ML20153D703
| ML20153D703 | |
| Person / Time | |
|---|---|
| Site: | Point Beach, La Crosse, 05000000 |
| Issue date: | 12/31/1987 |
| From: | WISCONSIN, STATE OF |
| To: | |
| Shared Package | |
| ML111711016 | List: |
| References | |
| CON-NRC-30-83-647 NUDOCS 8805090257 | |
| Download: ML20153D703 (43) | |
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STATF. OF WISCONSIN l
- 1987 La Crosse Boiling Water Reactor Environmental Radioactivity Survey NRC 30-83-647 I
l W15CONSN DMSCN OF H&M.TH f
- Wisconsin Daphrtment of Henith and Social Services Division of Health Bureau of Environsental Health Sectj.on of Radiation Protection P.O. Box 309 Madison Wisconsin 53701 I
i 8805090257 090429 PDR ADOCK 05000266 R DCD
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J Table of Contents s
t Page Number 1
Introduction l Sampling Techniques 1 c Analytical Procedures 2 ,
i j Quality Assurance 5 Sensitivities and Error -
Wisconsin 5 Sensitivities -
LACBWR 6 i Sample Collection Summary 7 I
i Results and Discussion 8 ;
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! References 14 i
Table 6 - Sample Summary for 1987. 15 ,
j Table 7 - Differences in Reported Wisconsin 17 j
and LACBWR results, i Table 8 -
EPA Cross Check Results 18 Lower Limit of Detection- LAC 8HR 24 i 4
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I List of Tables Table 1. WI DHSS sample collection summary for 1987. 7 Table 2. Missing sample report for 1987. 7 Table 3. Comparison of the yearly average for gross beta 8 i
activity from air particulate filters for 1987.
Table 4. Reported WI DHSS activities for cobalt-60 11 (Co-60) and cesium-137 (Cs-137) for bottom sedimente from the outfall site collected from 1985-1987.
Table $. Calculated doses to an average exposed 13 individual for WI DHSS samples with activities greater than MDC.
Table 6. Sample summary for 1987 from the environmental 15 split sample monitoring program conducted by WI DHSS and LACBWR.
Table 7. Disagreements in the comparison of WI DHSS 17 and LACBWR reported results from the environ-mental split monitoring program.
Table 8. EPA Cross Check results for 1986 & 1987. 18 Table 9. Air particulate (gross beta) and air iodine 26 (I-131) results for January - June, 1987.
Indicator site - Lock & Dam #8.
Table 10. Air particulate (gross beta) and air iodine 27 (I-131) results for J'ly - December, 1987.
Indicator site - Loci i Dam #8.
Table 11. Air particulate (gros beta) and air iodine 28 (I-131) results for January - June, 1987.
Control site - LaCrobse.
Table 12. Air particulate (gross beta) and air iodine 29 (I-131) results for July - December, 1987.
Control site - Lacrosse.
Table 13. Gamma isotopic results for January - December, 30 1987 from the monthly composite of air part-iculate samples. Indicator site - Lock & Dam #8.
Table 14. Gamma isotopic results for January - December, 31 1987 from the monthly composite of air part-iculate samples. Control site - Lacrosse.
Table 15. Analysis of surface water samples from January 32
- June, 1987. Indicator site - discharge channel. !
Table 16. Analysis of surface water samples from July - 33 December, 198T, Indicator site - discharge channel.
Table 17. Analysis of suvface water samples from January 34
- June, 1987. Control site - Lock & Dam #8.
. Table 18. Analysis of surface water samples from July - 35 December, 1987. Control site - Lock & Dam #8.
Table 19. Analysis of fish samples for 1987. 36 Table 20. Analysis of fish samples for 1987. 37 Table 21. Analysis of bottom sediments for 1987. 38 Table 22. Analysis of milk samples for 1987. 39 Table 23. Analysis of food products for 1987. 40
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STATE OF WISCONSIN l 1987 i
LA CROSSE BOILING WATER REACTOR l ENVIRONMENTAL RADIOACTIVITY SURVEY v
INTRODUCTION This report covering the calendar year 1987 is prepared under U.S.
Nuclear Regulatory Commission Contract NRC 30-03-647 by the State of Wisconsin, Department of Health and Social Services, Section of Radiation Protection. Results of environmental radioactivity monitoring are listed in tabular form. The data presented consists of duplicative split sample analysis conducted by the state radiation protection laboratary or subcontractor and the licensee. A brief description of sample collection techniques and analytical procedures conducted by the state laboratory is also given. A sample collection summary for 1987 is included in Table 6. The sample summary includes type and number of samples collected as well as the range of reported actisities for each type of sample analysis.
The La Crosse Boiling Water Reactor ceased operation on April 30, 1987 and has applied to the Nuclear Regulatory Commission for a possession-only license under 10 CFR Part 50. The etnvi ronmen t al monitoring programs conducted by the La Crosse Boiling Water Reactor and State of Wisconsin, Department of Health and Social Services, Section of Radiation Protection have remained the same during this reporting time period of January 1 through December 31, 1987.
SAMPLING TECHNIQUES Whenever possible a split sample is taken inorder to obtain a valid comparison between WI DHSS and LACBWR results. Split sampling involves the thorough mixing of a sample into a homogeneous mixture that is than split between WI DHSS and LACBWR.
Direct Radiation Thermoluminescent Dosimeters (TLD's)
Continuous monitoring of direct radiation is performed quarterly using l thermoluminescent dosimeters. The dosimeters are placed at 29 '
locations in the area of the La Crosse Boiling Water Reactor (LACBWR) nuclear power plant.
Air S_amples ,
l Continuous air samples are collected weekly from two stations. Air i particulate samples are collected on 47 mm. glass fiber filters. Air l
. iodine samples are collected using charcoal absorbers mounted downstream of the air particulate filters. The nominal sampling rate is 1-2.5 cubic feet of air per minute depending on the air pump used.
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Surface Water A split sample is collected monthly at a point close to the dischargo of the LACBWR eff1'uent channel, 0.1 mile W. This sample is a grab comple and is collected while the plant is discharging wastewater to the channel. A background surface water sample is also collected -
monthly from Lock and Dam #8, 0.7 mile N.
3 Milk A raw, split milk sample le collected monthly from one of three local farms located in the Genoa, Wisconsin area.
Sediment Sediment is collected from three locations in the Mississippi River channel on an annual basis.
Fish Game and scavenger fish are collected periodically from locations in the Mississippi River near the LACBWR nuclear power plant.
Food Products A blended sample of mixed vegetables is collected from local gardens.
ANALYTIC?t PROCEDURES The procedur given are condensed to present only the basic method.
The analysf of the samples has been subcontracted to the State Laboratory or Hygiene. A detailed description of the procedures used ,
is available from the State Laboratory of Hygiene.
l Air Particulate _ Samples - Beta Gamma Place the 47 mm. glass fiber filter on a 2-inch stainless steel planchet. Beta count in an external gas flow proportional counter.
Calculate activity correcting for counter efficiency. j Air Particulate Samples - Gamma The quarterly composite of air particulate filters is placed on a Ga(Li) detector and the gamma spectrum is collected. Scan the gamma spectrum for any peaks and print out regions of interest which would include possible plant attributable radionuclides. Calculate the activity for isotopes in the regions of interest, regardless if they are above or below the minimum detectable concentration, correcting for counter efficiency and for decay. .
Surface Water - Alpha, Beta Gamma Filter a 500 ml. aliquot of sample. Evaporate filtrate in a 2-inch 2
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stainless steel planchet. Place filter paper in a 2-inch stainless l steel planchet and dry at 103 degrees Celsius. Beta and alpha count the soluble and insoluble portions .i n an external gas flow proportional counter. Calculate activity correcting for counter effjciency and self-absorption.
5 Surface Water - Gamma Isotopic 9
. A 3.5 liter sample is placed in a Marinelli beaker and analyzed on a GeLi detector. Scan the gamma spectrwa for any peaks and print out regions of interest which would include possible plant attributable radionuclides. Calculate the activity for isotopes in the regions of interest, regardless if they are above or below the minimum detectable concentration, correcting for counter efficiency and for decay.
Surface Water - Iodine 131 Chemical Extraction A stable iodine carrier is added to a 2 liter sample of raw milk. The sample is passed through an anion exchange column and the iodine is removed from the resin by batch / extraction using Na001. After reduction to elemental iodine by hydroxylamine hydrochloride, the iodine is extracted into carbon tetrachloride reduced with bisulfite, and back extracted into water. The iodine is precipitated as palladous lodide with the chemical yield determined gravimetrically and counted in an external gas flow proportional counter. Calculate activity correcting for counter efficiency and for decay.
Surface Water - Strontium 89 and Strontium 90 Strontium and yttrium carriers are added to the surface water samples.
The procedure follows through a series of chemical separations whereby all in erfering substances are removed. Calcium is removed by precipitating strontium and barium by nitrate precipitation thereby leaving the calcium in solution. Radium is removed by co-precipitation with barium as a chromate. The ingrowing yttrium is separated from the parent strontium through the use of hydroxide scavenging. The purified strontium is converted to a carbonate and beta counted in an external gas flow proportional counter. After two weeks ingrowth yttrium-90 is separated from the strontium carbonate via a series of hydroxide precipitations and finally converted :o an oxalate and beta counted in an external gas flow proportional counter.
The strontium-90 activity is calculated from the yttrium-90 count and the strontium-89 activity is calculated using the previous calculation for strontium-90 as well as the total strontium activity from the strontium carbonate counting.
Vegetation o_r Food Product - Alpha, Beta and Gamma Isotopic Dry sample at 110 degrees Celsius, grind and weigh into a stainless steel planchet. Beta and alpha count in an external gas flow
. proportional counter. Calculate activity correcting for self-absorption and counter efficiency.
The food product sample is finely chopped. The sample is packed to the 500 mi mark of a 500 ml Marinelli beaker, weighed and counted on a 3
Ge(L1) detector. Scan the gamma spectrum for any peaks and print out regions of interest which would include possible plant attributable radionuclides. Calculate the activity for isotopes in the regions of interest, regardless if they are above or below the minimum detectable concentration, correcting for counter efficiency and for decay, a
Soil or Sediment -Alpha, Beta and Gamma Isotopic Dry sample at 110 degrees' Celsius, grind and weigh into a stainless -
steel planchet. Beta and alpha count in an external gas flow proportional counter. Calculate activity correcting for self-absorption and counter etficiency.
The dried soil is added to a 500 m1 Marinelli beaker, weighed and counted on a Ge(Li) detector. Scan the gamma spectrum for any peaks and print out regions of interest which would include possible plant attributable radionuclides. Calculate the activity for isotopes in the regions of interest, regardless if they are above or below the minimum detectable concentration, correcting for counter efficiency and for decay.
Milk - Gamma Isotopic Procedure same as for Surface Water.
Milk - Iodine 131 Chemical Extraction Procedure same as for Surface Water.
Milk - Strontium 90 Strontium and yttrium carriers are added to milk which has been aged two to four weeks. A one liter sample is passed successively through cation and anion exchange columns. The yttrium is eluted from the anion resin with hydrochloric acid, precipitated as yttrium oxalate, !
filtered and weighed to determine chemical yield. Beta count in an external gas flow proportional counter. Calculate the activity correcting for counter efficiency and for decay.
Fish - Gamma Isotopic An edible portion is placed in a 500 ml. Marinelli beaker. Place the sample on a GeLi detector and collect the gamma spectrum. Scan the i gamma spectrum for any peaks and print out regions of interest which would include possible plant attributable radionuclides. Calculate the activity for isotopes in the regions of interest, regardless if they are above or below the minimum detectable concentration, correcting for counter efficiency and for decay.
Direct Radiation Thermoluminescent dosimeters are supplied by the U.S. Nuclear Regulatory Commission. The err <osed TLD's are shipped to NRC Region I and are read by the Commission.
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QUALITY ASSURANCE The analysis of the samples is performed under subcontract with the State Laboratory of Hygiene (SLH). SLH maintains its own quality assurance program which was also reviewed by the NRC in January, 1985.
. Analytical procedures provide for routine replicate analyses to verify methods and instrument operation. Traceable sources are used to l regularly calibrate the counters and daily performance checks are made between calibrations. In addition, quality centrol charts are maintained on the counters.
SLH participates in the EPA Cross Check program. The quality assurance program that the SLH participates in include analysis of blind samples, air filters, food, milk, gamma in water, alpha-beta in water, iodine in water, strontium in water and tritium in water. The EPA Cross Check code for SLH is "AF". A complete listing of the EPA Cross Check results for 1986 and 1987 is included in Table 8.
