ML20069G464

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Radiological Environ Monitoring Program,1981
ML20069G464
Person / Time
Site: Susquehanna  Talen Energy icon.png
Issue date: 07/31/1982
From:
RADIATION MANAGEMENT CORP. (RMC)
To:
Shared Package
ML18031A398 List:
References
RMC-TR-82-03, RMC-TR-82-3, NUDOCS 8209290105
Download: ML20069G464 (126)


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{{#Wiki_filter:. RMC-TR-82-03 i SUSQUEHANNA STEAM ELECTRIC STATION Radiological Environmental Monitoring Program 1981 ANNUAL REPORT Prepared for PENNSYLVANIA POWER AND LIGHT COMPANY by RADIATION MANAGEMENT CORPORATION JULY 1982 hR OC 0 00 07 R PDR

RMC-TR-82-03 SUSQUEHANNA STEAM ELECTRIC STATION RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM 1981 ANNUAL REPORT Prepared for Pennsylvania Power and Light Company by Radiation Management Corporation JULY 1982

TABLE OF CONTENTS PAGE PROGRN1 SUMitARY ----------------------------------------- 1 INTRODUCTION ----------------------------------------- 5 PROGRN1 ----------------------------------------- 9 Sample Collection ----------------------------------------- 11 Data Interpretation ----------------------------------------- 12 Program Exceptions ----------------------------------------- 13 Program Changes ----------------------------------------- 14 RESULTS AND DISCUSSION --------------------------- ------------- 17 . Waterborne Pathway ----------------------------------------- 19 Airborne Pathway ----------------------------------------- 21 Ingestion Pathway ----------------------------------------- 23 Direct Radiation ----------------------------------------- 25 CONCLUSIONS ----------------------------------------- 27 REFERENCES ----------------------------------------- 31 LIST OF TAS! ES ----------------------------------------- 11 LIST OF FIGURES ----------------------------------------- ii LIST OF APPENDICES ----------------------------------------- ti / r

LIST OF TABLES s N0. PAGE

1. Synopsis of the Susquehanna SES Radiological Environmental Monitoring Program - 1981 ------------------------------ 35 I

i LIST OF FIGURES N0. PAGE

1. Average Concentrations of Tritium in Surface Water in the Vicinity of Susquehanna SES,1973 through 1981 ------- 36
2. Gross Beta Activity in Air Particulates in the Vicinity of Susquehanna SES Site,1981 ---------------- --------- 37
3. Average Ambient Radiation Levels in the Vicinity of Susquehanna SES, 1973 through 1981 --------------------- 38 LIST OF APPENDICES PAGE Appendix A -

Preoperational Environmental Radiological Moni-to ring Program Annual Summary ------------------- 39 Appendix B - S amp l e De s i g n ati on ------------------------------ 49 Appendix C - Data Tables ------------------------------------- 59 Appendix D - Synopsis of Analytical Procedures --------------- 113 i Appendix E - Results of the EPA Inter-Laboratory Comparison

Program ---------------------------------------- 127 Appendix F -

Site Specific Demographic Data ----------------- 137 ii

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PROGRN1 SUIf4ARY Since April 1972 Radiation flanagement Corporation (Rf1C) has conducted the Pre-operational Radiological Environmntal fionitoring Program (REl1P) for Pennsylvania Power and Light Company (PP&L) at the Susquehanna Steam Electric Station (SES). This report presents the analytical results for samples taken during 1981. A total of 3125 analyses on 2239 samples including direct radiation, surface water, well water, potable water, sediment, air particulates, air iodine, precipitation, milk, fish, food products, meat, game, vegetation, pasture grass and soil was performed in 1901. A variety of radionuclides, both naturally occurring and man-made, were detec-ted in the environs of the Susquehanna SES. llaturally occurring radionuclides were found at levels expected for that environment. The man-made radionuclides found, primarily in air particulates, precipitation and pasture grass, were the fission products typically found in nuclear weapon test fallout. In particular, f allout from the atmospheric nuclear weapon test by the People's Republic of China on October 16, 1980 was observed in samples collected in the first half of the year. The detection of this event indicates that the Susquehanna SES REf4P is sensitive to fluctuations in the radiological characteristics of the environment around Susquehanna SES. 3 L

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INTRODUCTION The Susquehanna SES will contain 2 BWR generating units, each with a capacity of about 1050 flWe. Units #1 and #2 are scheduled for initial criticality in 1982 and 1984, respectively. This site is located on a 1075 acre tract along the Susque-hanna River, five miles northeast of Berwick in Salem Township, Luzerne County, Pennsylvania. The area surrounding the site can generally be characterized as rural, with forest and agricultural lands predominating. flore specific information on the dem-ography, hydrology, meteorology and land use characteristics of the local area may be found in the Environmental Report (1), the Safety Analysis Report (2) and the Draft Environmental Statement - 0.L. (3) for Susquehanna SES. RMC has previously reported resulte fr - the preoperational radiological environ-mental monitoring program (REMP) from *i'2-1980 (4-12); the present document continues the series with coverage for 1981. It resents in detail the type and number of sam- .ples collected, the analyses performes and the data generated. 7

, '*4 PROGRAM

PROGRAft The preoperational REf1P continued in 1981 and will continue until initial criti-cality of Unit #1. At that time, the operational phase of the program will be insti-tuted and continue thereafter. The RE!!P was designed utilizing the guidance in the Branch Technical Position to the fluclear Regulatory Comission Regulatory Guide 4.8, Rev. 1,fiovember 1979(13) and ORP/SID 72-2, Environmental Radioactivity Surveillance Guide (14). The REftP was designed:

1. Te stablish baseline radiological characteristics of the environs of Susquehanna SES for comparison with future data;
2. To assure that media sampled and analyzed are sensitive to fluctuations in the radiological characteristics of the Susquehanna SES environs; and to assure that the program will be responsive to station radioeffluent discharge;
3. To monitor potential critical pathways of station radioeffluent to man.

Samples for the 1981 REftP were taken from direct, waterborne, airborne and inges-tion pathways with emphasis on those media which would yield data for the evaluation of radiation dose to man. Specific sampling locations were chosen on the basis of potential water use, site meteorology, local demography and land uses. Environmental sampling locations were divided into two classes, indicator and control. Indicator samples were those collected at locations which would be expected 1 to manifest future station effects, if any, and were selected on the basis of distance from the site, topography, hydrology, meteorology, demography, and drainage character-istics. Control samples were collected at locations which are expected to be unaffected by station operation. Table 1 summarizes the Susquehanna REMP as perfonned in 1981. Appendix A summarizes the results of the REf1P analyses and compares indicator and control location results. Appendix B describes the RMC coding system, which specifies sample type and location. Included in Appendix B. Table B-1 gives the pertinent information on individual sampling locations, while Maps B-1 and B-2 show the sampling locations. The data for individual i samples are presented in tabular form in Appendix C. A synopsis of the analytical pro-i cedures used for the samples appears in Appendix D. Appendix E contains the results of l RMC's participation in the EPA inter-laboratory comparison program. Appendix F contains l the results of. demographic data surveys perforned in 1981. Sample Collection l Waterborne pathways were examined by analyzing samples of surface water, ground water, potable (drinking) water and sediment. Surface, ground and potable water sam-i ples were collected in unused two gallon plastic containers weekly and monthly. Sus-quehanna River sediment was also sampled. l Airborne pathways were examined by analyzing air particulates, air iodine and pre-l cipitation. Air particulates were collected weekly on Gelman type-A/E, glass fiber fil-ters with low volume air samplers. Air iodine was collected on one inch deep Science l Applications, Inc. charcoal cartridges. Air sample volumes were measured with tempera- , ture-compensated dry-gas meters. Precipitation samples were collected in unused two ( gallon plastic containers monthly. l 11 l

Ingestion pathways were examined by analyzing samples of fish, milk, pasture grass, game, locally grown food products and soil. Several species of fish samples were collected in spring and late summer at both the control and indicator locations, filleted and frozen for shipment to RMC. Milk, food products and pasture grass were purchased directly from local fanners. Game samples were obtained by hunting or from road killed animals. Twelve plugs were collected at each location. Each plug was split into a topsoil sample and a subsoil sample. The twelve topsoil samples were combined to make one topsoil sample and the twelve subsoil samples were combined to make one subsoil sample. This resulted in one topsoil sample and one subsoil sample from each soil sampling location. Direct radiation measurements were made using thennoluminescent dosimeters (TLDs) consisting of calcium sulfate doped with thulium (CaS0 (Tm)). The TLDs were placed at locations designed to take advantage of local meteofologic and topographic charac-teristics and population distribution characteristics. Data Interpretation The radioanalytical and direct radiation data collected during 1981, together with that collected previously, will be used as a baseline with which operational data may be compamd. Several factors are important in the interpretation of the data. These factors are discussed here to avoid repetition in sections that follow. Within the data tables (Appendix C) a 95% ( 2 sigma) confidence interval is supplied for each result above the lower limit of detection (LLD) with the exception of strontium-89, -90 analyses, which are mported as minimum detectable level (MDL). Numerically, the LLD is equal to 4.66 times the square root of the quotient resulting from the background counts divided by the background counting time. The result is then divided by a dpm/ picocurie conversion factor, the counting e"ficiency and the sample volume. Whereas the MDL is equal to 3 times the square roct of the quotient resulting from the background counts divided by the background counting time. This result is then divided by the dpm/ picocurie conversion factor, the counter efficiency and the sample aliquot (the exact specifications of the calculations are noted in AppendixD). The MDL or LLD is reported when the 2 sigma error exceeds 100% of the calculated activity. The 2 sigma intervals represent the range of values into which 95% of repeated analyses of the same sample would fall. The LLD quoted for particu-lar sample types (Table C-29) are nominal values. The actual LLD is calculated for each sample analyzed and will show variability due to the amount of sample analyzed, the length of time between sample collection and counting, the length of time a par-ticular sample was counted and fluctuations in counting background. It is characteristic of environmental monitoring data that many results occur at or below the LLD. In this report, all results occurring at or below the relevant LLD were reported as being "less than" the LLD value. Results for each type of sample were grouped according to the analysis performed. Averages and standard deviations of these results were calculated when applicable. The calculated standard deviations of grouped data (by location or over time) repre-sent sample rather than analytical variability. For these calculations any values i below LLD were considered to be at the LLD; thus, these averages were biased high and the corresponding standard deviations were biased low. Averages were not calcu-lated when a group of data was composed of many (>50%) LLD values. 12

Program Exceptions 4 As the REMP for Susquehanna SES progressed in 1981, certain samples and analyses were inadvertently omitted from the schedule. These exceptions are delineated, and the reasons for the omission stated. However, taking into account all program excep-tions, it should be noted that the 1981 Susquehanna SES REMP had a 98% completion rate. Surface Water

1. The monthly samples from stations 12F1 and 12G2 for January and February were not collected because the river was frozen.
2. The monthly analysis for iodine-131 was omitted in February for station 6S5 due to a delay in sample shipment.
3. The weekly samples for iodine-131 analysis were not collected at station 12F1 in January and the first and second weeks of February because the river was frozen.
4. The weekly samples from station 3G2 were not collected in the first three weeks of January and the first week of February because the river was frozen.
5. The weekly sample from station 3G5 was not collected during the second week of February because the river was frozen.
6. Six weekly samples from May and June were lost in shipment. These were two samples from station SS8 and one sample each from stations ID3, 3G1, 3G2 and 3G5.
7. The weekly samples for iodine-131 analysis were not collected during the fourth week in December from stations 3G2 and 3G5 because the river was frozen.

Air Particulates and Air Iodine

1. No samples were received from station 12E1 between January 3 and January 11 due to a sampler malfunction.
2. No samples were received from station 12G1 between April 19 and April 26 due to a sampler malfunction.
3. No samples were received from station 7G1 between May 3 and May 10 due to a sampler malfunction.
4. Sample collection was missed on June 24 for station 7H1 due to collector error; therefore, the sample collected on July 2 represents a two week period.

Precipitation

1. No samples were received in January because the water was frozen.
2. No samples were received from stations 11S2 and 12G2 in February because the water was frozen.

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Milk

1. flo sample was available from station 7C1 and 8D1 in July and 7C1 in September because of the limited supply of goat milk.
2. 110 sample was received from station 8D1 from January to March because the goat was dry.

Food Products fio samples were received from stations 11D2 and 12F4 because the farmer who farms both farms did not plant this year. Pasture Grass fio sample was received from ctation 15A1 from January through March due to snow Cover. TLD flo sample was received from station 7F1 for the third quarter due to a loss in the field. Program Changes Additions to the program were made in 1981. These were added in order to better reflect any changes in radioactivity levels during Susquehanna SES operation. These changes are noted.

1. Surface water station 3H3 was changed to 3G5 when it was determined that the wrong designation had been in use.
2. Air particulate and air iodine stations 15S4 and 7G1 were added for weekly collection.
3. Goat milk station 7C1 was added for quarterly iodine-131 analysis. Pas-ture grass will be sampled during the months milk is not collected.
4. The fish control location designation was changed from 2G to 2H when it was determined that the wrong designation had been in use.
5. Analysis of topsoil and subsoil samples at fourteen locations was added.

Samples will be collected at three year intervals at which time the need for further collection will be evaluated.

6. TLD stations 3H1 and 3H2 were changed to 3G3 and 3G4 respectively, when it was determined that the wrong designations had been in use.
7. TLD station 14S2 was relocated to station 14S5 on June 29 in order to avoid obstructions.
8. Two TLD stations 15S4 and 10B3 were added as part of a continuing effort to upgrade the Environmental Monitoring Program.

14

l Some analyses were added as well. These are noted below.

1. Gross alpha and tritium analyses were changed from quarterly compo-site to monthly for potable water station 12il2 in April.
2. Iodine-131 and gamma spectrometry analyses were increased to semi-monthly for milk stations 12B2 SE1,13E3 and 10G1 during the-months when cows are on pasture, April to September.

Some deletions were made to the program since sufficient data is provided in the remaining program to monitor the radiological characteristics of the environment. These deletions are noted below.

1. Tritium and gamma spectrometry of precipitation samples were changed from monthly to quarterly composite beginning with the second quarter.
2. Food product samples.from stations SS6,11A3 and 12E3 were taken in 1980 as supplements for that year and therefore, were not collected in 1981.
3. Analysis of meat and game bones and egg shells was discontinued for 1981 samples.
4. A deer sample was not collected due to the difficulty in hunting and obtaining road kill samples.
5. The broad leaf vegetation sampling in the sectors with the highest D/Q was changed from 13S3 and 14S3 to 7S4 and 8S3 because new cal-culations indicated a change in the sectors with the highest D/Q for 1981.

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l t RESULTS AND DISCUSSION _ _ _ _ _ _ - _ _ _ _ _ _ _ - - _ - _ _ _ _ _ _ - _ - _ . - _ _ _ _ _ - _ _ - _ _ - _ _ _ _ _ _ _ _ _ - _ _ \

4 RESULTS AllD-DISCUSSI0fl All environmental sanples.and TLDs were analyzed by standard Ri1C analytical pro-cedures (15). A synopsis of these procedures appears in Appendix D. Since the preci-sion and accuracy of the analytical results is of paramount importance, R!iC devoted a i fraction (usually.15-20%) of all analyses to quality control including process quality control, instrument quality control, inter-laboratory cross-check analyses and compre-hensive data review. The results of Rl4C's QC program for 1981 are included in a sepa-rate RMC report (16). One important aspect in maintaining laboratory quality control is R!1C's participation in the United States Environmental Protection Agency (USEPA) inter-laboratory comparison program. This data appears in R!1C's annual QC report and is also presented as Appendix E to this report. The analytical results of the 1981 RE!!P have been divided into four categories: waterborne, airborne, ingestion and direct radiation. The individual sanples and anal-yses within each category provide an adequate means of estimating radiation. doses to individuals from the principal pathways. The analytical .results for the 1981 program i are summarized in Appendix A. The data for individual samples are presented in tabular fonn in Appendix C. The sensitivities stated in the Branch Technical Position were met for all samples (13). Waterborne Pathway The waterborne pathways of exposure from Susquehanna SES were evaluated by analyzing samples of surface water, well water, potable water and sediment. 1 Surface Water (Tables C-1, C-2, C-3 and C-4) The Susquehanna River was sampled monthly at seven locations. Daily grab samples were collected at 12H1 (Merck Company) then composited into a monthly sample. lionthly samples were also composited from weekly grabs at station SS8 (under the' power line) and station 6S5 (outfall area). fionthly grab samples were collected at station 103 (Mocanagua Substation), station 13E1 (Glen Brook Reservoir), station 12F1 (Bemick Bridge) and station 12G2 (between Bloomsburg and Bemick). Monthly surface water i samples were analyzed for gross beta, gamma emitters and iodine-131. Quarterly com-posites were analyzed for tritium, strontium-89 and -90. Weekly grab samples were collected from stations 103,12F1, 2F2 (Retmat Bridge), 3G1 (Lower Bridge Plynouth) 3G2 (flanticoke Bridge) and 3G5 (Market Street Bridge) and weekly composite samples were collected from stations SS8 and 12H1 in order to study the occurrence of detectable concentrations of iodine-131 in the river water. A mon-thly effluent water grab sample was collected at station 1D5 (Shickshinny Sewage Treat-ment facility) for iodine-131 analysis. Analysis for beta emitters in samples of surface water showed detectable activity in 72 of 80 sanples, with results. ranging from 1.0 to 6.9 pCi/1. The gross beta results were consistent with the data previously obtained from 1972-1980 (4-12). fliobium-95 was observed in five samples and ruthenium-103 was observed in one of eighty samples analyzed for gamma emitters. These nuclides were observed in the first half of the year and are consistent with the data obtained from air particulates and precipitation. The occurrence of these nuclides can be attributed to the atmospheric nuclear weapons test by the People's Republic of China. Potassium-40 and thorium-232 were observed in the June sample from station 12H1. This is probably due to sediment 19

contamination of the sample. These nuclides are typically found in sediment samples. Cobalt-60 was found in the April sample from station 12G2. Positive iodine results, in surface water, were reported in 68 of 402 samples with values ranging from 0.08 to 1.0 pCi/l. These results were observed sporadically during all months except April and at all weekly stations. Since~Susquehanna SES is not in operation, iodine-131 in the surface water can be attributed to other sources of contamination of the river. The analysis of tritium in surface water showed detectable activity in 17 of 28 samples with results ranging from 68 to 183 pCi/1. This is well below the action level of 20,000 pCi/l as quoted in the Branch Technical Position (13). The average tritium concentrations in surface water samples shows a gradual decline for the period 1973 to 1981. This is likely the result of a reduction in atmospheric tritium from nuclear detonations. Average tritium concentrations for all locations since 1973 were graphed in Figure 1. Positive tritium results are reported when the 2 sigma counting error is less than the result. In some cases, this may cause positive re-sults to be reported, which are lower than the calculated LLDs. For clarification of the method of calculation, see Appendix D, Analysis of Water Samples for Tritium. Levels of strontium-89 were below MDL (0.6 to 2.7 pCi/1) in twenty-four of twenty-eight samples. Strontium-89 was found in four samples. The range of con-centrations (0.4 to 0.8 pCi/1) was comparable to the MDL levels found in the other samples. Levels of detectable strontium-90 ranged from 0.2 to 1.1 pCi/l in ten of the twenty-eight samples. The MDL values ranged from 0.4 to 1.1 pCi/1. Well Water (Tables C-5, C-6 and C-7) Three wells, the peach stand on-site (4S2), the Serafin Farm (15A4) and the Berwick Water Co. (12F3), were sampled monthly. Gross beta and gamma analyses were performed on the monthly samples. Gross alpha and tritium analyses were performed on quarterly composites of monthly grab samples. Gross beta results showed positive values in twenty-six of thirty-six samples with results ranging from 1.2 to 7.4 pCi/1. LLDs ranged from 1.7 to 2.4 pCi/1. Potassium-40 was observed in two samples collected from station 15A4. Both results were below the LLD normally obtained for potassium-40. This indicates that these analyses were unusually sensitive, however the results may reflect actual concentrations. All other garmia emitting nuclides were less than LLD. All twelve results for gross alpha were below the LLD which ranged from 0.9 to 2.6 pCi/1. Six of twelve samples showed positive tritium results ranging from 72 to 150 pCi/1 with LLDs ranging from 118 to 122 pCi/1. Positive results for gross beta, gross alpha and tritium compared closely to the respective LLDs for those anal-yses and to results found in previous REMP reports (4-12). Potable (Drinking) Water (Tables C-8, C-9 and C-10) l Potable water was sampled monthly at two locations, the Berwick Water Company (12F3) and the Danville Water Company (12H2). In addition, weekly samples were col-lected from station 12H2 for iodine-131 analysis. Gross beta and gamma emitters were 20

analyzed monthly. Strontium-89 and -90 were analyzed as quarterly composites. Gross alpha and tritium were analyzed as quarterly composites for station 12F3 and monthly for station 12H2. Sixteen of twenty-four samples showed positive gross beta results ranging from 1.3 to 8.5 pCi/1 and averaging 2.4 pCi/1. All results from all gamma emitting nuclides were less than LLD. Two samples collected from January and one sample collected from flovember showed positive results (0.14-0.3 pCi/1) for iodine-131 analyses at the Danville Water Cor.pany. This was found to be consistent with iodine-131 activity in weekly surface water samples. All others were below the LLD. All fourteen results for gross alpha were below the LLD which ranged from 0.5 to 2.3 pCi/1. These results compare favorably to the EPA drinking water action level of 15 pCi/l for gross alpha (17). Nine of fourteen samples analyzed showed positive tritium results ranging from 70 to 383 pCi/1, with LLDs ranging from 102 to 122 pCi/l for the others. The results fall below the EPA tritium action level of 20,000 pCi/l for drinking water (17). The tritium results, for potable water, were consistent with results for tritium observed in surface water of the Susquehanna River. All results for strontium-89 were below the MDL of 0.6 to 1.7 pCi/1. Two detecta-ble concentrations of strontium-90 (0.2 and 0.5 pCi/1) were observed in eight samples. The MDL values ranged from 0.4 to 0.8 pCi/1. Sediment (Tables C-11 and C-12) Sediment samples were taken semiannually from three locations in the Susquehanna River. Samples were taken at Bell Bend (78), downstream near Hess Island (11C) and upstream near Gould Island (28). Samples were analyzed for gamma emitting nuclides, gross alpha, strontium-89 and -90. Naturally-occurring K-40, Ra-226 and Th-232 were detected in all samples. Be-7, from cosmic ray activity, was also observed in one of the six samples analyzed. Cs-137 was detected in all samples, with levels ranging from 0.06 to 0.14 pCi/g(dry). Zircon-ium-95, niobium-95, ruthenium-103, cerium-141 and cerium-144 were observed in the sedi-ment samples especially in the May samples. These nuclides were consistent with those observed in surface water and can be attributed to the atmospheric nuclear weapons test on October 16, 1980. Gross alpha analyses showed positive values for five of six samples, ranging from 5.2 to 14 pCi/g(dry). One sample analyzed for strontium-89 showed a positive result of 0.15 pCi/g(dry). This result is similar to the MDL values. All other strontium-89 re-sults were below the MDL of 0.1 pCi/g(dry). Three of six samples showed positive stron-tium-90 results ranging from 0.02 to 0.07 pCi/g(dry). The other results were below the MDL (0.03 to 0.07 pCi/g(dry)). Airborne Pathway The airborne pathways of exposure from Susquehanna SES were evaluated by analyzing samples of air particulates, air iodine cartridges and precipitation. Samples of air w2re collected at twelve stations; the Information Center (2S2), the biological labora-21

tory (SS4 and 505Q), the Golomb House (11S2), the transmission line at site 15 (15S4), the transmission line east of route 11 (981), the Mocanagua Substation (102), near Pond Hill (3D1), the Berwick Hospital (12E1), the Hazelton Chem Lab (7G1), at Blooms-burg (12G1) and the PP&L roof in Allentown (7HI). Station 7G1 began operation in March. Station 15S4 began operation in May. Air filters were analyzed weekly for gross beta and quarterly for gamma emitters, gross alpha and strontium-89 and -90. Air iodine was collected on charcoal cartridges in series with the air particulate filter at all stations. Stations 102, 3D1, 7G1 and 12G1 began sampling for air iodine in March while station 15S4 began operation in May. The charcoal cartridges have an efficiency of removal of elemental iodine of 99%. Precipitation samples were collected monthly from stations SS4,11S2,1D2 and 12G1 and analyzed for tritium and gamma emitters. Beginning in April, precipitation samples were composited and analyzed quarterly.

Air Particulates (Tables C-13, C-14 and C-15)

The gross beta concentrations of each sgmple was detemined weekly. These con-centrations ranged from 0.004 to 0.384 pCi/m in all samples. The wide range can be attributed to the fallout througiiout the year from the atmospheric nuclear weapon test by the People's Republic of China on October 16, 1980. By October 1981, gross beta levels had returned to pre October 1980 nuclear test levels. The annual average for all indicator stations was 0.097 pCi/ cubic meter and for all control stations was 0.094 pCi/ cubic meter. Figure 2 shows graphically the gross beta activity in air par-ticulates for 1981. Quarterly composites of air particulate filters from each location were analyzed by gamma spectrometry. Beryllium-7 was detected in forty-six of forty-seven samples. The presence of beryllium-7 throughout the year can be attributed to cosmic ray acti-vity. Cesium-137 was observed in nineteen of forty-seven samples. Manganese-54, niobium-95, zirconium-95, ruthenium-103, cerium-141 and cerium-144 were observed in samples from the first, second and third quarters. These may be attributed to the atmospheric nuclear weapon test by the People's Republic of China on October 16, 1980. Gross alpha analyses of quarterly composites showed positive resu of forty-seven samgles with values ranging from 0.0012 toaverage with the 0.0049 being 0.0026 pCi/m The strontium-89 analyses perfomed on the quarterly composites showed thirty-two of forty-seven samples with detectable activity. These ranged from 0.0005 to 0.0096 pCi/md . The positive strontium-89 results were primarily observed in the first, second and third quarters and can be attributed to the October 316, 1980 nuclear test. The MDLs forstrontium-89rangedbetween0.0003gnd0.0008pCi/m. Strontium-90 concentrations ranged between <0.0001 and 0.0017 pCi/m with the average being 0.0008 pCi/m3, Air Iodine (Table C-16) Of the 578 air samples analyzed for iodine-131, all were gelow the LLD. The de-tection limit for all analyses ranged from 0.003 to 0.07 pCi/m . Prccipitation(TableC-17) Eight of eighteen sanples showed positive tritium results, ranging from 127 to 267 pCi/1. All others were less than LLD (219 pCi/1). Beryllium-7, from cosmic radi-ation, was observed in seventeen samples ranging from 10 to 56 pCi/1. Zi rconium-95, 22

niobium-95, rutk.ilum-103, ruthenium-106, cesium-137, cerium-141 and cerium-144 were observed especially during the first and second quarters. This was consistent.with results observed in air particulates. The occurrence of these nuclides can be attri-buted to the atmospheric nuclear weapons test by the People's Republic of China in October 1980. Ingestion Pathway 4 Potential ingestion pathways of exposure for Susquehanna SES were evaluated by analyzing samples of milk, fish, food products, meat, game, pasture grass and soil. Milk (Tables C-18, C-19 and C-20) Cow milk samples were collected monthly from eight locations; 1282, 12B3, 6C1, 10D1,12D2, SEl,13E3 and 10G1. Samples were collected semi-monthly from April to September from stations 1282, SEl,13E3 and 10G1. Each monthly sample was analyzed for I-131, Sr-89 and -90 and gamma emitters. The additional samples were analyzed for iodine-131 and gamma emitters only. All of the 120 samples analyzed for iodine-131 were below the LLD. The LLDs ranged from 0.07 to 0.2 pCi/1. Potassium-40, as determined by gama spectrometry, was found in all milk samples with levels ranging from 1200 to 1700 pCi/1. Cesium-137 was found in 138 of 144 sam-ples with levels ranging from 1.2 to 9.6 pCi/1. Strontium-89 was detected in seventeen of ninety-six samples analyzed with results ranging between 1.3 and 5.3 pCi/1. The range of MDI. values for strontium-89 was 1.4 to 83 pCi/1. The wide range of values for the MDL was due to low chemical yields in i some of the samples and delays between sample collection and analysis which causes a large decay correction factor. The concentration of strontium-90 was positive in ! ninety-five of ninety-six samples analyzed and averaged 5.6 pCi/1. Due to the twenty-eight year half-life and biological assimilation, strontium-90 can be expected to re-main long after routine atmospheric testing has ceased. All strontium-89 and -90 analysis chemical yields have been verified by atomic absorption to determine calcium interference. Goat milk was sampled at two locations quarterly, or more frequently if sufficient milk was available. Goat milk was analyzed for iodine-131 only. Of the thirteen sam-ples analyzed, all were below the LLD. LLDs ranged from 0.1 to 1.8 pCi/1. The high LLDs observed for iodine-131 in goat milk are due to the small quantities which are available for analysis. Fish (Table C-21) Fish was collected from two locations. Three to seven fish of each species, enough to obtain one to two kilograms of filets, were collected at each location. The species

included were
walleye, white sucker and channel catfish. Analysis of the flesh for gamma emitters and strontium-89 -90 was performed on each species sampled.

