ML20217K432
| ML20217K432 | |
| Person / Time | |
|---|---|
| Site: | Duane Arnold  |
| Issue date: | 12/31/1997 |
| From: | Grob B, Vanmiddlesworth IES UTILITIES INC., (FORMERLY IOWA ELECTRIC LIGHT |
| To: | Beach B NRC OFFICE OF INSPECTION & ENFORCEMENT (IE REGION III) |
| References | |
| NG-98-0823, NG-98-823, NUDOCS 9805010215 | |
| Download: ML20217K432 (120) | |
Text
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/ES vtwr es Inc l 200 Frrst Street S E.
PO Bon 351 Cedar Rapics IA $2406-0351 Telephone 3 t9 398 4411 UTILITIES April 30, 1998 NG-98-0823 Mr. A. Bill Beach Regional Administrator Region III U. S. Nuclear Regulatory Commission 801 Warrenville Road Lisle, Illinois 60532-4351
Subject:
Duane Arnold Energy Center Docket No.: 50-331 Operating License No.: DPR-49 1997 Annual Radi11ogical Environmental Report
Dear Mr. Eeach:
Please find attached one (1) copy of the 1997 Annual Radiological Environmental Report for the Duane Arnold Energy Center. This report is transmitted in accordance with the Technical Specification (section 6.11.1.g) reporting requirements.
Sincerely, Gar D. VanMiddlesworth Plant Manager - Nuclear GDV/SF/hc Attachment cc: U:Sv-Nuclear-Regulatory Commission (original w/a)
Attn: Document Control Desk Mail Station Pl-37 Washington, D.C. 20555-0001 3
-t -
NRC Resident Inspector - DAEC (w/ attachments)
R. Laufer (NRC-NRR) (w/ at tachments) \ b/ ' '? [i 'Q E. Protsch - (w/o attachments)
K. Peveler - (w/o attachments)
J. Franz (w/o attachments)
DOCU (w/ attachments) ygR05010215 971231 g ADOCK 05000331 PDR An IES Incastr<es Comcam
W TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY 700 LANDWEHR ROAD NORTHBROOK ILLINOIS MKm:-2.110 (M7) 5644f/00
- f AX (H7) %4-4417 REPORT TO IES LTilLITIES,INC.
CEDAR RAPIDS, IOWA RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP)
FOR THE DUANE ARNOLD ENERGY CENTER CEDAR RAPIDS, IOWA DOCKET NO. 50-331 ANNUAL REPORT - PART I
SUMMARY
AND INTERPRETATION JANUARY - DECEMBER 1997 FOR SUBMITTAL TO THE NUCLEAR REGULATORY COMMISSION PREPARED AND SUBMITTED BY TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY PROJECT NO. 8001 P
Approved by: l8 0 O B-:c is drob!M.S.
jcal L?ad
PREFACE The staff members of'the Teledyne Brown Engineering Environmental Services, Midwest Laboratory were responsible for the acquisition of data presented in this report, with the exception of Appendices D and E, which were completed by DAEC personnel. All environmental samples, with the exception of aquatic, were collected by personnel of DAEC.
Aquatic samples were collected by University of Iowa Hygenic Laboratory personnel.
The report was prepared by the staff of TBEESML, with the exception of Appendices D and E, which were prepared by DAEC personnel.
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- TABLE OF CONTENTS No. Eage PREFACE.............................................................................................ii Lis t o f Tables . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . v Li s t o f Fi g u r es . .. . . .. . . . . . . . .. .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. . . . . . . . . . . . . . . . . . . . . . . . . . . . ..vi 1.0 INTRO DUCTIO N . . .. . . .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. . . . .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 2.0-
SUMMARY
...........................................................................................2 3.0 ENVIRONMENTAL RADIOLOGICAL MONITORING PROGRAM... .. .. ... 3 3.1 Program Design and Data Interpretation.. ... ..... .. ........... ...... .. .3 3.2 Program Description .............. .... .. .............. ..... ........................4 3.3 Progra m Execu tion .... . ... . ... . .... .. . .. . ... . ... ...... . . . . . . . . . . . . . . . .. . . . . . . . . . . . . . . . . . .....5 3.4 Laboratory Proced ures .................. ... .............. . .. . ... . .... . . ... .. . ... .....6 3.5 Program Modifications .. .... ........ .................. . . .....................6 4.0 RESU LTS AND DISCUSSION........... ............. ....... . ... . . .. . .... . . ... .. . . . . .. . 7 4.1 Atmospheric Nuclear Detonations and Nuclear Accidents.. . ... . .. 7 4.2 F rogra m Findings . .. .. . .. . ... ... . . . ... . .. . .. . .. . . . . . . . . . . .. . . . . . . . . . . . .. . . . . . . . . . . . . . . . . . 7 5.0 TABLES AND FIGURES ......................... .. . ........ ... . ... .. . . . . . . . . . . . . .. ... . . 10 6.0 RE FE RENCES CITE D..... . . . . .. ... . .... . .. .. . .. ... . . ..... .. . . .. . . . . .. . .. . . . . . . . .. . . . . . . . . . . . 2 8 APPENDICES A Interlaboratory Comparison Program Results.............. . ...................A-1' B Data Reporting Conventions .......... ..... ..... . ................ .. ... . . ... . ... ... . . . . .. . ..B-1 C Effluent Concentration Limits for Radioactivity in Air and Water Above Background in Unrestricted Areas... . . . ... .. .. ............ ....C-1 D Summary c,f the Land Use Census ........................... ......... .. ......... .. ...D- 1 E Annual Radiation Dose Assessment............ ................ .. .... .............E-1 i
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l TABLE OF CONTENTS (continued)
PART11 lhe Data Tabulations and Analyses.... ......... .... . ...... .... . . . ., ,,,j i
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i LIST OF TABLES No. Page {
4 5.1 Characteristic Properties of Isotopes Quantified in Gamma-spectroscopic Analyses .............................. ..... .... . ... .. . ...11 5.2 Sample Collection and Analysis Program,1997... .............. . . .. ....12 5.3 Sampling Locations, DAEC......... ......... ...... ........ .. ... .. . . . . . . . . . . .. .15 5.4 Type and Frequency of Collections ..................... .... ... . . ........ .. . . . .17 i 5.5 Sample Codes Used in Table 5.4......... . . . . ......... .......... .. ............18 5.6 Missed Collections and Analyses,1997.... ......... . . .. . ..... . . . . ...19 5.7 Radiological Environmental Monitoring Program Summary,1997. . . ... 20 In addition, the following tables are in the Appendices:
Aroendix A A-1 Interlaboratory Comparison Program Results,1997..... . .... . . . . . ... ... A 1 -1 A-2 Interlaboratory Comparison Program Results, Thermoluminescent Dosimeters (TL Ds) .. ... . .. . . . .. . .. .. . .. . . . . ... . . . . . . . . . . . . . . . . . . . . . . . . .. ..A2-1 A-3 In-house Spiked Samples ............... ........... . .......... .. ...... . .. . .............A3-1 A-4 In-house " Blank" Samples ...... .. . ... .... ..... .. . .. .. . . . . .. ... .. . . . . . . . . . . . .. . .. . . . . . . .... A 4- 1 A-5 In-house " Duplicate" Samples........ .. .. .... .... .. .. . . . . . . . . . . . . . . . . . . ..A5-1 A-6 Department of Energy MAPEP comparison results.. .. . . . . ...........A6-1 A-7 Environmental Measurements Laboratory Quality (EML) Assessment Program comparison results ........ ......... .... . .. .... .. . . . . . .. A7-1 Attachment A: Acceptance criteria for spiked samples. . . ... . .. ..A-2 Annendix C C-1 Effluent Concentration Limits for Radioactivity in Air and Water Above Background in Unrestricted Areas.. ..... . .. . . . .. . . .C -2 i
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i LIST OF FIGURES l Nn. Page 5.1 Radiological Environmental Monitoring Program Sampling Stations near the Duane Arnold Energy Center..... ....... ....... . .. . . . ..26 5.2 Radiological Environmental Monitoring Program Sampling Stations Ou isid e 0.5 Miles . . .. . ... . ..... . . . .. . . . . . . . . . . . . . .. . . . . ... . . . .. . . . . .. . . . . . . .. .27 l
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1.0 INTRODUCTION
This report summarizes and interprets results of the Radiological Environmental Monitoring Program conducted by Teledyne Brown Engineering Environmental Services, Midwest Laboratory at the Duane Arnold Energy Center, Palo, Iowa, during the period January -
December,1997. This Program monitors the levels of radioactivity in the air, terrestrial, and aquatic environments in order to assess the impact of the Plant on its surroundings.
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Tabulation of the individual analyses made during the year are included in Part 11 of this report.
I Duane Arnold Energy Center (DAEC) is located in Linn County on the Cedar River, Iowa, and j is operated by IES Utilities, Inc. The D'une Arnold Energy Center is a 565.7 MW(e) boiling
- water reactor. Initial criticality was attained on 23 March 1974. The reactor reached 100%
power on 12 August 1974. Commercial operation began on 1 February 1975.
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- 2.0
SUMMARY
' The Radiological Environmental Monitoring Program required by the U.S. Nuclear Regulatory Commission (NRC) Technical Specifications for the Duane Arnold Energy Center is described.
Results for 1997 are summarized and discussed.
Program findings show background levels of radioactivity in the environmental samples collected in the vicinity of the Duane Arnold Energy Center. No effect on the environment due to the operation of the Duane Arnold Energy Center is indicated.
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3.0 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM 3.1 Program Design and Data Interpretation The purpose of the Radiological Environmental Monitoring Program at the Duane j Arnold Energy Center (DAEC) is to assess the impact of the plant on its environment. '
For this purpose, samples are collected from the air, terrestrial, and aquatic environments and analyzed for radioactive content. In addition, ambient gamma radiation levels are monitored by thermoluminescent dosimeters (TLDs).
Sources of environmental radiation include the following:
(1) Natural background radiation arising from cosmic rays and primordial j radionuclides;
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1 (2) Fallout from atmospheric nuclear detonations; (3) Releases from nuclear power plants; and (4) Industrial and medical radioactive waste.
In interpreting the data, effects due to the DAEC operation must be distinguished from those due to other sources.
A major interpretive aid in assessment of these effects is the design of the monitoring
, program at the DAEC which is based on the indicator-control concept. Most types of samples are collected both at indicator locations (nearby, downwind, or downstream) and at control locations (distant, upwind, or upstream). A station effect would be indicated if the radiation level at an indicator location was significantly larger than that at the controllocation. The difference would have to be greater than could be accounted l for by typical fluctuations in radiation levels arising from other sources.
An additional interpretive technic ue involves analyses for specific radionuclides present l
in the environmental samples co..lected from the DAEC site. The DAEC's monitoring program includes analyses for strontium-90 and iodine-131, which are fission products, and tritium, which is produced by cosmic rays, atmospheric nuclear detonations, and t
also by nuclear power plants. Most samples are also analyzed for gamma-emitting isotopes with results for the following groups quantified: zirconium-95, cesium-137, and cerium-144. These three gamma-emitting isotopes were selected as radiological impact indicators because of the different characteristic proportions in which they appear in the l fission product mix produced by a nuclear reactor and that produced by a nuclear detonation. Each of the three isotopes is produced in roughly equivalent amounts by a reactor: each constitutes about 10% of the total activity of fission products ten (10) days after reactor shutdown. On the other hand, ten (10) days after a nuclear explosion, the contributions of zirconium-95, cerium-144, and cesium-137 to the activity of the resulting debris are in the approximate ratio 4:1:0.03 (Eisenbud,1963). The other group quantified consists of niobium-95, ruthenium-103 and -106, cesium-134, barium-lanthanum-140, and cerium-141. These isotopes are released in small quantities by nuclear power plants, but to date their major source of injection into the general environment has been atmospheric nuclear testing. Nuclides of the next group, manganese-54, cobalt-58 and-60, and zinc-65, are activation products and arise from activation of corrosion products. They are typical components of nuclear power plant effluents, but are not produced in significant quantities by nuclear detonations.
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3.1 Program Design and Data Interoretation (continued)
Nuclides of the final group, beryllium-7, which is of cosmogenic origin, and potassium-40, a naturally-occurring isotope, were chosen as calibration monitors and should not be considered radiological impact indicators.
Characteristic properties of isotopes quantified in gamma-spectroscopic analysis are presented in Table 5.1. Other means of distinguishing sources of environmental radiation can be employed in interpreting the data. Current radiation levels can be compared with previous levels, including those measured before the Plant became o perational. Results of the DAEC's Monitoring Program can be related to those obtained in other parts of the world. Finally, results can be related to events known to cause elevated levels of radiation in the environment, e.g., atmospheric nuclear detonations.
3.2 Program Description The sampling and analysis schedule for the environmental radiological monitoring program at the DAEC is summarized in Table 5.2 and is briefly reviewed below. Table 5.3 defines the sampling location codes used in Table 5.2 and specifies for each location its type (indicator or control) and its distance, direction, and sector relative to the reactor site. The types of samples collected at each location and the frequency of collections are presented in Table 5.4 using codes defined in Table 5.5.
To monitor the air environment, airborne particulates are collected on membrane filters by continuous pumping at twelve locations. Also, airborne iodine is collected by continuous pumping through charcoal filters at six of these locations. Nine of the twelve locations are indicators and three are controls (D-1, D-2, and D-13). Filters are changed and counted weekly. Particulate filters are analyzed for gross beta activity. If gross beta activity exceeds 10 times the yearly mean of the control samples gamma isotopic analysis is performed. Quarterly composites of airborne particulates from each location are gamma scanned on a germanium detector.
Charcoal filters are analyzed weekly for I-131 on all samples.
Ambient gamma radiation is monitored at twelve air sampling locations. In addition, gamma radiation is monitored at thirty-three special locations: seventeen in a circle within 0.5 mi. radius of the DAEC stack; six in 22.5 sectors within 1 mi. of the DAEC stack; and ten in 22.5 sectors between 1 and 3 miles of the DAEC stack. Two TLDs .
are placed at each location and are exchanged and analyzed quarterly, j l
Precipitation samples are collected monthly from one location and analyzed for gamma-emitting isotopes. Quarterly composites are analyzed for tritium.
Milk samples are collected monthly from five locations during the non-grazing season, l October through April, and biweekly during the grazing season, May 1 through l September 30. One location is a control (D-105) and the rest are indicators. All samples are analyzed for I-131 and gamma-emitting isotopes.
For additional monitoring of the terrestrial environment, grain, hay and broad leaf vegetation samples are collected annually, as available, from nine locations: one control ,
(D-105) and eight indicators (D-16, D-57, D-58, D-63, D-72, D-93, D-94, and D-106). !
Grain, hay and broad leaf (green leafy) vegetation samples are analyzed for gamma-4
Program Description (continued) emitting isotopes and at least one broad leaf vegetation is analyzed for iodine-131. If cattle are slaughtered for home use, a meat sample is collected annually, during or immediately following a grazing period from animals grazing on-site. The sample is analyzed for gamma-emitting isotopes. Also, potable ground water is collected quarterly from a treated municipal water system (D-53), the inlet to the municipal water treatment system (D-54) and four additional ground water locations (D-55, D-57, D-58, l and D-72). The samples are analyzed for gross beta and tritium. If gross beta activity exceeds 10 times the yearly mean of the control samples, gamma isotopic, strontium-89 l and strontium-90 analyses are performed.
t l Soil samples are collected once per year at two indicator locations (D-15 and D-16).
The samples are analyzed for strontium-90 and gamma-emitting isotopes.
Surface water is collected monthly from five river, pond and sewage effluent locations, one control (D-49) and four indicator (D-50, D-51, D-99, and D-107). All monthly samples are analyzed for gamma-emitting isotopes. Tritium analyses are performed on quarterly composites from each location. In addition, all samples from Location D-107 (plant sewage discharge) are analyzed for K-40 by flame photometry.
The aquatic environment is also monitored by upstream and downstream (D-49 and D-
- 61) semiannual collections of fish. River bottom sediment is also collected semiannually l at the plant's intake and discharge (D-50 and D-51) and downstream of the sewage l plant (D-107). The samples are analyzed for gamma-emitting isotopes.
3.3 Procram Execution I l
l The program was executed as described in the preceding section with the following exceptions:
(1) No air particulate sample was available from location D-13 for the week ending January 23,1997. The sample was lost in the field due to strong winds.
! (2) TLD data was not available for the third quarter,1997 from locations D-31 and D-91. The TLDs were lost in the field.
(3) TLD data was not available for the fourth quarter,1997 from location D-35. The i TLD was lost in the field. l (4) No milk was available from location D-93 and D-101 for January and February,
- 1997. The goats v'ere dry.
(5) No milk was available from location D-105 for the week ending June 17,1997.
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3.4 ' Laboratory Procedures All iodine-131 analyses in milk were made by using a sensitive radiochemical procedure which involves separation of the element by use of an ion-exchange resin and subsequent beta counting.
All gamma-spectrosco:>ic analyses were performed with high resolution germanium detectors. Levels of loc ine-131 in vegetation were determined by gamma spectrometry.
Levels of airborne iodine-131 in charcoal samples were measured by. gamma spectrometry.
Tritium levels were determined by the liquid scintillation technique.
Analytical Procedures used by TBEESML are on file and are available for inspection.
Procedures are based on those prescribed by the National Center for Radiological Health of the U.S. Public Health Service (U.S. Public Health Service,1967) and by the Health and Safety Laboratory of the U.S. Atomic Energy Commission (U.S. Atomic Energy .
Commission,1972).
Details of TBEESML's QA program are presented elsewhere (Teledyne Isotopes Midwest Laboratory,1992 ). The TBEESML QA Program includes participation in the
'Interlaboratory Comparison (Crosscheck) Program. Results obtained in the crosscheck program are presented in Appendix A.
3.5 Program Modifications There were no program modifications during the year,1997, i
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4.0 RESULTS AND DISCUSSION All of the scheduled collections and analyses were made on schedule except those listed in Table 5.6.
All results are summarized in Table 5.7 in a format recommended by the Nuclear Regulatory Commission in Regulatory Guide 4.8. For each type of analysis of each sample medium, this table lists the mean and range of all indicator and control locations. The locations with the highest mean and range are also shown.
The tabulated results of all measurements made in 1997 are not included in this section, although references to these results will be made in the discussion. The complete tabulation of the 1997 results is contained in Part II of the 1997 Annual Report on the Radiological Environmental Monitoring Program for the Duane Arnold Energy Center.
4.1 Atmospheric Nuclear Detonations and Nuclear Accidents There were no reported atmospheric nuclear tests in 1997. The last reported test was conducted by the People's Republic of China on October 16,1980. The reported yield was in the 200 kiloton to 1 megaton range.
There were no reported accidents at nuclear reactor facilities in 1997.
4.2 Program Findings Results obtained show background levels of radioactivity in the environmental samples collected in 1997. l Airborne Particulates The average annual gross beta concentration in airborne particulates was similar at indicator and control locations (0.023 and 0.024 pCi/m3, respectively) and similar to levels in 1984 (0.025 and 0.026 pCi/m3 , respectively), 1985 (0.024 pCi/m3 at both locations), in 1986 (0.024 pCi/m3, at both indicator and control locations), in 1987 (0.024 and 0.026 pCi/m3, respectively), in 1988 (0.026 and 0.028 pCi/m3 ,
respectively), in 1989 (0.026 and 0.029 pCi/m3, respectively), in 1990 (0.022 and 0.024 pCi/m3, respectively), in 1991 (0.023 and 0.022 pCi/m 3, respectively), in 1992 (0.022 and 0.023 pCi/m 3, respectively), in 1993 (0.022 and 0.023 pCi/m3, respectively), in 3 3 1994 (0.023 and 0.024 pCi/m , respectively),3in 1995 (0.025 and 0.024 pCi/m ,
respectively) and in 1996 (0.024 and 0.023 pCi/m , respectively). The average of 0.024 pCi/m3 orf 1986 does not include the results from May 15 to June 12,1986, which were influenced by the accident at Chernobyl.
A s 3 ring peak in beta activity had been observed almost annually for many years (Wi. son d al.,1969). It had been attributed to fallout of nuclides from the stratosphere (Gold d al.,1964). It was pronounced in 1981, occurred to a lesser degree in 1982, and did not occur from 1983 through 1997, in 1986, the spring peak could not be identified because it was overshadowed by the releases of radioactivity from Chernobyl. Gamma spectroscopic analysis of quarterly composites of air particulate filters yielded similar results for indicator and control locations. Beryllium-7, which is produced continuously in the upper atmosphere by cosmic radiation (Arnold and Al-Salih,1955), was detected 7
Airborne Particulates (continued) in all samples. All other gamma-emitting isotopes were below their respective LLD limits. No plant effect was indicated.
Airbome Iodine Weekly levels of airborne iodine-131 were below the lower limit of detection (LLD) of 0.07 pCi/m3 in all samples.
Ambient Radiation (TLDs)
At twelve air sampling locations, the TLD readings averaged 13.3 and 12.7 mR/ quarter for indicator and control locations, respectively. At locations within 0.5 mile,1.0 mile, and 3.0 mile radius of the stack, the measurements averaged 14.8 mR/ quarter,15.5 mR/ quarter, and 12.8 mR/ quarter, respectively. The average for all locations was 14.0 mR/ quarter. This is lower than the estimated average natural backgrou: .1 radiation for Middle America,19.5 mR/ quarter, which is based on data on Pages 71 and 108 of the report, " Natural Background Radiation in the United States" (National Council on Radiation Protection and Measurements,1975). The terrestrial absorbed dose (uncorrected for structural and body shielding) ranges from 8.8 to 18.8 mrad / quarter and averages 11.5 mrad / quarter for Middle America. Cosmic radiation and cosmogenic radionuclides contribute 8.0 mrad / quarter for a total average of 19.5 mrad / quarter. No plant effect was indicated, j
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Precioitation in precipitation, the tritium concentration was below the LLD of 330 pCi/L in all samples. No gamma-emitting isotopes were detected. No plant effect was indicated.
Milk lodine-131 results were below the detection limit of 1.0 pCi/L Ca all samples.
No gamma-emitting isotopes, except naturally occurring potassium-40, were detected in any milk samples. This is consistent with the finding of the National Center for Radiological Health that most radiocontaminants in feed do not find their way into milk due to the selective metabolism of the cow. The common exceptions are radioisotopes of potassium, cesium, strontium, barium, and iodine (National Center for Radiological Health,1968).
In summary, the milk data for 1997 show no radiologica! effects of the plant operation.
Ground Water The annual mean for gross beta activity measured 3.2 pCi/L and was similar to the levels observed in 1980 through 1996. The location with the highest mean (5.0 pui/L) was D-58, a farm 1.0 mile distant from the plant. Tritium was below the LLD of 330 pCi/L in all samples. No plant effect was indicated.
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l Vegetation Iodine-131 results in broadleaf vegetation were below the LLD level of 0.053 pCi/g wet weight in all samples.
Except for potassium 40, which was observed in all vegetation samples ( broadleaf, grain, and forage ), all other gamma-emitting isotopes were below detection limits in all samples. No plant effect is indicated.
Soil Strontium-90 was detected in both samples and averaged 0.051 pCi/g dry weight.
Cesium-137 was detected at an average concentration of 0.20 pCi/g dry weight. Both strontium-90 and Cesium-137 concentrations were similar to levels observed in 1987 (0.08 and 0.30 pCi/g dry weight, respectively), in 1988 (0.064 and 0.33 pCi/g dry weight, respectively), in 1989 (0.046 and 0.18 pCi/g dry weight, respectively), in 1990 (0.066 and 0.21 pCi/g dry weight, respectively), in 1991 (0.064 and 0.34 pCi/g dry weight, respectively), in 1992 (0.040 and 0.26 pCi/g dry weight, respectively), in 1993 (0.058 and 0.26 pCi/g dry weight, respectively), in 1994 (0.040 and 0.27 pCi/g dry weight, respectively),in 1995 (0.044 and 0.21 pCi/g dry weight, respectively) and in 1996 (0.050 and 0.17 pCi/g dry weight, respectively).
The only other gamma-emitting isotope detected was potassium-40 at an average concentration of 12.94 pCi/g dry weight. No plant effect on soil was indicated.
Surface Water Tritium was below the LLD level of 330 pCi/L in all samples.
All gamma-emitting isotopes were below their respective LLDs.
K-40 was measured at one location, D-107 (sewage effluent). The concentration ranged from 9.5 to 23.4 pCi/L and averaged 16.4 pCi/L.
No plant effect on the radioactivity of surface water was indicated.
Eish All gamma-emitting isotopes, except naturally-occurring potassium-40, in edible portions were below de+cction limits. The potassium-40 level was similar at both indicator and control locations (2.88 and 2.80 pCi/g wet weight, respectively). No plant effect on fish was indicated.
River Sediments River sediments were collected in June and September,1997, and analyzed for gamma-emitting isotopes. Traces of Cobalt-60 were detected in two samples from location D-107 (sewage effluent) at an average concentration of 0.20 pCi/g dry weight. Potassium-40 ranged from 5.15 to 10.99 pCi/g dry weight and averaged 7.25 pCi/g dry weight.
All other gamma-emitting isotopes were below detection limits.
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I 5.0 TABLES AND FIGURES 10
f Table 5.1 Characteristic properties of isotopes quantified in gamma-spectroscopic analyses.
Designation Comment Isotope Half-lifea i
! 1. NaturallyOccurring A. Cosmogenic Produced by interaction of cosmic Be-7 53.2 d
- rays with atmosphere B. Terrestrial Primordial K-40 1.26 x 109 y II. Fission Productsb '
Nuclear detonations constitute the major environmental source l A. Short-lived I-131 8.04 d Ba-140 12.8 d B. Other than Short-lived Nb-95 35.15 d i
Zr-95 65 d Ru-103 39.35 d Ru-106 368.2 d Cs-134 2.061 y Cs-137 30.174 y Ce-141 32.5 d Ce-144 284.31 d III. Activation Products Typically found in nuclear power Mn-54 312.5 d plant effluents Fe-59 45.0 d Co-58 70.78 d Co-60 5.26 y Zn-65 245 d l
a Half-lives are taken from Appendix E of Environmental Quarterly,1 January 1978, EML-334 l (U. S. Department of Energy,1978). l b Includes fission-product daughters. I l
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Table 5.2 Sample collection and analysis program,1997.
Exposure Sampling Location Pathway Sample Sampling and Type and Frequency and/or Point ' Description Collection Frequency of Analysis Sample Type-Airborne 'l Cedar Rapids (C) Continuous operation of Analyze for gross beta Particulates 2 Marion (C) sampler with sample activity more than 24 hours2.777778e-4 days <br />0.00667 hours <br />3.968254e-5 weeks <br />9.132e-6 months <br /> 3 Hiawatha collection at least once after filter change. Perform 5 Palo per week or as required gamma isotopic analysis on
'6 - Center Point by dust loading each sample having gross beta 7 Shellsburg - activity greater than ten 8 Urbana times the yearly mean of the
, 10 - Atkins control samples.
l 11 Toddsville l 13 Alburnett (C) Composite weekly samples to l 15 On-site North. form a quarterly composite (by l
16 On-site South location). Analyze quarterly composite for gamma isotopic.
Airborne Iodine 2 Marion (C) Continuous operation of Analyze each cartridge for 5 Palo sampler with sample iodine-131.
7 Shellsburg collection at least once 8 Urbana per week.
11 Toddville 15 On-site North Ambient 3 Air Particulate Two dosimeters Read gamma radiation dose Radiation 5-8 Locations continuously at each quarterly .
10,11 location. Both 13,15 dosimeters are changed 16 at least quarterly.
18-23, Within 0.5 mile of 28 32, Stack 33-42 Within 3.0 miles of Stack 43-48 Within 1.0 mile of 82 86, Stack 91 Surface Water - 49 Lewis Access (C) Once per month. Gamma isotopic analyses of 50 Plant Intake (C) each sample (by location).
51 Plant Discharge 99 Pleasant Creek Composite monthly samples to 107 Plant Sewage form quarterly composite (by Dischange location). Analyze quarterly composite for tritium.
(C) denotes control location. All other locations are indicators.
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I Table 5.2 Sample collection and analysis program,1997 (continued).
Exposure Sampling Location Pathway Sample Sampling and Type and Frequency and/or Point Description Collection Frequency of Analysis Sample Type '
Ground 53 Treated Grab sample at least Gross beta and tritium Water Municipal Water once per quarter activity analysis on (potable) 54 Inlet to Municipal quarterly sample. If gross Water Treatment beta is greater than ten System times the yearly mean of On-site well control samples, perform 55 Wells off-site and gamma isotopic and Sr-89 57,58 within 4 km of and Sr-90 analyses.
72 DAEC River 50 Plant Intake (C) At least once every Gamma isotopic analysis of ,
Sediment 51 Plant Discharge six months. each sample. {
107 Sewage Effluent Canal Vegetation 16,57, Farms that raise Annually at harvest Gamma isotopic analysis of 58,63, food crops time. One sample of edible portions. 1 72,93, each: grain, green 94,106, leafy, and forage. At 1-131 analysis on broadleaf 105 (C) least one sample vegetation.
should be broadleaf vegetation.
Fish 49 Cedar River One sample per 6 Gamma isotopic analysis on upstream of DAEC months (once during edible portions.
not influenced by January through July effluent (C) and once during Downstream of August through l 61 DAEC in influence December).
of effluent l Milkb 105 Control Farm near At least once per two Durine the crazine season: ,
l Amana, Iowa weeks during the Gamma isotopic and iodine- l grazing season. 131 analyses of each sample. l' Dairy Farms 63,93, within 10 miles of At least once per Durine the non-crazine season:
96,101 Site month during the Gamma isotopic and iodine-non-grazing season. 131 analyses of each sample.
(C) denotes control location. All other locations are indicators.
13
I i i
l Table 5.2 Sample collection and analysis program,1997 (continued).
, Exposure Sampling Location l Pathway Sample Sampling and Type and Frequency l and/or Point Description Collection Frequency of Analysis i
Sample Type i
l Precipitation On-site Monthly Gamma isotopic on all samples.
1 Tritium on .{ u a r t erly composites.
MeatC On-site Annually Ganuna lsotopic Soil 15,16 On-site Annually Gamma Isotopic and Sr-90.
- a Gamma isotopic analysis and analysis for gamma-emitting nuclides refer to high resolution gamma ray spectrum analysis. Any radionuclide detected at a concentration greater than the lower limit of detection (LLD) should be reported quantitatively; conversely, any radionuclide concentration less than the LLD should not be reported.
b The grazing season is considered to be May 1 through September 30.
c Meat was not collected in 1997; no animals slaughtered for home use.
i l
I I-l l
14
Table 5.3 Sampling locations, Duane Arnold Energy Center.
Sampling Location Code Type Distance and Sampling Direction from Site Point Location Description Stack D-1 C 1 Cedar Rapids 11 mi @ 135 SE D-2 C 2 Marion 11 mi @ 125'ESE D-3 3 Hiawatha 7 mi @ 130'SE D-5 5 Palo 3 mi@ 200 SSW D-6 6 Center Point 7 mi @ 0 N.
D-7 7 Shellsburg 6 mi @ 255 W D 8 Urbana 10 mi @ 345 NW D-10 10 Atkins 9 mi @ 210 SSW
- D-11 11 Toddville 4 mi O 90 E D-13 C 13 Alburnett 9 mi @ 70 ENE D-15 15 On-site, Northwest 0.5 mi @ 305 NW D-16' 16 On-site, South 0.5 mi G 190 SSE D-18 18 0.5 mi NNE
. D-19 19 0.5 mi NE D-20 20 0.5 mi ENE D-21 21 0.5 mi ENE D-22 22 0.5 mi E D-23 23 0.5 mi ESE D-28 28 0.5 mi WSW D-29 29 0.5 mi W D-30 30 0.5 mi WNW D-31 31 0.5 mi NW D 32 0.5 mi NNW D-33 33 3.0 mi N D-34 34 3.0 mi NNE D-35 35 3.0 mi NE-D-36 6 3.0 mi ENE D-37 37 3.0 mi E D 38 3.0 mi ESE D-39 39 3.0 nt SE D-40 40 3.0 mi JSE D 41 3.0 m.i S l D-42 42 3.0 mi SSE D-43 43 1.0 mi SSW D-44 44 1.0 mi WSW i D-45 45 1.0 mi W D-46 -46 1.0 mi WNW D-47 47 1.0 mi WNW !
D-48 48 1.0 mi NW i D-49 C- 49 Lewis Access, upstream of DAEC 4.0 mi NNW ;
D-50 C .50 Plant Intake i D-51 51 Plant Discharge- I D-53 53 Treated Municipal Water I D-54 54 Inlet to Municipal Water ;
Treatment System- !
D-55 55 On-site Well 15
Table 5.3 Sampling locations, Duane Arnold Energy Center (continued).
Sampling Location
~ Code' Type Distance and Sampling .
Direction from Site Point Location Description Stack D-57 57 Farm (Off-site Well) 1.0 mi WSW D-58 58 Farm (Off-site Well) 0.5 mi WSW-SW D-61 61 0.5 mi downstream of plant discharge
- D-63 63 Farm 1.5 mi WNW D-72 72 Farm 2.0 mi SSW D-82 82 0.5 mi SE D-83 83 0.5 mi SSE D-84 84 0.5 mi S D-85 85 0.5 mi SSW
. D-86 86 0.5 mi SW D-91 91 0.5 mi N D-93 93 Farm 2.8 mi NNE
' D-94 94 Farm 2.7 mi N D-96 96 Farm 8.0 mi SSW D-99 99 Pleasant Creek !.ake 2.5 mi WNW D-101 101 Farm 4.0 mi E D-105 C 105 Farm 21.3 mi SSW D-106 106 Farm 4.5 mi SE D-107 107 Sewage Effluent Canal On-site "C" denotes control location. All other locations are indicators.
)
16 ;
i
Table 5.4 Type and Frequency of collection.
1 Location - "," Weekly Monthly Quarterly Semiannually Annually i D-1 C AP TLD D-2 C AP,Al TLD l D-3 AP TLD D-5 AP,AI TLD D-6 AP TLD j
> D-7 AP,Al TLD D-8 AP,Al TLD D-10 AP TLD D-11 AP,Al TLD D-13 C AP TLD D-15 AP,Al TLD SO D-16 AP TLD SO, G D-18 through TLD D-23 D-28 through TLD D-42 D-43 through TLD D-48 D-49 C SW F D 50 C SW RS D-51 SW RS D-53 WW D-54 WW D-55 WW '
D-57 WW G D-58 WW G 1 D-61 F D-63 M G I D-72 WW G ;
D-82 through TLD '
D-86 l D-91 TLD i D-93 M G !
D-94 M G D-96 M D-99 SW D-101 M D-105 C M G D-106 M G D-107 SW RS On-site P ME "C" denotes control location. All other locations are indicators.
l-l 17
Table 5.5. Sample codes used in 5.4.
Code Description AP Airborne Particulates j Al Airbornelodine TLD Thermoluminescent Dosimeter P Precipitation M Milk WW Well Water G Vegetation ME Meat SO Soil SW Surface Water F Fish RS River Sediment l.
18 i
I
I l
i l Table 5.6. Missed collections and analyses, Duane Arnold Energy Center,1997.
i i
l l Collection Date Sample Analysis Location (s) or Period Comments l Milk I-131, Gamma D-93 01-07-97 Sample not available.
