ML20203B868

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Annual Environ Operating Rept,1985
ML20203B868
Person / Time
Site: Davis Besse Cleveland Electric icon.png
Issue date: 12/31/1985
From: Williams J
TOLEDO EDISON CO.
To: James Keppler
NRC OFFICE OF INSPECTION & ENFORCEMENT (IE REGION III)
References
1-628, NUDOCS 8604180275
Download: ML20203B868 (64)


Text

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EDISON Docket No. 50-346 JCE WrwAMs. JR Sww vce Aresdert-hrear (4'9]243 2300 License No. NPF-3 la's m sm t Serial No. 1-628 April 1, 1986 Mr. James G. Keppler Regional Administrator Region III United States Nuclear Regulatory Commission 799 Roosevelt Road Glen Ellyn, IL 60137

Dear Mr. Keppler:

Under separate cover, we are transmitting two (2) copies of the 1985 Annual Environmental Operating Report for the Davis-Besse Nuclear Power Station Unit No. 1. This report is submitted in accordance with Section 6.9.1.10 of the Davis-Besse Operating License Appendix A Technical Specifications, (n') Very truly yours, G! W:JSW:yml enclosure i cc: ) James M. Taylor, Director i Office of Inspection and Enforcement ' Unfted States Nuclear Regulatory Commission Washington, D. C. 20555 (20 copies) Learned W. Barry, Director Office of Resources Management United States Nuclent Regulatory Co= mission Washington, D. C. 20555 (2 copies) Harold Denton, Director Office of Nuclear Reactor Regulation United States Nuclear Regulatory Commission Washington, D. C. 20555 (1 copy) DB-1 NRC Resident Inspector [ p Davis-Besse Nuclear Power Station ( 1 copy)

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l REPORT I T0 i TOLED0 EDIS0N COMPANY - ) TOLEDO, OHIO I OPERATIONAL I RADIOLOGICAL ENVIRONMENTAL MONITORING FOR THE DAVIS-BESSE NUCLEAR POWER STATION UNIT NO. 1 OAK HARBOR, OHIO i ANNUAL REPORT - PART I l {

SUMMARY

AND INTERPRETATION JANUARY - DECEMBER 1985 ] 2 FOR SUBMITTAL TO THE NUCLEAR REGULATORY COMMISSION . PREPARED AND SUBMITTED l BY

TELEDYNE ISOTOPES MIDWEST LABORATORY i PROJECT NO. 8003 l

i , , i Approved by: s , ey LL4jS/ut l I L. G. Huebner j General Manager 3 February 1986 4 f i

I b l 1 iO I PREFACE The staff of Teledyne Isotopes Midwest Laboratory was responsible for the acquisition of the data presented in this report. Samples were collected by members of the staff of the Davis-Besse Nuclear Power Station and by local sample collectors. i The report was prepared by L. G. Huebner, General Manager, Teledyne Isotopes Midwest Laboratory. He was assisted in this report preparation by the staff members of Teledyne Isotopes Midwest Laboratory. i i i

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2 3.2-11 4 I'

iO l > l TABLE OF CONTENTS Page, No. 3.2-11 PREFACE . . . . . . . . . . . . . . . . . . . . . . . . . . Li s t of F i gure s . . . . . . . . . . . . . . . . . . . . . . 3.2-iv 3.2-v Li s t of Tabl es . . . . . . . . . . . . . . . . . . . . . . . 3.2-1

1.0 INTRODUCTION

3.2-2

2. 0 EXECUTIVE SUM ARY . . . . . . . . . . . . . . . . . . . . . ,

i I ENVIRONMENTAL RADIOLOGICAL MONITORING PROGRAM . . . . . . . 3.2-3 l 3.0 , 3.1 Methodology. . . . . . . . . . . . . . . . . . . . . . 3.2-3  ; l l 3.1.1 The Air Program . . . . . . . . . . . . . . . . 3.2-3 3.1.2 The Terrestrial Program . . . . . . . . . . . . 3.2-4 l 3.1.3 The Aquatic Program . . . . . . . . . . . . . . 3.2-6 3.1.4 Program Execution . . . . . . . . . . . . . . . 3.2-7 l 3.1.5 Census of Milch Animals . . . . . . . . . . . . 3.2-7 j 3.2 Results and Discussion . . . . . . . . . . . . . . . . 3.2-8 I 3.2.1 Atmospheric Nuclear Detonations . . . . . . . . 3.2-9 3.2.2 The Air Environment . . . . . . . . . . . . . . 3.2-9 3.2.3 The Terrestrial Environant . . . . . . . . . . 3.2-10 3.2.4 The Aquatic Environment . ........... 3.2-13 3.2.5 Summary and Conclusions . . . . . . . . . . . . 3.2-15 FIGURES AND TABLES. . . . . . . . . . . . . . . . . . . . . 3.2-16 4.0 3.2-31

5. 0 REFERENCES. . . . . . . . . . . . . . . . . . . . . . . . .

APPENDIX Interlaboratory Comparison Program Results . . . . . . A-1 A. l i I l 3.2-1ii L

1 1 { !6 i 4 LIST OF FIGURES l No. Caption g

4-1 Sampling locations on the site boundary of the Davis-J Besse Nuclear Power Station. . . . . . . . . . . . . . 3.2-17 l

j 4-2 Sampling locations (except those on the site periphery), j Davis-Besse Nuclear Power Station. . . . . . . . . . . 3.2-18 1 4 ] 1 I t i i i O a 3.2-fv s

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I d l a i i l LIST OF TABLES l i i No. Title pg. } j 4.1 Sampling Locations, Davis-Besse Nuclear Power Station, i Unit No. 1 . . . . . . . . . . . . . . . . . . . . . . 3.2-19 i j 4.2 Type and Frequency of Collections . . . . . . . . . . . . . 3.2-22 1 .! 4.3 Sample Codes Used in Table 4.2. . . . . . . . . . . . . . . 3.2-23 i j 4.4 Sampling Sumary ..................... 3.2-24 4.5 Environmental Radiological Monitoring Program Sumary . . . 3.2-25 i i 1 1 1 r i 1 i l t 3.2-v i I-- - - - _ _ _ _ _ _ _ _

f i l l

1.0 INTRODUCTION

Because of the many potential pathways of radiation exposure to man from both natural and man-made sources, it is necessary to document levels of radio-activity and the variability of these levels which exist in an area prior to the anticipated release of any additional radioactive nuclides. l To meet this objective, an extensive preoperational environmental radiological monitoring program was initiated for the Toledo Edison Company in the vicinity of the Davis-Besse Nuclear Power Station site. This program included collec-tion (both onsite and offsite) and radiometric analyses of airborne particu-lates, airborne iodine, ambient gamma radiation, milk, groundwater, meat and O wildlife, fruits and vegetables, animal and wildlife feed, soil, surface water, fish, and bottom sediments. Approximately 5 years of preoperational monitoring were completed in April 1977 by the same laboratory that currently operates under the name Teledyne Isotopes Midwest Laboratory (TIML). Fuel elements were loaded in Unit 1 on 23 through 27 April 1977 and the  ; initial criticality was achieved on 12 August 1977. Unit 1 achieved one ' hundred percent of its operational capacity on 4 April 1978. Approximately 8-1/2 years of operational monitoring was completed by the end of December I 1985. l This report presents the eighth full year of operational data for the Environ-mental Radiological Monitoring at the Davis-Besse Nuclear Power Station. The program was conducted in accordance with the Davis-Besse Nuclear Power Station Unit No.1 Technical Specifications: Appendix A to License No. NPF-3, Section 3/4.12.1. Appendix A to License No. NPF-3, Section 3/4.12.1 super-ceded Apendix B to License No. NPF-3, Section 3.2 on October 30, 1985. O 3.2-1

V 1 l l

2. 0 EXECUTIVE SINMARY Operational Nuclear Stations are required by Federal Regulations to submit Annual Operational Reports to the U.S. NRC. The reports must also include the results of the Radiological Environmental Monitoring Program.