SENSITIVITIES AND ERROR -
WISCONSIN DHSS Following the recommendations of the Health Physics Society, detection limits will be expressed as a minimum detectable concentration (MDC).
The minimum detectable concentration or MDC is an "a priori" estimate of the capability for detecting an activity concentration by a given measurement system, procedure, and type of sample. The MDC should not be viewed as an absolute activity concentration that can or cannot be detected. Minimum detectable concentrations (MDC) are based on the analysis performed and for gamma isotopic analysis have been calculated for a zero decay time. A listing of the WI DHSS MDC values is included in Table 6.
The WI DHSS definition for minimum detectable concentration follows closely the equation for the lower limits of detection as defined in the NRC contract NRC-30-83-647. Activities defined by the equation for MDC will be used in this report.
The MDC for each radioisotope has been calculated from the following equation:
4.66 sb MDC =
'E
- V
- 2.22
- y
- S
- exp(-dt)
Where:
MDC is the "a priori" lower limit of detection as defined above, as picoeuries per unit mass or volume, 5
sb is the standard deviation of the background counting rate or of the counting rate of a blank sample as appropriate, as counts per minute, E is the counting efficiency, as counts per disintegration, V is the sample size in units of mass or volume, ,
2.22 is the number of disintegrations per minute per picoeurie, Y is the fractional radiochemical yield, .when applicable, S is the self-absorption correction factor, d is the radioactive decay constant for the i particular radionuclide, and i t for environmental samples is the elapsed time between sample collection, or end of the sample collection period, and time of counting, )
i Guidelines adopted by the U.S. Environmental Protection Agency are '
used in the reporting of specific analyses. Results from specific l analyses will be reported whether the results are negative, zero, or positive. Caution should be exercised in the interpretation of individual negative values. While a negative activity value does not have physical significance, it is significant when taken together with other observations which indicate that the true value of a distribution is near zero. This procedure will allow all of the data to be reported and will allow a statistical evaluation without an arbitrary cutoff of small or negative numbers. An estimation of bias in the nuclide analyses as well as a better evaluation of distributions and trends in the environmental data is then possible.
It is important when reviewing the data in the following tables to compare the reported result to the actual minimum detectable concentration (MDC) for that analysis.
Results for specific analyses will be reported as an activity followed by an error term for that analysis. The error term is a plus or minus counting error term at the 2 sigma (95%) confidence interval and is printed as (+/-).
SENSITIVITIES -
LACOWR Lower limits of detection (LLD) or minimum detectable activity (MDA) '
as reported by LACBWR are defined in their manual LACBWR, HEALTH &
SAFETY DEPARTMENT PROCEDURE, LACBWR ENVIRONMENTAL MONITORING PROGRAM.
The method for calculating the LLD and a representative table of LLD's -
for LACBWR is included in this report. In most cases, reported activities for LACBWR are less than the required Nuclear Regulatory Commission LLD's.
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SAMPLE COLLECTION
SUMMARY
The following types and number.of samples were collected for WI DHSS and are listed in Table 1. An explanation for missing samples is 4 listed in Table 2.
Table 1. WI DHSS sample collection summary for 1987.
Sample Type Collection Number of Number of Number of and Locations Samples Samples Frequency
- Collected Missed ,
air particulate C/W 2 104 1 surface water G/M 2 24 0 sediment G/A 3 3 0 fish G/SA 1 8 0 food product G/A 2 2 0 milk G/M 3 12 0
- Collection type: C/ - continuous; G/ = grab Frequency: /W = weekly; /W = monthly; /Q = quarterly; /A = annually
/BW = bi-weekl); /SA = semi-annually Table 2. Missing sample report for 1987.
3- Sample type Date Location Explanation Air particulate 12/07/87-12/14/87 Lacrosse Pump was not operat'ng.
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l RESULTS AND DISCUSSION A sample collection summary for 1987 is included in Table 6. The '
sample summary includes the type and number of samples collected as ,
well as the range of reported activities for each type of sample
- analysis. Disagreements in the comparison of WI DHSS and LACBWR reported results from the environmental split sample monitoring program are listed in Table 7. Results from the individual sample analyses are listed in Tables 9-23.
Air Particulate WI DHSS and LACBWR maintain separate air sampling stations. The indicator site for both WI DHSS and LACBWR is located at Lock & Dam
- 8, 0.7 miles N. The control site for WI DHSS is located at the state office building in La Crosse, 16 miles N and for LACBWR at the Dairyland Power office in La Crosse.
A summary of reported activities by WI DHSS and LACBWR from the air particulate samples is included in Table 6. Results from the individual sample analyses are listed in Tables 9-12.
The yearly averages, from a log-normal distribution, for the gross beta analysis on the air particulate filters are given in Table 3.
The WI DHSS and LACBWR yearly averages for gross beta activity from the air particulate filters are comparable and showed no significant differences between their respective indicator and control sites.
A summary of reported gamma isotopic activities for WI DHSS and LACBWR from the monthly or quarterly air particulate filter composites is included in Table 6. Results from the individual sample analyses are listed in Tables 13-14.
Table 3. Comparison of the yearly average for gross beta activity from air ,
particulate filters for 1987. '
WI - Section of Radiation LACBWR l Protection 1 3
units of pC1/M l
1 Indicator Control Indicator Control l 0.016 + 0.002 0.014 + 0.002 0.023 1 0.002 0.022 1 0.002 8
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In the WI DHSS gamma isotopic analysis bery111um-7 (Be-7) was detected in all composites from both the indicator and control sites.
Bery111um-7 (Be-7) is a naturally occurring radioisotope that is constantly produced through nuclear reactions between cosmic rays and 4
nuclei in the atmosphere. All other radionuclides were below their respective MDC for the 1st, 2nd. 3rd and 4th quarter composites.
, LACBWR does not report naturally occurring radioisotopes and no comparison can be made-for the bery111um-7 (Be-7) reported by WI DHSS.
All of the reported radioisotopes by LACBWR for the monthly composites were at trace activity levels and all were less than the respective WI DHSS MDC.
At the observed lower levels of activity, the WI DHSS and LACBWR data are comparable in the gross beta and gamma isotopic analysis on the air particulate samples. Influence by the LACBWR nuclear facility on air quality is not evident when comparing the data from the indicator and control sites.
Air Iodine Air iodine samples are taken at the same sites as the air particulate camples.
A summary of reported air iodine activities for WI DHSS and LACBWR is included in Table 6. Results from the individual sample analyses are listed in Tables 9-12.
All reported WI DHSS and LACBWg air iodine measurements were below the required NRC LLD of 0.07 pC1/M for both the indicator and the control sites.
Surface Water The surface water samples are split samples taken as a grab sample on a monthly basis. The discharge channel is taken as the indicator site and Lock and Dam #8 is taken as the control site.
A summary of reported activities by WI DHSS and LACBWR from the monthly surface water samples is included in Table E. Disagreements in the reported WI DHSS and LACBWR results are listed in Table 7.
Results from the individual sample analyses are listed in Tables 15-18.
The WI DHSS and LACBWR reported activities from the monthly surface water samples taken at the control station, Lock & Dam #8, are all at background levels. All reported activities by WI DHSS and LACBWR for gamma isotopic and tritium analyses were less than the respective WI DHSS minimum detectable concentration (MDC) or LACBWR minimum detectable activity (MDA).
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Analysis of the surface water samples taken from the indicator site, discharge channel, by WI DHSS detected small activities of cobalt-60 (Co-60), manganese-54 (Mn-54), cesium-137 (Cs-137), s11ver-110 (Ag-110) and tritium (H-3). LACBWR analysis detected small activities of !
manganese-54 (Mn-54), cobalt-60 (Co-60), cesium-137 (Cs-137),
ruthenium-103 (Ru-103), cerium-141 (Ce-141) and tritium (H-3).
were comparable except for the disagreements listed in Table 7. The
- WI DHSS and LACBWR sample analysis reports were reviewed for possible problems in the sample analysis but no problems were noted.
All activities reported by either WI DHSS or LACBWR are below the standards for uncontrolled areas as specified in ICRP Report No.2 or 10 CFR 20.
Fish Both LACBWR and WI DHSS analyze the same samples with LACBWR first performing its analysis and then WI DHSS.
A summary of reported activities by WI DHSS and LACBWR from fish samples is included in Table 6. Results from the individual sample analyses are listed in Tables 19-20.
From the WI DHSS gamma isotopic analysis only naturally occurring potassium-40 (K-40) was detected in all samples.
LACBWR does not report naturally occurring radioisotopes. The reported LACBWR activities for zine-65 (Zn-65) and cobalt-60 (Co-63) were all less than the respective WI DHSS MDC.
At the low level of reported activities the WI DHSS and LACBWR data are comparable.
Bo_ttom Sediments Both WI DHSS and LACBWR analyze the same samples with LACBWR first performing its analysis and then WI DHSS.
A summary of reported activities by WI DHSS and LACBWR from bottom sediment samples is included in Table 6. Results from the individual sample analyses are listed in Table 21.
The gamma isotopic analysis of the upstream sample, Lock & Dam #8, by WI DHSS detected only naturally occurring potassium-40 (K-40) and naturally occurring radioisotopes from uranium and thorium decay series. Analysis by LACBWR detected only trace activities of cesium-137 (Cs-137). All reported activities by WI DHSS or LACBWR for the upstream site were less than the required NRC LLD's.
The highest act!-rities for both WI DHSS and LACBWR Were detected at the discharge point wi th' cobalt-60 (Co-60) and cesium-137 (Cs-137) 10
predominating and smaller detected activities for cesium-134 (Cs-134) zinc-65 (2n-65) and manganese-54 (Mn-54). Reported WI DHSS data from the discharge point for 1985-1987 for cobalt-60 (Co-60) and cesium-137 (Cs-137) is listed in Table 4. The discharge point is not necessarily the best site to observe trends of accumulated radioactivity versus time. From correspondence with Dairyland Poaor Cooperative environmental department personnel, their observations are e that the discharge point has a very small area to colle'et bottom
, sediment with larger aggregate predominating and that it also has a high scouring rate. The discharge site, however, is probably the only point available in the immediate area due to the large amount of riprap in the area.
From the downstream site, boat launch, WI DHSS detected activities above MDC values for naturally occurring potassium-40 (K-40) and naturally occurring radioisotopes from uranium and thorium decay series. LACBWR reported small activitfes for manganese-54 (Mn-54)and cesium-137 (Cs-137) which are less than the respective WI DHSS MDC nr NRC LLD.
The reported activities by WI DHSS and LACBWR are comparable for all three sites.
Milk The milk samples are obtained as grab samples on a monthly basis and are then split for analysis.
A summary of reported activities by WI DHSS and LACBWR from milk samples is included in Table 6. Results from the individual sample analyses are listed in Table 22.
WI DHSS detected naturally occurring potassium-40 (K-40) in all samples and cesium-137 (Cs-137) in one sample in its gamma isotopic analysis of the milk samples. All activities for iodine-131 were below its MDC of 0.40 pCi/1.
l Table 4. Reported WI DHSS activities for cobalt-60 (Co-60) and cesium-137 (Cs-137) for bottom sediments from the outfall site collected from 1985 - 1987.
Collection Co-60 Cs-137 (pC1/kg dry) 06/05/85 620 1 50 120 1 30 10/16/85 8620 2 170 17600 1 200 06/30/86 4390 1 120 3400 1 90 09/23/86 3360 2 100 2140 2 70 08/06/87 3390 1 110 2940 1 90 11
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l LACBWR reported activities for cesium-137 (Cs-137) in four samples. l All other radionuclides were below the respective LACBWR MDA. LACBWR does not report naturally occurring radioisotopes and a comparison is .
not possible with the WI DHSS data. I l
At the low level of reported activities the WI DHSS and LACBWR data ,
are comparable.
4 The reported data by WI DHSS for 1987 is comparable to data reported
- for previous years. Influence by the LACBWR facility in the milk pathway is not apparent from the milk sa.nples analyzed by either WI DHSS or LACBWR.
Vecetation - Food Products A split sample of food products was taken from two local farms. A blended sample of mixed vegetables was collected from each farm.
A summary of reported activities by WI DHSS and LACBWR from the food product sample is included in Table 6. Results from the individual sample analyses are listed in Table 23. ,
i WI DHSS detected only naturally occurring potassium-40 (K-40) above its MDC in its gamma isotopic analysis of the food product sample.
Activities for iodine-131 (I-131) were below its MDC of 60 pCi/kg.
LACBWR does not report naturally occurring radioisotopes and no other radioisotopes were reported above the respective LACBWR MDA.