Gamma spectrometry was performed on the flesh portions of fish samples. Naturally-occurring potassium-40 was detected in all twelve samples with results ranging from 3.1 to 3.7 pCi/g(wet). Cesium-137 was detected in eleven samples ranging from 0.009 to 4 23

0.016 pCi/g(wet). These results were consistent with those previously found. Since the station is not in operation, and there are no other nuclear power installations in the area, the man-made nuclide observed can probably be attributed to nuclear w::apons testing fallout. Strontium-89 was below the MDL (0.01 pCi/g(wet)) in all twelve samples. Stron-tium-90 was observed in three samples ranging from 0.002 to 0.007 pCi/g(wet). MDLs ranged from 0.003 to 0.006 pCi/g(wet). FoodProducts(TableC-22) Gamma spectrometry was used to analyze various types of food products collected from local farmers within the vicinity of Susquehanna SES. These include apples, honey, com, cabbage, cantalopes, potatoes, squash, strawberry plant and tomatoes. Naturally-occurring potassium-40 at levels of 0.72 to 10 pCi/g(wet) was found in all samples. Beryllium-7, from cosmic ray activity, was observed in the strawberry plant sample. Niobium-95 and cesium-137 were found in three samples which was not unexpected when compared with other fallout data observed in 1981. Meat (Table C-23) Meat samples consisting of eggs, chicken and duck were collected from two local farms. The flesh was analyzed for gamma emitters. Naturally-occurring potassium-40 was detected in all three samples, 0.9 to 2.9 pCi/ gram (wet). All other gamma emitters were below the LLD. Game (Table C-24) One deer sample and one squirrel sample were collected in the winter and the flesh was analyzed for gamma emitters. Naturally-occurring potassium-40 was found at levels of 2.5 and 2.7 pCi/g(wet), respectively. Cesium-137 was also found at a concentration of 0.10 and 1.5 pCi/g(wet), mspectively. These results were consistent with cesium-137 concentrations found in game samples (especially squirrels) analyzed in previous years (7). All other nuclides searched for were less than the LLD. Vegetation (Table C-25) Two leafy vegetation samples were collected on site and analyzed by gamma spectro-metry. Potassium-40 was found in both samples at concentrations of 7.9 and 8.1 pCi/g (wet). Beryllium-7, from cosmic ray activity, was found in one sample at similar levels to those found in pasture grass. Zirconium-95, niobium-95 and c' ium-144 were found in the samples and can be attributed to fallout from the atmosphce e nuclear weapons test on October 16, 1980. Pasture Grass (Table C-26) i Pasture grass was collected monthly at the closest farm. Pasture grass samples from station 7C1 and station 8D1 were collected when the goat milk was unavailable. Each sample was analyzed by gamma spectrometry. Potassium-40 was found in all twelve samples and ranged from 3.7 to 26 pCi/g(wet). Beryllium-7 was observed in seven of twelve samples with results ranging from 3.1 to 12 pCi/g(wet). The presence of beryl-lium-7 can be attributed to cosmic radiation. Niobium-95, zirconium-95, ruthenium-103, cesium-137, cerium-141 and cerium-144 were observed throughout the year and are consis-tent with levels observed in food products and vegetation. These nuclides can be 24

u t attributed to the atmospheric nuclear weapons test by the Peoples Republic of China on October 16, 1930. These nuclides are typically found in fallout from atmospheric nuclear weapons tests (4-12). Soil (Table C-27) Soil was collected at fourteen locations. A topsoil sample and a subsoil sample was collected at each location. Each sample was analyzed for gamma emitters. Naturally-occurring potassium-40 was observed in all twenty-eight samples ranging from 7.9 to 10 pCi/g(dry). Radium-226 and thorium-232, also naturally-occurring, were observed in all samples. These levels ranged from 0.49 to 2.7 pCi/g(dry) and from 0.55 to 2.9 pCi/g(dry), respectively. Niobium-95 was observed in twenty-one of twenty-eight samples with results ranging from 0.08 to 0.35 pCi/g(dry). Cesium-137 was observed in all samples and ranged from 0.17 to 2.2 pCi/g(dry). Niobium-95 and cesium-137 are typically observed in fallout from atmospheric nuclear weapons tests. The observance of niobiuar95 can be attributed to the most recent test by the Peoples Republic of China in October 1980. Direct Radiation (Table C-28) Direct radiation measurements were made on a quarterly basis. TLD packets were placed at 68 locations on and surrounding the Susquehanna SES. During 1981, 264 c uar-terly TLD packets were collected. Each packet included four dosimeters for a total of 1056 analyses. All TLD results presented in this report have been normalized to a standard month (30.4 days) to eliminate the apparent differences in data caused by variations in length of exposure period. The range of TLD results for indicator locations was 4.40 to 12.63 mrad / standard month and 4.44 to 7.16 mrad / standard month for control locations. Eleva-ted levels at locations 6S4 and 7S3 were due to on-site radiographic activity. The TLD analyses yielded an average dose equivalent rate of 6.31 mrad / standard month at all indicator locations, and an average dose equivalent rate of 5.98 mrad / standard month at all control locations. The projected annual dose from direct radiation computed from these results is 76 mrads, or 76 mrem assuming a quality factor of 1, at indicator locations, and 72 mrad or 72 mrem at the control locations. The EPA terrestrial and cosmic radiation dose rate calculated for the Wilkes-Barre area is 82 mrem / year, neglecting any neutron contribu-tion (18). This compares favorably with the average TLD measured dose rate of 75 mrem / year for all stations. This difference is not unexpected since the EPA values are gross general averages for an area and do not take into consideration specific terrestrial variations. The average dose rates for all monitoring locations since 1973 are plotted in Figure 3. The differences observed between locations or between sampling periods were similar to those found previously (4-12). 25

CONCLUSIONS I l r

CONCLUSIONS The Radiological Environmental Monitoring Program for Susquehanna SES was con-ducted during 1981 as a continuation of the program initiated in 1972. The data col-lected during 1981 further develops a baseline for comparison with future operational data. The purpose for the design and development of the Susquehanna SES REMP were:

1. To establish baseline radiological characteristics of the environs '

of Susquehanna SES for comparison with future data;

2. To assure that the media sampled and analyzed are sensitive to fluc-tuations in the radiological characteristics of the Susquehanna SES l environs; and to assure that the program will be responsive to station -

radioeffluent discharge;

3. To monitor potential critical pathways of station radioeffluent to man.

The 1981 REMP further establishes the baseline radiological characteristics for the vicinity of the Susquehanna SES. This is evident by the continuation of sampling. and analysis for the aquatic, atmospheric and terrestrial environments, as well as mon-itoring of direct radiation. The sampling and analysis of these media reflect the nor-mal background radiation found in this environment. l The media sampled by the Susquehanna REMP are sensitive to radiological fluctua-tions of the environment monitored. This is evident by the measured gradual decline in the surface water concentration of tritium, primarily due to the decrease in atmos-pheric nuclear detonations. Gross beta and gamma spectrometry analyses of air parti-culates are sensitive to atmospheric testing of nuclear weapons. Gamma analyses of surface water, sediment, air,~ food products, vegetation, pasture grass and so:1 samples showed low concentrations of radioactive nuclides from fallout from the October 16, 1980 abnospheric nuclear weapons test by the People's Republic of China. Iodine-131 was ob-served in surface water samples throughout the year. Since Susquehanna SES is not in operation, iodine-131 can be attributed to other sources of contamination of the river. These two instances indicate that the Susquehanna SES REMP is sensitive to radiological fluctuations of the environment. f Environmental ganna radiation measurements were made using thermoluminescent dosi-i meters. Results from the indicator and control locations were found not to be signi- ! ficantly different as would be expected in the absence of any source af gamma radiation. The media sampled by the Susquehanna REMP also monitors potential critical pathways of station radioeffluent to man. Monitoring of the waterborne pathway consisted of sampling surface water, well 4 water, potable water and sediment. These sample types were chosen to reflect the characteristics of normal background radiation for this medium. The airborne pathway was monitored by filtering and analyzing the particulate matter, by passing filtered air through a charcoal filter which was analyzed for the presence of iodine-131 and by analysis of precipitation. The ingestion pathway was monitored by the sampling and analysis of milk, fish, game, various food products, vegetation, pasture grass 29

and soil. The results obtained by analysis of these samples were consistent with previously measured levels of radioactivity in their respective media (4-12). The results obtained from analyses performed on the samples collected in the vicin-ity of the Susquehanna SES were expected for this environment. The levels and fluctua-tions of radioactivity detected are consistent with previously accumulated REl4P data (4-12). 30

l f l ) REFERENCES

REFERENCES (1) Pennsylvania Power and Light Conpany, "Susquehanna Steam Electric Station, Applicant's Environmental Report," Operating License Stage, May 1978. (2) Pennsylvania Power and Light Company, "Susquehanna Steam Electric Station, Final Safety Analysis Report," 1978. (3) United States Nuclear Regulatory Comission, Office of Nuclear Re-actor Regulations, " Draft Environmental Statement Related to the Operation of Susquehanna Steam Electric Station Units 1 and 2," Docket Nos. 50-387 and 59-388, June 1979. (4) Radiation Management Corporation, "Susquehanna Steam Electric Station, Radiological Environmental fionitoring Program, Report

      #1 (April - December 1972)" RMC-TR-73-14, July 1973.

(5) Radiation !!anagement Corporation, "Susquehanna Steam Electric Station, Preoperational Radiological Envimnmental lionitoring Program 1973," RMC-TR-74-07, May 1974. (6) Radiation Manaaement Corporation, "Susquehanna Steam Electric Station, Pmoperational Radiological Environmental Monitoring Program,1974 Annual Report," R!iC-TR-75-07, April 1975. (7) Radiation Managenent Corporation, "Susquehanna Steam Electric Station, Radiological Environmental Monitoring Program,1975 Annual Report," RMC-TR-76-05, May 1976. (8) Radiation Management Corporation, "Susquehanna Steam Electric Station, Radiolo3ical Environmental Monitoring Program,1976 Annual Report," RMC-TR-77-04, March 1977. (9) Radiation Managenent Corporation, "Susquehanna Steam Electric Station, Radiological Environmental Monitoring Program,1977 Annyal Report," RMC-TR-78-01, May 1978. (10) Radiation Management Corporation, "Susquehanna Steam Electric Station, Radiological Environmental Monitoring Program,1978 Annual Report," RMC-TR-79-01, April 1979. (11) Radiation Management Corporation, "Susquehanna Steam Electric Station, Radiological Environmental Monitoring Program,1979 Annual Report," RMC-TR-80-01, March 1980. (12) Radiation Management Corporation, "Susquehanna Steam Electric Station, Radiological Environmental Monitoring Program,1980 Annual Report," RMC-TR81-02, July 1981. (13) Branch Technical Position to the Nuclear Regulatory Commission Regulatory Guide 4.8, Rev.1, Novenber 1979. (14) United States Environmental Protection Agency, ORP/SID 722,

      " Environmental Radioactivity Surveillance Guide," June 1972.

i 33

l REFERENCES (cont.) (15) Radiation Management Corporation, "T1, Specifications for Analytical Instructions," August, 1978. (16) Radiation Management Corporation, " Quality Control Data - 1981 Annual Report," January,1982. (17) National Interim Primary Drinking Water Regulations, Safe Drinking Water Act, Public Law 93523, July 9,1976. (18) Oakley, Donald T. , Natural Radiation Exposum i_n_ n the United States, ORP/SID 72-1, United States Environmental Protection Agency, June 1972. 34

TABLE 1 SYrW515 0F THE SUSQUEHArctA SES RADIOLOGICAL ENY1R(NENTAL lollTORING PROGRAM 1981 SAFPLE SAffLING NLPEER OF N % ER ANALYSIS ANALYSIS ranER TYPE FREQUENCr SAPPLING COLLECTED TYPE FREQUENCY PERFORMED LOCATIONS MATERBO9PE PAT 4AV Surface Water M 8 80 Gross Beta M 30 I-131 M 57 Gama M 80 H-3 QC 28 S r-89 QC 28 S r-90 QC 28 W 7 345 I-131 W 345 Well dater M 3 36 Gross Beta M 36 Gama M 36 Gross Alpha QC 12

 /

Tritium QC 12 Fot.ble Water M 2 24 Gross Beta M 24 - Gama M 24 a Gross Alpha QC 14 Tritt um QC 14 Sr-89 QC 8 Sr 90 QC 8 W 1 52 1 131 W 52 5edtwnt SA 3 6 Gross Alpha SA 6 Gama SA 6 Sr M SA 6 S r-90 SA 6 ,

!  AIRBORNE PATHWAY

) Air Particulate W 12 605 Gross Beta W C05 } Gross Alpha QC 47 Gama QC 47 Sr-89 QC 47 Sr-90 QC 47 Air lodine W 12 578 I-131 W 578 Precipitation M 4 41 Trittum M/Q 18 Gama M/Q 18 INGESTION PATWWAY Milk M/5M 10 133 1-131 M/5M 133 Gama M/5M 120 Fish (Flesh) SA 2 12 Gansna SA 12 S r-89 5A 12 S r-90 SA 12 Food Products A 5 15 Gama A 16 Meat & Poultry (Flesh) SA 2 3 Gama SA 3 Game (Flesh) A 2 2 Gama A 2 Ve ptation M 2 2 Gama M 2 Pasture Grass M 3 12 Gama M 12 5011 A 14 28 Gama A 23 DIRfCT RADI ATION Dostmeters (TLDs) Q 68 264 Gama Dose Q 264 \ rate Total 2239 3125 35

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APPENDIX A PRE 0PERATIONAL ENVIRONTENTAL RADIOLOGICAL MONITORING PROGRAM ANNUAL

SUMMARY

_ . _ _ . _ . __ _ .._. .~ _ __ - - APPENDIX A PREOPERATIONAL EfWIR0fl1EfiTAL RADIOLOGICAL fiONITORING PROGRA!1 ANNUAL SufftARY Susquehanna SES Docket No.: 50-387 A 50-388 Berwick, Pa. January 1 to Decsiber 31, 1981 TYPE AND LOWER NLNBER OF MEDIUM OR PATHWAY TOTAL Nut 4BER L1ti!T OF ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST #4NUAL fiEAN CONTROL LOCATION NONROUTINE SAMPLED OF A'4ALYSES DETECTION fiEAN (2) NAf1E IIEAN (2) MEAN (2) REPORTED (UNIT OF MEASUREMENT) PERFOR*1ED (LLD) (1) RAf4GE DISTANCE i DIRECTION RANGE RANGE MEASUREMENTS Surface Water Gmss Beta 80 1.6 3.2 (43/44) 12G2 17 mi WSW 3.6 (12/12) 2.9 (29/36) 0 (pCi/l) (1.4-6.9) (1.7-6.9) (1.0-6.4) Gamma 80 K-40 7.8 51 (1/44) 12H1 26 mi WSW 51(1/12) - (0/36) 0 (51) (51) - Co-60 0.6 0.9 (1/44) 12G2 17 mi WSW 0.9 (1/10) - (0/36) 0 (0.9) (0.9) Nb-95 0.6 1.6 (3/44) SS8 0.8 mi E 2.9 (1/12) 2.3(2/36) 0 (1.4-1.9) (2.9) (1.6-2.9)

  $                        Ru-103                     0.G             -(0/44)                558 0.8 mi E              1.1(1/12)         1.1(1/36)         0 (1.1)             1.1)

Th-232 1.7 4.5 (1/44) 12H1 26 mi WSU 4.5 (1/12) - 0/36) 0 (4.5) (4.5) - I-131 402 0.06 0.24 (12/323) 2F2 7.2 mi NNE 0.29 (10/52) 0.27 (56/79) 0 (0.10-0.56) (0.14-0.6) (0.08-1.0) H-3 28 87 108 (10/16) 655 0.9 mi ESE 141 (2/4) 121 (7/12) 0 (68-183) (99-183) -(68-166) Sr-89 28 0.6 0.6 (2/16) 12F1 5.3 mi WSW 0.8 (1/4) 0.5 (2/12) 0 (0.4-0.8) (0.8) (0.5) Sr-90 28 0.4 0.6(7/16) 12F1 5.3 mi WSW 0.3 (2/4) 0.4 (3/12) 0 (0.3-1.1) (0.4-1,1) (0.2-0.8) i Well Water Gmss Beta 36 1.7 3.2 (18/24) 15A4 0.9 mi fM 4.1 (12/12) 1.9 (8/12) 0 i (pCi/1) (1.2-7.4) (1.5-7.4) (1.5-3.5) Gama 36 K-40 6.0 7.9(2/24) 15A4 0.9 mi TN 7.9 (2/12) -(0/12) 0 (6.3-9.5) (6.3-9.5) - Gmss Alpha 12 0.9 - (0/B) N/A - (0/4) - (0/4) 0 H-3 12 115 93 (4/8) 15A4 0.9 mi fM 125 (1/4) 119 (2/4) 0 (72-125) (125) (87-150)

APPEf401X A (cont.) PREOPERATIONAL EfNIR0!CtENTAL RADIOLOGICAL !10NITORING PROGRAli ANNUAL SUfftARY Susquehanna SES Docket No.: 50-387 & 50-388 Berwick, Pa. January I to Decerter 31, 1981 TYPE AND LOWER Nt1EER OF MEDIUM OR PATHWAY TOTAL NUMBER LittIT OF ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL MEAN CONTROL LOCATION NONROUTINE SAMPLED OF A*4ALYSES DETECTION MEAN (2) NAME HEAN (2) MEAN (2) REPORTED (UNIT OF MEASUREMENT) PERFORMED (LLD) (1) RANGE DISTANCE & DIRECTION RANGE RANGE MEASUREMENTS Potable Water Gross Beta 24 1.7 2.2(11/12) 12F3 5.2 mi WSW 2.8 (5/12) 2.8(5/12) 0 (pci/1)- (1.5-3.3) (1.2-8.5) (1.2-8,5) Gama 24 -(0/12) fvA fyA - (0/12) 0 1-131 52 0.07 0.23 (3/52) 12H2 26 mi WSW 0.23 (3/52) N/A 0 (0.14-0.3) (0.14-0.3) > Gross Alpha 14 0.5 - (0/10) N/A ft/A - (0/4) 0

  • H-3 14 102 131 f6/10) 12H2 26 mi MSW 131 (6/10) 10 1 ( 3/4) 0 N

(70-383) (70-383) (98-108) S r-89 8 0.6 - (0/4) N/A N/A - (0/4) O Sr-90 8 0.4 0.4f2/4) 12H2 26 mi WSk 0.4 (2/4) - (0/4) 0 (0.2-0.5) (0.2-0.5) - Sediment Gamma 6 (pCi/g-dry) Be-7 0.2 0.6 (1/4) 78 1.2 mi SE 0.6 (1/2) - (0/2) 0 (0.6) (0.6) - K-40 8.6 (4/4) 78 1.2 mi SE 10 ( 2/ 2) 9.7 (2/2) 0 ( 7.0-10) (10) (9.4-10) Nb-95 0.43 (4/4 7B 1.2 mi SE 0.69 (2/2 0.26 (2/2) 0 (0.14-1.1 (0.28-1.1 (0.22-0.29) Zr-95 0.07 0.31 (2/4 7B 1.2 mi SE 0.55 (1/2 0.13 (1/2) 0 (0.07-0.55) (0.55) (0.13) Ru-103 0.02 0.18 (1/4) 70 1.2 mi SE 0.18 (1/2) 0.04 (1/2) 0 (0.18) (0.18) (0.04) Cs-137 0 .10 (4/4) 7B 1.2 mi SE 0.14 (2/2) u.10 (2/2) 0 (0.06-0.14) (0.13-0.14) (0.10) Ce-141 0.04 0.11 (1/4) 78 1.2 mi SE 0.11 (1/2) - (0/2) 0 (0.11) (0.11) - Ce-144 0.1 0.4 (1/4) 7B 1.2 mi SE 0.4 (1/2) - (0/2) 0 (0.4) (0.4) - Ra-226 0.53 (4/4) 20 1.6 mi NNE 0.63 (2/2) 0.63 (2/2) 0 (0.38-0.67) (0.56-0.69) (0.56-0.69) Th-232 0.74 (4/4) 7B 1.2 mi SE 0.90 (2/2) 0.82 (2/2) 0 , (0.55-0.90) (0.90) (0.80-0.83)

                                                                                                                                                                    ?

_m _ _ _ _

APPENDIXA(cont.) PREOPERATIOf4AL EfWIRONltENTAL RADIOLOGICAL f10NITORING PROGRAll AtmuAL SulttARY Susquehanna SES Docket No.: 50-387 & 50-388 Bentick, Pa. January 1 to Decerter 31, 1981 TYPE AND LOWER MJEER OF MEDIUM OR PATHWAY TOTAL NUMBER LIMIT OF ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL MEAN CONTROL LOCATION NONRDUTINE SAMPLED OF ANALYSES DETECTION liEAN (2) NAME MEAf4(2) MEAN (2) REPORTED I (UNITOFMEASUREMENT) PERFORMED (LLD)(1) RANGE DISTANCE & DIRECTION RANGE RANGE MEASUREMENTS Sediment (cont.) Sr-89 6 0.05 0.15 (1/4) 78 1.2 mi SE 0.15 (1/2) - (0/2) 0 (pC1/g-dry) (0.15) (0.15) - Sr-90 6 0.03 0.07 (1/4) 7B 1.2 mi SE 0.07 (1/2) 0.03 (2/2) 0 (0.07) (0.07) (0.02-0.04) Air Particulates Gross Beta 605 97 (458/458) 554 0.8 mi E 107 (53/53) 94 (147/147) 0 (10~3pC1/m ) (4-384) (12-384) l8-348) Gama 47 Be-7 20 72 (34/35) 1554 0.6 mi NW 96 (3/3) 66 (12/12) O e (31-130) . (38-130) (27-110) w Mn-54 0.7 1.9 (2/35) 981 1.3 mi 5 2.1 (1/4) - (0/12) 0 (1.6-2.1) (2.1) - Nb-95 1.0 49 (26/35) 7G1 14 mi SE 67 (3/4) 52 (9/12) ) l (7.5-100) (12-9 7) ( 10-9 7) Zr-95 1.6 23(26/35) 7G1 14 mi SE 31 (3/4) 24 (9/12) L ( 3.5-47) (5.5-49) (5.5-49) Ru-103 1.0 12(17/35) 9B1 1.3 mi S 15 (2/4) 12 (6/12) 0 (9.2-15) (13-16) (9.5-17) Ru-106 6.8 24 (3/35) 252 0.9 mi NNE 27 (1/4) 22 ( 1/ 12) 0 (22-27) (27) '(22) Cs-137 0.8 3.5 (13/35) 1152 0.4 mi SW 4.5 (1/4) 3.0 (6/12) 0 (1.4-4.8) (4.5) (1.8-4.1) Ce-141 1.4 6.8(17/35) 1554 0.6 mi IM 11 (1/3) 7.5 (6/12) 0 (4.6-12) (11) (5.4-13) Ce-144 4.6 41 (25/35) 1554 0.6 mi fM 54 (2/3) 41 (8/12) 0 (15-86) (25-83) (14-78) Gross Alpha 47 0.6 2.8(34/35) SS4 0.8 mi E 3.2 (4/4) 2.2(12/12) 0 (1.4-4.9) (2.1-4.9) ( 1. 2-3. 2) S r-89 47 0.3 4.6 (23/35) 981 1.3 mi S 5.9 (3/4) 4.3 (9/12) 0 (6.5-7.0) (5.5-6.2) (0.2-9.6) Sr-90 47 0.1 0.9 (21/35) 554 0.8 mi E 1.3 (2/4) 0.6 (8/12) 0 (0.1-1.7) (0.9-1.7) (0.2-1.4) Air Iodine I-131 578 3.0 - (0/440) N/A N/A - (0/138) 0 (10-3 pC1/m3 ) ~ ' - I

                                                                                                           //

APPENDIX A (cont.) PREOPERATIONAL ENVIR0!C1 ENTAL RADIOLOGICAL MONITORING PROGRAM ANNUAL Suff4ARY Susquehanna SES Docket No.: 50-387 & 50-388 Berwick, Pa. January 1 to Decerber 31, 1981 TYPE AND LOWER NtNBER OF MEDIUM OR PATHWAY TOTAL NUMBER LIftIT OF ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL ftEAN CONTROL LOCATION NONROUTINE SAMPLED OF ANALYSES DETECTION MEAN (2) f4AME MEAN (2) MEAN (2) REPORTED (UNIT OF MEASUREMENT) PERFORMED (LLD) (1) RANGE DISTANCE & DIRECTION RANGE RANGE fEASUREMENTS ' Precipi tation H-3 18 183 213(6/14) 1152 0.4 mi SW 218(3/4) 135 (2/4) 0 (pC1/1) (181-267) (151-267) (127-142) Garria 18 Be-7 6.3 24 (13/14) 12G2 17 mi WSW 34 (4/4) 34(4/4) 0 (10-55) (21-56) (21-56) Nb-95 0.8 8.6 ( 8/14) 1152 0.4 mi SW 9.8(2/4) 6.2 (2/4) 0 (2.8-21) (8.5-11) (2.4-10) a Zr-95 1.1 7.1(6/14) 5S4 0.8 mi E 9.6 (1/5) 6.9 (2/4) O ^ (3.0-13) (9.6) (2. 7-11) Ru-103 0.7 5.8 (8/14) 102 4.0 mi N 6.3 (3/5) 5.8 (2/4) 0 (1.6-10) (1.7-10) (2.2-9.3) Ru-106 4.9 6.8 (1/14) 554 0.8 mi E 6.8 (1/5) -(0/4) 0 (6.8) (6.8) - Cs-137 0.5 1.3 (3/14) 554 0.8 mi E 1.8 (1/5) 1.0 (1/4) 0 (0.8-1.8) (1.8) (1.0) Ce-141 0.9 4.7 (5/14) SS4 0.8 mi E 5.2(2/5) 4.0 (2/4 0 (2.7-6.2) (4.2-6.2) (1.2-6.8 Ce-144 2.8 10 (5/14) 1152 0.4 mi SW 12 (1/4) 9.7 (3/4 0 (6.0-15) (12) (4.9-16) Milk I-131 133 0.07 - (0/115) N/A N/A -(0/18) 0 (pCi/1) - - Garuna 120 K-40 1441 (102/102) 6C12.7 mi ESE 1500 (12/12) 1411 (18/18) 0 (1100-1700) (1400-1600) (1300-1500) Cs-137 1.1 2.9 (96/102) 1203 2.0 mi WSW 4.6 (12/12) 3.8 (18/18) 0 (1.2-7.7) ( 2.6-7. 7) (2.4-9.6) Sr-89 96 1.4 3.4 ( 15/ 84) 12D2 3.7 mi WSW 5.3 (1/12) 3.2 (2/12) 0 ( 1. 7-5. 3) (5.3) (1.9-4.5) S r-90 96 5.3 (83/84) 1283 2.0 mi WSW 8.8(12/12) 1.'7(12/12) 0 (1.3-13) (2.2-13) (4.6-9.9)