Milk I-131, Gamma D-101 01-07-97 Sample not available.
AP Gross Beta D-13 01-23-97 Samplelost in strong wind.
Milk I-131, Gamma D-93 02-04-97 Sample not available.
Milk I-131, Gamma D-101 02-04-97 Sample not available.
Milk 1-131, Gamma D-105 06-17-97 Lost in shipment.
TLD - Ambient Gamma D-31, 91 3rd Qtr.,1997 Samples lost in the field.
TLD ' Ambient Gamma D-35 4th Qtr.,1997 Samples lost in the field.
l l
I l
l l
i i
l l
19 l
I
)
. Table 5.7 Radiological Environmental Program Summary.
. Name of Facihty . Duane Arnold Energy Center Docket No. 50-331 Location of Facility Lmn, Iowa Reporting Period January - December Iw7 (County, State) indicator Location with Highest Control Numtwr Sample Typeand . Locations Annual Mean Locations Non-
-Type Number of LLob Mean (F)C Mean (Fje Routine Mean (F)C (Units) Analysesa Ranaec Locationd Ranger Range Results' Airborne GB 623 0.004 0.023 (467/468) D 1,2,6 0.025 (154/155) 0.024 (154/155) O particulates (0.010-0.072) Alllocations had (0.013-0.067) (0.012-0.067)
(pCi/m3) identical means GS 48 Be-7 0.012 0.079 (36/36) D 1, Cedar Rapids, 0.091 (4/4) 0.088 (12/12) 0 (0.049-0.11) 11 mi.SE - (0.068 4.11) (0.054-0.11)
Nb-95 0.0021 <LLD - -
<LLD 0 Zr-95 0.0036 <LLD - -
<LLD 0 Ru-103 0.0020 <LLD - -
<LLD 0 Ru-106 0.014 <LLD - -
<LLD 0 Cs-134 0.0014 <LLD - -
<LLD 0 Cs-137 0.0016 <LLD - -
<LLD 0-Ce-141 0.0028 (LLD - -
<LLD 0 Ce 144 0.0072 <LLD - -
<LLD 0 Airborne 1131 312 0.07 <LLD - -
<LLD 0 lodme (pCi/m3)
TLD,AP Gamma 48 1 13.3 (36/36) D-7, Shellsburg, 19.3 (4/4) 0 12.7 (12/12)
- 1.ocations (7.1 37.1) 6 mi. W (11.0-37.1) (9.8-17.0)
(mR/ quarter)
TLD, within Camma 66 1 14.8 (66/66) D-31, None 19.7(3/3) 0 0.5 mi of Stack (10.3-23.5) 0.5 mi. NW (mR/ quarter)
(17.2-23.5) /
/
TLD, within Gamma 24 15.5 (24 /24) D-46, 1 17.4 (4/4) None 0 1.0 mi of Stack (10.8-20.0) 1.0 mi. WNW (14.9 20.0)
(mR/ quarter)
TLD, within Gamma 39 1 12.8 (39/39) D-37, None 16.4 (4/4) o 3.0 miof Stack (9.2-17.6) 3.0 mi E (15 0-17.6)
(mR/ quarter)
Precipitation H-3 4 330 <LLD - -
None 0 (pCi/L)
GS 12 Mn-54 7.3 <LLD - -
None 0 Fe 59 15.0 (LLD - -
None O Co-58 6.7 <LLD -
None 0
20
i Table 5.7 Radiological Envuonmental Program Summary.
Name of Facihty Duane Arnold Energy Center Docket No. 50-331 locationofFacihty Linn, Iowa Reporting Period January - December 1W7 (County, State) indicator Location with Highest Control Numtvr Sample Type and .
Locations Annual Mean Locations Non.
Type Number of LLob Mean (F)C Routine Mean (F)C Mean (F)c (Units) Analp a Rangec locationd Rangee Range Results" Precipitation Co-60 8.2 <LLD - -
None 0 (pCi/L)
(conhnued) Zn-65 20.5 <LLD - -
None 0 l
Nb-95 8.0 <LLD - - None 0 Zr 95 16.9 <LLD - -
None 0 l I-131 20.1 <LLD - - None O Cs-134 7.5 <LLD - - None O Cs-137 8.2 <tLD - + None 0 l~ Ba-140 44.0 <LLD - - None O La-140 12.7 <LLD - -
None O Mdk 1-131 85 1.0 <LLD - - <LLD. O
- . (pCi/L) l CS 85
.i l K-40 100 1560 (68/68) D-93, Farm 1710 (16/16) 1420 (17/17) 0 l
.(1000-2120)- 2.8 mi. NNE (1000-2000) (1230-1570)
Cs-134 15 <LLD - - <LLD 0
! Cs-137 18 <LLD - -
<LLD 0 i
Ba-140 60 <LLD - -
<LLD 0 l- La-140 15 <LLD - -
<LLD 0 l.
l^
- , Ground Water CB 24 1.2 3.2 (14/24) D-58, Farm 50(3/4) None 0
[ (pCi/L) (1,3-5.9) 1.0 mi. WSW-SW (4.3-5.9) l l H-3 24 330 <LLD - - None o l
t l Broadleaf I131' 5 0.053 <LLD . - None 0 i Vegetation (pCi/g wet) CS 5 K 40 0.5 - 2.94 (5/5) D-94, Farm 4.19 (1/1) None 0 (2.26-4.19) 2.7 mi. N Mn-54 <LLD 0.025 - -
None 0 Co-58 0.022 <LLD - - None O Co-60 0.025 <LLD - - None 0 l
Nb-95 0.033 <LLD - - None 0 ;
Zr-95 0.040 <LLD - - None O Ru-103 0 021 <LLD - - None 0 l
21
\
l
i Table 5.7 Radiological Environmental Program Summary.
Nameof Facility Duane Arnold Energy Center Dxket No. 50-331 location of Facility Linn, Iowa Reporting Period Januarv - December 1W7 (County, State)
Indicator location with Highest Control Number Sample Type and locations Annual Mean Locations Non-l Type Number of LLDb Mean (F)C Routine Mean (F)' Mean (F)c (Units) Analysesa Rangec Locationd Rangee Range Results" Broadleaf Ru-106 0.26 (LLD - -
None O Vegetation (pCi/g wet) Cs-134 0.024 <LLD - -
None 0 (contmued) i Cs 137 0.025 <LLD - -
None O Ce-141 0.046 <LLD - -
None O Ce-144 0.16 <LLD - -
None o i Vegetation (Grain) GS 7 (pCi/g wet)
K-40 0.5 3.55 (6/6) D-16, Onsite, 8.34 (1/1) 1.93 (1/1) 0 (2.19-8.34) 0.5mi. SSE l- Mn-54 0.014 <LLD -- -
<LLD 0 Co-58 0.017 (LLD - -
<LLD 0 Co-60 0.026 <LLD - -
<LLD 0 Nb-95 0.020 <LLD - -
<LLD 0 Zr-95 0.031 <LLD - -
<LLD 0 Ru-103 0.020 <LLD - -
<tLD 0 Ru-106 0.11 <LLD . - -
<LLD 0 Cs-134 0.018 <LLD - -
<.LLD 0 Cs 137 0.020 <LLD - -
<LLD 0 Vegetation CS 5 l (Forage)
(pCl/g wet) K 40 0.5 12.80 (4/4) D 63, Farm 19.13 (1/1) 16.84 (1/1) 0 (2.54-19.13) 1.5 mi. WNW Mn-54 0.054 <LLD <LLD 0
)
Co-58 0.046 <LLD - -
<LLD 0 1
Co-60 0.087 <tLD - -
<LLD 0 j Nb-95 <LLD i 0.045 - -
<LLD 0 1
Zr-95 0.090 (LLD - -
(LLD 0 Ru-103 0.059 <LLD - -
<LLD 0 Ru-106 0.27 (LLD - -
<LLD 0 i Cs 134 . 0.060 <LLD - -
<LLD 0 i 22 l
l l
1 Table 5.7 Radiological Environmental Program Summary.
Name of Facility Duane Arnold Energy Center Docket No. 50-331 location of Facility Linn, Iowa Reporting Period January - Decemtwr 1w7 (County, State)
Indicator location with Highest Control Number Sample Type and Locations Annual Mean Locations Non-Type Number of LLob Mean (F)C Routme Mean (F)C Mean (F)c (Units) Analyses a Rang,c Locationd Range e Range Results' Vegetation - Cs-137 - 0.063 <LLD - -
<LLD 0 rorage (pCi/g wet) Ce-141 0.062 <LLD - -
<LLD 0 fwn:tnued)
Ce-144 0.43 <LLD - -
<LLD 0 Soil Sr-90 2 0.01 0.051 (2/2) D-16, Onsite, None 0 0.057 (1/1)
(pCi/g dry) (0.044-0.057) ' O.5 mi. SSE GS 2 K-40 0.5 12.94 (2/2) D-15, Onsite 15.84 (1/1) None 0 (10.04 15.84) 0.5 mi. NW Mn-54 0.019 <LLD - - None O Co-58 0030 <LLD - - None O Co-60 0.023 <LLD. - -
None O Nb-95 0.046 <LLD - -
None 0 Zr-95 0.027 <LLD - - None 0 .
1 Ru-103 0.020 <LLD - -
None o Ru-106 0.12 <LLD - - None 0 C5-134 0.037 <LLD None 0 )
Cs 137 0.060 0.20 (2/2) D-16, Onsite, 0.28 (1/1) None 0 (0.12-0.28) 0.5 mi. SSE Ce-141 0.061 <LLD - -
None O Ce-144 0.14 <LLD - -
None O surface Water H-3 20 330 <LLD - -
(LLD 0 (pCi/L)
K-40 12 0.5 16.4 (12/12) D-107, Onsite 16.4 (12/12) None 0 (9.52 23.36) Sewage Effluent (9.52 23.36) 1-131 - 60 15 <LLD - -
<LLD 0 CS 60 Mn-54 15 <LLD - -
<LLD 0 Fe 59 30 <LLD - -
<LLD 0
. Co-58 15 <LLD - -
<LLD 0 l Co-60 15 <LLD - -
<LLD 0 l
- Zn-65 30 <LLD - -
<LLD 0 j 1
1 23 l
Table 5.7 RadiologicalEnvuonmentalProgramSummary.
l Nameof Facility Duane Arnold Energy Center , Docket No. 50-331 l location of Facility Linn, Iowa - Reportmg Period January - Decemtwr 1997
. (County, State) indicator Location with ti;; hest Control Number Sample Type and locations Annual Mean Locations Non.
Type- Number of . LLDb ' Mean (F)C Routine Mean (F)C Mean (F)c (Units) Analysesa Ranaec Locationd Rangec Range Results' surface Water Nb-95 15 <LLD - -
<LLD 0 (pCi/L) kontinued) Zr-95 30 <LLD - -
<LLD 0 Cs-134 15 <LLD - -
<LLD 0 Cs-137 18 <LLD - -
<LLD 0 Ba-140 60 <LLD - -
<LLD 0 La-140 15 <LLD - - <LLD 0 River GS 6 Sediments (pCi/g dry) K-40 1.0 7.20 (4/4) D-51, Plant 8.51 (2/2) 7.30 (2/2) 0 (5.15-10.99) Discharge (6.02-10.99) (6.50-8.22)
Mn-54 0.048 <LLD - -
<LLD 0 Co-58 0.045 <LLD - - <LLD 0 Co-60 0.025 0.20 (2/4) D-107, Sewage 0.20 (2/2) <LLD 0 (0.16-0.25) Effluent Canal' (0.16-0.25)
Nb-95 0.062 <LLD - -
<LLD 0 Zr45 0.099 <LLD - -
<LLD 0 Ru-103 0.048 <LLD - -
<LLD 0 Ru-106 0.32 <LLD - -
<LLD 0 Cs-134 0.055 (LLD - -
<LLD 0 Cs-137 0.041 <LLD - -
<LLD 0 Ce-141 0.066 <LLD - -
<LLD 0 Ce-144 0.16 <LLD - -
<LLD 0 Fish CS 6 (Edible Portions) K-40 0.5 2.80 (3/3) D-49, Lewis Access, 2.88 (3/3) 0 2.88 (3/3)
(pCi/g wet) (2.48-2.98) 4.0 mi. NNW (2.80-2.99) (2.80-2.99)
(LLD 0 Co-58 0.012 <tLD - -
<tLD 0 Co-60 0.011 <LLD - -
<LLD 0 Fe-59 0.043 <LLD -
<LLD 0
Zn-65 0.071 <LLD - -
<LLD 0 24
Table 5.7 Radiological Environmental Program Summary, Name of Facility Duane Arnold Energy Center Docket No. 50-331 locationof Facility Linn, Iowa Reporting Period January - December Iw7 (County, State) indicator Location with Highest Lontrol Number Sample . Type and locations Annual Mean Locations Non-i Type Number of LLob Mean (F)C Mean (F)( Routine Mean (F)c (Units) Analysesa Rangec Locationd Rangee Range Results' Fish Nb-95 0.043 <LLD - -
<LLD 0 (Edible Portions) Zr-95 0.038 <LLD - -
(LLD 0 (pCi/g wet)
(contmued) Ru-103 0.024 <LLD - -
<LLD 0 )
l Ru-106 0.15 .<LLD - -
<LLD 0 Cs-134 0.018 <LLD - -
<LLD 0 Cs-137 0.018 <LLD - -
<LLD 0 )
Ce-141 0.028 <LLD - -
<LLD 0 Ce-144 0.15 <LLD - - <LLD 0 8
GB = gross beta; GS = gamma scan.
b LLD = Nominal lower limit of detection based on 4 66 sigma counting error for the background sample.
c Mean and range based upon detectable measur2ments only. Fraction of detectable measurements at specihed locations is indicated in parentheses (F).
d Locations are specified by: (1) Name and code (Table 5.3); and (2) distance, direction, and sec*or relative to reactor site.
" Non-routine results are those which exceed ten times the control station value for the location. If a control station value is not available, ths +sult is considered non routme if it exceeds ten times the preoperational value for the location.
l I
l 4
25
[
l l
l Figure 5.1 Radiological Environmental Monitoring Program Sampling Stations near the Duane Arnold Energy Center.
BARRICADE g---- T h l CEDAR RIVER i
r____._ .15 - J l )Uo/
f l 6 I 3,2 H 18 /
< l /
I
> l t
I E l I l 6 I O 31 O / C i < S O f l
x l l
' U w 19 (\
g 30 < 20 I
o \
l x 107 I SWIKHY F DAEC f) /
$7 29 Sp j
/
g : 23 /
/
50 f
lllllllllllllllllll'lllllllll 86 __ ;
ll-16 f
g
, 85 9 83 82
,POWERPLANT RD l GATE 61 58
- - - - - Property Line
, 2000 feet ,
\
l l nl See Table 5.3 for sampling locations and Table 5.4 for Type and Frequency of collection.
26
Figure 5.2 Radiological Environmental Monitoring Program Sampling Stations Outside 0.5 Miles.
10 MILE RADIUS URBANA 3 08 N
CENTER POINT lg CEDAR RIVER
\ 5 MILE RADIUS 49 93 ALBURNETT 33 34 13 0 36 99 63 47 37 SHELLSBURG 46
- DAEC MDDN
, 07 45 38 9 101 SITE 43 39 72 O PALOS 05 106 41 i
03 HIAWATHA'
! e MARION MI 53 ATKINS ~ ,
54 S 10 !
I i
l I
I CEDAR I 105 RAPIDS
_ 01 i
t i
I See Table 5.3 for sampling locations and Table 5.4 for Type and Frequency of collection.
1 l
27 I l l l ;
6.0 REFERENCES
CITED Arnold, J. R. and H. A. Al-Salih.1955. Beryllium-7 Produced by Cosmic Rays. Science 121:
451-453.
I Eisenbud, M.1963. Environmental Radioactivity, McGraw-Hill, New York, New York, pp.
213,275 and 276.
Gold, S., H. W. Barkhau, B. Shlein, and B. Kahn,1964. Measurement of Naturally Occurring Radionuclides in Air, in the Natural Environment, University of Chicago Press, Chicago, Illinois, 369-382.
Hazleton Environmental Sciences .1981. Environmental Radiation Monitoring for the Duane Arnold Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January - December 1980.
Hazleton Environmental Sciences .1982. Environmental Radiation . Monitoring for the Duane Arnold Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January - December 1981 Hazleton Environmental Sciences .1983. Environmental Radiation Monitoring for the Duane Arnold Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, i January - December 1982.
i Hohenemser, C. M. Deicher, A. Ernst, H. Hofsass, G. Lindner, E. Racknagel. 1986.
l "Chernobyl," Chemtech. October 1986, pp. 596-605.
National Center for Radiological Health,1968. Radiological Health and Data Reports, Vol. 9, Number 12, 730-746.
l Teledyne Isotopes Midwest Laboratory.1995. Quality Control Program, Revision 0.
20 July 1995.
l 1
Teledyne isotopes Midwest Laboratory.1994. Quality Control Procedures Manual, Revision 18. 27 September 1994.
Teledyne Isotopes Midwest Laboratory.1992. Quality Assurance Program Manual, Revision 1, 20 August 1992.
Teledyne Brown Engineering Environmental Services, Midwest Laboratory. 1984 - 1998.
Environmental Radiological Monitoring Program for the Duane Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January - December,1983 -
1997.
Wilson, D. W., G. M. Ward and J. E. Johnson.1969. In Environmental Contamination by Radioactive Materials, International Atomic Energy Agency. p.125.
28 i
l APPENDIX A INTERLABORATORY COMPARISON PROGRAM RESULTS NOTE: Teledyne's Midwest Laboratory participates in intercomparison studies administered by U.S. EPA Environmental Monitoring Systems Laboratory, Las Vegas, Nevada. The results are reported in Appendix A. Also reported are results of International Intercomparison and Teledyne testing of TLD's, as well as, in-house spikes, blanks, duplicates and mixed analyte performance evaluation program results. Appendix A is updated four times a year; the complete Appendix is included in March, June, September and December monthly progress reports only.
= January,1997 through December,1997
(
l Accendix A l
Interlaboratory Comparison Procram Results i l
\ l Teledyne Brown Engineering Environmental Services Midwest Laboratory (formerly Hazleton i l Environmental Sciences) has participated in interlaboratory comparison (crosscheck) programs since the .
formulation of it's quality control program in December 1971. These programs are operated by agencies which supply environmental type samples (e.g., milk or water) containing concentrations of radionuclides known to the issuing agency but not to participant laboratories. The purpose of such a program is to 1 l provide an independent check on the laboratory's analytical procedures and to alert it to any po>sible l problems.
Participant laboratories measure the concentration of .pecified radionuclides and report them to the issuing agency. Several months later, the agency reports the known values to the participant laboratories and specifies control limits. Results consistently higher or lower than the known values or outside the control limits indicate a need to check the instruments or procedures used.
The results in Table A-1 were obtained through participation in the environmental sample crosscheck program for milk, water and air filters during the past twelve months. Data for previous years is available upon request.
This program is conducted by the U.S. Environmental Protection Agency Office of Research and Developement National Exposure Research Laboratory Characterization Research Division-Las Vegas, ,
l Nevada. i i 1 The results in Table A-2 were obtained for Thermoluminescent Dosimeters (TLDs), via various l International Intercomparisons of Environmental Dosimeters under the sponsorships listed in Table A-2.
l Also Teledyne testing results are listed.
Table A-3 lists results of the analyses on in-house " spiked" samples for the past twelve months. All j samples are prepared using NIST traceable sources. Data for previous years available upon request.
Table A-4 lists results of the analyses on in-house " blank" samples for the past twelve months. Data for previous years available upon request.
i l Table A-5 list results of the in-house " duplicate" program for the past twelve months. Acceptance is based on the difference of the results being less than the sum of the errors. Data for previous years available upon request.
The results in Table A 6 were obtained through participation in the mixed analyte performance evaluation program.
The results in Table A 7 were obtained through participation in the Environmental Measurement Laboratory Quality Assessment Program.
Attachment A lists acceptance criteria for " spiked" samples.
Out-of-limit results are explained directly below the result. .
Al 1
l l
12 31-97 ATTACHMENT A ACCEPTANCE CRITERIA FOR " SPIKED" SAMPLES LABORATORY PRECISION: ONE STANDARD DEVIATION VALUES FOR VARIOUS ANALYSES' One Standard Deviation Analysis Level for single determinations Gamma Emitters 5 to 100 pCi/ liter or kg 5.0 pCi/ liter
>100 pCi/ liter or kg 5% of known value 6
Strontium-89 5 to 50 pCi/ liter or kg 5.0 pCi/ liter
>50 pCi/ liter or kg 10% of known value 6
Strontium 90 2 to 30 pCi/ liter or kg 5.0 pCi/ liter
>30 pCi/ liter or kg 10% of known value Potassium-40 >0.1 g/ liter or kg 5% of known value Gross alpha s20 pCi/ liter 5.0 pCi/ liter
>20 pCi/ liter 25% of known value Gross beta $100 pCi/ liter 5.0 pCi/ liter i >100 pCi/ liter 5% of known value Tritium s4,000 pCi/ liter is = (pCi/ liter) =
169.85 x (known)*"
>4,000 pCi/ liter 10% of known value Radium 226,-228 <0.1 pCi/ liter 15% of known value Plutonium 0.1 pCi/ liter, gram, or sample 10% of known value Iodine-131, s55 pCi/ liter 6.0 pCi/ liter Iodine-129 6 >55 pCi/ liter 10% of known value Uranium 238, s35 pCi/ liter 6.0 pCi/ liter Nickel-63 6 >35 pCi/ liter 15% of known value 6
Technetium-99 Iron-55, 50 to 100 pCi/ liter 10 pCi/ liter
>100 pCi/ liter 10% of known value Others -
20% of known value
' From EPA publication, " Environmental Radioactivity Laboratory Intercomparison Studies Program, Fiscal Year,1981-1982, EPA-600/4-81-004.
- Teledyne limit.
A2
Table A-1. U.S. Environmental Protection Agency's crosscheck program, comparison of EPA and Teledyne's Midwest Laboratory results'.
Concentration in pCi/L' Lab Sample Date Teledyne Results EPA Result' Control Code Type Collected Analysis 2 Sigma' 1s, N=1 Limits STW-782 WATER Jan,1997 Sr-89 9.7 0.6 12.0 5.0 3.3 - 20.7 STW-782 WATER Jan,1997 Sr-90 24.0 1.0 25.0 5.0 16.3 - 33.7 STW-783 WATER Jan,1997 Gr. A1pha 10.0 1.4 5.2 5.0 0.0 - 13.9 STW-783 WATER Jan,1997 Gr. Beta 15.8 2.0 14.7 5.0 6.0 - 23.4 STW-784 WATER Feb,1997 I-131 86.0 2.0 86.0 9.0 70.4 - 101.6 STW-784 WATER Feb,1997 I-131 79.3 2.0 86.0 9.0 70.4 - 101.6 STWW-786 WATER Feb,1997 Ra-226 6.710.2 5.9 0.9 4.3 - 7.5 STWW-786 WATER Feb,1997 Ra-228 8.4 i l.1 8.2 2.1 4.6 - 11.8 STWW-786 WATER Feb,1997 Uranium 26.5 1.3 27.0 3.0 21.8 - 32.3 STW-787 WATER Mar,1997 H-3 7,594.0 279.7 7,900.0 790.0 6,529.4 - 9,270.6 STW-794 WATER Apr,1997 Gr. Alpha 44.3 1.6 48.0 12.0 27.2 - 68.8 STW-794 WATER Apr,1997 Ra 226 10.710.9 13.0 2.0 9.5 - 16.5 STW-794 WATER Apr,1997 Ra-228 4.7 0.4 3.110.8 1.7 - 4.5 All raw data and cakulations were reviewed for errors. The analysis was repeated with the technician observed by the lab supervisor; the result of the reanalysis 3.li0.5 pCi/L. The suspected cause of the higher result was the lower than expected recovery of barium tracer. No further action is planned at this time.
STW-794 WATER Apr,1997 Uranium 26.8 i 0.3 24.0 3.0 18.8 - 29.2 STW-795 WATER Apr,1997 Co-60 21.7 i 0.6 21.0 5.0 12.3 - 29.7 STW-795 WATER Apr,1997 Cs-134 27.311.2 31.0 5.0 22.3 - 39.7 STW-795 WATER Apr,1997 Cs-137 21.7i l.5 22.015.0 13.3 - 30.7 STW-795 WATER Apr,1997 Gr. Beta 98.2 2.1 102.1 15.3 75.6 - 128.6 STW-795 WATER Apr,1997 Sr-89 21.3 1.2 24.0 5.0 15.3 - 32.7 STW-795 WATER Apr,1997 Sr-90 12.7 0.6 13.0 5.0 4.3 - 21.7 STW-796 WATER Jun,1997 Ba-133 24.711.2 25.0 5.0 16.3 - 33.7 STW-796 WATER Jun,1997 Co-60 18.7 0.6 18.0 5.0 9.3 26.7 STW-796 WATER Jun,1997 Cs-134 19.7 0.6 22.0 5.0 13.3 - 30.7 STW-796 WATER Jun,1997 Cs-137 52.0 i 2.0 49.0 5.0 40.3 - 57.7 STW-796 WATER Jun,1997 Zn-65 101.0 2.0 100.0 1 10.0 82.7 - 117.3 STW-797 WATER Jun,1997 Ra 226 2.7 0.1 3.0 0.5 2.1 - 3.9 STW-797 WATER Jun,1997 Ra-228 2.3 0.3 3.1 0.8 1.7 - 4.5 l STW-797 WATER Jun,1997 Uranium 38.lil.0 40.3 4.0 33.4 - 47.2 STW-799 WATER Jul,1997 Sr-89 37.7 3.2 44.0 5.0 35.3 - 52.7
- STW 799 WATER Jul,1997 Sr-90 16.0 1.0 16.015.0 7.3 - 24.7 l STW-802 WATER Jul,1997 I-131 10.7 i 1.2 10.0 6.0 0.0 - 20.4 STW 800 WATER Jul,1997 Gr. Alpha 3.1 0.3 3.1 5.0 0.0 - 11.8 STW-800 WATER Jul,1997 Gr. Deta 13.9 0.2 15.1 5.0 6.4 - 23.8 STW-801 WATER Aug,1997 H-3 11,348.7 1 241.4 11,010.0 1 1,101.0 9,099.8 - 12.920.2 STW-803 WATER Sep,1997 Ra-226 20.010.8 20.0 3.0 14.8 - 25.2 l
Al-1
1 Table A 1. U.S. Environmental Protection Agency's crosscheck program, comparison of EPA and Teledyne's Midwest Laboratory results'.
6 Concentration in pCi/L d
Lab' Sample Date Teledyne Results EPA Result Control Code Type Collected Analysis 2 Sigma
- 1s, N=1 Limits STW-803 WATER Sep,1997 Ra-228 7.0 i 0.1 8.0 2.0 4.5 11.5 STW-803 WATER Sep,1997 Uranium 5.0 0.1 5.1 3,0 0.0 - 10.3 STW-811 WATER Nov,1997 Ba-133 97.3 5.0 99.0 10.0 81.7 - 116.3 STW-811 WATER Nov,1997 Co-60 28.3 t l.7 27.0 5.0 18.3 - 35.7 STW-811 WATER Nov,1997 Cs-134 9.7 1.0 10.015.0 1.3 18.7 STW-811 WATER Nov,1997 Cs-137 78.0 i 3.5 74.0 5.0 65.3 82.7 STW-811 WATER Nov,1997 Zn-65 76.7 2.1 75.018.0 61.1 - 88.9
- Results obtained by Teledyne Brown Engineering Environmental Services Midwest Laboratory as a participant in the environmental sample crosscheck program operated by the Intercomparisen and Calibration Section, Quality Assurance Branch, Environmental Monitoring and Support Laboratory, U.S.
Environmental Protection Agency (EPA), Las Vegas, Nevada.
- All results are in pCi/L, except for elemental potassium (K) data in milk, which are in mg/L; air filter l samples, which are in pCi/ Filter.
- Unless otherwise indicated, the TBEESML results are given as the mean 2 standard deviations for three determinations.
d USEPA results are presented as the known values and expected laboratory precision (1s,1 determination) and control limits as defined by the EPA.
i i
Al 2
Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (TLDs),
mR Lab Teledyne Results Known Average 12 Sigma Code TLD Type Date Measurement i 2 Sigma Value (All Participants) 2nd International Intercomoarison 115-2 CaF : Mn Bulb Apr,1976 2 Field 17.011.9 17.1 16.4 7.7 115-2 CaF2 : Mn Bulb Apr,1976 Lab 20.8 4.1 21.3 18.8 7.6 Second InternationalIntercomparison of Environmental Dosimeters conducted in April of 1976 by the Health and Safety Laboratory (HASL), New York, new York, and the School of Public Health of the University of Texas, Houston, Texas.
3rd International Intercomoarison 115-3 CaF2 : Mn Bulb Jun,1977 Field 30.7 i 3.2 34.9 i 4.8 31.5 3.0 115-3 CaF2 : Mn Bulb Jun,1977 Lab 89.616.4 91.7114.6 86.2 24.0 Third International Intercomparison of Environmental Dosimeters conducted in the summer of 1977 by Oak Ridge National Laboratory and the School of Public Health of the University of Texas, Houston, Texas.
4th International Intercomoarison 115-4 CaF2 : Mn Bulb Jun,1979 Field 14.lil.1 14.1 1.4 16.0 i 9.0 115-4 CaF2 : Mn Bulb Jun,1979 Lab, High 40.4 i 1.4 45.8 i 9.2 43.9113.2 115-4 CaF2 : Mn Bulb Jun,1979 Lab, Low 9.8i1.3 12.2 i 2.4 12.0 7.4 Fourth International Intercomparison of Environmental Dosimeters conducted in the summer of 1979 by the School of Public Health of the University of Texas, Houston, Texas.
5th International Intercomoarison 115-5A CaF2 : Mn Bulb Oct,1980 Field 31.4 i l.8 30.016.0 30.2 14.6 115-5A CaF2 : Mn Bulb Oct,1980 Lab,End 96.6 i 5.8 88.4 i 8.8 90.7 31.2 115-5A CaF2 : Mn Bulb Oct,1980 Lab, Start 77.4 i 5.8 75.217.6 75.8 40.4 Fifth International Intercomparison of Environmental Dosimeters conducted in the fall of 1980 at Idaho Falls, Idaho and sponsored by the School of Public Health of the University of Texas, Houston, Texas and the Environmental Measurements Laboratory, New York, New York, U.S. Department of Energy.
5th International Intercomoarison 115-5B LiF-100 Chips Oct,1980 Field 30.3 4.8 30.0 i 6.0 30.2 14.6 115-5B LiF-100 Chips Oct,1980 Lab,End 85.4 i 11.7 88.4 i 8.8 90.7 31.2 115-5B LiF-100 Chips Oct,1980 Lab, Start 81.1 i 7.4 75.2 i 7.6 75.8 40.4 Fifth International Intercomparison of Environmental Dosimeters conducted in the fall of 1980 at Idaho Falls, Idaho and sponsored by the School of Public Health of the University of Texas, Houston, Texas and the Environmental Measurements Laboratory, New York, New York, U.S. Department of Energy.
6th International Intercomoarison 115-6 Teledyne did not participate in the Sixth International Intercomparison of Environmental Dosimeters.
Zth International Intercomoarison 115-7A LiF-100 Chips Jun,1984 Fie1d 75.4 i 2.6 75.8 i 6.0 75.1 29.8 115-7A LiF-100 Chips Jun,1984 Lab, Co-60 80.0 i 3.5 79.9 i 4.0 77.9 i 27.6 115-7A LiF-100 Chips Jun,1984 Lab, Cs-137 66.6 i 2.5 75.0 i 3.8 73.0 22.2 i
A21 i
L l
)
i Table A-2. Crosscheck program results; Thermoluminescent Dosimeters. (TLDs).
mR
' Lab Teledyne Results Knmvn Average 2 Sigma Code TLD Type Date - Measurement f 2 Sigma Value (All Participants)
Seventh International Intercomparison of Environmental Dosimeters conducted in the spring and summer of 1984 at Las Vegas, Nevada, and sponsored by the U.S. Department of Energy, The Nuclear Regulatory Commission, and the U.S. Environmental Protection Agency.
7th International Intercomoarison
- l. 115-7B LiF-100 Chips Jun,1984 FieId - 71.5 i 2.6 75.816.0 75.1 29.8 115-7B LiF-100 Chips Jun,1984 Lab, Co-60 84.8 i 6.4' 79.9 4.0 77.9 27.6 l 115-7B LiF-100 Chips Jun,1984 Lab, Cs-137 78.8 i 1.6 75.0 t 3.8 73.0122.2 Seventh InternationalIntercomparison of Environmental Dosimeters conducted in the spring and summer of
!. 1984 at Las Vegas, Nevada, and sponsored by the U.S. Department of Energy, The Nuclear Regulatory j Commission, and the U.S. Environmental Protection Agency.
l 7th International Intercomoarison 1
115-7C CaSO.: Dy Jun,1964 Field 76.8 i 2.7 75.8 6.0 75.1 29.8 l Cards
, 115-7C CaSO.: Dy Jun,1964 Lab, Co-60 82.5 i 3.7 79.9 i 4.0 77.9 i 27.6 Cards f
115-7C CaSO.: Dy Jun,1964 Lab, Cs-137 l
79.023.2 75.013.8 73.0 t 22.2 ]
Cards Seventh International Intercomparison of Environmental Dosimeters conducted in the spring and summer of
' 1984 at Las Vegas, Nevada, and sponsored by the U.S. Department of Energy, The Nuclear Regulatory l Comnussion, and the U.S. Environmental Protection Agency. ]
8th International Intercomoarison l 115-8A LiF-100 Chips Jan,1986 Field, Site 1 29.5 1.4 29.711.5 28.9112.4 115-8A . LiF-100 Chips Jan,1986 Field, Site 2 11.310.8 10.410.5 10.119.1 I 115-8A LiF-100 Chips Jan,1986 Lab, Cs-137 13.7 i 0.9 17.210.9 16.2 i 6.8 Eighth InternationalIntercomparison of Environmental Dosimeters conducted in the fall and winter of 1985-1986 at New York, New York, and sponsored by the U.S. Department of Energy.
8th International Intercom _c arison 115-8B LiF-100 Chips Jan,1986 Field, Site 1 32.3 t l.2 29.7 1.5 28.9 12.4 115-8B LiF-100 Chips Jan,1986 Field, Site 2 9.0 1.0 10.410.5 10.1 i 9.0 115-8B . LiF-100 Chips Jan,1986 Lab, Cs-137 15.8 i 0.9 17.2 i 0.9 16.2 6.8
- i. Eighth International Intercomparison of Environmental Dosimeters conducted in the fall and winter of ,
1985-1986 at New York, New York, and sponsored by the U.S. Department of Energy. '
8th International Intercornnarison 115-8C ' CaSO : Dy Jan,1986 Field, Site 1 32.2 i 0.7 29.7 i 1.5 28.9 12.4 Cards 115-8C - CaSO.: Dy Jan,1986 Field, Site 2 10.610.6 10.410.5 10.1 9.0 Cards i 115-8C - CaSO.: Dy Jan,1986 Lab, Cs-137 18.110.8 17.2 i 0.9 16.2 6.8 Cards l
A2-2
Table A-2. Crosscheck program results; Thermoluminescent Dosimeters. (TLDs).
mR Lab Teledyne Results Known Average 2 Sigma C(xle TLD Type Date Measurement i 2 Sigma Value (All Participants)
Eighth International Intercomparison of Environmental Dosimeters conducted in the fall and winter of 1985-1986 at New York, New York, and sponsored by the U.S. Department of Energy.
