ML20206C445

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Radiological Environ Monitoring Program (REMP) for DAEC for Jan-Dec 1998
ML20206C445
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Site: Duane Arnold NextEra Energy icon.png
Issue date: 12/31/1998
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TELEDYNE BROWN ENGINEERING CO.
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NUDOCS 9905030037
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b Y TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY 5m uEOY"*

REPORT TO IES UTILITIES,INC.

CEDAR RAPIDS, IOWA RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP)

FOR THE DUANE ARNOLD ENERGY CENTER CEDAR RAPIDS, IOWA DOCKET NO. 50-331 ANNUAL REPORT - PART I

SUMMARY

AND INTERPRETATION JANUARY - DECEMBER 1998 FOR SUBMITTAL TO THE NUCLEAR REGULATORY COMMISSION PREPARED AND SUBMITTED BY TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY PROJECT NO. 8001 Approved by:

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1 PREFACE The staff members of the Teledyne Brown Engineering Environmental Services, Midwest Laboratory were responsible for the acquisition of data presented in this report, with the exception of Appendices D and E, which were completed by DAEC personnel. All environmental samples, with the exception of aquatic, were collected by personnel of DAEC.

Aquatic samples were collected by University of Iowa Hygenic Laboratory personnel.

The report was prepared by Teledyne Brown Engineering Environmental Services, Midwest Laboratory, wit:1 the exception of Appendices D and E, which were prepared by DAEC personnel.

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1 TABLE OF CONTENTS i

No.

Eage PREFACE.........................................................................................................ii Lis t of Tables....................................................................................

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Li s t o f Figu res..................................................................................................vi

1.0 INTRODUCTION

2.0

SUMMARY

.........................................................,.............................................2 3.0 ENVIRONMENTAL RADIOLOGICAL MONITORING PROGRAM............. 3 3.1 Program Design and Data Inter Program Description.................pretation............................................. 3 3.2

............................................................4 3.3 Program Execution................................................................................ 5 3.4 Labora tory Proced ures......................................................................... 6 3.5 Program Modifications......................................................................... 6 4.0 RESULTS AND DISCUSSION......................................................................... 7 i

4.1 Atmospheric Nuclear Detonations and Nuclear Accidents................. 7 4.2 Program Findings.................................................................................. 7 5.0 TAB LES AND FIG URES................................................................................ 10 6.0 REFE RENCES CITED.................................................................................... 2 8 APPENDICES A

Interlaboratory Comparison Program Results...............................................A-1 B

Da ta Reporting Conventions.........................................................................B-1 C

Effluent Concentration Limits for Radioactivity in Air and Water Above Background in Unrestricted Areas.........................................C-1 D

Summary of the Land Use Census...............................................................D-1 E

Annual Radiation Dose Assessment.............................................................E-1 lii

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TABLE OF CONTENTS (continued)

PARTII fage l

Da ta Tabula tions and Analyses.......................................................................i I

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1 LIST OF TABLES No.

Eage 5.1 Characteristic Properties of Isotopes Quantified in Gamma-spectroscopic Analyses..................................................................... 1 1 i

5.2 Sample Collection and Analysis Program, 199 8............................................ 1 2 l

5.3 Sampling Loca tions, DA EC.......................................................................... 15 5.4 Type and Prequency of Collections................................................................17 1

5.5 Sample Codes Used in Table 5.4................................................................... 18 i

5.6 Missed Collections and Analyses, 1998........................................................19 5.7 Radiological Environmental Monitoring Program Summary,1998................ 20 In addition, the following tables are in the Appendices:

Appendix A A-1 Interlaboratory Comparison Program Results,1998.....................................A1-1 A-2 Interlaboratory Comparison Program Results, Thermoluminescent Desimeters (TLDs)...........................................................................A 2-1 A-3 In-house Spiked Samples...............................................................................A 3-1 A-4 In-house " Blank" Samples.............................................................................A 4-1 A-5 In-house "Duplica te" Samples........................................................................A5-1 A-6 Deparhnent of Energy MAPEP comparison results.....................................A6-1 A-7 Environmental Measurements Laboratory Quality (EML) Assessment Program comparison results..............................................................A7-1 Attachment A: Acceptance criteria for spiked samples...............................A-2 Appendix C C-1 Effluent Concentration Limits for Radioactivity in Air and Water Above Background in Unrestricted Areas........................................C-2 v

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n LIST OF FIGURES EaSC 5.1 Radiological Environmental Monitoring Program Sampling Stations near the Duane Arnold Energy Center............................................... 2 6 5.2 Radiological Environmental Monitoring Program Sampling Stations Outsid e 0.5 Miles............................................................................... 2 7 1

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1.0 INTRODUCTION

This report summarizes and interprets results of the Radiological Environmental Monitoring Program conducted by Teledyne Brown Engineering Environmental Services, Midwest Laboratory at the Duane Arnold Energy Center, Palo, Iowa, during the period January -

December,1998. This Program monitors the levels of radioactivity in the air, terrestrial, and aquatic environments in order to assess the impact of the Plant on its surroundings.

Tabulation of the individual analyses made during the year are included in Part II of this report.

Duane Arnold Energy Center (DAEC) is located in Linn County on the Cedar River, Iowa, and is operated by IES Utilities, Inc. The Duane Arnold Energy Center is a 565.7 MW(e) boiling water reactor. Initial criticalik was attained on 23 March 1974. The reactor reached 100%

power on 12 August 1974. Ccf knercial operation began on 1 February 1975.

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2.0

SUMMARY

The Radiologicil Environmental Monitoring Program required by the U.S. Nuclear Regulatory Commission (NRC) Technical Specifications for the Duane Arnold Energy Center is described.

Results for 1998 are summarized and discussed.

Program findings show background levels of radioactivity in the environmental samples collected in the vicinity of the Duane Arnold Energy Center. With the exception of D-107, located within the owner controlled area, no effect on the environment due to the operation of the Duane Arnold Energy Center is indicated.

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r 3.0 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM 3.1 Procram Desien and Data Interpretation The purpose of the Radiological Environmental Monitoring Program at the Duane Arnold Energy Center (DAEC) is to assess the impact of the plant on its environment.

For this purpose, samples are collected from the air, terrestrial, and aquatic environments and analyzed for radioactive content. In addition, ambient gamma radiation levels are monitored by thermoluminescent dosimeters (TLDs).

Sources of environmental radiation include the following:

(1)

Natural background radiation arising from cosmic rays and primordial j

radionuclides; (2)

Fallout from atmospheric nuclear detonations; (3)

Releases from nuclear power plants; and (4)

Industrial and medical radioactive waste.

i In interpreting the data, effects due to the DAEC operation must be distinguished from those due to other sources.

A major interpretive aid in assessment of these effects is the design of the monitoring program at the DAEC which is based on the indicator-control concept. Most types of samples are collected both at indicator locations (nearby, downwind, or downstream) and at control locations (distant, upwind, or upstream). A station effect would be indicated if the radiation level at an mdicator location was significantly larger than that at the control location. The difference would have to be greater than could be accounted for by typical fluctuations in radiation levels arising from other sources.

An additional interpretive technic ue involves analyses for specific radionuclides present in the environmental samples collected from the DAEC site. The DAEC's monitoring program includes analyses for strontium-90 and iodine-131, which are fis tion products, and tritium, which is produced by cosmic rays, atmospheric nuclear detonations, and also by nuclear power plants. Most samples are also analyzed for gamma-emitting isotopes with results for the following groups quantified: zirconium-95, cesium-137, and i

cerium-144. These three gamma-emitting isotopes were selected as radiological impact indicators because of the different characteristic proportions in which they appear in the fission product mix produced by a nuclear reactor and that produced by a nuclear detonation. Each of t ne three isotopes is produced in roughly equivalent amounts by a reactor: each constitutes about 10% of the total activity of fission products ten (10) days after reactor shutdown. On the other hand, ten (10) days after a nuclear explosion, the contributions of zirconium-95, cerium-144, and cesium-137 to the activity of the resulting debris are in the approximate ratio 4:1:0.03 (Eisenbud,1963). The other group quantified consists of niobium-95, ruthenium-103 and -106, cesium-134, barium-i lanthanum-140, and cerium-141. These isotopes are released in small quantities by nuclear power plants, but to date their major source of injection into the general environment has been atmospheric nuclear testing. Nuclides of the next group, manganese-54, cobalt-58 and-60, and zinc-65, are activation products and arise from activation of corrosion products. They are typical components of nuclear power plant effluents, but are not produced in significant quantities by nuclear detonations.

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3.1 Program Design and Data Interoretation (continued)

Nuclides of the final group, beryllium-7, which is of cosmogenic origin, and potassium-40, a naturally-occurring isotope, were chosen as calibration monitors and should not be considered radiological impact indicators.

Characteristic properties of isotopes quantified in gamma-spectroscopic analysis are presented in Table 5.1.

Other means of distinguishing sources of environmental radiation can be employed in interpreting the data. Current radiation levels can be compared with previous levels, including those measured before the Plant became operational. Results of the DAEC's Monitoring Program can be related to those obtained in other parts of the world. Finally, results can be related to events known to cause elevated levels of radiation in the environment, e.g., atmospheric nuclear detonations.

3.2 Program Description The sampling and analysis schedule for the environmental radiological monitoring program at the DAEC is summarized in Table 5.2 and is briefly reviewed below. Table 5.3 defines the sampling location codes used in Table 5.2 and specifies for each location its type (indicator or control) and its distance, direction, and sector relative to the reactor site. The types of samples collected at each location and the frequency of collections are presented in Table 5.4 using codes defined in Table 5.5.

To monitor the air environment, airbome particulates are collected on membrane filters by continuous pumping at twelve locations. Also, airborne iodine is collected by continuous pumping through charcoal filters at six of these locations. Nine of the twelve locations are indicators and three are controls (D-1, D-2, and D-13). Filters are changed and counted weekly. Particulate filters are analyzed for gross beta activity. If gross beta activity exceeds 10 times the yearly mean of the control samples gamma isotopic analysis is performed. Quarterly composites of airborne particulates from each location are gamma scanned on a germanium detector.

Charcoal filters are analyzed weekly for I-131 on all samples.

Ambient gamma radiation is monitored at twelve sir sampling locations. In addition, gamma radiation is monitored at thirty-three special locations: seventeen in a circle within 0.5 mi. radius of the DAEC stack; six in 22.5* sectors within 1 mi. of the DAEC stack; and ten in 22.5 sectors between I and 3 miles of the DAEC stack. Two TLDs are placed at each location and are exchanged and analyzed quarterly.

Precipitation samples are collected monthly from one location and analyzed for gamma-emitting isotopes. Quarterly composites are analyzed for tritium.

Milk samples are collected monthly from five locations during the non-grazing season, October through April, and biweekly during the grazing season, May 1 through September 30. One location is a control (D-105) and the rest are indicators. All samples are analyzed for I-131 and gamma-emitting isotopes.

For additional mor.itoring of the terrestrial environment, grain, hay and broad leaf vegetation samples are collected annually, as available, from nine locations: one control (D-105) and eight edicators (D-16, D-57, D-58, D-63, D-72, D-93, D-94, and D-106).

Grain, hay and broad leaf (green leafy) vegetation samples are analyzed for gamma-4

Program Description (continued) j emitting isotopes and at least one broad leaf vegetation is analyzed for iodine-131. If cattle are slaughtered for home use, a meat sample is collected annually, during or immediately following a grazing period from animals grazing on-site. The sample is analyzed for gamma-emitting isotopes. Also, potable ground water is collected quarterly from a treated municipal water system (D-53), the inlet to the municipal water treatment system (D-54) and four additional ground water locations (D-55, D-57, D-58, and D-72). The samples are analyzed for gross beta and tritium. If gross beta activity exceeds 10 times the yearly mean of the control samples, gamma isotopic, strontium-89 and strontium-90 analyses are performed.

Soil samples are collected once per year at two indicator locations (D-15 and D-16).

The samples are analyzed for strontium-90 and gamma-emitting isotopes.

Surface water is collected monthly from five river, pond and sewage effluent locations, one control (D-49) and four indicator (D-50, D-51, D-99, and D-107). All monthly samples are analyzed for gamma-emitting isotopes. Tritium analyses are performed on quarterly composites from each location. In addition, all samples from Location D-107 i

(plant sewage discharge) are analyzed for K-40 by flame photometry.

The aquatic environment is also monitored by upstream and downstream (D-49 and D-

61) semiannual collections of fish. River bottom sediment is also collected semiannually at the plant's intake and discharge (D-50 and D-51) and downstream of the sewage plant (D-107). Tha samples are analyzed for gamma-emitting isotopes.

3.3 Program Execution The program was executed as described in the preceding section with the following exceptions:

(1)

TLD data was not available for the first and second quarters,1998 from location D-48. The TLDs were lost in the field.

(2)

TLD data was not available for the fourth quarter,1998 from locations D-18 and D-43. The TLDs were lost in the field.

(3)

No milk was available from location D-93 for the months of December and January,1998. No milk was available from location D-101 for January through April and December,1998. The goats were dry.

(4)

One cooler containing milk from location D-105, collected June 18,1998,and surface water from location D-49, collected June 15,1998 was lost in shipment.

(5)

Air particulate / Air iodine samples for all locations were missed for the week i

ending December 3,1998. The samples were collected and shipped according to l

specifications, but were misplaced by the laboratory.

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i 3.4 Laboratorv Procedures All iodine-131 analyses in milk were made by using a sensitive radiochemical procedure which involves separation of the element by use of an ion-exchange resin and subsequent beta counting.

All gamma-spectrosco sic analyses were performed with high resolution germanium detectors. Levels ofioc ine-131 in vegetation were determined by gamma spectrometry.

Levels of airborne iodine-131 in charcoal samples were measured by gamma spectrometry.

Tritium levels were determined by the liquid scintillation technique.

Analytical Procedures used by TBEESML are on file and are available for inspection.

Procedures are based on those prescribed by the Health and Safety Laboratory of the U.S. Dep't of Energy, Edition 28,1997, U.S. Environmental Protection Agency for Measurement of Radioactivity in Drinking Water,1980, and the U.S. Environmental Protection Agency, EERF, Radiochemical Procedures Manual,1964.

Details of TBEESML's QA program are presented elsewhere (Teledyne Isotopes Midwest Laboratory,1992 ). The TBEESML QA Program includes participation in the Interlaboratory Comparison (Crosscheck) Program. Results obtained in the crosscheck program are presented in Appendix A.

3.5 Procram Modifications There were no program modifications during the year,1998.

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7 4.0 RESULTS AND DISCUSSION All of the scheduled collections and analyses were made on schedule except those listed in Table 5.6.

All results are summarized in Table 5.7 in a format recommended by the Nuclear Regulatory Commission in Regulatory Guide 4.8. For each type of analysis of each sample medium, this table lists the mean and range of all indicator and control locations. The locations with the highest mean and range are also shown.

The tabulated results of all measurements made in 1998 are not included in this section, although references to these results will be made in the discussion. The complete tabulation of the 1998 results is contained in Part II of the 1998 Annual Report on the Radiological Environmental Monitoring Program for the Duane Arnold Energy Center.

4.1 Atmospheric Nuclear Detonations and Nuclear Accidents There were no reported atmospheric nuclear tests in 1998. The last reported test was conducted by the People's Republic of China on October 16,1980.

There were no reported accidents at nuclear reactor facilities in 1998.

4.2 Procram Findines Results obtained show background levels of radioactivity in the environmental samples collected in 1998.

Airborne Particulates The average annual gross beta concentrations in airborne particulates were identical at j

3 both indicator and control locations (0.024 pCi/m ) and were similar to levels observed i

from 1984 through 1997. The :esults are tabulated below. The data for 1986 does not include the results from May 19 to June 9,1986, which were influenced by the accident at Chernobyl.

Year Indicators Controls year Indicators Controls 3

3 Concentration (pCi/m )

Concentration (pCi/m )

1984 0.025 0.026 1992 0.022 0.023 1985 0.024 0.024 1993 0.022 0.023 1986 0.024 0.024 1994 0.023 0.024 1987 0.024 0.026 1995 0.025 0.024 1988 0.026 0.028 1996 0.024 0.023 1989 0.026 0.029 1997 0.023 0.023 l

1990 0.022 0.024 1998 0.024 0.0.24 1991 0.023 0.022 Average annual gross beta concentrations in airborne particulates.

Gamma spectroscopic analysis of quarterly composites of air particulate filters yielded similar results for indicator and control locations. Beryllium-7, which is produced 7

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Airborne Particulates (continued) continuously in the upper atmosphere by cosmic radiation (Arnold and Al-Salih,1955),

was detected in all samples. All other gamma-emitting isotopes were below their respective LLD limits. No plant effect was indicated.

AirbomeIodine Weekly levels of airborne iodine-131 were below the lower limit of detection (LLD) of 0.07 pCi/m3 n all sampas.

i Ambient Radiation (TLDs)

At twelve air sampling locations, the TLD readings averaged 14.7 and 14.4 mR/ quarter for indicator and control locations, respectively. At locations within 0.5 mile,1.0 mile, and 3.0 mile radius of the stack, the measurements averaged 16.9 mR/ quarter,18.6 mR/ quarter, and 15.2 mR/ quarter, respectively. The average for all locations was 16.1 mR/ quarter. This is lower than the estimated average natural background radiation for Middle America,19.5 mR/ quarter, which is based on data on Pages 71 and 108 of the report, " Natural Background Radiation in the United States" (National Council on Radiation Protection and Measurements,1975). The terrestrial absorbed dose (uncorrected for structural and body shielding) ranges from 8.8 to 18.8 mrad / quarter and averages 11.5 mrad / quarter for Middle America. Cosmic radiation and cosmogenic radionuclides contribute 8.0 mrad / quarter for a total average of 19.5 mrad / quarter. No plant effect was indicated.

Precipitation In precipitation, the tritium concentration was below the LLD of 330 pCi/L in all samples. No gamma-emitting isotopes were detected. No plant effect was indicated.

Milk Iodine-131 results were below the detection limit of 1.0 pCi/L in all samples.

No gamma-emitting isotopes, except naturally occurring potassium-40, were detected in any milk samples. This is consistent with the finding of the National Center for Radiological Health that most radiocontaminants in feed do not find their way into milk due to the selective metabolism of the cow. The common exceptions are radioisotopes of potassium, cesium, strontium, barium, and iodine (National Center for Radiological Health,1968).

In summary, the milk data for 1998 show no radiological effects of the plant operation.

Ground Water The annual mean for gross beta activity measured 2.9 pCi/L and was similar to the levels observed in 1980 through 1997. The location with the highest mean (5.2 pCi/L) was D-58, a farm 1.0 mile distant from the plant. Tritium was below the LLD of 330 pCi/L in all samples. No plant effect was indicated.

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Vegetation Iodine-131 results in broadleaf vegetation were below the LLD level of 0.040 pCi/g wet weight in all samples Except for potassium-40, which was observed in all vegetation samples ( broadleaf, grain, and forage ), all other gamma-emitting isotopes were below detection limits in all samples. No plant effect is indicated.

Snil Strontium-90 was detected in both samples and averaged 0.03' pCi/g dry w'eight.

Cesium-137 was detected at an average concentration of 0.15 pCi/g dry weight. Both strontium-90 and Cesium-137 concentrations were similar to levels observed in 1987 (0.08 and 0.30 pCi/g dry weight, respectively), in 1988 (0.064 and 0.33 pCi/g dry weight, respectively), in 1989 (0.046 and 0.18 pCi/g dry weight, respectively), in 1990 (0.066 and 0.21 pCi/g dry weight, respectively), in 1991 (0.064 and 0.34 pCi/g dry weight, respectively), in 1992 (0.040 and 0.26 pCi/g dry weight, respectively), in 1993 (0.058 and 0.26 pCi/g dry weight, respectively), in 1994 (0.040 and 0.27 pCi/g dry weight, respectively), in 1995 (0.044 and 0.21 pCi/g dry weight, respective:y), in 1996 (0.050 and 0.17 pCi/g dry weight, respectively) and in 1997 (0.051 and 0.20 pCi/g dry weight, respectively).

The only other gamma-emitting isotope detected was potassium-40 at an average concentration of 12.53 pCi/g dry weight. No plant effect on soil was indicated.

Surface Water Tritium was below the LLD level of 330 pCi/L in all samples.

All gamma-emitting isotopes were below their respective LLDs.

K-40 was measured at one location, D-107 (sewage effluent). The concentration ranged from 12,1-26.8 pCi/L and averaged 16.2 pCi/L.

No plant effect on the radioactivity of surface water was indicated.

Fish All gamma-emitting isotopes, except naturally-occurring otassium-40, in edible portions were below detection limits. The potassium 40 level was similar at both indicator and control locations (3.37 and 3.29 pCi/g wet weight, respectively). No plant effect on fish was indicated.

River Sediments River sediments were collected in May and September,1998, and analyzed for gamma-emitting isotopes. Cobalt-60 was detected in one sample from location D-107 (sewage effluent) at a concentration of 0.084 pCi/g dry weight. Cesium-137 was detected at two locations, D-107 (sewage effluent) at a concentration of 0.051 pCi/g dry weight, and D-51 (discharge) at a concentration of 0.034 pCi/g dry weight. Potassium-40 ranged from 7.38-9.26 pCi/g dry weight and averaged 8.68 pCi/g dry weight.

All other gamma-emitting isotopes were below detection limits.

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5.0 TABLES AND FIGURES

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Table 5.1 Characteristic properties of isotopes quantified in ganuna-spectroscopic analyses.

. Designation Comment Isotope Half-lifea

-I. NaturallyOccurring A. Cosmogenic Produced by interaction of cosmic Be-7 53.2 d rays with atmosphere B. Terrestrial Primordial K-40 1.26 x 109 y II. Fission Productsb Nuclear detonations constitute the major environmental source

- A. Short-lived I-131 8.04 d Ba-140 12.8 d B. Other than Short-lived Nb-95 35.15 d Zr-95 65 d Ru-103 39.35 d Ru-106 368.2 d Cs-134 2.061 y Cs-137 30.174 y Ce-141 32.5 d Ce-144 284.31 d III. Activation Products Typically found in nuclear power Mn-54 312.5 d plant effluents Fe-59 45.0 d Co-58 70.78 d Co-60 5.26 y Zn-65 245 d a Half-lives are taken from Appendix E of Environmental Quarterly,1 January 1978, EML-334 b (ndudes fission-product daughters.

U. S. Department of Energy,1978).

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Table 5.2 Sample collection and analysis program,1998.

Exposum Sampling Location Pathway Sample Sampling and Type and Frequency and/or Point Description Collection Frequency of Analysis Sample Type Airbome 1

Cedar Rapids (C) Continuous operation of Analyze. for gross beta Particulates 2

Marion (C) sampler with sample activity more than 24 hours2.777778e-4 days <br />0.00667 hours <br />3.968254e-5 weeks <br />9.132e-6 months <br /> 3

Hiawatha collection at least once after filter change. Perform 5

Palo per week or as required gamma isotopic analysis on 6

Center Point by dustloading each sample having gross beta 7 Shellsburg activity greater than ten 8

Urbana times the yearly mean of the 10 Atkins control samples.

11 Toddsville 13 Albumett (C)

Composite weekly samples to 15 On-site North form a quarterly composite (by 16 On-site South location). Analyze quarterly composite for gamma isotopic.

Airbome Iodine 2

Marion (C)

Continuous operation of Analyze each cartridge for 5

Palo sampler - with sample iodine-131.

7 Shellsburg collection at least once 8

Urbana per week.

11 Toddville 15 On-site North Ambient 1-3 Air Particulate Two dosimeters Read gamma radiation dose Radiation 5-8 Locations continuously at each quarterly.

10,11 location.

Both 13,15 dosimeters are changed 16 at least quarterly.

18-23, Within 0.5 mile of 28-32, Stack 33-42 Within 3.0 miles of Stack 43-48 Within 1.0 mile of 82-86, Stack 91 Surface Water 49 Lewis Access (C)

Once per month.

Gamma isotopic analyses of 50 Plant Intake (C) each sample (by location).

51 Plant Discharge 99 Pleasant Creek Composite monthly samples to 107 Plant Sewage form quarterly composite (by Discharge location). Analyze quarterly composite for tritium.

(C) denotes control location. All other locations are indicators.

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Table 5.2 Sample collection and analysis program,1998 (continued).

Exposum Sampling Location Pathway Sample Sampling and Type and Frequency and/or Point Description Collection Frequency of Analysis Sample Type Ground 53 Treated Grab sample at least Gross beta and tritium j

Water Municipal Water once per quarter activity analysis on (potable) 54 Inlet to Municipal quarterly sample. If gross Water Treatment beta is greater than ten System times the yearly mean of On-site well control samples, perform 55 Wells off-site and gamma isotopic and Sr-89 57,58 within 4 km of and Sr-90 analyses.

72 DAEC River 50 Plant Intake (C)

At least once every Gamma isotopic analysis of Sediment 51 Plant Discharge six months.

each sample.

i 107 Sewage Effluent Canal Vegetation 16,57, Farms that raise Annually at harvest Gamma isotopic analysis of 58,63, food crops time. One sample of edible portions.

72,93, each: grain, green 94,106, leafy, and forage. At I-131 analysis on broadleaf 105 (C) least one sample vegetation.

1 should be broadleaf 1

vegetation.

Fish 49 Cedar River One sample per 6 Gamma isotopic analysis on i

upstream of DAEC months (once during edible portions.

not influenced by January through July effluent (C) and once during Downstream of August through j

61 DAEC in influence December).

of effluent Milkb 105 Control Farm near At least once per two During the grazing season:

Norway, Iowa weeks during the Ganuna isotopic and iodine-grazing season.

131 analyses of each sample.

Dairy Farms 63,93, within 10 miles of At least once per During the non-grazing season:

96,101 Site month during the Gamma isotopic and iodine-non-grazing season.

131 analyses of each sample.

(C) denotes control location. All other locations are indicators.

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Table 5.2 Sample collection and analysis program,1998 (continued).

Exposure Sampling Location Pathway Sample Sampling and Type and Frequency and/or

- Point Description Collection Frequency of Analysis Sample Type Precipitation On-site Monthly Gamma isotopic on all samples.-

Tritium on quarterly composites.

Meate On-site Annually Gamma Isotopic Soil 15,16 On-site Annually Gamma Isotopic and Sr-90.

a Gamma isotopic analysis and analysis for gamma-emitting nuclides refer to high resolution gamma ray spectrum analysis. An

..ower limit of detection (LLD)y radionuclide detected at a concentration greater than the should be reported quantitatively; conversely, any radionuclide concentration less than the LLD should not be reported, b The grazing season is considered to be May 1 through September 30.

c Meat was not collected in 1998; no animals slaughtered for home use.

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t; Table 5.3 Sampling locations, Duane Arnold Energy Center.

Samplinglocation

. Code Type Distance and l

Sampling Direction from Site Point Location Description Stack D-1 C

1 Cedar Rapids 11 mi @ 135'SE D-2 C

2 Marion 11 mi @ 125'ESE D-3 3

Hiawatha 7 mi @ 130'SE D-5 5-Palo 3 mi @ 200'SSW D-6.

6 Center Point 7 mi @

0N D-7 7

Shellsburg 6 mi @ 255'W D-8 8

Urbana 10 mi @ 345NW D-10 10 Atkins 9 mi@ 210*SSW D-11 11 Toddville 4 mt @ 90*E D-13 C

13 Albumett 9 mi @ 70*ENE D-15 15-On-site, Northwest 0.5 mi @ 305'NW D-16 16 On-site, South 0.5 mi@ 190 SSE D-18 18 0.5 mi NNE D-19 19 0.5 mi NE D-20 20 0.5 mi ENE l

D-21 21 0.5 mi ENE D-22 22 0.5 mi E D-23 23 0.5 mi ESE i

l D-28 28 0.5 mi WSW D-29 29 0.5 mi W D-30 30 0.5 mi WNW l

D-31 31 0.5 mi NW D-32 32 0.5 mi NNW D-33 33 3.0 mi N D-34 34 3.0 mi NNE D-35 35-3.0 mi NE D-36 36 3.0 mi ENE D-37 37 3.0 mi E D-38 38 3.0 mi ESE D-39 39 3.0 mi SE D-40 40 3.0 mi SSE

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. D-41 41 3.0 mi S D-42 42 3.0 mi SSE l

D-43 43 1.0 mi SSW l

D-44 44 1.0 mi WSW D-45 45 1.0 mi W D-46 46 1.0 mi WNW r

l D-47 47 1.0 mi WNW D-48 48 1.0 mi NW D-49 C

49 Lewis Access, upstream of DAEC 4.0 mi NNW D-50 C

50 PlantIntake D-51 51 Plant Discharge D-53 53 Treated Municipal Water

-D-54 54 Inlet to MunicipalWater Treatment System D-55 55 On-site Well 15 l.

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Table 5.3 Sampling locations, Duane Arnold Energy Center (continued).

Sampling Location Code Type Distance and j

Sampling Direction from Site 1

Point Location Description Stack D-57 57 Farm (Off-site Well) 1.0 mi WSW D-58 58 Farm (Off-site Well) 0.5 mi WSW-SW D-61 61 0.5 mi downstream of plant discharge D-63 63 Farm 1.5 mi WNW D-72 72 Farm 2.0 mi SSW i

D-82 82 0.5 mi SE D-83 83 0.5 mi SSE D-84 84 0.5 mi S D-85 85 0.5 mi SSW D 86 86 0.5 mi SW D-91 91 0.5 mi N D-93 93 Farm '

2.8 mi NNE D-94 94 Farm 2.7 mi N D-96 96 Farm 8.0 mi SSW D-99 99 Pleasant Creek Lake 2.5 mi WNW D-101 101 Farm 4.0 mi E D-105 C

105 Farm 21.3 mi SSW D-106 106 Farm 4.5 mi SE D-107 107 Sewage Effluent Canal On-site "C" denotes control location. All other locations are indicators.

l 16

Table 5.4 Type and Frequency of collection.

b Weekly Monthly Quarterly Semiannually Annually Location D-1 C

AP TLD D-2 C

AP,AI TLD D-3 AP TLD D-5 AP,AI TLD D-6 AP TLD D-7 AP,Al TLD D-8 AP, Al TLD D-10 AP TLD D-11 AP, AI TLD D-13 C

AP TLD D-15 AP,AI TLD SO D-16 AP TLD SO,G D-18 through TLD D-23 D-28 through TLD D-42 D-43 through TLD D-48 D-49 C

SW F

D-50 C

SW RS D-51 SW RS D-53 WW D-54 WW D-55 WW D-57 WW G

D-58 WW G

D-61 F

D-63 M

G D-72 WW G

D-82 through TLD D-86 j

D-91 TLD i

l D-93 M

G D-94 M

G D-96 M

D-99 SW D-101 M

D-105 C

M G

D-106 M

G D-107 SW RS On-site P

ME I

"C" denotes control location. All other locations are indicators.