APPENDIX A (cont.) PREOPERATIONAL ErNIRONMENTAL RADIOLOGICAL MONITORING PROGRAM ANNUAL Str1 MARY Susquehanna SES Docke t No . 387 & 50-388 Berwick, Pa. January 1 to Decenter 31, 1981 TYPE AND LOWER nth 3ER OF MEDIUM OR PATHWAY TOTAL NUMBER LIMIT OF ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL ffEAN CONTROL LOCATION NONROUTINE SAMPLED OF ANALYSES DETECTION ltEAN (2) NAME MEAN (2) MEAN (2) REPORTED (UNIT OF MEASUREMENT) PERFORMED (LLD) (1) RANGE DISTANCE & DIRECTION RANGE RANGE MEASUREMENTS Fish Gamma 12 (pC1/9-we t) K-40 3.3(6/6) 2G 30 mi NNE 3.4 (6/6) 3.4 (6/6) 0 (3.1-3.7) (3.2-3.5) ( 3. 2-3.5 ) Cs-137 0.01 0.0 12 (5/6) 2G 30 mi NNE 0.012 (5/6) 0.0 12 (5/6) 0 (0.009-0.015) (0.009-0.016) (0.009-0.016) S r-89 12 0.006 - (0/6) N/A N/A -(0/6) 0 Sr-90 12 0.003 0.002(1/6) 2G 30 mi NNE 0.005(2/6) 0.005 (2/6) 0 3 (0.002) (0.002-0.007) (0.002-0.007) Food Products Gamma 16 (pC1/g-wet) Be-7 0.03 1.6 (1/11) 12F5 8.6 mi WSW 1.6 (1/1) -(0/5) 0 (1.6) (1.6) - K-40 3.0 (11/11) 12F5 8.6 mi WSW 10 ( 1/ 1) 3.1(5/5) 0 (0.72-10) (10) ( 1.9-4. 3) Nb-95 0.004 0 .10 (1/ 11) 12F5 8.6 mi WSW 0.10 ( 1/ 1) - (0/5) 0 (0.10) (0.10) - Cs-137 0.003 0.04 (2/11) 782 1.5 mi SE 0.07 (1/2) - (0/5) 0 (0.004-0.07) (0.07) - Meat & Poultry (Flesh) Ganma 3 (pci/g-we t) K-40 2.0 (3/3) 10D13.0 mi SSW 2.9 (1/1) No Contml 0 (0.93-2.9) (2.9) Location Game (Flesh) Gar:ma 2 (pCi/g-wet) K-40 2.6 (2/2) Indicator 2.7 (1/1) No Contml 0 (2.5-2.7) (2.7) Location Cs-137 0.08 (2/2) Indicator 1.5 (1/1) 0 (0.10-1.5) (1.5) Vegetation Gamma 2 (pCi/g-wet) Be-7 1.3 1.7 (1/2) 8S3 1.0 mi SSE 1.7 (1/1) No Contml 0 (1.7) (1.7) Location K-40 8.0 (2/2) 8S31.0 mi SSE 8.1 (1/1) 0 ( 7.9-8.1) (8.1) l

APPENDIXA(cont.) PREOPERATIONAL ENVIRONTENTAL RADIOLOGICAL tiONITORING PROGRAM ANirJAL SufW 4Y Susquehanna SES Docket No.: 50-387 & 50-388 Berwick, Pa. January 1 to Decerter 31, 1981 TYPE AND LOWER NUMBER OF MEDIUM OR PATHWAY TOTAL NUMBER LIMIT OF ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL fiEAN CONTROL LOCATION NONROUTINE SAMPLED OF ANALYSES DETECTION MEAN (2) f4AIE IEAtt (2) MEAN (2) REPORTED - (UNIT OF MEASUREMENT) PERFORMED (LLD) (1) RANGE DISTANCE & DIRECTION RANGE RANGE MEASUREMENTS Vegetation (cor t.) Nb-95 0 . 39 ( 2/ 2 7S4 1.0 mi SE 0.4 (1/1) No Control 0 (pC1/9-wet) (0.31-0.4 (0.4) Location Zr-95 0.3 0.18 (1/2 8531.0 mi SSE 0.18 (1/1) 0 (0.18) (0.18) Ce-144 0.9 0.5 (1/2) 853 1.0 mi SSE 0.5 (1/1) 0 (0.5) (0.5) Pasture Grass Gama 12 (pCi/g-wet) Be-7 1.1 5.5 (7/12) 15A1 0.9 mi fM 7.1(5/9) la Control 0 ( 1.2-12) (1.8-12) Location K-40 14 (12/12) 8D1 3.2 mi SSE 26 (1/1) 0 (3.7-26) (26) Nb-95 0.04 1.4 (8/ 12) 15A1 0.9 mi fM 2.1 (5/9) 0 (0.18-8.4) (0.18-8.4) $ Z r-95 0.% 2.3 (2/12) (0.4-4.2) 15A10.9 mi fM 2.3 (2/9 (0.4-4.2 0 Ru-103 0.04 1.5(1/12) 15A10.9 mi fM 1.5 (1/9 0 (1.5) (1.5) Cs-137 0.03 0.11 (3/12) 15A1 0.9 mi fM 0.14 (2/9) 0 (0.07-0.2) (0.07-0.2) Ce-141 0.08 1.9 (1/12) 15 A10.9 mi fM 1.9 (1/9) 0 (1.9) (1.9) Ce-144 0.3 5.3(1/12) 15A10.9 mi TM 5.3(1/9) 0 (5.3) (5.3) Soil Gamma 28 (pC1/g-dry) K-40 9.2 (24/24) 12F4 8.3 mi WSW 11 (2/2) 9.1 (4/4) 0 ( 7.9-11) (10-11) (8.1-10) Nb-95 0.05 0.17 (18/24) 3D2 3.4 mi HE 0.34 (1/2) 0.24 (3/4) 0 (0.08-0.34) (0.34) (0.15-0.35) Cs-137 0.49(24/24) 7G1 14 mi SE 2.2(2/2) 1.2 (4/4) 0 (0.14-2.2) (2.2) (0.19-2.2) Ra-226 0.82 (24/24) 3D2 3.4 mi NE 2.2 (2/2) 0.84 (4/4) 0 (0.58-2.7) ( 1.6-2. 7) (0.74-0.92) Th-232 0.89(24/24) 3D2 3.4 mi NE 2.4 (2/2) 1.0 (4/4) 0 (0.55-2.9) ( 1.9-2.9) (0.9-1.1)

APPENDIX A (cont.) PREOPERATIONAL EfNIR0ffiENTAL RADIOLOGICAL MONITORING PROGRAM ANNUAL SUtNARY Susquehanna SES Docket No.- 50-387 & 50-388 Berwick, Pa. January I to Decerber 31, 1981 TYPE AtiD LOWER NtNBER OF MEDIUM OR PATHWAY TOTAL NUMBER LIMIT OF ~ALL INDICATOR LOCATIONS LOCATION WITH HIGHEST ANNUAL MEAN CONTROL LOCATION NONROUTINE SAMPLED OF N4ALYSES DETECTION MEAN (2) NNIE HEAN (2) MEAN (2) REPORTED (UNIT OF MEASURC4ENT) PERFORMED (LLD) (1) RNiGE DISTNiCE & DIRECTION RANGE RN4GE MEASUREMENTS Anbient Radiation TLD 264 6.31(232/232) 6S4 0.2 mi ESE 10.39 (4/4) 5.98 (32/32) 0

                            $                      (mrem /std. mo.)                                                                            (4.40-12.63)                                        (7.90-12.63)     (4.44-7.16)

No detectable measurements were found. (1) The LIDS quoted are the lowest actual LLD obtained in th.e various media during the reporting period. A typical gamma LLD was determined for each searched for nuclide as found in Table C-29. Where all nuclides were <LLD for a specific media, no LLD was listed. Strontium-89 and -90 are reported as Linimum detectable levels (!Ols) rather than LLDs. (2) Mean and range are based upon detectable measurements only. Fraction of detectable measurements is indicated in parentheses. The mean (i) is defined as follows: X= X I i=1 Where: X 9

                                                                                                                                                                                  =  the activity of an individual measurement (1) n n    =

number of total measurements l

I l APPENDIX B SAMPLE DESIGNATION l i

APPENDIX B Table B-1 lists the sampling locations and includes both the distance and direc-tion from the Susquehanna SES and the media sampled at each location. Maps B-1 and B-2 show the sampling locations with respect' to the Susquehanna SES. Sample Designation Samples are identified-by a Ethree part code. The first two letters are the power station identification code, in this case "SS" for Susquehanna Steam Electric Station. The next three letters are for the media sampled. AIO = Air Iodine GAD = . Game, Deer AQF = Fish GAS = Gane, Squirrel AQS = Sedinent GMK = Goat Milk APT = Air Particulates IDM = Innersion Dose (TLD) EWA = Effluent Water MLK = Milk FPB = Food Products, Beef PAS = Pasture Grass FPE = Food Products, Eggs PWT = Potable Water, Treated FPF = Food Products, Fruit RWA = Precipitation FPG = Food Products, Grain SWA = Surface Water FPH = Food Products, Hor.ey_ WWA = Well Water FPL = Food Products, Leafy Vegetables VGT = Vegetation FPP = Food Prod.: cts, Poultry S0L = Soil FPV = Food Products, Vegetables The last four symbols are a location code based on direction and distance from the site. Of these, the first two represent each of the 16 angular sectors of 22-1/2 degrees centered about the reactor site. Sector one is divided evenly by the north axis and other sectors are numbered in a clockwise direction; i.e., 2=NNE, 3=NE, 4=ENE, etc. The next digit is a letter which represents the radial distance from the station: S = Site (I) location E = 4-5 miles off-site A = 0-1 miles off-site F = 5-10 miles off-site B = 1-2 miles off-site G = 10-20 miles off-site 1 C = 2-3 miles off-site H = >20 miles off-site D = 3-4 miles off-site The last number is the station numerical designation within each sector and zone; e.g., 1, 2, 2, . . . . f

1. Site is defined as that area within PP&L's property boundary.

t 51

TABLE B-1 SUSQUEHANNA SES RADIOLOGICAL EliVIRON!iENTAL f10NITORING PROGRAli SAfiPLING LOCATIONS 1981 LOCATION SAf4PLE CODE DESCRIPTION

  • TYPES INDN 0.9-1.4 mile ESE, At or below Discharge structure AQF INDMO 0-1.0 mile N, NNE and NNW GAS IS2 0.2 mile N, Security Fence IDri 2S2 0.9 mile NNE, Energy Information Center APT,AIO,IDt1 2S3 0.2 mile NNE, Security Fence IDit 2S4 0.9 mile NNE, Energy Information Center S0L 3S3 0.5 mile NE, Recreational Area Imi 3S4 0.3 mile NE, Security Fence IDt1 4S1 1.0 mile ENE, Susquehanna River Flood Plain IDfi 4S2 0.5 mile ENE, Site - Peach Stand WWA 4S3 0.2 mile ENE, Security Fence IDit SS1 0.8 mile E, North of Biological Consultants IDM 5S4 0.8 mile E, West of Biological Consultants APT,AIO,IDM, RWA 5S5 0.8 mile E. West of Biological Consultants SOL SS7 0.2 mile E, Security Fence IDfi SS8 0.8 mile E, Area under power line SWA h 6S4 0.2 mile ESE, Security Fence IDM 6S5 0.9 mile ESE, 0utfall Area SWA 7S1 0.2 mile SE on 230 KV tower ID!!

7S3 0.2 mile SE, Security Fence IDl1 7S4 1.0 mile SE, On Site VGT 8S2 0.2 mile SSE, Security Fence IDM 8S3 1.0 mile SSE, On Site VGT 9S1 0.3 mile S, Security Fence IDM 10S1 0.4 mile SSW, Security Fence IDM 11S2 0.4 mile SW, Golorb House APT, AIO ,IDM, RWA 11S3 0.3 mile SW, Security Fence IDt1 11S4 0.4 mile SW, Golomb House SOL 12S3 0.4 mile WSW, Security Fence IDM 52 j

TABLEB-1(cont.) SUSQUEHANNA SES RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAri SAMPLIl1G LOCATIONS 1981 LOCATI0ft SAMPLE CODE DESCRIPTION

  • TYPES 13S2 0.4 mile W. Security Fence IDM 13S3 0.6 mile ':1, Si te Boundary VGT

'14S2 0.4 mile WNW, Security Fence IDti 14 S5 0.5 mile WNW, Site Boundary IM1 15S3 0.3 mile NW, Security Fence IRi 15S4 0.6 mile NW, Transmission Corridor APT,AIO,IDM, SOL 16 S 1 0.3 mile NNW, Security Fence IDt1

'1A1          0.6 mile N, Thomas Residence                                       IM1 6A3          0.6 mile ESE, State Police                                         ID!!

7Al 0.4 mile SE, Kline Residence IDl1 11A2 0.6 mile SW, Shortz Residence ID1 15A1 0.9 mile NW, Serafin Farm PAS 15A3 0.9 mile NW, Serafin Farm I 31 15A4 0.9 mile NW, Serafin Farm WWA 16A2 0.8 mile NNV, Rysinski Farm IDil 2800* 1.6 miles NNE, Gould Island AQS 283 1.3 miles NNE, Luzerne Outerware IDt1 7B000 1.2 miles SE, Bell Bend AQS 782 1.5 miles SE, Heller's Orchard FPF,FPH '7B3 1.7 miles SE, Council Cup IDM 881 1.4 miles SSE, Gale Residence Imi 9B1 1.3 miles S, Transmission Line East of Route 11 APT,AIO,IDfi 982 1.3 miles S, Transmission Line East of Route 11 SOL 10B2 2.0 miles SSW, Algatt Residence IDM 10B3 1.7 miles SSW, Car-fiar IDt1 53

TABLEB-1(cont.) SUSQUEHANNA SES RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM SAMPLING LOCATIONS 1981 LOCATION SAMPLE CODE DESCRIPTION

  • TYPES 1281 1.3 miles WSW, Kisner Farm FPE , FPF,FPG ,FPP .

12B2 1.7 miles WSW, Shultz Farm MLK 1283 2.0 miles WSW, Young Farm MLK 1284 1.7 miles WSW, Shultz Farm IDM 16B000 1.1 miles NNW GAD 16B1 1.6 miles NNW, Walton Power Line IDM 6C1 2.7 miles ESE, Moyer Farm MLK 7C1 2.7 miles SE, Ferry Farm GMK, PAS 11C000 2.6 miles SW, Hess Island AQS 102 4.0 miles N, Near Mocanaqua Substation APT.AIO,IDM RWA 1D3 3.9 miles N, Near Mocanaqua Substation SWA 1D4 3.9 miles N, Near Mocanaqua Substation SOL IDS 3.9 miles N, Shickshinny Sewage Treatment Facility EWA 3D1 3.4 miles NE, Pond Hill APT,AIO,IDM 3D2 3.4 miles NE, Pond Hill S0L 801 3.2 miles SSE, Poltrock Farm GMK, PAS 8D2 4.0 miles SSE, Mowry Residence IDM 9D1 3.6 miles S, Smith Farm IDM 1001 3.0 miles SSW, Ross Ryman Farm MLK,FPP 10D2 3.0 miles SSW, Ross Ryman Farm IDM 1101 3.3 miles SW, Zehner Farm FPG FPL,FPV 11D3 3.3 miles SW, Zehner Farm S0L 11D4 3.5 miles SW, Lanning Farm S0L 12D2 3.7 miles WSW, Dogastin Fann ILK 12D3 3.7 miles WSW, Dogastin Residence IDM 1El 4.5 miles N. Lane Residence IDM 4E1 4.8 miles ENE, Pole #46422 N35-197 IDM SE1 4.5 miles E. Bloss Farm MLK SE2 4.5 miles E, Bloss Farm IDM 54

TABLEB-1(cont.) SUSQUEHANNA SES RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM SAMPLING LOCATIONS 1981 LOCATIQ1 SAMPLE CODE DESCRIPTION

  • TYPES 6El 4.7 miles ESE, St. James Church IDM-7El 4.2 miles SE, Harwood Trans. Line Pole #2 IDM 11El 4.7 miles SW, Jacobsen Residence IDM 12E1 4.7 miles WSW, Berwick Hospital APT,AIO,IDM 12E2 4.7 miles WSW, Berwick Hospital S0L 13E1 4.5 miles W, Glen Brook Reservoir SWA 13E3- 5.0 miles W, Dent Farm MLK 13E4 4.1 miles W, Kessler Farm IDM 14E1 4.1 miles WNW, Knouse Farm IDM 2F1 5.9 miles NNE,'St. Adalberts Cemetery IDM 2F2 7.2 miles NNE, Retreat Bridge SWA 3F1 9.1 miles NE, Valania Residence IDM 7F1- 9.0 miles SE, Conyngham School IDM 12F1 5.3 miles WSW, Berwick Bridge SWA 12F2 5.2 miles WSW, Berwick Substation IDM 12F3 5.2 miles WSW, Berwick Water Co. WWA,PWT 12F4 8.3 miles WSW, Lupini Farm SOL 12F5 8.6 miles WSW, Seescholtz Farm FPV, SOL 15F1 5.4 miles NW, Zawatski Fanm IDM 16F1 7.8 miles NNW, Hidlay Residence IDM 3G1 15 miles NE, Lower Bridge Plymouth SWA 3G2 11 miles NE, Nanticoke Bridge SWA 3G3 16 miles NE, WB Horton St. Substation IDM 3G4 17 miles NE WB Service Center IDM 3G5 19 miles NE, Market St. Bridge SWA 4G1 14 miles ENE, Mountain Top - Ind. Park IDM 7G1 14 miles SE, Hazelton Chem Lab APT,AIO,IDM, SOL 10G1 14 miles SSW, Davis Farm MLK 55
                                                    - - _ - -                                   J

TABLEB-1(cont.) SUSQUEHAliNA SES RADIOLOGICAL EllVIRONMEllTAL M0f11TORING PROGRAM SAf1PLIllG LOCATIONS 1981 LOCATI0ft SAMPLE CODE- DESCRIPTI0fl* TYPES 12G1 15 miles WSW, Bloomsburg, PA ' APT,AIO,IDM.RWAL 12G2 17 miles WSW, between Bloomsburg and Berwick, PA SWA, RWA ! 12G3 15 miles WSW, Bloomsburg State College S OL -. 12G4 10 miles WSW,. Kinery Residence IDM 2H000 30 miles Ni1E, flear Falls, PA AQF 2H1 21 miles fille, Yalick's Produce flear Dallas FPL,FPG,FPV

,   7H1              47 miles SE, PP&L roof, Allentown                                     APT,AIO,IDM 8H1-             92 miles SSE, RMC roof, Philadelphia                                  IDM 12H1             26 miles WSW, Merck Co.                                               SWA 12H2             26 miles WSW, Danville Water Company                                  PWT o       ' All distances measured from vent.
    *O       fio actual location is indicated since fish are sampled over an area which extends through 3 sectors (5, 6 and 7) near the outfall area.

C*o- Station code is omitted because no permanent locations exist; samples are taken based on availability. i l' P i i 56

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l APPENDIX C DATA TABLES

APPENDIX C DATA TABLES TABLE PAGE NO. TABLE TITLE Waterborne Pathway C-1 Concentrations of Beta Emitters in Surface Water Samples in - the vicinity of Susquehanna SES ----------------------------- 64 C-2 Concentrations of Gamma Emitters in Surface Water Samples i n the vi ci ni ty of Susquehanna SES -------------------------- 65 C-3 Concentrations of Iodine-131 in Surface Water and Effluent Water Samples in the vicinity of Susquehanna SES ------------ 66 C-4 Concentrations of Tritium and Strontium-89 and -90 in Quar-terly Composite Samples of Surface Water in the vicinity of Susquehanna SES --------------------------------------------- 70 C-5 Concentrations of Beta Emitters in Well Water Samples in the vicinity of Susquehanna SES --------------------------------- 71 C-6 Concentrations of Gamma Emitters in Well Water Samples in the vicinity of Susquehanna SES ----------------------------- 72 C-7 Concentrations of Alpha Emitters and Tritium in Quarterly Composite Samples of Well Water in the vicinity of Susque-hanna SES --------------------------------------------------- 73 . C-8 Concentrations of Beta Emitters and Gamma Emitters in Potable (Drinking) Water Samples in the vicinity of Susquehanna SES - 74 l C-9 Concentrations of Iodine-131 in Potable (Drinking) Water Samples in the vicinity of Susquehanna SES ------------------ 75 C-10 Concentrations of Alpha Emitters, Tritium and Strontium-89 and -90 in Quarterly Composite Samples of Potable (Drinking) Water in the vicini ty of Susquehanna SES -------------------- 76 C Concentrations of Gamma Emitters in Sediment. Samples from the Susquehanna River in the vicinity of Susquehanna SES ---- 77 C-12 Concentrations of Alpha Emitters and Strontium-89 and -90 in Sediment Samples from the Susquehanna River in the vici-n i ty o f Su sque h ann a SES ------------------------------------- 78 Airborne Pathway l l C-13 Concentrations of Beta Emitters in Air Particulate Samples in l th e vi ci ni ty of Susquehanna SES ----------------------------- 79 l- 61

APPENDIX C (cont.) DATA TABLES TABLE PAGE N0. TABLE TITLE . Airborne Pathway (cont.) C-14 Concentrations of Gama Emitters in Quarterly Composites of Air Particulate Samples in the vicinity of Susquehanna SES --- 83

, C-15  Concentrations of Alpha Emitters, Stmntium-89 and -90 in Quarterly Composites of Air Particulate Samples in the vici-ni ty o f Su sq ueh an na SES --------------------------------------      89 C-16  Concentrations of Iodine-131 in Filtered Air in the vicinity o f S u s q ueh a n n a S ES -------------------------------------------  90 C-17  Concentrations of Tritium and Gamma Emitters in Precipitation Samples in the vi ci ni ty of Susquehanna SES -------------------         93 Ingestion Pathway C-18  Concentrations of Iodine-131 in Milk in the vicinity of Sus-quehanna SES -------------------------------------------------            95 C-19  Concentrations of Gamma Emitters in Milk in the vicinity of Susquehanna SES ----------------------------------------------           96 C-20  Concentrations of Strontium-89 and -90 in Milk in the vicinity of Susquehanna SES -------------------------------------------           98 C-21  Concentrations of Gama Emitters and Strontium-89 and -90 in Fish Flesh in the vicinity of Susquehanna SES ----------------            100 C-22  Concentrations of Gama Emitters in Various Food Products in the vicinity of Susquehanna SES ------------------------------            101 C-23  Concentrations of Gama Emitters in Meat Samples in the vici-nity of Susquehanna SES --------------------------------------            102 C-24  Concentrations of Gamma Emitters in Game Samples in the vici-ni ty o f Sus q ue h anna SES --------------------------------------      103 C-25  Concentrations of Gamma Emitters in Ve9etation in the vicinity of Susquehanna SES -------------------------------------------            104 C-26  Concentrations of Gama Emitters in Pasture Grass in the vici-t        nity of-Susquehanna SES --------------------------------------            105 C-27  Concentrations of Gama Emitters in Soil Samples in the vici-ni ty o f Su s q ue h an n a SES --------------------------------------  106 62

APPENDIX C (cont.) DATA TABLES TABLE PAGE N0. TABLE TITLE Direct Radiation

     . C-28   Results of Quarterly TLD lieasurements.in the vicinity of Susquehanna SES ----------------------------------------------  107 l              Typi cal LLDs for Gama Spectrometry --------------------------  110 C-29

( t 1 l I ? I f 63

j -TABLE C-l'

                                                                            . CONCENTRATIONS OF BETA EMITTERS IN SURFACE WATER SAffLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/1        2 sigma STATION NO.                      JANUARY                     FEBRUARY            MARCH                 APRIL                  t1AY             JUNE s
 ,.                 SS-SWA-558                       1.51.2                      6.411.4            2.3 1.2              2.1 1,7                2.911.2            <2.2 SS-SWA-6S5                       1.4 1.2                     5.811.4            2.021.2              2.41.2                 3.811.2           2.lil.5 SS-SWA-1D3                       1.711.3                     5.511.4            5.111.4              3.911.4                2.4 1.3           2.711.2 SS-SWA-13E1                       <2.0                       2.021.2            1.511.2              3.1 1.4                 <1.8              <1.6 SS-SWA-12F1                         (1)                         (1)             2.911.2              3.9 1.4                1.91.2            3.311.2 SS-SWA-12G2                         (1)                         (1)             3.1*1.3              6.9 11.6               1.7 1.2           3.5 1.2-SS-SWA-12H1                      1.421.2                    '4.211.3            3.311.4              3.911.4                2.011.1           3.111.1
!                   Monthly Average                  1.6 0.5                     4.813.5            2.9 2.3              3.7t3.2                2.4 1.5-          2.2 2.3 STATION-NO.                       JULY                        AUGUST           SEPTEfEER           OCTOBER                 NOVEfEER          DECEfEER     YEARLY AVERAGE SS-SWA-SS8                       3.811.6                     3.311.4            2.921.1              2.5 1.1                3.9 1.3           2.511.1     3.0 2.5 SS-SWA-655                       3.811.6                     2.011.3            3.1*1.1              2.911.1                5.011.3           3.011.1     3.1 2.6 SS-SWA-103                       3.311.1                     3.121.3            4.3 1.3             '1.911.3                2.311.6           2.811.4     3.312.4 SS-SWA-13E1                      1.0t0.9                     1.8 1.2            1.711.1                <1.9                  <2.4              <2.0       1.811.1 SS-SWA-12F1                      2.8 1.1                     3.121.3            4.111.2              2.8 1.3                3.211.6            <2.0-      3.011.4 SS-SWA-12G2                      3.3 1.1                     6.0*1.5            3.721.2              3.2 1.3                2.311.6           1.9 1.3     3.6t3.4 SS-SWA-12H1                      5.311.4                     2.7i1.1            3.51.4               2.711.6                2.011.4           3.511.3     3.212.5

! Monthly Average 3.312.6 3.li2.8 3.3 1.8 2.61.0 3.0i2.2 2.5 1.2. l Grand ~

Average 3.012.4.

i (1) No sample was received because the river was frozen.