9th International Intercomoarison 115-9 The Ninth International Intercomparison of Environmental Dosimeters was not available to Teledyne's Midwest Laboratory.
10th International Intercornoarison 115-10A LiF-100 Chips Aug,1993 Field 25.7 1.4 27.011.6 26.4 10.2 113-10A LiF-100 Chips Aug,1993 Lab,1 22.7 t 1.6 25.911.3 25.0 9.4 115-10A LiF-100 Chips Aug,1993 Lab,2 62.712.6 72.7 1.9 69.8 20.3 The Tenth International Intercor.parison of Environmental Dosimeters conducted in 1993 at Idaho State University and sponsored by the U.S. Department of Energy and the Idaho State University.
10th International Intercomoarison 115-10B CaSO.: Dy Aug,1993 Fie1d 26.0 i 2.3 27.0 i 1.6 26.4 10.2 Cards 115-10B CaSO4 : Dy Aug,1993 Lab,1 24.1 i 1.7 25.9 i 1.3 25.0 9.4 Cards 115-10B CaSO4 : Dy Aug,1993 Lab,2 69.213.0 72.7 1.9 69.8 20.3 Cards l
The Tenth International Intercomparison of Environmental Dosimeters conducted in 1993 at Idaho State University and sponsored by the U.S. Department of Energy and the Idaho State University. .
lith International Intercomparison !
115-11 Apr,1997 f
'Ihe Eleventh International Intercomparison of Environmental Dosimeters was conducted in 1997 and was I organized by the Department of Energy's Environmental Measurements Laboratory in collaboration with Brookhaven National Laboratory and the NationalInstitute of Standards and Technology.
Results for the Eleventh InternationalIntercomparison were originally reported in error; The results are being re-evaluated and will be reported in a later update. l Teledyne Testing 89-1 LiF-100 Chips Sep,1989 Lab 2' ei 0.4 22.4 ND ND = No Data; Teledyne Testing was o ily performed by Teledyne.
l Chips were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in September,1989.
Teledvne Testing 89-2 CaSO.: Dy Nov,1989 Lab 20.9 1.0 20.3 ND Cards l
ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in June,1990.
i A2-3
Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (TLDs).
mR Lab Teledyne Results Known Average 2 Sigma Code TLD Type Date Measurement i 2 Sigma Value (All Participants)
Teledyne Testing 90-1 CaSO.: Dy Jun,1990 Lib 20.6 i 1.4 19.6 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in June,1990.
Teledyne Testing 90-2 CaSO.: Dy Jun,1990 Lab 100.814.3 100.0 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards were irradiated by Dosimetry Asssociates, Inc., Northville, MI, in October,1990.
Teledyne Testing 91-1 CaSO.: Dy Oct,1990 Lab,1 33.412.0 32.0 ND Cards 91-1 CaSO : Dy Oct,1990 Lab,2 55.2 i 4.7 58.8 ND Cards 91-1 CaSO : Dy Oct,1990 Lab,3 87.8 6.2 85.5 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in October,1991.
Teledyne Testing 92-1 LiF-100 Chips Feb,1992 Lab,1 11.110.2 10.7 ND 92-1 LiF-100 Chips Feb,1992 Izb,2 25.610.5 25.4 ND 92-1 LiF-100 Chips Feb,1992 Lab,3 46.410.5 46.3 ND ND = No Data; Teledyne Testing was only performed by Teledyne.
Chips were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in February,1992.
Ieledyne Testing 92-2 CaSO.: Dy Apr,1992 Reader 1, #1 20.1 i 0.1 20.1 ND Cards 92 2 CaSO.: Dy Apr,1992 Reader 1, #2 40.6i 0.1 40.0 ND Cards 92 2 CaSO.: Dy Apr,1992 Reader 1, #3 60.0il.3 60.3 ND Cards 92-2 CaSO.: Dy Apr,1992 Reader 2, #1 20.310.3 20.1 ND Cards 92-2 CaSO.: Dy .Apr,1992 Reader 2, #2 39.210.3 40.0 ND Cards 92-2 CaSO : Dy Apr,1992 Reader 2, #3 60.7 i 0.4 60.3 ND Cards A2-4
Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (~.L.Ds).
mR Lab Teledyne Results Known Average 2 Sigma Cw TLD Type Date Measurement 2 Sigma Value (All Participants)
ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards were irradiated by Teledyne isotopes,Inc., Westwood, New Jersey, in April,1992.
Teledvne Testing 93-1. Teledyne Mar,1993 Lab,1 10.0il.0 10.2 ND LiF-100 Chips 93-1 Teledyne Mar,1993 Lab,2 25.212.2 25.5 ND LiF-100 Chips 93-1 Teledyne Mar,1993 Lab,3 42.7 i 5.7 45.9 ND LiF-100 Chips ND = No Data; Teledyne Testing was only performed by Teledyne.
Chips were irradiated by Teledyne Isotopes,Inc., Westwood, New Jersey, in March,1993. Due to a potential error of 10-12% when cards where irradiated, results of the testing on the cards will not be published. Data is available upon request.
Teledyne Testing 94-1 Teledyne Nov,1994 Lab,1 15.6 i 0.4 14.9 ND LiF-100 Chips 94-1 Teledyne Nov,1994 Lab,2 30.2 i 0.4 29.8 ND LIF-100 Chips 94-1 Teledyne Nov,1994 Lab,3 59.2 i 0.3 59.7 ND LiF-100 Chips 94-1 CaSO : Dy Nov,1994 Reader 1, #1 14.9 i 0.1 14.9 ND Cards 94-1 CaSO.: Dy Nov,1994 Reader 1, #2 30.8 i 0.1 29.8 ND Cards 94-1 . CaSO.: Dy Nov,1994 Reader 1, #3 58.910.3 59.7 ND Cards 94-1 CaSO.: Dy Nov,1994 Reader 2, #1 15.4 i 0.2 14.9 ND Cards 94 1 CaSO.: Dy Nov,1994 Reader 2, #2 31.4 i 0.2 29.8 ND Cards 94 1 CaSO : Dy Nov,1994 Reader 2, #3 60.1 0.3 59.7 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in November,1994.
Teledvne Testing 95-1 LiF-100 Chips Mar,1995 Lab,1 16.1 i 0.2 15.7
'95-1 LiF-100 Chips Mar,1995 Lab,2 31.710.1 32.3 95-1 LiF-100 Chips Mar,1995 Lab,3 59.7 i 0.6 60.8 95-1 CaSO.: Dy Mar,1995 Reader 1, #1 16.410.1 15.7 ND Cards A2-5
i Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (TLDs).
mR Lab Teledyne Results Known Average 2 Sigma Code TLD Type Date Measurement
- 2 Sigma Value (All Participants) 95-1 CaSO.: Dy Mar,1995 Reader 1, #2 34.910.1 32.3 ND Cards 95-1 CaSO.: Dy Mar,1995 Reader 1, #3 64.4 1.5 60.8 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards and Chips were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in March,1995.
Teledene Testing 95-2 CaSO4 : Dy Mar,1995 Reader 2, #1 16.4 i 0.2 15.7 ND Cards 95-2 CaSO.: Dy Mar,1995 Reader 2, #2 33.9 i 0.4 32.3 ND Cards 95-2 CaSO : Dy Mar,1995 Reader 2, #3 60.5 i 0.3 60.8 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Cards and Chips were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in March,1995.
Teledyne Testing 96-1 LiF-100 Chips Mar,19% Lab,1 15.910.3 15.4 96-1 LiF 100 Chips Mar,1996 Lab,2 29.4 i 0.3 30.8 96-1 LiF-100 Chips Mar,1996 Lab,3 62.511.3 62.5 96-1 CaSO.: Dy Mar,1996 Reader 1, #1 14.4 i 0.1 15.4 ND Cards 96-1 CaSO : Dy Mar,1996 Reader 1, #2 31.8 i 0.1 30.8 ND Cards 96-1 CaSO.: Dy Mar,1996 Reader 1, #3 64.710.4 62.5 ND Cards Teledvne Testing 96-2 CaSO.: Dy Mar,1996 Reader 2, #1 14.3 i 0.4 15.4 ND Cards 96-2 CaSO.: Dy Mar,1996 Reader 2, #2 31.810.1 30.8 ND Cards 96 2 CaSO.: Dy Mar,1996 Reader 2, #3 68.610.1 62.5 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.
Chips and Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in March,1996.
! Teledvne Testing 97-1 LiF-100 Chips Mar,1997 Lab,1 13.4 i 1.4 15.0 97-1 LiF-100 Chips Mar,1997 Lab,2 29.8 i 0.6 30.1 97-1 LiF-100 Chips Mar,1997 Lab,3 63.4 i 0.9 60.2 A2-6 L
Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (TLDs).
mR Lab Teledyne Results Known Average 2 Sigma Code TLD Type Date Measurement t 2 Sigma Value (A11 Participants) 97-1 CaSO : Dy Mar,1997 Reader 1, #1 15.510.1 15.0 ND Cards 97-1 CaSO.: Dy Mar,1997 Reader 1, #2 34.010.1 - 30.1 ND Cards 97-1 CaSO.: Dy Mar,1997 Reader 1, #3 68.3 i 2.1 60.2 ND Cards Teledyne Testing 97-2 CaSO.: Dy Mar,1997 Reader 2, #1 16.8 i 0.3 15.0 ND Cards 97-2 CaSO.: Dy Mar,1997 Rer. der 2, #2 36.210.2 30.1 ND Cards 97-2 CaSO.: Dy Mar,1997 Reader 2, #3 69.610.2 60.2 ND Cards ND = No Data; Teledyne Testing was c,nly performed by Teledyne.
Chips and Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in March,1997.
1 A2-7
Table A 3. In-house " spike" samples.
Concentration in pCi/L' Lab Sample Date Teledyne Results Code Known Controf Type Collected Analysis 2s, n=1' Activity Limits SPW 844 WATER Jan,1997 Th 230 3.120 0.104 3.070 1.842 - 4.29s SPW 844 WATER Jan,1997 Th-232 3.355 0.108 3.070 1.842 - 4.298 SPW-548 WATER Feb,1997 Gr. Beta 43.881 1.305 41.860 31.860 - 51.860 SPM1534 MILK Feb,1997 Cs-134 48.649 1 4.940 56.400 46.400 - 66.400 SPMI 534 MILK Feb,1997 Cs-137- 54.700 8.450 52.300 42.300 - 62.300 SPM1-535 MILK Feb,1997 Sr-89 49.849 7.940 40.030 30.030 - 50.030 SPMI-535 MILK Feb,1997 Sr-90 48.856 1.740 50.300 40.240 60.360 SPW 536 : WATER Feb,1997 H3 27229.744 452.056 28234.000 22587.200 - 33SSO.800 SPW 547 WATER Feb,1997 Co-60 65.219 8.790 62.950 52.950 72.950 SPW-547 - WATER Feb,1997 Cs-134 52.996 8.000 56.430 46.430 - 66.430 SPW-547 WATER Feb,1997 Cs-137 60.419 12.900 52.320 42.320 - 62.320 SPW-600 WATER - Feb,1997 I131 72.182 1.009 66.300 53.040 - 79.560
- SPW-600 WATER Feb,1997 I-131(g) 68.816 14.800 66.300 39.780 - 76.300 SPCH-701 CH AL Feb,1997 1131(g) 1.171 1 0.023 1.080 0.648 - 1.512 SPAP 704 AIR FILTER Feb,1997 Gr. Beta 6.302 i 0.041 5.740 0.000 - 15.740 SPW-838 WATER Feb,1997 Ra-226 19.770 i 0.189 17.300 12.110 - 22.490 SPW-838 WATER Feb,1997 Ra-228 36.784 t 2.571 31.300 21.910 - 40.690 SPW-840 WATER Feb,1997 Sr-90 35.822 i 2.020 33.520 26.816 - 40.224 SPW-841 WATER Feb,1997 I 129 15.525 0.854 14.942 2.942 - 26.942 SPW-843 WATER Feb,1997 Fe-55 1.418 0.530 1.535 0.000 - 21.535 SPAP-2730 AIR FILTER Mar,1997 Cs-137 2.151 i 0.025 1.900
' 1.140- 2.660 SPMI-1670 MILK Apr,1997 Cs-134 50.282 8.920 53.600 43.600 - 63.600 SPMI 1670 MILK- Apr,1997 Cs-137 56.090 1 14.900 52.100 42.100 - 62.100 SPW-2073 WATER Apr,1997 Co-60 ' 54.077 1 4.280 51.300 41.300 - 61.300 SPW-2073 WATER Apr,1997 Cs-134 47.636 4.150 53.200 43.200 63.200 SPW-2073 WATER Apr,1997 Cs-137 60.688 5.760 52.100 42.100 62.100
- ~ SPW 2075 WATER Apr,1997 Gr. Alpha 34.554 2.677 41.300 20.650 - 61.950 SPW-2075 WATER Apt,1997 Gr. Beta 38.729 i 1.658 41.700 31.700 - 51.700 SPW 2546 WATER Apr,1997 H-3 25445.478 1 428.384 26257.000 21005.600 - 31508.400 SPF-3434 FISH May,1997 Cs-134 0.199 i 0.020 0.222 0.133 - 0.311 SPF-3434 FISH ' May,1997 Cs-137 0.234 i 0.037 0.227 0.136- 0.318
- l. SPW-3750 WATER Jun,1997 I-131 76.174 i 0.776 71.800 57.440 - 86.160
! .' SPW-3750 - WATER Jun,1997 I-131(g) 66.587 8.750 71.800 43.080 - 81.800 SPMI 3752 MILK Jun,1997 I-131 79.851 1 0.833 71.800 57.440- 86.160
. SPMI 3752 - MILK Jun,1997 I-131(g) 78.887 i 7.750 71.800 43.080 - 81.800 i' CHARCOAL SPCH-3754 Jun,1997 I-131(g) 81.869 0.317 76.600 45.960 - 86.600 l CANISTER I
SPMI-4216 MILK Jul,1997 Cs-134 38.265 5.450 39.500 29.500 - 49.500 SPMI-4216 MILK - Jul,1997 Cs-137 46.472 i 10.600 41.500 31.500 51.500 SPM1-4216 M1LK Jul,1997 I131 75.247 1 0.831 83.230 66.584 - 99.876 SPMI-4216 MILK Jul,1997 1-131(g) 84.872 i 7.010 83.230 49.938 - 93.230 A3-1
l- Table A-3. In-house " spike" samples.
l Concentration in pCi/ L' l Lab Sample Date Teledyne Results Known Control' Code Type Collected Analysis 2s, n=1' Activity Limits SPMI-4216 MILK Jul,1997 Sr-90 33.610 1 1.430 33.210 26.568 - 39.852 SPW-4420 WATER Jul,1997 Co-60 26.270 i 4.360 24.900 14.900 - 34.900 SPW-4420 WATER Jul,1997 Cs-134 36.591 1 5.040 39.540 29.540 - 49.540 SPW-4420 WATER Jul,1997 Cs-137 45.552 i 7.770 41.480 31.480 - 51.480 l SPW-4420 WATER Jul,1997 1131(g) 85.221 1 9.660 83.230 49.938 - 93.230 l SPW-4420 WATER Jul,1997 Sr-90 36.285 i 1.629 33.210 26.568 - 39.852 SPMI-4916 MILK Jul,1997 Cs-134 38.260 i 5.450 39.540 29.540 - 49.540 SPMl-4916 MILK Jul,1997 Cs-137 46.470 10.600 41.480 31.480 - 51.480 SPMI-4916 MILK Jul,1997 I-131(g) 84.870 1 7.010 83.230 49.938 - 93.230 SPW-5470 WATER Jul,1997 Fe-55 4.548 1 0.640 5.477 0.000 - 25.477 SPW-5472 WATER Jul,1997 H-3 41026.000 329.000 41578.000 33262.400 - 49893.600 SPW-5474 WATER Jul,1997 Gr. Alpha 49.266 1 2.081 41.305 20.653 - 61.958
- SPW-5474 WATER Jul,1997 Gr. Beta 44.450 i 1.334 41.406 31.406 - 51.406 SPF-5476 FISH Jul,1997 Cs-134 0.641 1 0.030 0.700 0.420 - 0.980 SPF-5476 FI5H Jul,1997 Cs-137 0.632 i 0.042 0.527 0.316 - 0.738 SPW-7500 WATER Oct,1997 Co-60 30.424 i 7.530 33.642 23.642 - 43.642 l SPW-7500 WATER Oct,1997 Cs-134 37.410 1 6.690 36.086 26.086 46.086 SPW-7500 WATER Oct,1997 Cs-137 52.845 1 11.300 41.221 31.221 - 51.221 The Cs-137 spike is suspect. No errors were found in the spectroscopy program and the Cs-134 and Co-60 test results on the same sample were very good. Sample results prepared with the new standard were 4 acceptable and will be reported in the next update of Appendix A. )
SPW-7500 WATER Oct,1997 I-131 78.126 i l.201 78.302 62.642 - 93.962 SPMI 7505 MILK Oct,1997 Cs-134 15.166 1 3.250 18.043 8.043 - 28.043 I
SPMI-7505 MILK Oct,1997 Cs-137 91.110 i 8.370 82.440 72.440 - 92.440 SPMI-7505 MILK Oct,1997 I-131 73.529 1 1.253 78.302 62.642 - 93.962 SPMI-7505 MILK Oct,1997 I131(g) 74.613 i 8.810 78.302 46.981 - 88.302 l
SPMI-7506 MILK Oct,1997 Sr-89 31.281 i 4.601 39.490 29.490 - 49.490 l SPMI-7506 MILK Oct,1997 Sr-90 31.545 i 1.388 32.990 26.392 - 39.588 SPCH-7727 CH AL Oct,1997 I-131(g) 0.450 1 0.050 0.440 0.264 - 0.616 l R SPAP-7730 AIR FILTER Oct,1997 Gr. Beta 3.080 1 0.030 3.040 1.824 - 4.256 (ss)
SPF-8485 FISH Nov,1997 Cs-134 0.306 i 0.025 0.318 0.191 - 0.445 SPF-8485 FISH Nov,1997 Cs-137 0.738 i 0.049 0.649 0.389 - 0.909 SPW-9315 WATER Nov,1997 Gr. Alpha 51.420 1 6.385 41.280 20.640 - 61.920 l SPW-9315 WATER Nov,1997 Gr. Beta 48.938 i 3.735 43.164 33.164 - 53.164 l SPW-9706 WATER Dec,1997 Gr. Alpha 40.480 1 4.598 41.2bd 20.640 - 61.920 SPW-9853 WATER Dec,1997 Co-60 44.900 8.290 42.080 32.080 - 52.080 SPW-9853 WATER Dec,1997 Cs-134 40.010 1 7.010 37.850 27.850 - 47.850 l
A3-2
Table A-3. In-house " spike" samples. -
Concentration in pCi/L' Lab Sample Date Teledyne Results _Known Control' Code Type Collected Analysis 2s, n=1' Activity Limits
- All results are in pCi/L, except for elemental potassium (K) in milk, which are in mg/L.; air filter samples, which are in pCi/ Filter; and food products, which are in mg/kg.
" All samples are the results of single determinations.
- Control limits are based on Attachment A, page A2 of this report.
NOTE: For fish, Jello is used for the spike matrix. For vegetation, Sawdust is used for the spike matrix.
I i
i l
A3 3
Table A-4. In-house " blank" samples.
Concentration pCi/L'.
Teledyne Results Acceptance Lab Sample Sample (4.66 Sigma)
Code Type Date - Analysis Criteria LLD Activitv" (4.66 Sigma)
SPW-845 WATER Jan 1997 Th-228 <0.9 -0.263 0.560 <1.000 SPW-845 WATER Jan 1997 Th-230 <0.2 0.191 0.236 <1.000 SPW 845 WATER Jan 1997 Th-232 <0.2 -0.018 0.145 < 1.000 SPMl 533 MILK Feb 1997 Cs-134 <2.7 -0.531 0.647 < 10.000 SPMI-533 MILK Feb l997 Cs-137 <5.5 0.526 3.380 < 10.000 SPW-2 WATER Feb l997 Ra-226 <0.1 0.000 0.034 <1.000 SPMI 533 MILK Feb l997 I-131 <0.5 -0.031 0.316 < 0.500 SPMI-533 MILK Feb l997 Sr-89 <0. 7 -0.994 0.952 <5.000 SPMI-533 MILK Feb 1997 Sr-90 N/A 1.695 0.439 <1.000 Low level of Sr-90 concentration in milk (1-5 pCi/L) is not unusual.
SPW-537 WATER Feb l997 Co-60 <3.1 0.065 0.179 < 10.000 SPW 537 WATER Feb l997 Cs-134 <3.5 0.905 1.100 < 10.000 SPW 537 WATER Feb l997 Cs-137 < 1.7 -1.430 1.800 < 10.000 SPW-537 WATER Feb l997 Gr. Alpha <0.4 -0.109 0.218 <l.000 SPW 537 WATER Feb 1997 Gr. Beta <0.9 -0.155 0.596 < 3.200 SPW-537 WATER Feb 1997 I-131 <0.4 -0.275 0.235 < 0.500 SPW-537 WATER Feb l997 Sr-89 <0.8 -0.167 0.557 <5.000 SPW-537 WATER Feb l997 Sr-90 <0.5 0.099 0.239 <1.000 SPW-842 WATER Feb l997 Fe-55 <0.7 -0.403 0.374 < 1000.000 SPW-842 WATER Feb l997 I-129 <0. 9 -0.129 0.442 <1.500 SPW-842 WATER Febl997 Ra-226 <0.04 0.013 0.026 <1.000 SPAP-2731 AIR FILTER Mar 1997 Co-60 <2.5 0.000 0.000 < 10.000 SPAP 2731 AIR FILTER Mar 1997 Cs-134 <2.6 -0.000 0.000 < 10.000 SPAP-2731 AIR FILTER ' Mar 1997 Cs-137 <2.9 0.000 i 0.001 < 10.000 SPMI-1669 MILK Apr1997 Cs-134 <5.5 0.069 0.118 < 10.000 SPMI 1669 MILK Apr1997 Cs-137 <3.8 0.717 2.4S0 < 10.000 SPW-2074 WATER Apr1997 Co-60 <3.6 0.857 3.380 < 10.000 SPW-2074 WATER Apr1997 Cs-134 <4.7 1.610 10.200 < 10.000 SPW-2074 WATER Apr1997 Cs-137 <5.0 1.800 i 3.200 < 10.000 SPW-2074 WATER Apr1997 Gr. Alpha <0.5 0.119 0.307 <1.000 SPW-2074 WATER Apr1997 Gr. Beta <1.3 0.464 0.720 < 3.200 SPW 2547 WATER Apr1997 H-3 < 150 12.822 75.126 < 200.000 SPW-5 WATER May1997 Ra 226 <0.03 -0.053 0.025 <1.000 SPF-3435 FISH May 1997 Cs-134 <0.015 -0.014 0.002 < 10.000 SPF-3435 FISH May1997 Cs-137 <0.016 0.001 1 0.011 < 10.000 SPW-6 WATER Jun1997 Ra-226 <0.04 -0.044 i 0.027 <1.000 A4-1
Table A-4. In-house " blank" samples.
Concentration pCi/L".
Teledyne Results Acceptance Lab Sample Sample (4.66 Sigma)
Code Type Date Analysis Criteria LLD Activitv" (4.66 Siema)
SPW-3751 WATER Jun1997 I-131 <0.3
-0.127 0.145 < 0.500 SPMI-3753 MILK Jun1997 I-131 <0.3 0.089 0.167 < 0.500 SPCH-3755 CHARCOAL Jun1997 I-131(g) <0.017 0.010 0.009 < 9.600 CANISTER SPMI-4217 MILK Jul1997 Co-60 <4.8 -0.392 1.230 < 10.000 SPMI-4217 MILK Jul1997 Cs-134 <3.0 -0.874 1.700 < 10.000 SPMI-4217 MILK Jul1997 Cs-137 <5.9 1.600 3.430 < 10.000 SPMI-4217 MILK Jul1997 I-131 < 0.3 -0.049 0.171 <0.500 SPW-4421 WATER Jul1997 Co-60 < 1.9 -4.660 4.750 < 10.000 SPW-4421 WATER Jul1997 Cs-134 <4.7 -1.450 3.090 < 10.000 SPW-4421 WATER Jul1997 Cs-137 < 5.7 0.739 4.550 < 10.000 SPMI-4217 MILK Ju!1997 St 89 <1.5 -0.165 1.901 < 5.000 SPMI-4217 MILK Jul 1997 St-90 N/A 1.677 0.418 <1.000 Low level of Sr-90 concentration in milk (1-5 pCi/L) is not unusual.
SPW-4421 WATER Jul1997 Sr-89 < 1. 7 0.917 1.547 <5.000 SPW-4421 WATER Jul1997 Sr-90 <0.6 0.341 0.332 <1.000 SPW-5471 WATER Jul1997 Fe-55 <733 48.157 448.317 < 1000.000 SPW-5473 WATER Ju11997 H-3 <161 22.700 58.200 < 200.000 SPW-5475 WATER Jul1997 Gr. Alpha <0.6 0.170 0.425 <1.000 SPW-5475 WATER Jul1997 Gr. Beta <0.5 0.173 1 0.473 < 3.200 SPF-5477 FISH Jul1997 Co-60 <0.011 -0.001 0.002 < 10.000 SPF-5477 FISH Jul1997 Cs-134 <0.015 0.005 0.008 < 10.000 SPF-5477 FISH Jul1997 Cs-137 <0.018 0.006 1 0.010 < 10.000 SPW-7501 WATER Oct 1997 1131 <0.4 0.010 0.009 < 0.500 SPW-7504 WATER Oct 1997 Sr-89 <1.1 -0.650 0.800 <5.000 SPW-7504 WATER Oct 1997 Sr 90 <0.4 0.150 0.210 <1.000 SPM1-7507 MILK Oct 1997 Co-60 <6.2 -1.190 16N < 10.000 SPMI-7507 MILK Oct 1997 Cs-134 <4.9 1.710 : ; 0 0 < 10.000 l
SPMI-7507 MILK Oc.t1997 Cs 137 <6.5 -0.232 : 3.740 < 10.000 SPMI-7507 MILK Oct 1997 1-131 <0. 3 -0.022 0.157 <0.500 SPMI-7507 MILK Oct 1997 Sr-89 < 1.0 0.862 1.107 <5.000 SPMI-7507 MILK Oct 1997 Sr-90 N/A 1.031 0.319 <1.000 Low level of Sr-90 concentration in milk (1-5 pCi/L) is not unusual.
RA-W-11 WATER Dec 1997 Ra-228 <0.7 0.134 1 0.318 <1.000 SPW-9852 WATER Dec1997 Co-60 <2.4 -1.600 1 9.460 < 10.000 SPW-9852 WATER Dec1997 Cs-134 <5.7 -0.450 2.340 < 10.000 A4-2
l
(
Table A-4. - In-house " blank" samples.
?:
Concentration pCi/L".
. Lab- Teledyne Results l- Sample Sample Acceptance
! Code Type (4.66 Siema) Criteria Date Analysis LLD A ctivi t v (4.66 Sigma)
SPW-9852 . WATER Dec1997 Cs-137 <6.0 2.190 3.550 < 10.000 y ' Liquid sample results are reported in pCi/ Liter, air filter sample results are in pCi/ filte results are in pC / charcoal, and solid sample results are in pCi/ kilogram.
The activity reported is the net activity result.
l l
l I
l t
i l
l I
l l
t l
l A4-3
Table A-5. In-house " duplicate" samples.
Concentration in pCi/L' L Lab hample First Second Averaged Codes
- Date Analysis Result Result Result SW - 42,43 Jan,1997 Gr. Beta 3.0753 1 0.9097 2.5036 1 0.8819 2.7894 0.6335 MI - 63,64 Jan,1997 Co-60 0.8960 2.5500 0.8290 1.4300 0.8625 z 1.4618 MI 63,64 Jan,1997 Cs 137 0.4480 i 2.0600 0.7240 1.3800 0.5860 1.2398 MI - 19,20 Jan,1997 Co-60 2.7900 2.6200 1.4300 2.4700 2.1100 1.8004 MI - 19,20 Jan,1997 Cs-137 -0.8750 2.7600 2.3900 1.9100 0.7575 1.6782 l Mi - 92,93 Jan,1997 I-131 0.0455 0.2124 0.1031 0.2405 0.0743 : 0.1604 MI - 92,93 Jan,1997 K-40 1,466.8000 129.0000 1,417.3000 163.0000 l 1,442.0500 103.9351 i WW - 116,117 Jan,1997 I-131 0.1299 t 0.2579 -0.0824 0.2359 0.0237 0.1747 LW - 146,147 Jan,1997 Co-60 -0.1850 0.4500 1.9100 16.9000 0.8625 8.45s'0 l LW - 146,147 Jan,1997 Cs-137 -0.8360 t 2.1600 0.2350 3.4500 -0.3005 i 2.0352 l- LW - 146,147 Jan,1997 Gr. Beta 6.9782 1.4082 7.8900 1.5599 7.4341 1.0507 LW - 224,225 Jan,1997 Co-60 1.8300 t 4.2500 -1.22003 0.9290 0.3050 2.1752 LW - 224,225 Jan,1997 Cs-137 -0.9650 3.4000 1.4500 1.7100 0.2425 1.9029 LW - 224,225 Jan,1997 Gr. Beta 6.2889 1.3951 7.3610 i 1.5370 6.8250 1.0379 WW - 321,323 Jan,1997 H-3 -5.4270i B0.6586 -14.4721 i 80.2518 -9.9496 56.8906 CW - 355,3S6 Jan,1997 Gr. Beta 3.1262 i 14 281 2.0589 1.4561 i 2.5925 1.0198 i CW - 355,356 Jan,1997 Gr. Beta -0.3849 i l.2993 0.4440 i l.3725 0.0296 0.9450 CW - 299,300 Jan,1997 Gr. Beta 2.4965 t l.0877 2.7913 1.4707 2.6439 0.9146 CW - 299,300 Jan,1997 Gr. Beta 0.2070 1.3507 0.7394 i 1.39J 0.4732 0.9715 SW - 441,442 Jan,1997 Co-60 -0.2460 i 1.3100 0.3250 0.3190 0.0395 i 0.6741 SW - 441,442 Jan,1997 Cs-137 0.0619 i 2.3900 3.0200 1 2.8400 1.5410 1.8559 SWU - 389,390 Jan,1997 Gr. Beta 2.7555 1 0.5392 2.6585 t 0.5182 2.7070 0.3739 ;
SWU - 339,390 Jan,1997 H-3 158.6398 i 94.8968 125.0455 i 93.5661 141.8427 66.6333 !
MI - 377,378 Jan,1997 I-131 0.1482 i 0.2260 0.0950 0.2541 0.1216 0.1700 MI- 377,378 Jan,1997 K-40 1,379.5000 1 122.0000 1,304.8000 113.0000 1,342.1500 83.1460
! MI- 377,378 Jan,1997 Sr-89 -0.4172 1 0.8436 -0.2671 0.7827 -0.3421 0.5754 MI - 377,378 Jan,1997 Sr-90 0.9881 1 0.3785 1.0431 1 0.3340 1.0156 0.2524 CW - 416,417 Jan,1997 Gr. Beta 3.7493 i l.2558 4.5363 i 1.1489 4.1428 0.8510 CW - 416,417 Jan,1997 Gr. Beta 0.1479 i l.3455 0.6807 1.3926 0.4143 0.9682 PW - 607,608 Jan,1997 Co-60 -0.4870 1 0.6140 0.8310 2.4300 0.1720 1.2532 l
l PW - 607,608 Jan,1997 Cs-137 -0.7370 i 2.6100 0.2580 3.0900 -0.2395 2.0224 PW - 607,608 Jan,1997 Gr. Beta 5.7315 i l.8872 5.5786 1 1.7689 5.6550 1.2933 1 CW - 846, 847 Jan,1997 Cr. Alpha 0.0484 i 0.4520 0.6758 0.4786 0.3621 0.3292 <
CW - 846,847 .Jan,1997 Gr. Beta 1.3287 0.5381 2.1250 0.5415 1.7268 0.3817 CW - 846,847 Jan,1997 H-3 1,518.5023 i 131.0155 1,631.7608 1 134.0877 1,575.1316 93.7344 CW - 846,847 Jan,1997 St-89 0.3800 0.5210 0.7406 1 0.8976 0.5603 0.5189 )
CW - 846,847 Jan,1997 Sr-90 0.1424 0.2458 0.7292 0.3717 0.4358 0.2228 AS-1
b i '
Table A-5. In-house " duplicate" samples. !
Concentration in pCi/L' Lab Sample First Second Codes
- Date Analysis Averaged Result Result Result WW - 576, 577 Feb,1997 H-3 150.9770 t 84.0813 241.2023 87.8687 196.0897 i 60.8083 MI- 486,487 Feb,1997 I-131 -0.0797 i 0.1694 -0.1161 0.1703 Mi- 486,487 -0.0979 0.1201 Feb,1997 K-40 1,278.2000 167.0000 j 1,316.5000 141.0000 1,297.3500 109.2817 MI - 486,487 Feb,1997 Sr-89 -0.8027 1 0.9962 -0.4554 0.9484 MI 486,487
-0.6290 0.6877 Feb,1997 Sr-90 1.8013 0.4825 4
1.4892 0.4537 1.6453 0.3312 MI - 510,511 Feb,1997 Co-60 0.6890 i 1.0200 -2.2000 4.1400 -0.7555 2.1319 MI - 510,511 Feb,1997 Cs-137 0.7830 i 2.5300 2.2400 3.2800 1.5115 2.1021 MI - 510,511 Feb,1997 I-131 0.0764 i 0.2227 0.0373 0.2345 0.0568 0.1617 MI - 531,532 Feb,1997 I-131 0.0368 i 0.1942 -0.0045 z 0.2095 0.0161 0.1429 MI - 531,532 Feb,1997 K-40 1,300.3000 i 178.0000 1,488.5000 156.0000 1,394.4000 118.3427 CW - 554,555 Feb,1997 Gr. Deta 3.6552 1.5170 2.7825 1.4922 3.2189 1.0639 CW - 554,555 Feb,1997 Gr. Beta 0.5033 i 1.0364 -0.2368 0.9931 0.1332 0.7177 MI- 632,633 Feb,1997 I-131 -0.2709 0.2349 -0.1024 0.1676 -0.1867 0.1443 M1 - 632,633 Feb,1997 i K-40 1,408.0000 1 165.0000 1,243.1000 145.0000 1,325.5500 1 109.8294 M1 - 723,724 Feb,1997 I-131 -0.0581 0.2376 0.2433 0.2658 0.0926 1 0.1783 MI - 723,724 Feb,1997 K-40 1,574.8000 1 218.0000 1,396.8000 i 162.0000 1,485.8000 135.8013 l LW - 757,758 Feb,1997 Gr. Beta 3.7439 i 0.9482 4.05471 0.9711 3.8993 0.6786 CW -083,884 Feb,1997 Gr. Beta 1.2996 i 1.2901 2.3358 1.3877 1.8177 0.9474 DW - 1030,1031 Feb,1997 Gr. Beta 2.0791 i 0.4817 2.0596 0.5098 2.0694 0.3507 DW - 1030,1031 Feb,1997 1-131 -0.1816 0.3127 -0.1217 0.3071 -0.1517 0.2192 SWU - 929,930 Feb,1997 Gr. Beta 2.4729 i 0.6238 2.9908 0.6691 2.7319 0.4574 SWU - 929, 930 Feb,1997 H-3 170.1477 i 84.5878 202.2735 65.9328 186.2106 60.2900 WW - 979, 980 Feb,1997 H-3 102.1168 i 92.0531 12.4533 88.3392 57.2850 63.7918 SW - 1370,1371 Feb,1997 H-3 50.6979 i 73.8916 8.0656 i 76.2734 21.3161 54.8669 LW -953,954 Mar,1997 Co-60 0.7490 t 1.7500 -1.3300 3.8800 -0.2905 2.1282 LW - 953,954 Mar,1997 Cs 137 -0.3220 1 2.2800 1.5500 1 2.7200 0.6140 1.7746 !