This report sumarizes the results of such a program. The program was conduc-ted in accordance with the Davis-Besse Nuclear Power Station Unit No.1 Technical Specifications: Appendix A to Licerde No. NPF-3, Section 3/4.12.1. Appendix A to License No. NPF-3, Section 3/4.12.1 superceded Appendix B to License No. NPF-3, Section 3.2 on October 30, 1985. This program included collection (both onsite and off site) and radiometric analyses of airborne O particulates, airborne iodine, ambient gamma radiation, milk, ground water, meat and wildlife, fruits and vegetables, animal and wildlife feed, soil, surf ace water, fish, and bottom sediments. Results of sample analyses during the period January - December 1985 are summarized in Table 4.5. Tabulations of data for all samples collected during this period, additional statistical analyses of the data, and graphs of data trends are presented in a separate report to the Toledo Edison Company (TIML 1986). Radionuclide concentrations measured at indicator locations were compared with levels measured at control locations and in preoperational studies. The comparisons indicate background-level radioactivities in all sanples collected. No station effect on the environment was indicated in any of the sampling media collected and analyzed. O 3.2-2

O 3.0 ENVIRONMENTAL RADIOLOGICAL MONITORING PROGRAM 3.1 Methodology The sampling locations for the Environmental Radiological Monitoring Program at the Davis-Besse Nuclear Power Station are shown in Figures 4-1 and 4-2. Table 4.1 describes the locations, lists for each its direction and distance from the station, and indicates which are indi-cator and which are control locations. The sampling program monitors the air, terrestrial, and aquatic environ-O ments. The types of sagles collected at each location and the fre-quency of collections are presented in Table 4.2 using codes defined in Table 4.3. The collections and analyses that comprise the program are described in the following pages. Finally, the execution of the program in the current reporting annual period (January - December 1985) is discussed. 3.1.1 The A;r Program Airborne Particulates The airborne particulate samples are collected on 47m diameter membrane filters of 0.8 micron porosity at a volumetric rate of approximately one cubic foot per minute. The filters are collected weekly from eleven locations (T-1. T-2, T-3, T-4, T-7, T-8, T-9, T-11, T-12 T-23, and T-27), placed in individual glassine protective envelopes, and dispatched by mail to TIML for radiometric analyses. The filters are stored at least five days af ter collection to allow for decay of' naturally-occurring short-lived radionuclides and then analyzed for gross beta activ-ity. The quarterly composites of all air particulate sagles from indicator locations (T-1, T-2, T-3, T-4, T-7, and T-8) and of all air particulate samples from control locations (T-9, T-11. T-12 T-23, and T-27) are gama scanned and analyzed for strontium-89 O and -90. 3.2-3

O v Airborne Iodine Each air sampler is equipped with a charcoal trap in-line af ter the filter holder. The charcoal trap at each location is changed _ at the same time as the particulate filter and analyzed f or iodine-131 immediately after arrival at the laboratory. Ambient Gamma Radiation The integrated gamma-ray background from natural radiation is measured with thermoluminescent dosimeters (TLD) . Monthly and quarterly TLDs are placed at thirteen (13) original locations (the eleven air sampling locations and locations T-5 and T-24). On 1 January 1980 eighteen (18) new TLD sangling locations were added to the program. Twelve locations (T T-49) were established at the site boundary ranging in distance from 0.5 mi to 1.2 mi from the stack. Six locations were established at a distance of 3.7 mi to 5.0 mi from the stack. Since about 50% of the outer 5 mi ring is over Lake Erie, only six additional locations were required to cover all sectors on the land. Each shipment of TLDs includes in-transit TL0s which are stored in a shield at the station and returned with the field TLDs af ter their removal. In-transit exposures are measured by the in-transit TL0s and subtracted from the field TLD measurements to obtain their net exposure. 3.1.2 The Terrestrial Program Milk Two-gallon milk samples are collected twice a month during the grazing period (May through October) and monthly during the rest of the year from two indicator locations (T-8 and T-20) and one control location (T-24). The milk samples are analyzed for iodine-131, strontium-89 and -90, calcium, stable potassium, and are gamma scanned. Groundwater One-gallon well water samples are collected quarterly from two indicator locations (T-7 and T-17) and from one control location (T-27). The gross beta activity is determined on the suspended and dissolved solids of each sample. The samples from control location (T-27) and composites f*om indicator locations (T-7 and (' x T-17) are also ganrna scanned and analyzed for strontium-89 and

           -90, and tritium.

3.2-4

O Edible Meat Semi-annually, domestic meat samples (chickens) are collected from one indicator location (T-32) and one control location (T-34) and one representative species of wildlife (muskrat or . raccoon) is collected onsite (T-31). In addition, one Canada i goose and one snapping turtle are collected annually onsite (T-31) or in the site vicinity (T-33). Gamma spectroscopic analysis is performed on the edible portions of each sample. Fruits and Vegetables Semiannually, at least two varieties of. fruits and vegetables are collected from each of the two indicator locations (T-8 and T-25) and from one control location (T-34). The edible portions are gamma scanned and analyzed for strontium-89 and -90. Green Leafy Vegetables Monthly, during the harvest season, green leafy vegetables are collected from one indicator location (T-36) and one control location (T-37). The samples are analyzed for iodine-131. O Should green leafy vegetables from private gardens be unavail-able, nonedible plants with similar leaf characteristics from the same vicinity may be substituted. Animal-Wildlife Feed Animal feed is collected semi-annually fro.n one indicator location (T-8) and one control location (T-34). Cattlefeed is collected during the first quarter and grass is collected during the third quarter. Also, once a year, a sample of smartweed is collected from location T-31 (onsite). Gamma'spgetroscopic analysis is performed on all sanples.  % N . N, s Soil , Once a year, soil samples are.. collected f rom'all el50eo air s sampling locations; six indicator' locations (T21, T-2, T-3,'T-4, T-7, and T-8) and five contrgillocations (T-9, T-11, T-12, T-23, and T-27). Gamma spectroscopic analysis ist performed on'.all samples.