TABLE C-2 CONCENTRATI0!is 0F Gaff tA E!!!TTERS* IN SURFACE WATER SA!!PLES IN THE VICINITY OF SUSQUEllANNA SES Results in Units of pC1/1 2 si ma 9 STATION NO. JANUARY FEBRUARY 11 ARCH APRIL 11AY JUNE RADI0 ACTIVITY SS-S'/A-SS8 tb-95 <0.9 2.9d).6 <0.8 <1.2 <2.9 <1.3 Ru-103 (0.9 1.110.6 <0.8 <1.1 <2.8 <1.2 Others <LLD (LLD <LLD <LLD <LLD <LLD SS-SWA-655 tb-95 <0.9 1.4 0.8 <1.2 <0.8 <1.7 <1.3 Others <LLD <LLD <tLD (LLD (LLD <LLD SS-SWA-ID3 tb-95 <0.8 1.6 0.7 <1.0 <0.9 <0.7 <0.8 Others <LLD (LLD <LLD <LLD <LL D <lLD SS-SWA-13E1 All(LLD All(LLD All<LLD All<LLD All<LLD A11 <LLD SS-SWA-12F1 tb-95 (1) (1) <0.9 <1.2 <0.7 1.60.8 Others <LLD <LLD <LLD <LLD SS-SWA-12G2 Co-60 (1) (1) <0.7 0.9 0.6 <0.9 <0.6 tb-95 <0.8 1.9 0.8 <1.1 <0.8 Others <LLD <LLD <LLD <LLD SS-SWA-12H1 K-40 <9.2 <9.7 <10 <16 <9.9 51 8 Th-232 <1.8 <2.0 <2.1 <3.1 <2.1 4.511.9 Others (LLD <LLD <LLD <LLD <LLD <LLD STATION NO. JULY AUGUST SEPTD1BER OCTOBER NOVEf1BER DECE!EER RADI0 ACTIVITY SS-SWA-558 tb-95 <0.7 <0.9 <0.6 <1.0 <0.8 <0.6 Ru-103 <0.7 <0.8 <0.6 <1.0 <0.9 <0.7 Others (LLD (LLD <LLD <LLD <LLD (LLD SS-SWA-655 tb-95 <1.1 <1.8 <0.7 <1.0 <0.9 <0.7 Others <LLD <LLD <LLD <LLD <LLD <LLD SS-SWA-103 tb-95 <0.8 <1.0 <1.3 (0.7 <1.0 <1.2 Others <LLD <LLD <LLD <LLD <LLD <LLD SS-SWA-13E1 All(LLD All(LLD All<LLD All<LLD All<LLD All<LLD SS-SWA-12F1 tb-95 <1.1 (0.7 <0.9 <0.9 <0.7 <0.9 Others (LLD <LLD <LLD (LLD <LLD (LLD SS-SWA-12G2 Co-60 <0.9 <0.8 <1.1 <0.6 <1.1 <1.0 tb-95 <1.2 <0.7 <1.9 <0.7 <0.7 <0.9 Others <LLD <LLD <LLD (LLD <LLD <LL D SS-SWA-12H1 K-40 < 10 <14 <10 <14 <0.8 <9.5 Th-232 <2.2 <2.9 <2.0 <2.8 <1.7 <2.0 Others <LLD <LLD <LLD (LLD <LLD <LLD

  • All other jama erdtters searthed for wem (LLD; typical LLDs am found on Table C-29.

(1) No sarple was mceived because the river was frozen. 65

44 5 6 4 00 0 0 0 8 9 9 8 9 8 E )100 0 1110 0 0100 0100 N 1 1 U (022 0 0009 0 0006 0001 J <11 < <<<1 < <<<2 < <(1 00 0 0 0 5 5 0 0 89 7 9 9 Y 1 A 1 0 0.)1 0 1 1.)1 0 0101 1 0111

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TABLE C-3 (cont.) C0!1CErlTRATI0fis OF 100IllE-131 Ill SURFACE WATER AfD EFFLUEl4T WATER SNtPLES Ill THE VICIf11TY OF SUSQUEHAtitiA SES Results in Units cf pCi/l ! 2 sigma STATION NO. JN1UARY FEBRUARY I4 ARCH APRIL  !!AY JU14E SS-SWA-3G1 <0.1 <0.1 <0.09 <0.1 <0.09 <0.1

                                                                                  <0.1              0.14 0.06                   <0.07             <0.1               <0.1      <0.1
                                                                                  <0 . 3               <0.1                     <0.08             <0.07              <0.08     <0.03
                                                                                  <0.1                 <0.07                    <0.09             <0.08               <0.1      (1)
                                                                                                                                <0.1 m SS-SWA-3G2                                                                      (3)                   (3)                    <0.08             <0.1               <0.03     <0.09 m                                                                                 (3)                 <0.1                     <0.09             <0.1               <0.1      <0.09 (3)                 <0.1                     <0.08             <0.07              <0.09     <0.08 0.14 0.06               <0.07                    <0.09             <0.07              <0.1       (1)
                                                                                                                                <0.1 SS-SWA-3G5                                                                     <0.1                 <0.1                    <0.07              <0.1               <0.08     <0.1.
                                                                                  <0.1                   (3)                   <0.09              <0.1               <0.1      <0.1
                                                                                  <0.3                 <0.09                   <0.07              <0.07              <0.09     <0.08
                                                                                  <0.09                <0.09                   <0.09              <0.09                (1)   0.19 0.06
                                                                                                                               <0.1 SS-SWA-12G2                                                                     (3)                   (3)                   <0.09              <0.1             0.10 0.05   <0.09 SS-SWA-12H1                                                                    <0.1                 (0.09                   <0.1               <0.08              <0.09     <0.1 SS-EWA-105                                                                     <0.1                 '0.1                    <0.1               <0.2               <0.09     <0.1

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H M M M M t/1 M eA N M M M M M M M M ww 69

TABLE C-4 CONCEMTRATIONS OF TRITItit* AND STRONTItt!-39** AND -90 IN QUARTERLY C0f1POSITE SM1PLES OF SURFACE WATER IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/l 2 signa JAN APRIL JULY OCT STATION NO. TO TO TO TO RADI0 ACTIVITY f1AR JUNE SEPT DEC SS-SWA-553 H-3 <96 127.59 166 74 129i75 S r-89 <2.4 <0.7 (0.6 <0.7 S r-90 0.8 0.6 0.220.2 <0.4 <0.5 SS-SWA-655 H-3 <96 99 59 183 74 <122 S r-89 <2.6 <0.7 <0.7 <0.8 S r-90 1.0 0.6 0.3*0.3 0. 3 +0. 3 <0.5 SS-SWA-1D3 H-3 99270 (87 68265 <112 Sr-89 0.5 *0.4 <1.1 <0.7 <0.7 S r-90 <0.4 <0.6 <0.4 <0.4 N SS-SWA-13E1 O H-3 96 70 <37 <105 160272 Sr-89 0.5 0.4 <1.2 <0.7 <0.7 Sr-90 <0.4 (0.6 <0.5 0.30.2 SS-SWA-12F1 H-3 <113(1) 113:54 68 65 99169 Sr-89 0.8 0.4 (1) <1.9 <0.7 <0.7 Sr-90 (0.4 (1) <0.9 1.120. 3 0.4 0.2 SS-SWA-12ra H-3 140271 (1) 106:54 78 66 100i69 Sr-89 0.4+0.4 (1) <1.5 <0.3 <0.7 S r-90 <0.4(1) <0.7 <0,5 0 .310 .2 SS-SWA-12H1 H-3 95 64 <103 <119 <111 Sr-89 <2.7 <0.7 <0.7 <1.0 Sr-90 <1.1 <0.4 0.5 0.3 <0.6 Tritium Avera9e 105 33 104 29 112 93 119 42 j

  • Positive tritium results are reported when the 2 sigma countin9 error is less than the resul ts. In sone cases, positive nesults to be reported are lower than the calculated LLDs. For clarification, check the rethod of calculation found in Apperdix D. Analysis of Sarples for Tritium.
   **     Sr-39 results are decay corrected to sarple stop date.

(1) Analysis of l1 arch sarple only since no sarple was collected in January or February due to freezing conditions.

TABLE C-5 CONCENTRATIONS OF BETA DtITTERS IN WELL WATER SAftPLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/l 2 sigma STATION NO. JANUARY FEBRUARY MARCH APRIL ltAY JUNE SS-WWA-452 <2.0 1.2 1.2 1.3tl.2 1.4;1.3 <1.9 <1.7 SS-WWA-15A4 1.7 1.3 4.61.4 4.021.3 4.01.4 5.4 1.4 3.7 1.3 SS-WWA-12F3 <2.1 1.6 1.2 1.6 1.2 1.5t1.3 3.51.4 <1.7 Monthly Average 1.90.4 2.5t3.7 2.3 3.0 2.313.0 3.6 3.5 2.4 2.3 STATION N0. JULY AUGUST SEPTDiBER OCTOBER N0VDiBEP DECUtBER YEARLY AVEPAGE SS-WWA-452 2.411.0 1.7 1.2 1.21.0 <1.9 <2.4 <2.0 1.80.8 SS-WWA-15A4 5.311.2 2.9 1.3 3.811.2 4.51.4 7.4 1.8 1.511.3 4.1 3.2 SS-WWA-12F3 1.61.0 2.211.3 1.611.1 1.911.3 <2.4 <2.1 2.011.1 Monthly Average 3.1 3.9 2.3 1.2 2.2 2.8 2.8 3.0 4.li5.8 1.90.6 Grand Average 2.6 2.9

TABLE C-6 COI1CEf1TRATI0ils 0F GA!!!A E!!ITTERS* I!1 WELL WATER SA!!PLES Ill THE VICIf1ITY OF SUSQUEHAllilA SES Results ia Units of pCi/l 2 signa STATI0t1 fl0. JAllUARY FEBRUARY ttARCh APRIL ltAY JUI1E SS-WWA-4S2 K-40 <3.7 <3.5 <9.0 <3.3 <11 <14 Othe rs <LLD <LLD <LLD <LLD <LLD <LLD SS-WWA-15 A4 K-40 9.5 5.3 <6.0 <3.9 <12 <9.5 <16 Others <LLD <LLD <LLD <LLD <LLD <LLD SS-WWA-12F3 K-40 <3.2 <9.0 <10 <14 <14 <15 Others <LLD <LLD <LLD <LLD <LLD <LLD STATI0f1 fl0. JULY AUGUST SEPTE!1BER OC.^7ER 110VEllBER DECE!!BER SS-WWA-452 K-40 <14 <16 <16 <16 <15 <9.1 Others <LLD <LLD <LLD <LLD <LLD <LLD SS-WWA-15 A4 K-40 <15 <10 <15 6.3 5.2 <11 <11 Others <LLD <LLD <LLD <LLD <LLD <LLD SS-WWA-12F3 K-40 <3.4 <9.2 <15 <9.2 <3.6 <3.5 Others <LLD (LLD <LLD <LLD <LLD <LLD

  • All other gamma emitters searched for were <LLD; typical LLDs are found on Table C-29.

t i l ' TABLE C-7 CONCENTRATIONS OF ALPliA E!!ITTERS AND TRITIUf1* If! OUAP,TERLY C0llPOSITE SAMPLES l ! 0F WELL WATER IN THE VICINITY OF SUSQUEHANNA SES  : ! Results in Units of pCi/l 2 sigma . STATION N0. JAN APR JUL OCT YEARLY l RADI0 ACTIVITY TO TO TO TO AVERAGE [

MAR JUN SEPT DEC >

t l SS-WWA-4S2

!        Alpha                                <1.7                       <1.8                    <2.3                        <1.6                        -

i Tritium 72 71 <118 73 65 102 69 91 45 0 SS-WWA-15 A4 Alpha <1.0 <1.0 <1.3 <0.9 - Tri tium 125 73 <118 <122 <115 -

                                                                                                                                                                            ?

I SS-WWA-12F3 I

,        Alpha                               <1.9                        <1.9                    <2.6                        <1.6                       -                   !

l Tritium 87 69 <118 <122 150 72 119 52 [ t I

  • Positive tritium results are reported when the 2 sigma counting error is less than the results. [

In some cases, positive results to be reported are lower than the calculated LLDs. For clari- l fication, check the method of calculation found in Appendix D,11nalysis of Samples for Tritium. i 4 l 4 i I

TABLE C-8 C0fiCENTRATIONS OF BETA DtITTERS AND GA!!!A EtITTERS* Il4 POTABLE (DRINKING) WATER SA!!PLES IN THE VICI!1ITY OF SUSQUEHAfiNA SES Results in Units of PCi/l 2 signa STATION NO. JANUARY FEBRUARY  !! ARCH APRIL  !!AY JUNE RADI0 ACTIVITY SS-PWT-12F3 Beta <2.1 <1.8 1.3 L 8.5tl.7 <1.8 <1.7 GarTaa Emitters All <LLD Al! <LL D All(LLD All<LLD All<LLD All <LLD SS-PWT-12H2 Beta 2.1 1.2 2.0 1.2 2.0 1.3 2.211.3 1.5 1.1 2.4 1.0 Gamma Emitters All <LLD All<LLD All<LLD All<LLD ,11 <LLD All<LLD N STATION N0. JULY AUGUST SEPTEfEER OCTOBER f0VE!!BER DECE!EER YEARLY RADI0 ACTIVITY AVERAGE S3-PWT-12F3 Beta 1.41.0 1.61.2 1.2 1.0 <1.9 <2.4 <2.0 2.324.0 Gamma Emi cers All<LLD All<LLD All <LLD All<LLD All(LLD All(LLD SS-PWT-12H2 Beta 3.3 1.3 2.3!1.1 2.0 1.3 <2.4 1.3 1.3 2.4 1.3 2.2 0.9 Gamma Emitters All <LLD All <LLD All<LLD All <LLD All<LLD All<LLD Beta Grand Average 2.322.3

  • Typical LLDs are found on Table C-29.

TABLE C-9 CONCENTRATIONS OF IODINE-131 If( P0 TABLE (DRINKING) tJATER SA!!PLES Il1 THE VICIfilTY OF SUSQUEHANilA SES SS-PWT-12il2 Results in Units of pCi/l 2 sib.na JANUARY FEBRUARY 11 ARCH APRIL  !!AY JUllE

       <0.1       (0.1              <0.09                  <0.1                   <0.1       <0.1
       <0.1       <0.1              <0.07                  <0.1                   <0.1       <0.1 di    0.3 0.2      <0.07             <0.1                   <0.08                  <0.1       <0.09 0.24 0.06       <0.09             <0.1                   <0.08                  <0.1       <0.1
       <0.1                                                                       <0 .1 JULY         AUGUST          SEPTE!1BER              OCTOBER               fl0VE!!BER DECEftBER
       <0.1       <0.09             <0.09                  <0.09                  <0.1       <0.1
       <0.09      <0.1              <0.08                  <0.09               0.14 0.06     <0.1
       <0.1       <0.1              <0.1                   <0.1                   <0.1       <0.09
       <0.1       <0.1              <0.08                  <0.1                   <0.09      <0.1
       <0.08                                               <0.1

TABLE C-10 CONCENTRATIONS OF ALPHA E!!ITTERS, TRITIlft AND STRONTIint-89* AND -90 IN QUARTERLY C0!!POSITE SA!!PLES OF P0 TABLE (DRI!1XING) WATER IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/l 2 sigra JAN APRIL JULY OCT STATION NO. TO TO TO TO RADI0 ACTIVITY  !!AR JUNE SEPT DEC SS-PWT-12F3 Alpha <1.9 <1.9 <2.4 <1.6 H-3 98 70 98 54 <122 103 69 Sr-89 <0.6 <1.7 <0.9 <0.7 S r-90 <0.4 <0.3 <0.5 <0.4 SS-PWT-12H2 Bf Alpha <0.5 (1) (1) (1) H-3 31 64 (1) (1) (1) S r-89 <1.5 <0.7 <0.7 <0.9 S r-90 <0.6 <0.4 0.2 0.2 0.5 0.4 APRIL MAY JUNE JULY AUGUST SEPTE!!BER OCTOBER NOVE!!BER DECE!13ER SS-PWT-12H2 Alpha <1.1 <1.4 <1.5 <2.3 <2.3 <1.3 <0.9 <1.2 <0.9 H-3 80 58 70154 <103 3G3 65 <122 <119 <102 97 71 77 63

  • Sr-89 results are decay corrected to sample stop date.

(1) Changed from quarterly analysis to monthly analysis in April 1981.

6 E 3 4 7 0 2 3 YG LA 2 0 0 0 0 0 RR - - 1 - - AE 0 2 4 0 6 8 EV 1 YA 9 0 0 0 0 0 y t i l i b 1 a 4 2 5 0 l 8 7 0 0 0 0 i

                       -         7        4        6                     a 5   3   0   0   0    0    0   0    2    0  0       v
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                 * -     0   0   0   4    0    8   0     0   0  1 C0       <        <  1     <   0    < <      5  6        n 11           7                                          o 1                    0         0             0  0
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s es iA t r 0H l et IE u wca TU s AQ e rx RS R 1 5 2 7 9 oe TU 3 9 0 0 0 0 f NS - 3 5 3 o E 3 4 0 0 0 0 0 0 2 0 0 dn _ CE 0 _ !iH * - e 0 4 0 2 0 0 0 0 9 0 he 0T

  • 0 < < 2 < 1 < < 6 3 cs C 1 81 9 ru l 2 0 0 0 0 aa O - ec R 5 se F 0 b A1 4 3 2 2 6 3 s

- S - 3 0 0 0 0 0 0 rd ee 5 - S3 3 1 0 0 0 0 0 2 0 0 tt 1 tt

                       - 0   0   3   9    4    0   0    0    6  3  ii 5   <   1   1   2    0    1   < <       5  3   mm 0   0    0    0 eo 0  0 as mi ae gd rco e

hn to oi t l a O lt N AS 3 7 1 4 6 2 NE 5 5 0 3 4 4 2 3 OT 7 0 9 9 1 1 1 1 2 2 IA - 4 - - - - - - - - TD e - r b u s e e a h

  • A B K Z N R C C C R T **

T S

TABLE C-12 C0!1CEllTRAT10!is 0F ALPHA EftITTERS AND Sr-39* AND Sr-90 Ill SEDIttEllT SAftPLES FROM THE SUSQUEHAf!NA RIVER 114 THE VICINITY OF SUSQUEHA!UA SES Results in Units of pCi/g(dry) 2 signa STATION NO. SS-AQS-28** SS-AQS-7B** SS-AQS-11C** YEARLY DATE 5-13-31 10-05-31 5-13-31 10-05-31 5-13-31 10-05-31 AVERAGE "o c Al pha <5.3 14t6 3.4 5.3 7.1 4.4 5.6t4.3 5.2 3.9 7.716.6 Sr-39 <0.1 <0.06 0.15 0.09 <0.06 <0.1 <0.05 - Sr-93 0.04 0.04 0.02 0.02 <0.07 0.07 0.02 <0.05 <0.03 0.05 0.04

  • Sr-39 results are decay corrected to the sanple stop date.
    **      Station code is omitted because no exact sanpling locations exist; sanples are taken based on availability.

TABLE C-13 CONCENTRATIONS OF 8 ETA E!!ITTERS IN AIR PARTICULATE SA!1PLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pCi/m3 2 si n SATLE SAMPLE SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT START DATE STOP DATE 252 554 SOSt} 1152 1554 981 ID2 3D1 12E1 AERAGE 12-29-80 1-03-81 79 3 G413 3423 77 3 - 00!3 7227 3213 8423 8028 1-03-81 1-11-81 47 6 120:13 43t5 4315 - 44 5 42 4 7127 (1) 59257 1-11-81 1-18-81 45 6 95211 35 9 99210 - 7427 73 3 7723 70 7 77234 1-18-81 1-25-81 151215 116212 132 13 104 10 - 121212 115t11 111111 103210 119132 1-25-81 2-01-81 9 5 !10 113 11 97 10 97 10 - 8529 86t9 109111 93 9 97220 2-01-81 2-08-81 100 10 99t10 116t12 97210 - 83 9 9129 105210 94 9 99218 2-08-81 2- 15-81 130113 98 10 99 10 114211 - 92 9 89 9 9019 77 3 99233 2-15-81 2-22-81 113211 121212 107 11 117 12 - Ila 11 112 11 129 13 120212 117213 g 2-22-81 3-01-81 85 9 126113 124212 35 9 - 8629 102 10 90 9 8213 93236 3-01-81 3-08-81 99 10 119212 103t10 106 11 - 98 10 90 9 101t10 94t9 101117 3-08-81 3-15-81 126 13 112211 120 12 129t13 - 123212 120212 103111 124112 120 114 3-15-81 3-22-31 146 15 281123 149r15 195119 - 154115 143214 130 13 151 15 169 t93 3-22-91 3-29-81 277228 230 23 217t22 235 23 - 226 23 221122 236124 250125 237 39 3-29-81 4-04-81 334 33 Mit34 325t33 343234 - 352 35 334t33 332233 346235 333217 4-04-81 4-12-81 292229 285229 279123 269227 - 286 29 265 27 268 27 272 27 277220 4-12-81 4 3 1 169217 219122 199 20 220222 - 203t21 222 22 192 19 199220 204136 4-19-81 4-26-81 158216 221 22 200 20 204 20 - 194 19 199!20 181213 180113 192138 4-26-81 5-03-81 191 19 225222 210221 207121 - 223 22 233i23 220 22 230 23 217228 5-03-81 5 81 224222 253225 245124 232123 241 24 (2) 233!2A 225 23 103210 259126 224294 5 81 5-17-81 191219 194t19 195219 181218 177218 133219 170 17 169 17 192219 184t20 5-17-81 5-25-31 372 37 334 33 357 36 373137 364236 376233 372237 352 35 M4234 366t26 5-25-81 5-31-31 246225 234223 235 23 229 23 231!23 233 23 232 23 214121 211 21 229222 5-31-31 6-07-31 141214 145 14 140 14 147 15 154 15 141t14 184 14 129213 129113 141216 6-07-81 6-14-31 162 16 148t15 150 15 146215 153215 143214 148215 144 14 162216 151214 6-14-81 6-21-31 87 9 34 3 37 9 3223 35 9 3619 81 3 3313 30i3 3415 6-21-81 6-28-81 124 12 (3) 103 10 106211 105110 97 10 116t12 (3) 107111 (3) 94 9 103211 107218

TABLE C-13 (cont.) CONCENTRATIONS OF DETA Eft 1TTERS IN AIR PARTICULATE SA!PLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pCi/rt3 2 2 signa SAMPLE SAMPLE SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SS-APT SIART DATE STOP DATE 252 554 505Q 1152 1554 981 1D2 3D1 12E1 A\TRAGE 6-28-81 7-05-81 117t12 (4) 115til 115 11 117 12 116 12 132 13 (4 ) 120212 (4 ) 41t4 123112 111!53 7-05-81 7-12-81 139214 129 13 127 13 129 13 133 13 127 13 132213 60 6 134113 123t48 7- 12-81 7- 19 -81 137114 122*12 45 5 136t14 122212 131 13 123 12 49t5 124112 110272 7- 19-8 1 7-26-81 99210 97 10 9229 94 9 90 9 93t9 92i9 4114 '13 10 33236 7-26-81 8-02-81 73t7 66f7 65 7 DO 3 73t7 76 3 7317 45!5 3313 70122 8-02-81 8-09-81 4815 50 5 48 5 50 5 53 5 52 5 5325 47 5 4525 5026 8-09-81 8-16-81 4915 4325 4214 4815 4715 50 5 4615 45 5 4725 4715 8-16-81 8-23-81 5415 47 5 47i5 41 4 49 5 5015 5015 4615 55i9 4918 8-23-81 8-30-81 50 5 53 6 4214 49 5 42 4 47 5 50 5 41 4 5015 4719 co O 8-30-81 9-06-81 3615 35 5 3614 3224 34 4 36 4 35 4 33 4 3314 3423 9-06-81 9-13-81 3424 3724 3614 33 4 3614 3914 33 3 35 4 33 4 36t4 9-13-81 9-20-81 2914 27 4 2914 26 4 2923 26 4 23 3 1925 28t4 2716 9- 20-81 9-27-81 2524 2314 25i3 23 3 2613 25 4 2723 10 2 2413 24211 9-27-81 10-04-81 20 4 1613 1522 20 3 1722 1723 17 3 1013 2114 1727 10-04-81 10-11-81 12i3 13t3 11 2 15 3 12 3 1823 13 3 412 14 6 12 6 10-11-81 10-18-81 2214 25t3 2013 2714 2513 2114 2223 20 3 18 4 2226 10-18-81 10-25-81 21 4 2313 21 3 2314 2113 22 4 23 3 1623 30 5 2227 10-25-81 11-01-81 1514 13c3 1323 13 4 1413 1414 1724 913 1623 14 5 11-01-81 11-09-81 25 4 21t3 2023 2023 23 3 2414 22 3 13 3 2313 2127 11-09-81 11-15-81 1924 2514 1723 22 4 1914 1714 19!3 1414 1913 1916 11-15-81 11-22-81 1613 14 3 13 3 1413 1323 1523 1423 913 1212 13 4 11-22-81 11-29-81 15t3 1213 1313 Idi3 17 3 15 3 14 3 1313 17 3 14i3 11-29-81 12-06-81 2014 1823 15t3 1623 2023 1623 1613 11z3 1413 1626 12-06-81 12-13-81 1313 14t3 13 3 13 3 13 3 1413 1213 10 2 1322 1322 12-13-81 12-20-81 16 3 1813 18t3 1723 1713 19 3 21t3 14 2 1612 17 4 12-20-81 12-28-81 22 3 2323 23 3 23 3 23 3 24!3 23 3 1722 2123 2224 12-28-91 1-03-82 21t4 2414 20 3 2113 2213 22 3 2323 1613 20t3 2115 Avera9e 101t176 1072135 93t173 101 176 75 162 100t177 931173 872160 1001175 Indicator Average 972174

TABLE C-13 (cont.) CONCENTRATI0:15 0F BETA D1ITTERS IN AIR PARTICULATE SA?FLES IN Tile VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pC1/n32 2 s19na SA?1PLE sat 1PLE SS-APT SS-APT SA!1PLE SA!1PLE SS-APT START DATE STOP DATE 7G1 12G1 START DATE STOP DATE 7H1 AVERAGE 12-28-30 1-03-81 - 79i8 12-30-80 1-05-81 247225 163t238 1 03-81 1-11-31 - 71 7 1-05-81 1-12-81 40 5 56 44 1-11-81 1-13-81 - 77t9 1-12-81 1-19-81 7013 74110 1-18-81 1-25-31 - 109111 1-19-81 1-27-31 113211 11116 1-25-81 2-01-31 - 3213 1-27-81 2-03-81 93 9 33216 2-01-81 2-03-81 - 7618 2-03-81 2-10-01 113:11 95152 - 2-03-81 2-15-31 - 33 9 2-10-8 1 2-17-81 102i10 95220 2-15-81 2-22-31 - 123213 2-17-31 2-24-31 145 15 137124 2-22-81 3-01-31 - 95t10 2-24-81 3-03-81 91 9 9316 3-01-81 3-03-31 103111 (5) 7713 3-03-81 3-10-31 103211 98236 3-08-81 3- 15-81 176 13 122212 3-10-81 3-17-31 162116 153tS6 3-15-81 3-22-31 143114 132213 3-17-31 3-24-81 121t12 132222 3-22-81 3-29-31 203121 211121 3-24-81 3-31-81 245 25 221241 3-29-81 4-04-31 321132- 351135 3-31-31 4-07-31 323232 332 34 4-04-81 4-12-31 245 25 262126 4-07-81 4-15-01 222122 243i40 4-12-31 4-19-31 221122 213221 4-15-81 4-21-G1 249125 223233 4-19-81 4-26-81 163t16 (1) 4-21-81 4-23-81 163116 163 4-26-81 5-03-81 233 23 226123 4-23-81 5-05-31 223222 227210 5-03-81 5 8 1 (1) 256i26 5-05-81 5-12-31 174217 215t116 5 8 1 5-17-31 175217 212 21 5-12-01 5-13-81 276 23 2212102 5-17-81 5-25-31 34n235 170217 5-18-81 5-27-81 344 34 2371203 5-25-81 5-31-31 224 22 111 11 5-27-31 6-03-31 171217 1692113 5-31-d1 6-07-81 138214 128t13 6-03-81 6-10-81 131213 132210 6-07-81 6-14-81 143t14 116t12 6-10-81 6-16-81 117*12 125t31 6-14-81 6-21-81 101110 82 8 6-16-81 7-02-81 86 9 (6) 90 20 6-21-81 6-28-81 110 11 57 6 (3) 84 53

TABLE C-13 (cont.) CONCENTRATI0f4S OF BETA E!!ITTERS IN AIR PARTICULATE SAftPLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pCi/n l 2 sigma SNiPLE SA;1PLE SS-APT SS-APT SA!1PLE SAftPLE SS-APT START DATE STOP DATE 7G1 12G1 START DATE STOP DATE 7H1 AVERAGE 6-28-81 7-05-31 124 12 5417 (4) 7-02-31 7-03-31 121112 100179 7-05-81 7-12-31 144 t14 113 11 7-03-31 7-15-81 143115 135133 7-12-81 7-19-31 127213 113 12 7-15-31 7-22-31 100 10 115127 7 8 1 7-26-31 93r10 34 3 7-22-31 7-29-31 36 9 39 15 7-26-31 3-02-31 74 7 3615 7-29-3 1 3-05-31 63 7 59 41 8-02-81 3-09-31 52 5 26 4 8-05-31 8-12-31 43 5 42123 8-09-81 3- 16-3 1 44 4 4215 3-12-81 3-19-31 3614 4113 8-16-81 8-23-31 50 5 4225 3-19-31 3-23-31 46 5 46 3 3-23-81 3-30-31 4324 36 5 3-28-31 9-04-81 4014 4027 8- 30-81 9-06-31 32 4 31 5 9-04-81 9-10-31 4215 35 12 9-06-81 9-13-31 36 4 23 5 9-10-31 9-16-31 4315 36115 9-13-81 9-20-31 3023 12 3 9-16-81 9-22-31 2514 22219 9-20-81 9-27-31 2513 1013 9-22-31 9-23-81 2714 21219 r$ 9-27-81 10-04-31 1623 14 5 9-23-31 10-05-31 1713 16 3 10-04-81 10-11-31 1413 1315 10-05-31 10-12-81 2914 19 18 10-11-81 10-18-31 21 3 25 6 10-12-31 10-17-31 26t5 2415 10-18-81 10-25-81 23t3 24 6 10-17-31 10-25-31 23 3 2311 10-25-81 11-01-31 12 3 11 4 10-25-31 10-31-31 17 4 13 6 11-01-31 11-09-31 1913 2014 10-31-31 11-03-31 2423 2115 11-09-81 11-15-31 20 3 15 6 11-03-31 11-14-31 25 4 20 10 11-15-31 11-22-31 12 2 14 3 11-14-31 11-23-31 16 3 14!4 11-22-81 11-29-31 13t3 13i5 11-23-31 11-30-31 20t3 15 3 11-29-81 12-06-31 13t3 1213 11-30-31 12-05-31 1715 1616 12-06-81 12-13-31 13 3 11t3 12-05-31 12-14-81 1221 12 2 12-13-31 12-20-31 20 3 323 12-14-31 12-21-31 1313 15113 12-20-81 12-28-31 1923 1113 12-21-81 12-23-31 2013 17110 12-28-31 1-03-32 2013 11 3 12-23-31 1-04-32 2413 13213 Average 97t180 341158 1011174 Control Average 941170

                                                                   - No result because the sampling station was not in operation.                    (4) Sampling period was 6-29-81 to 7-05-81.

