ML20134P244

Radioactive Effluent Rept for Jan-June 1985

ML20134P244
Person / Time
Site:	La Crosse File:Dairyland Power Cooperative icon.png
Issue date:	06/30/1985
From:	Taylor J DAIRYLAND POWER COOPERATIVE
To:	James Keppler NRC OFFICE OF INSPECTION & ENFORCEMENT (IE REGION III)
References
LAC-11065, NUDOCS 8509060212
Download: ML20134P244 (19)

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RADIOACTIVE EFFLUENT REPORT FOR THE LA CROSSE BOILING WATER REACTOR i (JANUARY 1, 1985 TO JUNE 30, 1985)

DAIRYLAND POWER COOPERATIVE

Docket No. $0-409 s

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8509060212 850630 PDR ADOCK 05000409 R PDR

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INTRODUCTION:

The La Crosse Boiling Water Reactor, also known as Genoa No. 2, is located on the east bank of the Mississippi River near Genoa, Vernon County, Wisconsin.- The plant was designed and constructed by the 3

Allis-Chalmers Manufacturing. Company. It was completed in 1967 and has a generation capacity of 50 MW (165 MW (th)). The reactor is owned and operated by Dairyland Power Cooperative (DPC).

4 For the first half of 1985, the plant has had a maximum dependable capccity factor (MDC net) of 64.6%, which included a 39 day refueling outage in March / April.

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The reactor went critical in July 1967 and first contributed electricity to DPC's system in April 1968. After completing full power tests in August 1969, the plant has been operating between 60% and 100% full i

power, with the exception of plant shutdowns for maintenance and repair.

In accordance with LACBWR Technical Specifications 6.9.3.a. and in compliance with.10 CFR 50.36a(a)(2), this document is the Radioactive

. Efiluent Report for the period ' January 1 through June 30, 1985.

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TABLE OF CONTENTS SECTION TITLE PAGE(S)

Radioactive Effluent Report 1.0 Regulatory Limits 1 2.0 Maximum Permissible Concentration 2 3.0 Average Energy 2 4.0- Analytical Methods 2&3 5.0 Batch Releases 3&4 6.0' Abnormal Releases 4 7.0 Estimated Total Analytical Error 4 11 WP4.17 ,

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TABLES TABLE NO TITLE PAGE(S) 1A Effluent and Waste Disposal Gaseous Effluent Release Summaries 5 IB Gaseous Effluents - Elevated Release 6&7 2A Liquid Release Summary 8 2B Liquid Effluents 9 3 Solid Waste and Irradiated Fuel Shipments 10 & 11 111 WP4.17

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RADIOACTIVE EFFLUENT REPORT i

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EFFLUENT AND WASTE DISPOSAL REPORT (Supplemental Information)

FACILITY Lacrosse Boiling Water Reactor LICENSEE DAIRYLAND POWER COOPERATIVE DOCKET No. 50-409

1. REGULATORY LIMITS

a. Gaseous Effluent Release Limits:

LACBWR's Technical Specifications for gaseous effluent releses of radioactive material limit the release rates, of the sum of the individual readionuclides, in curies per seconds, so that the dose rates to members of the public beyond the Effluent Release Boundary (p. iv) do not exceed 500 mrem / year to the whole body, 3000 mrem / year to the skin from noble gases, and 1500 mrem / year to a critical or3an from 3H, 131/1331 and particulates with half-lives greater than 8 days.

Also, in accordance with 10CFR50, Appendix 1, the Technical Specifications for gaseous effluent radioactive material limit the air dose to a member of the public from noble gases in areas beyond the Ef fluent Release Boundary to less than 5 mrad gamma and 10 mrad beta per calendar quarter and less than 10 mrad gamma and 20 mrad beta per calendar year. The dose limits from 3H, 131/133g and particulates with half lives greater than 8 days are less than 7.5 mrem per calendar quarter and less than 15 mrem per calendar year to any organ.

Cumulative dose contributions from gaseous effluent releases are determined in accordance with the LACBWR Of fsite Dose Calculations Manual at least onch each 31 days.