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3.1.3 The Aquatic Program Treated Surface Water Weekly grab samples of treated water are collected at one indi-cator location (T-28, Unit 1 treated water supply, onsite) l and two control locations (T-11 and T-12, Port Clinton and Toledo l filtration plants). The samples from each location are com-posited monthly and analyzed for gross beta activity in dissolved and suspended solids. Quarterly composites from indicator and combined control locations are gamma scanned and analyzed for strontium-89 and -90. Quarterly composites from each location are analyzed for tritium. Untreated Surface Water Weekly grab samples of untreated water from Lake Erie are col-lected from one indicator location (T-3) and one control location (T-11), and weekly composite samples are collected from the second control location (T-12). Samples at Locations T-11 and T-12 are collected from untreated water taps at Port Clinton and Toledo filtration plants, respectively. In addition, monthly composite samples are collected from cne in-plant water supply (T-28, Unit 1 O untreated water supply, onsite). The samples from each location are composited monthly and analyzed for gross beta activity in dissolved and suspended solids. Quarterly composites from com-bined indicator and combined control locations are gamma scanned and analyzed for strontium-89 and -90. Quarterly composites from one control location (T-11) and two indicator locations (T-3 and T-28) are analyzed for tritium. Beginning in June 1984, the frequency of analysis for tritium and gamma-emitting isotopes on samples from Location T-12 was changed from quarterly to monthly. Also, beginning in June 1984, weekly composite samples were collected from an additional location (T-50), composited monthly, and analyzed for tritium and gamma-emitting isotopes. Fish Two species of fish are collected semi-annually from each of two locations in Lake Erie; from one indicator location in the vicinity of the discharge (T-33) and one control location greater than 10 miles from the plant (T-35). The flesh is separated from the bones and analyzed for gross beta and gamma-emitting isotopes. 3.2-6 l .

Bottom Sediments Semi-annually, bottom sediments are collected from three loca-tions in Lake Erie; at two indicator locations, intake (T-29) and discharge (T-30), and at one control location about 5.3 I miles WNW from the plant (T-27). The samples are gamma scanned and analyzed for gross beta and strontium-89 and -90. 3.1.4 Program Execution . Program execution is summarized in Table 4.4. The program was executed as described in the proceding sections with the follow-ing exceptions:

1. There were no gross beta in air particulates nor airborne iodine-131 data from Location T-4 for the periods ending 11-25-85 and 12-02-85 because a calibr~ted a pump was not available.
2. There were no gross beta in air particulate nor airborne iodine-131 data from Location T-9 for the collection period ending 12-02-85 because a calibrated pump was not available.
3. There were no gross beta nor airborne iodine-131 data from Location T-23 for the period ending 07-15-85 because of a pump malfunction.

4 There were no TLD data for Location T-49 for the month of October,1985 because TLDs were lost in the field due to vandalism.

5. Untreated surf ace water from Lake Erie at sita boundary (T-3) was not collected during the month of February of 1985 because the lake was frozen.

3.1.5 Census of Milch Animals In compliance with Appendix B, Section 3.2 of the Technical Specifications for the Davis-Besse Nuclear Power Station, the annual census of milch animals was conducted on May 22, ?3, and 28, 1985 by Environmental Monitoring Group personnel, Davis-Besse Nuclear Power Station. O 3.2-7

O Results The results are shown as follows: Distance - Sector (meters) Animals ESE 21,240 Dairy goat SSE 4,000 Beef cattle 23,500 Dairy goat S 4,420 Beef cattle SSW 3,780 Beef cattle SW 4,740 Beef cattle 11,910 Dairy goat WSW 4,250 Dairy cows 8,100 Beef Cattle 14,480 Dairy goat . W 1,700 Beef cattle WNW 16,580 Dairy goat 3.2 Results and Discussion The results for the reportir.g period January to December 1985 are presen-ted in sunnary form in Table 4.5. For each type of analysis of each sampled medium, this table shows the annual mean and range for all indicator locations and for all control locations. The location with the highest annual mean and the results for this location are also given. The discussion of the results has been divided into three broad cate-

;          gories; the air, terrestrial, and aquatic envivironments. Within each category, samples are discussed in the order listed in Table 4.4.

Any references to previous environmental data for the Davis-Besse Nuclear Power Station refer to data collected by TIML (or its predecessor com-panies, Hazleton Environmental Sciences, NALC0 Environmental Sciences and Industrial BIO-TEST Laboratories, Inc.). The tabulated results of all measurements made during 1985 are not included in this section, although references to these results are made in the discussion. The complete tabulation of the results is submitted to the Toledo Edison Company in a separate report.

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3.2-8

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t O 3.2.1 Atmospheric Nuclear Detonations There were no reported atmospheric nuclear tests in 1985. The last reported test was conducted by the People's Republic.of China on 16 October 1980. The reported yield was in the 200 3 kiloton to 1 megaton range. 1 3.2.2 The Air Environment Airborne Particulates Gross beta measurements yielded annual means that were nearly identical at the five control locations and the six indicator locations (0.024 pCi/m3 and 0.022 respectively). The highest annual mean (0.027 pCi/m3) pCi/m3, was measured at the control location (T-23). i A spring peak in beta concentration had been observed almost annually for many years (Wilson et al., 1969). It had been attributed to f allout of nuclides from the stratosphere (Gold et al., 1964). It was pronounced in 1981 and occured to a lesser degree in 1982. However, the ,neak did not occur in 1983, 1984, or 1985. This was similar to the years 1976 and 1979. Strontium-89 and strontium-90 concentrations were below their respective LLDs of 0.005 and 0.001 pCi/m3 in all samples. Gamma spectroscopic analysis of quarterly composites of air particulate filters yielded similar results for indicator and control locations. The only gamma-emitting isotope detected was beryllium-7 which is produced continously in the upper atmosphere by cosmic radiation ( Arnold and Al-Salih, 1955). There was no indication of a station effect on the data. Airborne lodine Weekly levels of airborne iodine-131 were below the lower limit of detection (LLD) of 0.07 pCi/m3 in all samples with the following exceptions due to low volume resulting from power loss or pump malfunction: T-9 on 11-04-85 (<0.58); T-9 on 11-11-85 (<0.15); T-12 on 10-07-85 (<0.23); T-23 on 02-25-85 (<0.16); T-23 on 12-09-85 (<0.17); and T-23 on 12-23-85 (<0.14). 3.2-9

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Ambient Gamma Radiation At thirteen (13) regular locations the monthly TLDs measured a mean equivalent dose of 12.8 mR/91 days at the indicator locations and a mean of 14.4 mR/91 days at control locations. These results were in agreement -with the values obtained by quarterly TLDs and were similar to the levels observed in 1984 (11.6 mR/91 days and 13.0 mR/91 days, respectively). The highest annual means for monthly TLDs (18.8 mR/91 days) and for quarterly TLDs (19.6 mR/91 days) occured at indicator location T-8. At twelve special locations established at the site boundary, the mean equivalents were essentially identical to those measured at the regular indicator locations (13.8 mR/91 days and 14.1 1 mR/91 days, monthly and quarterly, respectively). Higher gama radiation levels measured at locations away from l the lake were also observed in previous years and are attributed to the higher potassium-40 content in the soil.