The WI DHSS and LACBWR results are comparable and influence by the LACBWR facility is not evident in food product samples, i
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Dose to an Average Individual Dose calculations for gaseous and 11guld effluent releases were performed according to the mathematical models illustrated in USNRC g Regulatory Guide 1.109, "Calculation of Annual Doses to Man from Routine Releases of Reactor Effluents for the Purpose of Evaluating e Compliance with 10 CFR Part 50, Appendix I". The doses, listed in
, Table 5, were calculated for the average exposed individual for WI DHSS samples with activities greater than MDC.
The dose to an average individual from exposure to bottom sediments (discharge channel) are due specifically to the detected gamma activities of cobalt-60 (Co-60) and cesium-137 (Cs-137). The outfall site, however, is not readily accessibly for individual use for recreational purposes including either fishing or swimming.
Doses resulting from gaseous and liquid effluent releases from the LACBWR nuclear facility are in compliance with 10 CFR Part 50, Appendix I.
The dose to an average individual from the ingestion of milk are most likely due to background levels of radiation attributable to fallout from previous atmospheric nuclear tests and not to the operation of the LACBWR facility. The dose to an average individual from the ingestion of milk are due specifically to the detected strontium-90 (Sr-90) activities.
The doses listed in Table 5 are well below the state and federal standards of 500 mrem / year.
Table 5. Calculated doses to an average exposed individual for WI DHSS samples with activities greater than MDC.
Average Exposed Individual (arem/ year)
Sample whole type Description population body bone thyroid allk yearly average infant 2,8 11.0 ---
child 2.6 10.1 ---
teenager 1.4 5.8 ---
adult 0.7 2.9 ---
bottom 08/06/87 outfall infant ---
sediment child 0.032 teenager 0.136 adult 0.024 13
R e f e r' e n e e s i
La Crosse Boiling Water Reactor, LACBWR, Health & Safety Department Procedure, LACBWR Environmental Monitoring Program, HSP-03.4, Issue 5, ,
pages 29,30. ,
Radiation Protection Standards, Federal Radiation Council, Report No.
2, September 1961.
[
U.S. Environmental Protection Agency, Upgrading Environmental l Radiation Data, Health Physics Society Committee Report HPSR-1 (1980),
EPA 520/1-80-012, August 1980.
U.S. Nuclear Regulatory Commission, Title 10, Part 20.
Wisconsin Department of Health and Social Services, Division of Health, Section of Radiation Protection. NRC 30-83-647, 1985 Annual Report, La Crosse Boiling Water Reactor. ;
Wisconsin Department of Health and Social Services, Division of Health, Section of Radiation Protection. !!RC 30-83-647, 1986 Annual Report, La Crosse Boiling Water Reactct, j i
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Table 6. Sample su mary fea 1987 free the environtental split sample monitoring progran conducted by W! 04S5 and LACSWR.
e Misconsin data LAC 8WRdata
' Sarple type l Number of l NRC Number of l MX Sarples 'a Analysis range l LLD Samples *a Analysis range
. (units) 0.003 104/102 gross beta 0.000 - 0.045 l.0.01 104/104 gress beta 0.009'- 0.041 air partjeulate (pCi/M) 8 gatea isetepic l 24 ga na isotopic 0.025 8/8 Be-7' O.06 - 0.14 l Be-7 *c 0.007 8/0 Ir-95 -0.002 - 0.001 l ---- 24/0 Zr,hb-95 <MDA *b 0.004 Ru-103 -0.001 - 0.001 l ----
24/0 Ru-103 <MDA *b 8/0 0.016 8/0 Ru-106 -0.001 - 0.004 l ----
24/0 Ru-106 (OA *b 0.002 8/0 Cs-134 -0.001-0.000.] 0.05 24/0 Cs-134 (M]A *b 0.002 8/0 Cs-137 -0.001 - 0.001 l 0.06 24/2 Cs-137 <C A *b - 0.010 0.005 8/0 Ce-141 -0.001 - 0.001 l ---- 24/1 Ce-141 < M4 *b - 0.0008 0.009 8/0 Ce-144 -0.001 - 0.001 1 ---- 24/0 Ce-144 (MDA *b 0.003 8/0 Co-60 <MX l 24/6 Co-60 <MDA *b - 0.003 0.003 8/0 Mn 54 (MX l 24/1 Mn-54 ( OA *b - 0.003 0.17 8/0 1-131 <MX l 0.07 24/0 1-131 (MDA *b 0.003 8/0 C0-57 <MX l ---- 24/1 Co-57 (NA *b - 0.0005 0.02 8/0 Cr-51 <OC 1 --- ' 24/1 Cr-51 (EA *b - 0.017 air iedi:e 0.045 104/0 I-131 -0.03 - 0.03 l 0.07. 104/0 1-131 <0.0012 - <0.0037 (pCi/M')
surface ster 1.6 24/24 gress beta 3.6 - 108 l 4 24/23 gross beta <1.1 - 70.6 (pC1/litea) 750 24/4 H-3 -250 - 8300 l 2000 24/4 H-3 (1287 - 9152 5.0 24/0 Sr-19 -0.9 - 0.9 { Sr-89 *c 1.2 24/2 Sr-90 0.0 - 1.4 l Sr-90 *c 24 gaes iseteef: l 24 gassa isetepic 9 24/3 Mn-54 32 l 15 24/4 Mn-54 < NA *b - 45 20 24/0 Fe-59 8 l 30 24/0 Fe-59 <MDA *b 13 24/0 Co-58 2 l 15 24/0 Co-58 (OA *b 11 24/3 Co 60 124 l' 15 24/3 Co-60 ( OA 8b - 119 22 24/0 Zn-65 18 1 30 24/0 Zn-65 <MDA *b 0.4 24/0 1-131 -0.2 - 0.2 l 1 24/0 1-131 <CA*b 13 24/0 Cs-134 9 l 15 24/0 Cs 134 (MA*b 12 24/3 Cs-137 34 l 18 24/3 Cs-137 (MA *b - 39 15 24/1 Zr-95 16 l 15 24/0 Zr-95 <MOA *b 15 24/0 La-140 5 l 15 24/0 Ba,La-140 <CA *b 12 24/1 A;-110 <MX - 14 l Ag 110 <CA *b fish 8 game isetecic l 8 games isctopic (pCi/kgwet) 550 8/8 K-40 2300 - 4600 l 8 K-l* *c i 40 8/0 M.n-54 2 l '130 8/0 Mn-54 (MA *b l 60 Fe-59 (MA *b l 120 8/0 Fe 59 l 260 8/0 54 8/0 Co-58 0 l 130 8/0 Co-58 <CA *b 50 8/0 Co-60 40 l 130 8/2 Co-60 <C A *b - 27 110 t/0 In-65 70 l 260 8/1 In-65 ( M A *b - 34 45 8/0 Cs-134 70 l 130 8/0 Cs-134 (CA *b 55 8/0 Cs-137 20 l 150 8/0 Cs 137 (NA *b 1 I
15
M l i
4 l
l Table 6. (continued)
Misconsin data LACfnRdata I
Saeple' type l Nueber of - l NRC Nutber of (units) l MDC Saeoles *a Analysis range l LLO Samples 'a Analysis range ,
bottom sediments $100 3/3 gross beta 9000 - 23000 l gross beta 'c (pCi/kgdry) .
3 gamma isote;ic l 3 gamma isetopic 60 3/1~ Mn-54 13 - 190- l ----. 3/3 Mn-54 26 - 166
' 10 3/0 ,Co 58' 8 - 50 , l -- -
3/0 Co-58 (MDA,8b 90 ' 3/1 -Co-60 17 - 3390 l - ,-- 3/1 Co-60 . <MDA *b - 3470 160 3/0 In-65 (MDC l 3/1 In-65 (EA *b - 59 60 3/0 Cs-134 18 - 40 l 150 3/1 Cs-134 (CA *b - 78. l 80 .3/2 C -137 50 - 2940 l 180 3/3 Cs-137 (O A *b - 3040
*c 450 3/3 . K 40 1500 - 16100 l K-40 100 3/3 Ra-226 210 - 500 l Ra-226 *c ;
150 3/3 Pb-214 180 - 410 l Pb-214 *e 1 150 3/3 81-214 240 - 500 l 81-214 *c
)
190 - 490 180 3/3 T1-208 l T1-208 *c I
110 3/2 At-228 160 - 450 l Ac-208 *e milk '2 ge-n isotecte i 12 g m a isotonic ;
(pCi/l) 200 12/12 K 40 1130 - 1610 1 12 K-40 8e O.4 12/0 1-131 -0.2 - 0.4 l 5, 12/0 1-131 (E A
- b 12 12/0 Cs-134 0-9 l 15 12/0 Cs-134 (CA *b j 12 12/1 Cs-137 18 l 18 12/4 Cs-137 (CA *b - 27 j 15 12/0 La-140 2 l 15 12/0 La 140 <MA*b ;
food croducts 2000 2/1 gress beta 700 - 3100 l 2 gross beta *c l (pC1/kg wet) 2 garaa isetc;ic l 2 gaera isctopic 300 2/0 Be-1__ -20~-(-5) l 2 _8e-7 *c 600 2/2 k-40 2100'- 2420 l 2/1 K-40 *e 50 2/0 Co 58 9 l 2/0 Co-fi (MA *b 55 2/0 Co-60 2 l 2/0 Co-60 <@A*b 80 2/0 Ir-95 (-5) 1 2/0 Zr-95 <MDA *b 60 2/0 1-131 4 l 60 2/0 1-131 <CA *b
$0 2/0 Cs 134 (-3) l 60 2/0 Cs-134 <OA *b 60 2/0 Cs-137 10 1 80 2/1 Cs-131- <CA*b l
- a - Naber cf sapples / nuaW of analyses detected above OC ce LLO. ,
- b - In rest cases, reported activities for LA08aR are less than the recaired NRC LLD's.
- c - Analysis not required.
l i
I 4 16
I 4
Table 7. Disa;reennts in the cercarisco of Wis:ensin and '.ACENR reported results from the ewironmental split sample monitorir.g pregram fer 1996.
Type Collection Description Wisconsin LACenR e surface water 03/10/97 discharge channel (H-3) 69001400 5212 i surfa:e water 05/12/87., dischargechannel (4-3) . 140f310 2076 surface water- 09/09/87 dis:hargechannel igressbeta) 22f2 6.2f1.0 surface water '10/13/87. dis:harge channel (gressbeta) 10825 59.812.4 surfa:ewater 10/13/87 discharge chaa.rel (H-3) 5700f300 2043
+
surface water 11/10/87 discharge channel (gressbeta) 106f5 10.622.6 surfa:e water 12/09/87 discharge chanre' (geessbeta) 85f5 46.712.2 surface water 12/08/87 discharge channel (Co-60) 70f15 26.6ft0.6 17
Table 8. U.S. Environmental Protection Agency's crosscheck program, comparison of EPA and State Laboratory of Hygiene (SLH) results.
