen Storage Sys Hazardous Consequence Analysis. Response Requested by 860630
ML20244D843
Person / Time
Issue date: 05/08/1986
From: Hulman L
Office of Nuclear Reactor Regulation
To: Neils G
BWR OWNERS GROUP
Shared Package
ML20244D847 List:
References
FOIA-88-198 NUDOCS 8605150229
Download: ML20244D843 (32)
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DISTRIBUTION CENTRAL FILE W 0 8 1986 PSB R/F F. Witt J. Kudrick G. Lainas Mr. G. H. Neils Chairman, Regulatory Advisory Committee BWR Owners Group II for Intergranular Stress Corrosion Cracking Research 414 Nicollet Hall Minneapolis, Minnesota 55401

Dear Mr. Neils:

SUBJECT:

GUIDELINES FOR PERMANENT BWR HYDRonFN WATER CHEMISTRY INSTALLATIONS - REQUEST FOR ADDITIONAL INFORMATION We have received the_" Guidelines for Permanent BWR Hydrogen Water Chemistry Installations" transmitted by your letter dated January 27, 1986. In addition, our review included consideration of Revision 1 of " Air Products Liquid Hydrogen Storage System Hazardous Consequence Analysis" dated October 1, 1985.

To complete our revieg we need the enclosed additional information. We request your response.by May 30, 1986 in order to meet a review completion date of June 30, 1986.

Any questions regarding this request may be addressed to Mr. Frank Witt (301-492-9440).

icia;. ::Ig.ud by:

2.. C. B1::en L. G. Hulman, Chief Plants Systems Branch Division of BWR Licensing

Enclosure:

As stated cc w/ enclosure:

L. Steinert (EPRI) bec w/ enclosure:

R. W. Houston B. D. Liaw S. Kim J. Zwolinski W. Hodges K. Campe W. Butler J. Lee C. Ferrell D. Muller M. Lamastra T. Thomas E. Adensam J. Levine D. Notley "See Previous Concurrence / Document Name on 5520: GUIDELINES BWR HYDRG WATER OFC : DBL: PSB*  : DBL:PSB*  : DBL: PSB*  : A BWR: DBL :  :  :

NAME : FWitt:ye  : JKudrick : LGHulman : Gl, rims  :  :  :

DATE : 5/6/86  : 5/6/86  : 5/6/86  : 5/D /86 :  :  :

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. *[ ~qi,, UNITED STATES E NUCLEAR REGULATORY COMMISSION 5 gin wAsMiwaTow, o, c.rosas i.hs s;I Request for Additional Information On Guidelines for Permanent BWR Hydrocen Water Chemistry Installation

1. Describe the guidance for the location of hydrogen monitors in areas of potential hydrogen release (such as the hydrogen supply, hydrogen injection, off gas, sump and purge / vent systems).'
2. Provide a revised Table 2-2 in the guidelines to indicate the complete instrumentation and controls for.the hydrogen addition system, including hydrogen supply and injection. Area hydrogen concentration monitors should be described as indicated in question one above and, we conclude, there should be a requirement for indication 'and high alarm functions, rather than a recommendation, as it is described in Table 2-2 presently.

This Table, or an additional one, should indicate the complete '

instrumentation and controls for the oxygen supply and injection systems.

3. Section 2.4.3 in the Guidelines should reflect the acceptance criteria in Standard Review Plan (SRP) 11.3 regarding hydrogen and oxygen monitoring in the off gas recombiner system. As indicated in SRP 11.3, an off gas system designed to withstand the effects of a hydrogen explosion should have one hydrogen analyzer with a!;tomatic control functions downstream of the recombiners and upstream of the delay portions ofi the off gas system. The hydrogen monitor should continuously monitor any residual hydrogen to account for a potential malfunction of the recombiners. For an off gas system not designed to withstand the effects of a hydrogen explosion, two independent hydrogen analyzers should be provided to verify that hydrogen is not present in the recombiner effluent. In view of the above hydrogen monitoring of the off gas system is needed in addition to the oxygen monitoring indicated in the Guidelines.

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4. In reference to the'results from laboratory testing and field testing at l Dresden 2, what will be the long term effect of hydrogen water chemistry, I

in association with improved water quality operational practices, on crud buildup within recirculation piping and on shutdown dose rate levels?

What radiological survey program will the BWR Owners Group recommend to determine long term trends in shutdown dose rate levels attributable to changes in practice with respect to recirculation piping and related facilities?