LW - 953,954 Mar,1997 Gr. Beta 3.7343 i 1.0079 4.6558 0.9898 4.1951 0.7063 SW - 1036,1037 j Mar,1997 Gr. Beta 1.7736 1 0.7279 2.1268 0.7453 1.9502 0.5209 l SW - 1576,1577 Mar,1997 H-3 219.6612 i 84.0956 250.7943 85.3666 235.2277 59.9156 I SW - 15'76,1577 Mar,1997 Sr-89 -0.5258 i 1.1183 -0.6149 0.9822 -0.5704 0.7442 SW - 1576,1577 Mar,1997 Sr-90 0.6723 0.3462 0.7181 0.3074 0.6952 0.2315 MI- 1055,1056 Mar,1997 I-131 0.1081 i 0.1729 0.0400 0.1677 0.0741 0.1204 MI- 1055,1056 Mar,1997 K-40 1,452.9000 i 126.0000 1,530.3000 i 124.0000 1,491.6000 88.3912 LW - 1120,1121 Mar,1997 Gr. Beta 2.5963 i 0.6078 1.8604 0.6077 2.2283 0.4298 MI- 1;58,1159 Mar,1997 I-131 0.0239 1 0.2040 0.0708 1 0.2015 0.0473 0.1434 MI- 1158,1159 Mar,1997 K-40 1,523.5000 i 152.0000 1,418.5000 i 157.0000 1,471.0000 109.2623 CW- 1187,1188 Mar,1997 Gr. Beta 4.8369 1 1.9131 3.4999 1.8196 1.1684 1.3201 AS-2
Table A 5. In-house " duplicate" samples.
Concentration in pCi/ L' Lab Sample First Second Averaged Codes" Date Analysis Result Result Result ;
CW - 1187,1186 Mar,1997 Gr. Beta 0.1481 t 1.5087 -0.0888 1.4896 0.0296 1.0601 LW 1145,1146 Mar,1997 Co-60 1.5000 3.3300 3.6600 6.9500 2.5800 3.8533 LW - 1145,1146 Mar,1997 Cs-137 1.6200 i 3.2500 -0.9330 4.1100 0.3435 2.6199 LW - 1145,1146 Mar,1997 Gr. Beta 4.2278 1 1.2135 3.5675 1.2356 3.8976 0.8659 MI - 1275,1276 Mar,1997 I-131 -0.0683 i 0.2309 0.3734 0.4565 0.1525 0.2558 MI - 1275,1276 Mar,1997 K 40 1,491.1000 193.0000 1,754.0000 177.0000 1,622.5500 130.9370 WW - 1309,1310 Mar,1997 H-3 4,282.8089 188.1304 4,034.4635 183.5207 4,158.6362 131.4086 SWT - 1519,1520 Mar,1997 Gr. Beta 2.5242 0.6065 2.0921 0.5846 2.3082 0.4212 WW - 1539,1540 Mar,1997 Gr. Beta 1.2878 i 0.6803 1.8468 0.7043 1.5673 0.4896 WW - 1539,1540 Mar,1997 H-3 -34.4755 72.6445 41.3706 76.1590 3.4476 52.6246 DW - 1688,1689 Mar,1997 Gr. Beta 4.5141 1 1.3660 4.6886 1 1.2681 4.6013 0.9319 DW - 1688,1689 Mar,1997 I-131 -0.1688 i 0.3758 0.3183 0.3363 0.0748 0.2522 SW - 2204,2205 Mar,1997 H-3 62.0000 152.0000 112.0000 152.0000 87.0000 107.4802 CW - 1909,1910 Mar,1997 H-3 435.8375 96.4774 430.4271 96.2750 433.1323 68.1483 LW - 1931,1932 Mar,1997 H-3 168.9801 83.1073 137.7304 81.7913 153.3552 58.3023 CW - 1599,1600 Mar,1997 Gr. Beta 3.4372 i 1.5949 3.4464 1.5289 3.4418 1.1047 CW - 1599,1600 Mar,1997 Gr. Beta 1.0978 1 0.9656 1.0340 i 0.9528 1.0659 0.6783 AP - 2572,2573 Mar,1997 Co-60 -0.0006 i 0.0102 -0.0002 0.0002 -0.0004 0.0051 AP - 2572,2573 Mar,1997 Cs-137 0.0008 1 0.0007 0.0000 0.0005 0.0004 0.0004 SWU - 2045,2046 Mar,1997 Sr-89 -0.0237 i 0.7179 0.1072 i 0.6305 0.0417 0.4777 SWU - 2045,2046 Mar,1997 Sr-90 0.3676 0.3471 0.1910 i 0.2933 0.2793 0.2272 MI - 1641,1642 Apr,1997 I-131 -0.6675 0.3099 -0.5511 0.3244 -0.6093 0.2243 MI - 1641,1642 Apr,1997 K-40 1,556.3000 i 111.0000 1,393.1000 160.0000 1,474.7000 97.3666 LW - 1763,1764 Apr,1997 Gr. Beta 2.3656 i 0.8258 2.1732 0.8478 2.2694 0.5917 LW - 1763,1764 Apr,1997 H-3 97.1488 i 79.2640 160.3540 t 82.0162 128.7514 57.0295 AP 1974,1975 Apr,1997 Sr-89 -0.0001 0.0006 -0.0005 0.0015 -0.0003 0.0008 AP - 1974,1975 Apr,1997 St-90 0.0001 1 0.0002 0.0001 1 0.0004 0.0001 0.0002 AP - 1994,1995 Apr,1997 Co-60 -0.0003 i 0.0013 0.0002 i 0.0007 -0.0000 0.0007 AP - 1994,1995 Apr,1997 Cs-134 -0.0001 0.0006 -0.0001 0.0016 -0.0001 0.0008 AP - 1994,1995 Apr,1997 Cs-137 -0.0002 1 0.0005 -0.0001 0.0005 -0.0002 0.0004 AP - 1994,1995 Apr,1997 I-131(g) -0.0001 0.0002 0.0001 0.0002 0.0000 0.0001 AP - 1994,1995 Apr,1997 K-40 0.0306 0.0192 0.0114 1 0.0180 0.0210 0.0132 WW - 1665,1666 Apr,1997 I-131 -0.4430 i 0.2674 -0.0311 1 0.2626 -0.2370 0.1874 WW - 1708,1709 Apr,1997 Gr. Beta 1.2245 0.6161 1.2858 t 0.6134 1.2551 0.4347 WW - 1785,1786 Apr,1997 Gr. Beta 2.9118 1 2.0703 0.3820 2.1095 1.6469 1.4779 WW - 1785,1786 Apr,1997 H-3 -19.0365 1 73.7753 -74.4153 1 71.1298 -46.7259 51.2402 WW - 1785,1786 Apr,1997 Sr-89 0.6539 1 0.6546 -0.4951 1 0.5197 0.0794 0.4179 l
AS-3 I l
l
Table A-5. In-house ',' duplicate" samples.
Concentration in pCi/L* !
Lab Sampie First Second Averaged Codes
- Date Analysis Result Result Result WW - 1785,1786 Apr,1997 Sr 90 -0.0023 0.2013 0.2468 0.2347 0.1223 0.1546 WW - 1737,1738 Apr,1997 Gr. Beta 15.0355 1.5075 15.6924 1.6231 15.3640 1.1076 WW - 1737,1738 Apr,1997 H3 13.8405 i 75.2790 -5.1902 74.3991 4.3251 52.9201 LW - 2848,2849 Apr,1997 Gr. Beta 2.4095 1 0.6377 1.7316 0.5601 2.0706 0.4244 MI - 1845,1846 Apr,1997 Co-60 0.0309 0.0778 -1.8500 22.4000 -0.9096 11.2001 MI - 1845,1846 Apr,1997 Cs-134 0.1600 i 0.1350 0.5860 2.2600 0.3730 1.1320 MI - 1845,1846 Apr,1997 Cs-137 0.7580 1.1500 0.6290 2.6700 0.6935 1.4536 MI- 1845,1846 Apr,1997 I131 -0.2586 0.2297 -0.0829 0.2149 -0.1708 0.1573 MI - 1845,1846 Apr,1997 I-131(g) -0.0707 i 0.2970 -0.7200 3.2700 -0.3954 i 1.6417 Mi- 1845,1846 Apr,1997 K-40 1,592.5000 52.5000 1,559.3000 127.0000 1,575.9000 68.7118 MI- 1845,1846 Apr,1997 Sr 89 0.2592 1.3259 -0.3095 0.8315 -0.0252 0.7825 MI - 1845,1846 Apr.1997 St-90 1.3583 i 0.3573 0.8755 0.2294 1.1169 0.2123 F - 2175,2176 Apr,1997 Gr. Alpha 0.0245 i 0.0359 0.0672 0.0377 0.0458 0.0260 F - 2175,2176 Apr,1997 Gr. Beta 2.3387 1 0.2713 1.7003 1 0.3684 2.0195 0.2288 F - 2175,2176 Apr,1997 K-40 2.5383 i 0.3610 2.5345 0.3640 2.5364 0.2563 F - 2175,2176 Apr,1997 Sr-89 0.0003 i 0.0053 0.0021 1 0.0048 0.0012 0.0036 F - 2175,2176 Apr,1997 Sr-90 -0.0002 0.0018 -0.0003 0.0016 -0.0002 0.0012 J SWU - 2091, 2092- Apr,1997 Gr. Beta 3.3295 t 0.6698 2.73 74 0.6670 3.0334 1 0.4726 SWU - 2091,2092 f Apr,1997 H-3 42.6019 i 76.2782 46.1034 76.4388 44.3526 53.9936 SWU - 2636,2637 Apr,1997 H-3 17.9011 i 75.4236 92.3927 i 78.7712 55.1469 54.5290 SL - 2432,2433 Apr,1997 K-40 1.8447 i 0.4400 1.6811 0.5400 1.7629 0.3483 WW - 2462, 2463 Apr,1997 Co-60 -0.5320 i 0.7550 0.4650 0.7810 -0.0335 0.5431 WW - 2462,2463 Apr,1997 Cs-137 0.6250 1 3.6500 -1.4600 3.4400 -0.4175 2.5078 WW - 2462,2463 Apr,1997 H-3 19.6154 i 75.4335 -21.9230 73.5027 -1.1538 52.6613 F - 2412,2413 Apr,1997 K-40 3.0009 0.1660 3.0594 i 0.1470 3.0302 0.1109 LW - 2550,2551 Apt,1997 Cr. Beta 2.0074 1 0.8317 3.6936 1 0.8973 2.8505 0.6117 LW - 2550,2551 Apr,1997 K-40 102.7800 i 55.6000 96 6520 54.9000 99.7160 39.0684 SP - 2806,2807 Apr,1997 Gr. Alpha 0.0245 i 0.3861 0.1365 0.3720 0.0805 0.2681 SP - 2806,2807 Apr,1997 Sr-89 -1.4194 6.8147 -5.6447 8.6109 -3.5321 5.4906 SP - 2806,2807 Apr,1997 St-90 2.6542 1 2.3158 7.1752 2.9780 4.9147 1.8862 PW - 2736,2737 Apr,1997 Co-60 0.1300t 4.6800 -0.6250 9.8400 -0.2475 5.4481 PW - 2736,2737 Apr,1997 Cs-137 -0.2740 1 4.2100 1.7400 3.3400 0.7330 2.6870 PW - 2736,2737 Apr,1997 Gr. Beta 2.8037 i l.5036 2.6658 1.4461 2.7348 1.0431 WW - 2712,2713 Apr,1997 H-3 1,482.0205 1 125.6515 1,596.1107 1 128.7524 1,539.0656 89.9520 SW - 2657,2658 May,1997 Gr. Beta 13.2739 i l.3358 13.1663 1.2719 13.2201 0.9222 S O - 2677, 2678 May,1997 Cs-137 0.1078 i 0.1000 0.2315 0.0507 0.1697 0.0561 S O - 2677, 2678 May,1997 Gr. Alpha 5.5187 3.4094 8.3190 1 4.0540 6.9189 2.6486 AS-4
l l
Table A-5.' In-house " duplicate" samples.
Concentration in pCi/L'
. Lab. Sample First Second Averaged Code.? Date Analysis Result Result Result S O - 2677,2678 May,1997 Gr. Beta 21.9926 2.7808 21.8461 3.0806 21.9193 t 2.0750 S O - 2677, 2678 May,1997 Sr 89 0.0075 0.0954 -0.0008 0.0808 0.0034 0.0625 S O - 2677, 2678 May,1997 Sr-90 0.0713 i 0.0197 0.0642 0.0164
' 0.0677 0.0128 MI- 2764,2765 May,1997 Co-60 0.0636 0.0966 -1.5300 7.2300 -0.7332 3.6153 MI 2764,2765 May,1997 Cs 137 5.5000 i 5.2800 1.7700 t 4.9900 3.6350 3.6324
- MI- 2764,2765 May,1997 I131 -0.1635 i o.1612 -0.0766 0.1452 -0.1201 0.1085 MI- 2828,2829 May,1997 I-131 -0.0153 0.2503 -0.0855 0.2257 -0.0504 0.1685 MI- 2828,2829 May,1997 K 40 1,786.4000 126.0000 1,897.0000 1 192.0000 1,841.7000 114.8260 G - 2879,2880 May,1997 Co-60 0.0044 i 0.1100 -0.0207 i 0.2030 -0.0081 0.1154 C - 2879,2880 May,1997 Cs-134 0.0081 1 0.0305 -0.0030 0.0133 0.0025 0.0166
- j. . G - 2.979,2880 May,1997 Cs-137 0.0006 0.0234 0.0013 1 0.0166 0.0010 0.0143 G -2'379,2880 May,1997 Gr. Beta 6.4712 0.2029 6.6206 0.1927 6.5459 i 0.1399 G - 2879,2880 May,1997 I131(g) 0.0093 i 0.0456 0.0220 1 0.6620 0.0157 1 0.3318
! G - 2879,2880 May,1997 K-40 6.2539 0.8340 5.7979 0.7160 6.0259 i 0.5496
! S O - 2904, 2905 May,1997 Co-60 -0.0097 0.0201 -0.0021 1 0.0224 -0.0059 i 0.0150 S O - 2904, 2905 May,1997 Cs-134 0.0348 1 0.0682 0.0208 i 0.1500 0.0278 0.0824 S O 2904, 2905 May,1997 Cs-137 0.2709 i 0.0541 0.2768 0.0463 0.2738 0.0356
- S 0 - 2904, 2905 May,1997 Gr. Beta 24.4695 1 2.3915
' 26.5459 2.5962 25.5077 1.7649 S O - 2904, 2905 May,1997 K-40 18.8100 i 1.0100 19.1610 0.8920 18.9855 0.6738 F - 2926,2927 May,1997 Co-60 0.0071 i 0.0082 -0.0010 i 0.0015 0.0031 0.0042
! F - 2926,2927 May,1997 Cs-137 -0.0047 i 0.0122 .-0.0029 i 0.0088 -0.0038 0.0075 SW - 3008,3009 May,1997 H-3 101.2957 i 91.5729 l 123.2634 92.4471 112.2795 65.0616
- MI- 3050,3051 May,1997 St-89 -0.1527 i 0.9022 0.0234 0.8795 -0.0646 0.6300
- j. MI- 3050,3051 May,1997 Sr 0.9779 i 0.3707 0.9427 1 0.3596 0.9603 0.2583
, F - 3070,3071 May,1997 Co-60 -0.0093 i 0.0979 0.0094 i 0.0303 0.0000 0.0512 I F - 3070,3071 May,1997 Cs-137 0.0064 i 0.0113 -0.0003 i 0.0078 0.0030 0.0069 l G - 3090,3091 May,1997 K-40 5.0649 i 0.2170 4.9752 1 0.2830 5.0201 0.1783 I- MI- 3116,3117 May,1997 I131 -0.1346 i 0.1762 -0.0964 0.1650 -0.1155 0.1207 F - 3277,3278 May,1997 Gr. Beta 2.9487 i 0.1093 l 3.0022 0.1035 2.9755 0.0753 F - 3277,3278 May,1997 K-40 2.8485 i 0.2780 2.4647 0.3130 2.6566 0.2093 MI- 3232,3233 May,1997 I-131 -0.1723 i 0.2021 i
-0.2680 1 0.2044 -0.2202 0.1437 MI- 3232,3233 May,1997 K-40 1,550.6000 i 121.0000 1,517.9000 141.0000 1,534.2500 92.9005 ;
BS 3311,3312 May,1997 Co-60 -0.0035 i 0.0348 -0.0044 1 0.0031 -0.0039 i 0.0175 BS - 3311,3312 May,1997 Cs-137 0.0676 i 0.0334 0.0677 i 0.0297 0.0676 1 0.0223 F - 3484,3485 May,1997 K-40 2.4582 t 0.3320 1.8380 i 0.2990 2.1481 0.2234 SW - 3533,3534 May,1997 H-3 95.4129 i 90.4309 -117.7172 1 89.5093 -106.5650 t 63.6193 WW - 3395,33% May,1997 I131 -0.1507 i 0.1841 -0.0473 1 0.2108 -0.0990 t 0.1399 AS-5
Table A-5. In-house " duplicate" samples.
Concentration in pCi/L' Lab Sample 6 First Second Averaged
' Codes Date Analysis Result Result Result F - 3720,3721 May,1997 K-40 2.6 % 3 1 0.4030 2.6623 0.3390 2.6343 0.2633 LW - 3464,3465 May,1997 Co-60 -0.2860 1 1.2700 -0.0583 0.0489 -0.1722 0.6355 LW - 3464,3465 May,1997 Cs-137 2.4600 1 2.8100 1.5000 1 3.2400 1.9800 2.1444
. LW - 3464,3465 May,1997 Gr. Beta 3.3532 i 0.9801 3.7723 1 0.9839 3.5628 0.6944 SW - 3883, 3884 May,1997 H-3 -20.5031 i 87.7694 124.8827 93.7412 52.1898 64.2084 M1 - 3513,3514 Jun,1997 I131 -0.1592 i 0.1592 -0.1028 i 0.1714 -0.1310 0.1170 M1 - 3513,3514 Jun,1997 K-40 1,560.3000 129.0000 1,521.9000 179.0000 1,541.1000 i 110.3200 P - 3794,3795 Jun,1997 H-3 109.9207 93.1034 24.2198 89.6079 67.0702 64.6100 F - 4049,4050 Jun,1997 K-40 2.8350 1 0.3980 3 0237 1 0.2420 2.9294 0.2329 MI- 3903,3904 Jun,1997 I-131 0.1550t 0.1840 -0.1290 0.1587 0.0130 0.1215 MI-3903,3904 Jun,1997 K-40 2,020.1000 i 142.0000 1,822.5000 1 188.0000 1,921.3000 117.8007 VE 3839,3840 Jun,1997 Gr. Alpha 0,2489 i 0.0857 0.1876 0.0698 0.2183 0.0553 VE - 3839,3840 Jun,1997 Gr. Beta 4.4859 1 0.4451 4.1281 0.4123 4.3070 1 0.3034 VE - 3839,3840 Jun,1997 K-40 5.4016 0.3360 4.6783 0.4282 5.0400 i 0.2721 F - 3928,3929 Jun,1997 Co-60
~
-0.0025 i 0.0121 0.0045 0.0034 0.0010 0.0063 F - 3928,3929 Jun,1997 Cs-134 0.0050 t 0.0115 -0.0030 i 0.0114 0.0010 0.0081 F- 3928,3929 Jun,1997- Cs-137 0.0841 1 0.0225 0.0796 i 0.0286 0.0818 0.0182 F - 3928,3929 Jun,1997 Gr. Beta 2.7146 i 0.0950 2,6357 0.0977 2.6752 0.0681 F - 3928,3929 Jun,1997 I-131(g) 0.0206 i 0.0449 0.0158 0.0458 0.0182 0.0321 F - 3928,3929 Jun,1997 K-40 1.8883 i 0.3970 1.4854 0.3780 1.6S69 0.2741 SWU - 3980,3981 Jun,1997 Gr. Beta 2.1443 1 0.6206 2.3149 0.6407 2.2296 0.4460 SWU - 3980,3981 Jun,1997 H-3 221.0233 i 89.9165 105.6271 65.0852 163.3252 61.8960 CW - 3948,3949 Jun,1997 Gr. Beta -0.4402 i l.0747 -0.3764 1.1259 -0.4083 1 0.7782
' SW - 4150,4151 Jun,1997 H-3 30.4430t 77.1886 56.0152 78.3895 43.2291 55.0068 MI- 4091,4092 Jun,1997 I131 -0.0475 i 0.1439 -0.0071 0.1516 -0.0273 0.1045 SWT - 4240,4241 Jun,1997 Gr. Beta 2.1204 i 0.6338 2.8553 i 0.6330 2.4879 1 0.4479 SW - 5186,5187 Jun,1997 H-3 190.3311 i 89.7491 192.1730 89.8246 191.2521 1 63.4889 DW - 4280,4281 Jun,1997 Gr. Alpha -0.4934 i 0.7635 -0.4930 0.7640 -0.4932 0.5401 DW - 4280,4281 Jun,1997 Gr. Beta 2.0633 i 0.8600 2.0630 i 0.8700 2.0631 0.6117 WW - 4811,4812 Jun,1997 H-3 48.4888 i 83.6998 50.3302 83.7808 49.4095 59.2133 CW - 5207,5208 Jun,1997 H-3 151.5810 i 88.1060 135.0114 87.4113 143.2962 1 62.0552 SW 4364,4365 Jun,1997 H-3 83.4415 i 83.9269 94.4046 84.4029 88.9230 59.5138 AP - 4983,4984 Jun,1997 Co-60 -0.0002 i 0.0009 0.0001 i 0.0007 -0.0000 0.0006 AP - 4983,4984 ' Jun,1997 Cs-137 0.0003 i 0.0004 -0.0001 i 0.0007 0.0001 i 0.0004 AP - 5004,5005 Jun,1997 Co-60 0.0002 1 0.0002 0.0003 0.0008 0.0002 1 0.0004 AP - 5004,5005 Jun,1997 Cs-137 -0.0002 i 0.0004 0.0002 0.0006 -0.0000 0.0004 DW - 4484,4485 Jun,1997 Gr. Beta 2.0708 i 0.6272 1.9172 1 0.5805 1.9940 0.4273 A5-6
Table A-5. In-house " duplicate" samples.
Concentration in pCi/L' Lab Sample First Second-Codes
- Date Analysis Averaged Result Result Result DW - 4484,4485 Jun,1997 H-3 39.2579 i 83.2425 66.8612 84.4541 53.0596 59.2913 SW - 4460,4461 Jul,1997 Gr. Beta 1.8471 i 0.7685 2.2801 0.778S 2.0636 0.5471 DW - 4510,4511 Jul.1997 H-3 1.2216 t 80.7150 21.3772 81.6249 11.2994 57.3967 AP - 4917,4918 Jul,1997 Co-60 0.0002 0.0003 0.0002 0.0006 0.0002 i 0.0003 AP - 4917,4918 Jul,1997 Cs-134 0.0002 1 0.0003 0.0002 0.0052 0.0002 0.0026 AP - 4917,4918 Jul,1997 Cs 137 0.0005 i 0.0004 0.0002 1 0.0004 0.0003 0.0003 AP - 4917,4918 Jul,1997 I-131(g) -0.0009 i 0.0017 0.0022 0.0762 0.0006 0.0381 AP - 4917,4918 Jul,1997 K-40 0.0239 0.0081 0.0305 0.0086 0.0272 0.0059 SP - 5024,5025 Jul,1997 Gr. Alpha 0.4224 0.9602 1.7836 1.2429 1.1030 0.'/853 SP - 5024,5025 Jut,1997 Sr-90 65.8931 i 7.2660 61.7118 6.1959 63.8024 4.7745 BS - 4573,4574 Jul,1997 K-40 11.9570 i 0.5550 12.0610 0.5170 12.0090 0.3792 WW - 4535,4536 Jul,1997 Co-60 -0.0955 i 0.4620 1.0800 1 1.5100 0.4923 0.7895 WW - 4535,4536 Jul,1997 Cs-137 -0.7200 2.3500 0.1650 i 3.3100 -0.2775 2.0297 WW - 4535,4536 Jul,1997 H-3 565.2121 1 103.8753 524.7523 102.4326 544.9822 72.9426 G - 4745,4746 Jul,1997 Co-60 -0.0147 i 0.1270 -0.0016 0.0036 -0.0082 0.0635 G - 4745,4746 Jul,1997 Cs-134 0.0055 1 0.03 % -0.0118 0.0963 -0.0032 0.0519 G - 4745,4746 Jul,1997 Cs-137 0.0057
- 0.0186 0.0132 i 0.0180 0.0095 0.0129 C - 4745,4746 Jul,1997 Gr. Beta 5.0148 1 0.1659 4.7792 0.1700 4.8970 0.1188 G - 4745,4746 Jul,1997 I-131(g) 0.0040 i 0.0078 0.0104 0.0269 0.0072 1 0.0140 G - 4745,4746 Jul,1997 K-40 4.5596 i 0.5840 4.1530 0.6150 4.3563 0.4241 SWU - 4832,4833 Jul,1997 Gr. Beta 2.7683 1 0.6756 3.4254 i 0.6591 3.0968 0.4719 LW - 4782,4783 Jul,1997 Co-60 2.8200 i 20.3000 1.9900 6.6500 0.4150 10.6807 LW - 4782,4783 Jul,1997 Cs-137 0.6730 i 3.2000 -0.6030 i 2.2500 -0.0350 i 1.9559 LW - 4782,4783 Jul,1997 Cr Beta 4.0046 i 1.0458 3.5274 1 0.9990 3.7660 0.7232 MI- 4897,4898 Jul,1997 1-131 -0.0412
- 0.2182 0.0463 0.2335 0.0026 0.1598 MI- 4897,4898 Jul,1997 K-40 1,531.3000 123.0000 1,270.5000 152.0000 1,400.9000 97.7663 CW - 5150,5151 Jul,1997 Gr. Beta 4.7218 t l.5818 4.2648 1.6666 4.4933 1.1488 CW - 5150,5151 Jul,1997 Gr. Beta -0.2253 t 1.0995 0.5464 1.2464 0.1605 0.8310 G - 5296,5297 Jul,1997 K-40 6.8000t 0.6000 8.2000 0.8000 7.5000 0.5000 WW - 5369,5370 Jul,1997 H-3 18,013.8557 i 373.4409 18,133.8988 i 374.6263 18,073.8773 264.4820 CW - 5321,5322 - Jul,1997 Gr. Beta 1.5612 i l.4170 1.3507 1.2764 1.4560 0.9535 CW - 5321,5322 Jul,1997 Gr. Beta -0.6334 i 1.0849 0.5162 1.2191 -0.0586 0.8160 WW - 5348,5349 Jul,1997 H-3 1,763.0308 i 139.9964 1,813.1908 141.3214 1,788.1108 99.4620 MI 5464,5465 Jul,1997 I-131 -0.2555 0.2878 -0.3511 1 0.2946 -0.3033 0.2059 MI- 5464,5465 jul,1997 K-40 1,282.9000 i 143.0000 1,380.0000 1 124.0000 1,331.4500 94 6375 VE - 5506,5507 Jul,1997 Gr. Beta 7.2756 2 0.2197 7.0057 2 0.2090 7.1407 0.1516 VE - 5506,5507 Jul,1997 K-40 8.1566 i 0.3970 8.18171 0.4360 8.1692 0.2948 A5-7
Table A-5. In-house " duplicate" samples.
Concentration in pCi/L' Lab Sample First Second Codes
- Date - Analysis Averaged Result Result Result WW - 5848,5849 - Jul,1997 H3- 51.6431 1 83.4870 40.4434 i 82.9847 46.0433 1 58.8569 WW - 5529,5530 ' Aug,1997. Gr. Beta 5.1545 1 2.1632 4.3564 1.9691 4.7555 1.4626 WW - 5529,5530 Aug,1997 H-3 235.5502 i 91.5917 372.4741 97.6610 304.0122 66.9453 MI- 5606,5607 Aug,1997 I-131 -0.0759 0.3043 -0.1020 1 0.3423 -0.0889 1 0.2290 SL - 5563,5564 Aug,1997 . Gr. Beta 1.9301 1 0.2206 2.0961 0.2125 2.0131 0.1531 SL - 5563,5564 Aug,1997 K-40 1.1254 i 0.3530 1.3185 1 0.4050 1.2220 0.2686 SL - 5563,5564 Aug,1997 St 89 -0.0078 i 0.0216 0.0096 1 0.0196 0.0009 0.0146 SL - 5563,5564 Aug,1997 St 90 0.0097 1 0.0059 0.0031 0.0048 0.0064 0.0038 SW - 5584,5585 Aug,1997 Gr. Beta 2.9875 0.7744 2.0205 1 1.0326 2.5040 0.6454 LW - 5678,5679 Aug,1997 Co-60 0.4180 1.2900 0.7270 1.4500 0.5725 0.9704 LW - 5678,5679 - Aug,1997 Cs-134 0.8140 0.6510 0.8540 i 0.4840 0.8240 0.4056 LW - 5678,5679 Aug,1997 Cs-137 1.1400 1.1800 0.7750 1.1900 0.9575 0.8379 LW - 5678,5679 Aug,1997 Gr. Beta 2.6926 1 0.6727 2.4242 0.6023 2.5584 0.4515 LW - 5678,5679 Aug,1997 I-131 -0.1036 1 0.3234 -0.0921 0.3371 -0.0m 0.2336 LW - 5678,5679 Aug,1997 - I-131(g) -10.1000 11.1000 -3.6000 1 5.8200 -6.85W i 6.2666 LW - 5678,5679 Aug,1997 K-40 137.0000 i 16.5000 124.0000 i 17.3000 130.5000 ! '1.9535 G - 5653,5654 Aug,1997 K-40 6.0419 i 0.5940 5.5554 0.5870 5.7987N 176 l l - CW - 5759,5760 Aug,1997 Gr. Beta 4.3051 1 1.5501 2.0048 1 1.4570 3.1550 1 1.0637 CW - 5759,5760 Aug,1997 Gr. Beta -0.5860 1.1030 -0.0177 1.1407 -0.3018 0.7934 CW - 5708,5709 Aug,1997 Gr. Beta 1.7190 i 1.4125 1.8843 1 1.4139 1.8017 i 0.9993 MI- 5891,5892 Aug,1997 I-131 0.0000 i 0.2400 0.1928 0.2253 0.0964 1 0.1646
' MI- 5891,5892 Aug,1997 K-40 1,438.6000 131.0000 1,218.6000 i 175.0000 -1,328.6000 109.3000
- MI- 5926,5927 Aug,1997 - I-131 -0.0311
- 0.1690 -0.1446 1 0.1748 -0.0879 0.1216 MI- 5926,5927 Aug,1997 K-40 1,577.8000 i 216.0000 1,429.9000 i 178.0000 1,503.8500 139.9464 SWU - 5972,5973 Aug,1997 H-3 274.7574 i 93.6817 157.2707 i 88.8812 216.0140 t 64.5681 CW - 6013,6014 Aug,1997 Gr. Beta 4.9801 i l.3048 4.5882 1.6114 4.7841 1.0367 CW - 6013,6014 Aug,1997 Gr. Beta -0.5668 1 1.0528 -0.6145 1 1.1307 -0.5907 0.7725 SL -. 6034,6035 Aug,1997 Co-60 0.0183 1 0.0235 0.0159 0.2550 0.0171 0.1280
- SL - 6034,6035 Aug,1997 Cs-134 0.0046 1 0.0136 0.0015 1 0.0020 0.0030 0.0069 SL - 6034,6035 Aug,1997 Cs-137 0.0118 1 0.0097 0.0175 0.0098 0.0147 0.0069 SL 6034,6035 Aug,1997 Gr. Beta 2.1826 0.1949 1.9837i 0.1773 2.0831 0.1317 SL - 6034,6035 Aug,1997 1-131(g) -0.0039 i 0.0134 0.0013 i 0.0060 -0.0013 0.0073 SL - 6034,6035 Aug,1997 K-40 1.6231 i 0.2940 1.4676 0.2750 1.5454 i 0.2013 CW - 6172,6173 Aug,1997 Gr. Beta 3.2828 t l.0951 3.7336 1 1.6212 3.5082 0.9782 CW 6172,6173 Aug,1997 Gr. Beta 1.2291 t l.3108 0.0271 1 1.1175 0.6281 0.8612 CW- 6080,6081 Aug,1997 Gr. Beta 2.4263 t l.5665 4.0378 1.5325 3.2321 1,0957 CW - 6080,6081 Aug,1997 G . Beta -0.0198 t l.1927 0.9870 1.1701 0.4836 0.8354 AS-8
I i
Table A 5. In-house duplicate" samples.
l Lab Sample First Second Codes
- Date Analysis Averaged Result Result Result VE - 6106 6107 Aug,1997 Co-60 0.0021 1 0.0173 0.0019 0.0087 0.0020 0.0097 I VE 6106,6107 Aug,1997 Cs-137 0.0017 1 0.0057 -0.0005 0.0072 0.0006 0.0046 l VE - 6149,6150 Aug,1997 Co-60 0.0043 0.1740 0.0004 0.0012 0.0024 1 0.0870 -
VE - 6149,6150 Aug,1997 Cs-137 -0.0026 i 0.0056 0.0018 0.0060 -0.0004 z 0.0041 MI- 6203,6204 Aug,1997 Co-60 2.3200 83 6000 0.7940 1 1.9700 1.5570 1 41.9116 MI - 6203,6204 Aug,1997 Cs-137 0.5560 i 3.0200 1.2900 2.6500 0.9230 2.0089 l MI 6203,6204 Aug,1997 l-131 -0.2456 1 0.3252 -0.16R4 + ^ '245 -0.2072 1 0.2297 VE - 6224,6225 Aug,1997 Co-60 -0.0042 1 0.0160 0.00 '78 0.0002 0.0089 VE - 6224,6225 Aug,1997 Cs-137 -0.0057 1 0.0131 0.L .7 0.0007 0.0070 VE - 6251,6252 Aug,1997 Gr. Beta 3.4988 i 0.1337 3.50L _ . ..J8 3.4998 0.0946 VE - 6251,6252 Aug,1997 K-40 3.8744 i 0.5410 3.3980 0.6150 3.6362 0.4095 MI- 6335,6336 Aug,1997 1-131 0.0196 i 0.2826 0.0564 0.2698 0.0380 0.1953 M1 - 6335,6336 Aug,1997 K-40 1,488.7000 1 128.0000 1,538.6000 116.0000 1,513.6500 86.3713 SL - 6982,6983 Aug,1997 Co-60 0.0869 i 0.0110 0.0888 0.0135 0.0879 i 0.0087 SL - 6982,6983 Aug,1997 Cs-137 0.0826 1 0.0110 0.0993 1 0.0165 0.0909 0.0099 SL - 6982,6983 Aug,1997 Gr. Beta -0.7733 1 0.1093 -0.6988 1 0.0989 -0.7361 i o.0737 WW - 6312, 6313 Aug,1997 H-3 4,401.6798 i 200.9023 4,585.7685 204.3507 4,493.7241 1 143.2837 LW - 6560,6561 Aug,1997 Gr. Alpha 0.4838 i 0.3847 0.7647 1 0.3421 0.6242 0.2574 LW - 6560,6561 Aug,1997 Gr. Beta 1.6502 i 0.3609 1.6339 1 0.3320 ' 5 010.2452 LW - 6560,6561 Aug,1997 H-3 164.1455 90.4249 131.5719 i 89.0337 147.8587 63.4501 LW - 6520,6521 Sep,1997 Gr. Beta 1.9762 i 0.5715 2.3786 1 0.6284 2.1774 0.4247 LW - 6520,6521 Sep,1997 H-3 104.7304 i 87.8580 66.4144 i 86.1708 85.5724 61.5314 CW - 6489,6490 Sep,1997 Gr. Beta 0.2448 i 1.3049 1.9046 t 1.3290 1.0747 0.9313 G - 6773,6774 Sep,1997 K-40 3.7979 i 0.2420 3.5568 0.3270 3.6774 0.2034 CW - 6796,6797 Sep,1997 Gr. Beta 3.3658 i 1.5585 5.0139 1.1808 4.1899 0.9777 CW - 6796,6797 Sep,1997 Gr. Beta -1.1040 i 1.0241 -0.7623 1.0723 -0.9332 0.7414 SWU - 7009,7010 Sep,1997 Gr. Beta 3.2034 i 0.6793 3.2645 0.6681 3.2339 0.4764 SWU - 7009,7010 Sep,1997 H-3 165.8491 1 90.5715 150.5986 89.9273 158.2239 t 63.8164 G - 6820,6821 Sep,1997 K-40 4.8113 i 0.4160 4.7307 0.5360 4.7710 0.3392 MI- 6886,6887 Sep,1997 1-131 0.0177 i 0.1519 0.0180 0.1520 0.0179 0.1074 Mi - 6886,6887 Sep,1997 K-40 1,241.7000 1 155.0000 1,062.0000 156.0000 1,151.8500 109.9557 WW - 7031,7032 Sep,1997 H-3 -38.0852 1 81.4466 -19.0426 i 82.3323 -28.5639 57.9054 CW - 6907,6908 Sep,1997 Gr. Beta 3.8333 1 1.5682 4.5001 1 1.6814 4.1667 1.1496 i CW - 6907,6908 Sep,1997 Gr. Beta -0.0397 i 1.1726 -0.1621 i 1.1478 -0.1009 : 0.8204 F - 7221,7272 Sep,1997 K-40 3.0101 i 0.3970 2.6722 1 0.4720 2.8412 0.3084 CW - 7177,7178 Sep,1997 Gr. Beta 0.5864 1 0.9867 2.3794 1.4286 1.4829 0.8681 CW - 7177,7178 Sep,1997 Gr. Beta -1.0971 i 1.0379 -0.1387 1.1507 0.6179 1 0.7748 AS-9
1 I '
i Table A-5. In-house " duplicate" samples.