   ^              The annual mean dose equivalent for all locations measured by
 ;                monthly and quarterly TL0s was 14.4 mR/91 days and was similar to that measured in 1980 (14.5 mR/91 days),1981 (14.8 mR/91 days),1982 (14.5 mR/91 days),1983 (13.2 mR/91 days), and 1984 (13.2 mR/91 days). This is lower than the estimated average natural background radiation for Middle America,19.5 mrad / quarter which is based on data on Pages 71 and 108 of the report " Natural Background Radiation in the United States" (National Council on Radiation Protection and Measurements, 1975).                   The terrestrial absorbed dose (uncorrected for structural and body shielding) ranges f rom 35 to 75 mrad / year and averages 46 mrad / year for Middle America.       Cosmic radiation and cosmogenic radionuclides contribute 32 mrad / year for an average of 78 mrad / year or 19.5 mrad / quarter.

3.2.3 The Terrestrial Environment Milk i A total of 54 analyses for iodine-131 in milk were performed

during the reporting period. All samples contained less than 0.5 pCi/l of iodine-131. l Strontium-89 was below the LLD levei of 2.0 pCi/l in all samples.

O 3.2-10 1

      - - - - - -          -      - . ~       __

lO Strontium-90 activity was detected in all samples collected and ranged f rom 0.7 to 2.8 pCi/1. The annual mean value for strontium-90 was slightly lower at the indicator locations than at ' the control locations (1.3 and 1.6 pCi/1, respectively). The location with the highest mean (1.6 pCi/l) was control -location T-24. The mean values were similar to those measured in 1977 } through 1984.

)

The concentrations of barium-140 and cesium-137 were below their ' respective LLDs in all sagles collected. f ] 1 Results for potassium-40 were similar at control and indicator locations (1270 and 1320 pCi/1, respectively). Indicator location T-20 had the highest mean (1350 pCi/1). \ Since the chemistries of calcium and strontium, and potassium.

!                  and cesium are similar, organisms tend to deposit ' cesium-137 in muscle tissue and strontium-89 and -90 in bones.       In order to i                  detect potential environmental accumulation of these radio-nuclides, the ratios of the strontium-90 activity to the weight of calcium and of the cesium-137 activity to weight of stable l                 potassium were monitored in milk. The measured concentrations of calcium and stable potassium were in agreement with previously l

determined values of 1.1610.08 g/l and 1.50f0.21 g/1, respectively

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(National Center for Radiological Health,1968). No statistically significant variations in the ratios were observed. j Groundwater (Well Water)

'                   Gross beta concentrations in suspended solids were below the LLD of 1.3 pCi/1 in all samples but one. The detected concentration
!                  was barely above the LLD level (1.4 pCi/1). Gross beta concentra-            l l

{ tions in dissolved solids averaged 3.2 pCi/1 at the indicator l locations and 2.8 pCi/l at the control location. The location with the highest annual mean was the indicator location T-17 and l averaged 3.3 pCi/1. The range of gross beta concentrations were j similar to those observed in 1978 through 1984. 4 I

 !                  Tritium concentration was below the LLD of 330 pCi/1 in all sag les.

i Strontium-89 and strontium-90 concentrations were below their respective LLDs of 2.0 pCi/l and 1.0 pCi/1 in all samples. } l 3.2-11

f% , V All samples were below the LLD of 10.0 pCi/l for cesium-137 concentration. The activities detected in well water were not significant when _ compared with the LLDs and were not attributable to the station operation. Edible Meat In the edible meat samples (chickens, muskrat, Canada goose, and snapping turtle) the mean potassium-40 concentration was 2.69 pCi/g wet weight for the indicator locations and 2.33 pCi/g wet weight for the control location. Cesium-137 concentration was below the LLD of 0.062 pCi/g wet weight in all samples. 1 Fruits and Vegetables Strontium-89 was below the LLD of 0.067 oCi/g wet weight in all samples. Strontium-90 was detected in eleven of sixteen samples and ranged from 0.002 to 0.032 pCi/g wet weight. The only gamma-emitting isotope detected was naturally-occurring potassium-40. The mean concentrations were 2.51 pCi/g wet weight for the indicator locations and 1.72 pCi/g wet weight for the control locations. The concentrations detected were identical or i similar to those detected in 1977 through 1984. All other gamma- l emitting isotopes were below their respective LLDs. . 1 1 Green Leafy Vegetables Green leafy vegetables (cabbage) collected during harvest season  ! were analyzed for iodine-131. All results were below the LLD of 0.039 pCi/g wet weight. All gamma-emitting isotopes except potassium-40 were below their respective LLDs. Potassium-40 concentration averaged 3.85 pCi/g wet weight and 2.07 pCi/g wet weight for indicator and control locations, respectively. No station effect was indicated. Animal-Wildlife Feed In grass, smartweed, and corn the only gama-emitting isotope detected was potassium-40. The annual mean K-40 concentration for the control location T-34 was 3.69 pCi/g wet weight compared to m the mean value of 4.37 pCi/g wet weight for indicator locations. All other gamma-emitting isotopes were below their respective LLDs. 3.2-12

i lO i Soil l i Soil samples were collected in June and November 1985 and ana-i lyzed for gamma-emitting isotopes. The predominant activity was potassium-40 which had a mean value of 15.1 pCi/g dry weight at-the indicator locations and 15.9 pCi/g dry weight at the control  :

locations. Cesium-137 concentration was above the . LLD of 0.12 pCi/g in. seven of the eleven samples. The mean concentration at the indicator locations were 0.31 pCi/g dry weight and 0.72 pCi/g
dry weight at the control locations. The highest cesium-137
concentration, 1.29 pCi/g, was detected at the control location  ;

T-9, 6.8 miles SW of station. The level of concentrations and l i distribution pattern was very similar to those observed in 1978 4 through 1984. 3.2.4 The Aquatic Environment , 4 Water Samples - Treated i l In treated water samples the gross beta activity in suspended j solids was below the LLD of 0.9 pCi/1 in all samples. The mean i gross beta concentration in dissolved solids was identical ! at indicator and control locations (2.2 pCi/1). The values are

similar to those measured in 1975 through 1984. Tritium activity was below the LLD of 330 pCi/1 in all sanples.

j Strontium-89 and strontium-90 concentrations were below the LLD levels of 1.4 pCi/1 and 0.9 pCi/1, respectively, in all samples. Cesium-137 level was below the LLD of 10 pCi/1 in all samples. Similar results were obtained in 1979 through 1984. t Water Samples - Untreated ,

In untreated water samples, ' the mean gross beta concentration in suspended solids averaged 2.1 pCi/l at - indicator locations and j 1.1 pCi/l at control locations. In dissolved solids the mean concentration was identical at -both indicator and control loca- I tions (3.0 pCi/1). For total residue, the mean concentrations 4 were 3.4 pCi/1 at indicator locations and .3.1 pCi/1 at control locations. None of these results show statistically significant differences between indicator and control locations.

1 The tritium concentration was below LLD of 330 pCi/1 in all but ! one sample. The detected concentration of. 360 pCi/l was barely above the LLD level and statistically is not significant.