17

(

r.-

Table 5.5. Sample codes used in 5.4.

I Code Description AP Airborne PaMculates AI AirborneIodine TLD Thermoluminescent Dosimeter l

P Precipitation M

Milk WW WellWater G

Vegetation ME Meat SO Soil SW Surface Water F

Fish RS River Sediment i

18

[

r Table 5.6. Missed collections and analyses, Duane Arnold Energy Center,1998.

l I

l Sample Collection Date l

Type Analysis Location (s) or Period Comments i

l l

MI I-131, Gamma D-93 01-06-98 Sample not received; goat dry.

MI I-131, Gamma D-101 01-06-98 Sample not received; goat dry.

MI I-131, Gamma D-101 02-03-98 Sample not received; goat dry.

MI I-131, Gamma D-101 03-05-98 Sample not received; goat dry.

TLD Ambient Gamma D-48 1st Qtr.

TLD lost in the field.

MI I-131, Gamma D-101 04-07-98 Sample not received; goat dry.

TLD Ambient Gamma D-48 2nd Qtr.

TLD lost in the field.

SW Gamma D-49 06-15-98 Sample lost in shipment.

MI I-131, Gamma D-105 06-18-98 Sample lost in shipment.

AP/AI Gross Beta, I-131 D-2,5,7,8,11,15 12-03-98 Samples misplaced by the AP Gross Beta D-1,3,6,10,13,16 12-03-98 laboratory.

MI I-131, Gamma D-93 12-01-98 Sample not received; goat dry.

MI I-131, Gamma D-101 12-01-98 Sample not received; goat dry.

TLD Ambient Gamma D-18 4th Qtr.

TLD lost in the field.

TLD Ambient Gamma D-43 4th Qtr.

TLD lost in the field.

I 19

f i

Table 5.7 Radiological Envimnmental Program Summary.

1 Name of Facility Duane Arnold Energy Center Docket No.

50-331 locationof Facility Linn, Iowa Reporting Period January December 1998 (County, State) i Indicator Location with Highest -

Control Number i

Sample Type and locations Annual Mean Locations Non-j Type Number of LLob Mean (F)C Mean (F)C Mean (F)c Routine (Units)

Analyses Rangec Locationd a

Rangec Range Results' Airbome GB 612 0.004 0.024 (459/459)

D-13, Alburnett, 0.026 (51/51) 0.024 (153/153)

O particulates (0.006-0.058) 9 mi. ENE (0.010-0.063)

(0.004-0.063) 3 (pCi/m )

GS 48 Be-7 0.012 0.081 (36/36)

D 13, Albumett, 0.092 (4/4) 0.084 (12/12) 0 i

(0.050-0.112) 9 mi. ENE (0.072-0.111)

(0.052-0.112)

Nb-95 0.0022

<LLD

<tLD 0

Zr-95 0.0032

<LLD

<LLD 0

Ru-103 0.0017

<LLD

<LLD 0

l Ru-106 0.014

<LLD

<LLD 0

l

\\

l Cs-134 0.0017

<LLD

<LLD 0

l Cs-137 0.0014

<LLD

<LLD 0

Ce-141 0.0026

<LLD

<LLD 0

Ce-144 0.0080

<LLD

<LLD 0

Airbome I131 306 0.07

<LLD

<LLD 0

lodine 3

(pCi/m )

TLD,AP Gamma 48 1

14.7 (36/36)

D-8, Urbana, 19.1 (4/4) 14.4 (12/12) 0 f

Locations (9.5-20.8) 10 mi.NW (16.6-20.8)

(12.4 17.8)

(mR/ quarter)

TLD, within Gamma 67 1

16.9 (67/67)

D-30, 20.5 (4/4)

None 0

i O.5 mi of Staek (9.3-24.0) 0.5 mi. WNW (17.4-24.0)

(mR/ quarter)

RD, within Gamma 21 1

18.6 (21/21)

D-48, 22.1 (2/2)

None 0

1.0 mi of Stack (13.1-24.1) 1.0 mL NW (21.0-23.2) r (mR/ quarter)

)

ED, within Gamma 40 1

15.2 (40/40)

D-37, 18.4 (4/4)

None 0

i 3.0 miof Stack (9.8-22.5) 3.0 mi. E (15.8-22.5)

(mR/ quarter)

Precipitation H3 4

330

<LLD None 0

(pCi/L)

GS 12 Mn-54 7.0

<LLD None 0

1 Fe-59 12.7

<LLD None O

Co-58 5.5

<LLD None 0

20

p i.

1

(

Table 5.7 Radiological Environmental Program Summary l

l Name of Facility Duane Arnold EnerKY Center Docket No.

50-331 Location of Facility Linn, Iowa Reporting Period January December 1998 (County, State)

Indicator Location with Highest Control Number l

Sample Type and Locations Annual Mean Locations Non-Type Number of Ltob Mean (F)C Mean (F)C Mean (F)c Routine (Units)

Analyses Rangec Locationd

~

Results' a

e Range Range Precipitation Co-60 7.1

<LLD None 0

i (pCi/L)

(continued) 2n-65 19.7

<LLD None 0

Nb-95 6.9

<LLD None 0

Zr.95 13.3

<LLD Nonc 0

l l-131 26.2

<LLD None O

Cs-134 8.0

<LLD None O

Cs-137 8.5

<LLD None 0

Ba 140 36.8

<LLD None 0

I La 140 14.0

<LLD None O

Milk 1-131 82 1.0

<LLD

<LLD 0

(pCi/L) l GS 82 K-40 100 1470 (65/65)

D-93, Farm 1730 (16/16) 1380 (17/17) 0 (700-2020) 2.8 mi. NNE (1400-2020)

(1240 1490)

Cs-134 15

<LLD

<LLD 0

Cs-137 18

<LLD

<LLD 0

Ba 140 60

<LLD

<LLD 0

La-140 15

<LLD

<LLD 0

i l

Ground Water CB 24 1.3 2.9 (15/24)

D-58, Farm 5.2 (4/4)

None 0

l (pCi/L)

(1.44.3) 1.0 mL WSW-SW (4.14.3)

H-3 24 330

<LLD None o

Broadleaf I-131 5

0.040

<LLD None O

Vegetation (pCi/g wet)

CS 5

K-40 0.5 2.17 (4/4)

D-105, Farm 4.03 (1/1) 4.03 (1/1) 0 (2.01 2.44) 21.3 mi. SSW Mn-54 0018

<LLD None O

Co-58 0.018

<LLD None O

Co-60 0.028

<LLD None O

Nb-95 0.030

<LLD None 0

Zr-95 0.054

<LLD None 0

1 Ru-103 0.019

<LLD None 0

21 o

Table 5.7 RadiologicalEnvironmentalFrogramSummary, Name of Facility Duane Arnold Energy Center Docket No.

50-331

!.ocation of Facility ;Linn, lowa Reporting Period January - December 1998 (County, State) -

Indicator Location with Highest Comrol Number Sample Type and locations Annual Mean Locations Non.

Type-Numberof LLob Mean (F)C Mean (F)C Mean (F)c Routine (Units)

Analyses Rangec Locationd a

Rangec Fange Result /

Broadleaf Ru-106 0.14

<LLD None O

Vegetation (pCi/g wet)

Cs-134 0.031

<LLD None O

teontinued)

Cs-137 0.027

<LLD None 0

Ce-141 0.031

<LLD None O

Cc-144 0.12

<LLD None O

Vegetation (Grain)

GS 7

(pCi/g wet)

K-40 0.5 '

3.97(6/6)

D-16, Onsite, 10.51 (1/1) 2.85 (1/1) 0 (2.40-10.51) 0 5 mi. SSE Mn-54 0.017

<LLD

<LLD 0

Co-58 0.016

<LLD

<LLD 0

Co-60 0.020

<LLD

<LLD 0

Nb-95 0.023

<LLD

<LLD 0

Zr-95 0.044

<LLD

<LLD 0

Ru-103 0.021

<LLD

<LLD 0

Ru-106 0.19

<LLD

<LLD 0

Cs-134 0.018

<LLD

<LLD 0

Cs.137 0.019

<LLD

<LLD 0

Ce-141 0.035

<LLD

<LLD 0

Ce-144 0.12

<LLD

<LLD 0

Vegetation GS 5

(Forage)

(pCi/g wet)

K-40 0.5 14.94 (4/4)

D.63, Farm 21.66 (1/1) 16.56 (1/1) 0 (7.88-21.66) 1.5 mi. WNW Mn-54 0.078

<LLD

<LLD 0

Co-58 0.039

<LLD

<LLD 0

Co-60 0.051

<LLD

<LLD 0

p Nb-95 0.047

<LLD

<LLD 0

Zr-95 0.10

<LLD

<LLD 0

Ru-103 0.062

<LLD

<LLD 0

Ru-106 0.65

<LLD

<LLD 0

Cs-134 0.056

<LLD

<LLD 0

22

Table 5.7 Radiological Environmental Program Summary.

Name of Facility Duane Arnold Energy Center Docket No.

50-331 Locationof Facility Linn, Iowa Reporting Period January - December 1998 (County, State)

Indicator Location with Highest Control Number Sample Type and locations Annual Mean Locations Non-i Type Number of LLDb Mean (F)C Mean (F)C Mean (F)c Routine (Units)

Analyses

  • Rangec Lncationd Rangec Range Results' V

n-Cs-137 0.042

<LLD

<LLD 0

(pCi/g wet)

Ce-141 0.059

<LLD

<LLD 0

(conunued)

Ce-144 0.23

<LLD

<LLD 0

~~

l

- l (pCi/g dry)

Seil Sr-90 2

0.01 0.036 (2/2)

D-15, Onsite 0.036 (1/1)

None 0

(0.035-0.036) 0.5 mL NW i

GS 2

K-40 0.5 12.53 (2/2)

D-15, Onsite 16.12 (1/1)

None 0

(8.93-16.12) 0.5 mi. NW Mn-54 0.030

<LLD None O

Co-58 0.054

<LLD None O

Co-60 0.028

<LLD None O

Nb-95 0.033

<LLD None 0

Zr-95 0.074

<LLD None O

Ru-103 0.035

<LLD None 0

1 Ru-106 0.32

<LLD None O

Cs-134 0.053

<tLD None O

Cs 137 0.060 0.15 (2/2)

D-16, Onsite, 0.22 (1/1)

None 0

(0.085-0.22) 0.5 mi. SSE Ce-141 0.082

<LLD None O

Ce-144 0.25

<LLD None 0

l l

<LLD 0

Surface Water H-3 20 330

<LLD (pCi/L)

K-40 12 0.5 16.2 (12/12)

D-107, Onsite 16.2 (12/12)

None 0

I (12.1-26.8)

Sewage Effluent (12.1 26.8) 1-131 60 15

<LLD

<LLD 0

GS 60 Mn-54 15

<LLD

<LLD 0

Fe-59 30

<LLD

<LLD 0

Co 58 15

<LLD

<LLD 0

Co-60 15

<LLD

<LLD 0

Zn45 30

<tLD

<LLD 0

23

E.

1 Table 5.7 RadiologicalEnvironmentalProgramSummary.

Name of Facility Duane Arnold Energy Center Docket No.

50-331 locationof Facility Linn, Iowa Reporting Period January - December 1998 (County, State)

Indicator Location with Highest Control Number Sample Type and locations Annual Mean Locations Non-Type Number of LLob Mean (F)C Mean (F)C Mean (F)c Routine (Units)

Analyses Rangec locationd a

Rangee Range Results' Surface Water Nb-95 15

<LLD

<LLD 0

(pCi/L)

(continued)

Zr-95 30

<LLD

<LLD 0

Cs-134 15

<LLD

<LLD 0

Cs-137 18

<LLD

<LLD 0

Ba-140 60

<LLD

<LLD 0

La-140 15

<LLD

<LLD 0

River GS 6

Sediments (pCi/g dry)

K-40 1.0 8.45 (4/4)

D-50, Plant Intake 9.14 (2/2) 9.14 (2/2) 0 (7.38-9.08)

(9.01-9.26)

(9.01-9.26)

Mn-54 0.024

<tLD

<LLD 0

Co-58 0.039

<LLD

<LLD 0

Co-60 0.026 0.084 (1/4)

D-107, Sewage 0.084 (1/2)

<LLD 0

Effluent Canal Nb-95 0.023

<LLD

<LLD 0

Zr-95 0.044

<LLD

<LLD 0

Ru-103 0.026

<LLD

<LLD 0

Ru-106 0.17

<LLD

<LLD 0

Cs-134 0.038

<LLD

<LLD 0

Cs-137 0.021 0 043 (2/4)

D-107, Sewage 0.051 (1/2)

<LLD 0

(0.034-0.051)

Effluent Canal Ce-141 0.063

<LLD

<LLD 0

Ce-144 0.12

<LLD

<LLD 0

i Fish CS 8

)

(Edible

)

Portions)

K-40 0.5 3.37 (4/4)

D-61, Downstream, 3.37 (4/4) 3.29 (4/4) 0 (pCi/g wet)

(2.97-3.58) 0.5 mi.

(2.97-3.58)

(2.94-3.57)

Mn-54 0.015

<LLD

<LLD 0

Co-58 0.019

<LLD

<LLD 0

l

<LLD 0

Co-60 0.023

<LLD Fe-59 0.047

<LLD

<LLD 0

Zn-65 0.039

<LLD

<LLD 0

24

I.

Table 5.7 RadiologicalEnvironmentalProgramSummary.

Name of Facility Duane Arnold Energy Center Docket No.

50-331 locationof Facility Linn, Iowa Reporting Period January - December 1998 (County, State)

Indicator Location with Highest Control Number Sample Type and locations Annual Mean Locations Non-Type Number of Ltob Mean (F)C Mean (F)C Mean (F)c Routine (Units)

Analyses Rangec locationd a

Rangec Range Results' l

Fish Nb-95 0.024

<LLD

<LLD 0

j (Edible I

Portions)

Zr-95 0.042

<LLD

<LLD 0

(pCi/g wet)

(continuaf)

Ru-103 0.022

<LLD

<LLD 0

Ru-106 0.13

<LLD

<LLD 0

Cs-134 0.024

<LLD

<LLD 0

Cs-137 0.014

<LLD

<LLD 0

Ce-141 0.033

<LLD

<LLD 0

Ce-144 0.069

<LLD

<LLD 0

l

  • GB = gross beta;GS = gamma scan.

b LLD = Nominal lower limit of detection based on 4.66 sigma counting error for the background sample.

c Mean and range based upon detectable measurements only. Fraction of detectable measurements at specified locations is indicated in parentheses (F).

d locations are specified by: (1) Name and code (Table 5.3); and (2) distance, direction, and sector relative to reactor site.

' Non-routine results are those which exceed ten times the control station value for the location. If a control c.stion value is not available, the result is considered non-routine if it exceeds ten times the preoperational value for the location.

I i

.y I

1 i

l 25

i Figure 5.1 Radiological Environmental Monitoring Program Sampling Stations near the Duane Arnold Energy Center.

l BARRICADE l-----}

b l

CEDAR RIVER i

j

)U o /

15 - - 3 I

f I

E I

/

3,2 H

18 l

\\

f I

l l

g j

(

l 6

d 31 O

/

i l

O

/

j I

o

\\

19 W

\\

30 20 \\

i a

l 107 I

x F

SWIM DAEC j

(

22 /

$7 29 (SD

/

l I

.~

23 /

)

~

/

i 50 28 H l l l l l l l l l'l l l l l l l lll l l l l l l l l ll y

?

16 86 _ _ _ g g

POWERPLANT RD l

85 9

83 82 GATE 61 58

- - - - - Property Line 2000 feet h

i

/

nl l

See Table 5.3 for sampling locations and Table 5.4 for Type and Frequency of collection.

26

I l

Figure 5.2 Radiological Environmental Monitoring Progr.am Sampling Stations Outside 0.5 Miles.

10 MILE RADIUS j

URBANA e 08 l

CENTER POINT CEDAR e 06 RIVER\\

5 MILE RADIUS i

49 l

I 94 i

93 ALBURNETT l

33 34 13 8 l

35 36 99 63 47 37 SHELLSBURG 46 3.70DDVIllE e DAEC e

4s e-43 j Sm 39 II 72 40 PALOe 42 05 106 41 I

HIAWATHA' 03 i

g MARION 96 02 P

'3 ATKINS 54 10 CEDAR 105 RAPIDS g

I See Table 5.3 for sampling locations and Table 5.4 for Type and Frequency of collection.

27

6.0 REFERENCES

CITED Arnold, J. R. and H. A. Al-Salih.1955. Beryllium-7 Produced by Cosmic Rays. Science 121:

451-453.

Eisenbud, M. 1963. Environmental Radioactivity, McGraw-Hill, New York, New York, pp.

213,275 and 276.

Gold, S., H. W. Barkhau, B, Shlein, and B. Kahn,1964. Measurement of Naturally Occurring Radionuclides in Air, in the Natural Environment, University of Chicago Press, Chicago, Illinois, 369-382.

Hazleton Environmental Sciences.1981. Environmental Radiation Monitoring for the Duane Arnold Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January-December 1980.

Hazleton Environmental Sciences.1982. Environmental Radiation Monitoring for the Duane Arnold Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January - December 1981 Hazleton Environmental Sciences.1983. Environmental Radiation Monitoring for the Duane Arnold Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January - December 1982.

Hohenemser, C. M. Deicher, A. Ernst, H. Hofsass, G. Lindner, E. Racknagel.

1986.

"Chernobyl," Chemtech. October 1986, pp. 596-605.

National Center for Radiological Health,1968. Radiological Health and Data Reports, Vol. 9, Number 12, 730-746.

Teledyne Isotopes Midwest Laboratory.1995. Quality Control Program, Revision 0.

20 July 1995.

Teledyne Isotopes Midwest Laboratory.1994. Quality Control Procedures Manual, Revision 18. 27 September 1994.

Teledyne Isotopes Midwest Laboratory.1992. Quality Assurance Program Manual, Revision 1, 20 August 1992.

Teledyne Brown Engineering Environmental Services, Midwest Laboratory. 1984 - 1999.

Environmental Radiological Monitoring Program for the Duane Arnold Energy Center, Annual Report - Part II, Data Tabulations and Analyses, January - December,1983 -

1998.

Wilson, D. W., G. M. Ward and J. E. Johnson.1969. In Environmental Contamination by Radioactive Materials, International Atomic Energy Agency. p.125.

28 L.

t i

I 4

1 APPENDIX A INTERLABORATORY COMPARISON PROGRAM RESULTS l

i i

NOTE: Teledyne's Midwest Laboratory participates in intercomparison studies administered by U.S. EPA Environmental Monitoring Systems Laboratory, Las Vegas, Nevada. The results are reported in

. Appendix A. Also reported are results of Intemational Intercomparison and Teledyne testing of TLD's, as well as, in-house spikes, blanks, duplicates and mixed analyte performance evaluation program results. Appendix A is updated four times a year; the complete Appendix is included in March, June, September and December monthly progress reports only.

January,1998-through December,1998

Appendix A Interlaboratory Cornparison Procrarn Results Taledyne Brown Engineering Environmental Services Midwest Laboratory (formerly Hazleton Environmental Sciences) has participated in interlaboratory comparison (crosscheck) programs since the formulation of it's quality control program in December 1971. These programs are operated by agencies which supply environmental type samples (e.g., milk or water) containing concentrations of radionuclides known to the issuing agency but not to participant laboratories. The purpose of such a program is to provide an independent check on the laboratory's analytical procedures and to alert it to any possible 1

problems.

Pirticipant laboratories measure the concentration of specified radionuclides and report them to the issuing agency. Several months later, the agency reports the known values to the participant laboratories and specifies control limits. Results consistently higher or lower than the known values or outside the control limits indicate a need to check the instruments or procedures used.

j The results in Table A-1 were obtained through participation in the environmental sample crosscheck program for milk, water and air filters during the past twelve months. Data for previous years is cvailable upon request.

This program is conducted by the U.S. Environmental Protection Agency Office of Research and Developement National Exposure Research Laboratory Characterization Research Division-Las Vegas, Nevada.

The results in Table A-2 were obtained for Thermoluminescent Dosimeters (TLDs), via various laternationalIntercomparisons of Environmental Dosimeters under the sponsorships listed in Table A-2.

Also Teledyne testing results are listed.

Ttble A-3 lists results of the analyses on in-house " spiked" samples for the past twelve montlts. All samples are prepared using NIST traceable sources. Data for previous years availab)e upon request.

Tcble A-4 lists results of the analyses on in-house " blank" samples for the past twelve months. Data for previous years available upon request.

Table A-5 list results of the in-house " duplicate" program for the past twelve months. Acceptance is based on the difference of the results being less than the sum of the errors. Data for previous years available upon request.

The results in Table A-6 were obtained through participation in the mixed analyte performance cvaluation program.

The results in Table A-7 were obtained through participation in the Environmental Measurement Laboratory Quality Assessment Program.

Attachment A lists acceptance criteria for " spiked" samples.

Out-of-limit results are explained directly below the result.

Al

f 12-31-98 ATTACHMENT A ACCEPTANCE CRITERIA FOR " SPIKED" SAMPLES LABORATORY PRECISION: ONE STANDARD DEVIATION VALUES FOR VARIOUS ANALYSES' One Standard Deviation Analysis '

Level for single determinations Gamma Emitters 5 to 100 pCi/ liter or kg 5.0 pCi/ liter

>100 pCi/ liter or kg 5% of known value Strontium-89 5 to 50 pCi/ liter or kg 5.0 pCi/ liter 6

>50 pCi/ liter or kg 10% of known value Strontium-90 2 to 30 pCi/ liter or kg 5.0 pCi/ liter 6

>30 pCi/ liter or kg 10% of known value Potassium-40

>0.1 g/ liter or kg 5% of known value Gross alpha s20 pCi/ liter 5.0 pCi/ liter

>20 pCi/ liter 25% of known value Gross beta

$100 pCi/ liter 5.0 pCi/ liter

>100 pCi/ liter 5% of known value Tritium s4,000 pCi/ liter is = (pCi/ liter) =

169.85 x (known)"

>4,000 pCi/ liter 10% of known value Radium-226,-228

<0.1 pCi/ liter 15% of known value Plutonium 0.1 pCi/ liter, gram, or sample 10% of known value Iodine-131,

- $55 pCi/ liter 6.0 pCi/ liter Iodine-129

>55 pCi/ liter 10% of known value 6

Uranium-238, 535 pCi/ liter 6.0 pCi/ liter

>35 pCi/ liter 15% of known value 6

Nickel-63 6

Technetium-99 50 to 100 pCi/ liter 10 pCi/ liter Iron-55,

>100 pCi/ liter 10% of known value Others" 20% of known value

  • From EPA publication, " Environmental Radioacuvity Laboratory Intercomparison Studies Program, Fiscal Year,1981-1982, EPA-600/4-81-004.
  • Teledynelimit.

A2

Table A-1.

U.S. Environmental Protection Agency's crosscheck program, comparison of EPA and Teledyne's Midwest Laboratory results'.

Concentration in pCi/L' Lab Sample Date Teledyne Results EPA Result' Control Code Type Collected Analysis

  • 2 Sigma
  • 1s, N=1 Limits STW-815 WATER Jan,1998 Sr-89 6.011.0 8.0*5.0 2.2 - 13.8 STW-815 WATER Jan,1998 Sr-90 27.3 1.2 32.0 5.0 26.2 - 37.8 STW-816 WATER Jan,1998 Gr. Alpha 31.2
  • 2.3 30.5
  • 7.6 21.7 - 39.3 STW-816 WATER Jan,1998 Gr. Beta 6.6*0.6 3.9 5.0 0.0 - 9.7 STW-817 WATER Feb,1998 I-131 111.1 0.9 104.9
  • 10.5 86.7 - 123.1 STW-818 WATER Feb,1998 Ra-226 14.9 1.3 16.0 2.4 11.8 - 20.2 STW-818 WATER Feb,1998 Ra-228 30.9 1.9 33.3 8.3 18.9-47.7 STW-818 WATER Feb,1998 U 25.8
  • 1.1 32.0
  • 3.0 26.8-37.2 The presence of U-232 in the sample interfered with the recovery calculation. Result of recalculation; i

28.2*1.2 pCi/L STW-823 WATER Mar,1998 H-3 2,151.0

  • 75.2 2,155.0
  • 348.0 1,551.2 - 2,758.8 STW-824 WATER Apr,1998 Gr. Alpha 48.3
  • 1.5 54.4
  • 13.6 30.8 - 70.8 STW-824 WATER Apr,1998 Ra-226 15.3
  • 0.9 15.0
  • 2.3 11.0 - 19.0 STW-824 WATER Apr,1998 Ra-228 7.8*1.0 9.3 2.3 5.3 - 13.3 STW-824 WATER Apr,1998 Uranium 5.1*0.1 5.0
  • 3.0 0.0 - 10.2 STW-825 WATER Apr,1998 Co-60 50.0 1.7 50.0*5.0 41.3 58.7 STW-825 WATER Apr,1998 Cs-134 20.7
  • 1.2 22.0
  • 5.0 13.3 - 30.7 STW-825 WATER Apr,1998 Cs-137 9.0 1.0 10.0 5.0 1.3 - 18.7 l

STW-825 WATER Apr,1998 Gr. Beta 92.1 3.2 94.7

  • 10.0 77.4 - 112.0 STW-825 WATER Apr,1998 Sr-89 5.3*1.5 6.0*5.0 0.0 - 14.7 STW-825 WATER Apr,1998 Sr-90 17.311.5 18.0
  • 5.0 9.3 - 26.7 STW-826 WATER Jun,1998 Ba-133 36.0
  • 1.0 40.0
  • 5.0 31.3 - 48.7 STW-826 WATER Jun,1998 Co-60 14.0*1.0 12.0 5.0 3.3 - 20.7 STW 826 WATER Jun,1998 Cs-134 26.7
  • 1.2 31.0*5.0 22.3 - 39.7 STW-826 WATER Jun,1998 Cs-137 32.7 3.8 35.0 5.0 26.3-43.7 STW-826 WATER Jun,1998 Zn-65 99.0
  • 11.8 104.0
  • 10.0 86.7-121.3 STW-827 WATER Jun,1998 Ra-226 4.7 0.4 4.910.7 3.7 - 6.1 STW-827 WATER Jun,1998 Ra-228 2.6
  • 0.7 2.1
  • 0.5 1.2 - 3.0 STW-827 WATER Jun,1998 Uranium 3.0*0.1 3.0*3.0 0.0 - 8.2 STW-831 WATER Jul,1998 Sr-89 19.0
  • 3.0 21.0
  • 5.0 12.3 - 29.7 STW-831 WATER Jul,1998 Sr-90 7.0+.0.0 7.0*5.0 0.0 - 15.7 i

STW-832 WATER Jul,1998 Gr. Alpha 5.8*0.4 7.215.0 0.0 - 15.9 STW-832 WATER Jul,1998 Gr. Beta 12.4 0.4 12.8

  • 5.0 4.1 - 21.5 STW-833 WATER Aug,1998 H-3 17,732.0
  • 31.0 17,996.0
  • 1,800.0 14,873.0- 21,119.0 STW-840 WATER Sep,1998 I-131 5.9t0.1 6.1
  • 2.0 2.6 - 9.6 STW-841 WATER Sep,1998 Ra 226 1.70.1 1.7 0.3 1.2 - 2.2 i

STW-841 WATER Sep,1998 Ra-228 6.1 0.6 5.7 1.4 3.3 - 8.1 STW-841 WATER Sep,1998 Uranium 8.2 i 0.5 9.1 3.0 3.9 - 14.3 A1-1

Table A-1.

U.S. Environmental Protection Agency's crosscheck program, comparison of EPA and Teledyne's Midwest Laboratory results*.

Concentration in pCi/L' Lab Sample Date Teledyne Results EPA Result' Control Code Type Collected Analysis 2 Sigma

  • 1s, N=1 Limits STW-844 WATER Nov,1998 Ba-133 54.7
  • 0.6 56.0 6.0 45.6 - 66.4 STW-844 WATER Nov,1998 Co-60 38.3 1.5 38.0*5.0 29.3 - 46.7 STW-844 WATER Nov,1998 Cs-134 91.0 6.0 105.0
  • 5.0 96.3 - 113.7 The average for Cs-134 from all participating laboratories was 97.11 pCi/L. Other isotopes tested for in this sample were well within the control limits. Values for Cs-134 were checked and confirmed. No further action is planned.

STW-844 WATER Nov,1998 Cs-137 109.7 5.8 111.0

  • 6.0 100.6 - 121.4 STW-844 WATER Nov,1998 Zn-65 121.0
  • 7.8 131.0 13.0 108.4 - 153.6

' Results obtained by Teledyne Brown Engineering Environmental Services Midwest Laboratory as a participant in the environmental sample crosscheck program operi.ted by the Intercomparison and Calibration Section, Quality Assurance Branch, Environmental Monitoring and Support Laboratory, U.S.

Environmental Protection Agency (EPA), Las Vegas, Nevada.

  • All results are in pCi/L, except for elemental potassium (K) data in milk, which are in mg/L; air filter samples, which are in pCi/ Filter.
  • Unless otherwise indicated, the TBEESML results are given as the mean
  • 2 standard deviations for three determinations.

USEPA results are presented as the known values and expected laboratory precision (1s,1 determination) d and contro111mits as defined by the EPA.