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b. Liquid Effluent Release Limits:

LACBWR's Technical Specifications limits for liquid effluent releases are limited to those concentrations of individual radionuclides such that the diluted discharge does not exceed 1 MPC in a 168 hour0.00194 days <br />0.0467 hours <br />2.777778e-4 weeks <br />6.3924e-5 months <br /> week averaged over the calendar year. For dissolved or entrained noble gases, the concentration is limited to a total activity concentration of 2 x 10-4 uci/ml. For alpha emitting radionuclides, the concentration is limited to a total activity 1

concentration fo 4.9 x 10-9 pCi/ml, based upon an actual alpha emitting radionuclide analysis performed on a representative water sample. The values reported in tables 2A and 2B, Liquid Effluents, are based on dilution with the j

combination of LACBWR and Genoa #3 condenser cooling water flow prior to a discharge to the Mississippi River. No credit is taken for further dilution in j

the mixing zone of the Mississippi River.

Also, in accordance with 10CFR50, Appendix 1, the dose commitment to a member of the public from radioactive materials released in liquid effluents to j areas beyond the Effluent Release Boundary are limited to less than 1.5 mrem I

whole body and 5.0 mrem organ per calendar quarter, and less than 3.0 mrem

! whole body and 10 mrem organ per calendar year via the critical ingestion pathway.

t Cumulative quarterly and annual dose contributions from liquid effluent releases are determined for the adult fish ingestion pathway in accordance with the LACBWR Of fsite Dose Calculation Manual at lease once each 31 days.

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c. Solid Radioactive Waste All solid radioactive wastes are handled in accordance with a Process Control Program as defined by LACBWR procedures in order to assure that all applicable transportation and burial site disposal requirements are met.

2. MAXIMUM PERMISSIBLE CONCENTRATION (MPC)

The MPC used to calculate permissible release rates are obtained from 10 CFR 20, Appendix B, Tables I and II. In addition, the following values are used:

Tritium in Water = 3 x 10-3 Ci/ml.

Tritium in Air = 2 x 10-7 pCi/cc.

3. AVERACE ENERGY The release rate limits for LACBWR are not based on average energy.

4. ANALYTICAL METHODS (a) Liquid Effluents Liquid ef fluent measurements for gross radioactivity are performed by Ce-Li gamma isotopic analysis of a representative sample from each tank discharged.

A composite sample is created by collecting representative aliquots of each sample from each tank batch discharged, and is analyzed monthly for Tritium, and quarterly for Strontium 89 and 90. The radiostrontiums are analyzed by a contractor. In addition, each batch discharged tank is analyzed for alpha activity concentration.

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(b) 1.irborne Particulates Airborne particulate releases are determined by Ge-Li gamma 4.sotopic analysis. This analysis is performed by analyzing a glass fiber filter paper taken from the stack monitor (Eberline SPING) which continuously isokinetically samples and monitors the stack effluent. This filter is changed and analyzed on an approximate weekly basis and analyzed within 7 days after removal. This illter is also analyzed for alpha activity. A quarterly composite of these filters is sent to a contractor for Sr 89 and 90 analysis.

(c) Radioiodines Radioiodine releases are determined by Ge-Li gamma analysis of a TEDA impregnated activated charcoal cartridge taken from the stack monitor which continuously isokinetically samples and monitors the stack effluent. This charcoal cartridge is changed approximately weekly and analyzed within 48 hours5.555556e-4 days <br />0.0133 hours <br />7.936508e-5 weeks <br />1.8264e-5 months <br /> after removal.

(d) Fission and Activation Gases The gaseous releases converted into concentration (UCi/cc) are continuously sampled from the stack release flow by two stack monitors, which are inline monitors. These gas concentrations (pCi/cc) are averaged by the monitors microprocessor and flowrate/ pressure compensated to obtain the daily gaseous release of the planc. A monthly grab gas sample is taken from a stack monitor. This sample is collected in a 3.7 liter gas Marinelli and gamma analyzed on the Ge-Li detector to determine the isotopic composition of the gaseous release mixture and the gaseous concentration to verify the stack WP-4.17

monitors indicated gaseous concentration (uCi/cc). The Marinelli isotopic concentration fractions are then multiplied times the daily total gaseous releases to determine the individual gaseous isotopic release concentration.

i (e) Tritiun Tritium releases are determined by taking a grab sample of the stack atmosphere at the effluent of the stack monitor. Tritium as triciated water, i is removed from the sample stream by condensation, using a cold trap containing i an organic compound and dry ice. The condensed water vapor is then distilled and the distrillate is analyzed for 3H concentration, pCi/ce, by internal liquid scintilation spectrophotometry and the results are expressed in terms of tritium relese rates. The tritium grab samples are obtained on at least a once/ month basis unless the upper reactor cavity is flooded, at which time the sampling fcequency is increased to at least once per 7 days.