Concentration in pCi/L' Lab Sample First Second Codes
- Date Analysis Result Averaged Result Result LW - 7198,7199 Sep,1997 Cr. Beta 1.6523 0.6116 2.3619 0.6044 VE - 7141,7142 2.0071 0.4299 Sep,1997 Co-60 0.0012 1 0.0118 -0.0001 0.0004 0.0005 0.0059 VE - 7141,7142 Sep,1997 Cs-137 -0.0011 0.0090 0.0081 0.0103 SWU - 7364,7365 0.0035 0.0068 Sep,1997 Gr. Deta 2.4372 i 0.6226 2.7949 0.6153 2.6160 0.4377 SWU - 7364,7365 Sep,1997 H-3 245.3799 i 94.1721 269.0627 95.1596 WW - 7408, 7409 257.2213 66.9398 Sep,1997 Co-60 0.4170 i 0.8010 2.0100 6.7100 1.2135 3.378S WW - 7408, 7409 Sep,1997 Cs-137 -0.2190 i 1.6500 0.8220 3.0600 WW - 7408,7409 0.3015 1.7383 Sep,1997 H-3 7,907.0011 264.0275 7,543.2790 258.5239 7,725.1400 184.7601 LW - 7765,7766 Sep,1997 Gr. A1pha 0.2614 1 0.4857 0.3882 1 0.5450 LW - 7765, 7766 0.3248 0.3650 Sep,1997 Gr. Beta 3.6490 0.5140 2.7232 1 0.'728 3.1861 0.3492 LW - 7765,7766 .Sep,1997 H-3 3,168.6312 i 176.2295 3,030.6146 ! 173.2010 3,099.6229 123.5470 AP - 8208,8209 Sep,1997 Co-60 0.0002 0.0004 0.0004 0.0008 AP - 8208,8209 0.0003 0.0005 Sep,1997 Cs-137 0.0003 0.0005 -0.0004 0.0006 -0.0000 i 0.0004 G - 7244,7245 Oct,1997 Gr. Beta 9.0000 i 0.3000 8.4000 0.3000 G - 7244,7245 Oct,1997 8.7000 i 0.2121 !
K-40 8.8853 i 0.7960 9.1594 1 0.7550 G - 7244,7245 Oct,1997 Sr-89 9.0224 0.5486 )
-0.0058 t 0.0181 -0.0056 0.0097 G - 7244,7245 Oct,1997
-0.0057 0.0103 Sr-90 0.0053 i 0.0052 0.0017 i 0.0029 0.0035 0.0029 G - 7265,7266 Oct,1997 K-40 6.5763 1 0.5250 6.0640 1 0.6540 SW - 7313,7314 6.3202 0.4193 Oct,1997 Gr. Beta 24.5727 2.0773 21.9706 2.0623 23.2717 1.4636 SW 7313,7314 Oct,1997 K-40 114.6700 41.9000 90.9920 37.6000 G - 7432,7433 102.8310 28.1486 ;
Oct,1997 Co-60 0.0073 1 0.0252 0.00411 0.0059 0.0057 0.0129 !
G - 7432,7433 Oct,1997 Cs-134 0.0057 0.0110 0.0009 0.0010 C - 7432,7433 0.0033 0.0055 Oct,1997 Cs-137 0.0863 1 0.0217 0.0835 0.0247 0.0849 0.0164 G - 7432,7433 Oct,1997 Gr. Beta 5.3675 1 0.2025 5.3318 1 0.2123 G - 7432,7433 5.3496 0.1467 Oct,1997 I-131(g) -0.0038 0.0069 0.0218 i 0.4830 C - 7432,7433 0.0090 0.2415 Oct,1997 K-40 4.4899 1 0.4020 4.9632 0.5470 4.7266 0.3394 j CW - 7339,7340 Oct,1997 Gr. Beta 0.2969 2 1.2051 -0.2575 0.8630 AP - 7537,7538 0.0197 0.7411 Oct,1997 Sr-89 0.0006 i 0.0008 -0.0001 0.0008 0.0002 0.0006 AP 7537,7538 Oct,1997 l Sr 90 -0.0001 i 0.0003 0.0001 1 0.0003 CW - 7560,7561 0.0060 0.0002 Oct,1997 Gr. Beta 3.7764 1.5088 3.7707 1.5155 3.7735 1.0692 CW - 7560,7561 Oct,1997 Gr. Beta 0.4496 1 1.1864 0.3374 1.2009 F - 7474,7475 0.3935 0.8440 Oct,1997 Co-60 -0.0010 i 0.0016 0.0020 0.0058 0.0005 0.0030 F - 7474,7475 Oct,1997 Cs-137 0.0071 1 0.0064 0.0001 0.0113 0.0036 0.0065 F - 7495,7496 Oct,1997 Co-60 0.0025 i 0.0076 0.0086 1 0.1430 0.0055 0.0716
( F - 7495,7496 Oct,1997 Cs-137 0.0078 i 0.0083 0.0044 1 0.0056 0.0061 0.0050 F - 7626,7627 Oct,1997 K-40 2.2464 1 0.3120 1.5663 0.3760 1.9064 0.2443 f CW - 7669,7670 Oct,1997 Gr. Beta 5.7005 1.8448 3.6801 1 1.7132 4.6&O3 1.2588 I i
l l
A5-10
Table A-5. In-house duplicate" samples.
Concentration in pCi/L' Lab Sample First Second Codes
- Date Analysis Averaged Result Result CW - 7669,7670 Result Oct,1997 Gr. Beta -0.0304 i 1.1674 0.1259 1.1344 0.0478 0.8139 WW - 7643, 7649 Oct,1997 Co-60 38.3320 4.3000 31.7400 3.3600 WW - 7648, 7649 Oct,1997 35.0360 2.7285 Cs-137 2.8800 i 2.3000 0.5180 1.9100 1.6990 1.4948 WW - 7648, 7649 Oct,1997 H-3 241.3364 i 105.7031 265.5372 106.6226 MI- 7787,7788 Oct,1997 253.4368 75.0692 1-131 -0.0456 i 0.2490 0.0257 0.2696 -0.0099 0.1835 M1 - 7787,7788 Oct,1997 K-40 1,514.0000 i 114.0000 1,684.0000 102.0000 1,599.0000 76.4853 S O - 8010, 8011 Oct,1997 Cs-137 0.3513 i 0.0712
)
0.3182 0.0693 0.3347 0.0497 S O - 8010, 8011 Oct,1997 K-40 22.4300 1 1.3200 22.0830 1.2900 SL - 8123,8124 Oct,1997 22.2565 0.9228 Cs-137 0.0368 i 0.0335 l 0.0242 0.0137 0.0305 0.0181 SL - 8123,8124 Oct,1997 K-40 2.8000 i 0.5510 2.5777 i 0.2960 F - 7915,7916 2.6889 0.3127 Oct,1997 Cs-137 0.0072 i 0.0118 0.0031 0.0085 0.0052 0.0073 MI- 7968,7969 Oct,1997 I131 -0.1451 0.3579 -0.4853 i 0.3455 MI - 7968,7%9 Oct,1997 0.3152 0.2487 K-40 1,324.1000 i 132.0000 1,313.0000 118.0000 1,318.5500 88.5268 MI - 7968,7969 Oct,1997 Sr-90 1.2892 i 0.4152 1.2892 0.7200 VE - 7934,7935 1.2892 0.4156 Oct,1997 Co-60 0.0071 0.1160 -0.0029 0.0139 0.0021 1 0.0584 VE - 7934,7935 Oct,1997 Cs-137 0.0022 1 0.0110 -0.0041 0.0099 SWU - 8946,8947 -0.0010 i 0.0074 Oct,1997 Gr. Beta 2.9772 1 0.6530 2.2888 0.5953 2.6330 1 0.4418 SWU - 8946,8947 Oct,1997 H-3 187.7210 i 97.3682 125.5659 94.9331 CW - 8230,8231 156.6435 1 67.9943 Oct,1997 Gr. Beta 3.6262 1 1.7126 4.9561 1.7938 4.2911 1.2400 CW - 8230,8231 Oct,1997 Gr. Beta 1.7276 1 0.9533 0.1316 1.1929 CW - 8100,8101 0.9296 0.7635 Oct,1997 Cr. Beta 4.1481 i 1.6095 4.5744 i 1.5764 4.3612 1.1264 CW - 8100,8101 Oct,1997 Gr. Beta ,
-0.5655 i 0 8528 0.9791 1.2280 SS - 8501, 8502 0.2068 0.7475 Oct,1997 Gr. Alpha 7.9580 3.4566 6.5709 3.1487 SS 8501, 8502 7.2645 2.3379 Oct,1997 Gr. Beta 19.4568 i 2.9472 17.6686 2.6664 18.5627 1.9872 SS - 8501, 8502 Oct,1997 K-40 12.4630 i 0.4450 13.4420 0.7910 12.9525 0.4538 CW - 8310,8311 Oct,1997 Gr. Beta 2.1293 i 1.4423 2.1830 1.4550 2.1562 1.0243 CW - 8310,8311 Oct,1997 Gr. Beta 0.1798 t l.1387 -0.0397 1.1504 0.0701 0.8093 CW - 8376,8377 Oct,1997 Gr. Beta 4.7932 i 2.0194 7.3047 1.3637 6.0490 1.2184 CW - 8376,8377 Oct,1997 Gr. Beta 0.5653 1.8020 -0.0566 1.7632 0.2544 1.2606 MI- 8442,8443 Oct,1997 1-131 -0.0290 0.2689 0.1059 1 0.2666 0.0384 0.1893 MI - 8442,8443 Oct,1997 K-40 1,591.7000 i 178.0000 j
1,456.0000 116.0000 1,523.8500 106.2309 I SWU - 8543,8544 Oct,1997 Gr. Beta 2.2027 i 0.6193 2.1585 0.6134 2.1806 0.4358 l SWU - 8543,8544 Oct,1997 H-3 120.4712 i 87.0152 174.9557 i 89.2606 147.7134 62.3280 WW - 8473,8474 Oct,1997 H-3 -28.9600 i 77.6404 27.1500 1 80.2139 -0.9050 55.8174 WW - 8566,8567 Oct,1997 Co-60 0.4520 i l.7400 0.3400 4.0500 0.3960 2.2040 WW - 8566,8567 Oct,1997 Cs-137 1.0300 i 2.2000 -0.7300 2.8600 0.1500 1 1.8041 LW - 8608,8609 Oct,1997 Gr. Beta 2.8483 1 0.6660 2.3035 0.6052 2.5759 0.4500 i i
A5-11
Table A-5. In-house " duplicate" samples.
Concentration in pCi/L' Lab Sample Codes
- First Second Date Analysis Result Averaged MI- 6587,8588 Result Result Nov,1997 I-131 -0.0013 i 0.1396 0.0109 0.1350 MI- 8587,8588 Nov,1997 0.0048 0.0971 K-40 1,441.6000 i 160.0000 {
WW - 8654,8655 1,499.6000 176.0000 1,470.6000 118.9285 Nov,1997 Gr. Beta 0.6704 1 0.5213 WW - 8654,8655 0.8560 0.5226 0.7632 0.3691 I Nov,1997 H-3 131.2268 i 87.3749 87.6861 85.5477 CW - 8753,8754 Nov,1997 Gr. Beta 109.4565 61.1408 5.4805 1.9992 4.3820 2.0409 CW 8753,8754 Nov,1997 Gr. Beta 4.9312 1.4285 0.2821 i 1.7806 0.1129 1.7701 F - 9131,9132 - Nov,1997 0.1975 : 1.2554 Cs-137 ~ 0.0576 t 0.0192 F - 9131,9132 0.0568 0.0171 0.0572 0.0129 Nov,1997 Gr. Beta 2.9445 i 0.0965 F - 9131,9132 3.0473 0.0919 2.9959 0.0666 i Nov,1997 K-40 2.3452 i 0.3460 2.4680 0.3260 CW - 8854,8855 Nov,1997 Gr. Beta 2.4066 1 0.2377 5.6208 t 1.7991 3.5028 i 1.6326 CW - 8854,8855 Nov,1997 Gr. Beta 4.5618 1.2147 0.0000 i 1.1731 0.6107 1.1604 WW - 9087,9088 Nov,1997 0.3053 0.8250 !
H-3 20.1985 81.0438 WW - 9160,9161 73.4489 1 83.4219 46.8237 58.1535 Nov,1997 Co-60 -0.9580 i 9.1800 -0.4340 4.2400 WW - 9160,9161 Nov,1997 -0.6960 i 5.0559 Cs 137 -0.1440 i 2.3300 SWT - 9341,9342 -0.5270 1 2.0700 -0.3355 1.5583 Nov,1997 Gr. Beta 1.4657 i 0.7780 CW - 9410,9411 2.7123 i 0.8202 2.0890 0.5652 !
Dec,1997 Gr. Beta 3.2958i t.5674 CW - 9410,9411 4.2062 1 1.5722 3.7510 1.1100 !
Dec,1997 Gr. Beta 0.6244 1 1.1948 CW - 9466,9467 -0.6229 1.0939 0.0007 0.8099 Dec,1997 ' Gr. Beta 1.6082 1 1.6557 CW - 9466,9467 2.0375 t l.6921 1.8228 1.1837 Dec,1997 Gr. Beta -0.0563 i 1.7639 WW - 9603,9604 -1.1838 i 1.6912 -0.6201 1 1.2218 Dec,1997 Co-60 1.7300 i 1.7600 -0.6190 i 0.7560 WW - 9603,9604 Dec,1997 0.5555 0.9577 Co-60 1.7300 i 1.7600
.WW - 9603, 9604 -0.0389 0.3420 0.8456 0.8965 Dec,1997 Cs-137 ,
0.4460 i 2.0800 0.0557 1.2900 LW - 9789,9790 Dec,1997 0.2509 1.2238 !
l Co-60 0.1010 i 0.1080 LW - 9789,9790 0.1510 2.0300 0.1260 1.0164 Dec,1997 Cs-137 1.0000 i 2.1300 0.9130 2.0300 LW - 9789,9790 Dec,1997 Gr. Beta 0.9565 1.4712 5.6924 i 1.0952 4.5180 0.7757 CW - 9947, 9948 Dec,1997 Gr. Beta 5.1052 0.6711 0.9320 1 0.9447 1.5072 0.9762 l AP - 10249,10250 Dec,1997 1.2196 0.6792 Co-60 0.0000 i 0.0001 AP - 10249,10250 0.0004 0.0016 0.0002 0.0008 Dec,1997 Cs-137 0.0005 i 0.0008 0.0002 1 0.0003 0.0004 0.0004
' All concentrations are reported in pCi/ liter, except solid samples, which are reported in pCi/ g
- Lab codes are comprised of the sample media and the sample numbers. Client codes have protect client anonymity.
A5-12
i Table A-6. Department of Energy's Mixed Analyte Performance Evaluation Program (MAPEP),
comparison of MAPEP and Teledyne's Midwest Laboratory results for various sample media'.
Concentration
- Lab Sample Date - Teledyne Results MAPEP Result d Control Code Type Collected Analysis iStandard Deviation
- 1s, N=1 Limits STW-751 WATER Sep,1995 Am-241 1.370 i 0.120 1.320 0.070 1.056 - 1.584 STW-751 WATER Sep,1995 Co-57 91.000 i 0.950 92.380 i 0.600 73.904 110.856 STW-751 WATER Sep,1995 Cs-137 55.000 1 0.500 58.770 1 0.730 47.016 - 70.524 STW-751 WATER Sep,1995 Mn-54 99.170 i l.600 99.080 1.000 79.264 - 118.896 STW-751 WATER Sep,1995 Pu-238 1.700 i 0.040 1.830 t 0.080 1.464 - 2.196 STW-751 WATER Sep,1995 Pu-239 1.380 i 0.220 1.340 i 0.060 1.072 - 1.608 STW-751 WATER Sep,1995 Sr-90 13.730 1 0.950 15.690 0.300 12.552 - 18.828 STW-751 WATER Sep,1995 U-234 0.630 i 0.070 0.650 1 0.050 0.520 - 0.780 STW-751 WATER Sep,1995 U-238 0.700 0.020 0.650 1 0.050 0.520 - 0.780 STSO-776 SOIL Sep,1996 Am-241 27.000 28.700 1 2.830 20.900 - 37.310 STSO-776 - Standard deviation of three determinations was not reported in the Mixed Analyte Performance Evaluation Program Summary .
STSO-776 SOIL Sep,1996 Co-60 879.000 812.000 83.500 568.400 - 1,055.600 STSO-776 SOIL Sep,1996 Cs-137 1,716.000 1,531.000 i 193.420 1,071.700 - 1,990.300 STSO-776 SOIL Sep,1996 Pu-238 13.000 15.900 i 1.770 11.130 - 20.670 STSO-776 SOIL Sep,1996 Pu-239/240 18.000 19.700 i 1.960 13.790 - 25.610 STSO-776 SOIL Sep,1996 St-90 441.000 536.000 i 57.110 375.200 - 696.800 i
STSO-776 SOIL Sep,1996 U-234/233 59.000 63.900 i 7.270 44.730 - 83.070 STSO-776 SOIL Sep,1996 U-238 60.000 64.000 6.360 44.800 - 83.200
- Results obtained by Teledyne Brown Engineering Environmental Services Midwest Laboratory as a participant in the Department of Energy's Mixed Analyte Performance Evaluation Program, Idaho Operations office, Idaho Falls, Idaho.
- All results are in Bq/kg or Bq/L as requested by the Department of Energy.
- ' Unless otherwise indicated, the TBEESML results are given as the mean i 1 standard deviations for three
! determinations.
d MAPEP results are presented as the known values and expected laboratory precision
. (1 sigma,1 determination) and control limits as defined by the MAPEP.
1 A6-1
Table A-7.
Environmental Measurements Laboratory Quality Assessment Program (EML),
comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.
Concentration in Bq/L' l
l Lab Sample Date Code Type Control Collected Analysis Teledyne Result' EML Resultd Limits' STW-755 WATER Mar,19% Am-241 0.800 1 0.100 0.766 0.013 0.660 1.560 STW-755 WATER Mar,1996 Co-60 33.600 i 1.000 32.800 1 0.580 0.870 - 1.170
! STW 755 WATER Mar,1996 Cs-137 42.800 1 1.300 38.300 0.881 0.900 - 1.250 STW-755 ~ WATER Mar,19% - Fe-55 109.000 i 21.700 83.000 3.440 0.270 - 1.620
- STW-755 WATER Mar,1996 H3 434.000 34.100 251.000 11.400 0.690 - 1.910 j STW-755 WATER Mar,19% Mn-54 41.900 1.400 38.400 1.160 0.880 - 1.210 STW-755 WATER Mar,19% Pu-238 0.900 0.100 0.982 0.0 74 0.680 - 1.330 STW-755 WATER Mar,1996 Pu-239 0.700 i 0.100 0.772 1 0.056 0.620 - 1.380 STW-755 WATER Mar,1996 St-90 2.200 0.700 1.450 t 0.034 0.730 - 1.650 l STW-756 WATER Mar,1996 Gr. Alpha
' 2,180.000 1 53.500 1,S50.000 185.000 0.550 - 1.310 STW-756 WATER Mar,1996 Gr. Beta 872.000 27.000 744.000 74.000 0.750 - 1.650 j STSO 757 ' SOIL Mar,1996 Am 241 6.230 1 2.880 3.690 1 0.454 0.520 - 2.410 l STSO-757 SO!L Mar,19% Cs-137 404.000 0.150 359.000 i 10.000 0.740 - 1.400 STSO-757 SOIL Mar,19% K-40 525.000 i 23.300 465.000 30.000 0.700 - 1.590 STSO-757 SOIL Mar,1996 Pu-238 42.300 1 1.590 43.000 1 2.440 0.220 - 1.990 STSO-757 - SOIL Mar,19% Pu-239 9.000 1 0.700 9.230 1 0.346 0.620 - 1.990 STSO-757 SOIL Mar,1996 Sr-90 1,200.000 i 32.300 1,340.000 t 113.000 0.580 - 2.960 STSO-757 SOIL Mar,1996 Uranium 68.200 i 2.400 71.700 4.150 0 270 - 1.480 STVE-758 VEGETATION Mar,1996 Am-241 6.100i l.300
' 5.600 1 0.184 0.580 2.860 STVE-758 VEGETATION Mar,19% Cm-244 6.000 i 1.200 4.440 0.202 0.400 1.870 STVE-758 VEGETATION Mar,19% Co-60 65.600 i 4.000 59.700 1 0.963 0.640 - 1.490 STVE-758 VEGETATION Mar,19% Cs 137 1,100.000 2 12.600 944.000 16.200 0.750 - 1.480 STVE-758 VEGETATION . Mar,19% K-40 1,190.000 61.600 1,030.000 i 33.000 0.450 - 1.510 STVE-758 VEGETATION Mar,1996 Pu-239 9.200 i 1.300 9.820 1.220 0.600 - 1.980 STVE-758 VEGETATION Mar,1996 Sr-90 1,210.000 t 32.200 1,300.000 52.400 0.500 - 1.370 STAF-759 AIR FILTER Mar,19% Am 241 0.270 i 0.040 0.189 i 0.007 0.620 - 1.930 STAF-759 AIR FILTER Mar,1996 Ce-144 23.200 i 1.020 33.300 i 3.300 0.610 - 1.310 STAF-759 AIR FILTER Mar,19% Co-57 6.050 1 0.130 8.900 0.900 0.630 - 1.290 STAF-759 AIR FF.TER Mar,1996 Co-60 26.500 1 0.430 29.500 2.900 0.740 - 1.250 STAF-759 AlR FILTER Mar,1996 Cs-134 12.900 1 0.280 14.700 i 1.460 0.700 - 1.210 STAF-759 AIR FILTER Mar,1996 Cs-137 6.200 t 0.900 6.640 1 0.700 0.720 - 1.320 STAF-759 AIR FILTER Mar,1996 Mn-54 3.270 0.350 3.440 1 0.380 0 760 - 1.330 STAF-759 AIR FILTER Mar,19% Pu-238 0.080 i 0.020 0.096 0.002 0.610 - 1.550 STAF-759 AIR FILTER Mar,19% Pu-239 0.090 0.020 0.093 0.003 0.670 - 1.580
- STAF-759 AIR FILTER Mar,1996 Ru-106 10.200 1 1.850 11.600 1.440 0.540 - 1.590 STAF-759 - AIR FILTER Mar,19% Sb-125 10.100 i 0.750 9.780 1 1.030 0.350 - 1.400 f STAF-759 AIR FILTER Mar,19% Sr-90 1.070 i 0.230 1.060 1 0.037 0.620 - 2.260 STAF-759 AlR FILTER Mar,19% Uranium 0.118 i 0.020 0.107 0.003 0.790 - 2.860 I A7-1
Table A 7.
Environmental Measurements Laboratory Quality Assessment Program (EML),
comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.
Concentration in Bq/L' Lab Sample Date Code Type Collected Analysis Control -
Teledvne Result' EML Resultd Limits' !
STAF-760 AIR FILTER Mar,19% Gr. Alpha 2.210 0.050 1.620 t 0.150 0.820 - 1.580 STAF-760 AIR FILTER Mar,19% Gr. Beta 1.950 1 0.040 1.770 0.150 0.750 1.940 STW-770 WATER Sep,1996 Am-241 1.300 i 0.200 1.0S0 0.040 0.640 1.730 STW-770 WATER Sep,1996 Co-60 65.000 1 2.210 61.100 0.730 0.920 - 1.180 STW-770 WATER Sep,1996 Cs-137 96.100 i 3.010 89.500 1.360 0.900 - 1.280 STW-770 WATER Sep,1996 Gr. Alpha 993.000t 12.200 1,210.000 121.000 0.500 - 1.290 l STW-770 WATER Sep,1996 Gr. Beta 579.000 i 8.070 540.000 54.000 0.600 - 1.640 l STW-770 WATER Sep,1996 H-3 488.000 34.600 587.000 58.000 0.650 J 1.910 STW-770 WATER Sep,1996 Mn-54 65.000 2.960 60.500 0.550 0.870 - 1.220 i STW-770 WATER Sep,1996 Pu-238 1.320 0.333 1.910 1 0.070 0.740 - 1.270 An investigation was conducted. No errors in calculations or transcription were noted. The analysis repeated in duplicate under the observation of the Technical Lead. No discrepancies were noted in the performance of the procedure. The result of the reanalysis was 2.14 0.11 Bq/L No further action is pla STW-770 WATER Sep,1996 Pu-239 0.698 0.247 0.840 0.030 0.780 - 1.420 STW-770 WATER Sep,1996 Sr-90 3.600 0.700 2.710 0.240 0.720 - 1.660 i STW-770 . WATER Sep,1996 U-234 0.5171 0.196 0.480 0.040 0.770 - 1.530 STW 770 WATER Sep,1996 U-238 0.416 1 0.118 0.480 1 0.370 0.770 - 1.350 STSO-771 SOIL Sep,1996 Am-241 15.600 1 3.830 13.500 0.510 0.520 - 2.650 STSO-771 SOlt Sep,1996 - Co-60 4.030 1 2.500 2.920 0.210 0.500 - 1.500 STSO-771 SOIL Sep,1996 Cs-137 1,750.000 1 24.400 1,550.000 1 22.200 0.800 - 1.340 STSO-771 SOIL Sep,19% K-40 369.000 1 59.500 300.000 1 25.000 0.730 - 1.670 STSO-771 SOIL Sep,1996 Pu-238 0.770 i 0.360 1.130 1 0.240 0.400 - 1.900 l STSO-771 SOIL Sep,1996 Pu-239 24.000 i l.940 21.800 1 1.080 0.660 1.930 STSO-771 SOlt Sep,1996 Sr-90 63.600 3.950 69.900 t 5.100 0.460 - 2.840 STSO-771 SOlt Sep,19% U-234 37.200 3.750 39.200 2.440 0.380 - 1.260 STSO-771 SolL Sep,1996 U-238 40.800 i 3.980 41.600 0.610 0.350 - 1.550 STVE-772 VEGETATION Sep,1996 Am-241 1.5301 0.884 1.230 t 0.410 0.680 - 2.780 STVE-772 VEGETATION Sep,1996 cm-244 0.612 0.495 0.830 0.120 0.490 - 1.690 STVE-772 VEGETATION Sep,1996 Co-60 14.000 i 4.420 10.900 0.710 0.620 1.420 STVE-772 VEGETATION Sep,1996 Cs-137 219.000 1 10.100 190.000 6.680 0.810 - 1,450 STVE-772 VEGETATION Sep,1996 K-40 1,160.000 i 99.400 992.000 29.000 0.790 - 1.500 STVE-772 VEGETATION Sep,1996 Sr-90 1,420.000 1 35.100 1,390.000 12.000 0.480 - 1.290
- STAP-773 AIR FILTER Sep,1996 Co-57 11.800 i 0.296
! 14.800 0.814 0.620 1.220 STAP-773 AIR FILTER Sep,1996 Co-60 9.230 1 0.402 8.640 1 0.431 0.740 1.240 l STAP-773 AIR FILTER Sep,1996 Cs-134 9.620 1 0.376 10.800 0.392 0.720 1.210 j STAP-773 AIR FILTER Sep,19% Cs-137 8.720 t 0.403 8.520 0.366 0.720 1.320 i
STAP-773 AIR FILTER Sep,19% Gr. Alpha 0.731 1 0.037 1.150 0.110 0.830 - 1.550 An investigation was conducted and a transcription error while calculating the result was discovered. The recalculated value is 1.1510.01Bq/ filter, No further action is planned. !
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Table A-7.
Environmental Measurements Laboratory Quality Assessment Program (EML),
comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.
Concentration in Bq/L' Lab Sample Da te Code Type Control Collected Analysis Teledyne Result' ,
EML Result' Limits' !
STAP-773 AIR FILTER Sep,1996 Gr. Beta 0.540 0.037 0.500 0.050 0.730 - 1.840 STAP 773 AIR FILTER Sep,1996 Mn-54 l 7.060 0.4 72 6.350 0.270 0.750 - 1.270 STAP-773 AIR FILTER Sep,1996 Ru-106 !
11.500 3.190 10.800 1.140 0.580 1.300 STAP-773 AIR FILTER Sep,1996 Sb-125 12.400 0.965
)
10.800 0.540 0.600 - 1.390 STW-788 WATER Mar,1997 Am-241 l 0.8401 0.220 0.837 0.028 0.640 - 1.730 STW-788 WATER Mar,1997 Co-60 96.000 t 3.500 90.850 1 1.150 0.920 1.180 STW-788 WATER Mar,1997 Cs-137 77.000 i 3.500 69.780 1.230 0.900 - 1.280 STW-788 WATER Mar,1997 Fe-55 l 175.500 1 25.400 235.000 20.000 0.310 - 1.540 STW-788 WATER Mar,1997 Gr. Alpha 1,042.600 1 36.800 1,130.000 10.000 0.500 - 1.290 STW-788 WATER Mar,1997 Gr. Beta 591.400 i 23.300 744.000 10.000 0.600 - 1.640 STW-788 WATER Mar,1997 H-3 272.000 1 29.700 250.300 4.200 0.650 1.910 STW-788 WATER Mar,1997 Mn-54 23.700 3.400 20.850 ! 0.310 0.870 - 1.220 STW-788 WATER Mar,1997 Pu-238 1.400 i 0.200 1.291 0.063 0.740 - 1.270 STW-788 WATER Mar,1997 Pu-239 0.900 0.100 0.850 0.050 0.780 - 1.420 STW-788 WATER Mar,1997 Sr-90 25.500 i l.700 23.200 1.350 0.720 - 1.660 STW-788 WATER Mar,1997 U 1.500 1 0.200 1.105 0.050 0.350 - 1.420 STSO-790 SOIL Mar,1997 Am-241 6.740 1 3.730 5.680 0.500 0.520 - 2.650 STSO-790 SOIL Mar,1997 Co-60 2.010i 1.170 1.060 0.120 0.500 - 1.500 The sample size was too small for an accurate measurement. The activity error overlap the known value.
STSO-790 SOIL Mar,1997 Cs 137 918.640 8.400 825.500 14.100 0.800 - 1.340 STSO-790 SOIL Mar,1997 K-40 359.140 32.100 334.250 7.140 0.730 - 1.670 STSO-790 SO!L Mar,1997 Pu-238 0.300 i 0.200 0.530 0.110 0.400 - 1.900 STSO-790 SOIL Mar,1997 Pu-239 132.420 1 5.170 134.930 17.100 0.660 1.930 STSO-790 SOIL Mar,1997 Sr-90 38.830 1 5.770 40.310 0.420 0.460 - 2.840 STSO-790 SOIL Mar,1997 U 79.260 3.800 81.270 4.830 0.270 - 1.360 STVE-791 VEGETATION Mar,1997 Am-241 1.673 1 0.688 1.183 0.113 0.680 - 2.780 STVE-791 VEGETAT10N Mar,1997 Cm-244 0.688 1 0.468 0.900 0.050 0.490 - 1.690 STVE-791 VEGETATION Mar,1997 Co-60 16.914 i 3.580 12.500 0.320 0.620 - 1.420 STVE-791 VEGETATION Mar,1997 Cs-137 216.667 1 9.383 189.250 7.270 0.810 - 1.450 STVE-791 VEGETATION Mar,1997 Pu-239 1.771 i 0.817 1.942 0.222 0.650 - 1.950 STVE-791 VEGETATION Mar,1997 Sr-90 361.130 1 19.715 361.000 43.300 0.480- 1.290 STAP-792 AIR FILTER Mar,1997 Co-57 9.528 i 0.230 10.810 1.000 0.620 - 1.220 l STAP-792 AIR FILTER Mar,1997 Co-60
' 5.325 i 0.266 5.010 0.300 0.740 - 1.240 STAP-792 AIR FILTER Mar,1997 Cs-134 10.767 i 0.337 10.880 i 1.000 0.720 - 1.210 STAP 792 AIR FILTER Mar,1997 Cs-137 9.116 i 0.404 8.700 0.800 0.720 - 1.320 STAP-792 AIR FILTER Mar,1997 Gr. Alpha 1.199 0.045 0.960 1 0.050 0.830 - 1.550 STAP-792 AIR FILTER Mar,1997 Gr. Beta 0.608 0.024 0.450 2 0.030 0.730 - 1.840 STAP-792 AIR FILTER Mar,1997 Mn-54 8.494 i 0.429 7.620 0.600 0.750 - 1.270 A7-3
Table A-7.