I l

)

l Al-2

(

. Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (TLDs).

mR Lab Teledyne Results Known Average i2 Sigma Code TLD Type Date Measurement i 2 Sigma Value (All Participants) lith International Intercomparison 115-11A LiF-1CJ Chips Apr,1997 Field 13.2il.0 19.0 17.8 i 8.4 115-11A LiF-100 Chips Apr,1997 Lab,Cs 32.1 i 2.0 58.1 55.219.9 The readings for LiF chips were low in both field and Lab Cs tests. No errors found in efficiency or test calculations, however the reader setting is suspect. Interlaboratory test comparisons for LiF were satisfactory.

lith International Intercomparison 115-11B CaSOp Dy Apr,1997 Field 19.lil.4 19.1 18.918.7 Cards 115-11B CaSOg Dy Apr,1997 Lab,Cs 55.7 i 4.1 58.3 55.2 i 14.9 f

Cards The Eleventh International 1ntercomparison of Environmental Dosimeters was conducted in 1997 and was f

organized by the Department of Energy's Environmental Measurements Laboratory in collaboration with Brookhaven National Laboratory and the NationalInstitute of Standards and Technology.

Teledvne Testing 96-1 LIF-100 Chips Mar,1996 Lab,1 15.9 i 0.3 15.4 96-1 LIF-100 Chips Mar,1996 Lab,2-29.4 i 0.3 30.8 96-1 LiF-100 Chips Mar,1996 Lab,3 62.5 i 1.3 62.5 96-1 CaSOp Dy Mar,1996 Reader 1, #1 14.4 i 0.1 15.4 ND-Cards 96-1 CaSOg Dy Mar,1996 Reader 1, #2 31.8 0.1 30.8 ND Cards 96-1 CaSOp Dy Mar,1996 Reader 1, #3 64.710.4 62.5 ND Cards Teledvne Testing 96-2 CaSOg Dy Mar,1996 Reader 2, #1 14.3 i 0.4 15.4 ND Cards 96-2 CaSOg Dy Mar,1996 Reader 2, #2 31.8 0.1 30.8 ND Cards 96-2 CaSOg Dy Mar,1996 Reader 2, #3 68.6 i 0.1 62.5 ND Cards ND = No Data;Teledyne Testing was only performed by Teledyne.

Chips and Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in March,1996.

Teledyne Testirig 97-1 LIF-100 Chips Mar,1997 Lab,1 13.4 i 1.4 15.0 97.-1 LiF-100 Chips Mar,1997 Lab,2 29.8 i 0.6 30.1 97-1 LiF-100 Chips Mar,1997 Lab,3 63.4 i 0.9 60.2 A2-1

r Table A-2. Crosscheck program results;Thermoluminescent Dosimeters. (TLDs).

rnR Lab Teledyne Results Known Average i2 Sigma Code TLD Type Date Measurement i 2 Sigma Value (All Participants) 97 1 CaSO : Dy Mar,1997 Reader 1, #1 15.5 i 0.1 15.0 ND Cards 97-1 CaSO.: Dy Mar,1997 Reader 1, #2 34.0 i 0.1 30.1 ND Cards 97 1 CaSO : Dy Mar,1997 Reader 1, #3 68.3 i 2.1 60.2 ND Cards Teledvne Testing 97-2 CaSO : Dy Mar,1997 Reader 2, #1 16.8i o.3 15.0 ND Cards 97-2 CaSO.: Dy Mar,1997 Reader 2, #2 36.2 i 0.2 30.1 ND Cards 97-2 CaSO.: Dy Mar,1997 Reader 2, #3 69.6 i 0.2 60.2 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.

Chips and Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in March,1997.

Teledyne Testing 98-1 LiF-100 Chips May,1998 Lab,1 15.Sil.3 16.7 98-1 LiF-100 Chips May,1998 Lab,2 23.9 i 0.9 32.4 98-1 LiF-100 Chips May,1998 Lab,3 59.8 i 1.9 60.2 98-1 CaSO.: Dy May,1998 Reader 1, #1 18.5i0.8 16.7 ND Cards 98-1 CaSO : Dy May,1998 Reader 1, #2 27.3 i 1.7 32.4 ND Cards 98-1 CaSO.: Dy May,1998 Reader 1, #3 70.0 i 4.7 60.2 ND Cards ND = No Data; Teledyne Testing was only performed by Teledyne.

Chips and Cards were irradiated by Teledyne Isotopes, Inc., Westwood, New Jersey, in May,1998.

l l

A2-2

p Table A-3. In-house " spike" samples.

Concentrationin pCi/L' Izb Sample Date Teledyne Results Known Control' 6

Code Type Collected Analysis 2s, n=1 Activity Limits SPW-77 WATER Jan,1998 Cs-137 78.64 7.76 77.23 67.23 - 87.23 SPW-129 WATER Jan,1998 ' Am-241 16.96 1.24 20.64 12.38 - 28.90 SPW-130 WATER Jan,1998 Ra-226 9.39

  • 0.14 10.35 7.25 - 13.46 SPW-130 WATER Jan,1998 Ra-226 12.74
  • 3.05 14.03 9.82 - 18.24 SPMI-498 MILK Jan,1998 Co-60 41.40 2 3.61 36.92 26.92 - 46.92 SPMI-498 MILK Jan,1998 Cs-134 31.78
  • 3.15 32.52 22.52 - 42.52 l

SPMI-498 MILK Jan,1998 Cs-137 37.03 2 4.57 38.56 28.56 - 48.56 SPW-499 WATER Jan,1998 Co-60 44.38 7.85 36.92 26.92 - 46.92 SPW-499 WATER Jan,1998 Cs-134 34.97

  • 7.78 32.52 22.52 - 42.52 SPW-499 WATER Jan,1998 - Cs-137 39.15
  • 10.40 38.56 28.56 - 48.56 SPW-594 WATER Jan,1998 H-3 45125.00
  • 568.00 45598.00 36478.40 - 54717.60 SPAP-5330 AIR FILTER Jan,1998 Cs-137 1.68
  • 0.02 1.90 1.14 - 2.66 l

SPW-664 WATER Feb,1998 U-234 2.63

  • 0.40 3.00 1.80 - 4.20 1

SPW-664 WATER Feb,1998 U-238 3.26

  • 0.49 3.00 0.00 - 15.00 l

SPCH-746 CHARCOAL Feb,1998 I-131(g) 1.73

  • 0.06 2.03 1.22 - 2.84 CANISTER SPVE-750 VEGETATION Feb,1998 I-131(g) 6.16
  • 0.14 5.43 0.00 - 15.43 SPW-790 WATER Feb,1998 I-131 136.35
  • 1.33 137.03 109.62 - 164.44

]

SPMI-791 MILK Feb,1998 I-131 132.63

  • 1.63 137.03 109.62 - 164.44 SPW-497 WATER Feb,1998 Gr. Alpha 43.73
  • 7.61 41.27 20.64 - 61.91 SPW-497 WATER Feb,1998 Gr. Beta 59.45
  • 2.90 61.70 51.70 - 71.70 SPW-9854 WATER Feb,1998 Gr. Alpha 62.60
  • 5.10 53.88 26.94 - 80.82 SPAP-748 AIR FILTER Feb,1998 Gr. Beta 1.72 0.02 1.66 0.00 - 11.66 SPW-1663_

WATER Feb,1998 Ra-226 14.44 0.50 13.80 9.66 - 17.94 SPW-1663 WATER Feb,1998 Ra-228 18.79

  • 1.58 18.29 12.80 - 23.78 SPW-1665 WATER Mar,1998 Ra-226 14.16
  • 0.29 13.80 9.66 - 17.94 SPW-1665 WATER Mar,1998 Ra-228 18.06
  • 1.70 18.29 12.80 - 23.78 SPW-1666 WATER Mar,1998 Sr-89 65.40
  • 2.70 75.94 60.75 - 91.13 SPW-1666 WATER Mar,1998 Sr-90 28.04
  • 1.22 32.65 26.12 - 39.18 SPAP-1728 AIR FILTER. Mar,1998 Gr. Beta 8.15 0.03 7.98 0.00 - 17.98 i

SPW-1998 WATER Apr,1998 Ra-226 13.70 0.33 13.80 9.66 - 17.94 SPW 1998 WATER Apr,1998 Ra-228 14.65

  • 1.38 18.20 12.74 - 23.66 SPW-792 WATER Apr,1998 Th-230 18.62
  • 2.85 17.39 10.43-24.35 SPW-2278 WATER Apr,1998 H-3 41641.00 2 552.00 43287.00 34629.60 - 51944.40 SPW-2284 WATER Apr,1998 Gr. Alpha 41.09 t 1.83 41.26 20.63 - 61.89 SPW-2284 WATER Apr,1998 Gr. Beta 32.01 1.10 30.72 20.72 - 40.72 SPMI-5451 MILK Apr,1998 Cs-137 80.78
  • 6.60 76.68 66.68 - 86.68

'SFW-5459 WATER Apr,1998 Co-60 48.50

  • 3.74 44.65 34.65 - 54.65 SPW-5459 WATER Apr,1998 Cs-137 42.31 4.32 38.34 28.34 - 48.34 SPW-2977 WATER May,1998 Ra-226 11.91 t 0.27 13.80 9.66 - 17.94 SPW-2977 WATER May,1998 Ra-228 16.26 1.67 18.00 12.60 - 23.40 A3-1 io

I i

Table A-3. In-house " spike" samples.

l Concentration in pCi/L' Lab Sample Date Teledyne Results Known Control' Code Type Collected Analysis 2s, n=1' Activity Limits l

SPAP-3041 AIR HLTER May,1998 Cs-137 2.00 0.02 1.89 1.13 - 2.65 SPW-3043 WATER May,1998 Gr. Alpha 40.49 2.57 41.25 20.63 - 61.88 SPW-3043 WATER May,1998 Gr. Beta 35.79 1.52 30.66 20.66-40.66 SPSO-3898 SOIL May,1998 Cs-134 0.11

  • 0.01 0.10 0.06 - 0.14 SPSO-3898 SOIL May,1998 Cs-137 0.48
  • 0.02 0.43 0.26 - 0.61 SPF-3900 HSH May,1998 Cs-134 0.36
  • 0.03 0.38 0.23 - 0.53 SPF-3900 HSH May,1998 Cs-137 0.29
  • 0.03 0.31 0.18 - 0.43 SPW-4162 WATER Jun,1998 Ra-226 12.98 0.18 13.80 9.66 - 17.94 1

)

spw.4162 WATER Jun,1998 Ra-228 16.73 1.62 17.80 12.46 - 23.14 SPW-5340 WATER Jun,1998 Gr. Alpha 41.38 1.87 41.25 20.62 - 61.87 SPW-5340 WATER Jun,1998 Gr. Beta 61.92 1.51 64.92 54.92 - 74.92 SPW-4718 WATER Jul,1998 Ra-226 12.93

  • 0.12 13.80 9.66 - 17.94 SPW-4718 WATER Jul,1998 Ra-228 13.13 1 1.59 17.67 12.37 - 22.97 SPCH-5129 CH C AL Jul,1998 I-131(g) 0.61 0.05 0.57 0.34 - 0.80 SPMI-5131 MILK Jul,1998 Cs-137 83.87 9.09 76.36 66.36 - 86.36 SPMI-5131 MILK Jul,1998 I-131 63.98
  • 0.'/7 61.03 48.82 - 73.24 SPMI-5131 MILK Jul,1998 I-131(g) 62.05 11.00 61.03 36.62 - 71.03 SPMI-5131 MILK Jul,1998 Sr-89 52.66 2.13 62.05 49.64 - 74.46 SPMI-5131 MILK Jul,1998 Sr-90 29.78 1.39 32.41 25.93 - 38.89 SPW-5134 WATER Jul,1998 H-3 20918.00 396.00 21666.00 17332.80 - 25999.20 SPW-5137 WATER Jul,1998 Co-60 44.96
  • 4.00 43.56 33.56-53.56 SPW-5137 WATER Jul,1998 Cs-137 72.05 5.84 76.36 66.36 - 86.36 i

l SPW-5137 WATER Jul,1998 I-131 52.07 0.69 61.03 48.82 - 73.24 SPW-5137 WATER Jul,1998 I-131(g) 58.78

  • 7.69 61.03 36.62 - 71.03 SPW-5136 WATER Jul,1998 Gr. Alpha 50.02
  • 2.28 41.24 20.62 - 61.86 i

SPW-5136 WATER Jul,1998 Gr. Beta 70.19

  • 1.88 64.80 54.80 - 74.80 SPAP-5611 AIR HLTER Jul,1998 Cs-137 1.68
  • 0.02 1.86 1.12 - 2.60 SPF-5453 HSH Jul,1998 Cs-137 0.33
  • 0.03 0.31 0.18 - 0.43 SPAP-5611 AIR HLTER Jul,1998 Cs-137 1.96 0.02 1.86 1.12 - 2.60 SPW-6091 WATER Aug,1998 Gr. Alpha 30.59
  • 1.69 41.23 20.62 - 61.85 SPW-6091 WATER Aug,1998 Gr. Beta 30.28
  • 1.17 30.48 20.48 - 40.48 SPW 6092 WATER Aug,1998 Ra-226 6.29 0.19 6.90 4.83 - 8.97 SPW-6092 WATER Aug,1998 Ra-228 7.85
  • 1.28 8.72 6.10 - 11.34 SPW-7143 WATER Sep,1998 Ra-226 12.31 t 0.48 13.79 9.65 - 17.93 SPW-7143 WATER Sep,1998 Ra-228 15.70 1.68 17.25 12.08 - 22.43 SPW-7144 WATER Sep,1998 Gr. Alpha 35.48
  • 1.65 33.97 16.99 - 50.96 SPW-7144 WATER Sep,1998 Gr. Beta 33.06 1 1.11 30.41 20.41 - 40.41 SPAP-7394 AIR HLTER Sep,1998 Gr. Beta 6.71 0.03 6.77 4.06 - 9.48 (ss) l SPMI-7592 MILK Sep,1998 Cs-137 34.40
  • 7.11 37.99 27.99 - 47.99 A3-2

o

~ Table' A 3. In-house " spike" samples.

Concentrationin pCi/L' Lab Sample -

Date Teledyne Results Known Control' Code Type Collected Analysis 2s, n=1' Activity Limits SPMI-7592' MILK

'SeP,1998 I-131 58.15 0.90 61.55 49.24 - 73.86 SPW-7594 -

WATER Sep,1998 Co-60 46.15

  • 8.78 42.34 32.34 - 52.34 SPW-7594 WATER -

Sep,1998 I-131 77.97

  • 0.81 82.07 65.66 - 98.48 SPW-7594 WATER Sep,1998 I-131(g) -

80.62 13.90 82.07 49.24 - 92.07 j

SPVE-7596 VEGETATION Sep,1998 I-131(g) 2.61

  • 0.08 2.46 1.48 - 3.44 AL SeP,1998 I-131(g) 1.41
  • 0.06' 1.28 0.77 - 1.79 SPCH-7615 CgAR ER SPF-1602 FISH Oct,1998 Cs-137 0.56 0.04 0.61 0.37 - 0.85 SPW-8178~

WATER Oct,1998 Gr. Alpha 25.22

  • 1.90 33.96 16.98 - 50.94 SFW-8178 WATER Oct,1998 Gr. Beta 30.20
  • 1.31 30.36 20.36 - 40.36 SPW-8179 WATER Oct,1998 Ra-226 11.12 t 0.16 13.80 9.66 - 17.94 SPW-8179 WATER Oct,1998 Ra-228 17.83 1.87 17.09 11.96 - 22.22 SPAP-8457 AIR FILTER Oct,1998 Cs-137 -

1.78

  • 0.02 1.84 1.10 - 2.58 3 PAP-8567 '

AIR FILTER ~ Oct,1998 Gr. Beta 6.54

  • 0.10 6.47 0.00 - 16.47 SPSO-9953 SOIL Oct,1998 Cs-134 0.08
  • 0.01 0.09 0.05 - 0.12 SPSO-9953

. SOIL Oct,1998 Cs-137 0.45

  • 0.01 0.43 0.26 - 0.60 SPW-9386 WATER Nov,1998 Ra-226 14.75
  • 0.47 13.80 9.66 - 17.94 SPW-9386 WATER Nov,1998 Ra-228 15.67
  • 1.59 16.95 11.87 - 22.04

. SPW-9387 WATER Nov,1998 Gr. Alpha 27.49 2.38 33.97 16.99 - 50.96 SPW-9387 WATER Nov,1998 Gr. Beta 36.04

  • 2.14 30.31 20.31 - 40.31 SPW-10347 WATER Nov,1998 Sr-90 4.30
  • 1.10 3.20 0.00 - 13.20 SPW-10345 WATER Nov,1998 H 38980.00
  • 548.00 38848.00 31078.40 - 46617.60 SPW-10340' WATER Dec,1998 Ra-226 6.73
  • 0.25 6.89 4.82 - 8.96 SPW-10340 WATER Dec,1998 Ra 228 7.44
  • 1.77 8.40 5.88 - 10.92 SPW-10341'.

WATER Dec,1998 Gr. Alpha 49.30

  • 3.35 33.97 16.99 - 50.96

. SPW-10341 WATER Dec,1998 Gr. Beta 33.63

  • 1.70 30.25 20.25 - 40.25 SPW-10389 WATER Dec,1998 U 4.10
  • 0.25 4.17 2.50 - 5.84

~ SPW-10390 WATER Dec,1998 U 4.29

  • 0.25 4.17 2.50 - 5.84
  • All results are in pCi/L, except for elemental potassium (K) in milk, which are in mg/L.; air filter samples, which are in pCi/ Filter; and food products, which are in mg/kg.

" All samples are the results of single determinations.

  • Controllimits are based on Attachment A, page A2 of this report.

NOTE: For fish, Jello is used for the spike matrix. For vegetation, Sawdust is used for the spike matrix.

A3-3

n

- Table A-4.

In-house " blank" samples.

Concentration pCi/L*.

Teledyne Results Acceptance Lab Sample Sample (4.65 Sigma)

Criteria Code Type Date Analysis LLD Activity *

(4.66 Sigma)

RA-1 WATER Jan1998 Ra-226

<0.015 0.018 0.011

<1.00 RA-1 WATER Jan1998 Ra-228

<0.8745 0.657 0.486

<1.00 SPW-333 WATER Jan1998 Am-241

<0.0934 0.015

  • 0.068

<1.00 SPW-495 WATER Jan 1998 Gr. Alpha

<0.3138 0.004 0.206

<1.00 SPW-495 WATER Jan1998 Gr. Beta

<0.8107 1.475

  • 0.612

< 3.20 SPW-495 WATER Jan1998 Sr-90

<0.8595 0.552 0.461

<1.00 SPMI-496 MILK Jan1998 Sr-89

<0.9576 0.595 0.864

< 5.00 SPMI-496 MILK Jan1998 Sr-90 N/A 0.813 *0300

<1.00 Low level of Sr-90 concentration in milk (1-5 pCi/L) is not unusual.

SPW-593 WATER Jan1998 H-3

<156.02 10.408 77.815

< 200.00 SPAP-5331 AIR FILTER Jan1998 Cs 137

<0.0009 0.000

  • 0.001

< 10.00 SPW-1662 WATER Feb 1998 Ra-226

<0.0134 0.041

  • 0.010

<1.00 SPW-1662 WATER Feb 1998 Ra-228

<0.889 0.386

  • 0.548

<1.00 SPW-793 WATER Febl998 I-131

<0.3448

-0.351 0.140

<0.50 SPMI-794 MILK Feb 1998 I-131

<0.3849

-0.005

  • 0.190

< 0.50 SPAP-749 AIR FILTER Feb 1998 Gr. Beta

<0.6 0.109

  • 0.381

< 3.20 SPW-1664 WATER Mar 1998 Ra-226

<0.0197 0.029 0.013

<1.00 SPAP-1729 AIR FILTER Mar 1998 Gr. Beta

<0.0014 0.000 0.001

< 3.20 SPW-1997 WATER Apr1998 Ra-226

<0.0139 0.006

  • 0.011

<1.00 SPW-2279 WATER Apr1998 H-3

<156.87 54.220

  • 80.200

< 200.00 SPW-2285 WATER Apr1998 Gr. Alpha

<0.3124

-0.056

  • 0.199

<1.00 SPW-2285 WATER Apr1998 Gr. Beta

<0.8822

-0.356

  • 0.569

< 3.20 SPMI-5450 MILK Apr1998 Cs-137

<5.27 0.529

  • 2.640

< 10.00 SPW-5458 WATER Apr1998 Co-60

<1.63

-1.930 15.900

< 10.00 SPW-5458 WATER Apr1998 Cs-137

<4.01 0.464 3.070

< 10.00 SPW-2976 WATER May1998 Ra-226

<0.0115 0.015 1 0.010

<1.00 SPW 2976 WATER May1998 Ra-228

<0.865 0.152

  • 0.420

<1.00 SPAP-3042 AIR FILTER May1998 Cs-137

<0.0010 0.000

  • 0.001

< 10.00 SPW-3044 WATER May1998 Gr. Alpha

<0.5036

-0.184 0.251

<1.00 i

SPW-3044 WATER May1998 Gr. Beta

<1.1494 0.140

  • 0.643

< 3.20 SPW-4161 WATER Jun1998 Ra-226

<0.0203 0.049

  • 0.014

<1.00 SPW-4161 WATER Jun1998 Ra-228

<0.802 0.221 0.400

<1.00 I

SPW-5339 WATER Jun1998 Gr. Alpha

<0.4785 0.098 2 0.322

<1.00 SPW-5339 WATER Jun1998 Gr. Beta

<1.0833 1.037

  • 0.735

< 3.20 SPW-4719 WATER Jul1998 Ra-226

<0.0117 0.047 0.010

<1.00 A4-1

F l

[

Table A-4.

In-house " blank" samples.

Concentration pCi/L'.

Teledyne Results Acceptance Lab Sample Sample (4.66 Sigma)

Criteria Code Type Date Analysis LLD Activity" (4.66 Sigma) l SPW-4719 WATER Jul1998 Ra-228

<0.435 0.389 2 0.251

<1.00 l

SPCH-5128 CHARCOAL Jul1998 I-131(g)

<0.0088

-0.001

  • 0.007

< 9.60 CANISTER SPMI-5130 MILK Jul1998 Co-60

<2.60

-1.090 25.300

< 10.00 SPMI-5130 MILK Jul1998 Cs-137

<4.43

-1.510 2.690

< 10.00 SPMI-5130 MILK Jul1998 I131

<0.444

-0.141 0.239

<0.50 SPMI-5130 MILK Jul1998 I-131(g)

<6.94

-1.710 t7.030

< 20.00 SPMI-5130 MILK Jul1998 Sr-90 N/A 1.320

  • 0.370

<1.00 Low level of Sr-90 concentration in milk (15 pCi/L) is not unusual.

SPW-5132 WATER Jul1998 H-3

<157

-81.700

  • 74.150

< 200.00 SPW-5135 WATER Jul1998 I131

<0.2796

-0.059

  • 0.152

< 0.50 SPW-5135 WATER Jul1998 Co-60

<1.90 3.260

  • 3.920

< 10.00 SPW-5135 WATER Jul1998 Cs-137

<3.29 1.110

  • 2.930

< 10.00 SPW-5135 WATER Jul1998 I-131(g)

<8.41 2.660

  • 7.660

< 20.00 SPW 5135 WATER Jul1998 Gr. Alpha

<0.3589 0.486

  • 0.274

<1.00 SPW-5135 WATER Jul1998 Gr. Beta

<0.8127 0.791 0.552

< 3.20 SPW-6093 WATER Aug1998 Gr. Alpha

<0.3766 0.104 t0.317

<1.00 SPW-6093 WATER Aug1998 Gr. Beta

<1.741

-0.339 t0.839

< 3.20 SPW-6093 WATER Aug1998 Ra-226

<0.0166 0.053 t0.012

<1.00 l

SPW-6093 WATER Aug1998 Ra-228

<0.670

-0.050 t0.304

<1.00 SPW-7145 WATER Sep1998 Gr. Alpha

<0.2485 0.192

  • 0.191

<1.00 SPW-7145 WATER Sep 1998 Gr. Beta

<0.7483 0.391 to.533

< 3.20 SPW-7145 WATER Sep1998 Ra-226

<0.0192 0.020

  • 0.012

<1.00 SPW-7145 WATER Sep1998 Ra-228

<0.997 0.033

  • 0.562

<1.00 SPAP-7395 AIR FILTER Sep 1998 Gr. Beta

<0.002

-0.001 0.001

< 3.20 SPMI-7593 MILK Sep1998 Cs-137

<5.41 1.470

  • 3.560

< 10.00 SPMI-7593 MILK Sep1998 I-131

<0.4127

-0.257 0.215

< 0.50 4

l SPMI 7593 MILK Sep 1998 I 131(g)

<9.60 4.120

  • 24.900

< 20.00 SPW-7595

' WATER Sep1998 Co-60

<4.60 2.320 ti.340

< 10.00 SPW-7595 WATER Sep1998 I-131

<0.2981

-0.223

  • 0.153

< 0.50 SPW-7595 WATER Sep1998 I-131(g)

<8.71 2.820

  • 6.660

< 20.00 SPVE-7597 VEGETATION Sep1998 I-131(g)

<0.0166

-0.001

  • 0.001

< 20.00 SPW-8180 WATER Oct1998 Ra-226 N/A 0.049

  • 0.015

<1.00 SPW-8180 WATER Oct1998 Ra-226

<0.0209 0.049 2 0.015

<1.00 SPW-8180 WATER Oct1998 Ra-228

< 0.840 0.666

  • 0.465

<1.00 A4-2 1

l Table A-4.

In-house " blank" samples.

j Concentration pCi/L*.

Teledyne Results Acceptance Lab Sample Sample (4.66 Sigma)

Criteria Code Type Date Analysis LLD Activity" (4.66 Sigma)

SPW-9388 WATER Novi998 Gr. Alpha

<0.74 0.270 2 0.480

<1.00 SPW-9388 WATER Novl998 Gr. Beta

<1.99 1.036 1.244

< 3.20 SPW-9388 WATER Nov1998 Ra-226

< 0.0203 0.039 0.013

<1.00 SPW-9388 WATER Novi998 Ra-228

<0.932 0.317 0.561

<1.00 SPW-10344 WATER Novi998 H-3

<175

-8.130

  • 86.410

< 200.00 SPW-10339 WATER Dec1998 Gr. Alpha

<0.95

-0.650

  • 0.570

<1.00 SPW 10339 WATER Dec1998 Gr. Beta

<1.80

-0.280

  • 1.180

< 3.20 SPW-10339 WATER Dec1998 Ra-226

<0.0261 0.020

  • 0.015

<1.00 SPW-10339 WATER Dec1998 Ra-228

<0.83 c 0.244 *0.418

<1.00

  • Liquid sample results are reported in pCi/ Liter, air filter sample results are in pCi/ filter, charcoal sample results are in pCi/ charcoal, and solid sample results are in pCi/ kilogram.
  • 'Ihe activity reported is the net activity result.

4 i

i i

A4-3

r.

Table A-5.

In-house " duplicate" samples.

Concentration in pCi/L' Lob Sample First Second Averaged Codes" Date Analysis Result Result Result WW-10052, 20053 Jan,1998 Gr. Beta 1.1720 2 0.6030 2.1820 t 0.6630 1.6770

  • 0.4481 CF-20, 21 Jan,1998 Gr. Beta 17.5458
  • 0.5866 17.6346 0.5614 17.5902 0.4060 CF-20, 21 Jan,1998 K-40 21.1870 0.6570 20.8610 0.7520 21.0240 0.4993 CF-20, 21 Jan,1998 Sr-90 0.0302 0.0085 0.0298
  • 0.0071 0.0300
  • 0.0055 WW-195,196 Jan,1998 Gr. Beta 2.9349
  • 0.6584 2.9020
  • 0.6291 2.9185
  • 0.4553 SW-298, 299 Jan,1998 H-3 144.2200 93.5400 92.1100 91.4500 118.1650
  • 65.4080 SW-349, 350 Jan,1998 Co-60 L1100 9.1700 1.7900
  • 2.4700 1.4500
  • 4.7484 SW-349, 350 Jan,1998 Cs-137

-2.4900 3.2300

-0.6700 2 1.9400

-1.5800 1.8839 CW-737,738 Jan,1998 H-3 559.2800 100.4400 524.8100 99.1900 542.0450 70.5812 PW-607, 608 Jan,1998 Co-60 0.3400 0.0340 0.7200 4.6200 0.5300 2 2.3101 PW-607, 608 Jan,1998 Cs-137 1.1700 1.8100

-0.0400

  • 1.8700 0.5650 L3012 SWU-531, 532 Jan,1998 Gr. Beta 3.4928 0.6902 3.9923 0.7129 3.7426 0.4961 LW-653, 654 Jan,1998 Gr. Beta 2.3404 0.5778 1.6742 1 0.5968 2.0073 0.4153 SW-587, 588 Feb,1998 Gr. Beta 3.2097 0.7915 2.1021
  • 0.7800 2.6559 0.5556 WW-897, 898 Feb,1998 Co-60 0.2600
  • 0.4800 0.4700 4.5900 0.3650 2.3075 WW-897, 898 Feb,1998 Cs-137 0.2800 1.8700 0.3200
  • 2.5200 0.3000 1.5690 WW-897, 898 Feb,1998 H-3 4,582.7400
  • 197.9300 5,013.4400
  • 205.6500 4,798.0900
  • 142.7132 CW-920,921 Feb,1998 Gr. Beta 8.1600
  • 1.3000 8.5200
  • 1.3000 8.3400 0.9192 CW-920, 921 Feb,1998 Gr. Beta 0.2500 1.2100 0.0000 1.2000 0.1250
  • 0.8521 CW-1378,1379 Mar,1998 Gr. Beta 2.6100 1.3700 4.1400
  • 1.5800 3.3750 1.0456 CW-1378,1379 Mar,1998 Gr. Beta

-0.1000 1.1000 0.0000 1.2000

-0.0500 0.8139 MI-1552,1553 Mar,1998 K-40 1,392.5000 133.0000 1,280.8000

  • 204.0000 1,336.6500 121.7631 WW-1406,1407 Mar,1998 Gr. Beta 7.0991 1 0.8467 7.0712
  • 0.5658 7.0852
  • 0.5092 LW-1921,1922 Mar,1998 Gr. Beta 2.9722
  • 0.6466 2.5972
  • 0.6466 2.7847
  • 0.4572 AP-2599,2600 Mar,1998 Co-60

-0.0003

  • 0.0004

-0.0003 0.0002

-0.0003

  • 0.0002 AP-2599,2600 Mar,1998 Cs-137

-0.0001 0.0004 0.0001 0.0005 0.0000

  • 0.0003

]

SW-2040, 2041 Mar,1998 H-3 6,004.3600

  • 224.0000 6,322.4700
  • 229.1400 6,163.4150
  • 160.2195

]

SW - 2040,2041 Mar,1998 H-3 6,322.4678

  • 229.1356 6,004.3639
  • 224.0020 6,163.4158 160.2186 i

AP-2620,2621 Mar,1998 Co-60 0.0005 2 0.0004 0.0009 i 0.0027 0.0007 0.0013 AP-2620,2621 Mar,1998 Cs-137 0.0005

  • 0.0005

-0.0000

  • 0.0006 0.0002
  • 0.0004 i

LW-2253,2254 Mar,1998 Gr. Beta 1.9075

  • 0.7042 2.1691 i 0.7478 2.0333 0.5136 AP-2487,2488 Mar,1998 Be-7 0.0569 0.0071 0.0601 0.0008 0.0585 0.0035 E-1966,1967 Apr,1998 Gr. Beta 1.1740
  • 0.0530 1.1530 0.0530 1.1635
  • 0.0375 E-1966,1967 Apr,1998 K-40 1.3900 0.1300 1.2422 0.1700 1.3161 0.1070 AP-2466,2467 Apr,1998 Be-7 0.0693 0.0158 0.0605 0.0113 0.0649 0.0097 WW-2012, 2013 Apr,1998 Co-60 0.6300 0.6200 2.6700
  • 2.3500 1.6500 1.2152 I

\\

)

A5-1 i

I

Table A-5.