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5 BATCH RELEASES a,

(a) All airborne effluent releases at LACBWR are from a single 1

Continuous-Elevated Release Point.

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(b) Liquid -

All liquid effluent releases at LACBWR are batch releases.-

This is summarized as follows:

! (1) Number of Batch Releases: 92

(2) . Total Time Period for Batch Releases

573.2 hours2.314815e-5 days <br />5.555556e-4 hours <br />3.306878e-6 weeks <br />7.61e-7 months <br /> 4

(3) Maximum Time Period for a Batch Release: 15.38 hours4.398148e-4 days <br />0.0106 hours <br />6.283069e-5 weeks <br />1.4459e-5 months <br /> 1 (4) Average Time Period for Batch Releases: 6.30 hours3.472222e-4 days <br />0.00833 hours <br />4.960317e-5 weeks <br />1.1415e-5 months <br /> l (5) Minimus Time Period for a Batch Release 0.8 hours9.259259e-5 days <br />0.00222 hours <br />1.322751e-5 weeks <br />3.044e-6 months <br /> i

j (6) Average Stream Flow Rate During Periods of Release of Effluent into a Flowing Stream:- 57,713 ft /sec j 6. ABNORMAL RELEASES - There were no abnormal releases of radioactivity in plant effluents as summarized as follows:

l (a) Liquid i

) (1) Number of Releases: None (2) Total Activity Released: NA

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(b) Gaseous j (1) Number of Releases: None (2) Total Activity Released: NA l 7. ESTIMATED TOTAL ANALYTICAL ERROR i

The reported analytical results contain the following estimated errors

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i Counting Error j; l Standard Deviation 4

1 j Sampling Volume Error j; 5% >

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The lower limits of detection (LLD) are expressed. in terms of a 4.66 o as

] defined in Technical Specifications.

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TABLE 1A EFFLUENT AND WASTE DISPOSAL REPORT (1985)

CASEOUS EFFLUENTS - SUMMATION OF ALL RELEASES l l UNIT l QTR l QTR l QTR l QTR l TOTAL l A. FISSION & ACTIVATION GASES

1. TOTAL RELEASE C1 1.72E3 2.39E3 4.11E3

2. AVERAGE RELEASE RATE FOR PERIOD UCi/Sec 2.21E2 3.04E2

3. PERCENT OF TECHNICAL SPECIFICATION GAMMA DOSE LIMIT  % 2.21El 2.68E1 B. IODINE I-131

1. TOTAL 10 DINE-131 Ci 6.18E-4 8.61E-4 1.48E-3

2. AVERAGE RELEASE RATE FOR PERIOD I-131 uCi/Sec 7.84E-5 1.12E-4 C. PARTICULATES

1. PARTICULATES W/ HALF- l LIVES > 8 DAYS C1 2.73E-4 3.22E-4*

2. AVERAGE RELEASE RATE l FOR PERIOD pCi/Sec 3.46E-5 4.19E-5*

3. GROSS ALPHA RADIOACTIVITY C1 4.57E-6 2.19E-5 D. TRITIUM

1. TOTAL RELEASE C1 2.72E0 5.92E0 2.64E0

2. AVERAGE RELEASE RATE FOR PERIOD UC1/Sec 3.45E-1 7.53E-1 E. H-3, I-131/133 & PARTICULATES PERCENT OF TECHNICAL SPECIFICATION DOSE LIMIT  % 2.60E-1 1.49E0

• Values do not include Sr 89/90. Not available from contractor. Will be updated as soon as possible.