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l Strontium-89 concentration was below the LLD of 2.0 pCi/l in all samples. Strontium-90 was detected in four of eight samples and the concentration was near the LLD level of 0.8 pCi/l ranging from 0.8 to 1.0 pCi/1. Cesium-137 concentration was below the LLD of 10.0 pCi/l for all locations. No plant effect was indicated. Fish The mean gross beta concentration in fish muscle was similar for l indicator and control locations (2.57 and 2.82 pCi/g wet weight, respectively). The predominant gamma-emitting isotope detected was naturally-occurring potassium-40. The mean potassium-40 concentration was i 2.82 pCi/g wet weight for the indicator location and 3.07 pCi/g wet weight for the control location. Cesium-137 concentration was i below the LLD level of 0.022 pCi/g wet weight in all samp?es but one. The detected concentration was 0.027 pCi/g wet weight, barely above the detection limit. The levels of concentra-tions were similar to those observed in 1978 through 1984. O No plant effect was indicated. Bottom Sediments , The mean gross beta concentration in bottom sediments was 30.5 pCi/g dry weight for indf cator locations and 16.6 pCi/g dry weight for the control location. The location with the highest mean was indicator Location T-30 (31.8 pCi/g dry weight). Indicator Location T-29 had the highest mean potassium-40 concentration l (17.0 pCi/g dry weight) which was the major contributor to the i gross beta activity at all locations. Concentrations of strontium-89 and strontium-90 were below the LLD levels of 0.038 and 0.009 pCi/g dry weight, respectively, in all samples. Cesium-137 concentration was not detected in any of the six samples above the LLD level of 0.054 pCi/g dry weight. Similar I levels, distribution, and composition of detected radionuclides l were detected in 1978 through 1984. O 3.2-14 , 1

O U 3.2.5 Summary and Conclusions Results of sigle analyses during the period January - December 1985 are sumarized in Table 4.5. Tabulations of data for all l samples collected during this period, additional statistical 4 analyses of the data, and graphs of data trends are presented in j a separate report to the Toledo Edison Company (TIML 1986). Radionuclide concentrations measured at indicator locations were compared with Irvels measured at control locations and in pre-operational stuaies. The comparisons indicate background-level radioactivities in all samples collected. No station effect on the environment was indicated in any of the sampling media collected and analyzed. 1 I 1 l O 3.2-15

_ m u--4,m.- _ . , ..s.m .- a A. ---4a --a .-a.a- . .i.a a a _ ._- ..-ea_ m as s.A.. __, m., - ._ - a.a- .. _ --a -.A

                                                                                                                                                                                                                                                               . a- a 4    am-  _e.A--

h I l l I 4 4.0 FIGURES AND TABLES 5 l t J l j 3.2-16

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O O O I

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Figure 1. Sampling locations on the site periphery of the Davis-Besse Nuclear Power Station.

O O O

                                                                                                          -                                                            v.

North Boss id\. x 7 h ' p/  ;;,. . , , 12 - Middle Boss 1. e , a g I Toledo WOregon y . . .

                                            ,                                                                    .                            S mi.                        23 I                                        ,' 27                                                                 5 South Boss 1.        .                                    I I                             [.     ' Kelleys I

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                                                                                                                               -{

Figure 2. Sampling locations (excepting those on the site periphery), Davis-Besse Nuclear Power Station, Unit No. 1.

Table 4.1 Sampling locations, Davis-Besse Nuclear Power Station, Unit No.1. Type of Code Locationa Location Description

T-1 I Site boundary, 0.6 miles NE of station, near intake canal.

T-2 I Site boundary, 0.9 miles E of station. T-3 I Site boundary,1.4 miles SE of station, near Toussaint River and storm drain. T-4 I Site boundary, 0.8 miles S of station, near Locust j Point and Toussaint River. 1 1 T-5 I Main entrance to site, 0.5 miles W of station. 3 T-7 I Sand Beach, 0.9 miles NNW of station.

, T-8         I         Earl Moore Farm, 2.7 miles WSW of station.

^ l T-9 C Oak Harbor, 6.8 miles SW of station. i T-11 C Port Clinton, 9.5 miles SE of station. T-12 C Toledo Water Treatment Station, airborne particulate i and iodine collected 23.5 miles WNW of station and water samples taken from Intake Crib 11.25 miles NW of station.

! T-17        I         Irv Fick's well oasite, 0.7 miles SW of station.

T-20 I Gaeth Farm, 5.5 miles WSW of station. l T-23 C Put-In-Bay Lighthouse,14.3 miles ENE of station. T-24 C Sandusky, 24.9 miles SE of station. 4 T-25 I Miller Farm, 3.7 miles S of station. T-27 C Magee harsh, 5.3 miles WNW of station. T-28 I Unit 1 treated and untreated water supply, onsite. T-29 I Lake Erie, intake area,1.5 miles NE of station. T-30 I Lake Erie, discharge area, 0.9 miles ENE of station. 3.2-19 i i . . _ _ _ . . _ _

1 i O Table 4.1 Sampling locations, Davis-Besse Nuclear Power Station, Unit No.1 (continued) Type of Code Locationa Location Description

T-31 I Onsite.

T-32 I land, within 5 miles radius of station. j T-33 I Lake Erie, within 5 miles radius of site. l T-34 C Land, greater than 10 miles radius of site. T-35 C Lake Erie, greater than 10 miles radius of site. T-36 I The private garden or farm having the highest X/Q. T-37 C The farm 10 to 20 miles from the site in the least prevalent wind direction. l i T-38 I Site boundary, 0.6 ENE of station near lake. T-39 I Site boundary, 1.2 miles ESE of station near ditch to Toussaint. T-40 I Site boundary, 0.7 miles SE of station near ditch to Toussaint. T-41 I Site boundary, 0.6 miles SSE of station near ditch to Toussaint. T-42 I Site boundary, 0.8 miles SSW of station by ECC. T-43 I Site boundary, 0.5 miles SW of station along Route 2 fence. T-44 I Site beundary, 0.5 miles W of station by railroad tracks. T-45 I Site boundary, 0.5 miles WNW of station on access road behind cooling tower. T-46 I Site boundary, 0.5 miles NW of station along access road. i T-47 I Site boundary, 0.5 miles N of station along access road by gate.

3.2-20 ,

d l Table 4.1 Sampling locations, Davis-Besse NQclear Power Station, Unit No. 1 (continued) 1 Type of Code Locationa Location Description T-48 I Site boundary, 0.5 miles NNE of station by lake. T-49 I Site boundary, 0.5 miles NE of station along access road by lake. T-50 I Erie Industrial Park, 4.5 miles ESE of station by Water Tower. T-51 I Daup Farm, 600 Tettau Road, Port Clinton, Ohio 4 4.5 miles SSE of the station. T-52 I Miller Farm, 3.7 miles S of site on West Camp Perry Western Road. 4 T-53 I Nixon Farm, 4.5 miles SSE of site on West Camp Perry j Western Road. l T-54 I M. Beier Farm, 4.8 miles WSW of site on Genzman Road T-55 I King Farm, 5 miles west of site on Route 2. a I = indicator locations; C = control locations. i f i O j 3.2-21