In-house " duplicate" sarnples.

Concentration in pCi/I

  • Lab Sample First Second Averaged Codes
  • Date Analysis Result Result Result WW-2012, 2013 Apr,1998 Cs-137 0.5800 1.5600 1.2800 2.2800 0.9300 1.3813 WW-2012, 2013 Apr,1998 H-3 616.5800
  • 100.3800 646.9400 t 101.4600 631.7600 71.3622 MI-2112,2113 Apr,1998 I-131

-0.0500 0.1600

-0.0500 t 0.1700

-0.0500 0.1167 CW-2225,2226 Apr,1998 Gr. Beta 1.8900 1.4200 2.6400 1.4100 2.2650 1.0006 CW-2225,2226 Apr,1998 Gr. Beta

-1.2600

  • 1.0300 0.1500 t 1.2500

-0.5550 0.8098 SWU-2302, 2303 Apr,1998 Gr. Beta 3.4606

  • 0.6485 3.2027
  • 0.6811 3.3317 0.4702 SWU-2302, 2303 Apr,1998 H-3 435.3500
  • 96.3410 593.3260 102.1870 514.3380 2 70.2207 CW-2325,2326 Apr,1998 Gr. Beta 16.1700 2.4300 14.3400 2.1600 15.2550 1.6256 CW-2325,2326 Apr,1998 Gr. Beta 5.0100 2 1.5900 5.9000
  • 1.7300 5.4550 1.1748 BS 2508,2509 Apr,1998 Cs-137 0.3186
  • 0.0538 0.2849
  • 0.0601 0.3018 0.0403 BS-2508, 2509 Apr,1998 Gr. Alpha 15.5814
  • 2.8742 15.4353
  • 5.7607 15.5084 3.2190 BS-2508, 2509 Apr,1998 Gr. Beta 26.4292 2.2859 30.1462
  • 4.3906 28.2877 2.4750 BS-2508, 2509 Apr,1998 K-40 18.6870
  • 1.2400 17.6740
  • 0.9500 18.1805 0.7810 BS-2508, 2509 Apr,1998 Sr-90 0.0490
  • 0.0150 0.0280
  • 0.0130 0.0385 t 0.0099 G-2531,2532 Apr,1998 Cs-137 0.2387 0.0353 0.2089
  • 0.0182 0.2238 i 0.0199 G-2531,2532 Apr,1998 K-40 10.2470
  • 0.5750 9.3951
  • 0.3670 9.8211 0.3411 DW-2790,2791 Apr,1998 Gr. Alpha 0.3001 t 0.2051 0.1634 0.2668 0.2318 0.1683 DW-2790,2791 Apr,1998 Gr. Beta 0.5947 i 0.2942 0.7350
  • 0.3478 0.6649 0.2278 MI-2368,2369 Apr,1998 K-40 1,176.4000
  • 162.0000 1,374.6000 108.0000 1,275.5000
  • 97.3499 MI-2368,2369 Apr,1998 Sr-89 0.2160
  • 1.0300

-0.3060 1.2300

-0.0450 0.8022 MI-2368,2369 Apr,1998 Sr-90 1.5430

  • 0.4910 1.1744
  • 0.4060 1.3587 0.3186 CW-3411,2412 Apr,1998 Gr. Beta 2.2800 1.0500 3.0100 1.5100 2.6450
  • 0.9196 SWU-2067, 2068 Apr,1998 Gr. Beta 2.4865
  • 0.7089 3.3197
  • 0.6627 2.9031
  • 0.4852 SS-2666, 2667 Apr,1998 Cs-137 0.0395
  • 0.0194 0.0299 0.0133 0.0347
  • 0.0118 SS-2666, 2667 Apr,1998 Gr. Beta 9.0977 2.0893 6.7058 1.9219 7.9018 1.4194 SS-2666, 2667 Apr,1998 K-40 5.3384
  • 0.2820 5.9439 0.4020 5.6412 0.2455 WW-2701, 2702 Apr,1998 H-3 184.5500
  • 86.5200 223.1700 88.1500 203.8600
  • 61.7579 WW-2850, 2851 Apr,1998 Co-60

-0.1700 1.6000

-0.3400 6.3800

-0.2550 3.2888 WW-2850, 2851 Apr,1998 Cs-137 0.2900 2.4800 2.1600

  • 2.0300 1.2250 1.6024 WW-2850, 2851 Apr,1998 H-3 5,665.6200
  • 217.4400 5,770.5600
  • 219.2100 5,718.0900 154.3804 SS-3004, 3005 Apr,1998 Gr. Alpha 6.6840
  • 4.0000 6.9820 4.4020 6.8330
  • 2.9740 SS.3004, 3005 Apr,1998 Gr. Beta 19.9460 i 3.1700 20.7720
  • 3.1970 20.3590
  • 2.2511 SS-3004, 3005 Apr,1998 K-40 15.1560
  • 0.9910 13.9010 0.5860 14.5285 0.5756 i

BS-3240, 3241 Apr,1998 Gr. Beta 7.5126 1.9277 8.4047 1.9386 7.9587 1.3669 BS-3240, 3241 Apr,1998 K-40 10.2890 x 0.5380 10.1520 2 0.3430 10.2205 0.3190 MI-2941,2942 May,1998 K-40 1,209.3000 152.0000 1,422.5000 193.0000 1,315.9000

  • 122.8342 i

A5-2

i f

Table A-5.

In-hcuse " duplicate" samples.

Concerstration in pCi/I' Lab Sample First Second Averaged 6

Codes Date Analysis Result Result Result S O-2962, 2963 May,1998 Cs-137 0.1835 0.0463 0.1531 0.0261 0.1683 0.0266 S O-2962, 2963 May,1998 Gr. Alpha 9.7590 3.4730 10.3360

  • 3.5720 10.0475 2.4910 l

S O-2962, 2963 May,1998 Gr. Beta 27.2230 2.8430 31.4690 3.0280 29.3460 2 2.0767 S O-2962, 2963 May,1998 K-40 23.0890 1.1600 21.6540

  • 0.8142 22.3715 0.7086 S O-2962, 2963 May,1998 Sr-90 0.0421 t 0.0117 0.0396 t 0.0146 0.0408 0.0094 LW 3048,3049 May,1998 Gr. Beta 1.9020
  • 0.6920 2.0920
  • 0.7010 1.9970 0.4925 WW-3097, 3098 May,1998 Gr. Beta 4.6000
  • 0.6640 4.4740
  • 0.6600 4.5370 0.4681 WW - 3173,3174 May,1998 H-3 155.2485
  • 83.4086 153.4076
  • 83.3273 154.3280 58.9500 F-3305,3306 May,1998 Gr. Beta 2.9966 0.1303 2.8744 0.1364 2.9355
  • 0.0943 F-3305,3306 May,1998 K-40 2.5354
  • 0.3690 2.5317 0.4260 2.5336 0.2818 SS-3463, 3464 May,1998 K-40 13.2060 0.6940 12.1740
  • 0.5670 12.6900
  • 0.4481 F - 3284,3285 May,1998 Co-60 0.0073 0.0286

-0.0054 0.0097 0.0009 2 0.0151 F - 3284,3285 May,1998 Cs-137

-0.0001 t 0.0047 0.0080 0.0095 0.0039 0.0053 CW - 3439,3440 May,1998 Gr. Beta 2.1268 1.3641 2.0093 1.1263 2.0681

  • 0.8845 G-3546,3547 May,1998 Be 7 0.7130
  • 0.2340 0.6940 0.1850 0.7035 0.1491 G-3546,3547 May,1998 Gr. Beta 10.7190 0.3340 10.9340
  • 0.3370 10.8265
  • 0.2372

(

G-3546,3547 May,1998 K-40 7.5468

  • 0.5310 7.8713 0.6930 7.7091 0.4365 BS-3669,3670 May,1998 Cs 137 0.2010
  • 0.0535 0.2022 0.0215 0.2016 0.0288 l

BS-3669,3670 May,1998 K-40 14.9080

  • 0.4820 16.1580 1.0800 15.5330 0.5913 F-3694,3695 May,1998 K-40 1.7695
  • 0.2850 1.6797
  • 0.3440 1.7246
  • 0.2234 PW - 3572,3573 May,1998 H3 49.8073
  • 97.6829 83.0122 98.9291 66.4098 69.5142 WW - 3763,3764 May,1998 Co-60 0.0478 0.0234 0.0551
  • 0.0311 0.0515 0.0195 WW - 3790,3791 May,1998 Co-60

-0.0847 0.6250 0.5220 10.9000 0.2187

  • 5.4590 WW - 3790,3791 May,1998 Cs-137 0.9210 1.9700 1.1200
  • 1.5000 1.0205
  • 1.2380 WW - 3790,3791 May,1998 H-3 723.8914
  • 114.0882 705.2824
  • 113.4795 714.5869 80.4576 F - 3715,3716 May,1998 Co-60

-0.0048

  • 0.0567 0.0077
  • 0.0214 0.0015 0.0303 l

F - 3715,3716 May,1998 Cs-137 0.0015 0.0090 0.0127

  • 0.0137 0.0071
  • 0.0082 l

BS - 3763,3764 May,1998 Cs-137 0.0884

  • 0.0206 0.0754
  • 0.0257 0.0819 0.0165 SWU-3882, 3883 May,1998 Gr. Beta 2.9052 0.6786 3.7390
  • 0.6595 3.3221 0.4731 SWU-3882, 3683 May,1998 H-3 43.3000 79.9590 34.1540 79.5400 38.7270 56.3916 CW-4314,4315 May,1998 H-3 441.3905 96.6703 424.7922
  • 96.0349 433.0913
  • 68.1319 F-3861,3862 May,1998 K-40 3.2973
  • 0.5280 3.6404 t 0.3530 3.4689 0.3176 CW - 4044,4045 May,1998 Gr. Beta 4.6775 1.6138 4.8186
  • 1.6342 4.7481 2 1.1484 CW - 4044,4045 May,1998 Gr. Beta

-0.7495 i 1.2072

-0.6833

  • 1.0704

-0.7164 0.8067 SW 4020,4021 Jun,1998 K-40 (FP) 1.0380 1.0380 1.0380 AP-4111,4112 Jun,1998 Be-7 0.1860 1 0.0833 0.2650

  • 0.1120 0.2255
  • 0.0698 A5-3 l

Table A-5.

In-house " duplicate" samples.

Concentration in pCi/L' Lab Sample First Second Averaged Codd Date Analysis Result Result Result ~

P-4183,4184 Jun,1998 H-3 22.7850 81.0520 44.7120 81.6170 33.7485

  • 57.5125 CW - 4195,4196 Jun,1998 Gr. Beta 2.9189 1.4811 2.8922 1.4740 2.9055 1.0448 CW - 4195,4196 Jun,1998 Gr. Beta

-0.4892 1.0638

-0.4909 1.1091

-0.4900 0.7684 WW-4410, 4411 Jun,1998 Gr. Beta 4.9907

  • 0.7658 5.7601 0 S338 5.3754
  • 0.5661 WW-4410, 4411 Jun,1998 H-3

-5.3910

  • 77.2770 66.4880
  • 80.5500 30.5485 55.8123 MI-4389,4390 Jun,1998 Co-60 0.1420 0.2080 1.4200
  • 13.6000 0.7810 6.8008 MI-4389,4390 Jurg1998 Cs-137 0.1810 t 2.7600 0.6020
  • 4.0700 0.3915 2.4588 MI-4389,4390 Jurt1998 I-131

-0.0469 0.2433

-0.1152 0.2559

-0.0811 0.1765 AP-4664,4665 Jurg1998 Be-7 0.1539 0.0750 0.2627 0.1220 0.2083 0.0716 MI-4685,4686 Jurt 1998 I-131

-0.1010 0.1620

-0.0221 0.1728

-0.0616 0.1184 SW - 4901,4902 Jun,1998 H-3 2,541.2239 156.4571 2,510.5125 1 155.7462 2,525.8682 110.3808 AP-5188,5189 Jun,1998 Be-7 0.0844 0.0163 0.0733 0.0117 0.0789 0.0100 SWU-4798, 4799 Jurv1998 Gr. Beta 1.9402 0.5398 1.8412

  • 0.5411 1.8907 0.3822 LW-4993,4994 Jun,1998 Gr. Beta 3.1224 0.6129 2.0740 0.5328 2.5982 0.4061 LW-4993,4994 Jun,1998 H-3 3,543.4600 184.5020 3,482.0770
  • 183.2600 3,512.7685 130.0242 WW-4819, 4820 Jul,1998 Gr. Beta 1.2760 0.6431 0.7313
  • 0.6161 1.0037 0.4453 WW-4819, 4820 Jul,1998 K-40 0.8650 0.0865 0.9515
  • 0.0950 0.9083
  • 0.0642 AP-5209,5210 Jul,1998 Be-7 0.1079 0.0180 0.0901 c 0.0107 0.0990 0.0105 AP-5392,5393 Jul,1998 De-7 0.0782
  • 0.0143 0.0885
  • 0.0144 0.0833 0.0101 AP-5413,5414 Jul,1998 Be-7 0.0625
  • 0.0072 0.0718
  • 0.0091 0.0671 0.0058 WW-4848, 4849 Jul,1998 Co-60 0.2220
  • 0.1290 0.5080
  • 0.8150 0.3650 0.4126 WW-4848, 4849 Jul,1998 Cs-134 0.9310
  • 2.0500 0.8130
  • 0.8130 0.8720
  • 1.1027 WW-4848, 4849 Jul,1998 Cs-137 0.7040 1.8700

-0.1190 1.8300 0.2925 1.3082 WW-4848, 4849 Jul,1998 H-3 37.2000

  • 89.2000

-13.0000

  • 87.0000 12.1000 62.3010 CW-4947,4948 Jul,1998 Gr. Beta 5.2400 1 1.5700 5.1900 1.5700 5.2150 1.1102 SW-7804, 7805 Jul,1998 Gr. Alpha 0.3147
  • 0.6025 1.7030 0.5568 1.0089
  • 0.4102 SW 7804,7805 Jul,1998 Gr. Beta 2.0032
  • 0.7183 2.5489
  • 0.6474 2.2761 0.4835 WW-4880, 4881 Jul,1998 Co-60 0.2540
  • 0.6210

-0.4430 0.8250

-0.0945 0.5163 WW-4880, 4881 Jul,1998 Cs-137 1.4600 1.2800 1.1400 2 2.0000 1.3000 1.1873 WW-4880, 4881 Jul,1998 H-3 308.5000 102.7000 328.9000 103.5000 318.7000 72.9033 G-5090,5091 Jul,1998 Be-7 1.5334

  • 0.2310 1.5696 0.2550 1.5515 0.1720 G-5090,5091 Jul,1998 K-40 6.2521
  • 0.4900 6.0430 0.4800 6.1476
  • 0.3430 SW-5281, 5282 Jul,1998 Gr. Alpha 5.7564
  • 1.0355 5.4517 i 0.9702 5.6041 0.7095 SW-5281, 5282 Jul,1998 Gr. Beta 8.8798
  • 0.7835 9.9157 0.8418 9.3978 i 0.5750 SW 5281,5282 Jul,1998 H-3 12.9950 1 87.9900 46.4090
  • 89.3890 29.7020 62.7149 VE 5323,5324 Jul,1998 K-40 9.4179 1 0.7440 8.3494 i 0.4700 8.8837 0.4400 A5-4

)

I Table A-5.

In-house " duplicate" samples.

l Concentrationin pCi/L'

)

Lsb Sarnple First Second Averaged.

Codes

  • Date Analysis Result Result Result SWU-5744, 5745 Jul,1998 Gr. Beta 2.0648 0.5650 2.4432
  • 0.6352 2.2540
  • 0.4251 VE-5302,5303 Jul,1998 Gr. Alpha 0.1233
  • 0.0458 0.0816 0.0381 0.1025
  • 0.0298 VE-5302,5303 Jul,1998 Gr. Beta 3.8738
  • 0.1201 3.4382
  • 0.1081 3.6560 0.0808 1

VE-5302,5303 Jul,1998 K-40 3,845.0000 384.0000 3,561.0000 419.0000 3,703.0000

  • 284.1729 G-5346,5347 Jul,1998 Be-7 1.0649
  • 0.3460 1.1877
  • 0.2220 1.1263 0.2055 G-5346,5347 Jul,1998 Gr. Beta 5.5890
  • 0.2200 5.4932 0.1571 5.5411 0.1352 G-5346,5347 Jul,1998 K-40 5.8497
  • 0.7760 6.4013
  • 0.5600 6.1255 0.4785 AP-5371,5372 Jul,1998 Be-7 0.2899
  • 0.0987 0.2565 0.0949 0.2732 0.0685 AP-5530,5531 Jul,1998 Be-7 0.2559
  • 0.0941 0.3365 0.0984 0.2962 0.0681 S 0-5556, 5557 Jul,1998 Gr. Beta 17.8997
  • 2.6057 15.8321 2.3577 16.8659 1.7570 CW-6134,6135 Jul,1998 Gr. Beta 4.8400 2 1.2300 4.0700 1.0900 4.4550 0.8217 j

AP-5721,5722 Jul,1998 Be-7 0.2175 0.0616 0.2461

  • 0.1180 0.2318 0.0666 SWU-5744, 5745 Jul,1998 H-3 223.9760 86.8830 209.4480 86.2730 216.7120 61.2203 WW-5836, 5837 Jul,1998 H-3 89.4980 80.6500 65.9720
  • 79.9940 73.2350 56.7967 WW-6176, 6177 Jul,1998 H-3 31.0590 81.2420 1.8270
  • 79.9170 16.4430 56.9802 WW-6176, 6177 Jul,1998 Gr. Beta 0.6954
  • 0.5544 1.3234
  • 0.5462 1.0094
  • 0.3891

)

LW-5965,5966 Aug,1998 Gr. Deta 3.1093 0.6160 2.2762

  • 0.6288 2.6928 0.4401 LW-5965,5966 Aug,1998 H-3 80.4580 1 82.3350 36.5020
  • 80.3920 58.6800 57.5368 G-5986,5987 Aug,1998 Be-7 2.2321 t 0.3670 1.9885 0.3010 2.1103
  • 0.2373 G-5986,5987 Aug,1998 K-40 5.4909 0.6280 6.3514
  • 0.7550 5.9212 0.4910 CW-6013,6014 Aug,1998 Gr. Beta 0.5400 1 1.2300 0.9900 1.2500 0.7650 0.8768 1

CW-6134,6135 Aug,1998 Gr. Beta 3.2200 1.5200 4.1200 1.1600 3.6700

  • 0.9560 F-6447,6448 Aug,1998 Gr. Beta 2.1416 0.0774 1.9173
  • 0.0791 2.0295 0.0553 F-6447,6448 Aug,1998 K-40 2.1309 0.2570 1.8657
  • 0.1280 1.9983 0.1436 AP-6467,6468 Aug,1998 Be-7 0.1612
  • 0.0873 0.1293
  • 0.1260 0.1453
  • 0.0766 VE-6489,6490 Aug,1998 Cs-134 1.0300 1.8700 0.1500 0.1000 0.5900
  • 0.9363 VE-6489,6490 Aug,1998 Cs-137 0.9500 i l.4300 0.6800
  • 2.0400 0.8150 1.2456 AP-6722,6723 Aug,I M Be-7 0.3063
  • 0.1590 0.3100
  • 0.0937 0.3082 0.0923 VE-6774,6775 Aug,1998 Be-7 0.5894 0.2720 0.4208 0.1520 0.5051 0.1558 VE-6774,6775 Aug,1998 Gr. Beta 5.9406 0.1789 5.6841 0.1706 5.8124
  • 0.1236 CW-6800,6801 Aug,1998 Gr. Beta 2.2300
  • 1.4400 2.1300 1.3100 2.1800 i 0.9734 l

LW-7129,7130 Aug,1998 Gr. Alpha 0.6433 0.3557 0.5551

  • 0.3614 0.5992 0.2535 LW-7129,7130 Aug,1998 Gr. Beta 2.4016 0.4281 2.3041 0.4447 2.3529 0.3086 LW-7129,7130 Aug,1998 H-3 170.2100
  • 87.3900 37.4100 81.5000 103.8100 59.7479 LW-7129, 7130 Aug,1998 H-3 154.7950 94.8090 104.6950 92.7500 129.7450
  • 66.3161 S 0-6943, 6944 Sep,1998 Co-60 0.1466 0.0399 0.1452
  • 0.0303 0.1459
  • 0.0251 i

A5-5 t

l l

Table A-5.

In-house " duplicate" samples.

Concentration in pCi/L' Lab Sample First Second Averaged 6

Codes Date Analysis Result Result Result ~

S O-6943, 6944 Sep,1998 Cs-137 15.1000 0.2000 15.7000 0.3000 15.4000 0.1803 5 0-6943, 6944 Sep,1998 K-40 16.5680 0.7660 17.3780 1.1000 16.9730 0.6702 CW-7043,7044 Sep,1998 Gr. Beta 4.5000 1.6000 4.9000 1.5000 4.7000 1.0966 VE-7250,7251 Sep,1998 Cs-134 0.0800 1.1800 0.4600 0.5100 0.2700 2 0.6427 VE-7250,7251 Sep,1998 Cs-137 0.1300

  • 0.7200 0.0100 0.3400 0.0700 0.3981 VE-7064,7065 Sep,1998 Cs-134

-0.1100 0.0800 0.1200 1.4900 0.0050 0.7461 VE-7064,7065 Sep,1998 Cs-137

-0.3600

  • 0.7600 0.0200 0.8200

-0.1700

  • 0.5590 VE-7171,7172 Sep,1998 Cs-134 0.0600 2 0.5200

-0.1300 13.1000

-0.0350 6.5552 VE-7171,7172 Sep,1998 Cs-137 0.6300

  • 0.5200 0.6800 0.8000 0.6550 0.4771 CW-7204,7205 Sep,1998 Gr. Beta 2.6900 1.4300 1.5600 1.3000 2.1250 0.9663 SW-6363,6364 Sep,1998 Gr. Beta 4.3450
  • 0.7618 4.1456 0.7464 4.2453
  • 0.5333 SW-6363, 6364 Sep,1998 H-3 133.9370
  • 82.9580 148.6820 83.6110 141.3095 58.8915 VE-7279,7280 Sep,1998 K-40 2.1575 0.2580 2.3167 0.3420 2.2371 0.2142 SWU-7452, 7453 Sep,1998 Gr. Beta 4.1567
  • 0.6600 4.1515 0.7395 4.1541
  • 0.4956 F 7819,7820 Sep,1998 K-40 3.0166 0.3920 2.7430 0.5190 2.8798 0.3252 CW-7375,7376 Sep,1998 Gr. Beta 1.7100
  • 1.1500 2.2000 1.1900 1.9550 0.8274 BS-7598,7599 Sep,1998 K-40 9.5919
  • 0.7430 8.9290
  • 0.4590 9.2605 0.4367 AP-7598,7599 Sep,1998 Be-7 0.0639 0.0188 0.0815
  • 0.0156 0.0727 0.0122 VE-7397,7398 Sep,1998 Cs-134 0.1900 2.6800 0.6300
  • 1.3500 0.4100
  • 1.5004 VE-7397,7398 Sep,1998 Cs-137

-0.0900 0.9400 0.5200

  • 0.9500 0.2150 t 0.6682 SWU-7452, 7453 Sep,1998 H-3 23.7170 i 81.6810

-19.3480

  • 79.6820 2.1845
  • 57.0548 SWT-7765,7766 Sep,1998 Gr. Beta 3.2443 0.6638 2.9078
  • 0.6593 3.0761 0.4678 WW - 7831,7832 Oct,1998 Co-60 0.6760
  • 2.3800 1.2100 1.4300 0.9430 1.3883 WW - 7831,7832 Oct,1998 Cs-137 0.2340
  • 1.3900 1.5900 2.1200 0.9120
  • 1.2675 WW - 7831,7832 Oct,1998 H-3 11.8861
  • 81.2490 21.2699 81.6813 16.5780
  • 57.6048 SW 7857,7858 Oct,1998 Gr. Beta 2.3410 0.7265 2.1443
  • 0.7591 2.2427 0.5254 S 0-7878, 7879 Oct,1998 Gr. Beta 19.3527
  • 4.1969 23.2850
  • 4.0731 21.3189 2.9242 S O-7878, 7879 Oct,1998 Sr-90 0.0034
  • 0.0110 0.0080 0.0130 0.0057 0.0085 AP, Oct,1998 Be-7 0.0680
  • 0.0527 0.0931
  • 0.0702 0.0806
  • 0.0439 WW-8073, 8074 Oct,1998 Gr. Beta 2.4196
  • 0.5973 3.1890
  • 0.6509 2.8043
  • 0.4417 WW-8073, 8074 Oct,1998 H-3 90.5270
  • 84.1470 113.3172 85.1690 101.9221
  • 59.8633 SS-8202, 8203 Oct,1998 Cs-137 0.0509 i 0.0284 0.0222
  • 0.0102 0.0365 2 0.0151 SS-8202, 8203 Oct,1998 Gr. Beta 4.5670
  • 1.9890 6.3930 2.0860 5.4800 1.4411 i

SS-8202, 8203 Oct,1998 K-40 7.2289

  • 0.6170 7.1271
  • 0.4380 7.1780
  • 0.3783 SS-8202, 8203 Oct,1998 K-40 6.9700 1 0.5400 7.1800 1 0.3800 7.0750 0.3302 W W 8358,8359 Oct,1998 Gr. Beta 1.0464
  • 0.5347 1.4246
  • 0.5276 1.2355 0.3756 AS-6

j

' Table A-5.

In-house " duplicate" samples.

Concentrationin pCi/I' Lab-Sample First Second Averaged Codes

  • Date Analysis Result Result Result I

WW-8358, 8359 Oct,1998 H 16.2810 2 81.9530 53.8530 83.6580 35.0670 58.5554

. BS - 8270,8271

. Oct,1998 Co-60 0.0151

  • 0.0090 0.0072
  • 0.0884 0.0111 0.0444 l ' ' BS - 8270,8271 Oct,1998 Cs-137 0.0732 0.0186 0.0913
  • 0.0451 0.0823 0.0244 AP, Oct,1998 Be-7 0.1094
  • 0.0878 0.1708
  • 0.0934 0.1401 0.0641 S O-7878, 7879 Oct,1998 K-40 16.3430
  • 0.9100 18.2150
  • 1.1000 17.2790
  • 0.7138 l

SL-8624,8625 Oct,1998 K-40 2.0091

  • 0.4260 1.9401
  • 0.3310 1.9746
  • 0.2697 l

SS-8689, 8690 Oct,1998 K-40 14.8820 2 0.8900 16.8160 1.2200 15.8490 0.7551 l

BS-8864, 8865

' Oct,1998 Co-60 0.1424 0.0225 0.1313

  • 0.0199 0.1368 0.0150 l

BS-8864, 8865 Oct,1998 Cs-137 0.0972 0.0204 0.1081

  • 0.0207 0.1026 0.0145 BS-8864, 8865 Oct,1998 K-40 9.5076
  • 0.4940 10.4040 t 0.5000 9.9558
  • 0.3514 S O-10497, 10498 Oct,1998 K-40 19.0930
  • 1.0800 19.7410
  • 0.9100 19.4170
  • 0.7061 S O-9098, 9099 Oct,1998 Cs-137 0.5240 0.0580 0.5300
  • 0.0390 0.5270 t 0.0349 S O-9098, 9099 Oct,1998

' K-40 17.7200

  • 1.0700 18.4100 0.8000 18.0650 0.6680 l

BS-11122,11123 Oct,1998 Be-7

.0.4800

  • 0.2700 0.3700
  • 0.2200 0.4250 0.1741 BS-11122,11123 Oct,1998 Co-60 0.0263
  • 0.0084 0.0291 0.0090 0.0277 0.0062 l'

BS-11122,11123 Oct,1998 Cs-137 0.2714

  • 0.0179 0.2747
  • 0.0167 0.2730 2 0.0122 BS-11122,11123 Oct,1998 K-40 9.0446
  • 0.2600 8.9737
  • 0.2760 9.0092 0.1896 VE-9182,9183 Oct,1998 Be-7 2.1684
  • 0.4480 1.8643 0.4300 2.0164 0.3105 VE-9182,9183 Oct,1998 K-40 4.9628
  • 0.6160 5.4867
  • 0.6600 5.2248 2 0.4514 VE-9203,9204 Oct,1998 Be-7 1.9163 0.6090 1.9606
  • 0.3870 1.9385 0.3608 VE-9203,9204 Oct,1998 Cs-137 0.2744
  • 0.0568 0.2623
  • 0.0361 0.2684
  • 0.0337 VE-9203,9204 Oct,1998 K-40 3.9727
  • 0.6770 4.0116
  • 0.4430 3.9922
  • 0.4045 F - 8773,8774 Oct,1998 Co-60 0.0013 2 0.0008 0.0024
  • 0.0037 0.0019 0.0019 l

F - 8773,8774 Oct,1998 Cs-137 0.0040

  • 0.0035 0.0027
  • 0.0088 0.0034
  • 0.0052 F - 8794,8795 Oct,1998 Co-60

-0.0062 t 0.0213 0.0011

  • 0.0065

-0.0026 0.0111 F-8794,8795 Oct,1998 Cs-137 0.0008 i 0.0076 0.0011

  • 0.0056 0.0010
  • 0.0047 S O-9119, 9120 Oct,1998 Cs-137 0.5500 t 0.0397 0.5500 0.0480 0.5500 0.0311 S O-9119, 9120 Oct,1998 K-40 20.2600
  • 1.0200 20.5090
  • 0.8050 20.3845
  • 0.6497 S O-9161; 9162 Oct,1998 Cs-137 0.7715
  • 0.0584 0.7532 0.0525 0.7624 0.0393 l

S O-9161, 9162 Oct,1998 K-40 18.1200

  • 1.1200 20.0600
  • 1.2000 19.0900 0.8207 WW - 9277,9278 Oct,1998 H-3 97.6157
  • 83.0917 64.2534
  • 81.5898 80.9345
  • 58.2261 j:. SWU-9014, 9015 Oct,1998 Gr. Beta 2.7210
  • 0.6386 3.3308
  • 0.6187 3.0259 0.4446 SWU-9014, 9015 Oct,1998 H-3 161.5360
  • 85.8760 157.8370 85.7160 159.6865 60.6670

. MI-9035,9036 Oct,1998 K-40 1,531.4000 129.0000 1,426.0000

  • 188.0000 1,478.7000 114.0011 F - 8972,8973 Oct,1998 Co-60

-0.0127 0.0489 0.0018

  • 0.0111

-0.0055 0.0251 F - 8972,8973 Oct,1998 Cs-137 0.0070

  • 0.0120

-0.0022 i 0.0070 0.0024 2 0.0069 i

A5-7

i Table A-5.