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TABLE IB EFFLUENT AND WASTE DISPOSAL SEMIANNUAL REPORT (1985)

CASEOUS EFFLUENTS - ELEVATED RFLEASE CONTINUOUS MODE lNUCLIDESRELEASED l UNIT l QTR l QTR l QTR l QTR l TOTAL l

1. FISSION GASES KRYPTON-85 CI KRYPTON-85M CI 6.92El 1.15E2 1.84E2 KRYPTON-87 CI _8.27El 1.09E2 1.92E2 KRYPTON-88 CI 1.95E2 2.82E2 4.77E2 XENON-133 CI 2.37E2 2.40E2 4.77E2 XENON-135 CI l.09E3 1.36E3 2.45E3 XENON-135M C1 2.31El 8.10El 1.04E2 XENON-138 C1 2.45El 6.49El 8.94El KR-89 CI

• 7.92E-2 XE-133M C1 3.00E-2 4.92E-2 XE-131M CI

• 3.83E2 3.83E2 XE-137 C1 2.48E0 1.44El 1.69El AR-41 CI

• 1.38El 1.38El CI CI TOTAL FOR PERIOD CI 1.72E3 2.66E3 4.38E3

2. 10 DINES 10 DINE-131 CI 6.18E-4 8.6LE-4 1.48E-3 IODINE-133 C1 3.71E-4 1.04E-3 1.41E-3 10 DINE-135 CI 1.48E-4 1.55E-4 3.03E-4 TOTAL FOR PERIOD CI 1.14E-3 2.06E-3 3.20E-3 l

3. SEE FOLLOWING PAGE FOR PARTICULATES.

• Indicates none detected or less than LLD WP4.17

TABLE IB - EFFLUENT AND WASTE DISPOSAL SEMIANNUAL REPORT (1985)

CASEOUS EFFLUENTS - ELEVATED RELEASE - (cont'd)

CONTINUOUS MODE l NUCLIDES RELEASED l UNIT l QTR l QTR l QTR l QTR l TOTAL l

3. PARTICULATES CI 7.17E-6 **

STRONTIUM-89 C1 * **

STRONTIUM-90 CESIUM-134 CI * *

• CESIUM-137 C1 2.37E-5 8.55E-6 3.23E-5 BARIUM-LANTHANUM-140 CL 1.81E-4 1.94E-4 3.75E-4 CO-57 C1 6.00E-8 2.00E-7 2.60E-7 CO-58 CI 1.00E-6 4.70E-6 5.70E-6 Co-60 C1 4.24E-5 6.48E-5 1.07E-4 CE-144 CI

• 6.80E-6 6.80E-6 CE-141 C1 2.42E-6 1.07E-6 3.49E-6 CR-51 CI 1.93E-6

• 1.93E-6 MN-54 C1 9.33E-6 2.15E-5 3.08E-5 FE-59 C1 ZN-65 CI

• 4.62E-6 4.62E-6 ZR-95 CI 1.77E-6 1.30E-6 3.07E-6 NB-95 C1 2.16E-6 3.14E-6 5.30E-6 RU-RH-106 CI

• 1.01E-5 1.01E-5 RU-103 C1 3.80E-7 9.30E-7 1 31E-6 C1 C1 CI CL CL

• Indicates none detected or less than LLD

• • Not availabic from contractor. Will be updated as soon as possible.

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TABLE 2A EFFLUENT AND WASTE DISPOSAL SEMIANNUAL REPORT (1985)

LIQUID EFFLUENTS - SUMMATION OF ALL RELEASES l UNIT l QTR l QTR l QTR l QTR l TOTAL l A. FISSION AND ACTIVATION PRODUCTS

1. TOTAL RELEASE (NOT INCL. l TRITIUM, CASES, ALPilA) C1 4.55E-1 6.34E-1*

2. AVERAGE DILUTED CONCEN- l l TRATION DURING PERIOD pCi/ml 3.82E-109.45E-9*

3. PERCENT OF MFC l LIMIT  % 5.19E-2 6.03E-2*

B. TRITIUM

1. TOTAL RELEASE C1 2.73E1 1.68E1 4.41El

2. AVERAGE DILUTED CONCEN-TRATION DURING PERIOD uCi/mi 4.56E-7 2.50E-7

3. PERCENT OF MPC l LIMIT  % 1.52E-2 8.33E-3 C. DISSOLVED AND ENTRAINED GASES

1. TOTAL RELEASE C1 2.29E-2 9.19E-3 3.21E-2

2. AVERAGE DILUTED CONCEN-l TRATION DURING PERIOD pCi/mi 3.82E-10 1.37E-10 i 3. PERCENT OF MPC l

LIMIT  % 1.27E-2 4.57E-2 D. GROSS ALPilA RADI0 ACTIVITY

1. TOTAL RELEASE Ci 3.02E-4 2.09E-3 2.39E-3 E. VOLUME OF WASTE RELEASED (PRIOR TO DILUTION) Liters 5.83E3 7.20E5 1.30E6 {

F. VOLUME OF DILUTION WATER USED DURING PERIOD Liters 6.00E10 6.71E10 1.27E11

• These values do not include Sr 89/90. The values were not available from contractor. Will be updated as soon as possible.