Concentration in pCi/ sample *a Sample Date Analysis SLH result EPA result Deviation Type Collected +/- 1 sigma +/- 1 sigma Known Water 01-10-86 Sr-89 32.0+/-1.2 31.0+/-5.0 0.3 Sr-90 13.3+/-0.7 15.0+/-1.5 -1.9 Water 01-24-86 Alpha 4.0+/-1.4 3.0+/-5.0 0.3 Beta 7.3+/-1.4 7.0+/-5.0 0.1 Food 01-31-86 Sr-89 No data provided 25.0+/-5.0 Sr-90 No data provided 10.0+/-1.5 I-131 19+/-9 20.0+/-6.0 -0.2 Cs-137 18+/-8 15.0+/-5.0 0.9 K 1030+/-170 950+/-143 1.0 Water 02-07-86 Cr-51 LT 40 38.0+/-5.0 Co-60 17+/-3 18.0+/-5.0 -0.2 Zn-65 38+/-6 40.0+/-5.0 -0.6 q Ru-106 LT 31 0.0+/-5.0 Cs-134 28+/-3 30.0+/-5.0 -0.6 Cs-137 23+/-3 22.0+/-5.0 0.5 l 1
Water 02-14-86 H-3 4913+/-370 5227+/-523 -1.C l Water 02-21-86 U (nat) 10+/-5 9.0+/-6.0 0.4 Water 02-28-86 I-131 9. 04 /--1. 0 9.0+/-6.0 0.0 Water 03-14-86 Ra-226 3.9+/-0.5 4.1+/-0.6 -0.7 Ra-228 11.9+/~1.8 12.4+/-1.9 -0.4 i Water 03-21-86 Alpha 15.7+/-1.5 15.0+/-5.0 0.2 l Beta 10.3+/-1.3 8.0+/-5.0 0.8 Water 04-04-86 I-131 0.0+/-1.5 9.0+/-6.0 -0.3 Filter 04-25-86 Alpha 19.0+/-1.5 15.0+/-5.0 1.4 Beta 47+/-2 47.0+/-5.0 0.1 Sr-90 17.0+/-1.5 18.0+/-1.5 -1.2 Cs-137 11.7+/-3 10.0+/-5.0 0.6 18
Table 8 (continued)
Concentration in pCi/ sample *a g Sample Date Analysis SLH result EPA result Deviation Type . Collected +/- 1 sigma +/- 1 sigma Known f
Blind 04-20-86 Alpha 14+/-2 17.0+/-5.0 -0.9 Beta 33+/-3 35.0+/-5.0 -0.7 Ra-226 3.1+/-0.4 2.90+/-0.44 0.7 Ra-228 2.1+/-0.3 2.00+/-0.30 0.8 l
U (nat) 3.7+/-5.0 5.0+/-6.0 -0.4 j Sr-89 6.7+/-0.9 7.0+/-5.0 -0.1 Sr-90 6.0+/-0.7 7.0+/-1.5 -1.2 Co-60 10+/-3 10.0+/-5.0 -0.1 Cs-134 4+/-2 5.0+/-5.0 -0.3 Cs-137 5+/-2 5.0+/-5.0 0.0 Water 05-09-86 Sr-89 5.0+/-2 5.0+/-5.0 0.0 Sr-90 5.0+/-1.5 5.0+/-1.5 0.0 Water 07-06-86 Cr-51 <38 0.0+/-5.0 Co-60 65+/-5 66.0+/-5.0 -0.5 Zn-65 86+/-5 86.0+/-5.0 0.0 Ru-106 47+/-5 50.0+/-5.0 -0.9 Cs-134 45+/-5 49.0+/-5.0 -1.4 Cs-137 8+/-5 10.0+/-5.0 -0.7 Water 06-20-86 Ra-226 7.3+/-1.3 8.6+/-1.3 -1.7 Ra-228 12.2+/-2.5 16.7+/-2.5 -3.1 ,
Milk 06-27-86 Sr-89 No data provided 0.0+/-5.0 Sr-90 16.6+/-1.7 16.0+/-1.5 0.8 I-131 39+/-5 41.0+/-6.0 -0.5 Cs-137 38+/-5 31.0+/-5.0 2.4 K 1660+/-120 16006/-80 1.4 Water 07-18-86 Alpha 8+/-2 6.0+/-5.0 0.7 Beta 18+/-2 18.0+/-5.0 -0.7 Food 07-25-86 Sr-89 No data provided 30+/-5 Sr-90 No data provided 19+/-1.5 1 I-131 24+/-5 30.0+/-6.0 - 1. 6 '
Cs-137 21+/-5 20.0+/-5.0 0.2 K 1180+/-120 1150+/-58 0.9 Water 08-08-86 I-131 41+/-10 45.0+/-6.0 -1.2 Water 08-22-86 U (Nat) 4+/-4 4.0+/-6.0 0.1 Water 09-12-86 Ra-226 6.5+/-0.9 6.1+/-0.9 0.8 4 Ra-228 10.3+/-1.5 9.1+/-1.4 1.5 19
Table 8 (continued)
Concentration in DCi/ sample *a Sample Date Analysis SLH result EPA result Deviation Type Collected +/- 1 sigma +/- 1 sigma Known. .
?
Filter 09-12-86 Alpha 20+/-2 22.0+/-5.0 -0.7 Beta 67+/-2 66.0+/-5.0 0.3 Sr-90 21.3+/-1.8 22.0+/-1.5 -0.8 Cs-137 28+/-5 22.0+/-5.0 2.0 Water 09-19-86 Alpha 11.3+/-2 15.0+/-5.0 -1.3 Beta 8.7+/-1.5 8.0+/-5.0 0.2 Water 10-10-86 Cr-51 61+/-10 59.0+/-5.0 0.6 Co-60 32+/-5 31.0+/-5.0 0.2 Zn-65 88+/-5 85.0+/-5.0 1.0 Ru-106 68+/-5 74.0+/-5.0 -2.2 Cs-134 29+/-5 28.0+/-5.0 0.3 Cs-137 46+/-5 44.0+/-5.0 0.5 Water 10-17-86 H-3 5300+/-300 5973+/-697 -2.0 Water 10-22-86 Alpha 39+/-2 40.0+/-5.0 -0.5 Beta 50+/-2 51.0+/-5.0 -0.2 Ra-226 6.2+/-1.0 6.0+/-0.9 0.3 Ra-228 3.5+/-0.8 5.0+/-0.8 -3.5 U (nat) 9.34 /-7.0 10.0+/-6.0 -0.2 Sr-89 10.7+/-2.5 10.0+/-5.0 0.2 Sr-90 3.7+/-1.5 4.0+/-1.5 -0.4 ;
Co-60 27+/-5 24.0+/-5.0 1.0 i Cs-134 11+/-4 12.0+/-5.0 -0.5 )
Cs-137 10+/-4 8.0+/-5.0 0.7 )
Water 11-21-86 Alpha 16+/-2 20.0+/-5.0 -1.4 Beta 23.7+/-2 20.0+/-5.0 1.3 Water 22-12-86 Ra-226 6.2+/-1.0 6.8+/-1.0 -1.0 Ra-228 10.5+/-1.7 11.1+/-1.7 -0.6 l
20
Table 8 (continued)
Concentration in poi / sample *a Sample Date Analysis SLH result EPA result Deviation
- . +/- 1 sigma Known Type Collected +/- 1 sigma e
Water 01-09-87 Sr-89 25+/-5 25.0+/-5.0 0.1 Sr-90 24.7+/-1.5 25.0+/-1.5 -0.4 Water 01-23-87 Alpha 10+/-2 11.0+/-5.0 -0.2 Beta 12.3+/-1.7 10.0+/-5.0 0.8 Food 01-30-87 Sr-90 No data provided 49.0+/-10.0 I-131 76+/-10 78.0+/-8.0 -0.4 Cs-137 89+/-8 84.0+/-5.0 1.6 K 1070+/-110 980+/-49 3.3 Water 02-06-87 Co-60 49+/-7 50.0+/-5.0 -0.5 Zn-65 92+/-8 91.0+/-5.0 0.5 Ru-106 90+/-?O 100.0+/-5.0 -4.2 Cs-134 50+/-8 59.0+/-5.0 -3.0 Cs-137 85+/-8 87.0+/-5.0 -0.6 Water 02-13-87 H-3 4200+/-400 4209+/-420 -0.2 Water 02-20-87 U 11+/-6 8.0+/-6.0 0.7 Milk 02-27-87 I-131 9.3+/-1.0 9.0+/-0.9 0.6 Water 03-13-87 Ra-226 7.4+/-1.1 7.3+/-1.1 0.2 Ra-228 8.1+/-1.1 7.5+/-1.1 0.9 Water 03-20-87 Alpha 3.7+/-1.5 3.0+/-5.0 0.2 Beta 14.0+/-1.8 13.0+/-5.0 0.3 Water 04-03-87 I-131 7.0+/-1.0 7.0+/-0.7 0.0 i Filter 04~10-87 Alpha 16+/-2 14.0+/-5.0 0.7 Beta 44+/-3 43.0+/-5.0 0.2 Sr-90 18.0+/-1.5 17.0+/-1.5 1.2 Cs-137 8+/-4 8.0+/-5.0 0.1
- Blind 04-20-87 Alpha 29+/-5 30.0+/-8.0 -0.3 Ra-226 3.4+/-1.0 3.9+/-0.6 -0.4 Ra-228 3.8+/-1.0 4.0+/-0.6 -0.7 U 6+/-5 5.0+/-6.0 0.3 Beta 66+/-5 66.0+/-5.0 -0.1 Sr-89 20+/-3 19.0+/-5.0 0.3 Sr-90 9.0+/-1.5 10.0+/-1.5 -1.2 Co-60 8+/-3 8.0+/-5.0 -0.5 Cs-134 17+/-3 20.0+/-5.0 -0.9 Cs-137 15+/-3 15.0+/-5.0 -0.1 t 21 I i
Table 8 (continued)
Concentration in pC1/ sample *a Sample Date Analysis SLH result EPA result Deviation Type Collected' +/- 1 sigma +/- 1 sigma Known
- s Water 05-08-87 Sr-89 39+/-3 41.0+/-5.0 -0.7 Sr-90 20.7+/-1.5 20.0+/-1.5 0.8 Water 05-22-87 Alpha 9+/-2 11.0+/-5.0 -0.8 Beta 9.3+/-1.8 7.0+/-5.0 0.8 Water 06-05-87 Cr-51 LT 45 41.0+/-5.0 Co-60 65+/-5 64.0+/-5.0 0.2 Zn-65 9+/-5 10.0+/-5.0 -0.3 Ru-206 66+/-5 75.0+/-5.0 -3.1 Cs-134 35+/-5 40.0+/-5.0 -1.6 Cs-137 77+/-5 80.0+/-5.0 -1.2 Water 06-12-87 H-3 3000+/-300 2895+/-357 0.4 Water 06-19-87 Ra-226 6.8+/-1.5 7.3+/-1.1 -0.8 Ra-228 19+/-2 15.2+/-2.3 2.6 Milk 06-26-87 Sr-89 No data provided 69.0+/-5.0 Sr-90 37+/-3 35.0+/-1.5 2.7 I-131 62+/-5 59.0+/-6.0 0.9 Cs-137 77+/-5 74.0+/-5.0 1.0 K 1680+/-190 1525+/-76 3.4 Water 07-24-87 Alpha 5.3+/-1.6 5.0+/-5.0 0.1 Beta 5.0+/-1.2 5.0+/-5.0 0.0 Food 07-31-87 Sr-89 No data provided 20.0+/-5.0 Sr-90 No data provided 30.0+/-1.5 I-131 76+/-7 80.0+/-8.0 -0.7 Cs-137 49+/-6 50.0+/-5.0 -0.2 K 1820+/-150 1680+/-84 2.9 '
Water 08-07-87 I-131 44+/-11 48.0+/ 6.0 -1.2 ;
Water 08-21-87 U 14+/-6 13.0+/-6.0 0.2 l Filter 08-28-87 Alpha 12.0+/-1.8 10.0+/-5.0 0.7 Beta 30.0+/-1.5 30.0+/-1.5 0.0 :
Sr-90 9.0+/-0.8 10.0+/-1.5 -1.2 Cs-137 12+/-5 10.0+/-5.0 0.7 Water 09-11-87 Ra-226 9.8+/-1.5 9.7+/-1.5 0.2 Ra-228 6.7+/-0.8 6.3+/-1.0 0.7 22 l
Table 8 (continued)
Concentration in pCi/ sample *a
,. Sample Date Analysis SLH result EPA result Deviation Type Collected +/- 1 sigma +/- 1 sigma Known s
Water 09-18-87 Alpha 4.0+/-1.8 4.0+/-5.0 -0.1 Beta 13.0+/-1.3 12.0+/-5.0 0.4 Water 10-09-87 Cr-51 55+/-5 70.0+/-5.0 -5.1 Co-60 15+/-4 15.0+/-5.0 -0.1 Zn-65 41+/-5 46.0+/-5.0 -1.9 Ru-106 48+/-6 61.0+/-5.0 -4.5 Cs-134 26+/-4 25.0+/-5.0 0.4 Cs-137 51+/-5 51.0+/-5.0 0.1 Water 10-16-87 H-3 4303+/-300 4492+/-449 -0.7 Water 10-21-87 alpha 32+/-3 28.0+/-7.0 1.0 beta 73+/-5 72.0+/-5.0 0.5 Ra-226 4.5+/-0.7 4.80+/-0.72 -0.7 Ra-228 4.5+/-0.5 3.60+/-0.54 2.8 ,
U (nat) 4+/-5 3.0+/-6.0 0.4 i Sr-89 16+/-3 16.0+/-5.0 0.0 Sr-90 9.7+/-1.5 10.0+/-1.5 -0.4 Co-60 14+/-5 16.0+/-5.0 -0.7 Cs-134 15+/-5 16.0+/-5.0 -0.5 Cs-137 22+/-4 24.0+/-5.0 -0.8 Water 11-20-87 alpha 7+/-2 7.0+/-5.0 0.0 i beta 20+/-2 19.0+/-5.0 0.5 Water 12-04-87 I-131 26+/-4 26.0+/-6.0 0.0 Water 12-11-87 Ra-226 4.6+/-0.6 4.80+/-0.72 -0.6 Ra-228 6.4+/-0.8 5.30+/-0.80 2.5 l
- a - pC1/ sample refers to the following:
Sample Units I I
water pCi/ liter milk pol / liter except for K mg/ liter food pCi/kg except for K mg/kg !
filter pC1/flater j 23 I
A_UACHMENT A RADIO-ENVIRONMENTAL SAMPLE ANALYSES MAXIMUM LOVER LIMITS OF DETECTION VALUES (LLD)a Sample Type !