(1) Sample was not received due to sampler malfunction. (5) Sampling was initiated on 3-01-81. (2) Sampling was initiated on 5-03-81. (6) Sample collection nissed on 6-24-31; data repre-(3) Sampling period was 6-21-81 to 6-29-81. sents a two week period.

TABLE C-14 CONCENTRATIONS OF GAfftA EftITTERS* IN QUARTERLY C0ftPOSITES OF AIR PARTIC1 LATE SAltPLES IN THE VICINITY OF SUSQUEHANNA $ES Results in Units of 10-3 pC1/m3 2 2 si9ma STATION NO Be-7 Mn-54 Nh-95 Zr-95 Ru-103 Ru-106 Cs-137 Ce-141 Ce-144 AND DATE SLAPT 152 12-28-80 to 48212 <0.8 50 5 25 3 9.612.0 <14 <1.3 6.211.7 20 6 3-29-81 3-29-81 to 88 17 <1.8 86 9 37 5 1223 27 14 4.4il.4 5.8 2.6 86t12 6-29-81 6-29-81 to 90116 <1.5 1222 4.611.8 <2.2 <17 <3.4 <1.9 2216 9-27-81

 $     9-27-81 to     32214             <1.4     <1.7          <2.5            <1.7            <10            <1.2   <1.6    <5.7 1-03-82 Avera9e        65 58               -

37277 17 33 - - - - 33272 SS-APT-SS4 12-28-80 to 62116 <1.6 4915 21 3 1222 <19 <2.0 7.012.1 1828 3-29-81 3-29-81 to 81119 <2.2 8328 39i5 14 3 <27 3.6il.9 5.812.3 71110 6-28-81 6-28-81 to 100!14 <1.3 15 2 7.311.9 <1.8 <15 2.511.0 <2.1 28 6 9-27-81 9-27-81 to 50t11 <1.2 <1.7 <2.1 <1.2 <11 <1.1 <2.1 <7.0 1-03-82 Average 73144 - 37273 17t33 - - - - 31156

TABLE C-14 (cont.) i CONCENTRATIONS OF GNT1A C1ITTERS* IN QUARTERLY COMPOSITES OF AIR PARTICULATE SAf1PLES IN THE VICINITY OF SUSQUEHANNA SES Results in bnits of 10~3 pCi/n3 2 2 signa STATION NO. Be-7 th-54 !b-95 Zr-95 Ru-103 Ru-106 Cs-137 Ce-141 Ce-144 AND DATE

55. APT-1152 12-28-90 to 45 11 <1.0 46 5 2113 10 2 <13 <1.4 6.511.3 1524 3-29-31 2-29-31 to 90223 <2.0 100110 42 5 1223 <37 4.511.7 6.712.8 33t11 6-28-81 6-28-81 co to 91 14 <1.1 1222 __ 4.7 1.5 <1.7 <14 <1.5 <2.6 1927
  • 9-27-81 9-27-81 to 41214 <1.5 <2.2 <3.0 <1.9 <15 <1.5 <3.2 <10 1-03-82 Ave rage 67155 -

40 38 18 36 - - - - 32169 SS-APT-1554 5-03-81 to 130 33 <3.7 93 10 4727 10 4 (43 4.4 2.5 11 4 33117 6-28-81 6-26-81 to 120115 <1.2 14 2 6.4!1.7 <1.6 <26 <1.5 <1.9 2527 9-27-81 J-27-81 to 38t13 <0.9 <1.5 <1.9 <1.0 <6.8 <0.9 <1.4 <4.6

      ' 03-82 Av; rage      962101        -

331105 18250 - - - - 38 81

TABLE C-14 (cont.) CONCENTRATIONS OF GNf1A Ef1ITTERS* IN QUARTERLY C0ff0 SITES OF AIR PARTICULATE SA!PLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pC1/m 31 2 510ma STATION NO. Be-7 Mn-54 Nb-95 Z r-95 Ru-103 Ru-106 Cs-137 Ce-141 Ce-144 AND DATE SS-APT-9BI 12-28-80 to 60113 <1.0 42 4 24 3 13 2 <12 <1.6 3.511.6 1515 3-29-81 3-29-81 to 80121 2.111.4 91 9 3715 16t3 <31 4.1 2.0 5.1 2.6 78112 6-29-81 6-29-81 to 92116 <1.3 1212 7.012.1 <1.6 <15 <1.4 <1.7 24 5 9-27-81 co

  • 9-27-81 to 48116 <1.6 <2.3 <3.3 <2.0 <14 <1.5 <3.1 <10 1-03-82 Average 70139 -

37100 13131 - - - - 32163 SS-APT-102 12-28-80 to 52115 <1.3 37 4 2013 9.621.3 <14 <1.5 5.511.6 1615 3-29-81 3-29-81 to 86122 <1.8 87 9 3514 11 3 22112 4.611.4 4.6 2.2 73 10 6-29-81 6-29-81 to 110t15 <1.2 1322 4.1 2.0 <2.0 <17 1.611.0 <2.1 2417 9-27-81 9-27-81 to <20 <0.9 <1.3 <1.9 <1.2 <6.8 <1.0 <2.4 <8.9 1-03-82 Avera9e 67 79 - 35176 15t31 - - - - 30i53

TABLE C-14 (cont.) CONCENTRATIONS OF GA'f1A EITITTERS* IN QUARTERLY C0t1POSITES OF AIR PARTICULATE SA!1PLES IN THE VICINITY OF SUSQUEHANNA SES Results in lnits of 10-3 pCi/n 3 2 si n STATION NO. Be-7 l1n-54 tb-95 Zr-95 Ru-103 Ru-106 Cs-137 Ce-141 Ce-144 AND DATE SS-APT-301 12-28-80 to 4~ 13 <1.2 37r4 1823 9.21.9 <14 <1.5 5.9 2.7 <16 3-29-81 3-29-81 to 94117 1.6 0.8 7828 34 4 11 2 24211 3.6 1.3 4.812.6 7121') 6-28-81 6-28-81 to 63113 <1.3 7.5 1.5 3.5 1.7 <2.0 <16 <1.2 <2.9 15 7 9-27-81 oo 9-27-81 to 31 11 <0.8 <1.5 <2.3 <1.2 <10 (2.1 se.1 < 7.4 1-03-82 Average 59154 - 31!70 14t30 - - - - - SS-APT-12E1 12-28-80 to 46 14 <1.0 3914 23:3 12 2 <15 <1.2 7.!!1.5 1615 3-29-81 3-29-81 to 66t17 <1.8 8328 3315 9.9 i3.0 <23 3.911.4 7.1 1.8 7118 6-28-81 6-28-81 to 100t17 <1.6 11 2 5.4i2.3 <2.0 <17 2.3 1.1 <2.7 2543 9-27-81 9-27-81 to 42110 <0.8 <1.0 <2.1 <1.1 <8.1 <0.8 <2.4 <8-6 1-03-81 Average 64153 - 34 73 17133 - - - - 30156

TABLE C-14 (cont.) CONCENTRATIONS OF GAfftA DtITit'RS* IN QUARTERLY COMPOSITES OF AIR PARTICULATE SAliPLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pC1/m3 2 signa STATION NO. Be-7 fin-54 Nb-95 Zr-95 Ru-10~ Ru-106 Cs-137 Ce-141 Ce-144 AND DATE SS- APT-7G1 12-28-80 to 97 33 <3.8 97210 49 7 1715 <39 <4.6 1314 34:18 3-29-81 3-29-81 to 78t24 <2.6 91 9 38 5 11 3 <25 3.411.6 5.712.9 78212 6-28-81 6-28-81 to 09213 <1.2 12 2 5.5 1.7 <1.7 <14 1.811.0 <1.4 20 5 9-27-81 cn 9-27-81 to 49 14 <1.3 <1.7 <2.4 <1.7 <14 <1.6 <2.5 (8.5 1-03-82 Avera9e 78242 - 50 101 24 47 - - - - 35261 SS-APT-12G1 12-28-80 to 40112 <1.0 36 4 20 3 1212 <13 <1.3 7.311.5 14 4 3-29-81 , 3-29-81 to 83224 <2.0 83 9 33 5 1213 (28 3.9 1.8 5.812.7 68112 6-29-81 6-29-81 to 70 t16 <1.2 10 2 6.612.0 <2.1 <12 2.5t1.2 <3.4 <14 9-27-81 9-27-81 to 27215 <2.1 <3.0 <4.1 <2.9 <22 <2.1 <4.5 <14 1-03-82 Average 55 52 - 34277 17131 - - - - -

TABLE C-la (cont.) CONCENTRATIONS OF GAfftA OtITTERS* IN QUARTERLY C0tPOSITES OF AIR PARTICULATE SA!1PLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of 10-3 pCf/m 3 t 2 signa STATION NO. Be-7 fin-54 Nb-95 Zr-95 Ru-103 Ru-106 Cs-137 Ce-141 Ce-144 AND DATE SS. APT-7H1 12-30-80 to 53!11 <1.2 49 5 25 3 9.5 1.6 <14 <1.3 7.921.6 2026 3-31-81 3-31-81 to 54 15 <2.4 74 7 31 4 9.9i2.1 22 12 4.12.0 5.411.7 65t7 7-02-81 7-02-81 to 110114 <1.3 12 2 5.5 1.4 <1.6 <14 2.1 0.9 <2.1 28 8 9-23-81 m 9-28-81 m to 46 10 <0.7 <1.1 <1.6 <1.4 ( 10 <1.2 <2.8 <9.0 1-04-82 Average 66159 - 34267 16229 - - - - 31149 SS-APT-5050 12-28-80 to 30123 <1.6 7523 3915 16 3 <20 <2.1 12 2 25 6 3-29-81 3-29-81 to 01 22 <1.9 91 9 39i4 1112 <27 4.8 1.3 5.712.4 73211 6-28-81 6-28-81 to 96 13 <1.0 1212 3.8 1.3 <1.2 <10 1.40.8 <2.0 1926 9-27-81 9-27-81 l to 51t11 <1.1 <1.2 <1.9 <1.3 <9.8 <1.1 <2.0 <6.6 1-03-82 Ave ra9e 77 38 - 45 90 21242 - - - - 31158

           .,11 other gama emitters searched for wem (LLD; typical LLDs are found on Table C-29.

TABLE C-15 CONCENTRATIONS OF ALPHA E!i!TTERS STRONT!!#1-89* AND -90 IN QUARTERLY C0!iPOSITES OF AIR PARTICULATE SA1PLES IN THE VICINITY OF SUSQUEHA'c4A SES Results in Units of 10~ pC1/m3 1 2 sigma STATION NO. JANUARY APRIL JULY OCTOBER RADIOACTIVITY TO TO TO TO YURLY l1 ARCH JUNE SEPTE!18ER DECE!1BER AVERAGE SS-APT-252 Alpha 2.610.6 4.511.4 3.1!0,5 2.3 0.4 3.1!2.0 Sr-89 4.911.0 6.021.1 1.3 0.4 <0.3 3.115.5 S r-90 (0.8 1.1 0.5 0.9 0.2 <0.2 0.8!0.8 SS-APT-554 Alpha 4.9 0.9 2.10.6 3.3 0.5 2.5t0.4 3.222.5 Sr-89 5.6!0.6 5.6+0.9 <0.8 <0.3 3.115.9 Sr-90 <0,5 1.710.5 0.9 0.3 <0 . 2 0.811.3 SS-APT-1152 Alpha 2.810.6 2.8 0.8 3.2 0.5 2.9t0.4 2.7 1.1 S r-89 4.711.0 6. 3 t0.9 1.120 .4 <0.3 3.115.7 Sr-90 <0.8 1.3io.4 0.410.2 <0.2 0.711.0 SS-APT-1554 Alpha -

                                                   <0.6(1)            3.420.5                     3to.4              2.112.8 Sr-89                          -

5.621.2 0.Si0.4 <0.3 2.116.0 Sr-90 - 1.60.7 0.8to.2 <0.1 0.811.5 SS-APT-505Q Alpha 4.610.8 2.020.6 1.1 0.4 2.5 0.4 3.lt2.3 Sr-89 6.3t0.9 6.0 0.8 0.9t0.3 <0.3 3.426.4 Sr-90 <0.4 1.4t0.4 0.30.2 0.10.1 0.621.2 SS- APT-981 Alpha 2.4 +0.5 2.2 0.6 3.610.5 2.3 C.4 2.611.3 Sr-89 5.5 0.8 6.2 0.9 6.0 0.4 <0.3 4.515.6 Sr-90 <0.7 1.6 0.4 0.6 0.2 <0.2 0.8ti.2 SS-APT-102 Alpha 3.20.6 1.70.5 3.4 0.4 2.2 0.4 2.611.6 Sr-89 3.610 .7 7.0 0.7 <0.5 <0.3 2.916.3 Sr-90 0.610.4 0.810.4 0.910.2 (0.1 0.6 0.7 SS-APT-3D1 Alpha 4.010.7 2.4 0.6 2.2'.0.4 1.40.3 2.522.2 Sr-89 4.8t0.6 5.4 0.8 <0.5 <0.3 2.815.5

   $r-90                       <0.5               1.1 0.4             0.5 0.2                    (0.2                0.610.8 I

SS- APT-12E1 Alpha 2.810.6 2.10.6 2.920.5 2.6 0.4 2.610.7 Sr-89 5.820 .8 6.521.0 1.0 0.4 <0.3 3.416.4 Sr-90 0.510.5 1.4 0.5 0.5 0.2 <0.2 0.711.0 SS-APT-7G1 Alpha 1.410.7 (2) 1.5 0.5 2.8 0.4 2.2 0.4 2.021.3 Sr-89 9.61.6 5.8 0.8 0.8 0.4 0.220.2 4.18.9 S r-90 <1.4 1.120.4 0.6 0.2 <0.2 0.821.1 SS-APT-12G1 i Alpha 3.210.6 1.7z0.6 2.6 0.5 1.20.3 2.221.8 ' Sr-89 5.0 0.8 4.5tl.0 <0.6 <0.4 2.614.9 Sr-90 0.6 0.4 1.4 0.5 0.5 0.2 <0.2 0.711.0 SS-APT-7H1 Alpha 2.4 0.5 1.9 0.4 3.2 0.5 2.020.4 2.421.2 Sr-89 6.0t0.7 1.4 0.3 5.420 .2 <0.3 3. 3 15 . 7 Sr-90 <0.6 0.320 .2 0.4 0.1 0.210.1 0.4 0.?

  • Sr-89 results are corrected for decay to the sample stop date.

[ (1) Station SS-APT-1554 be9an operation on 5-03-81; therefore, the second quarter composite contained only liay and l June samples. (2) Station SS-APT-7G1 began operation on 3-01-81; therefore, the first quarter composite contained only' the fiarch sample, 89

TABLE C-16 C0;1CEf4TRATIOils 0F 10DI!1E-131* I:4 FILTERED AIR !!4 THE VICI!1ITY OF SUSQUDIA!4'JA St:S Results in Units of 10-3 pCi/n3 r 2 s19m START STOP .SS-AIO SS-AID SS-AIO SS-AID SS-AIO SS-AIO SS-AIO SS-AIO SS-AIO SS-AIO SS-AIO DATE DATE 252 534 505Q 1152 1554 931 1D2 3D1 12E1 7G1 12G1 12-28-80 1-03-81 <12 <9.3 <9.3 (7.1 -

                                                                                   <9.3            -          -
                                                                                                                         <10      -        -

1-03-81 1-11-81 <8.8 (' <7.7 <7.2 -

                                                                                   <7.7            -          -

(1) - - 1-11-81 1-18-81 <73 (2) <21 <10 <11 -

                                                                                   <3.7            -          -
                                                                                                                         <9.9     -        -

1-18-31 1-25-81 <3.1 <7,6 <6.3 (6.7 -

                                                                                   <8.6            -          -
                                                                                                                         <6.6     -        -

1-25-81 2-01-81 <3.3 <9.3 <3.2 <7.0 -

                                                                                   <5.6            -          -
                                                                                                                         <9.0     -        -

2-01-81 2-08-81 <0.4 ':7.5 <3.1 <5.7 -

                                                                                   <6.6            -          -
                                                                                                                         <5.3     -        -

2-08-81 2-15-81 <8.6 (11 <7.0 <7.1 -

                                                                                   <6.9            -          -
                                                                                                                         <7.3     -        -

2-15-81 2-22-81 <7.9 <9.6 <3.0 <6.3 -

                                                                                   <7.0            -          -
                                                                                                                         <6.7     -        -

2-22-81 3-01-81 <7.2 <!2 (6.1 <6.1 -

                                                                                   <5.3            -          -

(5.9 - - e o 3-01-81 3-08-81 <9.1 <9.5 <6.4 <7.0 -

                                                                                   <5.3          (6.7 (3)   (7.9 (3)     <6.3   <6.9(3) <6.9 (3) 3-08-81  3-15-81 <8.6    <3.0         <6.2          <6.4              -
                                                                                   <6.4          <6.5       <6.2         <6.0   <6.4    <6.4 3-15-31  3-22-81 <7.5    <13          (5.9          <6.1              -
                                                                                   <6.1          (6.0       (G.3         <5.3   <6.2    <6.6 3-22-81  3-29-81 <8.2    <3.3         <3.2          <7.3              -
                                                                                   <3.7          <7.7       <7.6         <7.0   <7.5    <9.5 3-29-81  4-04-81 <11     <11          <11           <3.6              -
                                                                                   <10           <9.4       <10          <9.4   (9.2    <10 4-04-81  4-12-81 <6.7    <7.0         <G.0          <h.2              -
                                                                                   <5.7          <5.4       <6.1         <5.0   <6.2    <6.0 4-12-81  4-19-81 <9.0    <3.3         <3.1          <7.2              -
                                                                                   <7.5          <11        <10          <6.7   <6.1    (5.5 4-19-31  4-26-31 <7.5    <9.0         <7.6          <3.5              -
                                                                                   <7.5          <6.9       <7.7         <3.0   (9.3     (1) 4-26-31  5-03-81 <11     <7.2         <5.9          <f .3             -
                                                                                   <6.0          <5.6       <6.4         <4.0   <14     <9.5 5-03-81  5-10-81 <6.3    <3.6         <4.7          <7.3           <3.9(4)       <7.3          <5.3       <4.6         <5.7    (1)    <12 5-10-81  5-17-81 <6.9    <7.7         <5.6          <7.6           <7.9          <6.9          <3.7       <6.0         <4.4   <6.9    <11 5-17-81  5-25-81 <5.3    (6.0         <7.0          <6.3           <7.0         <5.9           <5.0       <5.5         <6.0   (9.2    <8.4 5-25-81  5-31-81 (9.6    <7.2         <10           <9.1           <10          <3.3           <7.9       <7.0         <5.6   <9.1    <11 5-31-81  6-07-81 <7.4    <5.7         <3.2          <7.4           <5.4         (6.9           <4.3      <5.0          (7.1   <7.9    <9.4 6-07-81  6-14-81 <9.1    <6.3         <3.9          <3.1           <6.3         <7.3           <5.3      <7.1          <11    <7.2    <9.5 6-14-81  6-21-Bi <8.0    <5.9         <3.5          <3.3           <5.1          <3.2          <5.1       <6.2         <4.9   <6.7    <11          !

6-21-81 6-28-81 <7.5(5) <11 <15 <9.3 <7.1 <6.2(5) <4.2(5) <6.2 <7.3 <13 <9.9 (5)

TABLEC-16(cont.) CONCENTRATIONS OF 10 DINE-131* IN FILTERED AIR IN THE VICINITY OF SUSQUEHA! CIA SES Results in Units of 10' pCi/m 2 si0na START STOP SS-AIO SS-AID SS-AIO SS-AIO SS-AIO SS-AIO SS-AIO SS-A10 SS-AIO SS-AIO SS-AIO DATE DATE 252 554 505Q 1152 1554 981 102 3D1 12E1 7G1 12G1 6-28-81 7-05-81 <13(6) <7.0 <9.2 <7.9 <5.1 <11(6) <7.3(6) <5.3 <6.2 <8.7 <16(6) 7-05-81 7-12-81 <13 <5.1 <7.2 <7.1 <5.9 <7.2 <5.1 <5.5 <12 <11 <15 7-12-81 7-19-81 <9.9 <4.6 <7.3 <7.0 <5.3 <6.1 <4.3 (5.1 <12 <7.3 <11 7-19-81 7-26-81 (6.6 <5.9 <5.1 (5.5 <4.5 <5.3 <5.2 <5.3 <5.3 <4.5 <8.5 7-26-81 8-02-81 <7.8 <6.5 <3.6 <7.1 <5.3 <6.4 <4.6 <5.7 (G.0 <5.6 <9.1 8-02-81 8-09-81 <6.7 <4.9 <5.1 <7.1 <7.4 (6.4 <5.8 (6.1 <5.1 <5.0 <8.4 8-09-81 8-16-81 (6.9 <6.2 <4.9 (6.0 <4.9 <5.8 <5.1 <7.6 <5.0 <5.3 <11 8-16-81 8-23-81 <6.0 <4.8 (4.4 <5.4 (4.6 <4.3 <3.9 <i.2 <15 <5.0 <8.1 8-23-81 8-30-81 <6.8 <9.3 <5.7 <6.5 <5.5 <7.0 <5.5 <6.6 <5.2 <6.5 <9.9 0 8- 30-81 9-06-81 (6.8 <7.3 <6.2 <6.0 <6.2 <3.4 (6.7 <6.6 <5.6 <5.4 <8.3 9-06-81 9-13-81 <8.2 (R.2 <7.7 <6.6 <5.2 <7.4 <5.1 <6.4 <4.5 <3.6 <15 9-13-81 9-20-81 <6.5 <6.6 <5.7 <7.0 <4.8 <6.9 <5.5 <9.9 <6.0 <4.9 <3.0 1 9- 20-81 9-27-81 <7.5 <5.6 <4.1 <5.4 <4.5 <6.3 <5.4 <4.3 (6.3 <5.3 <S.2 9-27-31 10-04-81 <8.6 <5.8 <4.7 (6.2 <4.7 <6.7 <4.9 (6.6 <3.1 (5.4 < 13 10-04-81 10-11-81 <7.9 <7.1 (6.2 <5.9 <5.6 <7.9 (6.1 <5.2 <17 (6.6 <17 10-11-81 10-18-81 <6.4 <6.7 <5.9 <6.6 <5.5 <7.0 <5.5 <6.6 <3.0 <7.5 <13 10-18-81 10-25-81 <7.5 <5.3 <5.5 <6.5 <5.2 (6.6 (5.6 <6.2 <10 <5.1 <13 10-25-81 11-01-81 <6.3 (5.0 <3.0 <5.8 <5.5 <6.6 <5.7 (6.7 <4.3 <5.4 <6.9 11-01-81 11-09-81 <5.7 <5.0 <4.3 <5.3 <4.6 <5.7 <4.4 <5.2 <3.7 <5.1 (6.9 11-09-81 11-15-81 <7.8 <6.5 <5.9 <7.1 <5.9 <7.8 <5.6 <7.1 <5.0 (6.2 <16 11-15-81 11-22-81 <7.1 <5.4 (8.3 <5.8 <5.7 <6.1 <6.0 <6.9 <7.0 <6.9 <8.6 11-22-81 11-29-81 <7.3 <6.3 <6.9 <5.5 <5.2 <6.4 <5.5 <7.4 <4.7 (6.6 <18 ' 11-29-81 12-06-81 <6.2 (6.0 <7.5 <4.8 <4.9 <6.1 <5.4 <4.7 <4.5 (7.6 <8.4 12-06-81 12-13-81 <6.4 <5.9 <5.5 <5.0 <5.0 <5.7 <5:1 <4.6 <4.5 <6.1 <8.3 12-13-81 12-20-81 <5.1 <4.6 <4.2 <6.5 (5.1 <6.1 (6.2 <4.6 <5.1 <6.0 <9.9 12-20-81 12-28-81 <4.6 <4.7 <5.4 <3.9 <3.7 <4.3 <4.0 <3.3 <3.4 <6.3 <7.8 12-28-81 1-03-82 <7.2 <5.8 <6.3 <5.8 <5.5 <5.9 <5.9 <4.5 <5.6 <6.6 (7.1 i

Tant! C-16 (cont.) CONCENTRATIONS 0F 10 DINE-131o IN FILTERED AIR IN THE VICINITY OF SUSquEHANNA SES Results in Units of 10-3 pCf/m 3 2 signa START STOP START STOP DATE DATE SS-AID-7H1 DATE DATE SS- AIO-7H1 12-30-30 1-05-81 <6.3 7-02-a2 7-03-31 (6.6 1-05-81 1-12-81 <6.7 7-03-31 7-15-31 <4.8 1-12-81 1-19-81 <14 7-15-3? 7-22-31 <5.2 1-19-81 1-27-81 <6.3 7-22-31 7-29-31 <4.4 1-27-31 2-03-81 <5.1 7-29-31 3-05-81 <5.5 2-03-31 2- 10 -8 1 <4.7 3-05-31 3-12-31 <3.5 2- 10 -31 2-17-81 <5.7 3-12-31 3-19-31 <3.3 2-17-81 2-24-81 <6.6 3-19-31 3-23-31 <5.0 2-24-31 3-03-81 <6.5 3-23-31 9-04-31 <5.6 3-03-31 3 8 1 <4.4 9-04 -31 9- 10-31 <9.4 3-10-81 3-17-91 <5.7 9-10-31 9-16-31 <4.7 3-17-81 3-24-31 <7.3 9-16-31 9-22-31 <5.6 3-24-81 3-31-81 <4.9 9-22-31 9-23-31 <6.0 r$ 3-31-31 4-07-31 <d.3 9-23-31 10-05-31 <5.5 4-07-81 4-15-31 <3.3 10-05-31 10-12-31 <5.2 4-15-81 4-21-01 (5.3 10-12-31 10-17-31 (9.6 4-21-81 4-23-31 (6.2 10-17-31 10-25-31 (9.0 4-28-81 5-05-31 <4.5 10-25-31 10-31-31 <7.4 5-05-81 5 81 <4.4 10-31-31 11-03-31 <5.4 5-12-31 5-18-01 <4.2 11-03-31 11-14-31 <6.4 5-18-81 5-27-81 <3.1 11-14-31 11-23-31 (6.8 5-27-31 6-03-81 <3.4 11-23-31 11-30-31 (5.1 6-03-81 6-10-81 <5.5 11-30-31 12-05-31 <15 6-10-81 6-16-81 <a.7 12-05-31 12-14-31 <4.0 6-16-81 7-02-81 <3.4(7) 12-14-31 12-21-81 (7.0 12-21-31 12-28-81 (5.3 12-23-31 1-Oa-32 (7.8 Iodine results are decay corrected to sample stop date.