O O O Table 4.2. Type and frequency of collection. 1 Sampling j Location Type Weekly Monthly Quarterly Semi-Annually Annually 1 I AP AI TLD TLD SO 2 I AP Al TLD TLD S0 3 I AP Al SWU TLD TLD SO 4 I AP Al TLD TLD S0 5 I TLD TLD i 7 I AP Al TLD a TLD WW b c SO 8 I AP AI TLD M TLD VE AF SO 9 C AP AI TLD TLD S0 11 C AP Al SWU SWT TLD TLD S0 12 C AP Al SWU SWT TLD TLD S0 17 I a WW 20 I M

!" 23 C AP AI TLD a

TLD SO

        ?                      24                               C                                              TLD M        TLD b

M 25 I VE 27 C AP Al TLD TLD WW BS 50 28 I SWU SWT 29 I BS 30 I BS 31 I WL SMW

32 I ME d

33 I F WF ST b c ! 34 C ME VE AF , 35- C F 36 I GLVc 37 C GLV 38-55 I TLD TLD 50 I SWU Semi-monthly during the grazing season, May through October. Two varieties from each locatioa 4 c Cattlefeed collected during the ist quarter, grass collected during 3rd quarter. Two species from each location. e

l }

)

Table 4.3. Sanple codes used in Table 4.2. Code Description l i i AP Airborne Particulate AI Airborne Iodine / TLD(M) Thermoluminescent Dosimeter - Monthly 1 TLD(Q) Thermoluminescent Dosimeter - Quarterly f j M Milk i WW Well Water (Ground Water) t ME Domestic Meat l

i VE Fruits and Vegetables

) GLV Green Leafy Vegetables AF Animal Feed (silage, grain, grass) l SMW Smartweed

;                                                 SWT                                                                  Surf ace Water - Treated SWU                                                                  Surf ace Water - Untreated i                                                 F                                                                    Fish 1

BS Bottom Sediments 50 Soil I i WL Wildlife (muskrat or raccoon) i j ST Snapping Turtle l

 ;                                                WF                                                                   Water fowl (goose) l l

l l0

3.2-23 J

i

O O I O Table 4.4 Sampling summary. Collection Number Number of Number of Sample Type and of Samples Samples Type Frequency a Locations Collected Missed Remarks Air Environment Airborne particulates C/W 11 568b 4 See text, Page 3.2-7 Airborne iodine C/W 11 568b 4 See text, Page 3.2-7 TLDs C/M 31 371 1 C/Q 31 124 0 Terrestrial Environment Milk (May-Oct) G/SM 3 36 0 (Nov-Apr) G/M 3 18 0 Groundwater G/Q 3 12 0 Edible Meat

a. Domestic meat G/SA 2 4 0
b. Wildlife (two species) G/SA 1 2 0
c. Waterfowl G/A 1 1 0
d. Snapping Turtle G/A 1 1 0

[ a Fruits and Vegetables (two G/SA 3 16 0 varieties from each location) Green leafy vegetables (during G/M 2 9 0 harvest season) Animal-wildlife feed

a. Cattlefeed G/A 2 -

2 0 Collected 1st Q

b. Grass or corn G/A 2 2 0 Collected 3rd Q
c. Smartweed G/A 1 1 0 Soil G/A 11 11 0 Aquatic Environment Treated surface water G/WM 3 156b 0 Untreated surface water G/WM 2 100b 4 COMP /WM 2 104b o COMP /M 1 12 0 Fish (twospecies) G/SA 2 8 0 Bottom sediments G/SA 3 6 0 a Type of collection is coded as follows: C/ = continuous; G/ = grab; COMP / = composite. Frequency is coded as follows: /WM = weekly composited monthly; /W = weekly; /SM = semi-monthly; /M = monthly; /Q = quarterly,
        /SA = semi-annually; /A = annually.

b Saraples are sent to laboratory weekly.

[

                                                                                                                                                        '%/

f\j Table 4.5 Environmental Radiological Monitoring Program tannary. hoe of Facility Davis-desse Nuclear Power $tation 00cket feo. 50-346 Location of Facility uttawa. Unto Heporting Period January - Ncemoer 1985 (Lounty, State) I Indicator Location witn reignest .cntrol Type and LoCattons enual Mean Locations Ascer ut Sant> le Type Amber of Mean (F)c Mean g) Mean (F) hon-rout ine Analyses * , LL0b dangeC Locationd Wange kange Mesults* (units) T-23, Put-in-tsay 0.021 (42/51) 0.024 (222/258) 0 i Airborne Gtt 568 0.009f 0.022 (306/310: ' Particulates (0.009-0.060) 14. 3 at Eht (0.008-0.045) (0.009-0.ub9) (pC t /m3) 0.005 (LLD - (LLu o Sr-89 8 - Sr -90 8 0.001 (LLD - - (LLD U 65 8 0.010 0.003 (4/4) NA9 - 0.u59 (4/4) 0 Be-7 ' (0.052-0.071) (0.042-0.073) ta K -40 0.0067 (LLD - - <LLu J { 0.0003 (LLD - <LLO O $ 70-95 - Zr -95 0.0011 (LLD - - (LLu J  ! Hu-103 0.0008 <tLD - - <LLD 0 Ra-106 0.0036 (LLU - - <LLD o Cs-134 0.00u4 <tL D - - (LLu a Cs-137 0.0004 <tLD - - <LLu J Ce -141 0.0009 <LLD - - (LLu 0 0.0020 <ttD - - (LLD 0 . Ce-144 t 0.07" (LLD - <Lto 0 Ai r t.orne I-131 568

      !Odine                                                                                                                                                                                                                                 I (pCi/m3)

TLD (Monthly) Gsana 156 1. 0 12.8 (84/84) T-8, Earl Moore Fars 18.8 (12/12) 14.4 ( 72/ 72) u (md/91 days) ( 8. 0-22. 9 ) 2. 7 mi w5d (16.1-24.9) (8.2-19.o) T-8, f arl Moore Fare 19.6 (4/4) 15.9 (24/24) o TLD (OJarterly) Giama 52 1. 0 13.8 (28/28) (mH/91 days) ( 9. 2-21. 5) 2. 7 :s1 wsw (18.7-21.5) (11.4-20.1)

A b C\ ld , Table 4.5 Environmental Radiological Monitoring Program Sunenary (continued)

                                     ' lame of Facility         Davis-Besse Eclear Power Station                           Docket No.                                 50-346 Location of Facility                          Ottawa, Ohio                              Reporting Period January - December 1985 (County, State)

Ir.dicator Location with Highest Control Sample Type and Locations Annual Mean Locations beer of Type Nunber of Mean (F)C Mean (F) Mean (F) Non-rcut ine Analysesa LLDb RangeC Locationd Range Range kesultse (Units) ' TLD (Monthly) Gamma 143 ' l.0 13.8 (143/143)

                                                                                                           -45, Site boundary                  20.0 (12/12)                          None              0 (mR/91 days)                                                        (6.1-26.7)                 0.5 mi WNW                          (16.6-26.7)