Water Airborne Particulate Fish Milk Sedicent i Ana lysis pCi/1 or Radioiodine (pCi/m3) (pCifrg, wet) (pci/1) (pci/kg Dry) !
Gross Beta 6 1 x 10-2 H-3 3500(2000)b Mn-54 15 130 Fe-59 30 260 Co-58, 60 15 130 30 260 Zn-65
$ ' Zr-95 30 Nb-95 15 I-131 3C 7x 10-2 Sc 5 x 10-2 130 15 150 Cs-134 15 150 18 180 Cs-137 18 6 x 10-2 1 60 Ba-140 60 20 La-140 20 (See Footnotes a, b, and c on following page.)
s WP35 u____ ____._.._m_ _ _ _ _ _ _ _ _ _ _ _ _ _ _ . _ _ _ _
. . . - ~ .. . ..
ATTACHMENT A - RADIO-ENVIRONMENTAL SAMPLE ANALYSES MAXIMUM LOWER LIMITS OF DETECTION VALUES (LLD)s - (Cont'd)
(a) Calculation of Lower Limits of Detection:
The LLD,is the smallest concentration of radioactive material in a sample that will be detected with 95:
probability with 5: probability of falsely concluding that a blank observation represents a "real" signal.
For a particular measurement system (which may include radiochemical separation):
4.66 ab '
LLD -
E x V x 2.22 x T x Exp(-Aat)
WHERE: -
LLD is the a priori lower limit of detection as defined above (as picocurie per unit mass or volum'e)..
sb is the standard deviation of the background counting rate or of the counting rate of a blank sample as appropriate (as counts per minute). Typical values of E, V, Y, and at shall be used in the calculations.
E is the counting efficiency (as counts per transformation).
u
- v. V is the sample size (in units of mass or volume).
2.22 is the number of transformations per minute per picoeurie.
Y is the fraction radiochemical, yield (when applicable).
1 is the radioactive decay constant for the particular radionuclide.
At is the elapsed time between sample collection (or end of the sample collection period) and time of counting.
(b) (2,000) LLD drinking water.
(c) LLD for gamma spectrum analyses not separation and specific isotopic analysis.
l Wr35
Table 1. Air particulate g oss beta and air iodine (I-131) results for January - June, 1987. Indicator site.
WISCONSIN DIVISION OF HEALTH LACBWR SECTIOld OF RADI ATION PROTECTION 1987
)
Heesurements in units of pCf/M'3
- WI - Section of Radi6 tie Protection data LAC 8WR data Lock & Den 88 Lock & Den 84 0.7 miles N 0.7 miles 1 Collectioneste Air Particulate Airlodine Collection date Air Particulate Air lodine 01/07/07 0.024+/-0.002 -0.001+/-0.017 01/06/87 0.027+/-0.002 <0.0023 01/14/07 0.016+/-0.002 0.006+/-0.04 01/13/47 0.026+/-0.002 <0.0020 01/21/87 0.017+/-0.002 -0.016+/-0.03 01/20/47 0.025+/-0.002 <0.0018 01/24/87 0.016+/-0.002 -0.003+/-0.02 01/24/47 0.020+/-0.002 (0.0023 02/04/07 0.00t+/-0.004 -0.003+/-0.05 02/03/07 0.020+/-0.002 <0.0022 02/11/87 0.000+/-0.001 -0.03+/-0.0 02/10/87 0.020+/-0.002 (0.11011 02/10/47 0.019+/-0.002 -0.017+/0.03 02/17/87 0.023+/-0.002 (0.0020 02/25/47 0.013+/-0.002 -0.013+/-0.04 02/24/47 0.022+/-0.002 <0.0020 03/03/07 0.016+/-0.002 -0.0i0+/-0.04 03/03/47 0.01t+/-0.002 <0.0017 03/11/87 0.011+/-0.002 -0.001+/-0.03 03/10/47 0.021+/-0.002 <0.0019 03/14/87 0.015+/-0.002 -0.02+/-0.02 03/17/87 0.023+/-0.002 (0.0016 03/25/97 0.013+/0.002 -0.0!+/-0.04 03/24/87 0.020+/-0.002 <0.0023 04/01/07 0.013+/-0.002 -0.006+/-0.04 03/31/87 0.015+/-0.002 <0.0021 04/01/47 0.016+/-0.002 -0.006+/-0.c4 04/07/47 0.025+/0.002 <0.0022 04/15/07 0.015+/0.002 -0.010+/-0.03 04/14/87 0.021+/-0.002 (0.0026 04/22/47 0,010+/-0.002 -0.013+/-0.03 04/21/47 0.016+/-0.002 <0.0022 04/29/47 0.013+/-0.002 0.003+/-0.04 04/20/87 0.014+/-0.002 <0.0022 G5/06/07 0.017+/0.002 -0.007+/-0.04 05/15/87 0.02t+/0.003 <0.0025 05/13/47 0.017+/-0.002 -0.015+/-0.04 05/12/47 0.021+/-0.002 <0.0026 !
05/20/47 0.014+/0.002 -0.001+/-0.03 05/19/87 0.021+/-0.002 <0.0023 05/27/87 0.00l+/-0.002 -0.02+/0.04 05/26/87 0.011+/0.002 <0.0036 06/03/87 0.013+/-0.002 0.003+/-0.04 06/02/t7 0.021+/-0.002 (0.0024 0$/10/07 0.013+/-0.002 -0.006+/0.03 06/09/47 0.025+/-0.002 <0.0027 08/17/47 0.01t+/-0.003 -0.000+/-0.03 06/16/87 0.027+/-0.003 <0.0026 08/24/47 0.017+/-0.002 -0.000+/-0.04 06/23/47 0.024+/-0.002 <0.0027 07/01/87 0.019+/-0.002 -0.003+/-0.03 06/10/47 0.021+/-0.002 <0.0025 D
26
1 l
l Tcblo 10. Air porticuleto groso bote end cir.icdino (I-131) rcculto for July - Decembar, 1987. Indicator site.
I WISCONSIN DIVISION OF HEALTH LACBWR l SECTION OF RADIATION PROTECTION 1987 lc --------------------------------------------------------------------------
MeasurementsinunitsofpCi/M'3 WI - Section of Radiation Protection data LAC 9WRdata Lu k & h a 88 Lxk & ha 88 0.7 miles N 0.7 miles N Collection date Air Particulate Air lodine Collectiondate Air Particulate Air lodine 07/08/87 0.018+/-0.002 -0.015+/-0.04 07/07/87 0.011+/-0.002 (0.0026 07/15/87 0.014+/ 5.32 -0.004+/-0.04 07/14/87 0.020+/-0.002 <0.0021 07/22/87 0.023+/ J.002 -0.004+/-0.04 07/21/87 0.027+/-0.003 <0.0021 07/29/87 0.019+/-0.002 -0.01+/-0.04 07/29/87 0.037+/-0.003 <0.0021 08/05/87 0.017+/-0.002 -0.006+/-0.03 08/04/87 0.028+/-0.003 <0.0029 08/12/87 0.018+/-0.003 -0.00$+/-0.05 08/11/87 0.023+/-0.002 (0.0028 08/19/87 0.018+/-0.002 -0.019+/-0.05 08/18/87 0.027+/-0.002 <0.0022 08/26/87 0.011+/-0.002 -0.010+/-0.04 08/25/87 0.023+/-0.002 <0.0023 09/02/87 0.015+/-0.002 0.016+/-0.03 09/01/87 0.024+/-0.002 <0.0024 09/09/87 0.017+/-0.002 0.001+/-0.03 09/08/87 0.027+/-0.002 (0.0024 09/16/87 0.013+/-0.002 -0.001+/-0.04 09/15/87 0.020+/-0.002 (0.0021 09/23/87 0.008+/-0.002 0.011+/-0.04 09/22/87 0.016+/-0.002 <0.0020 09/30/8f 0.020+/-0.003 0.003+/-0.04 09/29/87 0.034+/-0.003 <0.0020 10/07/97 0.010+/-0.002 0.00l+/-0.04 10/01/87 0.018+/0.002 <0.0023 10/14/87 0.015+/-0.002 -9.002+/-0.03 10/13/87 0.023+/-0.002 <0.0021 10/21/87 0.022+/-0.003 0.003+/-0.03 10/20/87 0.033+/-0.002 (0.0019 10/28/87 0.012+/-0.002 -0.003+/-0.03 10/27/87 0.021+/-0.002 (0.0020 ,
11/04/87 0.023+/-0.003 -0.005+/-0.03 11/03/87 0.023+/-0.002 (0.0021-j 11/11/87 0.017+/-0.002 0.007+/-0.03 11/10/87 0.023+/-0.002 <0.0026 11/18/87 0.023+/-0.003 -0.011+/-0.03 11/17/87 0.034+/-0.003 <0.0017 11/25/87 0.017+/-0.002 0.03+/-0.05 11/24/87 0.024+/-0.002 <0.0017 12/02/87 0.013+/0.002 0.000+/-0.03 12/01/87 0.009+/-0.002 (0.0019 12/09/87 0.012+/-0.002 0.001+/-0.03 12/08/87 0.015+/-0.002 (0.0018 12/11/87 0.015+/-0.002 -0.005+/-0.03 12/16/87 0.015+/-0.002 <0.0015 12/23/87 0.020+/-0.003 -0.016+/-0.04 12/23/87 0.021+/0.002 (0.0015 12/18/07 0.026+, 0.001 -0.006+/-c.03 12/29/87 0.031+/-0.002 <0.0012 i'
i
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27 I 1
a Tcblo 11. Air particulcto gro30 'bato cnd cir icdino (I-131) resulto for January - June, 1987. Control site.
WISCONSIN DIVISION OF HEALTH LACBWR SECTION OF RADIATION PROTECTIOtt 1987
~~~-~~~-- e e
Measurements in units of pC1/M'3 e
WI - Section of Aadiation Protection data LAC 8WRdata La Crosse La Crosse 15.8 miles N 16 miles N Collection date AirParticulate Airlodine Collectiondate Air Particulate Airlodine 01/05/87 0.024+/-0.002 0.002+/-0.03 01/06/87 0.038+/-0.003 <0.0024 01/12/87 0.022+/-0.002 -0.010+/-0.03 01/"3/87 0.026+/-0.002 <0.0024 01/19/87 0.018+/-0.002 0.00+/-0.02 01/20/87 0.017+/-0.002 <0.0021 01/26/87 0.017+/-0.002 0.006+/-0.016 01/28/87 0.019+/-0.002 <0.0029 02/02/87 0.018+/-0.002 -0.001+/-0.017 02/03/87 0.020+/-0.002 <0.0021 02/09/87 0.010+/-0.001 0.012+/-0.017 02/10/87 0.017+/-0.002 <0.0018 02/17/87 0.015+/-0.001 -0.003+/-0.03 02/17/87 0.018+/-0.002 <0.0021 02/23/87 0.011+/-0.002 -0.008+/-0.03 02/24/87 (0.0026 0.020+/-0.002 03/02/87 0.013+/-0.001 0.003+/-0.03 03/03/87 0.014+/-0.002 <0.0021 03/09/87 0.024+/-0.002 0.011+/-0.03 03/10/87 0.026+/-0.002 <0.0019 01/16/87 0.018+/-0.002 -0.003+/0.03 03/17/87 0.021+/-0.002 (0.0021 l 03/23/87 0.015+/0.002 0.00$+/-0.03 03/24/i? 0.017+/0.002 <0.0020 '
03/30/87 0.012+/-0.001 -0.003+/-0.03 03/31/87 0.011+/-0.002 <0.0019 04/06/87 0.014+/-0.001 -0.003+/-0.03 04/07/87 0.019+/-0.002 <0.0024 04/13/87 0.014+/0.002 -0.012+/-0.0i 04/14/87 0.014+/-0.002 (0.0022 04/20/87 0.010+/-0.001 -0.010+/-0.03 04/21/87 0.011+/-0.002 <0.0023 04/27/87 0.010+/0.002 -0.010+/0.03 04/28/67 0.012+/-0.002 <0.0021 05/04/87 0.018+/-0.002 -0.014+/-0.03 05/05/87 0.031+/0.003 <0.0032 05/11/87 0.017+/-0.002 -0.010+/-0.03 05/12/87 0.040+/-0.003 (0.0029 ,
05/18/87 0.012+/0.001 0.00+/-0.03 05/19/87 0.024+/-0.003 (0.0030 05/26/87 0.006+/-0.001 0.003+/-0.02 05/26/87 0.014+/-0.002 <0.0033 04/01/87 0.012+/-0.001 -0.003+/-0.011 06/02/87 0.024+/-0.003 <0.0031 1 06/08/87 0.013+/-0.001 -0.002+/-0.03 06/09/87 0.027+/-0.003 (0.0034 08/15/87 0.014+/-0.001 -0.003+/-0.02 06/16/87 0.030+/-0.003 <0.t 033 l 06/!!/87
- a 0.002+/-0.001 -0.001+/-0.03 06/23/87 0.024+/-0.003 (0.0034 !