  -        No nesult because sampling station was not in operation.

Sample was not received due to sampler malfunction. High LLD due to low sample volume. Sampling was initiated on 3-01-31. Sampling was initiated on 5-03-81. Sanpling period was 6-21-81 to 6-29-31. Sampling period was 6-29-81 to 7-05-31. Sample collection missed on 6-24-31; data represents a two week period.

TABLE C-17 CONCENTRATIONS OF TRITILEt AliD fiAlttA E!!ITTERS* IN PRECIPITATION SAftPLES Ifl THE VICINITY OF SUSQUEHAf4NA SES ResJits in Units of pCi/l 2 signa APRIL ** JULY OCTOBER STATION N0. TO TO TO YEARLY RADI0 ACTIVITY FEBRUARY ftARCl! JUNE SEPTE!1BER DECEttBER AVERAGE SS-RWA-554 Tri tiura <211 227 66 184 110 <193 <219 - Gamma Emitters Be-7 24 9 35 6 10 4 21 5 11 5 20 21 Zr-95 <2.3 9.6 1.1 <1.6 <1.3 <1.1 - Nb-95 3.41.0 21 2 3.2 0.6 <0.9 <0.8 6217 Ru- 103 4.5 1.0 9.41.0 1.6 0.6 <0.9 <0.7 3.417.3 Ru-106 <9.0 6.83.9 <5.5 <5.6 <5.0 - Cs-137 <0.9 1.80.6 <1.0 (0.7 <0.6 - Ce-141 4.2 1.6 6.2 0.9 <1.0 <1.4 <0.9 - Ce-144 <5.5 15i3 6.8 2.2 4.7 2.8 <2.8 7.0 9.4 0 SS-RWA-1152 Tri tium (1) 233 66 267 120 1511120 <219 218 97 Gamma Emitters Be-7 48 8 15 7 2415 <6.3 23 36 Zr-95 8.0 1.5 5.311.1 <1.2 <1.2 3.916.7 tb-95 11t1 8.511.1 '1.8 <0.8 5.3111 Ru-103 8.7 1.1 2.921.0 <0.8 <0.8 3.3 7.5 Ru- l')6 <8.8 <6.3 <4.9 <5.4 - Cs-137 1.2 0.6 <0.7 <0.5 <0.7 - Ce-141 5.0 1.4 <2.5 <1.8 <1.2 - Ce-144 12 4 <5.1 <5.4 <4.1 - SS-RWA-ID2 Tritium <211 215166 <183 <193 <219 - Gama Emitters Be-7 27 5 5517 24 5 22 6 19 26 29 29 ! Zr-95 3.91.0 13 1 3.0 0.7 <1.1 <1.6 4.519.7 Nb-95 5.5 0.8 13 1 2.8 0.5 <0.9 <1.1 5 10 Ru-103 7.2 0.8 10 1 1.70.6 <0.8 <1.0 4.1 8.4 Ru-106 <5.6 <8.5 <5.4 <5.5 <3.2 - Cs-137 <0.6 <0.9 0.d4.4 <0.6 <0.9 - Ce-141 2.7 1.2 5.5 1 3 <1.8 <1.0 <1.8 - Ce-144 <4 . 8 12 4 6.0*3.3 <3.3 <6.2 -

TABLE C-17 (cont.) CONCENTRATIONS OF TRITIIRt AND GA!!!A E!!ITTERS* IN PRECIPITATION SAftPLES IN TiiE VICINITY OF SUSQUEliANNA SES Results in Units of pCi/l 2 sigma APRIL *" JULY OCTOBER STATION NO. TO TO TO YEARLY RADI0 ACTIVITY FEBRUARY  !! ARCH JUNE SEPTE!!BER DECEl1BER AVERAGE SS-RWA-12G2 to Tri tium (1) 142 97 1271110 <193 <219 170 86

  • Gamma Emitters Be-7 56 7 23 5 34i6 21 6 34 32 Zr-95 11 1 2.70.8 <1.3 <1.9 4.29.1 Nb-95 10 1 7.4 0.5 <1.0 <1.2 3.7 8.6 Ru- 193 9.3tl.0 2.210.6 <1.0 <1.1 3.4t7.9 Ru-106 <3.8 <6.2 <5.9 <8.4 -

Cs-137 1.0i0.5 <0.7 <0.7 <0.9 - Ce-141 6.3 1.3 1.20.7 <1.4 <1.7 - Ce-144 I6i4 8.3 2.2 4.9 2.9 <5.7 3.7110

  • All other gama emitters rearched for were <LLD; typical LLDs are found on Table C-?.9.
  **       Beginnin9 in April 1931, tritium and ganna analyses of precipitation were performed on quarterly composite samples.

(1) No precipitation samples were collected because of weather conditions.

TABLE C-18 CONCENTRATIONS OF 10 DINE-131* IN !!!LK l'1 TliE VICINITY OF SUSQUEllANNA SES Results in Units of PC1/1

  • 2 signa STATION NO. JANUARY FEBRUARY f1 ARCH APRIL f1AY JUNE SS-Pt.K-1282 (0.1 <0.1 <0.1 <0.1 <0.1 <0.08
                                                                                           <0.1          <0.1       (0.09 SS-ML K-1283                <0.1             <0.1                <0.1                   <0.1          <0.1       <0.09 SS-MLK-6C1                  (0.1             <0.0 7              <0.1                   <0.1          <0.2       <0.03 SS-ftK-10D1                 <0.1             <0.1                <0.1                   <0.1          <0.1       <0.09 SS-MLK-12D2                 <0.1             <0.1                <0.1                   <0.1          <0.1       <0.09-SS-ML K-5El                 <0.1             <0.1                <0.09                  <0.1          (0.1       <0.03
                                                                                           <0.1          <0.1       (0.1 SS-ML K-13E3                <0.09            <0.09                <0.1                  (0.1          <0.1       <0.03
                                                                                           <0.1          <0.1       <0.1 SS-ML K-10G1                <0.1             <0.1                 <0.1                  (0.2          <0.1       <0.09
                                                                                           <0.1          <0.2       <0.1 SS-rgK.7C1                    -                 -                    -                    -              -
                                                                                                                    <0.4 (1)

SS-GMK-8DI (2) (2) (2) <0.2 <0.2 (0.2 STATION 10. JULY Atr.UST SEPTEl1BER OCTOBER NOVEftBER DECE!1BER SS-ML K- 1282 (0.1 <0.1 <0.08 <0.09 <0.09 <0.1

                               <0.1             <0.09               <0.1 i SS-MLK-12B3                   (0.1             <0.1                 <0.03                 <0.03         (0.09      <0.1 SS-ML K-6C1                 <0.09            <0.1                <0.09                  <0.09         <0.09      <0.09 SS-MLK-1001                 <0.1             <0.1                <0.1                   (0.09         <0.1       <0.08 SS-MLK-12D2                 <0.1             <0.03                <0.09                 <0.1          20 . 1     (0.1 SS-MLK-5El                  <0.1             <0.09                <0.1                  <0.08         <0.1       <0.1
                               <0.1             <0.1                 <0.1 SS-ML K- 13E3               <0.1             (0.09                <0.1                  <0.09         <0.08      <0.1
                               <0.09            <0.1                 <0.1 SS-ML K-10G1                <0.1             <0.1                 <0.1                  <0.1          <0.08      <0.1
                               <0.1             <0.1                 <0.1 SS-GMK-7C1                   (3)             <0.9                  (3)                  <0.5          <0.6       <1.8 SS-GMK-801                   (3)             <0.1                 <0.1                  <0.2          <0.2       (0.2 o      todine-131 asults are corrected for decay to the sarole stop date.
   -      No result because the sa@lin9 station was not in operation.

, Station SS-GMK-7C1 was initiated on June 22. 1901. Milk was not available January through liarch because the goat was dry. hat milk was not available; therefore. pasture grass was sa@ led. 95

7 9 8 0 7 7 9 8 3 0 0 1 0 8 1 1 0 0 1 0 0! 0 0 1 1 1 1 0 1 1 - 1 1 t 2 1 1 Ds 7 4 1 5 3 9 0 9 7 5 6 1 6 0C 1 2 2 2 2 2 1 4 2 2 2 2 3 2 K t L f

               -         0    0    0        0      0       0       0      0       0   0    0     0     8 S0           4    4    5        5      4       5       5      4       5   6    6     3     7 S4           1    1    1        1      1       1       1      1       1   1    1     1     1
                     -    2    i    2               t       t       2      !           1    2     2     2 K     0    0    0        0      0       0       0      0       0   0    0     0     7 0    0    0        0      0       0       0      0       0   0    0     0     6 4    4    5        5      4       5       5      4       5   6    6     3     4 1    1    1        1      1       1        1     1       1   1    1     1     1 S

E 7 9 8 9 9 8 0 0 8 8 S 3 1 0 8 3 1 0 0 0 0 0 1 l A - 1 2 l 0 1 0 01 2 l t t 2 r f 1 s 9 4 8 9 8 8 6 8 1 0 1 6 8 f CC A 6 1 1 1 1 1 4 4 3 3 3 3 2 2 H - E K U L Q I S - 0 0 0 0 0 0 0 0 0 0 0 0 1 U S0 6 4 5 5 5 5 4 4 4 6 6 6 7 S S4 1 1 1 1 1 1 1 1 1 1 1 1 1

                    -    2    1    t        t              t        t             t   2           t     t F               K    0    0    0        0      0       0        0     0       0   0     0 O                    0    0    0                                                              0    0 0      0       0        0     0       0   0     0     0    0 6    4    5        5      5       5       4      4       4   6     6    6     5 Y                    1    1    1        1      1       1       1      1       1   1     1    1     1 T    a I    m N   9 I  1 C    s I

V 2 E H T 1

      /

N 1 7 9 9 9 9 0 0 0 0 0 1 8 1 1 9 I C 3 1 p 1 ot 0 0 0 1 1 1 1

 - K      3 -                                      2               1 1       1        0     1     3 2           2 C   L  f   8s            6    1    7        0      9       7       9      5       2   7    5     2     6 I   o  2C E   1 t      1             2    3   2         4      4       7       5      6       5   4    3     4     4 L       s      -

B N t K A I i 1L T n !

  • U - 0 0 0 0 0 0 0 0 0 0 0 0 3 S S0 5 4 4 3 4 4 4 3 3 4 7 R n S4 1 1 1 1 1 1 6 4 1 1 1 1 1 1 2 E i - 1 1 2 2 2 T K 0 0 0 0 0 0 0 0 0 0 0 0 5 T s 0 0 0 0 0 0 0 1 t 5 4 4 3 0 0 0 0 0 2 1

l 1 1 4 4 4 3 3 4 7 6 4 1 1 C u 1 1 1 1 1 1 1 1 1 s A e 1 t R N G F O 7 9 7 08 89 70 98 80 79 0 0 2 3 S 1 O 1 0 10 00 2 01 00 01 N 2 -  ! 2 2 t 2 00 1 1 6 1 2 l t O Bs 5 1 5 96 34 29 98 93 37 4 1 6 8 I T 2C < < 1 1 1 11 11 11 23 A 11 21 2 1 1 R K T L N  ! E - 0 0 0 00 00 00 00 00 00 0 6 C S0 4 4 4 54 42 0 0 N 44 43 35 52 5 6 6 2 S4 1 1 1 11 11 11 11 11 l1 1 1 1 2 O - 1 t 2 22 1 2 2 2 2 2 i2 1 t 1 C K 0 0 0 00 00 00 00 00 00 0 0 0 0 0 1 0 00 00 00 00 00 00 0 0 0 1 4 4 4 54 42 44 43 35 52 5 6 6 4 1 1 1 11 11 11 11 11 11 1 1 1 1 R Y E R R N Y R B R E E E O R A T M E B B G IH A U H L S E B M M A TT U R C I E Y U T O E E R Ar i N B R R Y N L G P T V C E T0 A E A P A U U U E C O E V SM J F M A M J J A S O N D A

7 9 0 0 99 10 09 01 99 08 8 9 9 3 3 1 0 1 1 00 11 10 11 00 10 01 0 01 3 1 - 2 2 1 1 21 2 21 t 1 1 1 Gs 0 6 7 71 63 84 84 45 77 5 6 9 8 0C 1 3 9 3 33 33 53 24 23 32 3 3 2 3 K L M

               -        0  0   0    00    00       00     00    00     00     0    0   0   5 S0         4  4   5    54    44       45     43    34     44     5    5   3   3 S4         1  1   1    11    11       11     11    11     11     1    1   1   1
                     -  i   1   2   1 1    1 2      1 1    1 1      2   2 2    1        2   1 K    0  0   0    00    00       00     00    00     00     0    0   0   1 0  0   0    00    00       00     00    00     00     0    0   0   1 4  4   5    54    44       45     43    34     44     5    5   3   4 1  1   1    11    11       11     11    11     11     1    1   1   1 S

E 88 8 S 7 9 8 8 98 92 98 09 88 0 8 0 3 A 1 0 0 0 00 01 00 10 1t 00 00 1 0 1 1 N 3 - 2 1 1 N Es 3 4 1 91 64 05 02 21 45 0 2 7 0 A 3C H 1 1 2 3 12 24 44 43 33 23 3 2 1 3 E - U K Q S L I U - 0 0 0 00 00 00 00 00 00 0 0 0 6 S S0 5 5 6 64 54 55 44 45 43 5 5 4 5 S4 1 1 1 11 11 11 11 11 11 1 1 1 1 . F - t t 1 t 1 t t 1 2 t K 1 9 O 0 0 0 00 00 00 00 00 00 0 0 0 2 0 0 0 00 00 00 00 00 00 0 0 0 6 - Y 5 5 6 64 54 55 44 45 43 5 5 4 4 C T 1 1 1 11 11 11 11 11 11 1 1 1 1 I an e N l I g b C i a I s T V 2 n E o

 )    H T                                                                                       d
    . 1                                                                                      n t

n N / 7 10 81 88 7 u I i 7 7 0 08 90 99 9 9 4 o o C 3 f c K p 1 0 0 1 10 01 00 l1 00 0 0 0 2 ( L - 1 2 1 i1 0_1

                                                                 +

e I f l s 1 4 8 11 98 29 30 70 68 1 6 7 2 r 9  !! n EC a 1 5 2 2 3 22 2E 43 44 23 31 2 2 2 3

   -  N   s     -                                                                              s C    I  t    K                                                                               D E
  • i n

L f L L L S U - 0 0 0 00 00 00 00 00 00 0 0 0 3 B R S0 5 5 4 43 31 52 43 45 32 4 6 4 5 l A E n S4 1 1 1 11 11 11 11 11 11 1 1 1 2 a T T i - 2 t t 1 1 t tt 1 2 t t t c T K 0 0 0 00 01 00 00 00 00 0 0 0 2 i 1 s 0 0 0 00 00 00 00 00 00 0 0 0 7 p 1 f t 5 5 4 43 31 52 43 45 32 4 6 4 3 y E l 1 1 1 11 11 11 11 11 11 1 1 1 1 t u A s  ; 1 T e D R L A! L G < F O e r 7 1 7 1 8 0 6 7 8 6 e S 3 w N 1 2 0 5 0 3 1 0 1 0 0 7 0 1 O 2 - Ds 2 1 1 1 3 t 1 r I 1 4 1 5 1 4 0 1 9 o T 2C < < < < f A 1 1 1 4 2 2 1 2 2 1 R - d T K e 4 E 1 h c C - 0 0 0 0 0 0 0 0 0 0 0 0 8 r N S0 7 5 5 4 5 3 5 4 3 6 6 6 4 a S4 1 1 1 1 1 1 1 1 1 1 1 1 2 e _ O - r 1 2 t 2 1 C K 2 s 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 9 s 7 5 5 4 5 3 5 4 3 6 6 6 4 r 1 1 1 1 1 1 1 1 1 1 1 1 1 t e t i m e a m m a g r e h t R o Y E R R l N Y R B R E E E l R A M O IH TT A U U R H C L I E Y T S U E T E B O E B M N AGR E A AN N B R R Y N L G P T V C E TO A E A P A U U U E C O E V SM J F M A M J J A S O N D A

  • oN t

TABL_ C-20 CONCENTRATIONS OF STRONTIU:1-89* AND -90 IN l11LK IN THE VICINITY OF SUSQUEHANIM SES Results in Units of pCi/l 2 sigma STATION NO. JANUARY FEBRUARY l1 ARCH APRIL t%Y JUNE SS-MLK-1282 Sr-89 <5.8 <19 4.6 3.3 <5.3 <4.6 <9.3 Sr-90 4.9 1.3 1.9 1.1 <2.4 3.3!1.5 3.8 0.9 1.920.9 SS-MLK-1283 Sr-89 <1.9 <2.0 <1.4 5.2 3.7 <8.1 <11 S r-90 2.2 0.6 4.0 0.7 11 1 10 2 1312 1311 SS-MLK-6C1

 $   Sr-89 Sr-90 4.4 1.3 1.4 0.6
                          <11 4.4 0.7
                                                 <5.3 4.721.7
                                                                   <4.0 4.9 1.2
                                                                           <5.9 6.911.3
                                                                                   <15 6.021.5 SS-ML K-1001 Sr-89       <2.1    3.321.2                 <5.7              <3.5    <4.7    <3.9 S r-90     2.3:0.7  4.2 0.7                7.61.9           6.4 1.1  9.311.7 4.6*1.5 SS-MLK-12D2 Sr-89      5.321.7   <2.2                   <4.0              <2.7    <6.3    <7.5 Sr-90      2.2 0.8  2.3 0.9                3.4 1.2          2.110.8  2.922.0 9.212,7 SS-ML K-5 El Sr-89       <2.6     <14                    <3.5              <3.5    <7.2    <15 S r-90     1.9 0.8 4.61.0                  7.7il.3          7.0 1.1  5.712.3 8.725.3 SS-MLK-13E3 Sr-89       <56     3.821.0                 <2.5              <3.5    <6.4    <4.4 Sr-90      3.5 0.9 2.1 0.6                6.321.0           4.7 1.1  6.212.1 5.011.6 SS-MLK-10G1 Sr-89       <83    4.511.4                  <4.0              <5.3    <6.0    <11 Sr-90      7.51.3  4.6 0.8                7.6 1.6           9.41.6   9.912.0 7.911.1 l

l i l l

TACLE C-20 (cont.) CONCENTRATIONS OF STRONTIUti-89* AND -90 Ill it!LK IN THE VICINITY OF SUSQUElW4NA SES Results in Units of pCi/l 2 signa STATION !O. JULY AUGUST SEPTE!!BER OCTOBER tOVE:1BER DECE!1 DER AVERAGE r SS-ftK-12B2 Sr-89 <1.7 1.3to.9 <1.8 <1.9 <1.8 <1.5 - S -90 1.3t0.6 1.5 0.6 3.020.7 2.10.8 2.50.7 1.6 0.6 2.512.1 SS-ML K-12B3 Sr-89 <9.0 3.211.7 2.9t2.1 <4.4 <2.G <3.0 - Sr-90 1023 7.821.1 9.211.3 9.311.6 6.9 0.8 9.1 1.2 8.8 6.5 SS-ftK-6C1 Sr-89 3.2 2.2 <7.1 <3.6 <2.2 <2.7 <2.8 - Sr-90 6.7 1.3 7.2 1.4 7.5 1.4 3.8t0.9 7.7 1.1 6.011.0 5.623.7 $ SS-tLK-10D1 Sr-89 <3.7 2.1 1.3 <6.1 <2.4 <2.6 2.822.1 - S r-90 6.321.4 5.511.1 9.4 2.2 5.7 1.0 4.3 t0.9 6.7 1.2 6.024.2 SS-!1LK-12D2 Sr-89 <1.7 <1.9 <2.1 <1.9 <7.8 <3.6 - Sr-93 1.6 0.6 1.9 0.7 2.5 0.3 2.2!0.8 3.711.7 2.921.2 3.li4.0 SS-ft K-5El Sr-89 4.121.7 <2.0 <4.2 2.9 2.7 <18 <2.5 - S r-90 3.3 1.0 4.620.8 8.21.6 4.2 1.6 7.613.7 5.810.9 5.824.2 SS-ttK-13E3 Sr-89 1.711.3 <2.4 <3.8 <2.4 <5.4 <3.0 - Sr-90 2.9 0.8 5.4 1.0 6.311.4 4.411.0 7.311.3 6.311.1 5.0t3.2 SS-ML K-10G1 Sr-89 <27 <3.4 <3.4 1.911.6 <4.5 <3.5 - Sr-93 6.9 1.1 6.921.3 7.921.3 5.9il.0 8.5t1.6 9.211.4 7.7 3.0

  • Sr-89 results are decay corrected to sample stop date.

TABLE C-21 CONCENTRATIONS OF GA'ftA EftITTERS* A!O STRONTIUti-39** AND -90 IN FISH FLESH IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/9(wet) 2 signa STATION SAftPLE SAftPLE NUMBER TYPE DATE K-43 Cs-137 S r-39 S r-90 SS-AQF-INDICATOR White Sucker 4-01-81 3.2 0.3 <0.01 <0.009 <0.004 Walleye 4-01-81 3.2 K) . 3 0.009 0.005 <0.01 <0.005 4-01-31 Channel Catfish to 3.1!0.3 0.015 0.005 <0.009 <0.005 4-02-31 White Sucker 9-11-81 3.7 0.4 0.011+0.005 <0.003 <0.003 Walleye 9-11-01 3.7 0.4 0.010 0.005 <0.006 0.00220.002

    • 9-11-81 0

0 Channel Catfish to 3.1 0.3 0.013 0.005 <0.006 <0.003 9-15-31 SS- AQF-2 H*** White Sucker 4-06-31 3.4 0.3 0.011_+0.004 <0.006 <0.003 Walleye 4-06-31 3.2 0.3 0.012 0.004 <0.01 <0.006 4-06-81 Channel Catfish to 3.2 0.3 0.014 0.005 <0.007 <0.003 4-07-31 White Sucker 9-09-31 3.30.3 0.009 0.005 <0.006 (0.003 Walleye 9-09-81 3.5 0.a 0.016 0.006 <0.006 0.00220.002 9-09-31 Channel Catfish to 3.5 0.4 <0.01 <0.00 7 0.007 0.002 9-10-81 Avera9e 3.3 0.4 0.012 0.005 - -

  • All other.gama emitters searched for were <LLD; typical LLDs are found in Table C-29.
  **     Sr-89 msults are decay corrected to sample stop date.
  ***   Station code is omitted because no exact sampling locations exist; sanples are taken based on availability.

i TABLE C-22 CONCENTRATIONS OF GA*,t1A E!!!TTERS* IN VARIOUS FOOD PRODUCTS IN THE VICINITY OF SU3QUEHANNA SES Results in Units of pCi/g(wet) 2 sigma STATION NO. SA!1PLE DATE DESCRIPTION Be-7 K-40 Hb-95 Cs-137 SS-FP F-7B2 9-03-81 Apples <0.05 0.72 0.07 <0.008 <0.005 SS-FPH-782 ')-03-81

                                 .                Honey                      <0.3         1.0 0.4      <0.04    0.07 0.02 SS-FPF-1281            9-03-81          Apples                     <0.04       0.85 0.09     <0.006  0.004 0.002 SS-FPG-12B1            9-03-81          Corn                       <0.09        2.4 0.2      <0.01      <0.000 SS-FPL-1101            9-03-81          Cabbage                    <0.2         3.3 0.4      <0.03      <0.03
    ~     SS-FPV-11D1            9-03-81          Cantalopes                 <0.03        2.8 0.3      <0.005     <0.03 o

SS-FPG-11DI 9-03-81 Corn <0.1 2.4 0.2 <0.02 (0.01 SS-FPV-11DI 9-03-81 Potatoes <0.07 3.5 0.4 <0.01 <0.007 i SS-FPV-11D1 9-03-81 Squash <0.05 3.6 0.4 <0.007 <0.004 SS-FPV-1101 9-03-81 Tomatoes <0.04 2.3 0.2 <0.006 <0.003 SS-FPV-12F5 9-03-81 Strawberry Plant 1.6 0.6 1011 0.10 0.06 <0.09 SS-FPL-2H1 9-04-81 Cabbage <0.4 3.90.7 <0.05 <0.04 SS-FPG-2H1 9-04-81 Corn <0.08 2.6 0.3 <0.01 <0.007 SS-FPV-2H1 9-04-81 Squash <0.0 7 2.90.3 4.01 <0.006 SS-FPV-2H1 9-04-81 Tomatoes <0.03 1.9 0.2 <0.004 <0.003 SS-FPV-2H1 9-04-81 Potatoes <0.05 4.30.4 <0.008 <0.004

  • All other gamna emitters searched for wem <LLD; typical LLDs are found on Table C-29.

TABLE C-23 CONCENTRATIONS OF GAft1A E!!ITTERS* Ill flEAT SA!1PLES IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/g(wet) 2 sigma STATION N0. SA!1PLE DESCRIPTION K-40 DATE 5 m SS-FPE-12B1 12-19-81 Eggs 0.93 0.09 SS-FPP-12B1 12-19-81 Chicken 2.10.2 SS-FPD-10D1 12-19-81 Duck 2.9 0.3 All other gama emitters searched for were <LLD; typical LLDs are found on Table C-29.