In-house " duplicate" samples.

Concentration in pCi/L' Lab Sample First Second Averaged Codes

  • Date Analysis Result Result Result CW - 9414,9415 Oct,1998 Gr. Beta 2.6433
  • 1.5016 3.4161 1.5235 3.0297 1.0696 CW - 9414,9415 Oct,1998 Gr. Beta 0.3371 1.2445

-1.2723 1.1437

-0.4676

  • 0.8451 WW - 9256,9257 Oct,1998 Co-60

-1.2600

  • 0.9300

-1.5100 4.3900

-1.3850 2.2437 WW - 9256,9257 Oct,1998 Cs-137 0.6770

  • 3.4400 1.8800 3.6200 1.2785 2.4969 WW - 9256,9257 Oct,1998 H-3 4,953.1843 206.9523 5,147.0443 1 210.3507 5,050.1143 147.5438 l

LW-9479,9480 Oct,1998 Gr. Beta 2.0720

  • 0.5550 1.9860
  • 0.5500 2.0290 0.3907 BS-9349, 9350 Nov,1998 Cs-137 0.0239
  • 0.0156 0.0277
  • 0.0151 0.0258 0.0109 BS-9349, 9350 Nov,1998 Gr. Beta 8.4550 2.1970 6.4700 2.0840 7.4625 1.5141 BS-9349, 9350 Nov,1998 K-40 6.9294 0.4400 6.4650 0.4290 6.6972
  • 0.3073 MI-9437,9438 Nov,1998 I-131

-0.1516 i 0.2458

-0.0769 0.2776

-0.1143 0.1854 MI-9437,9438 Nov,1998 K-40 681.2300 128.0000 714.6700 122.0000 697.9500

  • 88.4138 MI-9526,9527 Nov,1998 Co-60 2.7000
  • 5.7200

-1.9500

  • 7.4300 0.3750
  • 4.6884 MI-9526,9527 Noy,1998 Cs-137

-2.2200

  • 2.8500 0.7490 2.1600

-0.7355 1.7880 MI-9526,9527 Nov,1998 I-131

-0.0873 0.2233

-0.0122

  • 0.2343

-0.0497

  • 0.1618 1

VE-9667,9668 Nov,1998 Gr. Beta 4.4810 0.1970 4.3670 0.1940 4.4240

  • 0.1382 VE-9667,9668 Nov,1998 K-40 4.2338
  • 0.2840 3.7245
  • 0.4880 3.9792
  • 0.2823 CW - 9761,9762 Nov,1998 Gr. Beta 2.3323 1 1.4667 2.6450
  • 1.4133 2.4887 1.0184 CW - 9761,9762 Nov,1998 Gr. Beta

-0.2608

  • 1.2213 0.9390 1.2890 0.3391
  • 0.8878 SWT-10167,10168 Nov,1998 Gr. Beta 2.1779
  • 0.5699 1.9517 0.5841 2.0648
  • 0.4080 CW - 10123,10124 Nov,1998 Gr. Beta 0.7677
  • 1.2537 1.4828
  • 1.3165 1.1252 0.9090

)

CW - 10123,10124 Nov,1998 Gr. Beta 0.4380

  • 1.2388

-0.3370 1.1818 0.0505

  • 0.8560 SW - 10263,10264 Nov,1998 Co-60

-0.9560

  • 1.1500 0.0517 0.1100

-0.4522

  • 0.5776 f

SW - 10263,10264 Nov,1998 Cs-137 0.3210

  • 2.0200

-0.2150

  • 3.3100 0.0530
  • 1.9388 SW - 10263,10264 Nov,1998 Gr. Beta 7.9278
  • 1.9497 6.7850 i l.9373 7.3564 1.3743 WW-9667, 9668 Nov,1998 Gr. Beta 2.2847
  • 0.6184 1.7189 0.5495 2.0018 0.4136 SW-10069,10070 Nov,1998 Gr. Alpha 1.6469
  • 0.5301 1.5758 0.5574 1.6114
  • 0.3846 SW 10069,10070 Nov,1998 Gr. Beta 3.4363 0.4683 3.5768
  • 0.4928 3.5066 0.3399 MI-10146,10147 Dec,1998 Calcium 0.7600
  • 0.0800 0.8000 0.0800 0.7800 0.0566 MI-10146,10147 Dec,1998 K-40 1,403.6000
  • 178.0000 1,372.9000
  • 149.0000 1,388.2500 116.0657 CW - 10527,10528 Dec,1998 H-3 749.0265 108.8588 822.9436
  • 111.3401 785.9851
  • 77.8570 S O-10573, 10574 Dec,1998 Cs-137 367.0300
  • 80.5000 337.1100 32.8000 352.0700
  • 43.4629 S O-10573, 10574 Dec,1998 Gr. Alpha 12.1661
  • 4.0570 9.1124 3.5682 10.6393 2.7014 S 0-10573, 10574 Dec,1998 Gr. Beta 24.7427 3.0098 26.7558
  • 3.1255 25.7493 2.1695 5 0-10573, 10574 Dec,1998 K-40 17,459.0000 1,260.0000 16,004.0000
  • 716.0000 16,731.5000 724.6130 AP-111M,11165 Dec,1998 Be-7 0.0598 0.0077 0.0610
  • 0.0061 0.0604 0.0049 MI-10686,10687 Dec,1998 K-40 1,320.3000 160.0000 1,350.3000 166.0000 1,335.3000
  • 115.2779 AS-8

~

Table A-5.

In-house " duplicate" samples.

Concentration in pCi/1

  • ILb Sample First Second Averaged 6

Codes Date Analysis Result Result Result '

WW - 10997,10998 Dec,1998 H-3 803.9290

  • 109.1145 771.1156
  • 108.0125 787.5223 76.7670 CW - 10793,10794 Dec,1998 Gr. Beta 2.6622 2 1.4937 3.4664 1.5461 3.0643 1.0749 CW - 10793,10794 Dec,1998 Gr. Beta

-0.5610

  • 1.8946

-0.1869

  • 1.9184

-0.3740

  • 1.3481 AP-9119,9120 Dec,1998 Be-7 0.1386
  • 0.0876 0.1016
  • 0.0396 0.1201 0.0481 WW - 10997,10998 Dec,1998 Co-60

-0.5400 1.2300 0.1850 0.5010

-0.1775 0.6641 WW - 10997,10998 Dec,1998 Cs-137

-0.0998 1.8800

-1.5000 2 2.7400

-0.7999 1.6615 AP - 11267,11268 Dec,1998 Co-60 0.0006

  • 0.0005 0.0002
  • 0.0002 0.0004 0.0003 AP -11267,11268 Dec,1998 Cs-137 0.0003
  • 0.0006

-0.0000 0.0004 0.0001

  • 0.0004 SWU-10920,10921 Dec,1998 Gr. Beta 2.6300 0.7110 2.2760 0.6910 2.4530 0.4957 SW-10969,10970 Dec,1998 Gr. Beta 2.5524
  • 0.7559 1.7077 0.7056 2.1301 0.5170 WW - 11018,11019 Dec,1998 H-3 72.8851
  • 81.0523 56.4860
  • 80.3116 64.6855 57.0513 AP-11225,11226 Dec,1998 Be-7 0.0643
  • 0.0133 0.0674 0.0087 0.0658 0.0080 AP - 11246,11247 Dec,1998 Co-60

-0.0001

  • 0.0001 0.0002 0.0003 0.0001

-0.0002 i 0.0004

-0.0001

  • 0.0004

-0.0001 0.0003 AP-10948,10949 Dec,1998 Be 7 0.1379

  • 0.0647 0.2164 0.0753 0.1772 0.0496 SWU-10920,10921 Dec,1998 H-3 364.3700
  • 93.2290 364.3700
  • 93.2290 364.3700 65.9229 AP-11079,11080 Dec,1998 Be-7 0.0680 0.0120 0.0680
  • 0.0120 0.0680 0.0085 WW-11101,11102 Dec,1998 Gr. Beta 2.2867 0.6521 2.2342 0.6525 2.2605
  • 0.4612 W W 11101,11102 Dec,1998 H-3 178.9370
  • 99.8660 165.4690 99.3450 172.2030 70.4320 BS-11222,11223 Dec,1998 Gr. Beta 7.4244
  • 1.8665 6.5452
  • 1.8652 6.9848
  • 1.3194 AP-11222,11223 Dec,1998 Be-7 0.1195 0.0713 0.1350
  • 0.0766 0.1272
  • 0.0523 A5-9

Table A-6.

Department of Energy's Mixed Analyte Performance Evaluation Program (MAPEP),

comparison of MAPEP and Teledyne's Midwest Laboratory results for various sample media'.

Concentration

  • Lab Sample Date Teledyne Results MAPEP Result' Control Code Type Collected Analysis istandard Deviation' Is, N=1 Limits SPSO-828 SOIL Jan,1998 Co-57 862.20 i S6.22 1,190.00 833.00 - 1,547.00 SPSO-828 SOIL Jan,1998 Co-60 886.60t S8.66 1,110.00 777.00 - 1,443.00 SPSO-828 SOIL Jan,1998 Cs-137 442.80 1 44.28 552.00 386.40 - 717.60 SPSO-828 SOIL Jan,1998 K-40 540.30 i 54.03 652.00 456.40 - 847.60 f

SPSO-828 SOIL Jan,1998 Mn-54 867.40 i S6.74 1,090.00 763.00 - 1,417.00 SPSO-828 SOIL Jan,1998 Ni-63 326.10 1 32.61 405.00 283.50 - 526.50 SPSO-828 SOIL Jan,1998 Pu-238 52.30 i 5.23 50.60 35.42 - 65.78 SPSO-828 SOIL Jart,1998 Sr-90 587.60 1 58.76 624.00 436.80 - 811.20 SPSO-828 SOIL Jan,1998 U-234/233 38.20 i 3.82 51.40 35.98 - 66.82 SPSO-828 SOIL Jan,1998 U-238 105.40 i 10.54 120.00 84.00 - 156.00 SPSO-828 SOIL Jan,1998 Zn-65 2,256.80 i 225.70 2,780.00 1,946.00 - 3,614.00 STW-814 WATER Jan,1998 Am-241 2.0510.21 2.13 1.49 - 2.77 STW-814 WATER Jan,1998 Co-57 253.00 i 25.30 277.50 194.25 - 360.75 STW-814 WATER Jan,1998 Co-60 133.00 1 13.30 132.46 92.72 - 172.20 STW-814 WATER Jan,1998 Cs-137 218.00 i 2.18 213.12 149.18 - 277.06 STW-814 WATER Jan,1998 Fe-55 397.80 i 39.80 492.10 344.47 - 639.73 STW-814 WATER Jan,1998 Mn-54 221.00 i 22.10 221.63 155.14 - 288.12 STW-814 WATER Jan,1998 Ni-63 265.50 i 26.50 358.90 251.23 - 466.57 STW-814 WATER Jan,1998 Pu-238 1.27 i 0.13 1.40 0.98 - 1.82 STW-814 WATER Jan,1998 Pu-239/240 3.16i 0.32 3.44 2.41 - 4.47 STW-814 WATER Jan,1998 Sr-90 33.40 1 3.34 32.12 22.48 - 41.76 STW-814 WATER Jan,1998 U-234/233 3.24 i 0.32 3.60 2.52 - 4.68 STW-814 WATER Jan,1998 U-238 0.09 i 0.01 0.00 0.00 - 0.10 STW-814 WATER Jan,1998 Zn-65 612.00t 61.20 588.30 411.81 - 764.79

' Results obtained by Teledyne Brown Engineering Environmental Services Midwest Laboratory as a participant in the Department of Energy's Mixed Analyte Performance Evaluation Program, 1

Idaho Operations office, Idaho Falls, Idaho.

l

  • All results are in Bq/kg or Bq/L as requested by the Department of Energy.
  • Unless otherwise indicated, the TBEESML results are given as the mean I standard deviations for three determinations.

MAPEP results are presented as the known values and expected laboratory precision d

(1 sigma,1 determination) and controllimits as defined by the MAPEP.

A6-1

Table A-7.

Environmental Measurements Laboratory Quality Assessment Program (EML),

comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.

I Concentration in Bq/L' Lob Sample Date Control Code Type Collected Analysis Teledyne Result' EML Result' Limits

  • STW-819 WATER Mar,1998 Co-60 14.80 0.60 13.60 1.20 0.92 - 1.18 STW-819 WATER Mar,1998 Cs-137 51.20
  • 1.20 46.00 1.70 0.90 - 1.28 STW-819 WATER Mar,1998 Fe-55 243.00 29.40 257.00 2.50 0.31 - 1.54 STW-819 WATER Mar,1998 Gr. Alpha 1,592.90 t 63.80 1,421.00 100.00 0.50 - 1.29 STW-819 WATER Mar,1998 Gr. Beta 2,509.00 67.10 2,200.00 100.00 0.60 - 1.64 STW-819 WATER Mar,1998 H-3 399.70
  • 32.50 218.30 i 6.51 0.65 - 1.91 The sample ws.s acidic, causing a breakdown of resin in the tritium column. The sample was neutralized to pH 7 and reanalyzed. Result of reanalysis: 178.3 15.5 Bq/L STW-819 WATER Mar,1998 Mn-54 61.70 1.30 57.00 1.90 0.87 - 1.22 STW-819 WATER Mar,1998 Pu-238 2.61
  • 0.27 2.53 0.06 0.78 - 1.42 I

STW-819 WATER Mar,1998 Pu-239 1.79 0.21 1.65

  • 0.06 0.78 - 1.42 STW-819 WATER Mar,1998 Sr-90 1.70 0.40 4.36 0.19 0.72 - 1.66 STW-819 WATER Mar,1998 U-238 0.50 0.20 0.40 0.04 0.77 - 1.35 STSO-820 SOIL Mar,1999 Am-241 1.67 1.11 2.68 0.21 0.52 - 2.65 f

STSO-820 SOIL Mar,1998 Cs-137 322.59

  • 4.57 329.50 9.26 0.80 - 1.34 STSO-820 SOIL Mar,1998 K-40 322.10 24.32 313.50
  • 10.15 0.73 - 1.67 STSO-820 SOIL Mar,1998 Pu-239 4.65
  • 1.66 5.31
  • 0.25 0.66 - 1.93 STSO-820 SOIL Mar,1998 St-90 9.89 3.83 13.09 0.28 0.46 - 2.84 STSO-820 SOIL Mar,1998 U-238 13.44 2 2.49 31.90 2.55 0.35 - 1.55 j

STVE-821 VEGETATION Mar,1998 Am-241 0.70 0.40 0.05 0.68 - 2.78 STVE-821 VEGETATION Mar,1998 Cm-244 1.78

  • 0.33 2.17 0.07 0.49 - 1.69 STVE-821 VEGETATION Mar,1998 Co-60 10.17
  • 1.54 10.58 0.21 0.62 - 1.42 STVE-821 VEGETATION Mar,1998 Cs-137 166.03
  • 3.46 181.50 2 7.14 0.81 - 1.45 STVE-821 VEGETATION Mar,1998 K-40 677.16 31.47 707.50 24.99 0.79 - 1.50 STVE-821 VEGETATION Mar,1998 Sr-90 315.31 15.06 359.01 6.02 0.48 - 1.29 STAF-822 AIR FILTER Mar,1998 Am-241 0.07 0.01 0.07
  • 0.00 0.68 - 2.01 STAF-822 AIR FILTER Mar,1998 Ce-144 7.77 0.62 8.21 0.80 0.60 - 1.50 STAF-822 AIR FILTER Mar,1998 Co-57 10.15
  • 0.11 11.11 2 0.85 0.62 - 1.22 STAF-822 AIR FILTER Mar,1998 Co.60 9.24
  • 0.16 9.09 0.73 0.74 - 1.24 STAF-822 AIR FILTER Mar,1998 Cs-134 18.98
  • 0.20 19.74 1.38 0.72 - 1.21 STAF-822 AIR FILTER Mar,1998 Cs-137 12.88 0.20 11.86 2 0.96 0.72 - 1.32 l

STAF-822 AIR FILTER Mar,1998 Mn-54 6.18 0.20 5.44 0.49 0.75 - 1.27 STAF-822 AIR FILTER Mar,1998 Pu-238 0.07

  • 0.02 0.07
  • 0.00 0.62 - 1.46 STAF-822 AIR FILTER Mar,1998 Pu-239 0.07
  • 0.02 0.06 0.00 0.62 - 1.46 STAF-822 AIR FILTER Mar,1998 Sb-125 13.54 0.56 12.16
  • 1.15 0.62 - 1.39 STAF-822 AIR FILTER Mar,1998 Sr-90 1.82
  • 0.21 1.76 i 0.04 0.66 - 2.65 A7-1

r Table A-7.

Environmental Measurements Laboratory Quality Assessment Program (EML),

comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.

6 Concentrationin Bq/L Lab Sample Date Control d

Code Type Collected Analysis Teledyne Result

  • EML Result Limits
  • STAF-822 AIR FILTER Mar,1998 U-238 0.39
  • 0.08 0.03
  • 0.00 0.78 - 3.00 The cause is unknown. A dilution problem is suspected, the result is approximately ten times the known value.

The calculations were reviewed, no error was found.

STSO-834 SOIL Sep,1998 Ac-228 54.10 3.30 52.60 2.90 0.50 - 1.50 STSO-834 SOIL Sep,1998 Di-212 55.40 10.30 58.30 5.90 0.50 - 1.50 STSO-834 SOIL Sep,1998 Bi214 28.50

  • 6.50 28.80 0.50 0.50 - 1.50 STSO-834 SOIL Sep,1998 Cs-137 915.70
  • 8.20 954.00
  • 38.00 0.80 - 1.34 STSO-834 SOIL Sep,1998 K-40 296.20 39.90 314.00 13.00 0.73 - 1.67 STSO-834 561L Sep,1998 Pb-212 53.60
  • 1.50 52.80 3.70 0.50 - 1.50 STSO-834 SOIL Sep,1998 Pb-214 31.00 5.90 29.10
  • 1.20 0.50 - 1.50 STSO-834 SOIL Sep,1998 Ra-226 115.30
  • 2.20 29.00 1.00 0.00 - 3.00 Acceptable results according to EML Data is under review.

i l

STSO-834 SOIL Sep,1998 Sr-90 37.40 1.90 39.63 1 0.00 0.46 - 2.84 STSO-834 SOIL Sep,1998 T1-208 20.10 3.10 18.30

  • 1.10 0.50 - 1.50 l

STW 835 WATER Sep,1998 Co-60 49.30

  • 2.80 49.40 1.20 0.92 - 1.18 STW-835 WATER Sep,1998 Cs-137 50.10
  • 3.20 50.00 1.70 0.90 - 1.28 STW-835 WATER Sep,1998 Fe-55 140.60
  • 9.20 139.00 2.00 0.31 - 1.54 STW-835 WATER Sep,1998 Gr. Alpha 1,178.30 47.20 1,080.00
  • 60.00 0.50 - 1.29 STW-835 WATER Sep,1998 Gr. Beta 1,613.60
  • 171.80 1,420.00 60.00 0.60 - 1.64 STW-835 WATER Sep,1998 H-3 102.20 4.50 76.20
  • 2.90 0.65 - 1.91 STW-835 WATER Sep,1998 Mn-54 35.90
  • 3.40 32.40 1.40 0.87 - 1.22 STW-835 WATER Sep,1998 Sr-90 3.00
  • 0.90 2.11
  • 0.18 0.72 - 1.66 STAF-837 AIR FILTER Sep,1998 Co-60 9.30
  • 0.30 9.16
  • 0.58 0.74 - 1.24 STAF-837 AIR FILTER Sep,1998 Cs-137 22.40 0.50 22.47
  • 1.03 0.72 - 1.32 STAF-837 AIR FILTER Sep,1998 Mn-54 5.30
  • 0.30 4.92 0.40 0 75 - 1.27 STAF-837 AIR FILTER Sep,1998 Sb-125 10.00
  • 0.80 8.89
  • 0.55 0.60 - 1.39

{

STAF-838 AIR FILTER Sep;1998 Gr. Alpha 2.20

  • 0.10 1.65
  • 0.16 0.83 - 1.55 l

STAF-838 AIR FILTER Sep,1998 Gr. Beta 2.80

  • 0.10 2.16 i 0.07 0.73 - 1.84 STAF-838 AIR FILTER Sep,1998 Sr-90 1.10
  • 0.10 1.12
  • 0.05 0.66 - 2.65 STVE-839 VEGETATION Sep,1998 Co-60 18.10 1.50 20.00
  • 1.00 0.62 - 1.42 l

STVE-839 VEGETATION Sep,1998 Cs-137 340.40 i 4.80 390.00

  • 20.00 0.81 - 1.45 STVE-839 VEGETATION Sep,1998 K-40 417.50 t 28.20 460.00 20.00 0.79 - 1.50 STVE-839 VEGETATION Sep,1998 Sr-90 672.50 32.50 606.00 40.00 0.48 - 1.29 l

1 A7-'2

Table A-7.

Environmental Measurements Laboratory Quality Assessment Program (EML),

comparison of EML and Teledyne's Midwest Laboratory results for various sample media'.

Concentration in Bq/L' Lab Sample Date Control Code Type Collected Analysis Teledvne Result' EML Result

  • Limits'

' The Environmental Measurements Laboratory provides the following nuclear species : Air Filters, Soil, Tissue, Vegetation and Water. Teledyne does not participate in the Tissue program.

  • Results are reported in Bq/L-' with the following exceptions: Air Filter results are reported in Bq/ Filter', Soil results are reported in Bq/Kg-8, Vegetation results are reported in Bq/Kg'. The results of elemental Uranium are reported in ug/filtei', g, or ml.
  • Teledyne results are reported as the mean of three determinationsistandard deviation.

The EML result listed is the mean of replicate determinations for each nuclide*the standard error of the mean.

d

  • The controllimits are reported by EML and are established from percentiles of historic data distributions (1982-1992). The evaluation of this historic data and the development of the controllimits is presented in DOE

]

report EML-564.

l i

l A7-3

l I

i h

8 APPENDIX B DATA REPORTING CONVENTIONS l

l i

i

)

B-1

[z u

i Data Reporting Conventions 1.0. All activities except gross alpha and gross beta are decay corrected to collection time or the end of the collection period.

2.0. hgle Measurements Each single measurement is reported as follows:

xis where x = value of the measurement; s = 2a counting uncertainty (corresponding to the 95% confidence level).

In cases where the activity is found to be below the lower limit of detection L it is reported as

<L where L = the lower limit of detection based on 4.66o uncertainty for a background sample.

3.0. Duplicate analyses 3.1 Individual results:

x1 i s1 x2 i s2 Reported result:

xis where x = (1/2)(x1 + x2) s = (1/2) k sf + s$

3.2. Individual results:

<L3

<L2 Reported result: <L where L = lower of L and L2 1

3.3. Individual results: xi s l

<L Reported result:

xi s if x 2 L;

<L otherwise B-2 i-

~

4.0. Computation of Averages and Standard Deviations 4.1 Averages and standard deviations listed in the tables are computed from all of the individual measurements over the period averaged; for example, an annual standard deviation would not be the average of quarterly standard deviations. The average i and standard deviation s of a set of n numbers xi,x2 x are defined as follows:

n x=fEx I(x-x)2 n-1 4.2 Values below the highest lower limit of detection are not included in the average.

4.3 If all of the values in the averaging group are less than the highest LLD, the highest LLD is reported.

4.4 If all but one of the values are less than the highest LLD, the single value x and associated two sigma erroris reported.

4.5 In rounding off, the following rules are followed:

4.5.1. If the figure following those to be retained is less than 5, the figure is dropped, and the retained figures are kept unchanged. As an example,11.443 is rounded off to 11.44, 4.5.2. If the figure following those to be retained is equal to or greater than 5, the figure is dropped and the last retained figure is raised by 1. As an example,11.445 is rounded off to 11.05.

i B. 3 l

l-

APPENDIX C Maximum Permissible Concentrations of Radioactivityin Air and Water Above Background in Unrestricted Areas I

l t

C-1 l

Table C-1.

Maximum permissible concentrations of radioactivity in air and water above naturalbackground in unrestricted areas,

a I

Air Water Iodine-131b 0.29 pCi/m3 Strontium-89 8,000 pCi/L Strontium-90 500 pCi/L Cesium-137 1,000 pCi/L Barium-140 8,000 pCi/L Iodine-131 1000 pCi/L Potassium-40c 4,000 pCi/L 6

Tritium 1 x 10 pCi/L a Taken from Code of Federal Regulations Title 10, Part 20, Table 2 and appropriate footnotes. Concentrations may be averaged over a period not greater than one year.

b From 10 CFR 20 but adjusted by a factor of 700 to reduce the dose resulting from the air-grass-cow-milk-child pathway, c A natural radionuclide.

l l

C-2 l

l

APPENDIX D

SUMMARY

OF THE LAND USE CENSUS 4

D-1

l Appendix D Summary of the Land Use Census l

l The Duane Arnold Energy Land Use Census for 1998 was completed during the fourth j

week of September 1998. All milk animals and gardens greater than 500 square feet were q

identified within three miles for each of the 16 meteorological sectors. If none were l

identified within the three mile range, additional surveys were performed out to a distance l

of five miles. The Cedar River was surveyed by boat on July 24th 1998 for water use l

downstream of the DAEC to Cedar Rapids.

There were 154 gardens found during the performance of the 1998 Census. This number exceeds the number of gardens found in the 1997 survey by 7. This difference can be attributed to the removal of 21 gardens and the addition of 28 new gardens.

Milk animallocations remained unchanged since the 1995 census. Two of the locations have goats that do not provide samples during the winter months.

]

The locations of the nearest resident for each sector remained the same. Twenty-one new homes were built or were under construction within three miles of the DAEC, compared to the 22 new homes identified in 1997. Most of the new houses built were located in the sectors between the plant and Cedar Rapids (ESE and SE).

l The Cedar River survey revealed no new withdrawals of river water compared to previous surveys. Irrigation of the strawberry farm in Palo and fishing remain the only food pathway uses of river water between the DAEC and Cedar Rapids.

l As a result of this census, no adjustments were made to the MIDAS dose projection

~

software model.

D-2 i

1 l

APPENDIX E ANNUAL RADIATION DOSE ASSESSMENT t

j E-1

1 l

i

)

Appendix E 4

Annual Radiation Dose Assessment The annual offsite radiation dose to a member of the public was determined by assessment

)

of environmental dosimeter results and by calculations based on monitored effluent j

releases.

Section A.

Dose Contribution from Direct Radiation Direct radiation dose from the operation of the DAEC was reported by TLDs placed at locations in the surrounding environment as described in the Offsite Dose Assessment Manual (ODAM).

1. Pre-operational and 1998 TLD results were compared using a paired difference test.

No significant differences in the TLD populations were observed for the 0.5 mile and one mile TLD populations using a confidence level of 99%.

j 4

2. As stated in Part 1, page 8 of this report, no plant effect was indicated by the TLDs when dose results were compared to the estimated average natural background for Middle America.

Section B.

Estimated Offsite Dose from Efnuent Releases The contribution of dose to a member of the public most likely to be exposed from effluent releases was calculated by the Meteorological Information and Dose Assessment System (MIDAS) computer program in accordance with ODAM. The calculation methods follow those prescribed by Reg. Guide 1.109. Because there were no nuclides detected in the environment at or beyond the site boundary that were due to the operation of the DAEC, no comparison of calculated dose from stack releases and dose calculated from environmental contamination was performed.

Results of the MIDAS dose calculations are discussed below and are shown in tabular form on page E-4

1. There were no releases of radioactive material to liquid effluents in 1998.
2. The dose to air from noble gases released was 1.48E-03 mrad from gamma radiation at 535 meters SSW and 2.27E-02 mrad beta radiation at 535 meters SSW.
3. The total body dose equivalent to the maximally exposed individual from noble gases was 1.81E-03 mrem, at 805 meters West.

E-2

4. The skin dose equivalent to the maximally exposed individual from noble gases was 1.84E-03 mrem, at 805 meters West.
5. The maximally exposed organ due to iodines and particulates with half-lives greater than eight days was the thyroid of a child at 805 meters West, with and estimated dose equivalent of 8.01E-03 mrem.

==

Conclusion:==

No measurable dose due to the operation of the DAEC was detected by environmental TLDs in 1998. The calculated doses are below the regulatory limits stated in Appendix 1 to 10 CFR 50 and in 40 CFR 190.