5. To what extent will site specific wind direction and speed characteristics play a role in the dispersion of hazardous chemicals with respect to

, plant structures and the decision of where facilities will be placed?

6. To increase the sensitivity of leak testing of installed hydrogen and oxygen systems, a leak detector (based on a mass speedometer principle of l operation) should be considered instead of the less sensitive soap bubble test given in the guidelines.
7. Why doesn't the Water Chemistry Control Section (6.1.4) in the guidelines stress the importance of implementation of the BWR Water Chemistry Guidelines? For example, designers and operators should better understand that integranular stress corrosion cracking can be mitigated by controlling the ionic. content in the reactor water by improved water chemistry and reducing the dissolved oxygen in the reactor water by hydrogen injection into the feedwater.

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8. Provide a discussion of the oxygen addition system to the feedwater to meet the feedwater oxygen levels provided in the BWR Water Chemistry Guidelines.
9. It is stated that the curve in Figure 4-2 used to illustrate the concept of dynamic response strength of structures represents many data points for home damages during World War II.1, 2 Provide specific

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l references for the data used in constructing the curve (i.e., specific formulas, tables, etc.). Provide discussions of the step-by-step methodology used for constructing the damage curve (Figure 4-2) and the safe distance curves (for example, Figures 4-6 and 4-3), and relate each step to specific formulas or data.

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10. Provide an evaluation of the damage and safe distance curves discussed in question nine above. The evaluation may consist of a detailed structural response calculation, a simple bounding conservative calculation, or a comparison of the curves with other industry wide approved curves (ASME, ASCE or others) where use of such curves has been

,, demonstrated to be adequate in conjunction with experimental or historical evidence.

11. It is stated in page 4-2 of the Guidelines that " Simultaneous failure of multiple vessels is not addressed because the inherent strength of the vessel is such that it is not susceptible to failure from outside forces (e.g., seismic, tornado missiles, etc.)." Provide a discussion of

" inherent strength" in terms of quantitative engineering considerations and design features that fully supports your conclusion.

12. Provide a detailed analysis of the seismic and tornado design provisions of the liquid hydrogen vessels and supports.
13. Discuss why designing for tornado and earthquake effects are not considered for the storage vessels and piping associated with gaseous hydrogen and oxygen.
14. In Section 8.2.1 of the guidelines, dual Main Steam Line Radiation Monitor (MSLRM) setpoints are recommended for plants at which credit is l taken for MSLRM - initiated isolation during the Control Rod Drop Accident (CRDA). Provide a discussion of how setpoints will be readjusted by operators during hydrogen injection, and what equations are to be used in deriving the actual setpoint values.

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15. Discuss the liquid oxygen vessel and piping system design with respect to external events such as seismic, flood, tornado, etc. (see Section 4.2.1).
16. Describe how the Figure 4-9 was constructed. )

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17. Discuss how flaw (cracks) propagation within vessel and pipe walls with aging was evaluated. Also, discuss QA and inspection programs for detecting initial as well as subsequent flaw growth (for both liquid hydrogen and oxygen tanks).

., 18. I'. is noted from Figure 4-8 in the guidelines that a one inch pipe break releasing 5.5 Kgms/sec of liquid hydrogen can produce explosive f concentrations at distances of up to 1300 feet, and flammable concentrations at distances up to 5,500 feet. Describe the guidelines to be used to guard against liquid hydrogen or oxygen and/or dense heavier-than-air gases entering nearby confined spaces (e.g., vents, sewer systems 8 , buildings, etc.). Using a well defined Probabilistic Risk Assessment (PRA) analysis provide an estimate of the probability for flammable concentrations entering nearby confined spaces. Independently of the PRA, provide an analysis of the consequences on safety related equipment and structures following a detonation within such confined spaces.

The analysis should assume both a large breach and a one inch diameter line failure. The analysis should also include consideration of lor.alized detonations in small structures or cavities and the potential for triggering a free-air-detonation of a plume.

19. Figure 4-8 of the guidelines indicates that a one inch pipe break releases hydrogen at 5.5 Kgms/sec and produces explosive concentrations 1300 feet downwind. Evaluate the thermal flux and overpressure consequences of a delayed ignition / detonation of the hydrogen plume at centroids located at various distances from the point of release up to 1300 feet.