_ .. . _ . _ . _ _ . _ _ _ . . . . . _ . _ _ - ~ . __ _ -- TABLE C-24 CONCENTRATI0llS OF GNt1A EMITTERS

  • IN GA!!E SA!!PLES IN THE VICIllITY OF SUSQUEHAllNA SES j Results in Units of PCi/g(wet) . 2 sigma l STATION 110. SA!1PLE DESCRIPTI0ll K-40 Cs-137 DATE 1

5 SS-GAS-Indicato r** .12-29-31 to Squirrel 2.7 0.3 1.5 0.2 12-30-31 SS-GAD-16B*** 11-30-81 Deer Flesh 2.5 0.3 0.10 0.01

  • All other gama emitters searched for were <LLD; typical LLDs are found on Table C-29.
              **                    Indicator stations are IA, 2A and 15A.                                                                                              !
              ***                  Station code is omitted because no exact station exists; samples are taken based on availability.                                                                                                                        i i

i I ~

TABLE C-25 CONCENTRATIONS OF GNt1A E!!!TTERS* IN VEGETATION IN THE VICINITY OF SUSQUEHAM1A SES Results in Units of pC1/g(wet) 12 sigma STATION NO. SR1PLE DESCRIPTION Be-7 K-40 Zr-95 lb-95 Ce-144 a DATE SS-VGT-754 8-05-81 Vegetation <1.3 7.9 2.1 <0.3 0.4 0.1 <0.9 SS-VGT-853 8-05-31 Vegetation 1.7 0.5 8.lil.2 0.18 0.07 0.3720.06 0.5 0.2

  • All other gania emitters searched for were <LLD; typical LLDs are found on Table C-29.

l

TABLE C-26 CONCENTRATIONS OF GAtt1A EMITTERS

  • IN PASTURE GRASS IN THE VICINITY OF SUSQUEHANNA SES Results in Units of pCi/g(wet) i 2 sigma STATION NO. SAMPLE DESCRIPTION Be-7 K-40 Zr-95 Nb-95 Ru-103 Cs-137 Ce-141 Ce-144

_ DATE SS-PAS-15 A1 1-31-81 (1) Grass SS-PAS-15 A1 2-28-31 (1) Grass SS-PAS-ISAI 3-29-31 (1) Grass SS-PAS-15A1 4-10-81 Grass 1211 17!2 4.2 0.4 8.410.8 1.50.2 0.20.1 1.9 0.3 5.310 .8 SS-PAS-15A1 5-08-81 Grass <1.6 20 3 (0.4 0.7 0.2 <0.2 <0.2 <0.3 <1.1 SS-PAS-15A1 6-05-81 Grass <1.3 1312 0.4 0.2 0.70.1 <0.2 <0.2 <0.3 <1.0 h SS-PAS-15 A1 6-29-81 Grass <1.1 16 2 <0.2 0.30.1 <0 .1 <0.1 <0.3 <1.1 SS-P AS-15 A1 8-05-81 Grass <1.2 16 2 <0.3 <0.2 <0.1 <0.1 <0.2 <0.9 SS-PAS-15A1 9-04-81 Grass 3.10.7 6.811.3 <0.2 0.18 0.07 <0.1 (0.1 <0.2 <0.9 SS-PAS-15A1 10-09-81 Grass 1.3 0.2 3.720 .5 <0.06 <0.04 <0.04 <0.03 <0.08 <0.3 SS-PAS-15A1 11-06-81 Grass 3.7 0.9 1412 <0.2 <0.1 <0.1 <0.1 <0.2 <0.9 SS-PAS-ISA1 12-04-81 Grass 10 1 6.3 0.9 <0.1 <0.1 <0.03 0.07 0.04 <0.1 <0 .+ SS-PAS-7C1(2) 6-30-81 Grass <1.7 17 3 <0.4 0.510.1 <0.2 <0.2 <0.3 <1.3 SS-PAS-7C1 (2) 9-04-81 Grass 1.90.6 1212 <0.2 0.3110.08 <0.1 <0.1 <0.1 <0.4 SS-PAS-8D1 (2) 6- 30-81 Grass 1.2 0.4 26 3 <0.1 0.26 0.07 <0.08 0.07 0.04 <0.2 <0.6 All other gama emitters searched for were <LLO; typical LL0s are found on Table C-29. Indicates that no LLO was calculated for that nuclide in that redia. (1) No sample was collected due to snow cover. (2) Pasture grass is samled frmi SS-PAS-7C1 and SS-PAS-801 durin9 the months milk is not collected.

99 8 97 9 8 88 9 7 8 87 2 00 10 00 01 01 00 23 11 10 10 01 00 11 11 3 2 00 00 00 00 00 00 00 00 00 00 00 00 00 00

             -       i        1        1    2 1      11       12       1 t    11          1  1t     11      1 2     1   1 2 48                                 36 h

T 97 8. 08 41 65 90 8.1 79 77 99 00

8. 7 7
7. 95 97 57 55 10 91 00 0

0 00 0 6. 0 0 O0 12 11 0 0 . 6. 0 11 01 0 0 0 00 77  ; 67 65 89 66 ' 89 66 78 66 90 99 6 00 00 00 00 00 23 11 00 00 00 00 00 00 2 0. d. 2 00 00 00 00 00 00 00 00 00 00 00 00 1 00 00

             -                1        1       1     1!       1        1          1    t        1   11              11  1 a    48       73       09      75       88       80       67     10       55    39     38      98     34   62 R     66       67       54      78       55       56                       78    65     77      55     87   89 S                                                                   12     11 E              00       00       00      00       00       00                       00    00     00      00     00   00 S

A N N A H E U Q S 33 43 8 33 57 23 44 33 43 43 33 43 U 7 00 00 10 00 00 00 12 00 00 00 00 00 22 00 S 3 1 00 00 00 00 00 00 00 00 00 00 F - 1 1 12 1 2 2 i 1 00 t 00 1 00 00 1 2 O s 78 16 9 04 78 28 42 87 43 91 09 11 22 69 Y C 11 32 2. 7 21 46 21 33 33 33 32 33 21 1 12 22 T 00 00 0 00 00 00 00 00 00 00 00 's 0 I N a I C g n . I i 9 2 V s - E 2 C H e T i 3 44 43 33 34 2 5 3 4 4 34 34 55 6 l 00 00 00 00 0 N I

       )

y 5 9 0. 00 6 00 00 00 00

0. 6 00 01 06 00 06 00
0. 5 00 00 00 00 00 00 00
0. 0 00 b

T a r - 1 1 2 1 1 1 1 21 1 S d b 60 02 18 43 42 00 40 30 90 60 21 23 55 20 n E N 7 2 L P ( g 1.< 21 10 21 11

1. < 3. < 2. < 1.< 1< 21 21 31
2. < o
       /         0        00       00      00       00       0        0      0        0     0      00      00     00   0     d
- 1 i                                                                                                                       n C  N S

C p u E o f L L f B A I o e O r T S s a t N i s I n 09 89 09 09 9 88 9 00 88 99 00 D U 0 L

  • 4 10 00 10 10 10 00 01 11 11 00 )1 00 10 1 11 L S n - 1 1 1 1 1 1 1 t 1 2 1 i 1 1 1 1 R K E

T i s 93 38 88 79 98 87 98 07 1 8 37 19 3.1 0 00 11 67 90 l0 l1 52 14 00 11 l a T t 99 3 99 78 89 38 c i I l p N u y E s t e A t R  ; f D A' , L L G < F N e O O r S I T e N P ll ll ll ll ll ll ll ll ll ll ll ll ll ll w O I ii ii ii ii ii ii ii ii ii ii ii ii ii ii r I T R C oo ooss oo ss ss oo oo ss oo ssoo oo ss oo ssoo ooss oo ssoo oo ss ss ss ss ss f o A S pb pb pb pb pb pb pb pb pb pb pb pb pb pb R E ou ou ou ou ou ou ou ou ou ou ou ou ou ou d T D TS TS TS TS TS TS TS TS TS TS TS TS TS TS e N h E c C r N a O e C s s r E 1 1 1 1 1 1 1 1 1 1 1 1 1 1 e t LE 8 8 0 8 8 8 8 8 8 8 8 3 8 3 t PT - - - - - - - - - - - - - - i 1A 7 7 7 7 7 8 8 8 8 7 8 8 8 8 m ND 1 1 1 1 1 1 1 1 1 1 1 1 1 1 e S - - - - - - - - - - - - - - 8 8 3 8 8 8 8 8 8 8 8 8 8 8 a m m a g r e

               .                                                                                                            h 4       4                                 3        4     2      4       5           3     t O     4        5        5       5        2       4         2      D        D     E      F       F      1    G      o N     5        5        1       5        8        0        D      1        1     2      2       2      G    2 2        5        1       1        9       1         3      1        1     1      1       1      7    1    l N       -        -        -       -        -       -         -      -        -     -      -       -       -   -  l O     L        L        L       L        L         L       L      L        L     L      L       L      L    L    A I     0        0        0       0        Q       0         0      0        0     O     0        0     0     0 T     5        5        5       5        S       5         5      5        5     S     5        5      5    5 A       -        -        -       -        -       -         -      -        -     -      -       -       -   -

T S S S S S S S S S S S S S S S S S S S S S S S S S S S S S

  • i
                                                                 . TABLE C-28
;                                RESULTS OF QUARTERLY TLD 11EASURC1ENTS IN Tile VICINITY OF SUSQUEHANNA SES Results in Units of mrem / standard month
       . STATION              ~ JANUARY             APRIL                     JULY                  OCTOBER          . ANNUAL-NO.                TO'                TO                        TO '                    TO             AVERAGE 4

MARCH JUNE SEPTC1BER DECE!EER SS-IDM-152 . .6.45io.80 5.9910.60 6.5610.95 7.16 0.76 6.54 0.96 i

  • SS-IDM-252 5.5710.94 ' 5.98 0.54 6.10 0.23 6.54 0.00 6.05 0.30 l -SS-IDM-253 6.0610.10 6.47 0.41 6.78 0.37 6.9110.93 6.56 0.76 SS-IDM-333 5.5620.24 5.43io.45 6.06 0.90 5.8211.04 5.7220.56 SS-IDM-3S4 6.00to.26 5.9510.39 6.1410.58 -6.46i0.88 6.14 0.46 SS-IDM-451~ '5.25 0.26 5.56 0.27 5.19 0.14 5.72 0.15 5'.43 0.50
  ,         55-I % 453     - 7.15 0.50            6.1610.15               6.26 0.92                 6.77 0.94        6.59 0.92-SS-IDM-551       5.2210.17            5.37 0.12               5.38 0.47                 5.49 0.31-       5.3710.22 SS-IDM-SS4       5.91*0.50            5.81 0.99               6.10 0.49                 6.8510.36        6.17 0.94 SS-IDH-SS7       6.0510.61            5.93 0.67               6.35 0.61                 6.49 0.46        6.22 0.43 j            SS-IDM-6S4     12.6311.19             7.90 1.02              10.65 0.13              10.3711.36         10.3913.33 j          SS-IDM-751       5.9610.38            5.60 0.65               5.29 0.33                 5.0010.48        5.66 0.53 SS-I W 7S3       9.0211.08            5.02 0.43               7.80tl.01                 8.46 0.71        7.73 2.79 SS-IDM-852.      7.1411.01           '6.26 0.39               6.58 0.57                 6.57 0.64        6.6410.73 1

S5-I % 951 6.38 0.80 6.00 0.63 5.52 0.31 6.2310.00 6.0510.77

        .SS-IDM-10S1         5.6910.51            5.34 0.24               5.8610.53                 6.43 0.17        5.96 0.65 SS-IDM-11S2      5.7120.31            5.53 0.41               5.84 0.41                 5.24 0.75        5.59 0.52 SS-IDM-1153      5.84 0.61            5.13 0.32               5.99 0.33                 6.1010.35        5.73 0.82 SS-IDM-1253      7.04 0.41            6.83 0.33               7.5920.47                 7.4711.05        7.2320.71 ~

j SS-IDM-13S2 6.4410.75 6.68 0.07 6.69 0.68 7.06 0.38 6.7210.51.

.SS-IDM-14S2 6.2010.35 (1) - - - 6.2020.35 i SS-IDM-14SS - 5.92 0.72 11.0721.61 7.55il.12 8.13 5.26
        ' SS-IDM-1553        6.52 1.01            6.5330.69               8.06 0.23                 7.64 0.72        7.1911.57
        'SS-IDH-1554                 -                  -

5.5710.31 (2) - 6.11 0.30 5.84 0.76

            $$-IDM-1651      6,5010.58            6.79 0.90               7.22i0.48                 7.20 0.59        6.93t0.69
            $$-IDM-1A1
                         ^

5.4810.39 6.3720.41 6.43 0.94 6.72 0.82 6.2611.08 SS-IDM-6 A3 5.6811.08 6.4610.53 6.69 0.81 6.7410.68 6.3910.93

            $5-IDH-7Al       5.7910.93            6.0010.56               6.09 0.74                 6.36 0.90        6.06*0.47 SS-IDM-11A2      4.4010.20            4.5710.31               5.6210.66                 5.9720.43        5.1411.55 :

SS-IDM-15 A3 5.57 0.31 6.1720.28 6.30io.99 6.5410.73 6.1510.83 i

-SS-IDM-16A2 4.7010.24 5.00 0.40 5.8520.33 6.34 tl.08 5.6711.39 i

107

3 I Tt.BLE C-28 (cont.) 4 RESULTS OF QUARTERLY TLD NEASUREMEliTS IN THE VICINITY OF SUSQUEHANNA SES Results in Units of mrem / standard month STATION JANUARY -APRIL JULY OCTOBER ANNUAL NO. TO TO TO TO AVERAGE MARCH JUNE SEPTEMBER DECEMBER u. SS-IDM-283 5.44 0.32 5.8710.31 6.8510.46 6.7110.98 6.2211.35 1-SS-IDM-783 5.56 0.65 6.33 0.31 6.3320.49 6.99 0.11 6.3011.17

           -SS-IDM-881           5.0311.14         6.05t0.40                    5.7220.59                  6.41 0.54                       5.8011.17
SS-IDM-9B1 5.2920.65 5.6910.77 5.4920.93 6.3010.25 5.6910.87 SS-IDM-1082 4.52 0.63 4.6521.10 5.1010.32 5.51 0.43 4.9510.90 a SS-IDM-1083 -

5.3810.69(3) 5.3510.57 6.0410.79 5.59 0.78 -

          - SS-IDM-12B4          5.70 0.43         5.99.+0.49                   6.0210.27                  6.5510.46                       6.07 0.71
;           SS-IDM-16B1'         5.21 0.72         5.36 0.49                    5.3110.45                  5.9010.34                       5.45t0.62 l           SS-IDH-ID2           5.54t0.57         6.0210.49                    6.3610.90                  7.13 0.26                     . 6.26*1.34 SS-IDM-301           6.3910.72         7.06 0.43'                   7.3620.70                  7.31 0.86                       7.0310.89 SS-IDM-802           6.0110.12         6.34 0.68                    6.08 0.75                  6.79 0.56                       6.31*0.71 SS-IDH-901           6.4120.67         6.08 0.28                    6.42 0.51                  6.7010.34                       6.40 0.51-SS-IDM-10D2          6.1110.97         5.3310.28                    6.63i0.48                  6.')710.41                      6.2611.43 SS-IDM-12D3          6.4311.02         6.7410.41                    6.5620.72                  7.22 0.58                       6.74 0.69 SS-!DM-1El           5.1710.98         5.2910.57                    5.4410.48                  6.0910.42                       5.5010.82 a            SS-IDM-4E1           6.0710.57         6.2810.65                   6.4320.74                   7.0210.58                       6.45 0.82 SS-I % 5E2           6.7221.12         6.4310.62                   7.15 0.40                   6.7411.05                       6.76 0.59 i            SS-IDM-6El           7.49 0.57         6.9510.96                   7.7211.28                   8.13t0.08                       7.5720.98         ;

SS-I W 7El 5.74t0.59 5.84t0.48 6.7410.89 7.3910.70 6.4311.57 SS-IDM-11El 4.98t0.89 5.0010.92 5.34i0.41 5.59t0.62 5.23 0.59 SS-IDM-12E1 5.6810.81 6.3410.45 6.4010.90 6.05 0.47 6.12 0.66 SS-IDM-13E4 6.4010.34- 6.30i0.44 6.4611.17 7.0510.22 6.5510.68 l SS-IDM-14E1 6.6911.63 6.16 0.42 6.41 0.10 6.60t0.92 6.47 0.47 SS-IDH-2F1 5.3210.29 6.44t0.49 5.65 0.49 6.8321.84 6.06 1.39 l.

SS-IDM-3F1 5.5710.47 6.6721.16 5.66 0.30 6.54t0.34 6.11il.15 SS-IDM-7F1 5.2810.39 6.3110.20 (4) 6.4310.52 6.0121.26 i SS-IDM-12F2 6.4110.74 6.6610.39 6.54 0.24 7.0111.21 6.6610.52 f

i SS-IDM-15F1 6.15tl.28 7.02t0.58 6.80 1.03 7.3110.64 6.8220.99 l SS-IDH-16F1 5.97*0.18 6.2110.36 6.3520.59 6.5821.03 6.2810.51 SS-IDM-3G3 6.7710.67 6.6710.33 6.6610. " 7.16 1.32 6.02 0.47 1 SS-IDM-3G4 6.2110.22 6.72il.21 6.55 0.93 6.5810.73 6.5210.43

  • i 1

108 I ew,,,- e n -n na-- ,, e a_- ,.-~v -- r -,.w,<- . , , , -

                                                                                                   . , - .      .---n--y,, -. - . , , ,,    p. ,-  --  , --,

i l 1 TABLE C-28 (cont.) RESULTS OF QUARTERLY TLD MEASUREMEi4TS IN THE VICINITY OF SUSQUEHAfUlA SES Results in Units of mrem / standard month STATION JANUARY APRIL JULY OCTOBER AN!iUAL NO. TO TO TO TO AVERAGE MARCH JUi4E SEPTEftBER DECEM3ER SS-IDM-4G1 5.8210.21 6.2111.24 5.59 0.39 6.7010.17 6.08 0.97 SS-IDM-7G1 6.3110.23 6.6710.20 6.32t0.57 7.11 0.31 6.60io.75 SS-IDM-12G1 5.0010.57 4.73 0.30 5.02 0.37 5.5010.09 5.0610.64 SS-IDM-12G4 6.28t0.52 6.8711.26 6.8010.69 7.03 0.29 6.7510.65 SS-IDM-7H1 4.5210.49 4.4510.09 4.44i0.54 4.8310.50 4.56i0.37 SS-IDM-8H1 5.41t0.57 5.05!0.71 5.39 0.13 5.9810.41 5.4610.77 Average 6.0212.25 6.05tl.31 6.3512.14 6.6611.60 Grand Average 6.27 1.92 No result because sampling station was not in operation. Station 1452 was moved to 1455 on 6-29-01. Station began operation on 6-29-81.

l. Station began operation on 4-05-81.

l TLD lost in field. I 109

TABLE C-29 TYPICAL LLDs* FOR GAfMA SPECTR0fETRY SURFACE WELL POTABLE AIR WATER WATER WATER SEDI!1ENT PRECIPITATION HILK NUCLIOE (pC1/1) (pC1/1) (pC1/1) (pC1/9-dry) PARTgCULATEg) (10- pC1/m (pC1/1) (pC1/1) Be-7 4.9 5.2 4.8 0.2 2.0 6.3 9.1 K-40 8.0 6.0 7.9 ** 9.2 ** 7.4 Cr-51 5.0 5.3 5.8 0.2 10 6.1 9.9 Mn-54 0.5 0.5 0.5 0.03 0.8 0.5 1.1 Co-57 0.3 0.3 0.3 0.02 0.5 0.4 0.6 00-5 8 0.5 0.5 0.5 0.02 0.7 0.6 1.2 Fe-59 1.1 1.2 1.1 0.05 1.1 1.3 3.6 Co-60 0.6 0.6 0.6 0.03 0.9 0.6 1.4 Zn-65 1.1 1.1 1.1 0.06 1.5 1.2 3.5 Zr-95 0.9 0.9 0.9 0.07 1.6 1.1 2.1 Nb-95 0.6 0.7 0.7 ** 1.0 0.8 1.4 ZrNb-95(I) - 0.7 0.5 - - - - Ho-99 1.7 3.5 3.2 0.1 6.7 7.6 13 Ru-103 0.6 0.7 0.6 0.02 1.0 0.7 1.2 Ru-106 4.6 4.4 4.4 0.2 6.8 4.9 8.4 Ag-110m 4.4 0.5 0.5 0.03 0.8 0.5 1.0 Sb-125 1.5 1.5 1.5 0.06 2.4 1.6 2.6 Te-129m 19 21 19 0.8 29 23 45 I-131 0.9 1. 2 1.7 0.2 2.3 1.5 2.5 I-133 100 - 110 - - - - Cs-134 0.5 0.5 0.5 0.03 0.6 0.5 0.9 Cs-II3 0.7 0.9 0.7 0.03 0.8 1.1 2.2 Cs-137 0.5 0.5 0.5 ** 0.8 0.5 1.1 Ba-140 3.1 3.6 3.2 0.2 6.0 4.7 8.8 La-160 1.0 1.2 1.0 0.04 0.8 1.5 1.8 Bala-140 - 2.2 2.0 - - - - Ce-141 0.7 0.7 0.8 0.04 1.4 0.9 1.4 Ce-144 2. 7 2.7 2.8 0.1 4.6 2.8 4.7 Ra-226 1.0 1.0 1.0 ** 1.9 1.2 1.9 Th-232 1.6 1.8 1.8 ** 2.3 1.7 3.0 Np-2 M 9.8 19 14 0.8 28 47 87 110

TABLEC-29(cont.) TYPICAL LLDs* FOR GAlfiA SPECTROMETRY FOOD MEAT GAME SOIL PASTURE FISH PRODUCTS (Flesh) (Flesh) (Flesh) VEGETATION GRASS NUCLIOE (pCi/g-wet) (pC1/g-wet) (pCi/g-wet) (pC1/g-wet) (pCi/g-wet) (pC1/g-dry) (pC1/g-wet) B2-7 0.6 0.02 0.05 0.1 0.3 1.1 1.2 K-40 ** - ** ** ** ** ** Cr-51 0.07 0.04 0.06 0.2 0.3 0.6 0.3 Mn-54 0.006 0.003 0.005 0.009 0.03 0.07 0.03 Co-57 0.003 0.002 0.004 0.01 0.02 0.04 0.03 Co-58 0.007 0.003 0.006 0.01 0.03 0.07 0.03 Fe-59 0.02 0.009 0.01 0.03 0.07 0.2 0.07 Co-60 0.006 0.004 0.008 0.009 0.03 0.08 0.04 Zn-65 0.02 0.008 0.01 0.02 0.07 0.02 0.07 Zr-95 0.01 0.006 0.01 0.02 0.06 0.2 0.06 Nb-95 0.009 0.004 0.006 0.01 0.05 - 0.04 ZrNb-95 III - - - - - - - Mo-99 0.5 0.2 0.4 0.5 0.3 0.3 0.3 Ru-103 0.008 0.004 0.006 0.02 0.04 0.08 0.04 Ru-106 0.05 0.02 0.04 0.08 0.3 0.7 0.3 Ag-110m 0.006 0.003 0.005 0.02 0.04 0.07 0.03 Sb-125 0.02 0.007 0.01 0.03 0.08 0.2 0.06 Te-129m 0.3 0.003 0.2 0.5 1.3 2.7 1.2 I-131 0.03 0.02 0.02 0.05 0.08 0.1 0.08 I-133 - - - - - - 21 Cs-134 0.005 0.002 0.005 0.008 0.04 0.07 0.03 t Cs-136 0.02 0.01 0.01 0.02 0.06 0:1 0.05 Cs-137 0.01 0.003 0.005 ** ** 0.08 0.03 I Ba-140 0.07 0.05 0.06 0.1 0.3 0.5 0.2 La-140 0.02 0.009 0.01 0.02 0.06 0.1 0.06 Bala-140 - - - - - - - Ce-141 0.009 0.006 0.01 0.03 0.05 - 0.08 Ce-144 0.03 0.01 0.03 0.05 0.1 0.09 0.3 Ra-226 0.01 0.005 0.01 0.02 ** 0.02 0.06 Th-232 0.02 0.008 0.02 0.03 ** 0.02 0.09 Np-239 - 0.9 3.1 3.5 1.7 1.2 1.5 Decay cormcted to sample stop date. The large LLDs are due to short half-life. Indicates a positive concentration was measund in all sanples analyzed. Indicates that no LLD was calculated for that nuclide in that media. (1) Not decay corrected. 111

s k - _ _ i i APPENDIX D SYNOPSIS OF ANALYTICAL PROCEDURES d

GROSS ALPHA ANALYSIS OF SAMPLES

   ' Total Water (AO)

A 250 ml aliquot is evaporated to dryness and transferred to a preweighed, 2" x 1/4" ringed planchet and reweighed. The planchet is then counted in a low background gas-flow proportional counter. Seif-absorption corrections are made based on the measured residue weight and calculated thickness. The calibration standard used is Pu-239.. A 250 mi sample of distilled water is evaporated in the same manner and used as a blank. Sediment (A9) A 200 mg portion of finely divided sedimer;t is . slurried with water, transferred to a planchet and dried. The sample is counted in a low background, gas-flow propor-tional counter. Self absorption corrections are made on the basis of the weight of material counted. An empty planchet is prepared with water and used as a blank. Air Particulates (AE) A 20% aliquot of the leached sample is evaporated to dryness on a preweighed, 2" x 1/4", ringed, stainless steel planchet and the planchet is reweighed. The planchet is counted in a low background, gas-flow proportional counter. Self absorption cor-rections are made on the basis of residual weight. An unused filter paper is pre-pared in the same manner and counted as the blank. Calculations of the results, the two sigma error and the lower limit of detection (LLD). Result (pCi/vol or mass) = ((S/T) - (B/t)) / (2.22 V E TF) 2 2 sigma error (pCi/vol or mass) = 2 ((S/T ) + (B/t2))1/2 / (2.22 V E TF) LLD (pCi/vol or mass) = 4.66 (B1/2) / (2.22 V E TF t) Where: S = Gross counts of sample including blank B = Counts of blank E = Fractional Pu-239 counting efficiency T = Number of minutes sample was counted t = Number of minutes blank was counted V = Volume of aliquot (liters, cubic meters or grams) TF = Transmission factor (based on net weight of sample in counting planchet) 115

GROSS BETA ANALYSIS OF SAlfLES Total Water (BO) A 250 ml aliquot is evaporated to dryness and transferred to a preweighed, 2" x 1/4" ringed planchet and reweighed. The planchet is then counted in a low background gas-flow proportional counter. Self-absorption corrections are made based on the measured residue weight and calculated thickness. The calibration standard used is Sr Y-90. A 250 ml sample of distilled water is evaporated in the same manner and used as a blank. Calculations of the results, the two sigma error and the lower limit of detection (LLD). Result (pCi/l) = ((S/T) - (B/t)) / (2.22 V E TF) 2sigmaerror(pCi/1) = 2 ((S/T2 ) + (B/t 2))1/2 / (2.22 V E TF) LLD(pCi/1) = 4.66 (B1/2) / (2.22 V E TF t) Where: S = Gross counts of sample including blank B = Counts of blank E = Fractional Sr Y-90 counting efficiency T = Number of minutes sample was counted t = Number of minutes blank was counted V = Sample aliquot size (liters) TF = Transmission factor (based on net weight of sample in counting planchet) Air Particulates (BD) After a delay of two to five days, allowing for the radon-222 and radon-220 (thoron) daughter products to decay, the filters are counted in a gas-flow proportional counter. An unused filter paper is counted as the blank. Calculations of the results, the two sigma error and the lower limit of detection (LLD). Result (pCi/m3) = ((S/T) - (B/t)) / (2.22 V E) 2 2 2 sigma error (pCi/m3 ) = 2 ((S/T ) + (B/t ))1/2 / (2.22 V E) LLD (pCi/m3 ) = 4.66(B1/2) / (2.22 V E t) Where: S = Gross counts of sample including blank B = Counts of blank E = Fractional Sr-90-Y-90 counting efficiency T = Number of minutes sample was counted t = Number of minutes blank was counted V = Sample aliquot size (cubic meters) 116

ENVIRONENTAL D0SIMETRY (D1) By RMC definition, a thermoluminescent dosimeter (TLD) is considered one end of a capillary tube containing calcium sulfate (Tm) powder as the thermolumi-nescent material. This material was chosen for its characteristic high light output, minimal thermally induced signal loss (fading), and negligible self-dosing. The energy response curve has been flattened by a conplex multiple element energy compensator shield supplied by Panasonic Corporation, manufac-turer of the TLD reader. There exists four dosimeters per station sealed in a polyethylene bag to demonstrate : integrity at the time of measurement, and for visualization of the sample placenent instructions. The zero dose is determined from TLDs located in the lead shield found at RMC, Philadelphia. Following the predesignated exposure period the TLDs are placed in the TLD reader. The reader heats the calcium sulfate (Tm) and the measured light emission (luminescence) is used to calculate the environmental radiation - exposum. Data are normalized to standard machine conditions by correcting machine settings to designated values before readout. Data am also corrected for in-transit dose using a set of TLDs kept in a lead shield in the field, enposed only during transit. The average dose per exposure period, and its associated error is then calculated. The Cs-137 source is used to expose TLDs as a reference sample. An absorbed dose in tissue is detennined using the 0.955 rad / Roentgen conversion factor and dose equivalent (mrem) by using a quality factor of 1. Calculation of results and two sigma error: Gross TLD (1) = (TLD(1)-DO(1)) x CF (i) x CF (ins) x 0.955 mrad /mRoentgen ITD = NET (site 9) - (NET (RMC 0) (D(sta) / D (RMC 0))) NET TLD(i) = gross TLD(i) - ITD n AVG = ((sigma NET TLD) / n) (D(STD) / D (EX)) i=1 ERROR (95%CL) = t(n-1) (sigma NET TLD (1) / n) (D(STD) / D (EX)) whem: GrossTLD(i) = Individual TLD reading corrected to standard instrunent conditions TLD(1) = Gross mading of dosimeter i

                              =

NET TLD(i) Net dose obtained during exposure period ig*ge field CF(ins) = Correction factor of reader = (6.21) (ELS- ) ELS = External light source DO(i) = Zero for dosimeter, i CF(i) = Calibration factor for dosimeter i ITD = In-transit dose NET site)0 = Mean of n dosineters in site lead shield NET RMC)0 = Mean of n dosimeters in RMC lead shield 117

i' D(sta) = Exposure period of station D(RMCO) = Exposure period of RMC0 AVG = Mean exposure per standard exposure period at a given station n = Number of readings D(EX) = Days exposed D(STD) = Days in standard exposure period t(n-1) = T-distribution (student) factor for 95% CL sigma NET TLD(i) = Standard deviation of n readings of liET TLD(1) ERROR = The 95% confidence limit error of AVG a 1 i 4 i I i 118 l ~ . .- - .