Estimated Maximum Offsite Individual Doses for 1998 Type Age Distan:e Direction Dose or Dose Annual 10 CFR l Group (meters)

Equivalent 50, Appendix I p (mrem)

Limit Direct Radiation None (as measured by TLDs)

Liquid Releases None Noble Gas Gamma Air Dose 535 SSW l.48E-03 mrad 10 rr. rad Beta Air Dose 535 SSW 2.27E-02 mrad 20 mrad Total Body All 805 W

l.81E-03 mrad Skin All 805 W

l.84E-03 mrad Particulates & lodines Organ Dose Child -

805 W

8.01E-03 15 mrem Thyroid mrem No Appendix I limit but is used to determine compliance with 40 CFR 190 limits of 25 mrem total body and 75 mrem thyroid.

E-3

Y TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY sus 5i?"

REPORT TO IES UTILITIES,INC.

CEDAR RAPIDS, IOWA RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP)

FORTHE DUANE ARNOLD ENERGY CENTER CEDAR RAPIDS, IOWA Docket No. 50-331 ANNUAL REPORT - PART II y

DATA TABULATIONS AND ANALYSES JANUARY - DECEMBER 1998 PREPARED AND SUBMITTED BY i

TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES MIDWEST LABORATORY PROJECT NO. 8001 f

I Reviewed and 4

i Approved by

,b O

Bronia rob M.

/

Techi al L a April 23,1999 i

m I

TABLE OF CONTENTS Section g

' List of Tables............................................................................................,,,,,,,iii

1.0 INTRODUCTION

.............................................................................................y 2.0 LISTING OF MISSED SAMPLES.....................................................................vi 3.0 D ATA TA B LES............................................................................................v i

t i

t i

i I

11

LIST OF TABLES bh Title Eage 1

Airborne particulates collected at Location D-1, (Cedar Rapids),

an alysis for gross be t a................................................................... 1 - 1 2

Airborne particulates and iodine collected at Location D-2 (Marion),

analysis for gross beta and iodine-131............................................ 2-1 3

Airborne particulates collected at Location D-3 (Hiawatha), analysis f o r g r o s s b e t a............................................................,.................... 3 - 1 4

Airborne particulates and iodine collected at Location D-5 (Palo),

analysis for gross beta and iodine-131..................................... 4-1 5

Airborne particulates collected at Location D-6 (Center Point),

analysis for gross be ta....................................................................... 5 - 1 6

Airborne particulates and iodine collected at Location D-7, (Shellsburg), analysis for gross beta and iodine-131.......................... 6-1 7

Airborne particulates and iodine collected at Location D-8 (Urbana),

analysis for gross beta and iodine-131............................................. 7-1 8

Airborne particulates collected at Location D-10 (Atkins), analysis f o r gr os s b e ta....................................................................................... 8 - 1 9

Airborne particulates and iodine collected at Location D-11 (Toddville), analysis for gross beta and iodine-131............................ 9-1 10 Airborne particulates collected at Location D-13 (Alburnett),

i ana: ysis for gross beta................................................................... 10-1 11 Airborne particulates and iodine collected at Location D-15 (on-site, north), analysis for gross beta and lodine-131...............................11-1 12 Airborne particulates collected at Location D-16 (on-site, south),

analysis for gross be ta....................................................................... 12-1 13 Airborne particulate samples, quarterly composites of weekly samples, analysis for gamma-emitting isotopes..........................13-1 1

14 Ambient gamma radiation (TLD), quarterly exposure................................14-1 15 Milk samples, analysis for iodine-131 and gamma emitting isotopes...........15-1 16 Ground water samples, analysis for gross beta and tritium................

.16-1 17 Vegetation samples (broadleaf), analysis for iodine-131 and gamma-emitting iso topes........................................................................... 17-1 iii l

L

r LIST OF TABLES (continued) hkh Iltle.

Eage 18 Vegetation samples (hay and grain), analysis for gamma-emitting isotopes............................................................................................18-1 19 Surface water samples, analysis for iodine-131 and gamma-emitting isotopes...............................................................................................19-1 20 Surface water samples, analysis for potassium-40, iodine-131 and gamma-emitting isotopes.................................................................... 2 0- 1 i

21 Surface water samples, quarterly composites of monthly samples, a nalysis for tri ti u m............................................................................ 21 - 1 22 Fish samples, analysis for gamma-emitting isotopes.................................... 22-1 23 River sediment samples, analysis for gamma-emitting isotopes................... 23-1 24 Precipitation sam,ples, analysis for gamma-emitting isotopes...................... 24-1 25 Precipitation samples, quarterly composites of monthly samples, an alysis for tri ti um......................................................,...................... 2 5 - 1 26 Meat samples, analysis for gamma-emitting isotopes.................................. 26-1 27 Soil samples, analysis for strontium-90 and gamma-emitting l

isotopes..............................................................................................27-1 l

l 1

1 i

l 1

1 iv

o

1.0 INTRODUCTION

The following constitutes a supplement to the Annual Report for the Radiological Environmental Monitoring Program conducted at the Duane Arnold Energy Center, Palo, Iowa in 1998. Results of completed analyses are presented in the attached tables.

For information regarding sampling locations, type and frequency of collection, and sample codes, please refer to Part 1, Tables 5.3 - 5.5 and Figures 5.1 and 5.2.

I 1

l-V

F i

[

2.0 IMTING OF MISSED SAMPIM l

__y l

Sample Collection Date l

Type Analysis location (s) or Period Cornments MI I-131, Gamma D-93 01-06-98 Sample not received; goat dry.

l MI I-131, Gamma D-101 01-06-98 Sample not received; goat dry.

j '

MI I-131, Gamma D-101 02-03-98 Sample not received; goat dry.

MI I-131, Gamma D-101 03-05-98 Sample not received; goat dry.

TLD Ambient Gamma D-48 1st Qtr.

TLD lost in the field.

MI I-131, Gamma D-101 04-07-98 Sample not received; goat dry.

TLD Ambient Gamma D-48 2nd Qtr.

TLD lost in the field.

SW Gamma D-49 06-15-98 Sample lost in shipment.

MI I-131, Gamma D-105 06-18-98 Sample lost in shipment.

AP/AI Gross Beta, I-131 D-2,5,7,8,11,15 12-03-98 Samples misplaced by the AP Gross Beta D-1,3,6,10,13,16 12-03-98 laboratory.

MI I-131, Gamma D-93 12-01-98 Sample not received; goat dry.

MI I-131, Gamma D-101 12-01-98 Sample not received; goat dry.

TLD Ambient Gamma D-18 4th Qtr.

TLD lost in the field.

TLD Ambient Gamma D-43 4th Qtr.

TLD lost in the field.

vi

3.0 DATA TABLES i

l I

l Vil l

F DUANE ARNOLD Table 1. Airborne particulates, analysis for gross beta.

Location: D-1 (Cedar Rapids) 8 Units: pCi/m Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m')

Gross Beta Collected (m )

Gross Beta 8

Reauired LLD DA10 0410 01-08-98 245 0.020 2 0.003 07-09-98 285 0.018 0.0%

01-15-98 287 0.039 1 0.004 07-16-98 287 0.018 1 0.003 01-22-98 284 0.051

  • 0.004 07-23-98 284 0 616
  • 0.003 01-29-98 286 0.052 0.005 07-30-98 267 0.016 0.003 02-05-98 285 0.031 0.003 08-06-98 286 0.011 2 0.003 02-12-98 288 0.025 0.003 08-13-98 284 0.023 0.003 02-19-98 285 0.029 0.003 08-20-98 285 0.029 2 0.003 02-25-98 242 0.019 0.003 08-27-98 285 0.039 t 0.004 03-05-98 327 0.014 i 0.003 09-04-98 324 0.031 0.004 03-12-98 286 0.020 1 0.003 09-09-98 206 0.040 2 0.005 03-19-98 285 0.020 0.003 09-17-98 323 0.028 0.004 03-26-98 286 0.021 1 0.003 09-24-98 290 0.022 t 0.003 04-02-98 284 0.010 t 0.003 09-30-98 244 0.037 0.004 1st Quarter Mean
  • s.d.

0.027 0.013 3rd Quarter Mean s.d.

0.025

  • 0.010 04-09-98 284 0.011 0.003 10-07-98 285 0.016 0.003 04-16-98 285 0.019 0.003 10-14-98 287 0.014
  • 0.003 04-23-98 286 0.016 0.003 10-22-98 325 0.029 i 0.004 04-30-98 288 0.019 1 0.003 10-29-98 287 0.037 0.004 05-07-98 283 0.018 0.003 11-05-98 282 0.016 2 0.003 05-14-98 289 0.013 0.003 11-12-98 287 0.028 0.004 05-21-98 284 0.004 2 0.002' 11-19-98 286 0.039 0.004 05-28-98 284 0.004
  • 0.002' 11-25-98 248 0.016 0.004 12-03-98*

06-04-98 286 0.014 0.003 06-10-98 244 0.008 0.003 12-10-98 285 0.025 0.004 06-18-98 327 0.014 0.003 12-17-98 287 0.018 1 0.003 06-25-98 286 0.015 0.003 12-23-98 246 0.017 z 0.004 07-02-98 285 0.015 0.003 12-30-98 281 0.034

  • 0.004 2nd Quarter Mean s.d.

0.013 0.005 4th Quarter Mean

  • s.d.

0.024 0.009 Cumulative Average 0.022 Previous Annual Average 0.025

  • Filter light.
  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

1-1

DUANE ARNOLD Table 2. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131'.

Location: D-2(Marion)

Units: pCi/m' Collection: Continuous, weekly exchange.

Date Volume D te Volume Collected (m')

Gross Beta Collected (m')

Gross Beta Reauired LLD Qa1Q DAID 01-08-98 246 0.018 2 0.003 07-09-98 285 0.022 1 0.003 01-15-98 288 0.035

  • 0.004 07-16-98 287 0.026 0.003 01-22-98 283 0.050 1 0.004 07-23-98 283 0.024 0.003 01-29-98 286 0.055 0.005 07-30-98 286 0.026 0.003 02-05-98 285 0.036 0.004 08-06-98 286 0.016 1 0.003 02-12-98 288 0.033 0.004 08-13-98 284 0.029 1 0.003 02-19-98 285 0.027 0.003 08-20-98 285 0.034 0.004 02-25-98 243 0.018 0.003 08-27-98 285 0.041
  • 0.004 03-05-98 326 0.012
  • 0.003 09-04-98 325 0.031 2 0.004 03-12-98 286 0.021 0.003 09-09-98 206 0.046 0.006 03-19-98 285 0.022 0.003 09-17-98 323 0.028 0.004 03-26-98 286 0.019 1 0.003 09-24-98 290 0.022 0.003 04-02-98 284 0.014 0.003 09-30-98 244 0.039 0.004 1st Quarter Mean s.d.

0.028 0.013 3rd Quarter Mean s.d.

0.030

  • 0.009 I

04-09-98 284 0.013

  • 0.003 10-07-98 285 0 013
  • 0.003 04-16-98 285 0.018 1 0.003 10-14-98 284 0.016 0.003 04-23-98 286 0.016
  • 0.003 10-22-98 328 0.026 1 0.003 04-30-98 288 0.017
  • 0.003 10-29-98 287 0.040 0.004 05-07-98 282 0.016
  • 0.003 11-05-98 283 0.018 0.004 05-14-98 289 0.023
  • 0.003 11-12-98 287 0.020 0.003 05-21-98 284 0.026 0.003 11-19-98 286 0.033 1 0.004 05-28-98 283 0.019 0.003 11-25-98 248 0.017 0.004 12-03-98*

06-04-98 287 0.015

  • 0.003 06-10-98 243 0.012 0.003 12-10-98 285 0.026 0.004 06-18-98 328 0.019 2 0.003 12-17-98 286 0.022 1 0.004 06-25-98 286 0.018 1 0.003 12-23-98 246 0.021 0.004 07-02-98 284 0.021 0.003 12-30-98 282 0.038 0.004 2nd Quarter Mean s.d.

0.018 0.004 4th Quarter Mean s.d.

0.024

  • 0.009 Cumulative Average 0.025 Previous Annual Average 0.025 8
  • Iodine-131 concentrations are <0.07 pCi/m unless noted otherwise.
  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

2-1 I

DUANE ARNOLD Table 3. Airborne particulates, analysis for gross beta.

Location: D-3(Hiawatha)

Units: pCi/m*

Collection: Continuous, weekly exchange.

Date

. Volume Date Volume Collected (m')

Gross Beta Collected (m )

Gross Beta 8

Required LLD Qa1Q Qa1Q 01-08-98 239 0.015 t 0.003 07-09-98 285 0.024 0.003 01-15-98 287 0.028 2 0.004 07-16-98 285 0.024 0.003 01-22-98 283 0.044 2 0.004 -

07-23-98 285 0.024 0.003 01-29-98 286 0.044 0.004 07-30-98 285 0.022 0.003 02-05-98 285 0.028 2 0.003 08-06-98 288 0.018 0.003 02-12-98 288 0.028 0.003 08-13-98 284 0.025

  • 0.003 02-19-98 285 0.031 0.003 08-20-98 285 0.032
  • 0.003 02-25-98 243 0.018 t 0.003 08-27-98 285 0.041 0.004 03-05-98 326 0.012 2 0.003 09-04-98 324 0.028 0.004 03-12-98 286 0.019 0.003 09-09-98 206 0.046 0.006 03-19-98 285 0.022 0.003 09-17-98 323 0.025 0.003 03-26-98 287 0.020 0.003 09-24-98 290 0.024 0.003 04-02-98 284 0.008 0.002 09-30-98 245 0.033 0.004 1st Quarter Mean
  • s.d.

0.024

  • 0.011 3rd Quarter Mean
  • s.d.

0.028 0.008 04-09-98 284 0.011 0.003 10-07-98 285 0.012 2 0.003 04-16-98 285 0.015 i 0.003 10-14-98 286 0.017 0.003 04-23-98 286 0.016

  • 0.003 10-22-98 326 0.024 0.003 04-30-98 287 0.016 0.003 10-29-98 287 0.033 0.004 07-98 283 0.022
  • 0.004 11-05-98 282 0.012 0.003 05-14-98 283 0.021 2 0.003 11 12 98 288 0.019 0.003 05-21-98 282 0.030 2 0.003 11-19-98 286 0.033 0.004 05-28-98 286 0.018 0.003 11-25-98 245 0.015 0.004 12-03-98' 06-04-98 286 0.020 0.003 06-10-98 244 0.010 0.003 12-10-98 285 0.022 0.004 06-18-98 327 0.020
  • 0.003 12-17-98 287 0.016 0.003 06-25-98 287 0.016
  • 0.003 12-23-98 245 0.020 1 0.004 07-02-98 284 0.019 0.003 12-30-98 283 0.031 i 0.004 2nd Quarter Mean
  • s.d.

0.018

  • 0.005 4th Quarter Mean s.d.

0.021 0.008

)

Cumulative Average 0.023 Previous Annual Average 0.023

  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

3-1

DUANE ARNOLD Table 4. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131*.

Location: D-5(Palo)

Units: pCi/m' Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m')

Gross Beta Collected (m')

Gross Beta Reauired LLD QQ1D Q210 01-08-98 245 0.015

  • 0.003 07-09-98 284 0.020 0.003 01-15-98 286 0.031 1 0.004 07-16-98 285 0.019 0.003 01-22-98 286 0.044 1 0.004 07-23-98 285 0.022
  • 0.003 01-29-98 286 0.047 0.004 07-30-98 286 0.023 0.003 02-05-98 285 0.029 0.003 08-06-98 285 0.021 0.003 02-12-98 287 0.031
  • 0.004 08-13-98 285 0.028 0.003 02-19-98 284 0.027
  • 0.003 08-20-98 285 0.031 0.003 02-25-98 244 0.019 i 0.003 08-27-98 285 0.040
  • 0.004 03-05-98 327 0.012 0.003 09-04-98 324 0.031 0.004 03-12-98 285 0.021 0.003 09-09-98 205 0.048 0.006 03-19-98 285 0.023 2 0.003 09-17-98 325 0.028 1 0.004 l

03-26-98 285 0.020 1 0.003 09-24-98 287 0.026 0.004 l

04-02-98 285 0.027

  • 0.003 09-30-98 246 0.038 0.004 1st Quarter Mean s.d.

0.027 0.010 3rd Quarter Mean i s.d.

0.029 0.009 04-09-98 284 0.012 0.003 10-07-98 283 0.017 2 0.003 04-16-98 285 0.019 0.003 10-14-98 285 0.017 0.003 04-23-98 286 0.016

  • 0.003 10-22-98 328 0.026 0.003 04-30-98 286 0.019 0.003 10-29-98 286 0.037
  • 0.004 05-07-98 283 0.020 t 0.003 11-05-98 284 0.013 0.003 05-14-98 283 0.018 0.003 11-12-98 284 0.021 0.003 05-21-98 285 0.023 1 0.003 11-19-98 286 0.038 0.004 05-28-98 284 0.017
  • 0.003 11-25-98 245 0.020 0.004 12-03-98

06-04-98 274 0.017 0.003 06-10-98 244 0.010 t 0.003 12-10-98 286 0.028 2 0.004 06-18-98 327 0.017 1 0.003 12-17-98 286 0.024 2 0.004 06-25-98 286 0.015

  • 0.003 12-23-98 243 0.020 0.004 07-02-98 286 0.018
  • 0.003 12-30-98 284 0.038 0.004 2nd Quarter Mean s.d.

0.017 0.003 4th Quarter Mean

  • s.d.

0.025

  • 0.009 Cumulative Average 0.024 Previous Annual Average 0.023
  • Iodine-131 concentrations are <0.07 pCi/m' unless noted otherwise.
  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

4-1

DUANE ARNOLD Table 5. Airborne particulates, analysis for gross beta.

Location: D-6 (Center Point)

Units: pCi/m' Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m*)

Gross Beta Collected (m')

Gross Beta Reauired LLD Da10 Da1Q 01-08-98 245 0.019 0.003 07-09-98 284 0.024 2 0.003 01-15-98 286 0.035 0.004 07-16-98 285 0.027

  • 0.003 01-22-98 285 0.054
  • 0.004 07-23-98 285 0.021 1 0.003 01-29-98 286 0.052 0.005 07-30-98 287 0.023 1 0.003 02-05-98 285 0.039 0.004 08-06-98 286 0.020 0.004 02-12-98 287 0.031 0.004 08-13-98 284 0.025 0.003 02-19-98 284 0.026 0.003 08-20-98 286 0.034 0.004 02-25-98 245 0.017 0.003 08-27-98 285 0.042 0.004 03-05-98 327 0.012 0.003 09-04-98 324 0.028 0.004 03-12-98 285 0.018 2 0.003 09-09-98 206 0.039 0.005 03-19-98 285 0.023 0.003 09-17-98 324 0.028 t 0.004 03-26-98 285 0.020 0.003 09-24-98 289 0.025 t 0.003 04-02-98 285 0.012 2 0.003 09-30-98 246 0.036 1 0.004

)

i 1st Quarter Mean i s.d.

0.028 0.014 3rd Quarter Mean s.d.

0.029 0.007 04-09-98 284 0.010 0.003 10-07-98 284 0.015 0.003 04-16-98 284 0.017 2 0.003 10-14-98 285 0.016 0.003

)

04-23-98 286 0.016 0.003 10-22-98 328 0.023 0.003 04-30-98 286 0.016 0.003 10-29-98 286 0.040 0.004 05-07-98 283 0.015 0.003 11-05-98 283 0.018 0.004 05-14-98 288 0.022 1 0.003 11-12-98 286 0.023 0.003 05-21-98 284 0.030 0.003 11-19-98 287 0.036 0.004 05-28-98 285 0.022 0.003 11-25-98 245 0.019 1 0.004 12-03-98' 06-04-98 286 0.021

  • 0.003 06-10-98 244 0.012 i 0.003 12-10-98 286 0.025
  • 0.004 06-18-98 328 0.023 0.003 12-17 98 286 0.021 0.004 06-25-98 284 0.016 0.003 12-23-98 244 0.018 i 0.004 07-02-98 286 0.021
  • 0.003 12-30-98 284 0.033 0.004 2nd Quarter Mean s.d.

0.019 0.005 4th Quarter Mean i s.d.

0.024 0.008 i

Cumulative Average 0.025 Previous Annual Average 0.025

  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

5-1

g DUANE ARNOLD Table 6. Airbome particulates and charcoal canisters, analyses for gross beta and iodine-131'.

Location: D-7(Shellsburg)

Units: pCi/m*

Collection: Continuous, weekly exchange.

Date Volume Date Volume 8

Collected (m )

Gross Beta Collected (m')

Gross Beta Required LLD 041Q 0410 01-08-98 245 0.019 i 0.003 07-09-98 283 0.022 0.003 01-15-98 286 0.034

  • 0.004 07-16-98 286 0.028 i 0.003 01-22-98 286 0.054 0.004 07-23-98 285 0.024 0.003 01-29-98 286 0.058 0.005 07-30-98 286 0.026
  • 0.003 02-05-98 285 0.028 0.003 08-06-98 285 0.020
  • 0.004 02-12-98 287 0.029 0.003 08-13-98 285 0.026 0.003 02-19-98 284 0.028 0.003 08-20-98 285 0.038 t 0.004 02-25-98 244 0.020 0.004 08-27-98 285 0.041
  • 0.004

)

03-05-98 327 0.012

  • 0.003 09-04-98 324 0.030
  • 0.004 03-12-98 285 0.017 0.003 09-09-98 205 0.050 0.006 03-19-98 285 0.028 0.004 09-17-98 324 0.027 0.004 03-26-98 285 0.021 0.003 09-24-98 287 0.022 2 0.003 04-02-98 285 0.016 2 0.003 09-30-98 246 0.032 t 0.004 i

1st Quarter Mean

  • s.d.

0.028 0.014 3rd Quarter Mean

  • s.d.

0.030 0.009 04-09-98 284 0.012 0.003 10-07-98 283 0.015

  • 0.003 04-16-98 285 0.019 0.003 10-14-98 285 0.006
  • 0.002' 04-23-98 286 0.012 0.003 10-22-98 328 0.023 1 0.003 04-30-98 286 0.022 0.003 10-29-98 286 0.032
  • 0.004 05-07-98 283 0.019
  • 0.003 11-05-98 283 0.009
  • 0.003 05-14-98 288 0.015 0.003 11-12-98 286 0.022
  • 0.003 05-21-98 285 0.023 0.003 11-19-98 287 0.033 0.004 05-28-98 284 0.017 0.003 11-25-98 245 0.016
  • 0.004 12-03-98' 06-04-98 279 0.020 0.003 06-10-98 246 0.011 0.003 12-10-98 286 0.027 0.004 06-18-98 325 0.019
  • 0.003 12-17-98 286 0.026 0.004 06-25-98 286 0.018 0.003 12-23-98 244 0.022
  • 0.004 i

07-02-98 286 0.019

  • 0.003 12-30-98 283 0.037 2 0.004 2nd Quarter Mean
  • s.d.

0.017

  • 0.004 4th Quarter Mean s.d.

0.022 0.010 l

Cumulative Average 0.024 Previous Annual Average 0.023 8

  • Iodine-131 concentrations are <0.07 pCi/m unless noted otherwise.
  • Filter caked with dirt. Extremely heavy precipitate.

+

  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

6-1

DUANE ARNOLD Table 7. Airbome particulates and charcoal canisters, analyses for gross beta and iodine-131*.

Location: D-8(Urbana)

Units: pCi/m' Collection: Continuous, weeldy exchange.

Date Volume Date Volume Collected (m')

Gross Beta Collected (m')

Gross Beta Reauired LLD QS10 041.Q 01-08-98 245 0.018

  • 0.003 07-09-98 284 0.021 0.003 01-15-98 286 0.033 t 0.004 07-16-98 285 0.026
  • 0.003 01-22-98 285 0.039 i 0.004 07-23-98 285 0.021 0.003 01-29-98 286 0.043
  • 0.004 07-30-98 286 0.021 2 0.003 02-05-98 285 0.033 0.003 08-06-98 286 0.020 0.004 02-12-98 287 0.030 0.003 08-13-98 284 0.026 0.003 02-19-98 281 0.029 0.003 08-20-98 286 0.033 0.004 02-25-98 244 0.018 1 0.003 08-27-98 285 0.036 0.004 03-05-98 327 0.013 0.003 09-04-98 324 0.025 2 0.003 03-12-98

^85 0.021

  • 0.003 09-09-98 205 0.041 0.006 03-19-98 285 0.026 0.004 09-17-98 324 0.026
  • 0.004 03-26-98 285 0.024 0.003 09-24-98 289 0.025 0.004 04-02-98 285 0.014 0.003 09-30-98 246 0.034 0.004 1st Quarter Mean s.d.

0.026

  • 0.009 3rd Quarter Mean
  • s.d.

0.027 0.007 04-09-98 284 0.012

  • 0.003 10-07-98 284 0.014 0.003 04-16-98 285 0.020 0.003 10-14-98 285 0.016 0.003 04-23-98 286 0.020 t 0.003 10-22-98 328 0.024 1 0.003 04-30-98 286 0.022 0.003 10-29-98 286 0.027 2 0.004 05-07-98 284 0.024 0.004 11-05-98 283 0.017 0.003 05-14-98 288 0.019 2 0.003 11 12-98 284 0.021 0.003 05-21-98 285 0.028 0.003 11-19-98 286 0.037 0.004 05-28-98 285 0.019 i 0.003 11-25-98 245 0.017 0.004 12-03-98

06-04-98 286 0.019 0.003 06-10-98 244 0.009 i 0.003 12-10-98 286 0.024 2 0.004 06-18-98 327 0.020 0.003 12-17-98 286 0.019 1 0.003 06-25-98 297 0.016 0.003 12-23-98 244 0.016 0.004 07-02-98 271 0.020 0.003 12-30-98 284 0.039 t 0.004 2nd Quarter Mean s.d.

0.019 0.005 4th Quarter Mean s.d.

0.023

  • 0.008 Cumulative Average 0.024 Previous Annual Average 0.024

' Jodine-131 concentrations are <0.07 pCi/m' unless noted otherwise.

  • No Data; Refer to Table 2.0, Listing of Missed Samples".

7-1

r-DUANE ARNOLD l

Table 8. Airbome particulates, analysis for gross beta.

Location: D-10(Atkirts) 8 Units: pCi/m Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m')

Gross Beta Collected (m')

Gross Beta Reauired LLD Da1Q QalD 01-08-98 245 0.018 0.003 07-09-98 285 0.021 2 0.003 01-15-98 288 0.033 0.004 07-16-98 287 0.023 0.003 01-22-98

~7 0.051 0.004 07-23-98 284 0.022 0.003 01-29-98 256 0.052 0.005 07-30-98 287 0.025 0.003 02-05-98 285 0.032 0.003 08-06-98 286 0.016 0.003 02-12-98 288 0.030 0.003 08-13-98 284 0.028 t 0.003 02-19-98 285 0.031 0.003 08-20-98 285 0.036 2 0.004 02-25-98 242 0.021

  • 0.004 08-27-98 285 0.042 0.004 l

03-05-98 327 0.014 i 0.003 09-04-98 326 0.029 0.004 03-12-98 285 0.023 2 0.003 09-09-98 205 0.040 t 0.006 l

03-19-98 285 0.027

  • 0.004 09-17-98 322 0.026
  • 0.004 l

03-26-98 287 0.026

  • 0.003 09-24-98 291 0.028 i 0.004 l

04-02-98 282 0.017 1 0.003 09-30-98 244 0.037 0.004 l

1st Quarter Mean

  • s.d.

0.029 0.012 3rd Quarter Mean i s.d.

0.029

  • 0.008 04-09-98 284 0.012 1 0.003 10-07-98 285 0.014 0.003 l

04-16-98 282 0.020 0.003 10-14-98 286 0.015 t 0.003 l

04-23-98 286 0.021 0.003 10-22-98 325 0.024 0.003 04-30-98 288 0.022 0.003 10-29-98 288 0.037 0.004 05-07-98 283 0.023

  • 0.004 11-05-98 281 0.016 0.003 05-14-98 289 0.020 0.003 11-12-98 277 0.024
  • 0.003 05-21-98 285 0.028 i 0.003 11-19-98 286 0.037 1 0.004 05-28-98 283 0.016
  • 0.003 11-25-98 245 0.021 0.004 i

12-03-98' 06-04-98 285 0.019 1 0.003 06-10-98 244 0.013 t 0.003 12-10-98 286 0.028 0.004 06-18-98 328 0.020 0.003 12-17-98 286 0.023 0.004 06-25-98 277 0.016 0.003 12-23-98 246 0.023 0.004 07-02-98 271 0.017

  • 0.003 12-30-98 276 0.039 2 0.004 2nd Quarter Mean 2 s.d.

0.019

  • 0.004 4th Quarter Mean s.d.

0.025 1 0.009 Cumulative Average 0.025 Previous Annual Average 0.024

  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

8-1

DUANE ARNOLD l

Table 9. Airborne particulates and charcoal canisters, analyses for gross beta and iodine-131'.

i Location: D-11 (Toddville)

Units: pCi/m' Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m')

Gross Beta Collected (m')

Gross Beta Reauired LLD QSID D.fl0 01-08-98 246 0.019 0.003 07-09-98 286 0.021 0.003 j

01-15-98 287 0.037 2 0.004 07-16-98 285 0.022 1 0.003 1

01-22-98 283 0.046.+ 0.004 07-23-98 285 0.019 0.003 01-29-98 286 0.050. 0.005 07-30-98 285 0.023 0.003 02-05-98 285 0.030

  • 0.003 08-06-98 288 0.015 2 0.003 02-12-98 288 0.029
  • 0.003 08-13-98 284 0.024 t 0.003 02-19-98 285 0.031 0.003 08-20-98 285 0.031 0.003 02-25-98 244 0.017
  • 0.003 08-27-98 286 0.039 0.004 I

03-05-98 326 0.010 i 0.002 09-04-98 324 0.030 0.004 03-12-98 286 0.019 2 0.003 09-09-98 206 0.042 0.006 l

03-19-98 285 0.025 0.004 09-17-98 323 0.025 0.003 03-26-98 286 0.025 i 0.003 09-24-98 287 0.025 2 0.003 04-02-98 284 0.019 1 0.003 09-30-98 245 0.035 0.004 1st Quarter Mean s.d.

0.027

  • 0.012 3rd Quarter Mean
  • s.d.