Environmental Measurements Laboratory Quality Assessment Program (EML),
comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.
Concentration in Bq/L" Lab Sample Date Code Type Control Collected Analysis Teledyne Result' EML Result d Limits
- STAP-792 AlR FILTER Mar,1997 Pu-238 0.022 i 0.016 0.100 0.006 0.620 - 1.460 The cause of the deviation for the transuranic analysis (Pu-238,239, U) is unknown. A dilution error is suspected.The analysis is being repeated.
STAP-792 AIR FILTER Mar,1997 Pu-239 0.031 1 0.010 0.119 0.006 0.500 - 1.500 STAP 792 AIR FILTER Mar,1997 Sb-125 14.118 1.099 12.330 1.000 0.600 - 1.390 STAP-792 AIR FILTER Mar,1997 Sr-90 1.291 0.2 75 1.450 0.149 0.660 - 2.650 STAP-792 AIR FILTER Mar,1997 U 0.150 0.020 0.211 0.008 0.808 - 3.360 STW-805 WATER Sep,1997 Co-60 23.630 1 1.450 23.300 1.200 0.920 - 1.180 STW-805 WATER Sep,1997 Cs-134 63.500 1 2.600 66.000 2.600 0.500 - 1.500 STW-805 WATER Sep,1997 Cs-137 34.880 1 2.430 34.300 1.700 0.900 - 1.280 STW-805 WATER Sep,1997 Fe-55 101.730 33.530 115.000 10.000 0.310 1.540 STW-805 WATER Sep,1997 Gr. Alpha 597.000 12.000 557.000 60.000 0.500 - 1.290 STW-805 WATER Sep,1997 Gr. Beta 985.000 i 13.000 712.000 70.000 0.600 - 1.640 STW-805 WATER Sep,1997 H-3 227.600 i 1.800 115.000 6.000 0.650 - 1.910 The sample was acidic, causing a breakdown of resin in the tritium column. The sample was neutralized to pH 7 and reanalyzed. Results of reanalysis: 116.2 3.6 Bq/L.
STW-805 WATER Sep,1997 Mn-54 38.480 3.230 37.800 1.900 0.870 - 1.220 STW-805 WATER Sep,1997 Sr-90 3.460 i 0.690 2.940 i 0.180 0.720 - 1.660 STVE-806 VEGETATION Sep,1997 Co-60 32.330 5.560 32.400 1.600 0.620 - 1.420 STVE-806 VEGETATION Sep,1997 Cs-137 627.330 1 16.670 624.000 31.000 0.810 - 1.450 STVE-806 VEGETATION Sep,1997 K-40 1,091.670 1 95.180 1,130.000 70.000 0.790 - 1.500 STVE-806 VEGETATION Sep,1997 Sr-90 1,335.000 1 32.000 1,434.000 75.000 0.480 - 1.290 STSO-807 SOIL Sep,1997 Cs-137 1,239.440 1 22.460 810.000 40.000 0.800 - 1.340 The sample size was not standard. The sample was reanalyzed using a different geometry. Results of reanalysis: Cs-137 - 813.li9.0 Bq/kg; K 275.9 34.6 Bq/kg.
STSO-807 SOIL Sep,1997 K-40 478.000 i 29.000 315.000 i 70.020 0.730 - 1.670 STSO-807 SOIL Sep,1997 Pu-239 10.800 0.400 10.160 0.370 0.660 - 1.930 STSO-807 SOIL Sep,1997 Sr 90 31.480 1 5.560 34.750 1.000 0.460 - 2.840 STSO-807 SOIL Sep,1997 U 57.000 1.100 72.900 0.850 0.270 - 1.360 STAP-808 AIR FILTER Sep,1997 Gr. Alpha 1.820 i 0.080 1.490 1 0.090 0.830 - 1.550 STAP-808 AIR FILTER Sep,1997 Gr. Beta 3.250 i 0.080 3.000 0.140 0.730 - 1.840 STAP-808 AIR FILTER Sep,1997 Pu-238 0.230 1 0.100 0.210 0.007 0.620 - 1.460 STAP-808 AIR FILTER Sep,1997 U 0.130 0.100 0.110 t 0.004 0.800 - 3.360 STAP-809 AIR FILTER Sep,1997 Ce 144 16.250 i 1.670 19.120 t 0.700 0.500 - 1.500 STAP-809 AIR FILTER Sep,1997 Co-57 )
10.570 i 0.270 12.640 1 0.430 0.620 - 1.220 l STAP-809 AIR FILTER Sep,1997 Co-60 9.820 1 0.270 10.730 10.900 0.740 - L240 '
! STAP-809 AIR FILTER Sep,1997 Cs-134 24.700 i 0.490 28.170 0.730 0.720 - 1.210 STAP-809 AIR FILTER Sep,1997 Cs-137 ,
7.240 i 0.370 7.310 i 0.250 0.720 - 1.320 l STAP-809 AIR FILTER Sep,1997 Mn-54 6.800 1 0.430 6.720 0.270 0.750 - 1.270 l A7-4 l
Table A 7. Environmental Measurements Laboratory Quality Assessment Program (EML),
comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.
Concentration in Bq/L" j Lab Sample Date Code Type Control Collected Analysis Teledyne Result' EML Result' Limits' STAP-809 AIR FILTER Sep,1997 Sb-125 17.980 1.270 16.120 2 0.790 0.600 - 1.390 STAP-809 AIR FILTER Sep,1997 - Sr-90 2.830 0.370 l 2.760 : 0.100 0.660 - 2.650
- The Environmental Measurements Laboratory provides the following nuclear species : Air Filters, Soil, Tissue, Vegetation and Water. Teledyne does not participate in the Tissue program.
- Results are reported in Sq/L with the following exceptions: Air Filter results are reported in Bq/ Filter, Soi results are reported in Bq/Kg, Vegetation results are reported in Bq/Kg.
' Teledyne results are reported as the mean of three determinatians standard deviation.
- The EML result listed is the mean of replicate determinations for each nuclide the standard error of the mean.
' 7; controllimits are reported by EML as the ratio of Reported Value / EML Value and are established from per<. atiles of historic data distributions (1982-1992). The evaluation of this historic data and the development of the controllimits is presented in DOE report EML-564.
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APPENDIX B DATA REPORTING CONVENTIONS B-1
Data Reporting Conventions 1.0 All activities except gross alpha and gross beta are decay corrected to collection time or the end of the collection period.
2.0. Single Measurements Each single measurement is reported as follows:
x s where x = value of the measurement; s = 20 counting uncertainty (corresponding to the 95% confidence level).
In cases where the activity is found to be below the lower limit of detection L it is reported as
<L where L = the lower limit of detection based on 4.660 uncertainty for a background sample.
3.0. Duplicate analyses 3.1 Individual results: x1 is1 x2 i s2 Reoorted result: xis where x = (1/2)(x3 + x2) s = (1/2) k sf + s!
3.2. Individual results: <Li
<L2 Reoorted result: <L where L = lower of L 3and L2 3.3. Individual results: xis
<L Reoorted result: x i s if x 2 L;
<L otherwise B. 2
4.0 Computation of Averages and Standard Deviations 4.1 Averages and standard deviations listed in the tables are computed from all of the individual measurements over the period averaged; for example, an annual standard deviation would not be the average of quarterly standard deviations. The average x and standard deviation s of a set of n numbers x3, x2 xnare defined as follows:
x=fEx s= I(x- x)2 n-1 L
l 42 Values below the highest lower limit of detection are not included m the average.
4.3 If all of the values in the averaging group are less than the highest LLD, the highest LLD is reported.
4.4 If all but one of the values are less than the highest LLD, the single value x and associated two sigma error is reported.
4.5 In rounding off, the following rules are followed:
l 4.5.1. If the figure following those to be retained is less than 5, the figure is dropped, and the retained figures are kept unchanged. As an example,11.443 is rounded off to 11.44.
4.5.2. If the figure following those to be retained is equal to or greater than 5, the figure is dropped and the last retained figure is raised by 1. As an example,11.445 is rounded off to 11.45.
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4 APPENDIX C l Effluent Concentration Limits for Radioactivity in Air and Water Above Backgromid in Unrestricted Areas C-1
l Table C-1. Effluent concentration limits for radioactivity in air and water above natural background in unrestricted areasa ,
Air Water Iodine-131b 0.29 pCi/m3 Strontium-89 8,000 pCi/L Strontium-90 500 pCi/L l
Cesium-137 1,000 pCi/L Barium-140 8,000 pCi/L l
Iodine-131 1000 pCi/L i l
Potassium-40C 4,000 pCi/L Tritium 1 x 106 pCi/L l
a Taken from Code of Federal Regulations Title 10, Part 20, Table 2 and appropriate footnotes. Concentrations may be averaged over a period not greater than ene year.
b From 10 CFR 20 but adjusted by a factor of 700 to reduce the dose resnit.ng from the air-grass-cow-milk-child pathway.
c A natural radionuclide.
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APPENDIX D
SUMMARY
OF THE LAND USE CENSUS 1
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L Appendix D SummaIV of the Land Use Census The Duane Arnold Energy Land Use Census for 1997 was completed during the third week of September 1997. All milk animals and gardens greater than 500 square feet were identified within three miles for each of the 16 meteorological sectors. If none were identified within the three mile range, additional surveys were performed out to a distance of five miles. The Cedar River was suneyed by boat on July iIth 1997 for water use downstream of the DAEC to Cedar Rapids.
l There were 147 gardens found in the 1997 Census. This number exceeds the number of gardens found in the 1996 survey by 10. This difference can be attributed to the removal of 47 gardens and the addition of 57 new gardens.
Milk animals locations remained unchanged since the 1995 census. Two of the locations j have goats that do not provide samples during the winter months.
l The locations of the nearest resident for each sector remained the same. Twenty-two new homes were built or were under construction within three miles of the DAEC, compared to the thirty new homes identified in 1996. Most of the new houses built were located in the sectors between the plant and Cedar Rapids (SSE, and SE) and in Palo (S and SSW).
A listing of the newly identified homes is attached.
The Cedar River survey revealed no new withdrawals of river water compared to previous j surveys. Irrigation of the strawberry farm in Palo and fishing remain the only food i pathway uses of river water between the DAEC and Cedar Rapids.
l Several adjustments were made to the MIDAS dose projection model based on the results of this census. They include changes to the location of the nearest gardens for the NNE, ENE, ESE, SE, SSW, SW and WNW sectors.
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I APPENDIX E l
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ANNUAI. RADIATION DOSE ASSESSMENT l
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Appendix E Annual Radiation Dose Assessment The annual offsite radiation dose to a member of the public was determined by assessment of environmental dosimeter results and by calculations based on monitored effluent releases.
Section A. Dose Contribution from Direct Radiation Direct radiation dose from the operation of the DAEC was reported by TLDs placed at locations in the surrounding environment as described in the Offsite Dose Assessment Manual (ODAM).
- 1. Pre-operational and 1997 TLD results were compared using a paired difference test.
No significant differences in the TLD populations were observed for the 0.5 mile and one mile TLD populations using a confidence level of 99%.
- 2. As stated in Part 1, page 8 of this repon, no plant effect was indicated by the TLDs when dose results were compared to the estimated average natural background for Middle America.
Section B. Estimated Offsite Dose from EfHuent Releases The contribution of dose to a member of the public most likely to be exposed from effluent releases was calculated by the Meteorological Information and Dose Assessment System (MIDAS) computer program in accordance with ODAM. The calculation methods follow those prescribed by Reg Guide 1.109. Because there were no nuclides detected in the environment at or beyond the site boundry that were due to the operation of the DAEC, no comparison of calculsted dose from stack releases and dose calculated from environmental contamination was performed.
Results of the MIDAS dose calculations are discussed below and are shown in tabular form on page E-4
- 1. There were no releases of radioactive material to liquid effluents in 1997, i
- 2. The dose to air from noble gases released was 2.76E-03 mrad from gamma radiation at 455 meters South and 2.87E-04 mrad beta radiation at 4022 meters WNW. .
)
- 3. The total body dose equivalent to the maximally exposed individual from noble gases was 1.78E-03 mrem, at 805 meters West.
E-2
- 4. The skin dose equivalent to the maximally exposed individual from noble gases was 1.82E-03 mrem, at 805 meters West.
- 5. The maximally exposed organ due to iodines and particulates with half-lives greater than eight days was the thyroid of a child at 805 meters West, with and estimated dose equivalent of 5.62E-03 mrem.
==
Conclusion:==
No measureable dose due to the operation of the DAEC was detected by environmental TLDs in 1997. The calculated doses are below the regulatory limits stated in Appendix I to 10 CFR 50 and in 40 CFR 190.
Estimated Maximum Offsite Individual Doses for 1997 ;
Type Age Distance Direction Dose or Dose Annual 10 CFR Group (meters) Equivalent 50, AppendixI (mrem) Limit Direct Radiation None *
(as measured by TLDs)
Liquid Releases None Noble Gas Gamma Air Dose 481 S 2.76E-03 mrad 10 mrad Beta Air Dose 4022 WNW 2.87E-04 mrad 20 mrad ;
Total Body All 805 W l.78E-03 mrad * )
i Skin All 805 W l.82E-03 mrad * '
Pr.rticulates & lodines l Organ Dose Child - 805 W 5.62E-03 15 mrem Thyroid mrem
- No Appendix I limit but is used to detennine compliance with 40 CFR 190 limits of 25 mrem total body and 75 mrem thyroid.
E-? ~
T TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY 700 LANDWEHR ROAD NORTHBROOk ILLINO!S 60062 2310 (M7) $644?DO
- f AX (647) $64-4517 REPORT TO IES UTILITIES,INC.
CEDAR RAPIDS, IOWA RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP)
FOR THE DUANE ARNOLD ENERGY CENTER CEDAR RAPIDS, IOWA Docket No. 50-331 ANNUAL REPORT - PART II DATA TABULATIONS AND ANALYSES JANUARY - DECEMBER 1997 PREPARED AND SUBMITTED BY TELEDYNE BROWN ENGINEERING ENVIRONMENTAL b?RVICES MIDWEST LABORATORY PROJECT NO. 8001
('+
Reviewed and f f Approved by / 'J/ ; 0 ; ')
Brm ia pdob,'M.S.
Te Qc pl Lead b
- April 2,1998
TABLE OF CONTENTS Section Pace Lis t of Ta bles . . . .. . . . . . . . . . . . . . . ... . . . . . . . . . . . . . . . . . . . . . . . . . . . . ...iii
1.0 INTRODUCTION
. .. ....... .... .... .. . . .. ... . . . . . . . . .. .. .. . . .v 2.0 LISTING OF MISSED SAMPLES ..... ... ....... . . . . . . . . . . . . . . .vi 3.0 DAT A TA B LES .. ... . . . . . . . ... . . .. . . . .. .... . . . . . .. .. . . . . . . . . . . ..vii 1
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I LIST OF TABLES h Title Page 1
Airborne particulates collected at Location D-1, (Cedar Rapids),
analysis for gross beta ...... ..... . .... ... .. . . . . . .1-1 2 Airborne particulates and iodine collected at Location D-2 (Marion),
analysis for gross beta and iodine-131... .. . . . .. . .2-1 3 Airborne particulates collected at Location D-3 (Hiawatha), analysis for gross beta.. .. .. . . . . . . . . .. . . . . .3-1 l 4 Airborne particulates and iodine collected at Location D-5 (Palo),
analysis for gross beta and iodine-131.. . . .4-1 5 Airborne particulates collected at Location D-6 (Center Point),
analysis for gross beta . ... .. .. . ... ... . . . . . . . . . . . . . . ..5-1 l
6 Airborne particulates and iodine collected at Location D-7, (Shellsburg), analysis for gross beta and iodine-131. . . . . .6-1 i
7 Airborne particulates and iodine collected at Location D-8 (Urbana),
analysis for gross beta and iodine-131.. .. . . . . . . . .7-1 8 Airborne particulates collected at Location D-10 (Atkins), analysis for gross beta... . . . . . . . . . . .. .. . . . . . .8-1 9 Airborne particulates and iodine collected at Location D-11 (Toddville), analysis for gross beta and iodine-131. . .. . . . 9-1 10 Airborne aarticulates collected at Location D-13 (Alburnett),
ana;ysis for gross beta . . ... . . . . . . . . . . . . .10-1 11 Airborne particulates and iodine collected at Location D-15 (on-site, north), analysis for gross beta and iodine-131.. .11-1 12 Airborne particulates collected at Location D-16 (on-site, south),
analysis for gross beta ..... .. . . . .12-1 13 Airborne particulate samples, quarterly composites of weekly samples, analysis for gamma-emitting isotopes.. .13-1 14 Ambient gamma radiation (TLD), quarterly exposure . . .14-1 15 Milk samples, analysis for iodine-131 and gamma emitting isotopes.. .15-1 16 Ground water samples, analysis for gross beta and tritium.. . . . . . . .16-1 17 Vegetation samples (broadleaf), analysis for iodine-131 and gamma-emitting isotopes.. . . . . .. .. .17-1 I
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LIST OF TABLES (continued) h Title Page i
18 Vegetation samples (hay and grain), analysis for gamma-emitting isotopes.. . . .. .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .18-1 19 Surface water samples, analysis for iodine-131 and gamma-emitting isotopes .. ... ..... ... . . . . . . , - . . . . . . . . . . . .. . . . . . . . . .. .19-1 20 Surface water samples, analysis for potassium-40, iodine-131 and gamma-emitting isotopes.... .. . . . . . . . . . . . .. .. .20-1 21 Surface water samples, quarterly composites of monthly samples, analysis for tritium...... .. .. . .. .. .. . ... . .21-1 22 Fish samples, analysis for gamma-emitting isotopes .. . .. . . . .22-1 23 River sediment samples, analysis for gamma-emitting isotopes.. .23-1 ;
24 Precipitation samples, analysis for gamma-emitting isotopes.. .24-1 25 Precipitation samples, quarterly composites of monthly samples, {
analysis for tritium... . . . . . . . .. .. . . . . . . . .. .25-1 !
26 Meat samples, analysis for gamma-emitting isotopes . . . . . . .26-1 :
27 Soil samples, analysis for strontium-90 and gamma-emitting isotopes.. .. . . . . . . . . . . . . . . . . . . . . .. . . . . . . . . . 27-1 iv w
1.0 INTRODUCTION
The following constitutes a supplement to the Annual Report for the Radiological Environmental Monitoring Program conducted at the Duane Arnold Energy Center, Palo, Iowa in 1997. Results of completed analyses are presented in the attached tables.
For information regarding sampling locations, type and frequency of collection, and sample codes, please see Tables 5.3 - 5.5 and Figures 5.1 and 5.2 of Part I.
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.2.0 LISTING OF MISSED SAMPIP4 I Collection Date I
Sample Location (s) or Period Com.ments l
Milk I-131, Gamma D-93 01-07-97 Sample not available.
Milk I-131, Gamma D-101 01-07-97 Sample not available.
AP Gross Beta D-13 01-23-97 Samplelost in strong wind.
Milk I-131, Gamma D-93 02-04-97 Sample not availzble.
Milk I-131, Gamma D-101 02-04-97 Sample not available.
Milk I-131, Gamma D-105 06-17-97 Lost in shipment.
TLD Ambient Gamma D-31, 91 3rd Qtr.,1997 Samples lost in the Feld.
TLD Ambient Gamma D-35 4th Qtr.,1997 Samples lost in the field.
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1 3.0 DATA TABLES 4
l i
V55
DUANE ARNOLD Table 1. Airborne particulates and charcoal canisters, analysis for gross beta.
Location: D-1 (Cedar Rapids)
Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Cross Beta Required LLD Qa1Q 0310 01-09-97 286 0.028 0.004 07-10-97 285 0.015 I 0.003 01-16-97 285 0.029 i 0.004 07 17-97 285 0.023 0.003 01-23-97 287 0.022 0.003 07 24-97 286 0.023 0.003 01-30-97 284 0.028 i 0.004 07-31-97 286 0.024 0.004 02-06-97 285 0.029 1 0.004 08-07 97 286 0.025 0.003 02-12-97 246 0.024 0.003 08-14-97 284 0.025 0.003 02-20-97 325 0.033 1 0.004 08-21-97 286 0.020 0.003 02-27-97 286 0.022 i 0.003 08-28-97 285 0.041 0.004 03-06-97 286 0.021 1 0.003 09-04-97 286 0.032 0.003 03-13-97 284 0.023 0.003 09-11-97 285 0.030 0.004 03-20-97 285 0.023 1 0.003 09-18-97 286 0.043 0.004 l 03-27-97 288 0.021 0.003 09-25-97 286 0.024 0.004
- 04-03-97 282 0.014 0.003 10-02-97 286 0.023
- 0.003 1st Quarter Meanis.d. 0.024 1 0.005 3rd Quarter Mean s.d. 0.027 0.008 04-10-97 284 0.017 1 0.003 1()-09-97 235 0.036 0.004 04-16-97 246 0.026 1 0.004 10-16-97 285 0.027 0.003 04-24-97 326 0.021 i 0.003 10-23-97 286 0.024 0.004 05-01 97 289 0.016 0.003 10-30-97 '277 0.032 0.004 05-08-97 147' O.040 1 0.006 11-06-97 286 0.021 0.003 05 15-97 287 0.013 1 0.003 11-12-97. 245 0.016 0.003 05-22-97 284 0.014 1 0.003 11-20-97 327. 0.039 0.004 05-29-97 285 0.017 i o.003 11-26-97 244 0.059 0.005 06-04-97 245 0.013 1 0.003 12-04 97 327 0.025 0.003 06-12-97 328 0.018 i 0.003 12-11-97 285 0.013 0.003 '
06-19-97 284 0.015 1 0.003 12-18 s7 284 0.037 0.004 06-26-97 285 0.021 0.003 12-26-97 326 0.031 0.003 07-03-97 286 0.020 1 0.003 01-02-98 285 0.022 0.003 2nd Quarter Mean s.d. 0.019 1 0.007 4th Quarter Mean s.d. 0.029 0.012 1
Cumulative Average: 0.025 Previous Annual Average: 0.024
' Low volume due to power loss at substation.
1-1
DUANE ARNOLD Table 2. . Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131'.
Location: D-2 (Marion)
Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired LLD g g 01-09-97 287 0.029 i 0.004 07-10-97 285 0.016 1 0.003 01-16-97 285 0.031 i 0.004 07-17-97 285 0.024 0.003 01-23-97 287 0.023 1 0.003 07-24-97 286 0.025 0.003 01-30-97 285 0.026 i 0.004 07-31-97 287 0.030 0.004 02-06-97 285 0.028 i 0.004 08-07-97 286 0.029 0.003 02-12-97 246 0.027 1 0.004 08-14-97 283 0.022 0.003 02-20-97 324 0.035 i 0.004 08-21-97 287 0.017 0.003 02-27-97 287 0.024 1 0.003 08-28-97 284 0.037 0.004 03-06-97 286 0.026 0.003 09-04-97 287 0.026 0.003 03-13-97 284 0.025 i 0.003 09-11-97 284 0.027 1 0.003 03-20-97 284 0.024 i 0.003 09-18-97 286 0.037 0.004 03-27-97 289 < 0.003 6 09-25-97 286 0.023 0.003 04-03-97 282 0.016 1 0.003 10-02-97 288 0.020 1 0.003 1st Quarter Mean s.d. 0.026 1 0.005 3rd Quarter Meants.d. 0.026 0.007 04-10-97 286 0.017 1 0.003 10-09-97 284 0.033 0.004 04-16-97 246 0.025 1 0.004 10-16-97 265 0.028 0.003 04-24-97 325 0.020 i 0.003 10-23-97 285 0.022 0.004 05-01-97 285 0.020 0.003 10-30-97 284 0.029 0.004 08-97 285 0.018 i 0.003 11-06-97 286 0.021 1 0.003 05-15 97 287 0.013 i 0.003 11-12-97 245 0.016 0.003 05-22-97 284 0.016 1 0.003 11-20-97 327 0.043 0.004 05-29-97 285 0.016 i 0.003 11-26-97 243 0.067 0.005 06-04-97 245 0.014 i 0.004 12-04-97 327 0.027 0.003 06-12 97 329 0.023 0.003 12 11-97 284 0.013 0.003 06-19-97 283 0.016 1 0.003 12-18-97 307 0.036 1 0.004 06-26-97 284 0.024 0.003 12-26-97 326 0.033 0.003 07-03-97 287 0.023 i 0.004 01-02-98 284 0.022 0.003 1 2nd Quarter Mean s.d. 0.019 1 0.004 4th Quarter Mean s.d. 0.030 2 0.014 i
Cumulative Average: 0.025 Previous Annual Average: 0.023
' lodine-131 concentrations are <0.07 pCi/m*unless otherwise noted.
- Filter density light. l l
2-1 1
i
I t
i DUANE ARNOLD - 1 Table 3. Airborne particulates and charcoal canisters, analysis for gross beta.
Location: D-3 (Hiawatha)
! Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume l Collected (m*) Gross Beta Collected (m') Gross Beta l Reauired 11D g g 01-09-97 288 0.026 i 0.003 07-10-97 284 0.013 0.003 01 16-97 285 0.030 i 0.004 07-17-97 286 0.018 0.003 01-23 287 0.022 0.003 07-24-97 286 0.021 0.003 01-30-97 284 0.026 1 0.004 07-31-97 283 0.023 i 0.004 q l 02-06-97 285 0.031 1 0.004 08-07-97 288 0.029 0.003 ;
02-12-97 246 0.026 i 0.004 08-14-97 285 0.024 i 0.003 02-20-97 325 0.031 i 0.004 08-21-97 290 0.021 0.003 )
02-27-97 286 0.025 1 0.003 08-28 282 0.040 0.004 03-06-97 285 0.022 i 0.003 09-04-97 286 0.029 1 0.003
- 03-13-97 285 0.027 i 0.003 09-11-97 285 0.028 0.003 03-20-97 285 0.019 i 0.003 09-18-97 285 0.037 1 0.004 03-27-97 288 0.019 1 0.003 09-25-97 286 0.023 0.003 l 04-03-97 282 0.013 0.003 10-02-97 286 0.024 0.003 l l, 1st Quarter Meanis.d. 0.024 1 0.005 3rd Quarter Meanis.d. 0.0251 0.007
! 1 10-97 285 0.017 i 0.003 10-09-97 285 0.041 0.004
! 04-16-97 246 0.024 1 0.004 10-16-97 285 0.030 0.003 04-24-97 326 0.019 i 0.003 10-23-97 285 0.025 0.004 05-01-97 285 0.020 1 0.003 10-30-97 287 0.030 2 0.004 05-08-97 285 0.017 0.003 11-06-97 286 0.020 0.003 05-15-97 286 0.014 0.003 11-12-97 245 0.016 0.003 05-22-97 283 0.013 1 0.003 11-20-97 326* < 0.003 05-29-97 284 0.013 0.003 11-26-97 245 0.055 0.005 06-04-97 246 0.014 i 0.004 12-04-97 326 0.023 i 0.003 06-12-97 328 0.015 i 0.002 12-11-97 285 0.011 0.003
! 06-19-97 284 0.013 i 0.003 12-18-97 285 0.036 0.004 06-26-97 284 0.018 0.003 12-26-97 325 0.027 0.003 07-03-97 287 0.018 1 0.003 01-02-98 287 0.016 0.003 l 2nd Quarter Mean s.d. 0.016 0.003 4th Quarter Mean s.d. 0.027 0.012 Cumulative Average: 0.023 '
Previous Annual Average: 0.022
' Filter light; Particulates allowed to bypass filter due to bad seal.
3-1
1 DUANE ARNOLD Table 4. Airbome particulates and charcoal canisters, analyses for gross beta and iodine-131',
1,ocation: D-5 (Palo)
Units: pCi/m' l
Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Required LLD Q&10 Qa1Q l
l i
l 01-09-97 287 0.033 i 0.004 07-10-97 286 0.015 0.003 01-16-97 286 0 029 i 0.004 07-17-97 285 0.022 0.003 01-23-97 286 0.019 0.003 07-24-97 286 0.024 1 0.003 l
30-97 284 0.025 i 0.004 07-31-97 284 0.025 0.004 l l 02-06-97 285 0.033 i 0.004 08-07-97 287 0.027 1 0.003 02-12-97 246 0.027 1 0.004 08-14-97 285 0.022 0.003 l
02-20-97 325 0.029 0.003 08-21-97 287 0.016 0.003 02-27-97 286 0.024 0.003 08-28-97 284 0.031 1 0.004 03-06-97 286 0.027 1 0.003 09-04-97 286 0.023 0.003 l 03-13-97 284_ 0.026 0.003 09-11-97 285 ' O.018 0.003 l
03-20-97 286 0.025 i 0.003 09-18-97 285 0.031 0.004 03-27-97 286 0.020 1 0.003 09-25-97 287 0.019 0.003 l 04-03-97 285 0.014 t 0.003 10-02-97 287 0.019 0.003 1st Quarter Meanis.d. 0.025 1 0.005 3rd Quarter Mean s.d. 0.022 0.005 1
!- 04-10-97 284 0.020 1 0.003 10-09-97 284 0.028 0.004 04-16-97 247 0.022 i 0.004 10-16-97 285 0.023 0.003 04-24-97 324 0.020 i 0.003 10-23-97 286 0.021 0.003 05-01-97 286 0.015 1 0.003 10-30-97 271 0.028 0.004 05-08-97 286 0.020 1 0.003 11-06-97 285 0.016 0.003 l 05-15-97 286 0.015 1 0.003 11-12-97 245 0.014 0.003 05-22-97 284 0.013 0.003 11-20-97 326 0.035 0.004 05-29-97 286 0.013 0.003 11-26-97 245 0.059 0.005 06-04-97 245' O.010 0.003 12-04-97 326 0.017 1 0.003 06-12-97 328 0.015 1 0.002 12-11-97 285 0.012 0.003 06-19-97 284 0.015 i 0.003 12-18-97 285 0.032 0.004 06-26-97 284 0.018 0.003 12-26-97 325 0.029 0.003 07-03-97 286 0.016 i 0.003 01-02-98 286 0.021 1 0.003 2nd Quarter Mean s.d. 0.016 0.003 4th Quarter Mean s.d. 0.026 0.012 l
Cumulative Average: 0.023 Previous Annual Average: 0.024 Iodine-131 concentrations are <0.07 pCi/m' unless otherwise noted.
i 4-1 l
t
DUANE ARNOLD Table 5. Airborne particulates and charcoal canisters, analysis for gross beta.
l Location: D-6 (Center Point)
( Units: pCi/m' l Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Ikouired I I D g g i 01-09-97 287' O.036 1 0.004 07-10-97 286 0.016 1 0.003
- j. 01-16-97 285 0.035 i 0.004 07-17-97 285 0.025 0.003 01-23-97 286 0.015 0.003 07-24-97 284 0.026 1 0.003 01-30-97 285 0.021 1 0.003 07-31-97 286 0.032 0.004 02-06-97 285 0.027 i 0.004 08-07-97 287 0.028 0.003 02-12-97 246 0.026 1 0.004 08-14-97 285 0.021 0.003
! 02-20-97 325 0.034 0.004 08 21-97 287 0.020 0.003 02-27-97 286 0.022 i 0.003 08-28-97 284 0.035 0.004 03-06-97 285 0.022 1 0.003 09-04-97 286 0.027 1 0.003 03-13-97 284 0.024 1 0.003 09-11-97 285 0.027 0.003
!- 03-20-97 285 0.019 i 0.003 09-18-97 281 0.038 0.004 03-27-97 250 0.022 i 0.003 09-25-97 287 0.020 0.003 l 04-03-97 282 0.015 i 0.003- 10-02-97 287 0.020 0.003 l 1st Quarter Meanis.d. 0.024 1 0.007 3rd Quarter Mean s.d. 0.026 1 0.006
'04-10-97 284 0.019 i 0.003 10-09-97 284 0.038 0.004 04-16-97 246 0.032 0.004 10-16-97 285 0.030 0.003 04-24-97 324 0.025 0.003 10-23-97 286 0.023 1 0.004 1 05-01-97 285 0.019 i 0.003 10-30-97 286 0.029 t 0.004 l 05-08-97 286 0.021 i 0.003 11-06-97 285 0.024 0.003 05-15-97 286 0.014 0.003 11-12-97 246 0.016 1 0.003 05-22-97 284 0.017 1 0.003 11-20-97 325 0.037 0.004 I
05-29-97 286 0.012 i 0.003 11 26-97 245 0 061 0.005 06-04-97 245 0.019 0.004 12-04-97 326 0.027 0.003 2 06-12-97 329 0.019 0.003 12-11-97 285 0.014 0.003 06-19-97 283 0.016 0.003 12-18-97 285 0.040 0.004 06-26-97 284 0.023 0.003 12-26-97 326 0.035 0.003 07-03-97 286 0.021 i 0.003 01-02-98 286 0.026 1 0.003 2nd Quarter Mean s.d. 0.020 0.005 4th Quarter Mean s.d. 0.031 0.012 Cumulative Average: 0.025 Previous Annual Average: 0.026 5-1
DUANE ARNOLD Table 6. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131' Location: D-7 (Shellsburg)
Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired LLD g g 01-09-97 287 0.026 i 0.003 07-10-97 286 0.013 0.003 01-16-97 286 0.033 1 0.004 07-17-97 285 0.019 1 0.003 01-23-97 286 0.020 0.003 07-24-97 286 0.023 0.003 01-30-97 284 0.025 0.003 07-31-97 284- 0.025 0.004 ~
02-06-97 285 0.032 1 0.004 08-07-97 287 0.025 0.003 02-12-97 246 0.027 t 0.004 08-14-97 285 0.018 0.003 02-20-97 325 0.029 0.003 08-21-97 287 0.015 0.003 02-27-97 -286 0.023 i 0.003 08-28-97 284 0.032 0.004 03-06-97 286 0.024 i 0.003 09-04-97 286 0.024 0.003 03-13-97 284 0.026 i 0.003 09-11-97 285 0.024 0.003 03-20-97 286 0.019 i 0.003 09-18-97 285 0.034 0.004 j 03-27-97 286 0.019 i 0.003 09-25-97 287 0.018 0.003 04-03-97 285 0.015 0.003 10-02-97 287 0.021 0.003 1st Quarter Meanis.d. 0.024 1 0.005 3rd Quarter Mean s.d. 0.022 0.006 6
04 10-97 284 0.016 i 0.003 10-09-97 131 0.034 i 0.007 04-16-97 247 0.024 i 0.004 10-16-97 285 0.027 0.003 10-23-97
{
04-24 97 324 0.017 i 0.003 286 0.019 0.003 j 05-01 97 286 0.018 1 0.003 10-30-97 286 0.025 0.003 05-08-97 286 0.016 1 0.003 11-06-97 285 0.018 0.003
. 05-15-97 286 0.012 i 0.003 11-12-97 245 0.017 0.003 05-22 2t'4 0.013 1 0.003 11 20-97 326 0.034 0.004 -
05-29 286 0.012 1 0.003 11-26-97 245 0.051 0.005 06-04 245 0.016 0.004 12-04-97 326 0.024 0.003 06-12-97 328 0.012 i 0.002 12-11-97 286 0.011 0.003 1 06-19-97 284 0.016 1 0.003 12-18-97 -285 0.038 0.004 06-26-97 284 0.017 i 0.003 12-26-97 326 0.034 0.003 07-03-97 286 0.017 i 0.003 01-02-98 286 0.026 0.003 2nd Quarter Mean s.d. 0.016 1 0.003 4th Quarter Mean s.d. 0.027 2 0.011 i Cumulative Average: 0.023 Previous Annual Average: 0.023
- Iodine-131 concentrations are <0.07 pCi/m' unless otherwise noted.