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TABLE 2B EFFLUENT AND WASTE DISPOSAL SEMIANNUAL R8 PORT (1985)

LIQUID EFFLUENTS NUCLIDES RELEASED UNIT QUARTER QUARTER QUARTER QUARTER CI 7.00E-4 **

STRONTIUM-89 C1 1.69E-3 **

STRONTIUM-90 CESIUM-134 C1 9.50E-4 1.66E-3 CESIUM-137 C1 2.39E-2 3.66E-2 10 DINE-131 C1 1.27E-2 4.54E-2 COBALT-58 CI 8.33E-3 7.80E-3 COBALT-60 C1 2.50E-1 3.71E-1 IRON-59 CI 1.64E-3 4.48E-3 ZINC-65 C1 3.32E-3 3.04E-3 j MANGANESE-54 C1 3.84E-2 4.67E-2  ;

f CI 6.71E-3 2.28E-3 CHROM 1UM-51 Z1RCONIUM-N10BIUM-95 CI 1.17E-3 1.73E-3 MOLYBDENUM-99 CI 4.99E-3 9.53E-4 TECHNETIUM-99M CI 1.57E-2 5.69E-3 i BARIUM-LANTHANbM-140 CI 2.11E-2 5.67E-3 CERIUM-141 C1 3.91E-4 4.67E-4 CE-144 CI 1.40E-3 6.34E-4 i CO-57 CI 4.42E-4 1.01E-4 1-133 C1 2.31E-2 1.31E-2

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1-135 C1 1.00E-2 4.51E-3 NP-239 CI 1.36E-2 7.13E-4 i

l RU-103 C1 9.65E-4 7.19E-2 l RU-RH-105 CI 2.4LE-3 1.20E-3

! RU-RH-106 CI 6.40E-4 3.04E-3 SR-91 C1 5.38E-3 1.52E-3 1l SR-92 C1 1.09E-3 5.5LE-4 1-132 C1 3.41E-4 2.21E-4 NA-24 CI 2.02E-4 1.29E-3 W-187 C1 1.99E-4

• AG-110M CI 2.79E-4 1.33E-3 i ZR-97 C1 2.73E-5 4.89E-5 CS-136 Cl 1.83E-4

• CL-38 C1 1.82E-5

• NB-97 CI 1.46E-3 3.24E-3 BA-139 CI 3.24E-5 0.60E-4 MN-56 CI 3.23E-5 5.10E-5 Y-92 CI 1.50E-3

• TOTAL FOR PERIOD ( ABOVE) CI 4.55E-1 6.34E-1 i

XF.NON-133 CI 7.78E-3 2.04E-3 l XENON-135 CI 1.10E-2 4.60E-3 XE-131M CI

• 1.10E-3 XE-133M C1 3.86E-5 1.46E-5 XE-135M C1 4.60E-3 1.32E-3 l 3.22E-6 1.82E-5 KR-85M C1 KR-87 CI 5.62E-5 1.07E-4 KR-88 CI 1.60E-5

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• Indicates none detected or less than LLD

• • Not available from contractor. Will be updated as soon as possible.

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TABLE 3 EFFLUENT AND WASTE DISPOSAL SEMIANNUAL REPORT (1985)

SOLID WASTE AND IRRADIATED FUEL SHIPMENTS A. SOLID WASTE SHIPPED OFFSITE FOR BURIAL OR DISPOSAL (NOT IRRADIATED FUEL) 6-MONTH 6-MONTH