0.027 0.008 04-09-98 283 0.012 2 0.003 10-07-98 285 0.016 0.003 04-16-98 286 0.019 0.003 10-14-98 286 0.017 0.003 04-23-98 285 0.018 0.003 10-22-98 325 0.025 0.002 04-30-98 287 0.022 0.003 10-29-98 287 0.036 0.004 05-07-98 283 0.020 0.003 11-05-98 283 0.020 2 0.004 i

05-14-98 287 0.018 0.003 11-12-98 288 0.024 0.003 05-21-98 285 0.027 2 0.003 11-19-98 286 0.037 0.004 05-28-98 284 0.020 0.003 11-25-98 245 0.017 0.004 12-03-98*

06-04-98 284 0.020 0.003 06-10-98 244 0.012 0.003 12-10-98 286 0.026 2 0.004 06-18-98 327 0.018 0.003 12-17-98 286 0.020 0.004 06-25-98 285 0.014 0.003 12-23-98 245 0.019 0.004 07-02-98 286 0.020 0.003 12-30-98 282 0.037 0.004 l

2nd Quarter Mean

  • s.d.

0.018 0.004 4th Quarter Mean

  • s.d.

0.025 0.008 i

Cumulative Average 0.024 Previous Annual Average 0.024 5

  • Iodine-131 concentrations are <0.07 pCi/m unless noted otherwise.
  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

9-1 l

l l

n 1

- DUANE ARNOLD l

Table 10. Airborne particulates, analysis for gross beta.

1 location: D-13 Units: pCi/m' Collection: Continuous, weekly exchange.

Date Volume Date Volume l

Collected (m')

Gross Beta Collected (m')

Gross Beta Reauired LLD QS10 QS10 I

01-08-98 244 0.019

  • 0.003 07-09-98 284 0.021 2 0.003 l

01-15-98 286 0.039 2 0.004 07-16-98 285 0.024 2 0.003 l

01-22-98 285 0.054 0.004 07-23-98 285 0.021 0.003 01-29-98 286 0.058 0.005 07-30-98 286 0.024 0.003 02-05-98 285 0.033

  • 0.003 08-06-98 286 0.018 2 0.003 02-12-98 287 0.027 0.003 08-13-98 284 0.024 0.003 02-19-98 284 0.027
  • 0.003 08-20-98 286 0.039 0.004 02-25-98 244 0.019 i 0.003 08-27-98 285 0.047 2 0.005 03-05-98 327 0.013
  • 0.003 09-04-98 324 0.037
  • 0.004 03-12-98 285 0.016
  • 0.003 09-09-98 206 0.063 0.006 03-19-98 285 0.018
  • 0.003 09-17-98 324 0.036 0.004 03-26-98 285 0.019 0.003 09-24-98 289 0.028 0.004 04-02-98 285 0.011 1 0.003 09-30-98 246 0.056
  • 0.005 1st Quarter Mean i s.d.

0.027

  • 0.015 3rd Quarter Mean s.d.

0.034

  • 0.014 04-09-98 284 0.010
  • 0.003 10-07-98 284 0.026 0.004 04-16-98 284 0.015 2 0.003 10-14-98 286 0.020 2 0.003 04-23-98 286 0.016 0.003 10-22-98 326 0.037 0.004 04-30-98 286 0.017 0.003 10-29-98 286 0.049 0.005 05-07-98 283 0.018
  • 0.003 11-05-98 283 0.014
  • 0.003 05-14-98 288 0.019 i 0.003 11-12-98 288 0.022
  • 0.003 05-21-98 284 0.025 0.003 11-19-98 283 0.034 t 0.004 05-28-98 285 0.016 0.003 11-25-98 245 0.019 t 0.004 12-03-98*

06-04-98 282 0.021

  • 0.003 06-10-98 243 0.012
  • 0.003 12-10-98 286 0.022 0.004 06-18-98 328 0.020 0.003 12-17-98 286 0.022
  • 0.004 06-25-98 286 0.016
  • 0.003 12-23-98 244 0.021
  • 0.004 07-02-98 286 0.011
  • 0.003 12-30-98 284 0.038 1 0.004 2nd Quarter Mean s.d.

0.017 0.004 4th Quarter Mean

  • s.d.

0.027 1 0.010 l

Cumulative Average 0.026 4

Previous Annual Average 0.023

' No Data; Refer to Table 2.0, "1.isting of Missed Samples".

l l

10-1

DUANE ARNOLD Table 11. Airbame particulates and charcoal canisters, analyses for gross beta and iodine-131*.

Location: D-15(On-site)

Units: pCi/m' Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m')

Gross Beta Collected (m')

Gross Beta Required i ID QR1Q Q,Q10 01 08-98 246 0.017 1 0.003 07-09-98 281 0.014 0.003 01-15-98 286 0.031

  • 0.004 07-16-98 287 0.015
  • 0.003 01-22-98 285 0.045
  • 0.004 07-23-98 285 0.013 0.003 01-29-98 285 0.043 0.004 07-30-98 286 0.013 0.003 02-05-98 285 0.029 0.003 08-06-98 285 0.015 1 0.003 02-12-98 286 0.034 0.004 08-13-98 285 0.021 t 0.003 02-19-98 284 0.028
  • 0.003 08-20-98 285 0.024 t 0.003 02-25-98 244 0.017
  • 0.003 08-27-98 285 0.029 0.004 03-05-98 327 0.013 0.003 09-04-98 325 0.020 0.003 03-12-98 285 0.018 0.003 09-09-98 205 0.029 0.005 03-19-98 285 0.023 2 0.003 09-17-98 324 0.019 t 0.003 03-26-98 285 0.022 0.003 09-24-98 287 0.019 i 0.003 04-02-98 284 0.014 0.003 09-30-98 246 0.027 2 0.004 1st Quarter Mean
  • s.d.

0.026 i 0.010 3rd Quarter Mean

  • s.d.

0.020

  • 0.006 04-09-98 285 0.013 0.003 10-07-98 283 0.012 0.003 04-16-98 285 0.017 0.003 10-14-98 284 0.010 0.003 04-23-98 286 0.014 1 0.003 10-22-98 327 0.021 0.003 04-30-98 286 0.018 1 0.003 10-29-98 287 0.029 0.004 1

05-07-98 284 0.019

  • 0.003 11-05-98 283 0.014 2 0.003 05-14-98 287 0.015 0.003 11 12-98 286 0.019
  • 0.003 05-21-98 286 0.020 0.003 11 19-98 267 0.026
  • 0.004 05-28-98 285 0.016 i 0.003 11-25-98 264 0.014 1 0.004 6

12-03-98 06-04-98 279 0.014 0.003 06-10-98 244 0.007 2 0.003 12-10-98 286 0.026 2 0.004 06-18-98 326 0.014 0.002 12-17-98 286 0.020 0.004 06-25-98 286 0.010 1 0.003 12-23-98 216 0.015 0.004 07-02-98 288 0.015

  • 0.003 12-30-98 284 0.021 i 0.003 2nd Quarter Mean s.d.

0.015 0.004 4th Quarter Mean s.d.

0.019 0.006 Cumulative Average 0.020 Previous Anrnal Average 0.022

  • lodine-131 concentrations are <0.07 pCi/m' unless noted otherwise.
  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

11-1

DUANE ARNOLD Table 12. Airbome particulates, analysis for gross beta.

Location: D-16(On-site) 3 Units: pCi/m Collection: Continuous, weekly exchange.

Date Volume Date Volume Collected (m") -

Gross Beta Collected (m')

Gross Beta Required LLD Q,Q1Q Q,Q10

.01-08-98 246 0.013

  • 0.003 07-09-98 281 0.016 1 0.003 01-15-98 286 0.028 t 0.004 07-16-98 287 0.022 0.003 01-22-98 2L5 0.040 2 0.004 07-23-98 285 0.020 2 0.003 01-29-98 286 0.039 0.004 07-30-98 287 0.021 0.003 02-05-98 285 0.029 0.003 08-06-98 285 0.012 0.003 02-12-98 286 0.028
  • 0.003 08-13-98 285 0.024 0.003 j

02-19-98 285 0.030 0.003 08-20-98 285 0.031 0.003

}

02-25-98 244 0.021 0.004 08-27-98 285 0.030 0.004 l

03-05-98 327 0.011 t 0.003 09-04-98 325 0.025 0.003 03-12-98 285 0.024 0.003 09-09-98 205 0.037 0.005 03-19-98 285 0.026

  • 0.004 09-17-98 325 0.024
  • 0.003 03-26-98 285 0.023 1 0.003 09-24-98 288 0.021 0.003 04-02-98 285 0.013 0.003 09-30-98 246 0.031 t 0.004 1st Quarter Mean
  • s.d.

0.025 0.009 3rd Quarter Mean s.d.

0.024 0.007 04-09-98 275 0.012 0.003 10-07-98 283 0.015 0.003 04-16-98 281 0.018 1 0.003 10-14-98 284 0.014 2 0.003 04-23-98 286 0.016

  • 0.003 10-22-98 327 0.018 0.003 04-30-98 286 0.017 1 0.003 10-29-98 288 0.038 0.004 05-07-98 284 0.019 i 0.003 11-05-98 283 0.020 0.004 05-14-98 287 0.019
  • 0.003 11-12-98 286 0.019 0.003 05-21-98 283 0.024 2 0.003 11-19-98 286 0.035
  • 0.004 05-28-98 284 0.017
  • 0.003 11-25-98 246 0.016
  • 0.004 12-03-98' 06-04-98 287 0.017 0.003 06-10-98 244 0.009
  • 0.003 12-10-98 286 0.024 1 0.004 06-18-98 326 0.015 1 0.003 12-17-98 286 0.021 2 0.004 06-25-98 287 0.013 t 0.003 12-23-98 244 0.024 2 0.004 07-02-98 287 0.017 2 0.003 12-30-98 283 0.035 0.004 2nd Quarter Mean s.d.

0.016 0.004 4th Quarter Mean s.d.

0.023 0.008 Cumulative Average 0.022 Previous Annual Average 0.023

  • No Data; Refer to Table 2.0, " Listing of Missed Samples".

12-1

{

r DUANE ARNOLD Table 13. Airborne particulates, analyses for gamma-emitting isotopes.

Collection: Quarterly Composite Units: pCi/m3 Location D-1 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2469 DAP-5395 DAP-8255 DAP-11232 Volume (m')

3670 3711 3670 3386 Be-7 0.069 s. 0.013 0.077 0.012 0.097

  • 0.014 0.052 0.011 Zr-95

< 0.0016

< 0.0008

< 0.0008

< 0.0017 Nb-95

< 0.0014

< 0.0007

< 0.0012

< 0.0010 Ru-103

< 0.0012

< 0.0004

< 0.0009

< 0.0009 Ru-106

< 0.0042

< 0.0059

< 0.0067

< 0.0071 Cs-134

< 0.0004

< 0.0008

< 0.0009

< 0.0009 I

Cs-137

< 0.0009

< 0.0008

< 0.0008

< 0.0006 Ce-141

< 0.0007

< 0.0013

< 0.0015

< 0.0013 Ce-144

< 0.0018

< 0.0048

< 0.0045

< 0.0038 Location D-2 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2470 DAP-5396 DAP-8256 DAP-11233 Volume (m')

3671 3709 3669 3387 Be-7 0.066 0.019 0.110 0.017 0.112 0.013 0.054 0.016 I

Zr-95

< 0.0007

< 0.0007

< 0.0018

< 0.0021 Nb-95

< 0.0008

< 0.0006

< 0.0005

< 0.0017 Ru-103

< 0.0007

< 0.0003

< 0.0007

< 0.0012 Ru-106

< 0.0081

< 0.0046

< 0.0045

< 0.0086 Cs-134

< 0.0016

< 0.0004

< 0.0007

< 0.0005 Cs-137

< 0.0010

< 0.0007

< 0.0006

< 0.0005 Ce-141

< 0.0017

< 0.0012

< 0.0011

< 0.0016 Ce-144

< 0.0029

< 0.0048

< 0.0016

< 0.0035 Location D-3 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2471 DAP-5397 DAP-8257 DAP-11234 Volume (m')

3664 3704 3670 3385 Be-7 0.052 1 0.009 0.100 0.016 0.111 0.015 0.073 0.021 Zr-95

< 0.0009

< 0.0007

< 0.0023

< 0.0026 Nb-95

< 0.0009

< 0.0007

< 0.0014

< 0.0009 Ru-103

< 0.0009

< 0.0006

< 0.0005

< 0.0014 Ru-106

< 0.011

< 0.0059

< 0.0050

< 0.010 Cs-134

< 0.0005

< 0.0017

< 0.0007

< 0.0007 Cs-137

< 0.0009

< 0.0007

< 0.0007

< 0.0010 Cc-141

< 0.0009

< 0.0019

< 0.0017

< 0.0015 Ce-144

< 0.0044

< 0.0028

< 0.0022

< 0.0033 13-1

q DUANE ARNOLD

. Table 13. Airbome particulates, analyses for gamma-emitting isotopes.

Cuection: Quarterly Composite Units: pCi/m3 Location D-5 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code ~

DAP-2472 DAP-5398 DAP-8258 DAP-11235 Volume (m')

3670 3693 3667 3380 Be-7 0.067 0.011 0.095

  • 0.013 0.101 0.015 0.058 0.012 Zr-95

< 0.0023

< 0.0009

< 0.0009

< 0.0017 Nb-95

. < 0.0006

< 0.0006

< 0.0014

< 0.0010 Ru-103

< 0.0010

< 0.0008

< 0.0005

< 0.0009 I

Ru-106

< 0.0072

< 0.0062

< 0.0067

< 0.0058 j

Cs-134

< 0.0005

< 0.0017

< 0.0005

< 0.0007

. Cs-137

< 0.0007

< 0.0006

< 0.0006

< 0.0007.

Ce-141

< 0.0014

< 0.0011

< 0.0011

< 0.0015 Ce-144

< 0.0050 '

< 0.0043 -

< 0.0022

< 0.0033 Location D-6 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2473 DAP-5399

. DAP-8259 DAP-11236 Volume (m')

3670 3708~

3671 3384 Be-7 0.060 0.013 0.112 t 0.013 0.106 0.016 0.052 t 0.016 Zr-95

< 0.0007

< 0.0011

< 0.0007

< 0.0032 Nb-95

< 0.0009

. < 0.0008

< 0.0005

< 0.0008 Ru-103

< 0.0008

< 0.0003

< 0.0012

< 0.0017 Ru-106

< 0.0028

< 0.0042

< 0.0034

< 0.014 Cs-134

< 0.0016

< 0.0016

< 0.0004

< 0.0011 Cs-137

< 0.0008

< 0.0008

< 0.0007

< 0.0014 Ce-141

< 0.0019

< 0.0020

< 0.0009

< 0.0020 Ce-144

< 0.0059

< 0.0053

< 0.0030

< 0.0048 Location D-7 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2474 DAP-5400 DAP-8260 DAP-11237

Volume (m')

3670 3703 3666 3382 Be-7.

0.069 0.014 0.110 0.014 0.100

  • 0.017 0.063 0.014 Zr-95

< 0.0010

< 0.0011

< 0.0017

< 0.0022

]

Nb < 0.0016

< 0.0003

< 0.0013

< 0.0006 Ru-103

< 0.0005

< 0.0008

< 0.0012

< 0.0012 Ru 106

< 0.0072

< 0.0040

< 0.0067

< 0.0061 Cs-134

< 0.0003

< 0.0003

< 0.0003

< 0.0005 Cs-137

< 0.0010

< 0.0012

< 0.0004

< 0.0004 Ce-141

< 0.0015

< 0.0020

< 0.0008

< 0.0009

' Ce-144

< 0.0051

< 0.0048

< 0.0047

< 0.0033 j

f 13 2

l DUANE ARNOLD Table 13. Airborne particulates, analyses for gamma-emitting isotopes.

Collection: Quarterly Composite Units: pCi/m3 Location D-8 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2475 DAP-5401 DAP-8261 DAP-11238 Volume (m')

3669 3708 3669 3381

- Be-7 0.079 0.014 0.111

  • 0.016 0.112 0.017 0.061. 0.015 Zr-95

< 0.0006

< 0.0006

< 0.0015

< 0.0023 Nb-95

< 0.0003

< 0.0004

< 0.0015

< 0.0016 Ru-103

< 0.0006

< 0.0009

< 0.0006

< 0.0006 Ru-106

< 0.0080

< 0.0043

< 0.0039

< 0.0088 Cs-134

< 0.0016

< 0.0016

< 0.0007

< 0.0011 Cs-137

< 0.0009

< 0.0008

< 0.0009

< 0.0005 i

Ce-141

< 0.0010

< 0.0019

< 0.0014

< 0.0022 Ce-144

< 0.0021

< 0.0054

< 0.0033

< 0.0065 Location D-10 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2476 DAP-5402 DAP-8262 DAP-11239 Volume (m')

3668 3685 3671 3367 Be-7 0.075 0.014 0.103 0.015 0.098 0.015 0.060 0.013 Zr-95

< 0.0012

< 0.0009

< 0.0015

< 0.0012 Nb-95

< 0.0015

< 0.0013

< 0.0009

< 0.0006 Ru-103

< 0.0006

< 0.0008

< 0.0011

< 0.0005 Ru-106

< 0.0067

< 0.0025

< 0.0034

< 0.0041 i

Cs-134

< 0.0010

< 0.0015

< 0.0005

< 0.0005 Cs-137

< 0.0007

< 0.0008

< 0.0007

< 0.0004 Ce-141

< 0.0017

< 0.0014

< 0.0013

< 0.0013 Ce-144

< 0.0036

< 0.0019

< 0.0024

< 0.0021 Location D-11

- Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2477 DAP-5403 DAP-8263 DAP-11240 Volume (m')

3671 3706 3669 3384 Be-7 0.066

  • 0.013 0.107
  • 0.015 0.098 0.017 0.053 0.017 Zr-95

< 0.0012

< 0.0008

< 0.0022

< 0.0017 Nb-95

< 0.0005

< 0.0008

< 0.0008

< 0.0006 i

Ru-103

< 0.0006

< 0.0010

< 0.0008

< 0.0011 l

Ru-106

< 0.0070

< 0.0053

< 0.0038

< 0.0058 Cs-134

< 0.0007

< 0.0004

< 0.0007

< 0.0004 Cs-137

< 0.0007

< 0.0010

< 0.0008

< 0.0008 Ce-141

< 0.0012

< 0.0014

< 0.0011

< 0.0009 Ce-144

< 0.0043

< 0.0039

< 0.0049

< 0.0033 r

13-3

DUANE ARNOLD Table 13. Airborne particulates, analyses for gamma-emitting isotopes.

Collection: Quarterly Composite Units: pCi/m3 Location D-13 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2478 DAP-5404 DAP-8264 DAP-11241 Volume (m')

3668 3705 3670 3381 Be-7 0.072 1 0.011 0.111

  • 0.016 0.110 0.019 0.073 1 0.014 Zr-95

< 0.0005

< 0.0006

< 0.0014

< 0.0012 j

Nb-95

< 0.0009

< 0.0008

< 0.0019

< 0.0010 Ru-103

< 0.0004

< 0.0010

< 0.0008

< 0.0012 Ru-106

< 0.0076

< 0.0033

< 0.0056

< 0.0087 Cs-134

< 0.0015

< 0.0006

< 0.0010

< 0.0010 Cs-137

< 0.0008

< 0.0009

< 0.0007

< 0.0012 Ce-141

< 0.0015

< 0.0007

< 0.0026

< 0.0012 Ce-144

< 0.0039

< 0.0041

< 0.0055

< 0.0060 Location D-15 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2479 DAP-5405 DAP-8265 DAP-11242 Volume (m')

3667 3707 3666 3353 Be-7 0.064 0.013 0.092 0.012 0.071 0.015 0.050 0.012 Zr-95

< 0.0007

< 0.0010

< 0.0019

< 0.0008 Nb-95

< 0.0008

< 0.0009

< 0.0013

< 0.0010 Ru-103

< 0.0003

< 0.0008

< 0.0008

< 0.0009 Ru-106

< 0.0030

< 0.0030

< 0.0007

< 0.0037 Cs-134

< 0.0016

< 0.0005

< 0.0005

< 0.0006 Cs-137

< 0.0009

< 0.0006

< 0.0004

< 0.0003 Ce-141

< 0.0015

< 0.0008

< 0.0013

< 0.0012 Ce-144

< 0.0054

< 0.0039

< 0.0031

< 0.0027 Location D-16 Quarter 1st Quarter 2nd Quarter 3rd Quarter 4th Quarter Lab Code DAP-2480 DAP-5406 DAP-8266 DAP-11243 Volume (m')

3670 3699 3669 3382 Be-7 0.068 0.013 0.100 0.016 0.073

  • 0.014 0.058 0.019 Zr-95

< 0.0008

< 0.0015

< 0.0014

< 0.0026 Nb-95

< 0.0005

< 0.0006

< 0.0013

< 0.0022 Ru-103

< 0.0008

< 0.0010

< 0.0009

< 0.0017 Ru-106

< 0.0036

< 0.0050

< 0.0072

< 0.013 Cs-134

< 0.0017

< 0.0002

< 0.0004

< 0.0012 Cs-137

< 0.0007

< 0.0010

< 0.0008

< 0.0013 Ce-141

< 0.0018

< 0.0017

< 0.0013

< 0.0015 Ce-144

< 0.0045

< 0.0049

< 0.0041

< 0.0080 13-4

DUANE ARNOLD Table 13. Area monitors (TLD), Quarterly,1998.

Units: mR/91 days Air Stations 1st Otr.

2nd Otr.

3rd Otr.

.4th.Q1 D-1(C) 12.5

  • 0.2 13.7 0.2 163 i 0.2 13.4 0.2 D-2 (C) 12.910.2 13.1 0.3 16.2 03 12.4 i 03 D-3 12.7
  • 0.2 12.6 0.2 15.9 0.2 11.9 0.2 D-5 12.9 i 03 13.3
  • 03 173
  • 03 13.5203 D-6 123
  • 0.2 13.9 03 16.2203 13.7 0.3 D-7 12.6
  • 0.2 15.0 03 17.0 03 153 103 D-8 16.6
  • 0.2 20.120.4 20.8 0.4 18.8
  • 0.4 D-10 14.1
  • 0.2 14.5 0.2 20.020.2 15.0 0.2 D-11 9.7
  • 0.2 10.2 0.2 13.210.2 9.5 0.2 D-13 (C) 13.8
  • 0.2 15.6 0.2 17.8 0.2 15.0
  • 0.2 D-15 14.8 0.2 13.8
  • 03 17.8
  • 03 14.7
  • 03 D-16 15.6 i 0.2 12.9
  • 0.2 17.4 0.2 13.8 0.2 Mean s.d.

13.4 1.8 14.1 2.3 17.2

  • 2.0 13.9 2.2 l

i W/In 0.5 mi. of Stack D-18 15.6

  • 0.2 103 0.2 193 t 0.2 ND' D-19 14.1 0.2 11.5 03 18.2
  • 0.3 16.7
  • 0.2 D-20 16.5 i 03 13.6
  • 0.2 20.2
  • 0.2 18.2 0.2 D-21 17.110.2 123 0.2 21 3 0.2 17.0.0.2 D-22 14.920.2 11.7 03 18.6 03 16.7 0.2 D-23 14.120.2 93 *0.2 17.6
  • 0.2 15.0 0.2 D-28 17.8 0.2 143 0.2 22.3
  • 0.2 18.0
  • 0.2 D-29 19.2 0.2 16.0 0.3 23.4 03 20.4 03 D-30 18.9
  • 0.2 17.4 0.2 24.0 0.2 21.6
  • 0.2 D-31 19.6 0.2 16.9 0.2 233 t 0.2 20.7 03 D-32 19.6
  • 0.2 17.2 0.2 23.9 0.2 13.8
  • 0.2

{

D-82 14.5

  • 0.2 103
  • 0.2 18.2 0.2 14.5
  • 0.2 D 83 15.7
  • 0.2 12.7 0.2 19.2 0.2 16.3
  • 0.2 D-84 15.6
  • 0.2 11.8 03 19.4 03 15.3203 D-85 15.2
  • 0.2 12.6 0.2 19.8
  • 0.2 15.5 0.2 D-86 17.6 0.2 14.3 0.2 22.0 0.2 163 0.2 D-91 16.6
  • 0.2 15.9 t 0.4 18.4 t 0.4 17.0 t 0.2 Mean s.d.

16.6

  • 1.9 13.4 2.6 20.5 2.2 17.1
  • 2.2 14-1

1 l

DUANE ARNOLD l

Table 13. Area monitors (TLD), Quarterly,1998.

Units: mR/91 days l

W/in 1.0 mi. of 1st Otr.

2nd_Otr.

3rd Otr.

4th Otr.

S. tack l

D-43 14.7

  • 0.2 13.1
  • 0.2 19.9 i 0.2 -

ND' D-44 18.3 0.2 15.9 0.4 24.1 t 0.4 19.920.2 D-45 14.6

  • 0.2 13.1
  • 0.2 18.3 0.2 16.6 0.2 D-46 18.5 t 0.2 17.4 0.2 22.3 0.2 20.8 i 0.3 D-47 17.5 i 0.2 15.9 0.3 21.6 0.3 19.0
  • 2.5 D-48 ND' ND' 23.2 0.2 21.0 0.3

]

Mean s.d.

16.7

  • 1.9 -

15.1 i 1.9 21.6 2.1 19.5

  • 1.8 W/in 3.0 mi. of Stack I

)

i D-33 13.0

  • 0.2 9.820.2 17.4 0.2 13.8
  • 0.2 D-34 13.0
  • 0.2 11.3
  • 0.8 17.4 0.8 14.9
  • 0.4 D-35 14.1 0.2 10.2
  • 0.2 17.5 0.2 13.4 0.3 D-36 15.3
  • 0.2 12.520.2 19.7
  • 0.2 15.0 0.3 D-37 18.1
  • 0.2 15.8 0.4 22.5
  • 0.4 17.2 0.2 D-38 15.6 0.2 13.1 0.2 21.2 0.2 15.9 0.2 D-39 15.910.2 13.9 0.2 20.0 0.2 15.4
  • 0.2 D-40 14.8
  • 0.2 12.2
  • 0.2 14.6
  • 0.2 14.7 0.2 D-41 15.2
  • 0.2 12.6
  • 0.2 19.1
  • 0.2 15.4
  • 0.2 D-42 13.1
  • 0.2 11.8
  • 0.2 18.2
  • 0.2 14.9 0.4 Mean t s.d.

14.8

  • 1.6 12.321.7 18.8
  • 2.2 15.1
  • 1.1 I

l

  • ND = No data; TLD lost in the field.

14-2

DUANE ARNOLD Table 15. Milk samples, analyses for iodine-1^1 and gamma emitting isotopes, Collection: Monthly during non-grazing season (October 1 through April 30): biweekly i

during grazing season (May 1 through September 30)

Location D-63 Date Lab Concentration (pCi/L)

Collected Code I-131 K-40 Cs-134 Cs-137 Ba-140 La-140 01-06-98 DMI -88

<1.0 1280

  • 100

< 15

< 18

< 60

< 15 02-03-98

-658

<1.0 1320 110

< 15

< 18

< 60

< 15 03-05-98

-1335

< 1.0 1370 *110

< 15

< 18

< 60

< 15 04-07-98

-2140

<1.0 1350 i130

< 15

< 18

< 60

< 15 05-05-98

-3031

<1.0 1380 110

< 15

< 18

< 60

< 15 05-19-98

-3678

< 1.0 1210 150

< 15

< 18

< 60

< 15 06-02-98

-4094

<1.0 1340 180

< 15

< 18

< 60

< 15 06-16-98

-4404

< 1.0 1350 1180

< 15

< 18

< 60

< 15 06-30-98

-4780

< 1.0 1310 120

< 15

< 18

< 60

< 15 07-14-98

-5294

< 1.0 1440 140

< 15

< 18

< 60

< 15 07-28-98

-5764

< 1.0 1440 110

< 15

< 18

< 60

< 15 08-11-98

-6233

< 1.0 1360 190

< 15

< 18

< 60

< 15 08-25-98

-6729

< 1.0 1340 120

< 15

< 18

< 60

< 15 09-09-98

-7121

< 1.0 1350 160

< 15

< 18

< 60

< 15 09-22-98

-7566

< 1.0 1160 160

< 15

< 18

< 60

< 15 10-06-98

-8043

< 1.0 1210 160

< 15

< 18

< 60

< 15 11-03-98

-9434

< 1.0 1390 170

< 15

< 18

< 60

< 15 12-01-98

-10192

< 1.0 1150 170

< 15

< 18

< 60

< 15 Location D-93 Date Lab Concentration (pCi/L)

{

Collected Code I-131 K-40 Cs-134 Cs-137 Ba-140 La-140 01-06-98 ND*

02-03 DMI -659

<1.0 1400 *130

< 15

< 18

< 60

< 15 03-05-98

-1336

<1.0 1710 210

< 15

< 18

< 60

< 15 04-07-98

-2141

<1.0 1660 180

< 15

< 18

< 60

< 15 05-05-98

-3032

<1.0 1690 180

< 15

< 18

< 60

< 15 05-19-98

-3679

<1.0 1760 120

< 15

< 18

< 60

< 15 06-02-98

-4095

<1.0 2020 *210

< 15

< 18

< 60

< 15 06-16-98

-4405

<1.0 1900 130

< 15

< 18

< 60

< 15 06-30-98

-4781

<1.0 1830 i130

< 15

< 18

< 60

< 15 07-14-98

-5295

<1.0 1600 2 120

< 15

< 18

< 60

< 15 07-28-98

-5765

<1.0 1840 180

< 15

< 18

< 60

< 15 08-11-98

-6234

<1.0 1450 *170

< 15

< 18

< 60

< 15 08-25-98

-6730

<1.0 1860 190

< 15

< 18

< 60

< 15 09-09-98

-7122

<1.0 1780 160

< 15

< 18

< 60

< 15 09-22-98

-7567

<1.0 1660 2 200

< 15

< 18

< 60

< 15 10-06-98

-8044

< 1.0 1870 210

< 15

< 18

< 60

< 15 11-03-98

-9435

<1.0 1670

  • 190

< 15

< 18

< 60

< 15 12-01-98 ND'

  • ND=No data; sample not available.