3 06/28/87 0.014+/-0.001 0.003+/-0.03 04/30/87 0.023+/-0.003 <0.0030 i
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- a - Leser bete activity due to a sissing gasket in cartridge holdea.
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28
l Tablo 12. Air particulcto grecc bato end cir icdino (I-131) rcoulto y for July - December,1937. Control site. '
WISCONSIN DIVISION OF- HEALTH LACBWR SECTION OF D^ JIATION PROTECTION 1987 g _____......________. ___________ ____________....__________.... _________
Neesur m ts in units of pCi/0 3 s
WI
- Section of Rad 14 tion Protection data LAC HR data La Crosse La Crosse 15.6 miles N 16 ailes N Collection 6te Air Particulate Air lodine Collectica date Air Particulate Air lodine 07/06/87 *a 0.003+/-0.001 -0.011+/-0.02 07/07/87 0.017+/-0.032 <0.0035 07/t3/87 0.016+/-0.001 -0.003+/-0.02 07/14/8f 0.021+/-0.003 <0.0032 07/20/87 0.019+/-0.001 -0.002+/-0.03 07/21/87 0.033+/-0.003 <0.0020 07/27/87 0.018+/-0.002 -0.00!+/-0.03 07/29/87 0.029+/-0.003 <0.0034 08/03/87 0.019+/-0.002 -0.008+/-0.02 08/04/87 0.033+/-0.004 <0.0040 08/10/87 0.011+/-0.001 -0.002+/-0.03 08/11/81 0.023+/-0.003 (0.0030 08/17/87 0,017+/-0.002 -0.002+/0.03 08/18/87 0.024+/-0.003 (0.0028 08/24/87 0.012+/-0.002 -0. 002 +/-0.M 08/25/87 0.026+/-0.003 (0.0032 04/31/87 0.013+/-0.001 -0.003+/-0.02 09/01/87 0.027+/-0.003 <0.0035 09/08/87 0.016+/-0.001 -0.012+/-0.03 09/08/87 0.029+/-0.003 <0.0037 09/14/87 0.014+/-0.002 -0.002+/-0.03 09/15/87 0.022+/-0.003 <0.0030 09/21/87 0.013+/0.001 0.002+/-0.03 09/22/87 0.015+/-0.002 (0.0027 09/28/87 0.018+/-0.002 -0.002+/-0.02 09/29/87 0.040+/-0.003 <0.0034 10/05/87 0.011+/0.001 -0.002+/0.02 10/06/87 0.018+/-0.002 <0.0032 10/12/87 0.009+/0.001 -0.010+/-0.02 10/11/81 0.024+/-0.003 <0.0033 10/19/87 0.023+/0.002 -0.002+/0.02 10/20/87 0.041+/0.003 (0.0030 10/26/87 0.012+/0.001 -0.002+/-0.03 10/27/l 0.015+/-0.002 <0.0022 11/02/87 0.016+/-0.001 -0.002+/0.02 11/03/87 0.019+/-0.002 <0.0021 11/09/87 0.020+/0.002 0.001+/0.02 11/10/87 0.020+/-0.002 <0.0028 11/16/87 0.023+/-0.002 0.009+/-0.02 11/17/87 0.032+/-0.002 (0.0022 11/23/87 0.014+/-0.001 -0.004+/-0.02 11/24/87 0.022+/-0.002 <0.001?
11/30/47 0.013+/-0.001 -0.006+/-0.02 12/01/87 0.009+/-0.002 <0.0019 12/07/87 0.010+/-0.001 0.000+/-0.02 12/08/87 0.015+/-0.002 (0.0017 12/14/87 *b 8b 12/18/87 0.013+/-0.002 <0.0019 12/21/87 0.019+/-0.002 0.009+/-0.02 12/23/87 0.030+/-0.003 (0.0018 12/20/07 0.025+/-0.002 -J.002+/-0.02 12/29/47 0.032+/-0.002 (0.0016
- a - Lower beta a:tivity due to a missing gasket in cartridge holder.
8 b - Seaple w s not collected. Pump us off during the period of 12/07/87-12/14/87.
l 29 [
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Tob10 13. G mmo icatcpic roaulto for Jcnucry - Dacmb c, 1987 frcm the quarterly composite of air particulate samples.
Indicator site - Lock & Dam #8.
WISCONSIN DIVISION OF HEALTH LAC 8WR SECTION OF RADIATION PROTECTION 1987 NeesurementsinunitsofpCi/M'3 8 NI - Section of Radiation Protection data Lock & Dan 88 0.7 miles N 1st @arter 2nd @arter 3rd @ arter 4th @arter Be-7 0.097+/0.018 0.14+/0.02 0.089+/-0.018 0.09+/-0.02 Zr-95 0.000+/-0.003 -0.001+/0.003 0.000+/-0.004 -0.002+/-0.005 Ru-103 0.000+/-0.f.02 0.000+/-0.002 -0.001+/-0.002 0.000+/-0.003 Ru-106 0.001+/-0,000 0.002+/-0.007 0.001+/-0.007 0.000+/-0.012 1-131 0.003+/4.07 0.04+/-0.06 -0.003+/0.07 -0.02+/-0.11 Cs-134 0.000+/-0.001 0.000+/-0.001 0.000*/-0.001 -0.001+/-0.001 Cs-137 0.000+/-0.001 0.000+/0.001 -0.001+/0.001 -0001+/-0.001 Co-141 0.000+/-0.003 0.000+/-0.(03 0.001+/-0.003 -0.001+/-0.005 Co-144 0.001+/-0.004 0.000+/-0.005 -0.001+/-0.004 -0.001+/-0.007
!sotopes other than those reported were not detected.
LAC 8WR data Lock & Oas 38 0.7 miles N January February March April May hna Be 7 NA NA NA NA NA NA Zr,Nb-95 (OA (OA (OA <OA (OA <OA Ru-103 (OA (MDA <MDA (MDA <0A (MDA Ru-106 (CA <O4 (CA (OA <M0A <CA l-131 (OA (MDA <0A <OA (MDA <OA Cs-134 <0A <cA <@A (MDA (OA <M4 Cs-137 (OA 0.0010+/0.0003 (CA (OA (MDA 0.00096/0.0007 Co-141 (OA (OA <cA (M0A (OA <cA Cs-144 <0A <0A <OA (MDA <0A (OA Co-60 <CA 0.0004+/-0.0007 (OA (OA 0.0034+/-0.0011 0.0027+/-0.0012 July August September October hoveeber December Be-7 NA NA NA NA NA NA Zr Nb-15 (OA <cA <@A <@A <0A <cA Ru-103 <0A <0A <0A <0A <OA <0A Ru-106 (OA (OA (OA <0A (OA <OA l-131 (OA <cA <OA <0A <0A <04 C -134 (OA <0A <0t <McA <@A <OA Cs-137 (OA <0A <0A (OA <cA <OA Co-141 (OA (OA <0A <0A (OA <0A .
Co-144 (OA <cA <ct <0A <0A <0A Cr-51 (OA <0A <@A <OA 0.011+/0.007 (OA Mn 54 (OA <cA <MDA <0A <OA 0.002t+/-0.0007 NA - Naturally occurring radioisotopes are not usually specifically analyzed for.
30
Tcblo 14. Gamma icatcpic rctulto fer Jtnucry - December, 1987 from th3 qucrterly ccmp20ito of cir p rticulcto ocmplco.
Control site - La Crosse.
WISCONSIN DIVISION OF HEALTH' LAC 8WR SECTION OF RADIATION PROTECTION 1987 Measurements in units of PCi/M*!
i MI - Section of Radiation Protection data La Crosse 15.6 miles k t 1stQuarter 2ndQuarter 3rdQuarter 4thQuarter 63-7 0.096+/0.013 0.111+/-0.013 0.087+/-0.011 0.060+/-0.010 Zr-95 0.000+/-0.002 -0.001+/-0.002 0.001+/-0.002 -0.001+/-0.002 Ru-103 0.000+/-0.001 0.001+/-0.001 -0.001+/-0.001 0.000+/-0.001 Ru-106 0.000+/-0.004 0.004+/-0.004 -0.001+/-0.004 0.002+/-0.004 l-131 -0.01+/-0.04 -0.002+/-0.04 -0.007+/-0.04 -0.003+/-0.05 Cs-134 0.000+/-0.001 0.000+/-0.001 0.000+/-0.001 0.000+/-0.001 Co-131 0.000+/-0.001 0.001+/-0.001 0.000+/-0.001 0.000+/-0.001 Ce 141 0.001+/-0.102 0.000+/-0.002 0.000+/-0.002 0.000+/-0.001 Ce-144 0.000+/-0.002 0.000+/-0.003 0.000+/-0.002 0.000+/-0.002 Isotopes other than those reported were not detected.
LAC 8WR La Crosse 16 miles N January February March April May June Be-7 NA NA NA NA NA NA Ir-95 <CA <CA <OA (MDA (OA (MDA Ru-103 <OA <0A (OA (MDA <0A <0A Ru-106 <0A (OA <OA (MDA <MDA (MDA l-131 (OA (MOA (OA (MDA (OA (OA Cs-134 (OA <MDA <PDA, <OA <M0A (OA Cs-137 <OA <0A <0A <OA <04 (OA Ce-141 <OA 0.0000+/-0.0003 (OA <OA <OA (OA Ce-144 (OA <0A (OA <0A <OA <0A Co-60 (OA 0.0011+/-0.0009 (OA <OA <0A 0.0036+/-0.0016 July August September October November Deceeber l Se-1 NA NA NA NA NA NA Ir-l$ (OA (OA (OA (OA (OA <OA Rv-103 (OA (OA (CA <CA <0A (OA Ru-106 <0A <CA (OA (OA (OA (OA I l-131 (CA (OA (OA (OA (OA (OA Co-134 (OA (OA (OA (OA (OA (OA Cs-137 (OA (OA (OA (OA (OA (OA Co-141 (OA (OA (OA (OA (OA (OA
. Co-144 (OA (OA (OA (OA (OA (OA Co 60 <0A <CA <CA <OA 0.002+/-0.002 (OA Co-57 (OA <On <CA (OA 0.0006+/-0.0003 (OA NA - Naturally ocevering radioisotopes are not usually specifically analyzed for.
31
Table 15. Analysis of surface water samples from January - June, 1987, Indicator site.
DISCONSIN DIVISION OF HEALTH LACBWR SECTION OF RADIATION PROTECTION 1987
.-------------------------------------------------------------- -g MeasurementsinunitsofpCi/ liter Effluent channel '
WI - S u tton of Radiation Protection data 0.1 mile W
- Collection Date 01/13/87 02/10/87 03/10/87 04/14/87 05/12/87 06/09/87 Gross Alpha sol. 2.2+/-1.9 1.1+/1.5 4+/! 1.1+/-1.4 1. 4 +/- 1. 5 0.7+/-1.6 Gross Alpha-insel 0.4+/-0.8 -0.1+/0.6 1.3+/-0.9 1.3+/-0.9 0.5+/0.8 1.5+/-0.9 Gross Beta sol. 1.1+/-1.5 3.6+/-1,3 8.7+/-1.6 4.8+/-1.4 5.1+/-1.4 4.3+/-1.4 Gros Beta-insol. 5.1+/-1,3 0.8+/-1.0 3.0+/-1.1 0.9+/-1.0 4.8+/-1.4 1.9+/-1.0 N-1 610+/-310 90+/310 6900+/-400 300+/-320 140+/-310 -750+/-320 3r-89 0.6+/-0.4 0.0+/-0.4 0.5+/-0.3 0.0+/-0.4 0.0+/-0.4 0.1+/-0.4 Sr-90 1.4+/-0.4 0.0+/-0.4 0.5+/0.3 0.4+/-0.4 0.3+/-0.4 0.3+/-0.4 1 131 -0.2+/0.1 0.0+/-0.1 0.1+/0.1 -0.1+/-0.1 0.0+/-0.2 0.z+/-0.1 Ganas Isotopic Mn-54 5+/6 1+/-5 -1+/-6 -1+/-5 -1+/-5 -1+/-5 Fe-59 b/-10 -1+/9 -3+/-9 0+/-10 0+/-9 -3+/-9 Co-58 -1+/5 -2+/-5 -2+/-7 0+/-5 -3+/-5 -!+/-5 Co-60 $+/-7 0+/5 4+/-6 0+/-6 -1+/-6 -2+/-5 In 65 -2+/-11 2+/-11 4+/-12 -3+/-11 -2+/-14 4+/-14 C -134 6+/-6 3+/6 1+/-6 2+/-6 -2+/-6 0+/-6 C -137 8+/7 -!+/-6 1+/6 -1+/-6 -1+/-6 -1+/-7 Ir 95 6+/14 -5+/-15 (+/-14 -5+/-13 1+/-13 -1+/-13 8a,La 140 -2+/6 0+/6 2+/-7 1+/-8 -4+/-6 -2+/6 Isotopes other than those reported were not detected.