1. TYPE OF WASTE UNIT PERIOD PERIOD TOTAL

a. SPEhT RESINS, FILTER SLUDGES, m' 9.63 9.63 EVAPORATOR BOTTOMS, ETC. Ci 1.76 E2 1.76 E2

b. DRY COMPRESSIBLE WASTE,CONTAMI- m3 -- --

NATED EQUIPMENT, ETC. C1 -- --

c. IRRADIATED COMPONENTS, CONTROL m' -- --

RODS, ETC. Ci -- --

d. OTHER (DESCRIBE) n' -- --

Ci - -

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Activity (C1)

2. ESTIMATE OF MAJOR NUCLIDE COMPOSITION 6-MONTH 6-MONTH (BY TYPE OF WASTE) PERCENT PERIOD PERIOD

a. Mn-54 7.10E0 1.25El Co-57 1.18E-2 2.07E-2 Co-60 4.71El 8.29El Zn-65 1.37E0 2.41E0 Cs-137 9.20E0 1.62E1 Ce/Pr-144 1.78E-L 3.14E-L H-3 5.14E-3 9.05E-3 C-14 1.22E-2 2.15E-2 Fe-55 2.64EL 4.65El Ni-59 5.63E-2 9.91E-2 Ni-63 4.81EO 8.46E0 Sr-90 3.87E-1 6.81E-1 Tc-99 5.91E-5 1.04E-4 U-235 7.95E-7 L.40E-6 U-238 6.70E-7 1.18E-6 Pu-238 7.50E-3 L.32E-2 Pu-239/240 4.20E-3 7.40E-3 Pu-241 3.36E-L 5.91E-1 An-24L 3.20E-3 5.63E-3 Co-242 1.70E-2 3.00E-2 Co-244/243 1.48E-3 2.6LE-3 Fe-59 9.83E-2 L.73E-1 Nb-95 2.31E-2 4.0tE-2 Ru-103 1.76E-2 3.09L-2 WP4.17

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TABLE 3 - (cont'd)

EFFLUENT AND WASTE DISPOSAL SEMIANNUAL REPORT (1985)

SOLID WASTE AND IRRADIATED FUEL SHIPMENTS

2. ESTIMATE OF MAJOR NUCLIDE COMPOSITION (BY TYPE OF WASTE)

ACTIVITY (CI) 6-MONTH 6-MONTH PERCENT PERIOD PERIOD Cs-134 5.68E-L 1.00E0 Ce-141 1.59E-2 2.80E-2 Sr-89 1.64E-1 2.88E-1 1-129 2.75E-3 4.84E-3 Co-58 1.66E0 2.93E0

3. SOLID WASTED DISPOSITION NO. OF SHIPMENTS MODE OF TRANSPORTATION DESTINATION 2 SOLE USE BARNWELL, SC B. IRRADIATED FUEL SHIPMENTS (DISPOSITION)

FO. OF SHIPMENTS MODE OF TRANSPORTATION DESTINATION NONE WP4.17

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D DA/RYLAND h [k COOPERATNE eo Boxsi7 2 sis EAST AV SOUTH = L A CROSSE W1SCONSIN 51601 (608) 788 4 000 August 30, 1985 In reply, please refer to LAC-Il065 P31011TY F~JII'@

$ r- l Mr. James G. Keppler, Regional Administrator U. S. Nuclear Regulatory Commission [ ~Q-y/ j{~,

Region III ~

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799 Roosevelt Road -)- } b -k;ii-~~ i Clen Ellyn, IL 60137 C

SUBJECT:

DAIRYLAND POWER COOPERATIVE LA CROSSE BOILING WATER REACTOR (LACPJJR)

PROVISIONAL OPERATING LICENSE NO. DPR-45 RADIOACTIVE EFFLUEfC REPORT FOR THE PERIOD JANUARY THROUGH JUNE 30, 1985

Dear Mr. Keppler:

In accordance with 10 CFR 50,36a(a)(2), this letter serves to transmit to you the Radioactive Effluent Report for the La Crosse Boiling Water Reactor i (LACBWR) for the period January I through June 30, 1985. j If you have any additional questions, please contact us.

Sincerely, t DAIRYLAND POWER COOPERATIVE

'f' j/?fW/  ;

James W. Taylor l General Manager FL LL4 dh Enclosures cc: Mr. Richard C. DeYoung (10 copies) #

Mr. Dennis M. Crutchfield (3 copies) j [ i NRC Resident Inspector (1 copy) f D. Sherman, ANI Library (l copy) 8 l l SEP 3 885 l WP4.17

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