6 Low volume due to power loss at substation.
l 6-1 h
DUANE ARNOLD Table 7. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131' Location: D-8 (Urbana)
Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired LLD ggig g 01-09-97 287 0.030 1 0.004 07-10-97 286 0.013 0.003 1 l
01 16-97 286 0.029 0.004 07-17-97 285 0.023 0.003 01-23-97 286 0.021 i 0.003 07-24-97 286 0.023 1 0.003 01-30-97 285 0.027 1 0.004 07-31-97 284 0.028 0.004 02-06-97 285 0.031 i 0.004 08-07-97 287 0.029 i 0.003 02-12-97 246 0.026 0.004 08-14-97 285 0.023 1 0.003 02-20-97 325 0.033 i 0.004 08-21-97 288 0.019 0.003 02-27-97 286 0.027 i 0.003 08-28-97 283 0.039 i 0.004 l 03-06-97 286 0.024 0.003 09-04-97 286 0.026 0.003 03-13-97 284 0.024 i 0.003 09-11-97 285 0.028 0.003 03-20-97 286 0.024 1 0.003 09-18-97 274 0.033 I 0.004 03-27-97 288 0.020 i 0.003 09-25-97 287 0.022 i 0.003 04-03-97 283 0.019 i 0.003 10-02-97 287 0.022 ! 0.003 l
1st Quarter Mean s.d. 0.026 1 0.004 3rd Quarter Mean s.d. 0.025 0.006 04-10-97 284 0.018 t 0.003 10-09-97 284 0.035 0.004 1 04-16-97 246 0.023 0.004 10-16-97 285 0.030 0.003 04-24-97 324 0.021 i 0.003 10-23-97 286 0.019 0.003 i 05-01-97 285 0.017 i 0.003 10-30-97 272 0.028 0.004 l 05-08-97 286 0.019 i 0.003 11-06-97 285 0.016 1 0.003 05-15-97 286 0.014 1 0.003 11-12-97 245 0.013 0.003 05-22-97 284 0.012 0.003 . 11-20-97 326 0.038 0.004 05-29-97 286 0.016 1 0.003 11-26-97 245 0.063 0.005 1 06-04-97 245 0.017 0.004 12-04-97 326 0.024 0.003 l 06-12-97 329 0.017 0.003 12-11-97 285 0.012 2 0.003 06-19-97 283 0.014 0.003 12-18-97 285 0.039 0.004 06-26-97 281 0.025 i 0.003 12 26-97 326 0.031 0.003 l 07-03-97 286 0.018 i 0.003 01-02-98 286 0.021 0.003 !
2nd Quarter Mean s.d. 0.018 1 0.004 4th Quarter Mean s.d. 0.028 1 0.014 Cumulative Average: 0.024 Previous Annual Average: 0.025
- Iodine-131 concentrations are <0.07 pCi/m' unless otherwise noted.
i 7-1
I DUANE ARNOLD j Table 8. Airborne particulates and charcoal canisters, analysis for gross beta.
! Location: D-10 (Atkins)
I Units: pCi/m' Collection: Continuous, weekly exchange.
l Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta -
Reauired I f D galg g j
)
01-09-97 286 0.022 0.003 07-10-97 284 0.013 0.003 l 01-16-97 285 0.026 i 0.003 07-17-97 285 0.020 0.003
! 01-23-97 287- 0.020 i 0.003 07-24-97 285 0.027 0.003 l 01-30-97 285 0.026 i 0.004 07-31-97 286 0.026 0.004 I
02-06-97 285 0.029 i 0.004 08-07-97 287 0.027 1 0.003 l 02-12-97 247 0.024 0.003 08-14-97 282 0.020 0.003 02-20-97 323 0.030 i 0.003 08-21-97 281 0.016 0.003 02-27-97 286 0.024 i 0.003 08-28-97 290 0.037 0.004 03-06-97 286 0.022 i 0.003 09-04-97 286 0.024 0.003 I 03-13-97 284 0.021 i 0.003 09-11 97 285 0.020 0.003 l 03-20-97 285 0.019 i 0.003 09-18-97 286 0.032 0.004 03-27-97 283 0.020 i 0.003 09-25-97 286 0.018 0.003 j 04-03-97 289 0.015 0.003 10-02-97 284 0.024 0.003 l 1st Quarter Mean s.d. 0.023 1 0.004 3rd Quarter Mean s.d. 0.023 0.007 l
l 04-10-97 284 0.017 0.003 10-09-97 285 0.032 0.004 l 04-16-97 246 0.024 0.004 10-16-97 280 0.029 0.003 04-24-97 326 0.018 1 0.003 10-23-97 285 0.021 0.003 l 05-01-97 284 0.021 0.003 10-30-97 275 0.028 0.004 l 05-08-97 284 0.018 i 0.003 11-06-97 286- 0.020 0.003 6
1 05-15-97 286 0.015 i 0.003 11-12-97 245 0.021 0.004 05-22-97 286 0.013 1 0.003 11-20-97 327 0.039 0.004 05-29-97 284 0.014 0.003 11-26-97 244 0.072 0.005 06-04-97 245 0.013 0.004 12-04-97 327 0.029 0.003 I j 06-12-97 328 0.018 0.003 12-11 97 285 0.012 2 0.003 ;
! 06-19-97 284 0.016 i 0.003 12-18-97 284 0.043 0.004 !
06-26-97 285 0.023 0.003 12-26-97 327 0.032 0.003 07-03-97 288 0.019 0.003 01-02-98 285 0.025 0.003 2nd Quarter Mean s.d. 0.018 1 0.003 4th Quarter Mean s.d. 0.031 0.015 i
Cumulative Average: 0.024 Previous Annual Average: 0.025
- Volume estimated; Collector reported timer failure, data suggests a normal sampler pump run-time.
8-1 l
I r
l DUANE ARNOLD I
l Table 9. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131*.
Location: D-11 (Toddville)
Units: pCi/m' Collection: Continuous, weeldy exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired I LD g g 01-09-97 288 0.030 0.004 07-10-97 285 0.012 0.003 01-16-97 284 0.033 i 0.004 07-17-97 286- 0.021 1 0.003 01-23-97 287 0.020 1 0.003 07-24-97 286 0.022 0.003 j 01-30-97 284 0.022 0.003 07-31-97 283 0.029 0.004 l 02-06-97 285 0.028 1 0.004 08-07-97 287 0.026 0.003 02-12-97 246 0.029 0.004 08-14-97 286 0.022 0.003 l.
i 02-20-97 325 0.032 1 0.004 08-21-97 290 0.017 1 0.003 02-27-97 286 0.022 i 0.003 08-28-97 281 0.033 1 0.004
! 03-06-97 285 0.023 i C.003 09-04-97 286 0.023 0.003 03-13-97 284 0.022 i 0.003 09-11 97 285 0.025 i 0.003 03-20-97 286 0.023 i 0.003 09-18-97 285 0.034 0.004 03-27-97 289 0.015 i 0.003 09-25-97 286 0.024 0.003 04-03-97 282 0.015 1 0.003 10-02-97 286 0.024 0.003 1st Quarter Meanis.d. 0.024 1 0.006 3rd Quarter Meanzs.d. 0.024 0.006 04-10-97 284 0.022 1 0.003 10-09-97 285 0.037 1 0.004 04-16-97 246 0.029 i 0.004 10-16-97 285 0.031 0.003 04-24-97 325 0.023 0.003 10-23-97 285 0.023 0.004 05-01-97 286 0.019 0.003 10-30-97 287 0.028 0.004 05-08-97 273 0.018 1 0.003 11-06-97 286 0.020 0.003 05-15-97 286 0.017 i 0.003 11-12-97 245 0.017 1 0.003 05-22-97 285 0.014 1 0.003 11-20-97 326 0.038 1 0.004 05-29-97 284 0.016 1 0.003 11-26-97 245 0066 0.005 06-04-97 245 0.014 0.004 12-04-97 327 0.026 0.003 06-12-97 329 0.016 0.003 12-11-97 286 0.015 0.003 06-19-97 284 0.016 1 0.003 12-18-97 284 0.043 0.004 06-26-97 284 0.021 0.003 12-26-97 325 0.034 0.003 07-03-97 287 0.018 i 0.003 01-02-98 285 0.024 0.003 2nd Quarter Mean s.d. 0.019i 0.004 4th Quarter Mean s.d. 0.031 0.013 i
I Cumulative Average: 0.024 Previous Annual Average: 0.026
- kidine-131 concentrations are <0.07 pCi/m' unless otherwise noted. l l
9-1
i DUANE ARNOLD Table 10. Airborne particulates and charcoal canisters, analysis for gross beta. I Location: D-13
+
Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired LLD QQ1g Q,q1g l
01-09-97 287 0.024 1 0.003 07-10-97 286 0.015 2 0.003 j 01-16-97 286 0.025 1 0.003 07-17-97 285 0.025 0.003 01-23-97 NDa - 07-24-97 286 0.027 0.003 01-30-97 285 0.023 1 0.003 07-31-97 284 0.018 0.003 02-06-97 285 0.029 1 0.004 08-07-97 287 0.031 0.003 02-12-97 246 0.023 i 0.003 08-14-97 285 0.020 0.003 02-20-97 325 0.029 i 0.003 08-21-97 288 0.019 i 0.003 02-27-97 286 0.019 i 0.003 08-28-97 284 0.033 0.004 03-06-97 286 0.018 0.003 09-04-97 286 0.025 0.003 03-13-97 284 0.020 1 0.003 09-11-97 285- 0.023 0.003 03-20-97 285 0.020 0.003 09-18-97 281 0.036 0.004 03-27-97 290 0.017 i 0.003 09-25-97 287 0.021 0.003 04-03-97 282 0.014 i 0.003 10-02-97 286 0.022 0.003 1st Quarter Meanis.d. 0.022 0.005 3rd Quarter Mean s.d. 0.024 2 0.006 04-10-97 284 0.012 i 0.003 10-09-97 284 0.032 0.004 l 04-16-97 246 0.021 i 0.004 10-16-97 284 0.029 0.003 04-24-97 324 0.018 0.003 10-23-97 288 0.019 0.003 05-01-97 286 0.017 0.003 10-30-97 237 0.031 0.004 05-08-97 285 0.018 1 0.003 11-06-97 285- 0.015 0.003 05-15-97 286 0.012 1 0.003 11-12-97 245 0.012 0.003 05-22-97 286 0.016 i 0.003 11-20-97 325 0.034 0.004 05 29-97 284 0.015 0.003 11 26-97 245 0.057 0.005 06-04-97 245 0.015 i 0.004 12-04-97 326 0.024 1 0.003 06-12-97 326 0.016 i 0.003 12-11-97 286 0.012 0.003 06-19-97 136 0.018 1 0.006 12-18-97 285 0.042 0.004 06-26-97 245 0.022 0.003 12-26-97 327 0.033 0.003 07-03-97 286 0.020 1 0.003 01-02-98 286 0.024 0.003 2nd Quarter Mean s.d. 0.017i 0.003 4th Quarter Mean s.d. 0.028 z 0.013 Cumulative Average: 0.023 Previous Annual Average: 0.023
- ND = No data; Sample lost in strong winds.
I l
10-1 ,
DUANE ARNOLD Table 11. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131' Location: D-15 (On-site)
Units: pCi/m' Collection: Continuous, weekly exchange.
Date Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired LLD g g 01-09-97 288 0.031 i 0.004 07-10-97 286 0.011 0.003 01-16-97 286 0.032 i 0.004 07-17-97 285 0.021 0.003 01-23-97 286 0.021 i 0.003 07-24-97 285 0.019 0.003 01-30-97 285 0.025 1 0.004 07-31-97 284 0.029 0.004 02-06-97 285 0.032 i 0.004 08-07-97 287 0.025 i 0.003 02-12-97 246 0.027 1 0.004 08-14-97 285 0.015 0.003 02-20-97 325 0.032 1 0.004 08-21-97 286 0.012 0.003 02-27-97 286 0.023 0.003 08-28-97 285 0.027 0.004 03-06-97 285 0.021 1 0.003 09-04-97 286 0.020 0.003 03-13-97 285 0.023 1 0.003 09-11-97 285 0.020 0.003 03-20-97 286 0.025 0.003 09-18-97 285 0.029 0.004 03-27-97 286 0.016 1 0.003 09-25-97 287 0.016 0.003 04-03-97 285 0.014 i 0.003 10-02-97 285 0.019. 0.003 1st Quarter Meanis.d. 0.025 1 0.006 3rd Quarter Mean s.d. 0.020 1 0.006 04-10-97 284 0.017 i 0.003 10-09-97 285 0.031 1 0.004 04-16-97 246 0.025 1 0.004 10-16-97 285 0.025 0.003 04-24-97 324 0.021 1 0.003 10-23-97 285 0.021 0.003 05-01-97 286 0.018 0.003 10-30-97 287 0.025 0.003 05-08-97 285 0.019 1 0.003 11-06-97 285 0.017 0.003 05-15-97 286 0.013 1 0.003 11-12-97 245 0.014 0.003 05-22-97 285 0.013 1 0.003 11-20-97 326 0.036 0.004 05-29-97 286 0.014 i 0.003 11-26-97 245 0.061 0.005 06-04-97 245 0.012 0.003 12-04-97 326 0.023 0.003 06-12-97 328 0.018 i 0.003 12-11-97 285 0.010 0.003 06-19-97 284 0.014 i 0.003 12-18-97 285 0.035 0.004 06-26-97 284 0.018 0.003 12-26-97 325 0.027 0.003 07-03-97 286 0.017 0.003 01-02-98 286 0.019 0.003 2nd Quarter Meant.s.d. 0.017 0.004 4th Quarter Mean s.d. 0.026 0.013 Cumulative Average: 0.022 Previous Annual Average: 0.022
- lodine-131 concentrations are <0.07 pCi/m' unless otherwise noted.
11-1
DUANE ARNOLD Table 12. Airborne particulates and charcoal canisters, analysis for gross beta.
Location: D-16 (on-site)
Units: pCi/m' Collection: Continuous, weekly exchange.
Oate Volume Date Volume Collected (m') Gross Beta Collected (m') Gross Beta Reauired LLD Q,Q10 0111g 01-09-97 288 0.033 1 0.004 07-10-97 286 0.013 2 0.003 01-16-97 281 0.031 1 0.004- 07-17-97 285 0.020 0.003 01 23-97 286 0.022 1 0.003 07-24-97 285 0.021 0.003 01-30-97 285 0.028 1 0.004 07-31-97 284 0.022 1 0.004 02-06-97 285 0.026 1 0.004 08-07-97 287 0.024 0.003 02 12 97 246 0.027 0.004 08-14-97 285 0.026 0.003 02-20-97 325 0.033 1 0.004 08-21-97 287 0.018 1 0.003 02-27-97 286 0.023 1 0.003 08-28-97 284 0.033 ! 0.004 03-06-97 285 0.024 1 0.003 09-04-97 286 0.023 0 003 03-13-97 285 0.026 1 0.003 09-11-97 285 0.023 1 0.003 03-20-97 286 0.026 i 0.003 09-18-97 285 0.030 0.004 03-27 97 286 0.019 0.003 09-25-97 287 0.018 1 0.003 04-03-97 285 0.013 0.003 10-02-97 284 0.019 0.003 1st Quarter Meanis.d. 0.025 1 0.006 3rd Quarter Mean s.d. 0.022 0.005 04-10-97 284 0.017 1 0.003 10-09-97 285 0.034 0.004 04 16-97 246 0.028 1 0.004 10-16-97 285 0.028 0.003 04-24-97 324 0.023 i 0.003 10-23-97 285 0.020 i 0.003 05-01-97 278 0.021 i 0.003 10-30-97 287 0.025 0.003 05-08-97 285 0.021 1 0.003 11-06-97 285 0.015 2 0.003 05-15-97 286 0.012 1 0.003 11 12-97 245 0.015 0.003 05-22-97 285 0.015 i 0.003 11-20-97 326 0.029 0.004 05-29 97 286 0.016 i 0.003 11-26-97 245 0.057 ! 0.005 06-04 97 244 0.014 1 0.004 12-04-97 326 0.023 0.003 06-12-97 329 0.015 i 0.002 12-11-97 285 0.010 0.003 Ot>-19-97 284 0 013 1 0.003 12-18-97 285 0.033 0.004 06-26-97 284 0.015 1 0.003 12-26-97 325 0.028 1 0.003 07-03-97 286 0.017 1 0.003 01-02-98 286 0.015 0.003 2nd Quarter Meants.d. 0.018 0.004 4th Quarter Mean s.d. 0.026 0.012 Cumulative Average: 0.023 Previous Annual Average: 0.024 12-1
1 l
DUANE ARNOLD Table 13. Airborne particulate samples; analysis for gamma emitting isotopes.
Collection: Quarterly composite of weekly samples Units: pCi/m' Location D-1 Qunter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code L. iP-2331 DAP-4960 DAP-8169 DAP-10203 i Volume 3709 3576 3712 3742 i Be-7 0.076 i 0.018 0.11 0.014 0.11 1 0.014 0.068 0.011 Zr-95 < 0.0017 < 0.0014 < 0.0006 < 0.0018 Nb-95 < 0.0021 < 0.0009 <0.0008 < 0.0008 Ru-103 < 0.0006 < 0.0006 < 0.0006 < 0.0008 I Ru-106 < 0.0142 < 0.0084 < 0.0058 < 0.0032 Cs-134 < 0.0014 < 0.0007 < 0.0009 < 0.0004 Cs-137 < 0.0016 < 0.0010 < 0.0006 < 0.0008 Ce-141 < 0.0021 < 0.0009 < 0.0011 < 0.0011 Ce-144 < 0.0072 < 0.0024 < 0.0028 < 0.0027 Location D-2 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2332. DAP-4961 DAP-8170 DAP-10204 Volume 3711 J 3711 3714 3767 Be-7 0.083 0.014 0.11 1 0.011 0.091 1 0.013 0.071 1 0.010 Zr-95 < 0.0017 < 0.0009 < 0.0010 < 0.0008 Nb-95 < 0.0012 < 0.0004 < 0.0007 < 0.0009 Ru-103 < 0.0006 < 0.0007 < 0.0013 < 0.0004 Ru-106 . < 0.0077 < 0.0065 < 0.0034 < 0.0030 Cs-134 < 0.0009 < 0.0006 < 0.0006 < 0.0006 Cs-137 < 0.0007 < 0.0003 <0.0005 < 0.0007 Ce-141 < 0.0007 < 0.0010 < 0.0022 < 0.CK)04 Ce-144 < 0.0015 < 0.0038 <0.0050 <0.0020 Location D-3 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2333 DAP-4962 DAP-8171 DAP-10205 Volume 3511 3709 3712 3752 Be-7 0.075 1 0.015 0.087 1 0.011 0.11 0.017 0.051 0.010 Zr-95 < 0.0023 < 0.0018 < 0.0008 < 0.0013 Nb-95 < 0.0015 < 0.0010 < 0.0005 < 0.0009 Ru-103 < 0.0014 < 0.0008 < 0.0005 < 0.0005 Ru-106 < 0.0044 < 0.0056 < 0.0030 < 0.0031 Cs-134 < 0.0006 < 0.0007 < 0.0007 < 0.0006 Cs 137 < 0.0011 < 0.0009 < 0.0004 < 0.0006 Ce-141 < 0.0019 < 0.0011 < 0.0008 < 0.0011 Cc-144 < 0.0040 < 0.0048 < 0.0032 < 0.0036 1
13-1
DUANE ARNOLD Table 13. Airborne particulate samples; analysis for gamma emitting isotopes.
Collection: Quarterly composite of weekly samples Units: pCi/m'
! Location D-5 l Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter
! Lab Code DAP-2334 DAP-4963, 4 DAP-8172 DAP-102%
Volume 3712 3710 3714 3734 l Be 7 0.073 1 0.015 0.089 0.009 0.073 0.013 0.055 1 0.009 Zr-95 <0.0019 < 0.0010 < 0.0036 < 0.0014 Nb-95 <0.0012 < 0.0005 < 0.0014 <0.0010 Ru-103 < 0.0004 < 0.0007 < 0.0011 <0.0006 Ru-106 < 0.0059 < 0.0057 < 0.0019 < 0.0048 Cs-134 <0.0005 < 0.0006 <0.0003 < 0.0006 I Cs-137 < 0.0009 < 0.0009 < 0.0006 < 0.0003 Ce-141 < 0.0011 < 0.0006 < 0.0023 < 0.0007 l Ce-144 < 0.0037 < 0.0017 < 0.0036 < 0.0030 Location D-6 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter l Lab Code DAP-2335 DAP-4965 DAP-8173 DAP-10207, 8 Volume {
3671 3708 3710 3750 l be-7 0.059 i 0.010 0.10 1 0.020 0.11 1 0.015 0.059 1 0.007 l l
! Zr-95 < 0.0013 < 0.0015 < 0.0011 < 0.0011 l
Nb-95 < 0.0006 < 0.0020 < 0.0009 < 0.0006 ;
Ru-103 < 0.0005 < 0.0014 < 0.0011 < 0 0714 l Ru-106 < 0.0039 < 0.0109 < 0.0093 <0.0049 .
Cs-134 < 0.0007 < 0.0007 < 0.0008 .<0.0006 i' Cs-137 < 0.0008 < 0.0010 < 0.0006 < 0.0005 Ce-141 < 0.0012 < 0.0019 <0.0018 < 0.0009 Ce-144 < 0.0048 < 0.0038 < 0.0025 < 0.0028 Loce.. ion i D-7 '
Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2336 DAP-4966 DAP-8174 DAP-10209 ;
Volume 3712 3710 3714 3598 ;
Be-7 0.072 1 0.023 0.090 0.012 0.081 1 0.013 0.056 0.011 Zr-95 < 0.0016 < 0.0018 <0.0014 < 0.0015 Nb-95 < 0.0020 < 0.0005 < 0.0005 < 0.0009 Ru-103 < 0.0020 <0.0007 <0.0018 <0.0009 Ru-106 < 0.0089 < 0.0053 < 0.0060 < 0.0055 Cs-134 <0.0009 < 0.0004 < 0.0005 < 0.0003 Cs-137 < 0.0010 < 0.0006 < 0.00% < 0.0009 Ce-141 <0.0021 < 0.0007 < 0.0028 < 0.0010 Ce-144 < 0.0041 < 0.0032 < 0.0047 < 0.0031 13- 2
DUANE ARNOLD l
l Table 13. Airborne particulate samples; analysis for gamma emitting isotopes.
l Collection: Quarterly composite of weekly samples Units: pCi/m' Location D-8 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2337 DA P-4%7. DAP-8175 DAP-10210 Volume 3713. 3705 3703 3736 De-7 0.070 1 0.015 0.11 i 0.013 0.11 i 0.016 0.064 i 0.018 Zr-95 < 0.0015 < 0.0016 < 0.0006 < 0.0023 Nb-95 <0.0015 < 0.0004 <0.0004 <0.0015 Ru-103 < 0.0012 < 0.0007 < 0.0009 < 0.0014 Ru 106 < 0.0095 < 0.0034 < 0.0054 <0.0088 Cs-134 < 0.0007 < 0.0007 < 0.0005 < 0.0013 l Cs-137 < 0.000 ) < 0.0008 < 0.0005 < 0.0009 Ce-141 < 0.0017 < 0.0013 < 0.0014 <0.0024 Ce-144 < 0.0028 < 0.0017 ' < 0.0040 < 0.0058 l Location D-10 Quarter 1st Quarter 2nd Quarter . 3rd Quarter 4th Quarter Lab Code DAP-2338 DAP-4968 DAP-8176 DAP-10211 Volume 3711 3710 3707 3521 Be-7 0.063 1 0.013 0.11 i 0 013 0.10 0.017 0.073 1 0.013 Zr-95 < 0.0012 < 0.0017 < 0.0007 < 0.0021 Nb-95 < 0.0008 < 0.0012 < 0.0007 <0.0004
[
i Ru 103 < 0.0009 < 0.0004 < 0.0004 < 0.0009 '
Ru 106 < 0.0032 < 0.0073 < 0.0025 < 0.0073 Cs-134 < 0.0003 . < 0.0008 < 0.0004 < 0.0008 C5-137 < 0.0008 <0.0008 < 0.0008 < 0.0010 Ce-141 < 0.0018 < 0.0014 < 0.0017 < 0.0009 Ce-144 < 0.0046 <0.0041 <0.0044 <0.0022 Location D-11 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2339 DAP-4969 DAP-8177 DAP-10212 Volume 3711 3698 3712 3751
! Be-7 0.067 0.013 0.11 1 0.021 0.091 1 0.014 0.062 0.010 l ' Zr-95 < 0.0024 < 0.0019 < 0.0007 < 0.0009 l
Nb-95 < 0.0012 < 0.0017 < 0.0010 < 0.0004 Ru-103 < 0.0010 < 0.0013 < 0.0010 <0.0008 Ru-106 < 0.0054 < 0.0108 < 0.0037 <0.0048 Cs-134 < 0.0005 < 0.0010 < 0.0005 <0.0005 Cs-137 < 0.0004 <0.0010 < 0.0004 < 0.0006 Cc-141 < 0.0007 < 0.0021 < 0.0018 < 0.0015 Ce-144 < 0.0038 < 0.0047 < 0.0051 <0.0048 I
I 13- 3
I DUANE ARNOLD Table 13. Airborne particulate samples; analysis for gamma emitting isotopes.
Collection: Quarterly composite of weekly samples Units: pCi/m' Location D-13 l Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter i Lab Code DAP-2340 DAP-4970 DAP-8178 DAP-10213 I Volume 3427 3519 3710 3703 I Be-7 0. % 9 i 0.013 0.101 0.018 0.10 0.015 0.054 1 0.009 Zr-95 < 0.0025 < 0.0012 < 0.0011 < 0.0011 Nb-95 < 0.0012 < 0.0014 < 0.0008 < 0.0008
- Ru-103 < 0.0007 <0.0012 < 0.0010 <0.0009 l: Ru-1% < 0.0047 < 0.0077 < 0.0030 < 0.0030 Cs 134 < 0.0008 < 0.0013 < 0.0008 < 0.0002 Cs-137 <0.0010 <0.0010 <0.0005 < 0.0004 Ce-141 < 0.0013 < 0.0017 < 0.0025 < 0.0006 Ce-144 < 0.0037 <0.0033 <0.0046 <0.0034 Location D-15 l Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter I Lab Code DAP-2341 DAP-4971 DAP-8179 DAP-10214 Volume 3714 3709 3711 3750 Be-7 0.068 1 0.016 0.087 i 0.012 0.073 1 0.014 0.049 1 0.013 Zr-95 < 0.0025 < 0.0017 < 0.0004 < 0.0021 Nb-95 < 0.0011 < 0.0006 < 0.0009 < 0.0012 Ru-103 < 0.0011 < 0.0006 < 0.0009 < 0.0010 Ru-106 < 0.0060 < 0.0056 < 0.0067 < 0.0063 Cs-134 < 0.0004 < 0.0004 < 0.0006 < 0.0005 Cs-137 < 0.0009 < 0.0008 < 0.0004 < 0.0006 Ce-141 < 0.0019 <0.0011 < 0.0019 < 0.0017 Ce-144 <0.0058 < 0.0018 < 0.0047 < 0.0022 Location D-16 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP 2342 DAP-4972 DAP-8180 DAP-10215 Volume 3709 3701 3710 3750 Be-7 0.080 1 0.019 0.10 0.015 0.073 0.014 0.049 0.014 Zr-95 < 0.0032 < 0.0016 < 0.0004 < 0.0011 Nb-95 < 0.0008 < 0.0009 < 0.0009 < 0.0020 Ru-103 l
< 0.0016 < 0.0008 < 0.0009 < 0.0014 !
Ru-106 < 0.0108 < 0.0097 < 0.0067 <0.0049 Cs-134 < 0.0009 < 0.0003 < 0.0006 < 0.0012 Cs-137 < 0.0013 < 0.0004 < 0.0004 < 0.0010 Ce-141 < 0.0014 < 0.0006 < 0.0019 <0.0020 Ce-144 < 0.0053 < 0.0025 <0.0047 < 0.0062 l
l 13-4
DUANE ARNOLD l Table 14. Ambient gamma radiation (TLDs), quarterly exposure,1997.
I Units: mR/91 days 1st Otr 2nd Ouarter 3rd Ouarter 4th Ouarter Air Stations D-1 10.510.2 10.6 i 0.2 11.2 0.3 15.7 0.5 D-2 12.110.2 9.8 i 0.2 12.310.2 15.4 0.4 D-3 11.3 i 0.3 9.4 i 0.3 11.2 0.2 14.7 0.3 D-5 12.010.2 9.3 i 0.2 12.7 i 0.2 15.8 0.4 i
D-6 11.4 i 0.3 8.9 0.3 11.3 i 0.2 15.9 0.3 I D-7 11.0 i 0.3 37.1 i 0.2 12.0t 0.2 17.0 0.3 l D-8 15.9 i 0.2 14.310.3 16.0 i 0.2 20.9 0.4
! D-10 11.6 0.2 11.31 0.2 12.7 0.2 17.4 0.3 D-11 9.0 i 0.2 7.1i 0.2 9.2i 0.2 12.1 0.3 D-13 13.21 0.2 11.210.2 13.610.2 17.0 0.3 D-15 11.610.2 9.9 1 0.2 12.4 0.2 15.7 0.5 l D-16 12.110.2 10.8 i 0.2 13.510.2 15.6 0.4
! ~
' Meants.d. M.8 1.6 12.517.9 12.311.7 16.1 2.0 W/in 0.5 mi. of Stack
! D-18 12.610.2 11.7 0.2 14.210.2 16.4 i 0.6 i D-19 10.9 i 0.4 12.3 i 0.2 12.110.2 15.8 0.4 i
D-20 13.61 0.2 15.8 i 0.2 14.7 i 0.3 19.5 0.4 D-21 13.7 0.2 14.4 i 0.3 15.9 0.2 18.3 0.3 D-22 12.4 i 0.2 12.7 i 0.3 12.610.2 16.9 0.3 D-23 10.5 i 0.2 10.710.2 11.31 0.3 15.6 0.5 D-28 13.3 i 0.2 15.8 i 0.2 15.7 0.2 18.5 0.3 D-29 14.8 i 0.3 17.510.2 17.010.2 20.9 0.5 D-30 14.9 i 0.3 17.21 0.2 17.8 0.2 20.2 0.4 l D-31 17.2 0.2 18.3 i 0.3 N D' 23.5 0.3 i D-32 16.51 0.2 15.8 0.2 17.71 0.2 21.01 0.3 D-82 10.3 0.2 10.3 i 0.2 13.1 0.2 13.7 0.3 D-83 11.61 0.2 12.7 i 0.2 13.6 0.2 15.810.3 D-84 12.0 i 0.2 12.8 i 0.2 14.0 0.2 15.3 0.3 D-86 1 .2 02 i0 1 .8 0 7. 0.3 D-91 10.8 0.5 12.8 0.2 ND' 15.5 0.5 Mean s.d. 13.0 2.1 14.012.4 14.6 2.0 17.622.6
- ND = No data; TLD lost in the field.
14-1
f l
DUANE ARNOLD Table 14. Ambient gamma radiation (TLDs), quarterly exposure,1997.
Units: mR/91 days l 1st Otr 2nd Ouarter 3rd Ouarter 4th Ouarter I W/in 1.0 mi. of l Stack D-43 10.8 i 0.2 12.310.2 13.1 0.2 15.31 0.3 D-44 14.3 i 0.3 16.0 i 0.2 16.910.2 18.9 0.3 l D-45 10.910.3 12.310.2 13.1 i 0.2 16.6 0.3 D-46 14.9 i 0.4 16.9 i 0.2 17.61 0.2 20.0 0.3
! D-47 14.2 0.2 14.410.2 16.2 0.2 19.410.3 D-48 15.0 i 0.3 15.9 i 0.2 17.1 0.2 19.6 0.3 l Meanis.d. 13.412.0 14.612.0 15.712.0 18.3 1.9 l W/in 3.0 mi. of l Stack D-33 9.2i 0.2 9.2 1 0.3 11.410.2 12.910.3 D-34 9.6 1 0.2 10.610.2 11.9 0.2 13.3 0.3 l D-35 10.7 i 0.2 10.610.2 12.51 0.2 N D*
D-36 12.31 0.2 11.21 0.2 14.0 0.2 14.8 0.3 D-37 15.0 i 0.2 15.810.2 17.6 0.2 17.31 0.3 D-38 12.2 i 0.2 12.910.2 14.71 0.3 15.71 0.3 f
4 D-39 12.2 0.2 12.31 0.2 14.4 0.2 ' 15.91 0.4
, D-40 11.1 i 0.3 11.510.2 13.2 0.2 14.7 0.3 '
D-41 11.3 i 0.2 11.9 0.2 13.51 0.2 14.7 0.3 D-42 9.9 0.2 11.3 1 0.2 11.2 i 0.3 14.1 0.3 Meanis.d. 11.4 1.7 _ _ _ _11.711.8 13.411.9 14.811.4 l
- ND = No data; TLD lost in the field.