LA08uRdata Ef fluent channel 0.1 mile W Collection Date 01/13/87 02/10/87 03/10/87 04/14/87 05/12/87 06/09/87 Gross Alpha <19.3 <20 5 <17.1 (19.7 <16.4 <14.7 Gross Beta 5.86+/-0.84 2.49+/-0.71 4.29+/-0.84 4.22+/-0.95 6.54+/-0.86 1.87+/-0.70 H3 <1391 <1287 $272 <1307 2076 (1988 i
Gaasa Isotopic ph-54 13.ft/-4.0 <MDA (MDA <MDA (MDA (MDA I Fe-59 (MDA <MDA <MDA (MDA (MDA <MDA Co 58 (MDA (MDA (MDA <MDt <MDA (MDA C~60 (MDA (MDA (MDA (MDA (MDA (MDA In-65 <MDA <MDA (MDA <MDA <M0A (MDA l-131 (MDA (MOA (MDA <MDA (MDA (MDA Cs-114 (MDA (MOA (MDA (MDA (MDA (MDA l Cs-;J1 (MDA (MDA (MDA (MDA (MDA (MDA .
Ir-95 <MDA <MDA (MDA (MDA <MDA <MDA 8a,La-140 (MDA (MDA (MOA (MDA (MDA (MDA Ce-141 (MDA (MDA 1.2+/4.5 <MDA <MDA (MDA 32 1
i Tcble 16. Analysis of surface water samples from July - December, 1987. Indicator site.
WISCONSIN DIVISION OF HEALTH LAC 8WR SECTION OF RADIATION PROTECTION 1987 6
8 MeasurementsinunitsofpCi/11 tea Effluent channel
. WI - Section of Radiation Protection data 0.1 mile W Collection Date 07/14/87 08/11/87 09/08/87 10/13/87 11/10/87 12/08/87 6 mss Alpha-sol. 4+/-2 0.1+/-1.5 0.6+/-1.6 4.0+/-1.9 5+/-2 1.9+/-1.6 Gross Alpha-insol 0.2+/-0.8 0.5+/-0.9 1.3+/-1.0 4.0+/-1.3 3.6+/-1.2 3.1+/-1.2 Gross Beta-sol. 4.7+/-1.4 3.7+/-1.3 6.3+/-1.5 48+/-3 49+/3 32+/-3 Gross Bota-insel. 1.2+/-1.0 2.3+/-1.0 15.2+/-1.7 60+/-3 57+/-3 53+/-3 H-3 400+/-440 370+/-570 260+/-330 57006/-300 8300+/-400 180+/-210 Se-89 0.2+/-0.4 0.6+/-0.4 0.2+/0.4 -0.9+/-0.4 0.3+/-0.5 -0.4+/-0.4 Se-90 0.5+/-0.4 0.0+/-0.4 0.2+/-0.4 1.3+/-0.4 0.9+/-0.6 0.4+/-0.3 1-131 0.3+/-0.2 -0.1+/-0.2 -0.1+/-0.2 -0.1+/-0.2 -0.1+/-0.2 0.0+/-0.2 Gamma Isotopic m-54 -2+/-5 2+/-6 3+/-6 32+/-8 20+/-11 25+/-9 Fe-59 -1+/-10 -2+/-9 1+/-10 -3+/-12 3+/-20 8+/-15 Co-58 -1+/-5 2+/-5 0+/-5 -4+/-7 2+/-11 2+/-7 Co-60 -1+/-5 2+/-6 10+/-7 56+/-10 124+/-18 70+/-15 In-65 2+/-11 -1+/-11 -1+/-11 -7+/-15 -1+/20 18+/-14 Cs-134 0+/-7 2+/-6 0+/-6 -3+/-7 6+/9 9+/-7 Cs-137 0+/-7 -4+/-6 -1+/6 34+/-7 27+/-12 30+/-10 Ir-95 -!+/-15 1+/-13 -8+/-16 -3+/-14 16+/-20 5+/-16 Ba,La-140 -1+/-6 -1+/-8 -1+/-7 -1+/-6 -2+/-9 0+/-7 A;-110 14+/-7 Isotopes other than those reported were not detected, l.AC8WR data Effluent channel 0.1 mile W Collection Date 07/15/87 08/11/87 09/08/87 10/13/87 11/10/87 12/08/87 Gross Alpha (13.1 (13.3 (13.4 <21.9 <19.9 (24.3 Gross tota 4.4+/-0.9 3.7+/-0.7 6.2+/-1.0 59.8+/-2.4 10.6+/-2.6 46.7+/-2.2 H-3 <1427 <1470 <1400 2043 9162 <1486 Genna Isotopic m-54 <0A (OA <CA 44.7+/-7.1 26.3+/-5.6 9.3+/-6.6 Fe-59 (OA (OA (ROA <0A (RCA <CA Co-58 <0A <0A (OA <OA <CA <0A Co-60 (RDA (OA (OA 52.2+/-11.5 118.8+/-13.8 26.6+/-108 In ll (OA <OA (CA <OA (OA <0A 1-131 <0A (OA <MDA (RDA <0A (OA C 134 (OA <OA (CA (OA (RDA (OA Cs-137 (OA <CA (MDA 38.3+/-l.6 39.3+/-6.8 30.8+/-4.9 Ir-95 (MDA <rDA <MDA (MDA (MDA <0A Ba,La 140 (OA (OA <OA (OA (OA <OA Ru-103 (OA (OA (OA 7.6+/-3.2 (OA (OA 33
\
Table 17. Analysis of surface water samples from January - June, 1987. Control site - Lock & Dam #8.
WISCONSIN DIVISION OF HEALTH LAC 8WR SECTION OF RADIATION PROTECTION 1987 MeasurementsinunitsofpCi/ liter '
4 W! - Section of Radiation Protection data Lock & Den 88 0.7 miles N Collection Date 01/13/87 02/10/87 03/10/87 04/14/87 05/12/47 06/09/87 BrossAlpha-sol. 0.2+/-1.4 1.2+/-1.4 1.2+/-1.4 0.5+/-1.2 1.8+/-1.6 1.2+/-1.7 Gross Alpha-insel -0.1+/0.7 0.1+/-0.7 0.5+/-0.8 0.2+/-0.7 0.0+/-0.1 1.3+/-0.8 Gross Beta-sol. 3.5+/-l.3 4.0+/-1.3 4.9+/-1.4 4.0+/-1.3 4.6+/-1.3 3.8+/-1.3 Gross Beta-insel. 1.7+/-1.0 0.3+/-0.8 1.9+/-1.1 0.1+/-0.9 0.0+/-0.1 1.3+/-1.0 H-3 -100+/-300 -11t+/-310 100+/300 220+/310 100+/-310 -8 4 /-320 3r-89 -0.2+/-0.5 -0.1*/-0.4 0.4+/0.4 0.0+/0.4 0.0+/-0.3 0.9+/0.4 SF-90 1.0+/-0.4 0.1+/-0.4 0.5+/-0.3 0.2+/-0.4 0.3+/-0.3 0.1+/-0.4 1 131 -0.1+/-0.1 0.1+/-0.1 0.0+/-0.1 -0.1+/-0.1 0.2+/-0.2 -0.2+/-0.1 Genes isotopic M-54 -2+/5 -2+/-5 -4+/-? -4+/-7 1+/6 -2+/-5 Fe-59 -1+/9 1+/-9 -5+/-14 0+/-14 -3+/-12 -3+/-11 00-58 -1+/-5 -1+/-5 0+/-7 1+/8 0+/5 -5+/-6 Co-10 0+/6 1+/-7 0+/8 0+/8 1+/-5 -1+/-5 In-15 3+/-12 7+/-12 -15+/-11 1+/-16 6+/-12 -6+/-11 Co-134 3+/6 2+/-7 1+/8 2+/-7 4+/6 -3+/5 C 137 0+/-l 3+/6 -10+/-9 -4+/8 2+/6 0+/-l Ir-ll 5+/13 6+/-14 -10+/-16 -4+/18 -3+/-13 0+/-12 La-140 -1+/6 -1+/6 1+/-8 5+/-11 -2+/6 -2+/8
!setopes other then those reported were not detected.
LACtMR data Lock & Den 38 0.7 miles N Collection Date 01/13/87 02/10/87 03/10/87 04.14/87 05/12/87 06/09/87 Scots Alpha (19.3 (20.5 <17,1 <19.7 (16.4 <14.7 Gross Beta 2.15+/0.59 2.76+/-0.17 2.81+/-0.75 <1.12 2.75+/-0.62 1.41+/-0.67 H-3 (1396 (1287 <1305 (1307 (1808 (1988 6eenaIsotopic Mn 54 <MDA <MDA (MDA (MDA <MDA (MDA l Fe 59 (MDA <MDA (MDA <MDA (MDA Co-58 (MDA (MDA l (MDA (MDA (MDA <MDA <MDA !
Co IO (MDA (MDA (MDA (MDA (MDA . l
<MDA
!a 65 <MDA <MDA (MDA <pDA <MDA <pDA l l-131 (MDA (MDA <MDA < mD,
<MDA <mDA Cs 134 (MDA (MDA <pDA l
<MDJ <MDA <MDA Cs-137 <pDA
- l (MDA (MDA < pDJ, <pDA <pDA l IP 95 <MDA <MDA <MDA <MDa <MDA <MDA l Ba.La-14 0 <MDA <MDA <MDA <MDt <MDA <MDA {
34
Toble 18. Analysis of surface water samples from July - December, 1987. Control site -
Lock & Dam #8.
WISCONSIN DIVISION OF HEALTH LACBWR SECTION OF RADIATION PROTECTION 1987 8 MoesurementsinunitsofpC1/ liter s
WI - Section of Radiation Protection data Lock & Dee Il 0.7 miles N Collection Date 07/14/87 08/11/87 09/08/87 10/13/87 11/10/87 12/08/87 Gross Alpha-sol. 2.4+/-1.8 0.6+/-1.7 0.4+/-1.5 0.2+/-1.2 0.5+/-1.3 0.5+/-1,3 Gross Alpha-insol 0.4+/-C.7 -0.1+/-0.8 -0.2+/-0.7 0.1+/-0.7 0.7+/-0.7 0.0+/-0.6 Gross Ista-sol. 4.9+/-1.4 3.6+/-1.3 4.1+/-1.4 3.9+/-1.4 3.7+/-1.3 4.2+/-1.3 Gress Beta-insel. 0.9+/-1.0 -0.1+/-0.8 1.0+/-0.9 0.2+/-0.9 2.4+/-1.0 -0.3+/-0.9 H-3 860+/-440 130+/-570 -160+/-320 -90+/-250 100+/-270 -140+/-280 Sr-89 0.8+/-0.4 0.5+/-0.4 0.1+/-0.4 -0.4+/-0.3 -0.4+/-0.4 0.0+/-0.4 Sr-90 0.0+/-0.4 0.0+/-0.4 0.0+/-0.4 1.0+/-0.3 0.0+/-0.4 0.0+/-0.3 1-131 -0.1+/-0.2 0.1+/-0.2 -0.2+/-0.2 -0.1+/-0.2 -0.2+/-0.2 -0.2+/-0.2 6eena Isotopic Mn-54 0+/-5 -2+/-5 -1+/-5 2+/-6 0+/-5 -1+/-5 Fe-59 -3+/-9 1+/-10 3+/-11 -2+/-10 3+/-10 1+/-11 Co-58 -1+/-5 2+/-5 0+/-5 -2+/-! 1+/-5 0+/-6 Co-60 0+/-6 -1+/-5 0+/-5 0+/-5 0+/-6 -1+/-6 In-65 1+/-11 10+/-12 -2+/-11 -1+/-11 4+/-12 -4+/-11 Cs 134 -2+/6 -1+/-6 -1+/-6 3+/6 -2+/-6 -2+/-6 Cs-137 -1+/-8 -3+/-6 -1+/-6 4+/-6 -1+/-6 -1+/-6 IP-95 -l+/-13 -l+/-15 -8+/-16 1+/-14 -2+/-13 -6+/-13 La-140 -1+/-6 -2+/-6 1+/-7 -2+/-9 5+/-9 -6+/-7 Isotopes other than those reported were not detected.