(Inner Ring i Site Boundary) TLD (@arterly) Gama 48 1. 0 14.1 (48/48) T-45, Site boundary 20.4 (4/4) None i 0 i i (mR/91 days) ( 7. 3-23.1) 0.5 mi WW (17.3-23.1) (Inner Ring Site Boundary) ' l 0 TLD (Monthly) Gansna 72 1. 0 16.2 (72/72) T-50. Erie Industrial 17.2 (12/12) None . 4 (mR/91 days) (9.7-26.5) , Park, 4.5 mi ESE of (13.5-20.8) t (Outer Ring, app. ' Station by Water i 5 mi distant) l Tower 3 w i T-50, Erie Industrial

  • TLD(@arterly) Gama 24 1. 0 17.7(24/24) - 20.3 (4/4) None f G (mR/91 days) (13.2-22.4) Park, 4.5 mi ES8. of (19.3-21.5) l m. l' Station by Water i N (Outer Ring, app.
  • Tower , l 5 mi distant) l L

Milk (pC1/1) 1-131 54 0. 5 (LLD ,

                                                                                                                                            !          -                             (LLD              0 Sr-89      54    2. 0              <LLD           4
                                                                                                                 -                                     -                             <LLD              0
                                             ;Sr-90       54    0. 5            1.3(36/36) !            T-24. Tof t's Dairy                    1.6 (14/18)                     1.6 (18/18)             0                !

(0.7-2.8)  ; 24.9 al SE (1.0-2.2) (1.0-2.2) GS 54 I K-40 100 1320 (36/36) i T-20, Gaeth Farm 1350 (18/18) 1270 (18/18) 0 (1050-1480) 5.5 mi WSW (1050-1480) (1170-1460) Cs-137 10 <LLD -. - <LLD 0 ) 84-140 10 (LLD - - (LLD 0 (g/1) Ca 54 0. 5 0.9 (36/ 36) T-8. E. Moore Farm , 0.9 (18/18) 0.9 (18/18) 0 ( 0. 6-1. 2) , 2.7 al WSW (0.6-1.2) (0.7-1.2) T-20, Gaeth Farm 0.9 (18/18) 5.5 mi WSW (0.6-1.1) T-24, Tof t's Dairy 0.9 (18/18) 24.9 mt SE (0.7-1.2) K 54 0.04 1. 5 (36/ 36) T-20 Gaeth Farm 1.5 (18/18) 1.4 (18/18) 9 0 I 3 1 (stable) (1.2-1.1) 5.5 mi WSW (1.2-1.7) (1.3-1.6) (pCi/q) Sr-90/Ca 54 0.5 1. 5 ( 36/ 36 ) T-24. Tof t's Dairy 1.8 (18/18) 1.8 (18/18) 0 (0. 7- 3. 5) 24.9 al SE (1.0-2.3) (1.0-2.3) (pti/q) Cs-137/K 54 8.3 <LLD - - (LLD 0

O O O Table 4.5 Environmental Radiological Monitoring Program Sumrury (continued) itw of Facility 0 avis-Besse Nuclear Power Station Docket No. 50-346 Location of facility Ottawa, Ohio Reporting Period January - December 1985 (Lounty, State? Indicator Location with Highest Control Sample Type and Locations Annual Mean Locations Nunt>er of Type Number of Mean (F)c Mean (F) Mean (f) Non-routine Analyse 5 8 LLDb RangeC Locationd Range Range Resultse (tini ts ) T-17. Erv Fick's Well 1.4 (1/4) <LLD 0 Well Wau- lGB(55) 12 1. 3 1.4 (1/4) (pC t /1) j

                                                                                   -        0.7 ml SW                                                                      -

AG8 (DS) 12 1.0 3.2 (8/8) T-l?, Erv Fick's Well 3.3 (4/4) 2.8 (4/4) 0 (2.8-4.1) 0.7 mi SW (2.8-4.1) (1.0-5.2) l l l GB (TR) 12 3.4 (8/8) T-17 Erv Fick's Well 3.6 (4/4) 2.8 (4/4) . 0 (2.8-4.8) 0.7 ml SW (2.8-4.8) (1.0-5.2) H-3 12 330 <tLD - - <tLD 0

                       ;Sr-89           8     2. 0                    (LLD                          -                                                                      -             ,     <LLD                 0 8     1. 0                     (LLD                         -                                                                      -                   (LLD                 0 fSr-90
  • F i GS 8 f

ra Cs-137 10.0 (Lt D - - (LLD 0 I' 4 N Edible Meat GS 8  ; I K-40 0.1 2.69 (6/6) T-31, Onsite 3.64 (2/2) ' 2.33 (2/2) 0 (1.13-4.42) 0.6 mi NE (2.86-4.42) (2.25-2.40) I 0 Cs-137 0.062 (LLD - - <LLD Sr-89 0.067 (LLD - <LLD 0 Fruits and 16 - Vegetables 0 ' * (pCi/g wet) Sr-90 16 0.002 0.009 (7/11) T-25 Miller Farm 0.012 (4/5) 0.002 (4/5) (0.002-0.032) 3.7 mi 5 (0.002-0.032) (0.002-0.003) l G5 16 K-40 0.50 2.51 (11/11) T-8, > bore Farm 2.54 (6/6) 1.72 (5/5) 0 (1.11-5.19) 2.7 mi W5W (1.11-4.99) (0.92-2.70) , Nb-95 0.030 <tLD - - <LLD  ! O j (LLD 0 I Zr-95 0.050 (LLD - - { 0.24 <LLD - - <LLD 0 Ru-106 Cs-137 0.034 <LLD - - <LLD  ; O 0.047 (LtD - - <tLD 0 Ce-141 0.20 <t LD - <LLD 0 Ce-144 -

_ _ . _ _ . _ . _ _ _ _ _ _ . _ _ _ . . _ _ . _ _ _ _ _ _ _ ____._.. _ _. _ ______ _ m_ _ _. ._.___m _ . . . _ _._ _ _ _ _ _ _. _ 1 O Table 4.5 Environmental Radiological Monitoring Program Sununary (continued) Name of Facility Davis-Besse Nuclear Power Station Docket No. 50-346 Location of Facility Ottawa, Ohio Reporting Period January - Decenter 1985 (Lounty, State) Indicator Location with Highest Control .: Sam le Type and Locations Annual Mean Locations N aber of i Type Number of Mean (F)c Mean (F) Mean (F) Non-routine (tInits) Analysesa LLDb p3ngec Locationd Range Range Resultse

]

Green Leafy I-131 9 0. 0 39 <tLD - - (LLD 0 9 Vegetables I  ; j (pC1/g wet) GS 9  ! 4 i - l K-40 0.1 3.85 (4/4) T-36, Miller Farm  ! 3.85 (4/4) 0 3.7 at S (3.21-4.81)

f. 2.07 (5/5)

(1.42-2.51) (3.21-4.81) , 1 Nb-95 0.028 <tLD - - <tLD  ! 0 i i Zr-95 0.050 <Lt D - - <LLD u , i Cs-131 0.033 <t L D - - (LLD tl 0 i w

        *                                                                                                                                                                                                                                                          ]

Ce-141 0.052 <tLD - - , <tLD O m , 0.23 (LLD h 4 Ce-144 <LLD - - O j ,  ; I N.imal-Wildlife i GS 5  ; Feed i  ; j (pCl/g wet) Be-1 0.31 . 0.45 (1/3) T-31, Onsite 0.45 (1/1) 3