GAMMA SPECTROMETRY OF SAMPLES Water (G1) Four liters of sample is reduced to 100 ml and sealed in a standard container. The container is counted with a Ge(Li) detector coupled to a multi-channel' pulse-height - analyzer. The counting time is 50,000 seconds. Milk (G7) A three liter aliquot is dried at 175 C, ashed at 500 C until no carbon residue is present, compressed and sealed in a standard container. The container is counted with a Ge(Li) detector, coupled to a multi-channel pulse-height analyzer. The counting time is 50,000 seconds. Dried Solids (G8) A large quantity of the sample is dried at a low temperature, less than 100 C. A 100 gram aliquot (or the total sample if less than 100 grams) is taken, compressed to unit density and sealed in a standard container. The container is counted with a Ge(L1) detector, coupled to a multi-channel pulse-height analyzer. The counting time is 50,000 seconds. Air Dried Solids (GA) A large quantity of sample is air dried, compressed to a known geometry and sealed in a standard container. The container is counted with a Ge(Li) detector, coupled to a multi-channel pulse-height analyzer. The counting time is 50,000 seconds. Air Particulate (GB) All samples received for the month are mixed and sealed in the standard container. The container is counted with the high resolution Ge(Li) detector, coupled to a multi-channel pulse-height analyzer. Calculation of results, two sigma error and the lower limit of detection (LLD). The data are obtained by smoothing the spectrum to minimize the effects of random statistical fluctuations. Peaks are identified by changes in the slope of the gross spectrum. The net area, in counts, above the baseline is detennined. The i calculations of the _results, two sigma error and the lower limit of detection (LLD) l for each nuclide are then expressed in activity (pCi) per unit volume or mass (liters or grams). RESULT = ((S/T) - (B/t)) / (2.22 E V F) (pCi/vol. mass) 2 2 SIGMA ERROR = ((S/T ) + (B/t ))1/2 / (2.22 E V F) (pCi/vol or mass) l 119

LLD = 4.66 (6 S)1/2 / (2.22 E V F T) (pCi/vol. or mass) where: S = Net area, in counts, of sample (Region of spectrum of interest) B = Net area, in counts, of background (Rogion of spectrum of interest) T = Number of minutes sample was counted t = Number of minutes background was counted E = Detector efficiency for energy of interest V = Sample aliquot size (liters, cubic meters or gramd F = Fractional gamma abundance (specific for each emitted nuclide)

          =  Channel number Q

120

AllALYSIS OF SAIFLES FOR TRITIUM Water (H2) A 15 ml aliquot of the sample is vacuum distilled to eliminate dissolved gasses and non-volatile matter. The distillate is frozen in a trap cooled with a dry ice-isopropanol mixture. Eight (8) ml of the distillate are mixed with ten (10) ml of Insta-Gel liquid scintillation solution. The sample is then counted for tritium in a liquid scintillation counter. A sample of low tritium (< 50 pCi/l) water is vacuum distilled as a blank and is counted with each batch of samples. In the calculation of the result it is assumed that the condensated and original sanple are of equivalent volumes. The volume change associated with the removal of dissolved gases and non-volatile matter is not significant compared to the other errors in the analysis. Calculations of the results, the two sigma error and the lower limit of detection (LLD). RESULT (pC1/1) = ((S/T) - (8/t)) / (2.22 V E) 2 2 2SIGMAERROR(pCi/1) = 2((S/T)+(B/t))1/2 / (2.22 V E) LLD (pCi/l) = 4.66 (B1/2) / (2.22 V E t) where: 5- = Gross counts of sample including blank B = Counts of blank E = Fractional H-3 counting efficiency T = Number of minutes sample was counted t = Number of minutes blank was counted V = Sample aliquot size (liters) I l 121

AllALYSIS OF SAliPLES FOR 10DillE-131 tiilk or Water (10) The initial stable iodide concentration in milk is determined with an iodide ion specific electrode. Thirty milligrams of stable iodide carrier is then added to four (4) liters of milk. The iodide is removed from the milk by passage through ion-exchange resin. The iodide is eluted from the resin with sodium hypochlorite, and purified by a series of solvent extractions with the final extraction into a toluene phase. The toluene phase is mixed with a toluene-based liquid scintillation solution. The sample is then counted in a beta-gated gamma coincidence detector, shielded by six inches of steel. Distilled water is used as a blank. The yield is calculated from stable iodide recovery based on the recovered volume. Results are corrected for decay from the sampling time to the middle of the counting period, using a half-life value for I-131 of 8.06 days. The data are obtained by smoothing the spectrum to minimize random statisti-cal fluctuations. Iodine-131 is identified by changes in the slopa of the gross spectrum, and noting the net area, in counts, above the baseline pro-hetion. The calculations of the results, the two sigma error and the lower limit of detection (LLD) for iodine-131 are then expressed in activity (pCi) per unit volume (liter). Calculation of results, two sigma error and the lower limit of detection fl Lle,. RESULT = S / (2.2P. E V Y F T) (pCi/1) 2 SIGl1A ERROR = 2 (S+B)l/2 / (2.22 E V Y F T) (pCi/1) LLD = 4.66 (BI! ) / (2.22 E V Y T) (pCi/1) where: S = Sample counts in I-131 peak B = Baseline counts in region of I-131 peak T = flumber of minutes sample was counted E = I-131 counting efficiency V = Sample aliquot size F = Fractional garrna abundance (0.824 for I-131) Y = Chemical yield of Iodine i Air Cartridges (II) i An iodine adsorber composed of charcoal is emptied into an aluminum can (6 cms high by 8 cms in diameter) and counted with a llaI(Tl) detector, coupled to a multi-channel pulse height analyzer. 122

The data am obtained by smoothing the spectrum to minimize random statistical fl uctuations. Iodine-131 is identified by changes in the slope of the gross spectrum, and noting the net area, in counts, above the baseline projection. The calculations of the msults, the t.fo sigma error and the lower limit of detection (LLD) for iodine-131 are then expressed in activity (pCi) per unit volume. RESULT 3

           =

S / (2.22 E V F T) (pCi/m )

                   =

2(S+B)1/2 / (2.22 E V F T) 2 SIG'y) ERROR (pCi/m LLD 4.66(.63(Q1/2)g)1/2 / (2.22 V E F T) (pCi/m'3=) where: S = Sanple counts in I-131 peak B = Baseline counts in region of I-131 peak T = Number of minutes sample was counted Q = Channel number (36 for I-131) E = I-131 counting efficiency V = Sample aliquot size F = Fractional gamma abundance (0.824 for I-131) l { i 123

ANALYSIS OF SAMPLES FOR STROUTIUM-89 AND -90 Total Water (SD, TO) A two liter aliquot of sample is used. Stable strontium carrier is added to the liquid to facilitate chemical separation of Sr-89 and -90, and to determine the strontium recovery. Strontium concentration and purification is ultimately realized by at least two precipitations of strontium nitrate in concentrated nitric acid. Additional iron / rare earth hydroxide precyitations and barium chromate separations are performed to remove suspected interfering nuclides. The purified strontium is converted to a carbonate for weighing and counting. Soon after the separation, the sample is counted in a low-background gas-flow proportional counter. After about 14 days, the sample is recounted, then Sr-89 and -90 activities are calculated on the basis of Y-90 ingrowth and Sr-89 decay. A sample of distilled water is used as a blank. Milk (S4, T4) A one and half liter aliquot of milk is ashed to destroy organic material and tL:a dissolved in concentrated mineral acid. Stable strontium is added to the eluted liquid or dissolved ash to facilitate chemical separation of Sr-89 and -90, and to determine the strontium recovery. Strontium concentration and purification is ultimately realized by at least two precipitations of strontium nitrate in concentrated nitric acid. Additional iron / rare earth hydroxide precipitations and barium chromate separations am performed to remove. suspected interferring nucl ides. The purified strontium is converted to a carbonate for weighing and counting. Soon after the separation, the sample is counted in a low-background gas-flow proportional counter. After about 14 days, the sample is recounted, then Sr-89 and -90 activities are calculated on the basis of Y-90 ingrowth and . Sr-89 decay. A sample of distilled water is used as a blank. Sediment (S6, T6) after being dried. Stable strontium Sediment carrier is samples added to are leached chemical facilitate with hcl and HN0, ion of Sr-89 and -90 and for determi-isolat nation of the strontium recovery in the procedure. Strontium concentration and purification is ultimately realized by at least two precipitations of strontium nitrate in concentrated nitric acid. Additional hydroxide precipitations and bar-ium chromate separations are performed. The purified strontium is converted to a carbonate for weighing and counting. Gross beta counts are made soon after the strontium isolation and again after a 14 day interval and Sr-90 and Sr-89 activities are calculated on the basis of appropriate Sr-89 decay and Y-90 ingrowth equations. A sample of distilled water is used as a blank. Organic Solids (S8, T8) A 250 g wet portion of the sample is ashed, then dissolved in concentrated nitric or mineral acid. Stable strontium carrier is added to the dissolved sample to facil-itate chemical separation of Sr-89 and -90, and to determine the strontium recovery. Strontium concentration and purification is ultimately realized by at least two pre-cipitations of strontium nitrate in concentrated nitric acid. Additional iron / rare earth hydroxide precipitations and barium chromate separations were performed. The purified strontium is converted to a carbonate for weighing and counting. Soon after the separation, the sample is counted in a low-background gas-flow proportional counter. After about 14 days, the sample is recounted, then Sr-89 and -90~ activities am calculated on the basis of Y-90 ingrowth and Sr-89 decay. A sample of distilled water is used as a blank. 124

A Air Particulates (SA,TA) Air particulate filters are leached with hcl and HH0 Stable strontium carrier is added to facilitate chemical isolation of Sr-89 atld -90 and for determination of the strontium recovery. Strontium concentration and purification is ultimately malized by at least two precipitations of strontium nitrate in concentrated nitric acid. Additional iron / ram earth precipitations and barium chromate separations

 . are performed to remove suspected interfering nuclides. The purified strontium is converted to a carbonate for weighing and counting. Gross beta counts are made soon after the strontium isolation and again after a 14 day interval and Sr-90 and Sr-89 activities are calculated on the basis of appropriate Sr-89 decay and Y-90 ingrowth equations. Unused filter papers are used as a blank.

Calculations of the results, the two sigma errors and minimum detectable levels (MDL) for Sr-89, -90 are expressed in activity (pCi) per unit volume (liter) or mass (gram). RESULT Sr-90 = ((Z(S1-B1) - (S2-B2)) / (2.22 K V E9 Y T) (pCi/vol. or mass) 2 2 2 SIGMA ERROR Sr-90 = 2 (Z (Sl+B1) + S2+B2)1/2 / (2.22 (K )1/2 V E9 Y T) (pCi/vol or mass) MDL Sr-90 = (-9 -6(2 B2+Z(S1-B1) + 2.25 + Z2 (Sl+B1))1/2 / 2 K) / (2.22 V E9 Y T) (pCi/vol. or mass) RESULT Sr-89 = (F(S1-B1) + H(S2-B2)) / (2.22 V E8 Y T exp. ( .693t4/52.7)) (pCi/vol. or mass) 2 SIGft1 ERROR Sr-89 = 22(F (31,gy) # 2g (S2+B2))1/2 / (2.22 V E8 Y T exp. ( .693t4/52.7) (pCi/vol or mass) MDL Sr-89 = (F(X-B1) + H(S2-B2)) / (2.22 V E8 Y T exp. ( .693t4/52.7)) (pCi/vol. or mass) where: Sr-89(1) = Sr-89 counts on first count Sr-89(2) = Sr-89 counts on second count S r-90 = Counts of Sr-90 Y-90(1) = Counts of Y-90 on first count Y-90(2) = Counts of Y-90 on second (after equil.) S1 = Sr-89(1) + Sr-90 + Y-90(1) + B(1) S2 = Sr-89(2) + Sr-90 + Y-90(2) + B(2) B1 = Background counts in first count B2 = Background counts in second count t1 = Time in hours from separation time to S1 t2 = Time in days from separation time to S2 t3 = Time in days from S1 to S2 t4 = Time in days from sampling date to separation date El = 1 - exp ( .693t1/64 hours) E2 = 1 - exp ( .693t2/2.667 days) Z = exp ( .693t3/52.7 days)

                        =

R E9/EY H = (1 + E1/R) /K 125

K -= Z (E1/R + 1) (E2/R) F = 1 - (Z/K) - Z (E1/KR)

                =             2 C               (-9 F B1) - 9 H2 (S2+B2) + (F B1) - 2 F H B1 S2+2 F H B1 B2 2          ?                  +(H(S2-B2))2 B       =- 2 F H (S2-B2) - (2 F B1) - 9 F-2
       'X       =       ((B2_4p2     C)    - B) / =(2 F ).

.f E9 = Counting eff, of Sr-90 .3590. .7082 X (Wt. in g of strontium carbonate) EY = Counting eff. of. Y-90 = .4380 .1337 X (Wt. in 9 of strontium carbonate) E8 = Counting eff of Sr-89. = .4568 .2060 X (Wt. in 9 of-strontium carbonate) T = Number of minutes sample and blank were counted Y = Yield 1- 'V = Sample aliquot size (liters, cubic meters or grams) 6 i 6 W i t i 126

I APPEllDIX E l RESULTS OF THE EPA If4TER-LABORATORY C0f4 PARIS 0f1 PROGRAF 4

IllTER-LABORATORY C0f1 PARIS 0ft PROGRAM RMC participates in the EPA radiological interlaboratory comparison (cross check) program. This participation includes a number of analyses on various sample media as found in the Susquehanna SES REf1P. As a result of participation in the program an objective measure of analytical precision and accuracy as well as a bias esti-mation of Rl4C results is obtained. Of the 113 analyses performed, 99 fell within the EPA mean and standard deviation. Reference 16 discusses any discrepancies be-tween the data. Tables E-1, E-2, E-3, E-4 and E-5 sunnarize the results of the 1981 samples.

                                                                                        \

129

TABLE E-1 INTER-LABORATORY COMPARIS0NS GROSS ALPHA AND BETA IN WATER (pCi/ liter) and AIR PARTICULATES (pCi/ filter) SAMPLE RMC EPA All Participants DATE RMC # TYPE ANALYSIS MEAN s.d. MEANis .d. MEAN s.d. Jan 43613 Water a 1012 95 93 1981 B 40 3 44 5 44i6 March 53663 APT a 33 1 30 8 32+5 1981 S 742(a) 50 5 56 11 March 54441 Water a 26 3 25 6 24 6 1981 S 31 2 25 5 2815 April 54841 Water a 64 7 91 23 76 24 1981 S 134 9 141 7 140 91 May 55883 Water a 25 2 21 5 19i5 1981 6 15 2 14 5 16 4 June 56994 APT a 30 2 28 7 32i6 1981 8 7915 (a) 54 5 64 10 July 57789 Water a 19 3 22 6 13 5 1981 8 16 1 15 5 17 4 Sept 60388 Water a 48 4 33 8 28 8 1981 S 26 1 28 5 25i6 Sept 60776 APT a 27 3 25 6 26 6 1981 8 63 7 51 5 61 10 Oct 62491 Water a 52 5 80 20 70 17 1981 s 106 3 111 6 103 15 Nov 64277 Water a 24 2 21 5 20 5 1981 s 21 1 23 5 23i5 (a) Investigation confirmed results. The low standard deviation indicates good agreenent among the three samples that RMC received. Gross alpha < s spec and strontium-90 analyses of these samples agreed with EPA mean, i,. sss beta discrepancy between RMC and the EPA is due to either contaminattu, at RMC or an error in preparation by the EPA. I 131

TABLE E-2 INTER-LABORATORY COMPARIS0NS GAffiAll) SAMPLE RMC EPA All Participants DATE RMC # TYPE IS0 TOPE MEANis.d. MEAN s.d. MEAN:s.d. Jan 43514 tiilk I-131 <203 (a) 26 10 26 6 1981 Cs-137 4213 43 9 42 7 Ba-140 <177 0 45 K 1647 0 1550 134 1529 155 Feb 44441 Water Cr-51 <67 0 49 11 1981 Co-60 25*1 25 5 25 4 Zn-65 8911 85 5 89 11 Ru-106 <28 0 50143 Cs-134 35 2 36 5 33 5 Cs-137 51 4i5 52 March 44815 Food I-131 103 6 119 12 123 13 1981 Cs-137 s'9 2 5315 53 6 Ba-140 <51 0 0 K 2933 0 2640 132 2749 311

  !! arch 53663      APT            Cs-137           14 1            14 5          1614 1981 April   54841      Water          Co-60            <4                0              0 1981                             Cs-134           12 3            10 5          10 3 Cs-137           16 1            15 5          15 3 May     55248      Milk           I-131            2412            26 6          27 7 1981                             Cs-137           21 2            22 5          23 3 Ba-140           <26               0               0      -

K 1777 77 1559 78 1563 104 June 56246 Water Cr-51 < 39 0 15 23 1981 Co-60 17 3 17 5 17 3 Zn-65 <6 0 0 Ru-106 <27 15 5 12 9 Cs-134 20 2 21 5 20 3 Cs-137 30 2 31 5 31 5 June 56994 APT Cs-137 15 4 1615 20 5 1981 July 57331 Food I-131 78 8 82 8 87 15 1981 Cs-137 43 1 45 5 46 6 Ba-140 0 0 0 K 2739 68 26401172 2819i323 132

TABLE E-2 (cont.) IllTER-LABORATO COMPARIS0flS t GAf1MA , SAMPLE R!tC EPA All Participants

             . DATE       M4C #      TYPE           IS0 TOPE       MEAN s.d. MEAfl s.d.        MEAll s.d.

July 57812 Milk I-131 <8 0 77 1981 Cs-137 31 1 31 5 32 4 Ba-140 <25 0 0 K 1136 49 1600180 1593 99 Sept 60776 APT Cs-137 18 3 19 5 24 6 1981 Oct 62282 Water Cr-51 <75(a) 34 5 36 9

   ,r 1981                                Co-60            25 2      22 5              23 3 Zn-65            25 2      24 5              24i4 Ru-106           <29         0                  0 Cs-134           21 1      21 5              20 4 Cs-137           33 2      32 5              33i4 Oct       62491     Water           Co-60            <3          0                  0 1981                                Cs-134           11 1      12 5              12 2 Cs-137           16 1      15 5              16 3 Oct       62547     Milk            I-131            53 1      52 6              53 7 1981                                Cs-137           26t2      25 5              27 3 Ba-140           s17         0                  0 K              1526 0    1530 77           1532 108 flov      63205     Food            Co-60            26 2      30 5              30 4 1981                                Cs-137           27 1      33 5              34 4 B a- 140         <35         0                 66 K              211310    2730 137          2758 331 (1)  Results reported in pCi/ liter for milk and water, pCi/ sample for air particulates, and pCi/ kilograms for food products except K which is reported in mg/ liter for milk and mg/ kilogram for food products.

(a) Sample was not analyzed within one half-life resulting in large LLD due to a long decay period. 133

TABLE E-3 INTER-LABORATORY COMPARIS0!iS TRITIUM IN WATER pCi/ liter SAMPLE RMC EPA All Participants DATE RMC # TYPE ANALYSIS MEAN s.d. MEAN s.d. MEAN s.d. Feb 44003 Water H-3 1680 137 1760 341 1778 230 B81 Apr 53660 Water H-3 2727 6 2710 355 2717 373 1981 June 56309 Water H-3 2053 32 1950 344 1946 241 1981 Aug 58155. Water H-3 2693 40 2630 354 2616 361 1981 Oct 61071 Water H-3 2467 106 2210 348 2133 214 1981 Dec 64936 Water H-3 2637 90 2700 355 2676 244 1981 l l l 134

TABLE E-4 IllTER-LABORATORY C0f1 PARIS 0NS 10 DINE-131 IN WATER pCi/ liter SA!1PLE RMC EPA Ali Participants DATE RMC # TYPE A!1ALYSIS MEAN s.d. I1EAfl s.d. ;1EA!,~s .d. Apr 53750 Water I-131 31 3 30 6 29 5 1981 Aug 58205 Water I-131 66 5 73 7 72 7 1981 Dec 64544 Water I-131 64 3 76 8 '9 10 1981 135

TABLE E-5 - If4TER-LA80RATORY STR0flTIUM-89 Afl0 STR0f1 TIUM-90ll COMPARIS0!iS ) SAMPLE Rf1C EPA All Participants DATE RMC # TYPE AtlALYSIS MEAll s.d. ME All s . d. MEAfl s.d. Jan 43229 Wate r S r-89 24 11 1625 15i5 1981 S r-90 27 7 34 2 32 5 Jan 43514 flilk S r-89 <8 0 29 37 1981 S r-90 22 3 20 3 19 3 March 44815 Food S r-89 74 13 (a) 47 5 43 18 1981 S r-90 32 2 29 2 2718 March 53663 APT Sr-90 16 2 18+2 17 3 1981 Apr 54841 Wate r Sr-39 3216 38 5 34i9 1981 S r-90 29 5 28 2 26 7 May 54879 Wate r S r-89 51 2 36 5 32 10 1981 S r-90 26 10 22 2 2216 May 55248 Milk S r-89 92 25i5 2216 1981 S r-90 91 11 2 10 i3 June 56994 APT Sr-90 18 2 19 2 19 3 1981 July 57331 Food S r-89 36 14 44 5 44i9 1981 S r-90 2311 31 2 29 3 July 57812 Milk Sr-89 20 7 25 5 24 6 1981 S r-90 16 0 17 2 16 2 Sept 59585 Wate r S r-89 21 5 23 5 22 3 1981 S r-90 6i2 11 2 11 2 Sept 60776 APT Sr-90 16 1 16 2 17 3 1981 Oct 62491 Water S r-89 24 7 21 5 22i6 1981 S r-90 96 14 2 13 3 Oct 62547 Milk Sr-89 26 2 23 5 22 5 1981 S r-90 17 2 18 2 18 3 flov 63205 Food Sr-89 31i6 38 5 35 6 1981 S r-90 21 2 23 2 23 4 (1) Results reported in pCi/l for water and milk, pCi/ filter for air particulates, and pCi/kg for food. (a) Very low yields for all samples and long decay period from collection to analysis resulted in questionable results. 136

l l APPENDIX F SITE SPECIFIC DEMOGRAPHIC DATA

) .. . . .

SITE SPECIFIC DEMOGRAPHIC DATA The Branch Technical Position (13) requires the annual collection of certain demographic data in order to determine if any changes to the REMP are necessary. The nearest milk producer and vegetable garden over 50 square meters in each sec-tor must be determined. The nearest residence in each sector was also detennined. Dairy Animal Survey In August 1981, a dairy animal survey was performed in the vicinity of the Susquehanna Steam Electric Station. The information, pertaining to the location of the nearest dairy animal (within 5 miles) is listed in Table F-1. Since there are no changes in the location of the nearest dairy animal, no change in the REMP is necessary. Vegetable Garden Survey The location of the nearest vegetable garden over 50 square meters in each sector is listed in Table F-2. In addition, broad leaf vegetation was collected from gardens in the sectors with the two highest D/Q and analyzed for iodine-131. This data appears in Table C-25. Residence The location of the nearest resiom..ee in each sector is listed in Table F-3. 139

l TABLE F-1 NEAREST DAIRY ANI!4AL OPERATION BY SECTOR Sector Di rection 1931 Distance 1 li >5 2 NNE >5 3 f4E >5 4 ENE 3.7 5 E 2.7 6 ESE 2.4 7 SE 2.1+ 8 SSE 3.2+* 9 S 2.4 10 SSW 3.0* 11 SW 3.5 12 WSW 1.7* 13 W 5.0* 14 WNW >5 15 NW 0.9* 16 NNW 4.2

 +    Goat fann, o    Participant in Susquehanna SES Radiological Environmental fionitoring Program.

1 1 140

TABLE F-2 fiEAREST VEGETABLE GARDEtiS Sector Di rection 1981 Distance 1 fi 0.6 2 f1HE 1.0 3 fiE 2.3 4 Ef4E 2.4 1 I 5 E 0.5 6 ESE 1.4 7 SE 0.4 8 SSE 0.7 9 S 1.2 10 SSW 1.5 11 SW 0.6 12 WSW 1.2 l 13 W 1.3 14 Wi4W 0.7 15 fiW 0.9 16 fifiW 1.4 141

TABLE F-3 NEAREST RESIDEllCE Sector _ Distance (ftiles) Residence 1 11 0.6 Bruce Thomas 2 Nile 1.0 L. ii. Robbins 3 NE 2.3 John Henry Owner: Norman Reinhimer 4 ENE 2.1 James Cruise [ 5 E 0.5 Dorothy Walters Owner: PPal 6 ESE 0.5 Christopher Zwolinski Owner: Robert Zwolinski 7 SE 0.4 Dennis Kline Owner: Harry Kline 8 SSE 0.7 John Naunczek 9 S 1.1 J. D. Bower Frank Rehrig 10 SSW 1.5 11 SW 0.6 Stanley Shortz 12 WSW 1.2 William Kisner 13 W 0.8 W. Johnson 14 WiiW 0.7 l1. E. Folk 15 NW 0.9 11. Serafin 16 NNW 0.6 William lietzler 142 ________ _ _}}