LAC 8MR data Lock 6 Das 38 !
0.7 miles N Collection Dete 07/14/87 08/11/87 09/08/87 10/13/87 11/10/87 12/08/07 Gross Alpha <13.1 < 13 .3 <13.4 <21.9 <19.9 <24.3 Gross Beta 2.3+/-0.7 3.1+/-0.6 2.0+/-0.7 2.4+/-0.8 3.2+/-0.8 2.6+/-0.8 H3 <1427 <1470 (1400 <1512 <1480 <1486 6eena Isotopic t-54 (MDA (OA (MCA (OA (MDA (MDA Fe-59 (MOA (MOA (MCA <MDA <MDA (MCA Co-58 (CA (OA <OA (RDA (OA (OA Co-80 <CA (OA (OA (MDA (OA (MDA In-65 (OA (OA (OA <0A (OA (OA l-131 (OA (OA (OA (OA (OA (OA Cs 134 (OA (OA (OA (OA (OA (OA Co-137 (OA (OA (OA (OA (OA (OA Zr-95 (OA (OA (OA (OA (OA (OA la,La-140 (OA (OA <OA <0A (OA (CA 35
Table 19. Analysis of *1sh samples for 1987.
WISCONSIN DIVISION OF HEALTH LACBWR SECTION OF RADIATION PROTECTION 1987
'l s
Measurements in units ofP Ci/k0(wet)
WI - Section of Radiation Protection data Collection Date 02/18/87 02/18/87 04/22/87 04/22/07 Type carp sheephead carp walleye Genee lectopic K 40 2600+/500 3100+/600 2300+/-600 4600+/-700 Mn-54 2+/-20 1+/20 -2+/30 -2+/-20 Fe 59 1t+/-70 16+/-60 -l+/-80 60+/-70 Co-58 -3+/-30 -3+/-30 -6+/-30 0+/-30 Co-60 40+/-30 5+/-30 20+/30 -4+/10 In-65 10+/-60 1+/70 10+/-10 19+/-60 Cs-134 4+/-20 20+/10 1+/30 1+/-20 Cs-137 17+/-30 10+/-30 -8+/-30 -3+/-30 Isotopes other than those reported were not detected.
LAC 9WR data Collection Date 02/18/87 02/18/07 04/22/87 04/22/87 fype carp sheephead carp walleye Geese Isotopic l K 40 NA NA NA NA
)
m 54 (OA (MCA <0A (OA j Fe-59 (MDA (OA (MOA (RCA 1 Co-58 (O4 (OA <OA <0A Co-60 27.4+/-13.2 26.1+/-18.2 <ROA (RDA In-65 <NA (OA <m0A 34.2+/-12.3 C -134 < C.A <01. (NOA (CA Cs-137 (CA (OA (MDA <CA NA - Naturally occurring radioisotopes are not usually specifically analyzed for.
36
Tcble 20. Analysis of fish samples for 1987.
WISCONSIN DIVISION OF HEALTH LACBWR SECTION OF RADIATION PROTECTION 1987 i
n _____________________________ ______________________________________
Ressurements in units of pC1/kg (met)
N! - Section of Radiation Protection Collection Cate 08/06/87 01/06/81 10/22/87 10/22/87 fype carp malleye carp walleye Geena Isotock K-80 3400+/-500 3700+/-600 3300+/-300 3900+/-500 m-54 -l+/-20 -1+/-20 1+/-11 0+/-20
-Fe59 -4+/-50 -7+/-60 6+/-30 19+/-50 Co-58 -2+/-20 -4+/-30 -2+/-16 -2+/-30 Co-60 18+/-20 -5+/-30 -3+/-14 20+/-30 In-65 -7+/-60 40+/-70 70+/-30 0+/-50 Cs-134 11+/-20 -2+/-20 15+/-12 -9+/-20 Cs-137 6+/-18 20+/-30 13+/-13 12+/-20
!sotopes other than those reported were not detected.
LAC 8WR data Collection Date 08/06/77 08/06/87 10/22/87 10/22/81 l
7ype carp walleye carp walleye Genoa Isetopic K-40 NA NA NA NA t-54 <CA (RDA (OA <MA Fe-59 (RDA <pDA (OA (MA l Co-58 <RDA (RCA (MDA (OA Co-60 (RDA (MDA (RDA (OA In-65 <EA <oA <cA <RDA Cs-134 (MA (RCA <RDA <RDA l
Cs-137 (MA (RDA (RDA (ROA i
0 - Naturally occurring radioisotopes are not specifically analynd for.
l i
l 37 i
)
1 I
Toblo 21. Anclycio of bottom ocdim:nto for 1987.
WISCONSIN DIVISION OF HEALTH LAC 8WR SECTION OF RADIATION PROTECTION 1987 MeasuresentsinunitsofpCi/kg(dry) '
WI - Section of Radiation Protection data 4
Collection Date 08/06/87 08/06/87 08/06/87 5 Type bottonsed. botton sed, bottoa sed, e
Location upstrean discharge downstrece Analysis Grossbeta(dry) 23000+/-5000 8000+/-4000 9000+/4000 Grossalpha(dry) -1700+/-5000 1600+/-6000 300+/-6000 Genna Isotopic h 54 20+/-30 190+/60 13+/-20 Co-58 30+/-50 50+/-10 0+/-30 Co-60 40+/-40 3390+/-110 17+/-30 Cs-134 40+/-50 40+/-60 18+/-20 Cs-137 90+/-30 2940+/-90 50+/-20 K-40 16100+/-900 7500+/-600 0000*/-600 8
Ra-226 4 500+/-40 370+/-40 210+/-20 Pb-214 *a 410+/-70 360+/-90 180+/-50 81-214 8a 500+/-70 H0+/-100 240+/-50 Il-208 8a 490+/-100 200+/-130 190+/-80 Ac 228 e a 450+/-130 160+/-200 260+/-100
- a - The naturally occurring radioisetepes Ac-228 and TI-208 are froe the Thorium 232 decar series.
Ra-226 Pb 214, and 81-214 are from the Uraqiwe-238 decay series.
Isotopes other than those reported weae not detected.
LAC 8#R data Collection Cate 01/06/87 Ot/st/if 08/06/87 i Type bottos sed, bettes sed. bottoa sed. <
Location upstreat discharge downstreat Analysis Grossbeta(dry) NA NA NA l reossalpha(dry) NA NA NA GeenaIsotopic m-54 26.1+/-l.1 166+/-15 21.6+/-5.2 Co-58 <MCA (MCA <RDA Co-60 <MDA 3470+/-44 (ROA ;
Cs-134 <m0A 77.6+/-12.3 (MOA l Cs-137 69.3+/8.4 1040+/-33 10.4+/-6.5 l in-65 (m0A $91+/-27 (MOA -
l K 40 NA NA NA Ra-226 *a NA NA NA Pb-214 *a NA NA NA i 11-214 *a NA NA NA T1-208 8a NA NA NA Ac-228 8a NA NA HA j
NA - Anal *',1s a not required. '
38
l Table 22. Analysis of milk semples for 1987.
WISCONSIN DIVISION OF HEALTH LACBWR l SECTION OF RADIATION 1987 g MeasurseentsinunitsofpCi/ liter A. Relin - 2.1 siles ht P. Relin - 1.0 miles NE
' N! - Section of Radiation Protxtion data Pedretti - 1.4 alles SE 7
Collection date 01/13/87 02/10/07 03/10/07 04/14/07 05/12/97 04/0!/87 Location P. Aalin Pedretti A. Malin P. Relin Pedretti P. Relin isotoper I-131 -0.2+/-0.1 0.0+/-0.1 0.2+/-0.1 0.0+/-0.1 0.2+/-0.1 0.0+/0.1 La-140 -1+/-6 0+/-6 1+/-6 -1+/-6 -1+/-6 -1+/-7 Cs-134 9+/-7 6+/-6 0+/-t 6+/t 6+/-7 4+/-6 Cs 137 0+/-t 0+/-t 1+/-I 14+/t 3+/-t -1+/-7 K-40 1430+/-100 1400+/-140 156fs+/-190 1370+/-100 1530+/-190 1160+/-170 Sr-90 2.7+/-0.4 4.8+/0.7 2.8+/-0.5 2.2+/-0.7 5.7+/-0.8 3.7+/-0.7 Collection date 07/14/07 08/11/87 09/08/47 10/13/87 11/10/87 12/09/07 Location A. Malin Pedretti A. Malin Pedretti P Relin A. Ralin Isotope:
1-131 -0.1+/-0.2 0.0+/-0.2 -0.1+/-0.2 0.1+/-0,2 0.1+/-0.2 0.4+/-0.2 La-140 2+/t 1+/-l -1+/7 -1+/-7 -1+/-7 1+/-t Cs-134 4+/-6 3+/-6 4+/-7 8+/-l 7+/-7 4+/-7 Cs-137 -1+/10 1+/-t i+/-7 3+/-7 7+/t -1+/-9 K-40 1350+/-110 1330+/-180 1600+/200 1600+/-190 1130+/170 1610+/-110 St-90 3.2+/0.7 4.2+/-0.7 2.3+/-0.5 3.3+/-1.0 1,5+/-0.6 2.2+/-0.6 Isotopes other than those reported ware not detected.
LAC 9 H data Collectiondate 01/13/47 02/10/47 03/10/47 04/14/47 05/12/87 06/09/07 Location P. Ralin Pedretti A. h iin P.Malin Pedretti P. Malin
!setooe:
1-131 (OA (OA <RDA <OA <@A <OA la,La 140 (OA (OA <OA (OA (OA (OA Cs 134 (ROA (MCA (ROA (MOA (ROA (MDA Cs-137 15.5+/-4.6 (NOA (RDA 27.3+/-7.0 II.t+/-5.5 WA K 40 NA NA NA NA NA NA Collectiondate 07/14/47 08/11/87 03/08/87 10/13/47 11/10/87 12/09/47 Location A. Relin Pedretti A. Melin Pedretti P. Relin A. kalin Isotope:
!131 (ROA (OA (OA (OA (OA (OA la140 (OA (OA (OA (OA (OA (OA Co-134 (OA (OA (OA (OA (OA (OA Cs-137 5.6+/-2.8 (OA (OA (OA (44 (OA K 40 NA NA NA hA MA NA NA - Naturally occurring radioisoteres are usually not specifically analyzed for.
39
s Table 23. Analysis of food product samples for 1987, WISCONSIN DIVISION OF HEALTH LAC 8WR SECTION OF RADIATION PROTECTION 1987 4
ReasurementsinunitsofpCi/kilogree(set) I
, WI - Section of Radiation Protection data 1
Collection Date 09/02/17 09/01/87 Type food product food product Location Schroeder Pedretti Analysis Gross beta 3100+/-300 700+/-2100 Gross alpha 0+/-200 -1200+/-3000 Ganaa Isotopic Be-7 -5+/50 -20+/-120 K-40 2420+/-150 2100+/300 Co-58 -1+/-l l+/-14 Co-60 -1+/8 2+/-15 ZP-t$ -t3+/-16 -5+/-30 l-131 -4+/-10 4+/-JD Cs-134 -7+/l -3+/-13 Cs-137 -1+/-l 10+/-15 Isotopes other than those reported were not detected.
1 LAC 4WR date J
Collection Date 09/02/47 09/01/87 Type food product food oroduct Location Schroeder Pedretti Analysis Gross alpha NA NA Gross beta NA NA Geena Isotopic Be-7 NA NA K-40 NA NA Co-58 (OA <E/
Co-60 <EA <MA 3 IP-l! (OA <cA I-131 (OA <OA
- i Cs-134 <CA (MA
- Cs 137 <cA <cA NA - The isotope was not specifically analy m for.
40
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