15-1

DUANE ARNOLD Table 15. Milk samples, analyses for iodine-131 and gamma emitting isotopes, Collection: Monthly during non-grazing season (October 1 through April 30): biweekly during grazing season (May 1 through September 30) 1.acation D-96 Date Lab Concentration (pCi/L)

Collected Code I-131 K-40 Cs-134 Cs-137 Ba-140 La-140 01-06-98 DMI -89

< 1.0 1460 160

< 15

< 18

< 60

< 15 02-03-98

-660

< 1.0 1310 t 160

< 15

< 18

< 60

< 15 03-05-98

-1337

< 1.0 1420 170

< 15

< 18

< 60

< 15 04-07-98

-2142

< 1.0 1510 190

< 15

< 18

< 60

< 15 05-05-98

-3033

<1.0 1440 170

< 15

< 18

< 60

< 15 05-19-98

-3680

< 1.0 1370 170

< 15

< 18

< 60

< 15

)

06-02-98

-4096

<1.0 1350 150

< 15

< 18

< 60

< 15 06-16-98

-4406

<1.0 1470

  • 180

< 15

< 18

< 60

< 15 06-30-98

-4782

<1.0 1390 140

< 15

< 18

< 60

< 15 07-14-98

-5296

<1.0 1290 150

< 15

< 18

< 60

< 15 07-28-98

-5766

<1.0 1420 170

< 15

< 18

< 60

< 15 08-11-98

-6235

<1.0 1270

  • 190

< 15

< 18

< 60

< 15

)

08-25-98

-6731

<1.0 1520 170

< 15

< 18

< 60

< 15 09-09-98

-7123

<1.0 1470 140

< 15

< 18

< 60

< 15 09-22-98

-7568

<1.0 1320 1 170

< 15

< 18

< 60

< 15 10-06-98

-8045

<1.0 1360

  • 170

< 15

< 18

< 60

< 15 11-03-98

-9436

<1.0 1420 m140

< 15

< 18

< 60

< 15 12-01-98

-10193

< 1.0 1470 190

< 15

< 18

< 60

< 15 Location D-101 Date Lab Concentration (pCf /L)

Collected Code I-131 K-40 Cs-134 Cs-137 Ba-140 La-140 01-06-98 ND' 02-03-98 ND' 03-05-98 ND' 04-07-98 ND' 05-05-98 DMI -3034

<1.0 1400 120

< 15

< 18

< 60

< 15 05-19-98

-3681

<1.0 1420

  • 170

< 15

< 18

< 60

< 15 06-02-98

-4097

<1.0 1730 120

< 15

< 18

< 60

< 15 06-16-98

-4407

< 1.0 1630 *140

< 15

< 18

< 60

< 15 06-30-98

-4783

<1.0 1400

  • 210

< 15

< 18

< 60

< 15 07-14-98

-5297

<1.0 1390 170

< 15

< 18

< 60

< 15 l

07-28-98

-5767

<1.0 1610 190

< 15

< 18

< 60

< 15 08-11-98

-6236

<1.0 1590 i130

< 15

< 18

< 60

< 15 l

08-25-98

-6732

< 1.0 1600 190

< 15

< 18

< 60

< 15 l

09-09-98

-7124

<1.0 139C 110

< 15

< 18

< 60

< 15 09-22-98

-7569

<1.0 1480 180

< 15

< 18

< 60

< 15 10-06-98

-8046

<1.0 1270 120

< 15

< 18

< 60

< 15 11-03-98

-9437,8

<1.0 700 90

< 15

< 18

< 60

< 15 12-01-98 ND' 1

  • ND=No data; sample not available.

15-2 e

DUANE ARNOLD Table 15. Milk samples, analyses for iodine-131 and gamma emitting isotopes, Collection: Monthly during non-grazing season (October 1 through April 30): biweekly during grazing season (May 1 through September 30)

Location D-105 Date Lab Concentration (pCi/L)

Collected Code I-131 K-40 Cs-134 Cs-137 Ba-140 La-140 01-06-98 DMI -90

<1.0 1290 110

< 15

< 18

< 60

< 15 02-03-98

-661

< 1.0 1360 160

< 15

< 18

< 60

< 15 03-05-98

-1338

< 1.0 1370 130

< 15

< 18

< 60

< 15 04-07-98

-2143

<1.0 1450 170

< 15

< 18

< 60

< 15 05-05-98

-3035

<1.0 1480 200

< 15

< 18

< 60

< 15 05-19-98

-3682

<1.0 1300 120

< 15

< 18

< 60

< 15 06-02-98

-4098

<1.0 1320 170

< 15

< 18

< 60

< 15 06-18-98 ND' 06-30-98

-4784

<1.0 1360

  • 170

< 15

< 18

< 60

< 15 07-14-98

-5298

<1.0 1450

  • 110

< 15

< 18

< 60

< 15 07-28-98

-5768

<1.0 1410 120

< 15

< 18

< 60

< 15 08-11-98

-6237

<1.0 1340

  • 120

< 15

< 18

< 60

< 15 08-25-98

-6733

<1.0 1340 110

< 15

< 18

< 60

< 15 09-09-98

-7125

< 1.0 1360 100

< 15

< 18

< 60

< 15 09-22-98

-7570

< 1.0 1240 180

< 15

< 18

< 60

< 15 10-06-98

-8047

<1.0 1440 120

< 15

< 18

< 60

< 15 11-03-98

-9439

<1.0 1490 180

< 15

< 18

< 60

< 15 12-01-98

-10194

< 1.0 1440 170

< 15

< 18

< 60

< 15

  • ND=No data; sample lost in shipping.

15-3

DUANE ARNOLD l

Table 16. Well water samples, analyses for gross beta and tritium.

Collection: Quarterly Units: pC1/L Location D-53 Treated MunicipalWater l

Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DWW-1785 DWW-5299 DWW-8073,4 DWW-10703 Gross Beta 3.8 0.7 2.3

  • 0.6 2.8 0.4 3.3

< 161

< 176

< 161

< 157 Location D-54 Inlet to Municipal Water Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DWW-1786 DWW-5300 DWW-8075 DWW-10704 Gross Beta 3.2

  • 0.7 3.1
  • 0.6 3.6 1 1.0 3.1 0.7 H-3

< 161

< 176

< 161

< 157 Location D-55 On-site Well Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DWW-1787 DWW-4408 DWW-8076 DWW-10705 Gross Beta

< 1.0

< 1.0

< 1.0

< 1.0 4

H-3

< 161

< 156

< 161

< 157 Location D-57 Bull Farm Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DWW-1788 DWW-4409 DWW-8077 DWW-10706 Gross Beta 1.8 0.6 1.2 0.6

< 1.3 1.4

< 161

< 156

< 161

< 157 Location D-58 Franz Farm Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DWW-1789 DWW-4410,11 DWW-8078 DWW-10707 Gross Beta 4.1

  • 0.7 5.4 0.6 6.3
  • 1.1 5.0 t 0.8 H-3

< 161

< 156

< 161

< 157 Location D-72 Van Note Farm Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

l Lab Code DWW-1790 DWW-4412 DWW-8079 DWW-10708 l

Gross Beta 1.120.6

< 1.0

< 1.0 1.5 0.6 H-3

< 161

< 156

< 161

< 157 16 DUANE ARNOLD Table 17. Vegetation (broadleaf), analyses for iodine-131 and other gamma-emitting isotopes.

Collection: Annually Units: pCi/g wet Indicator location' D-57 D-93 D-94 D-106 Lab Code DVE-5775 DVE-5776 DVE-5777 DVE-5779 Date Collected 7/28/98 7/28/98 7/28/98 7/28/98 Sample Type Cabbage Cabbage Cabbage Cabbage K-40 2.01

  • 0.40 2.16 0.36 2.06

< 0.008

< 0.011

< 0.014

< 0.011 Co-58

< 0.010

< 0.011

< 0.008

< 0.006 Co 60

< 0.010 -

< 0.017

< 0.022

< 0.016 Nb-95

< 0.018

< 0.019

< 0.019

< 0.013 Zr-95

< 0.039

< 0.035

< 0.054

< 0.022 Ru-103

< 0.011

< 0.015

< 0.019

< 0.009 Ru-106

< 0.14

< 0.13

< 0.12

< 0.12 I-131

< 0.036

< 0.028

< 0.029

< 0.016 Cs-134

< 0.012

< 0.011

< 0.017

< 0.015 Cs-137

< 0.013

< 0.019

< 0.022

< 0.016 Ce-141

< 0.031

< 0.027

< 0.014

< 0.023 Ce-144

< 0.065

< 0.12

< 0.090

< 0.11 Control Location D-105 Lab Code DVE-5778 Date Collected 7/28/98 Sample Type Cabbage K-40 4.03

< 0.018 Co-58

< 0.018 Co-60

< 0.028 Nb-95

< 0.030 Zr-95

< 0.026 Ru-103

< 0.017 Ru-106

< 0.14 I-131

< 0.040 Cs-134

< 0.031 Cs-137

< 0.027 Ce-141

< 0.029 Ce-144

< 0.089 17-1

r- -- _

DUANE ARNOLD

~ Table 18. Vegetation (hay and grain), analyses for gamma-emitting isotopes.

Collection: Annually Units: pCi/g wet i

Location D D-57 D-58 D-63 D-72 Lab Code DVE-9045 DVE-9046 DVE-9047 DVE-9048 DVE-9049 Date Collected 10/23/98 10/27/98 10/27/98 10/27/98 10/27/98 l

Sample Type Soybeans Com Com Com Com l'

K - 10.51 0.47 2.982 0.41 2.482 0.28 2.40 0.46 2.52 0.30 l

Mn-54

< 0.014

< 0.017

< 0.010

< 0.012

< 0.004 I

Co-58

< 0.009

< 0.012

< 0.007

< 0.007

< 0.008 Co-60

< 0.020

< 0.017

< 0.008

< 0.006

< 0.004 Nb-95

< 0.017

< 0.022

< 0.008

< 0.011

< 0.010 l

Zr < 0.044

< 0.018

< 0.012

< 0.028

< 0.019 Ru-103

< 0.016

< 0.011

< 0.006

< 0.012

< 0.010 j

Ru-106

< 0.13

< 0.19

< 0.054

< 0.17

< 0.11 l

Cs-134

< 0.017

< 0.017

< 0.012

< 0.010

- < 0.013 Cs-137

< 0.019

< 0.017

< 0.006

< 0.015

< 0.012 Ce-141

< 0.029 '

< 0.025

< 0.016

< 0.028

< 0.013 Ce-144

< 0.072

< 0.089

< 0.065

< 0.092

< 0.083 l

l l

Location D-105 D-106 Lab Code DVE-9050 DVE-9051 Date Collected 10/27/98 10/27/98 Sample Type --

Com Com K-40 2.85

< 0.014

< 0.017 Co-58

< 0.016

< 0.014 CcH50

< 0.016

< 0.016 l

Nb-95

< 0.022

< 0.023 Zr-95 '

< 0.015

< 0.017 Ru-103 -

< 0.016

< 0.021 Ru-106

< 0.11

< 0.11 Cs-134

< 0.014

< 0.018 Cs-137

< 0.010

< 0.017 Ce-141

< 0.028

< 0.035 Ce-144

< 0.12

< 0.066 18-1

F DUANE ARNOLD Table 18. Vegetation (hay and grain), analyses for gamma-emitting isotopes.

Collection: Annually Units: pCi/g wet Location D-16 D-57 D-63 D-72 D-105 (C)

Lab Code DVE-9440 DVE-9441 DVE-9442 DVE-9443 DVE-9444 Date Collected 11/3/98 11/3/98 11/3/98 11/3/98 11/3/98 Sample Type Grass Hay

. Hay Hay Hay K-40 7.88 1.68 12.87 0.88 21.66 i 0.76 17.36 1.11 16.56 0.93 Mn-54

< 0.078

< 0.039

< 0.014

< 0.043

< 0.037 Co-58

< 0.039

< 0.031

< 0.028

< 0.018

< 0.033 Co-60

< 0.043

< 0.023

< 0.035

< 0.051

< 0.036 Nb-95

< 0.047

< 0.031

< 0.029

< 0.045

< 0.036 Zr-95

< 0.091

< 0.047

< 0.039

< 0.10

< 0.091 Ru-103

< 0.062

< 0.033

< 0.029

< 0.021

< 0.030 Ru-106

< 0.65

< 0.28

< 0.23

< 0.19

< 0.32 Cs-134

< 0.030

< 0.056

< 0.043

< 0.054

< 0.024 Cs-137

< 0.038

< 0.027

< 0.031

< 0.038

< 0.042 Ce-141

< 0.057

< 0.041

< 0.055

< 0.030

< 0.059 Ce-144

< 0.23

< 0.095

< 0.12

< 0.14

< 0.22 l

18-2

f l

DUANE ARNOLD j

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

i Collection: Monthly Units:

pCi/L Location:

D-49 l

Date Collected 01-09-98 02-24-98 03-23-98 l

Lab Code DSW-230 DSW-1112 DSW-1779 Mn-54

<15

<15

<15 l

Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 l

Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15

{

Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 l

La-140

<15

<15

<15 Date Collected 04-27-98 05-26-98 06-15-98 i

Lab Code DSW-2748 DSW-3855 NS' Mn-54

<15

<15 Fe-59

<30

<30 l

Co-58

<15

<15 Co-60

<15

<15 Zn-65

<30

<30 Nb-95

<15

<15 Zr-95

<30

<30 1-131

<15

<15 Cs-134

<15

<15 I

Ce137

<15

<15 Ba-140

<60

<60 La-140

<15

<15 a NS= No sample; Sample lost in shipment.

19-1

f DUANE ARNOLD l

l Table 19. Surface water samples, analyses foriodine-131 and gamma-emitting isotopes.

Collection: Monthly Units:

pCi/L Location:

D-49 l

Date Collected 07-28-98 08-25-98 09-22-98 Lab Code DSW-5770 DSW-6734 DSW-7587 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 Date Collected 10-23-98 11-03-98 12-14-98 Lab Code DSW-9038 DSW-9445 DSW-10697 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 1-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<.60

<60

<60 La-140

<15

<15

<15 l

t 19-2

T:

DUANE ARNOLD l

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

j Collection: Monthly l

_ Units:

pCi/L Location:

D-50.

Date Collected 01-09-98 02-24-98 03-23-98 l

l' Lab Code DSW-231 DSW-1113 '

DSW-1780 Mn-54

<15

<15

<15

' Fe-59

<30

<30

<30 Co-58

<15

<15

<15 l

Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 l

Ba-140

<60

<60

<60 La-140

<15

<15

<15 Date Collected 04-27-98 05-26-98 06-15-98 Lab Code DSW-2749 DSW-3856 DSW-4414 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co 60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131-

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137 -

<15

<15

<15 Ba-140

<60

<60

<60

_ La-140

. <15

<15

<15 I

l-l 19-3

f; i'

DUANE ARNOLD i

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

j.

Collection: Monthly Units:

pCi/L Location:

D-50 Date Collected 07-28-98 08-25-98 09-22-98 Lab Code DSW-5771 DSW-6735 DSW-7588 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 l

Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 I

Date Collected 10-23-98 11-03-98 12-14-98 Lab Code DSW-9039 DSW-9446 DSW-10698 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 1

Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15-

<15

<15 l

Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 l

19-4

Ib DUANE ARNOLD i

i l

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

l Collection: Monthly Units:

pCi/L l

Location:

D-51 Date Collected 09-98 02-24-98 03-23-98 1

Lab Code DSW-232 DSW-1114 DSW-1781 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

- <15

<15

<15 Date Collected 04-27-98 05-26-98 06-15-98 Lab Code DSW-2750 DSW-3857 DSW-4415 Mn <15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 CW

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15

" Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140.

<60

<60

<60 La-140

<15

<15

<15 l

l 19-5 l

I DUANE ARNOLD i

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

Collection: Monthly Units:

pCi/L Location:

D-51.

. Date Collected 07-28-98

'08-25-98 09-22-98 Lab Code

. DSW-5772 DSW-6736 DSW-7589 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 1-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15.

<15

<15 Date Collected 10-23-98 11-03-98 12-14-98 Lab Code DSW-9040 DSW-9447 DSW-10699 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 19-6

y

)

5 DUANE ARNOLD i

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

Collection: Monthly Units:

pCi/L -

Location:

D-99 l

l Date Collected

~01-09-98.

02-24-98 03-23-98 l

l Lab Code DSW-233 DSW-1115 DSW-1782 l

l Mn <15

<15

<15 l

Fe-59

<30

' 30

<30 l

Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

.<30

<30 l

I-131

<15

<15

<15 l

Cs-134

<15

<15

<15 l

Cs-137

<15

<15

<15 l

Ba-140

<60

<60

<60 l

La-140

<15

<15

<15 Date Collected 04-27-98 05-26-98 06-15-98 Lab Code DSW-2751 DSW-3858 DSW-4416 Mn-54

<15

<15

<15 l

Fe-59

<30-

<30

<30 Co-58

<15

<15

<15 CW

<15

<15

<15

- Zn <30

<30

<30 j.

Nb-95

<15

<15

<15 I

Zr <30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15-

<15

' Ba-140

<60-

<60

<60 La-140

<15

<15

<15 19-7

[;

l DUANE ARNOLD t

Table 19. Surface water samples, analyses for iodine-131 and gamma-emitting isotopes.

Collection: Monthly Units:

pCi/L Location:

D-99 Date Collected 07-28-98 08-25-98 09-22-98 Lab Code DSW-5773 DSW-6737 DSW-7590 l

Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 Date Collected 10-23-98 11-03-98 12-14-98 I

Lab Code DSW-9041 DSW-9448 DSW-10700 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 l

Co-58

<15

<15

<15 L

Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 j

I-131

<15

<15

<15 i

Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 19-8

DUANE ARNOLD l

t L

Table 20. Surface water samples, analyses for potassium-40 by flame photometry, iodine-131 and gamma-emittingisotopes.

Collection: Monthly Units:

pCi/L Location:

D-107 Date Collected 01-09-98 02-24-98 03-23-98 Lab Code DSW-234 DSW-1116 DSW-1783 K-40 (fp) 18.2 18.2 18.2 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 i

Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 Date Collected 04-27-98 05-26-98 06-15-98 Lab Code DSW-2752 DSW-3859 DSW-4417 K-40 (fp) 26.8 12.1 12.1 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Cc-60

<15

<15

<15 i

Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La 140

<15

<15

<15 i

20-1 I

j g

DUANE ARNOLD e

Table 20. Surface water samples, analyses for potassium-40 by flame photometry, iodine-131 and gamma-emittingisotopes.

Collection: Monthly Units:

pCi/L Location:

D-107 Date Collected 07-28-98 08-25-98 09-22-98 Lab Code -

DSW-5774 DSW-6738 DSW-7591 K-40 (fp) 15.6 12.1 13.0 Mn-54

<15

<15

<15 Fe-59

<30

<30

<30 Co-58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 1-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba 140

<60

<60

<60 La-140

<15

<15

<15 D

Date Collected 10-23-98 11-03-98 12 14-98 Lab Code DSW-9042 DSW-9449 DSW-10701 K-40 (fp) 15.6 15.6 16.4 Mn-54

<15

<15

<i5 Fe-59

<30

<30

<30 Go 58

<15

<15

<15 Co-60

<15

<15

<15 Zn-65

<30

<30

<30 Nb-95

<15

<15

<15 Zr-95

<30

<30

<30 I-131

<15

<15

<15 Cs-134

<15

<15

<15 Cs-137

<15

<15

<15 Ba-140

<60

<60

<60 La-140

<15

<15

<15 20-2

DUANE ARNOLD Table 21. Surface water, analysis for tritium.

Collection: Quarterly composites of monthly samples.

Units: pCi/L Location D-49 Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DSW-2133 DSW-4626 DSW-7602 DSW-10908 H-3

< 157

< 157'

< 167

< 153 Location D-50 Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DSW-2134,5 DSW-4627 DSW-7603 DSW-10909 H3

< 157

< 159

< 167

< 157 Location D-51 Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DSW-2136 DSW-4628 DSW-7604 DSW-10910 H-3

< 157

< 156

< 167

< 153 Location D-99 Feriod 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DSW-2137 DSW-4629 DSW-7605 DSW-10911 H-3

< 157

< 156

< 167

< 153 l

l Location D-107 Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

Lab Code DSW-2138 DSW-4630 DSW-7606 DSW-10912 r

H-3

< 157

< 156

< 167

< 153

  • The composite for the second quarter includes collections from April and May,1998 only.

The June,1998 collection was lost in shipment.

l 21-1

DUANE ARNOLD Table 22. Fish, analyses of edible portion for gamma-emitting isotopes.

Collection: Semiannually Units: pCi/g wet Location Upstream, D-49 Lab Code DF-3861,2 DF-3863 DF-8069 DF-8070 Date Collected 5/21/98 5/21/98 10/2/98 10/2/98 Sample Type Carp Carpsucker Carp Carpsucker K-40 3.47 0.32 3.18 0.29 2.94 0.41 3.57 0.41 Mn-54

< 0.006

< 0.009

< 0.010

< 0.014 Fe-59

< 0.037

< 0.027

< 0.036

< 0.041 Co-58

< 0.013

< 0.014

< 0.019

< 0.014 Co-60

< 0.007

< 0.009

< 0.016

< 0.023 Zn-65

< 0.034

< 0.015

< 0.030

< 0.026 Nb-95

< 0.018

< 0.012

< 0.009

< 0.023 Zr-95

< 0.016

< 0.013

< 0.022

< 0.041 Ru-103

< 0.010

< 0.011

< 0.018

< 0.018 Ru-106

< 0.11

< 0.076

< 0.13

< 0.13 Cs-134

< 0.016

< 0.009

< 0.016

< 0.016 Cs-137

< 0.011

< 0.008

< 0.009

< 0.007 l

Ce-141

< 0.019

< 0.014

< 0.029

< 0.026 l

Ce-144

< 0.056

< 0.069

< 0.069

< 0.089 Location Downstream, D-61 Lab Code DF-3864 DF-3865 DF-8071 DF-8072 Date Collected 5/21/98 5/21/98 10/2/98 10/2/98 Sample Type Carp Carpsucker Carp Carpsucker K-40 2.972 0.41 3.56 z 0.25 3.582 0.45 3.38 0.46 Mn.54

< 0.011

< 0.008

< 0.010

< 0.015 Fe-59

< 0.016

< 0.022

< 0.039

< 0.047 l

Co-58

< 0.009

< 0.010

< 0.017

< 0.019 l

Co-60

< 0.015

< 0.011

< 0.020

< 0.021 Zn-65

< 0.023

< 0.008

< 0.039

< 0.027 Nb-95

< 0.022

< 0.011

< 0.024

< 0.010 l

Zr-95

< 0.020

< 0.014

< 0.042

< 0.021 Ru-103

< 0.022

< 0.010

< 0.018

< 0.013 Ru-106

< 0.078

< 0.058

< 0.086

< 0.13 Cs-134

< 0.013

< 0.003

< 0.008

< 0.024 Cs-137

< 0.008

< 0.008

< 0.014

< 0.014 Ce-141

< 0.033

< 0.010

< 0.033

< 0.033 Cc-144

< 0.084

< 0.051

< 0.087

< 0.054 22-1 i

.)

i DUANE ARNOLD l

Table 23. River sediment, analysis for gamma-emitting isotopes.

i-Collection: Semiannually Units: pCi/g dry j

Location D-50 (C)

Lab Code DBS-3852 DBS-7598,9 Date Collected 5/20/98 9/16/98 K-40 9.01 0.49 9.2610.44 Mn-54

< 0.010

< 0.012 Fe-59

< 0.028

< 0.041 Co-58

< 0.021

< 0.025 Co-60

< 0.012

< 0.013 Zn-65

< 0.070

< 0.054 Nb-95

< 0.007

< 0.012 Zr-95

< 0.019

< 0.011 Ru-103

< 0.009

< 0.020 Ru-106

< 0.12

< 0.096 Cs-134

< 0.014

< 0.025 I

Cs-137

< 0.021

< 0.006 Ce-141

< 0.022

< 0.041 Ce-144

< 0.069

< 0.087 1

Location D-51 Lab Code DBS-3853 DBS-7600 Date Collected 5/20/98 9/16/98 I

K-40 9.08 0.51 8.34 i 0.47 Mn-54

< 0.012

< 0.015 1

Fe-59

< 0.026

< 0.028 Co-58

< 0.007

< 0.026 Co-60

< 0.018

< 0.013 Zn-65

< 0.070

< 0.065 Nb-95

< 0.021

< 0.016 l

Zr-95

< 0.040

< 0.017 l

Ru-103

< 0.019

< 0.026 Ru-106

< 0.15

< 0.049 Cs-134

< 0.016

< 0.033 Cs-137 0.034 2 0.016

< 0.016 Ce-141

< 0.032

< 0.022 Ce-144

< 0.11

< 0.066 23-1 l.

DUANE ARNOLD Table 23. River sediment, analysis for gamma-emitting isotopes.

Collection: Semiannually Units: -pCi/g dry Location D-107 Lab Code DBS-3854 DBS-7601 Date Collected 5/20/98 9/16/98 K-40 7.38

< 0.024

< 0.013 Fe < 0.039

- < 0.031 Co-58

< 0.039

< 0.026

. Co-60 0.084

  • 0.026

< 0.021 Zn-65

< 0.11

< 0.083 Nb-95

< 0.019

< 0.023 Zr-95

< 0.044

< 0.032 Ru 103

< 0.026

< 0.010 Ru-106

< 0.17

< 0.058 Cs-134

< 0.020

< 0.038 Cs-137

< 0.020 0.051 t 0.020 Ce-141

< 0.063

< 0.050 Ce-144

< 0.12

< 0.098 i

l 23-2 L

l, DUANE ARNOLD I

Table 24. Precipitation samples, analyses for gamma emitting isotopes.

j Collection: Monthly l

Units:

pCi/L l

Location:

DAEC 1'

i Date Collected 01-09-98 02-24-98 03-28-98 L.ab Code DP-235 DP-1117 DP-1784 Mn-54

< 7.0

< 3.6

< 4.9 Fe-59

< 8.6

< 5.4

< 6.1 Co.58

< 3.6

< 2.1

< 2.6 Co-60

< 6.2

< 4.8

< 4.8 Zn-65

< 19.7

< 5.1

< 6.1 Nb-95

< 4.7

< 2.9

< 4.9 Zr-95

< 7.5

< 3.0

< 10.9 I-131

< 12.3

< 4.0

< 6.5 Cs-134

< 7.9

< 6.7

< 4.8 Cs-137

< 6.3

< 3.8

< 5.8 Ba-140

< 29.0

< 14.3

< 10.4 l

La-140 -

< 4.3

< 3.4

< 4.5 Date Collected 04-27-98 05-26-98 06-15-98 I

1 Lab Code DP-2753 DP-3860 DP-4413 Mn-54

< 3.7

< 4.0

< 3.8 l

Fe-59

< 3.7

< 9.6

< 6.7 Co-58

< 2.8

< 2.8

< 4.0 l

. Co-60

< 5.0

< 4.0

< 5.7 l

Zn-65

< 4.1

< 7.5

< 6.2 i

Nb-95

< 4.9

< 5.5

< 5.7 Zr-95

< 9.0

< 5.4

< 6.0 I-131

< 6.9

< 5.4

< 6.2 Cs-134

< 8.0

< 6.2

< 5.9 Cs-137

< 2.7

< 5.7

< 5.2 Ba-140

< 12.5

< 16.1

< 25.4 La-140

< 2.9

< 2.3

< 2.8 14-1

DUANE ARNOLD Table 24. Precipitation samples, analyses for gamma emitting isotopes.

Collection: Monthly Units:

pCi/L Location:

DAEC Date Collected 07-28-98 08-26-98 09-30-98 Lab Code DP-5769 DP-6739 DP-8080 Mn-54

< 3.8

< 5.5

< 4.1 Fe-59

< 9.4

< 5.8

< 7.8 Co-58

< 3.4

< 5.5

< 2.5 Co-60

< 3.5

< 5.0

< 2.8 Zn-65

< 6.8

< 5.9

< 7.7 Nb-95

< 4.1

< 3.8

< 6.9 Zr-95

< 8.3

< 13.3

< 7.5 I-131

< 3.0

< 6.5

< 12.4

{

Cs-134

< 3.7

< 6.9

< 4.0 l

Cs-137

< 3.4

< 8.5

< 3.7 Ba-140 -

< 9.9

< 32.9

< 24.3 La-140

< 3.1

< 6.7

< 9.0 Date Collected 10-23-98 11-03-98 12-14-98 Lab Code DP-9037 DP-9450 DP-10702 Mn-54

< 4.9

< 2.9

< 6.2 Fe-59

< 12.7

< 10.5

< 10.2 Co-58

< 4.1

< 5.4

< 3.3 Co-60

< 2.1

< 3.9

< 7.1 Zn-65

< 8.4

< 16.5

< 17.2 Nb-95

< 5.5

< 4.4

< 4.2 Zr-95

< 9.8

< 7.6

< 7.9 I-131

< 26.2

< 9.0

< 7.1 Cs-134

< 5.3

< 5.8

< 3.8 Cs-137

< 4.5

< 3.4

< 6.9 l

Ba-140

< 36.8

< 24.2

< 21.8 l

La-140

< 14.0

< 7.1

< 4.4 24-2 L.

r DUANE ARNOLD

- Table 25. Precipitation samples, analysis for tritium.

Collection: Quarterly composites of monthly samples.

Units: pCi/L Location Duane Arnold Period 1st Qtr.

2nd Qtr.

3rd Qtr.

4th Qtr.

_ Lab Code DP-2139_ -

DP-4625 DP-7607 DP-10913 H-3

< 157

< 156

< 167

< 153 25-1

DUANE ARNOLD l

Table 27. Soil, analysis for strontium-90 and gamma-emitting isotopes.

Collection: Annually -

Units: pCi/g dry Location D D-16 Lab Code DSO-9043 DSO-9044 i

Date Collected' 10/26/98 10/26/98 Sr-90 '

O.036

  • 0.013 0.035
  • 0.010 K-40 16.12 1.03 8.93 t 0.40 l-Mn-54

< 0.030

< 0.013 l

Fe-59

< 0.066

< 0.028 Co-58

< 0.054

< 0.018 Co-60

< 0.028

< 0.016 Zn-65

< 0.17

< 0.058 j

Nb-95

< 0.033

< 0.022 Zr-95

< 0.074 -

< 0.040 Ru-103

< 0.035

< 0.011 Ru-106

< 0.32

< 0.13 Cs-134

' < 0.053

< 0.017 Cs-137 0.085

  • 0.040

~ 0.22

  • 0.024 Ce-141

< 0.082

< 0.025 Ce-144

< 0.25

< 0.079 27 1