14-2
l DUANE ARNOLD l Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
l Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-63 l
Lab Code DMI-91 DMI-505 DMI-1051 DMI-1639 DMI-2827 Date Collected 1/7/97 2/4/97 3/4/97 4/1/97 5/6/97 1131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 K-40 12401140 1350 i 140 1410i90 1410 130 1420 160 l Cs-134 < 15.0 <15.0 < 15.0 < 15.0 < 15.0 l
Cs-137 < 18.0 <18.0 < 18.0 < 18.0 < 18.0 l Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 l La-140 <15.0 <15.0 < 15.0 < 15.0 < 15.0 Lab Code DMI 3230 DMI-3610 DMI-051 DMI-4475 DMI-5007 Date Collected 5/20/97 6/3/97 6/17/4* 7/1/97 7/15/97 I-131 < 1.0 < 1.0 < 1.9 < 1.0 < 1.0 K-40 1350 i 130 14101 110 1500 i 120 1470 120 14601170 Cs-134 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 <18.0 < 18.0 < 18.0 <18.0 Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 <o0.0 La-140 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 Lab Code DMI-5460 DMI-5830 DMI-6205 DMI-6626 DMI-7081 Date Collected 7/29/97 8/12/97 8/26/97 9/9/97 9/23/97 1-131 < 1.0 <1.0 < 1.0 < 1.0 < 1.0 K-40 1250 110. 1410i120 1440 120 1430 120 1360 170 Cs-134 <15.0 <15.0 <15.0 <15.0 < 15.0 i Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 ,
Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 - l La-140 <15.0 <15.0 <15.0 < 15.0 < 15.0 15-1
QQANE ARNOLD Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-63 Lab Code DMI-7521 DMI-8591 DMI-9391 l
Date Collected 10/7/97 11/4/97 12/2/97 I-131 <1.0 < 1.0 < 1.0 K-40 12701150 12401150 12801140 l Cs-134 < 15.0 < 15.0 <.15.0 l Cs-137 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 <15.0 1
l l
l 15- 2
I l
DUANE ARNOLD Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-93 l
Lab Code ND* ND' DMI-1052 DMl 1640 DMl-2828, 9 Date Collected 1/7/97 2/4/97 3/4/97 4/1/97 5/6/97 1-131 - -
<1.0 < 1.0 < 1.0 K-40 - -
1570 1 130 1790 170 1840 110 Cs-134 - -
< 15.0 < 15.0 < 15.0 Cs-137 - -
<18.0 < 18.0 < 18.0 Ba-140 - -
< 60.0 < 60.0 < 60.0
)
La-140 - -
<15.0 < 15.0 < 15.0 '
Lab Code DMI-3231 DMI-3611 DMI-4052 DMI-4476 DMI-5008 Date Collected 5/20/97 6/3/97 6/17/97 7/1/97 7/15/97 1-131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 K-40 1740 200 1660i170 1810A190 16501 170 16801130 Cs- 134 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 Da-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 La-140 <15.0 < 15.0 <15.0 < 15.0 < 15.0 Lab Code DMI-5461 DMI-5831 DMI-6206 DMI-6627 DMI-7082 Date Collected 7/29/97 8/12/97 8/26/97 9/9/97 9/23/97 1-131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 l K-40 1760 180 1770i130 1940 i 200 1810 200 1750: 170 Cs-134 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 1
15- 3
DUANE ARNOLD Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-93 Lab Code DMI-7522 DMI-8592 DMI-9392 Date Collected 10/7/97 11/4/97 12/2/97 1-131 < 1.0 < 1.0 < 1.0 K-40 2000 i 200 1660 i 180 1000190 Cs-134 <15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 l
I 15-4
QUANE ARNOLD Table 15. Milk s.amples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-96 Lab Code DMI-92, 3 DMI-506 DMI-1053 DMI-1641, 2 DMI-2830 Date Collected 1/7/97 2/4/97 3/4/97 4/1/97 5/6/97 l
l-131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 K 40 14401100 1440t100 1460i 140 1470 100 1520 160 Cs-134 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 Ba 140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 <15.0 <15.0 < 15.0 l
l Lab Code DMI-3232, 3 DMI 3705 DMI-4053 DMI-4477 DMI-5009 Date Collected 5/20/97 6/3/97 6/17/97 7/1/97 7/15/97 j 1-131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 K-40 1530 i 90 1500 120 14601170 1450 160 1520 160 Cs-134 < 15.0 <15.0 <15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 Ba 140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 i La-140 <15.0 < 15.0 < 15.0 < 15.0 < 15.0 i Lab Code DMI-5462 - DMI-5832 DMI-6207 DMI-6628 DMl-7083 l Date Collected 7/29/97 8/12/97 8/26/97 9/9/97 9/23/97 1131 < 1.0 <1.0 < 1.0 < 1.0 < 1.0 K-40 15401110 15101170 14801 180 14101 120 1470 170
, Cs-134 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 I. Cs-137 <18.0 <18.0 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 <15.0 < 15.0 < 15.0 1
15- 5
)
DUANE ARNOLD Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biw eekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-96 Lab Code DMI-7523 DMI-8593 DMI-9393 Date Collected 10/7/97 11/4/97 12/2/97 I-131 < 1.0 < 1.0 < 1.0 K-40 1470 180 16801180 1370 i 150 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 1
15-6
DUANE AItNOLD i
Table 15. : Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L Location: D-101 Lab Code ND' ND' DMI-1054 DMI-1643 DMI-2831 Date Collected 1/7/97 2/4/97 3/4/97 4/1/97 5/6/97-1131 - -
< 1.0 < 1.0 < 1.0 )
K-40 - -
1270 140 1680 140 1550 160 Cs-134 - -
< 15.0 < 15.0 < 15.0 Cs-137 - -
<18.0 <18.0 < 18.0 Ba-140 - -
< 60.0 < 60.0 < 60.0 La 140 - -
<15.0 < 15.0 <15.0 :
Lab Code DMI-3234 DMI-3612 DMI-4054 DMl-4478 DMI-5010 l Date Collected 5/20/97 6/3/97 6/17/97 7/1/97 7/15/97 I131 < 1.0 < 1.0 < 1.0 < 1.0 <1.0 K-40 1730i180 1800 i 190 2120i 220 1690 120 1820 180 Co-134 <15.0 <15.0 <15.0 < 15.0 < 15.0
)
Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 ?
Da 140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 La 140 <15.0 <15.0 <15.0 <15.0 < 15 0 Lab Code DMI-5463 DMI 5833 DMI-6208 DMI-6629 DMI-7084 Date Collected 7/29/97 8/12/97 8/26/97 9/9/97 9/23/97 I-131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 K-40 1530 i 190 17501210 1570 190 1690 170 1820 130 Cs-134 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 <18.0 Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 15- 7 .
l
DUANE ARNOLD I Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30); biweekly during grazing season (May 1 through September 30)
Units: pCi/L J Location: D-101 Lab Code DMI-7524 DMI-8594 DMI-9394 Date Collected 10/7/97 11/4/97 12/2/97 I-131 < 1.0 < 1.0 <1.0 K-40 1680 i 200 1810 i 210 14101110 Cs-134 < 15.0 < 15.0 <15.0 Cs-137 <18.0 <18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 < 15.0 < 15.0 l
l l
15- 8
DUANE ARNOLD l Table 15. Milk samples, analyses for iodine-131 and ganuna-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 33); biweekly during grazing season (May 1 through September 30)
Units: - pCi/L Location: D-105 l-l Lab Code DMI-94 DMI-507 DMI-1055, 6 DMI-1644 DMI-2832 l Date Collected 1/7/97 2/4/97 3/4/97 4/1/97 5/6/97
( l131 <1.0 <1.0 < 1.0 < 1.0 < 1.0 K-40 1570 i 180 1490 i 140 1490i90 1420i150 1510 170 Cs-134 <15.0 < 15.0 < 15.0 < 15.0 < 15.0 l Cs-137 < 18.0 < 18.0 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 - < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 < 15.0 < 15.0 i
Lab Code DMI-3235 DMI-3706 ND' DMI-4479 DMI-5011 Date Collected 5/20/97 6/3/97 6/17/97 7/1/97 7/15/97 I-131 < 1.0 < 1.0 -
< 1.0 < 1.0 K-40 13701140 1280 i 170 -
1380i 160 15001190 Cs-134 <15.0 <15.0 -
< 15.0 <15.0 Cs-137 <18.0 <18.0 -
< 18.0 <18.0 Ba-140 < 60.0 < 60.0 -
< 60.0 < 60.0 La 140 <15.0 <15.0 -
< 15.0 < 15.0 Lab Code DMI-5464, 5 DMI-5834 DMI-6209 DMI-6630 DMI-7085 Date Collected 7/29/97 8/12/97 8/26/97 9/9/97 9/23/97 1-131 < 1.0 < 1.0 < 1.0 < 1.0 < 1.0 K-40 1330190 1420i170 1430 i 120 15401170 1390 120 Cs-134 < 15.0 < 15.0 < 15.0 < 15.0 <15.0 Cs-137 < 18.0 <18.0 < 18.0 <18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 < 60.0 < 60.0 i La-140 <15.0 < 15.0 < 15.0 < 15.0 < 15.0 l
l i
l 15- 9 l
l DUANE ARNOLD i
Table 15. Milk samples, analyses for iodine-131 and gamma-emitting isotopes.
Collection: Monthly during non-grazing season (October 1 through April 30), biweekly during grazing season (May 1 through September 30)
Units: pCi/L-Location: D-105 Lab Code DMI-7525 DMI-8595 DMI-9395 Date Collected 10/7/97 11/4/97 12/2/97 i
1-131 < 1.0 < 1.0 < 1.0 K-40 1310 170 12301150 15401180 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 < 18.0 < 18.0 < 18.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 i
(
- ND = No Data; sample not received. l l
1 l
l l
l l
15-10
DUANE ARNOLD I
l Table 16. Well water samples, analyses for gross beta and tritium.
l Collection: Quarterly j Units: pCi/L l
l Location D-53 Treated Municipal Water Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DWW-1536 DWW-4084 DWW-7126 DWW-9541 Gross Beta 2.2 0.6 2.710.7 4.6i o.6 1.610.4 H-3 < 330 < 330 < 330 < 330 i
Location D-54 Inlet to Municipal Water Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DWW-1537 DWW-4085 DWW-7127 DWW-9542 Gross Beta 3.5 0.8 4.3 0.8 3.210.6 3.0 0.6 H-3 < 330 330 < 330 < 330 Location D-55 On-site Well Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DWW-1538 DWW-4086 DWW-7128 DWW-9543 Gross Beta < 1.2 < 0.9 < 0.9 0.9 0.5 Fi-3 < 330 < 330 < 330 < 330 Location D-57 Bull Farm Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DWW-1539, 40 DWW-4087 DWW-7129 DWW-9544 Gross Beta 1.6 i 0.5 1.110.5 1.4 i 0.5 1.3 0.5 H-3 < 330 < 330 < 330 < 330 Location D-58 Franz Farm Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quart?r Lab Code DWW-1541 DWW-4088 DWW-7130 DWW-9545
- Cross Beta 5.910.9 4.310.7 4.9 0.6 1.020.4 I
H-3 < 330 < 330 < 330 < 330 1
i 1
16-1 I
I
DUANE ARNOLD Table 16. Well water samples, analyses for gross beta and tritium.
Collection: Quarterly Units: pCi/L
- Location D-72 Van Note Farrn l
l Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter
- Lab Code DWW-1542 DWW-4089 DWW-7131 DWW-9546 Gross Beta < 1.0 < 0.8 < 0.8 < 0.8 H-3 < 330 < 330 < 330 < 330 l
i i
t f
l l
l i
t 16 2 l l
l
DUANE ARNOLD l
Table 17. Vegetation samples (broadleaf), analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Annually Units: pCi/g wet Location D-57 D-93 D-94 D-105 D-106 Lab Code DVE-5012 DVE-5013 DVE-5014 DVE-5015 DVE-5016 Date Collected 7/15/97 7/15/97 7/15/97 7/15/97 7/15/97 Sample Type Lettuce Cabbage Lettuce Cabbage Cabbage K-40 3.5010.47 2.34 i 0.37 4.19 i 0.35 2.43 0.38 2.2610.42 Mn-54 < 0.008 < 0.012 < 0.019 < 0.025 < 0.010 Co-58 < 0.016 < 0.009 < 0.016 < 0.022 < 0.008 Co-60 < 0.025 < 0.023 < 0.020 <0.023 < 0.010 Zr-95 < 0.040 < 0.023 < 0.023 < 0.037 <0.032 Nb-95 < 0.020 < 0 014 < 0.021 < 0.033 < 0.017 Ru-103 < 0.019 < 0.010 <0.018 < 0.021 < 0.013 Ru-106 < 0.190 < 0.105 < 0.163 < 0.255 < 0.129 l-131 < 0.035 < 0.034 <0.036 < 0.053 < 0.028 Cs-134 < 0.023 < 0.007 < 0.023 < 0.022 < 0.024 Cs-137 < 0.021 < 0.021 < 0.023 < 0.025 <0.012 Cc-141 < 0.025 < 0.015 < 0.029 < 0.046 < 0.037 Ce-144 < 0.146 < 0.076 < 0.100 < 0.164 < 0.112 17-1
l DUANE ARNOLD Table 18. Vegetation samples (hay and grain), analysis for gamma-cmitting isotopes.
Collection: Annually Units: pCi/g wet Location D-16 D-16 D-57 D-57 D-58 Lab Code DVE-5816 DVE-7224 DVE-5817 DVE-8276 DVE-8277 Date Collected 8/12/97 9/26/97 8/12/97 10/20/97 10/20/97 l
Sample Type Grass Soy Beans Hay Com Com K-40 2.5410.54 8.3410.26 9.1210.60 2.70 i 0.34 2.19 0.36 Mn-54 < 0.016 < 0.007 < 0.032 <0.014 <0011 Co-58 < 0.023 < 0.006 < 0.031 < 0.007 < 0.011 Co-60 < 0.037 < 0.012 < 0.038 < 0.020 < 0.020 Zr-95 <0.067 < 0.013 < 0.056 < 0.022 <0.016
' Nb-95 < 0.018 < 0.010 < 0.030 < 0.011 < 0.020 Ru-103 < 0.025 < 0.007 < 0.021 < 0.013 <0.016 Ru-1% < 0.217 < 0.083 < 0.131 < 0.104 < 0.112 Cs-134 < 0.033 <0.011 <0.029 < 0.010 <0.013 Cs-137 < 0.042 < 0.009 < 0.031 < 0.015 < 0.018 Ce-141 < 0.040 <0.020 < 0.042 < 0.021 <0.014 Ce-144 < 0.181 < 0.070 < 0.169 < 0.083 < 0.086 Location D-63 D-63 D-72 D-93 D-105 Lab Code DVE-5818 DVE-8278 DVE-8279 DVE-5828 DVE-5829 Date Collected 8/12/97 10/20/97 10/20/97 8/12/97 8/12/97 Sample Type Hay Com Com Hay Hay K-40 19.13 i 0.87 2.6210.35 2.71 i 0.42 16.39 i 0.59 16.84 1.57 Mn-54 <0.029 < C 008 < 0.009 <0.020 < 0.054 Co 58 <0.035 < 0.017 < 0.008 <0.017 <0.046 Co-60 < 0.048 < 0.009 < 0.026 < 0.027 < 0.087 Zr-95 < 0.066 < 0.031 <0.030 <0.024 <0.090 Nb-95 < 0.034 < 0.015 < 0.020 < 0.015 <0.045 Ru-103 < 0.015 < 0.008 < 0.015 < 0.016 < 0.059 Ru-106 < 0.270 < 0.083 < 0.080 < 0.164 < 0.251 Cs-134 < 0.040 < 0.014 < 0.018 < 0.020 < 0.060 Cs-137 < 0.033 < 0.009 < 0.020 < 0.022 <0063 Ce-141 < 0.059 < 0.013 < 0.030 <0.042 <0.062 Ce-144 < 0.235 < 0.060 <0.071 <0.154 <0.430 J
l i
l l
t 18-1
DUANE ARNOLD Table 18. Vegetation samples (hay and grain), analyses gam.ma-emitting isotopes.
Collection: Annually l Units: pCi/g wet Location D-105 D-106 Lab Code DVE-8280 DVE-8281 Date Collected 10/20/97 10/20/97 Sample Type Com Com
)
K-40 1.93 i 0.24 2.75 i 0.43 Mn-54 <0.009 < 0.014 Co-58 < 0.006 < 0.015 Co-60 <0.012 < 0.010 Zr-95 <0.011 < 0.018 Nb-95 < 0.007 < 0.014 Ru-103 <0.009 < 0.020 Ru-106 <0.054 < 0.067 Cs-134 < 0.010 <0.016 Cs-137 < 0.011 < 0.016 Ce-141 < 0.021 <0.019 Ce-144 < 0.048 < 0.069 l'
1
! l I
f 1
18-2
- DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly Units: pCi/L
- Location: D-49 Lab Code DSW-344 DSW 901 DSW-1530 Date Collected 1/22/97 2/19/97 3/24/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 <15.0 < 15.0 Co-60 < 15.0 <15.0 < 15.0 7.n-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 < 15.0 < 15.0 1-131 < 15.0 < 15.0 < 15.0 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 < 15.0 < 15.0 < 15.0 l Ba-140 < 60.0 < 60.0 e 60.0 La-140 <15.0 < 15.0 < 15.0 l
Lab Code DSW-2392, 3 DSW 3423 DSW-4144 -
Date Collected {
4/21/97 5/27/97 6/18/97 Mn-54 <15.0 <15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 < 15.0 <15.0 < 15.0 2n-65 < 30.0 < 30.0 < 30.0 Zr 95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 < 15.0 <15.0 1-131 <15.0 <15.0 < 15.0 Cs-134 <15.0 <15.0 <15.0 j Cs-137 < 15.0 < 15.0 < 15.0 Da-140 . < 60.0 < 60.0 < 60.0 La 140 <15.0 <15.0 < 15.0 l
19- 1
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes. ;
Collection: Monthly Units: pCi/L Location: D-49 Lab Code DSW 5178 DSW 6211 DSW-7086 Date Collected 7/18/97 8/26/97 9/22/97 Mn-54 <15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 < 15.0 < 15.0 1-131 < 15.0 < 15.0 < 15.0 '
Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 <15.0 Lab Code DSW-8152 DSW 9199 DSW-9535 Date Collected 10/20/97 11/21/97 12/10/97 Mn-54 <15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co < 15.0 <15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 1-131 <15.0 < 15.0 < 15.0 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 <15.0 <15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 < 15.0 < 15.0 19- 2 l 1
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly I Units: pCi/L Location: D-50 l
l l Lab Code DSW-345 DSW-902 DSW-1531 Date Collected 1/22/97 2/19/97 3/20/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 <15.0 < 15.0 Co-60 <15.0 <15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0
! l-131 <15.0 <15.0 < 15.0 Cs-134 <15.0 <15.0 < 15.0 Cs-137 <15.0 <15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 <15.0 l
Lab Code DSW 2394 DSW-3424 DSW-4145 l
Date Collected 4/16/97 5/21/97 6/16/97 Mn-54 <15.0 <15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 <15.0 <15.0 < 15.0 l Co-60 <15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 I-131 <15.0 <15.0 < 15.0 Cs-134 <15.0 < 15.0 < 15.0 Cs-137 < 15.0 <15.0 < 15.0 Ba 140 < 60.0 < 60.0 < 60.0 l La-140 <15.0 <15.0 <15.0 l
l l
I l
l 19-3 i
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly -
Units: pCi/L Location: D-50 Lab Code DSW-5179 DSW-6212 DSW-7087 Date Collected 7/15/97 8/21/97 9/17/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 <15.0 <15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 <15.0 < 15.0 1-131 <15.0 <15.0 < 15.0 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 <15.0 <.15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 <15.0 Lab Code DSW-8153 DSW 9458 DSW-9536 Date Collected 10/16/97 11/19/97 12/10/97 Mn-54 <15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 <15.0 < 15.0 1 131 < 15.0 < 15.0 < 15.0 Cs-134 <15.0 < 15.0 < 15.0 Cs-137 < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La 140 < 15.0 < 15.0 < 15.0 19-4
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly l Units: pCi/L Location: D-51 l
l Lab Code DSW-346 DSW-903 DSW-1532 Date Collected 1/22/97 2/19/97 3/20/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 l Co-58 <15.0 < 15.0 < 15.0 l Co-60 <15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 I
Zr-95 < 30.0 < 30.0 < 30.0 i Nb-95 <15.0 <15.0 < 15.0 I-131 l
<15.0 < 15.0 < 15.0 l Cs-134 <15.0 < 15.0 < 15.0 Cs-137 < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 < 15.0
. < 15.0 < 15.0 I
Lab Code DSW 2395 DSW-3425 DSW-4146 Date Collected 4/16/97 5/21/97 6/16/97 Mn-54 < 15.0 < 15.0 < 15.0 l
Fe-59 < 30.0 < 30.0 < 30.0 l Co-58 <15.0 < 15.0 < 15.0 l
Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 1131 <15.0 < 15.0 < 15.0 Cs-134 <15.0 <15.0 < 15.0 1 Cs-137 < 15.0 < 15.0 < 15.0 l Ba-140 < 60.0 < 60.0 < 60.0 '
La-140 <15.0 <15.0 <15.0 l
l l
I' 19 5
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly Units: pCi/L Location: D-51 Lab Code DSW-5180 DSW-6213 DSW 7088 Date Collected 7/15/97 8/21/97 9/17/97 Mn-54 <15.0 <15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 <15.0 <15.0 < 15.0 Co-60 <15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30 0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 1-131 <15.0 < 15.0 < 15.0 Cs-134 <15.0 < 15.0 < 15.0 Cs-137 <15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 < 15.0 Lab Code DSW-8154 DSW-9459 DSW-9537 Date Collected 10/16/97 11/19/97 12/10/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 <15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 < 15.0 < 15.0 1-131 <15.0 < 15.0 < 15.0 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-1/0- <15.0 < 15.0 < 15.0 1
l 19- 6
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly Units: PCi/L Location: D-99 t
Lab Code DSW-347 DSW-904 DSW-1533 Date Collected 1/22/97 2/19/97 3/24/97 Mn-54 <15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 <15.0 <15.0 < 15.0 Co-60 <15.0 <15.0 < 15.0 Zn-61 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 < 15.0 < 15.0 1131 <15.0 < 15.0 < 15.0 Cs-134 <15.0 < 15.0 < 15.0 Cs-137- < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 < 15.0 <15.0 <15.0 Lab Code DSW-2396 DSW-3426 DSW-4147 Date Collected 4/21/97 5/27/97 6/18/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 <15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 1-131 <15.0 <15.0 < 15.0 Cs-134 < 15.0 < 15.0 - < 15.0 Cs-137 <15.0 <15.0 < 15.0 Ba-140 < 60.0 ' < 60.0 < 60.0 La-140 <15.0 < 15.0 <15.0 i
I 19 7 i
I I
DUANE ARNOLD Table 19. Surface water samples, analyses for iodine-131 and other gamma-emitting isotopes.
Collection: Monthly Units: pCi/L Location: D-99 Lab Code DSW-5181 DSW-6214 DSW-7089 Date Collected 7/18/97 8/26/97 9/22/97 Mn-54 <15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 <15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 1-131 <15.0 <15.0 < 15.0 Cs-134 < 15.0 < 15.0 < 15.0 Cs-137 <15.0 < 15.0 < 15.0 Ba 140 < 60.0 < 60.0 < 60.0 La 140 <15.0 <15.0 < 15.0 Lab Code DSW-8155 DSW-9200 DSW-9538 Date Collected 10/20/97 11/21/97 12/10/97 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr 95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 <15.0 < 15.0 1-131 <15.0 < 15.0 < 15.0 C5-134 < 15.0 < 15.0 < 15.0 C5-137 < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 <15.0 <15.0 < 15.0 19- 8
1 l
DUANE ARNOLD l
Table 20. Surface water samples, analyses for potassium-40 by flame photometry (fp), iodine-131 and other gamma-emitting isotopes.
Collection: Monthly i
Units: PC i/L Location: D-107 Lab Code DSW-348 DSW-905 DSW-1534 Date Collected 1/22/97 2/25/97 3/24/97 K-40(fp) 18.17 9.52 17.30 l
Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 l~ Co-58 < 15.0 < 15.0 < 15.0 l Co-60 <15.0 <15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 l Nb-95 <15.0 <15.0 < 15.0 1-131 <15.0 <15.0 < 15.0 Cs-134 <15.0 < 15.0 < 15.0 Cs-137 < 15.0 <15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 l La-140 < 15.0 < 15.0 < 15.0 l
Lab Code DSW-2397 DSW-3427 DSW 4148 Date Collected 4/21/97 5/27/97 6/18/97
!- K-40(fp) 23.36' 14.71 11.25 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 Co-60 <15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 l Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 <15.0 <15.0 < 15.0 1-131 <15.0 <15.0 < 15.0 t C3-134 < 15.0 < 15.0 < 15.0 l . Cs-137 < 15.0 < 15.0 < 15.0 l Ba-140 < 60.0 < 60.0 < 60.0 l .. La-140 <15.0 < 15.0 < 15.0 l
l 20-1
RUANE ARNOLD Table 20. Surface water samples, analyses for potassium-40 by flame photometry (fp), iodine-131 and other gammasmitting i otopes.
Collection: Monthly Units: pCi/L Location: D-107 Lab Code DSW-5182 DSW-6215 DSW-7090 Date Collected 7/18/97 8/26/97 9/22/97 K-40(fp) 11.25 21.63 12.11 Mn-54 < 15.0 < 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 <15.0 <15.0 < 15.0 Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 Nb-95 < 15.0 < 15.0 < 15.0 1-131 <15.0 <15.0 < 15.0 Cs 134 <15.0 <15.0 < 15.0 Cs 137 < 15.0 < 15.0 < 15.0 Ba-140 < 60.0 < 60.0 < 60.0 La-140 < 15.0 < 15.0 < 15.0 Lab Code DSW-8156 DSW-9201 DSW-9539 Date Collected 10/20/97 11/21/97 12/10/97 K-40(fp) 17.30 22.49 17.30 Mn-54 < 15.0 c 15.0 < 15.0 Fe-59 < 30.0 < 30.0 < 30.0 Co-58 < 15.0 < 15.0 < 15.0 -
l Co-60 < 15.0 < 15.0 < 15.0 Zn-65 < 30.0 < 30.0 < 30.0 Zr-95 < 30.0 < 30.0 < 30.0 l Nb-95 <15.0 < 15.0 < 15.0 l l-131 < 15.0 <15.0 < 15.0
- j. Cs-134 <15.0 < 15.0 < 15.0 L Cs 137 < 15.0 < 15.0 < 15.0 l Ba-140 < 60.0 < 60.0 < 60.0 La 140 < 15.0 . <15.0 <15.0
- Corrected data.
20- 2
DUANE ARNOLD Table 21. Surface water samples, analysis for tritium.
Collection: Quarterly composites of monthly samples Units: pCi/L Location D-49 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DSW-1920 DSW-5188 DSW-8614 DSW-10115 H-3 < 330 < 330 < 330 < 330 Location D-50 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DSW-1923 DSW-5189 DSW-8615 DSW-10116 H-3 < 330 < 330 < 330 < 330 Location D-51 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DSW-1924 DSW-5190 DSW-8616 DSW-10117 H-3 < 330 < 330 < 330 < 330 Location D-99 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DSW-1919 DSW-5191 DSW-8617 DSW-10118 H-3 < 330 < 330 < 330 < 330
' Location D-107 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DSW-1921 DSW-5192 DSW-8618 DSW-10119 l H-3 < 330 < 330 < 330 < 330 i
21- 1 l
l
DUANE ARNOLD Table 22. Fish samples, analysis of edible portion for gamma-emitting isotopes.
Collection: Semiannually Units: pCi/g wet Location Upstream D-49 Lab Code DF-4046 DF-4047 DF 7221,2 Date Collected 6/6/97 6/6/97 9/19/97 Sample Type Carp Buffalo Carp K-40 2.80 i 0.37 2.99 i 0.37 2.84 i 0.31 Mn-54 < 0.010 <0.014 <0.012 Fe-59 <0.032 <0.035 < 0.031 Co-58 < 0.016 < 0.009 < 0.009 l Co-60 < 0.007 < 0.016 < 0.006 Zn-65 < 0.042 < 0.028 <0.033 Zr-95 < 0.019 <0.040 <0.019 Nb-95 < 0.022 < 0.025 < 0.017 Ru-103 <0.012 < 0.017 < 0.018 Ru-106 < 0.098 < 0.093 < 0.054 Cs-134 < 0.008 < 0.014 < 0.014 Cs-137 < 0.013 < 0.014 < 0.007 Ce-141 < 0.012 < 0.020 < 0.025 Ce-144 < 0.067 <0.087 <0.069 Location Downstream D-61 Lab Code DF-4048 DF-4049, 50 DF-7223 Date Collected 6/6/97 6/6/97 9/19/97 Sample Type Carpsucker Carp Carp K-40 2.4810.53 2.9310.23 2.9810.52 i Mn-54 < 0.019 < 0.009 - < 0.022
! Fe-59 <0.025 < 0.010 < 0.043 j Co-58 < 0.012 < 0.008 <0.009 l Co-(0 < 0.010 < 0.011 < 0.008 Zn-65 < 0.032 <0.013 < 0.071 I Zr-95 < 0.038 < 0.013 < 0.022 Nb-95 < 0.011 < 0.007 < 0.043 Ru 103 <0.020 < 0.006 < 0.024
- Ru-106 < 0.125 <0.070 < 0.151 Cs-134 < 0.014 < 0.006 < 0.018 Cs-137 < 0.018 <0.006 < 0.013 Ce-141 < 0.016 < 0.014 < 0.028 Ce-144 < 0.057 ' < 0.037 <0.150 l
22 1 j
l DUANE ARNOLD Table 23. River sediment samples, analysis for gamma-emitting isotopes.
Collection: Semiannually Units: PCi/g dry Location D-50 Lab Code DBS-4055 DBS-7123 Date Collected 6/4/97 9/17/97 K-40 6.5010.42 8.2210.38 Mn-54 <0.020 < 0.011 Co-58 <0.025 <0.013 Co-60 < 0.013 < 0.011 Zr-95 <0.061 <0.012 Nb-95 < 0.031 < 0.017 Ru-103 - <0.023 < 0.012 Ru-1% < 0.115 < 0.058 Cs-134 < 0.021 < 0.033 -
Cs 137 < 0.019 - < 0.016 Ce-141 < 0.043 <0.029 Ce-144 <0.087 < 0.088 Location D-51 Lab Code DBS-4056 DBS-7124 Date Collected 6/4/97 9/17/97 K-40 6.024 0.59 10.99 t 0.62 Mn-54 < 0.019 < 0.018 Co-58 < 0.026 < 0.035 Co-60 < 0.025 < 0.019 Zr-95 < 0.076 <0.044 Nb-95 < 0.033 < 0.029 Ru-103 < 0.036 <0.016 Ru-106 < 0.167 < 0.173 Cs-134 < 0.028 < 0.051 Cs-137 < 0.022 < 0.019 Ce-141 <0.042 < 0.066 Ce-144 < 0.157 <0.079 1
j 23 1
DUANE ARNOLD 1
Table 23. River sediment samples, analysis for gamma-emitting isotopes.
l Collection: Semiannually Units: pCi/g dry Location D-107
! Lab Code DBS-4057 DBS-7125 l Date Collected 6/4/97 9/17/97 K-40 5.15 i 0.69 6.62i o.93 Mn-54 < 0.048 < 0.043 Co-58 < 0.045 < 0.026 Co-60 0.248 0.039 0.159 0.051 Zr-95 < 0.056 < 0.099 Nb-95 < 0.034 < 0.062 Ru-103 <0.037 < 0.048 Ru-106 < 0.311 < 0.319 Cs-134 <0.055 <0.053 Cs-137 < 0.041 <0.038 Ce-141 < 0.050 < 0.060 Ce-144 <0.120 < 0.129 i
i l
23- 2
DUANE ARNOLD Table 24. Precipitation samples, analysis for gamma-emitting isotopes.
Collection: Monthly Units: pCi/L Location: Duane Arnold Lab Code DP-349 DP-900 DP-1535 Date Collected 1/22/97 2/19/97 3/24/97 Mn-54 <7.0 < 3.5 <3.9 Fe-59 <8.5 <7.9 <2.4 Co-58 <6.3 <2.3 <5.4 Co-60 <8.0 <4.4 < 2.9 Zn-65 < 16.9 < 5.7 < 15.3 Zr-95 <11.2 <8.2 < 4.3 Nb-95 <5.7 < 3.7 < 4.0 1-131 <7.1 <8.0 < 8.8 Cs-134 <3.4 < 3.6 <3.4 C5-137 <5.8 < 4.8 < 2.8
, Ba-140 < 39.1 <19.5 < 11.1 l La 140 <8.3 <3.6 < 3.8 Lab Code DP-2398 DP-3422 DP-4149 Date Collected 4/21/97 5/27/97 6/18/97 Mn-54 <3.0 < 4.1 <5.7 Fe-59 < 4.8 <9.1 < 4.6
! Co-58 < 1.7 <5.9 < 3.6 Co-60 <2.7 < 4.2 < 5.8
' Zn-65 < 9.7 <6.2 <5.5 Zr-95 <6.7 <9.8 < 7.6 Nb-95 < 1.5 < 3.6 < 5.3 l I-131 <3.2 < 9.0 < 9.5 Cs-134 <2.9 < 4.7 < 7.1 Cs-137 <3.1 <3.9 < 4.8 l Ba 140 < 12.2 < 27.8 < 27.4 l La-140 < 1.6 <5.2 <3.5 l
I I
l i
24-1
DUANE ARNOLD Table 24. Precipitation samples, analysis for gamma-emitting isotopes Collection: Monthly Units: pCi/L Location: Duane Arnold Lab Code DP-5183 DP-6216 DP-7132 Date Collected 7/18/97 8/26/97 9/23/97 Mn-54 < 4.3 <6.6 < 6.4 Fe-59 < 11.9 <5.7 < 11.6
^ Co-58 <5.1 <5.6 < 2.8 Co-60 < 4.9 <6.8 < 6.6 Zn-65 <7.7 < 10.0 < 9.6 Zr-95 <5.6 < 13.7 < 14.3 Nb-95 <5.9 <6.0 < 7.0 1-131 < 12.9 < 13.6 <8.0 Cs-134 <3.6 < 4.5 < 7.5 Cs-137 <5.8 <8.2 < 6.6 Ba-140 < 37.6 < 36.1 < 24.0 La-140 <7.2 <7.3 < 4.3 Lab Code DP-8157 DP-9460 DP-9540 Date Collected 10/20/97 11/19/97 12/10/97 Mn-54 < 2.7 <6.8 <7.3 Fe-59 <. 3.3 <15.0 <5.6 Co-58 < 1.6 < 6.7 - <5.1 Co-60 < 3.2 <4.7 <8.2 Zn-65 < 10.6 < 11.4 < 20.5 Zr-95 <7.5 <8.7 < 10.3 Nb-95 <2.4 <8.0 <7.7 I-131 < 4.2 < 20.1 < 7.8 ;
Cs-134 < 1.9 < 6.8 <5.1 l Cs-137 <3.4 <7.9 < 6.6 !
Ba 140 < 10.5 < 44.0 < 35.0 l l '
La 140 < 2.5 <12.7 < 8.8 24- 2
DUANE ARNOLD Table 25. Precipitation samples, analysis for tritium.
Collection: Quarterly composites of monthly samples Units: pCi/L Location Duane Arnold Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DP-1922 DP-5193 DP-8619 DP-10137 H3 < 158 < 185 < 160 < 160 l
i l
25-1
DUANE ARNOLD Table 27. Soil samples, analyses for strontium-90 and gamma-emitting isotopes.
Collection: Annually Units: pCi/g dry l
l Location D-15 D-16 '
Lab Code DSO-7121 DSO-7122 Date Collected 9/23/97 9/23/97 t
Sr-90 0.044 0.011 0.057 i 0.016 K-40 15.84 i 0.64 10.042 i 0.46 Mn-54 < 0.019 < 0.012 Co-58 < 0.030 <0.021 Co-60 < 0.023 < 0.013 Zr-95 < 0.018 < 0.027 Nb-95 < 0.046 < 0.028 l Ru-103 < 0.020 < 0.018 Ru-106 <0.118 < 0.053 Cs-134 < 0.032 < 0.037 Cs-137 0.120 i 0.027 0.282 i 0.026 Ce-141 < 0.061 <0.035 Ce-144 <0.143 < 0.068 i
l l
l l
l 27-1