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20. Page 4-10 of the guidelines states that the detonation limits of hydrogen are in the range of 18.3 - 59 percent. Recent data indicates that hydrogen detonations have been observed at concentrations as low as 13.8 percent 4 Review this recent data for inclusion in the guidelines.
21. Page 4-9, Torando and Tornado Missiles, of the guidelines indicates'that tornado missiles are a potential cause of storage vessel failure for all known commercially available liquid hydrogen storage vessels. Provide quantitative estimates of the potential for tornado missile induced ignition of hydrogen. If non-ignitions cannot be ruled out, provide a dispersal analysis of tornado missile induced hydrogen releases under

. post-tornado wind conditions.

22. Figure 4-7 and 4-8 of the guidelines refer to " safety related air intake." This term should be modified to include all air pathways into confined spaces, since many confined space detonation may produce damaging effects on safety related structures elsewhere.
23. In the Cleveland, Ohio, LNG tank failure8 , tank insulating material soaked with LNG was dispersed by the tank explosion and fell on roofs where it ignited. Indicate if the tank insulathg material used in the cryogenic liquid hydrogen storage tanks could produce similar " flaming missiles,"

and their potential effects on safety related plant structures.

24. Provide an analysis addressing the potential for hydrogen release and detonation / deflagration due to lightning effects. Describe guidance on lightning protective systems.
25. NASA procedures require purging liquid hydrogen systems and components with nitrogen, not nitrogen or air as given in Section 3.2.2.4.5 of the guidelines Since, trapped air could initiate a fire or explosion, it is our position that only nitrogen should be used.

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26. Provide an analysis of the hazards associated with onsite storage of compressed gaseous storage of hydrogen compared with storage of liquid hydrogen. The comparison with the liquid hydrogen accident analyses should include considerations of the probabilities and consequences of hydrogen release, dispersion, ignition, deflagration, and detonation.
27. List and analyze the potential hazards and the associated consequences of potential releases of oxygen from the onsite storage of liquid oxygen.

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REFERENCES

1. Jarrett, P. E. , " Derivation of British Explosion Safety Distance," Annals of the New York Academy of Science, Volume 152, 1968.
2. TM-5-1300, U.'S. Army Technical Manual.
3. Report to the Congress of the United States by the Comptroller General,

" Liquified Energy Gases Safety" July 31, 1978, Volume 1, Section 4, pages 24 and 26.

4. NUREG/CR-2726 " Light Water Reactor Hydrogen Manual" pages 2-51, June 1983.

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BOSTON EDISON COMPANY B00 BovLsTON ETREET SDSTON, MA55ACNumETTm 02199 j

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Mr. T. E. Landry Environmental Protection Agency Compliance Branch JFK Federal Building, Room 2103 Boston, MA 02203

Dear Mr. Landry:

The Boston Edison Company is in the process of installing a permanent hydrogen injection system at the Pilgrim Nuclear Power Station (PNPS). The purpose of the hydrogen injection system is to inject hydrogen into the reactor coolant, via the feedwater system, to reduce the dissolved oxygen concentration.

Reducing the dissolved oxygen concentration and maintaining high purity in the reactor coolant should reduce the susceptibility of reactor piping and materials to intergranular stress corrosion cracking. This process is referred to as Hydrogen Water Chemistry (HWC). The hydrogen injection system utilizes electrolytic generation of hydrogen and oxygen on-site.

Boston Edison requests permission for 2-3 gallons per minute of scrubber effluent from the Gas Generator Scrubber, associated with the hydrogen injection system, to be discharged through the PNPS intake embayment storm drain. There will be a concentration of approximately 18 ppb (parts per billion) of potassium hydroxide (KOH) in the discharge effluent. The KOH will increase the pH of this total discharge (which consists of source demineralized water plus a trace of KOH) by 0.5 standard units. Wash-down water from a 500 gallon caustic holding tank may be added to this discharge on a weekly basis containing less than 18 ppb of KOH. Discharge of this effluent will be continuous for the life of PNPS beginning in the Fall of 1986.

He would appreciate a response to this request by June 1, 1986.

If additional information is required please contact Mr.,R. D. Anderson at 849-8935.

Very truly yours,

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BWR Project Directorate #1 ,

1 Division of Licensing Office of Nuclear Reactor Reg.

U.S. Nuclear Regulatory Commission Washington, D. C. 20555 Dr. Thomas E. Murley Regional Administrator Office of Inspection & Enforcement Region I 631 Park Avenue King of P: ussia, PA 19406 Mr. Richard Crettan Massachusetts Division of Water Pollution Control Permit Section - 7th Floor One Winter Street Boston, MA 02198 I

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