                                                                                                                                                                                                                                                      <tLD         l             0               t 0.6 mi NE                               ,

i K-40 0.1 4.37 (3/3) T-31, Onsite 4.90 (1/1) , 3.69 (2/2) O  ; l t (2.69-5.51) 0.6 mi NE I - (2.56-4.81) I i 4

                        ,                               i 1                              I Nb-95                                                             0.040         <LL D                                     -                                          -                       <LLD                       0    [

I I Zr-95 0.063 <tLD - - <LLD  ! 0 f 0.036 <LLD - - (LLD 0 4 fRu-103 l 1 t Ru-106 0.35 <tLD '- - <LLD 0 i t Cs-131 0.041 (LLD - - i <LLD 0

                                                                                                                                                                                                                                              +

4 Ce-141 0.062 <LLD - - j (LLD 0 ,

                                                                                                                                         <tLD                                                                                                          (LLD                      0    I Ce-144                                           0.29                                                    -                                          -               6 Soil                                    GS                                                    11 (pCi/g dry)

Be-7 3.61 <LLD - - <tLD 0 K-40 1.0 15.1 (6/6) T-9 Oak Harbor 25.9 (1/1) 15.9 (5/5) 0 4 ( 5. 9-25. 5 ) 6.8 mi SW  ; ( 7. 0-25.9 ) Zr-95 0.65 <t L D - - (LLD 0 Nb-95 1.17 <LLD - - (LLD 0 _ _ _ _ _ .m.-3 -

                                                                                                                                                                                                                                                                                            -3

f'] Q N b Table 4.5 Environmental Radiological Monitoring Program Surinary (continued) Name of Facility Davis-Besse Nuclear Power Station Docket No. 50-346 Location of Facility Ottawa, Ohio Reporting Period January - December 1985 (County, State) l l Indicator Location with Highest Control Sample Type and ' t Locations Annual Mean Locations Nurrber of Type Number of Mean (F)C , Mean (F) Mean (F) Non-rout i ne (Units) Analyses 8 ' LLDb RangeC i .Locationd Range Range , Resultse i 1 i ' 5011 l Ru-103 O.074 <tt D - - <LLD 0 ' (pCi/g dry) f (cont'd) [ Ru-l% 1.16 <L t D - j

                                                                                                                                                           -                    <LLD                   0
                        ; Cs-137                               0.12                              0.31 (2/6)           T-9, Oak Harbor       l1.29(1/1)                      0.72'(5/5)                 0 (0.31-0.31)           6.8 mi SW                           -

(0.31-1.29) Ce-141 1.75  ; <LLD -

                                                                                                                                                           -                    <LLD                   0
                                                                                                                                            '                                                          0 Ce-144                             0.80                                <t L D                  -                               -                    (LLD w    Treated Surface        GB (SS) 36                          0. 9                          ;     <tLD                    -                               -                    <LLD            l      0 Water                                                                                   }                                               l                                                  l I

rv (pCi/l) GB (05) 36 1.0 , 2.2 (12/12) f ( 1. 3-2. 8) T-il, Port Clinton 9.5 mi SE 'l 2.3 ( 1. 7-(12/12)

3. 4 )

2.2 (24/24) (1.3-3.4) 0 GB (TR ) 36 1.0 2.2 (12/12) T-II, Port Clinton 2.3 (12/12) 2.2 (24/24) 0 9.5 mi SE ' I i (1.3-2.8) i ( 1. 7-3. 4 ) (1.3-3.4) < 9 H-3 12 330 ' <t L D - - (LLD 0 i , 1 Sr-89 8 1.4  ! <t L D . - j - (LLD 0  ! t

                                                                                                                                             '                                                                    l Sr-90                        8      0. 9                                (LL D                   -                               -                    (LLD                   0
                                                                                                                                             !                                                                    I
                        ' GS                            8                                    l                    I
                                                                                                                                              '                                                        0 Cs-137                            10.0                                 rLLD                    -                               -                    (LLD l

tintreated Surf ace ! G8 (SS) 47 0. 9 2.1 (4/23) T-3, Lake Erie Site i 2.1 (4/11) 1.1 (4/24) 0 Water . (1,1-3.8) Boundary, 1.4 mi SE (1.1-3.8) (0.9-1.3) , (pct /1)  ! G8 (DS) 47 1.0 3.0 (23/23) T-3, Lake Erie Site 3.2 (!!/11) 3.0 (24/24) 0 (1.7-4.9) Boundary, 1.4 al SE (2.1-4.9) (2.0-5.6) GB (TR) 47 1.0 l 3.4 (23/23) T-3, Lake Erie Site 4.0 (12/12) 3.1 (24/24) 0 l (1. 7-8. 7) Boundary, 1.4 at SE ' ( 2.1 -8. 7 ) (2.0-5.6) H-3 36 j330 <t L D T-12, Toledo Water , 360 (1/12) 360 (1/12) 0 . Intake,11.25 mi NW - - Sr-89 8 2. 0 <LtD - - (LLD 0

(-. tU) (w./ ) (v) Table 4.5 Environmental Radiological Monitoring Program Sumary (continued) Name of Facility Davis-Besse Nuclear Power Station Docket No. 50-346 Location of Facility Ottawa, Ohio Reporting Period January - December 1985 (County, State) Indicator Location with Highest Control Sanple Type and Locations Annual Mean Locations Nuntjer of Type Number of Mean (F)c Mean (F) Mean (F ) Non-routine (Units) Analysesa Ltob Rangec Location 1 Range Range Results* Untreated Surf ace Sr-90 8 0. 8 1.0 (3/4) NAi 1.0 (3/4) 0.8 (1/4) 0 l Water (pCl/1) (0.6-1,3) 0.6-1.3 - 1 I GS 32 i l , I l Cs-133 10 (LLD - - <t L D i 0 l t l Tish GB 8 0.1 , . 57 (4/4) . T-35, Lake Erie 2.82 (4/i) 2.82 (4/4) . 0 (pCi/g wet) l (1.20-3.50) i 15 mi NE (2.44-3.15) (2.44-3.15) i GS 8 i K-40 0.1 2.82 (4/4)  ! T-35, Lake Erie 3.07 (4/4) 3.07 (4/4) 0

                                                                                          ;  (2.43-3.38)     i        15 mi NE                                   (2.94-3.19)         (2.94-3.19)

F Cs-137 0.022 (LLD l T-35, Lake Erie 0.027 (1/4) , 0.027 (1/4) j 0 15 mi NE 7 , j j - O 6 1. 0 30.5 (4/4) T-30, Lake Erie 31.8 (2/2) 16.6 (2/2) I O Bottom Sediments l GB l l Discharge I (pCi/q dry) i (26.2-37.2)  ; (26.2-37.3) (14.4-18.8) 8 6 0.9 mi WNW , I . Sr-89 6 0.0 38 <LLD

                                                                                                                          -                                           -                 (LLD       !        O Sr-90                    6                         0.009         0.030 (3/4)             T-30. Lake Erie,                            0.041 (1/4)            <tLD                0 0.013-0.041              Discharge                                       -                                              i 0.9 mi WNW GS                       6 K-40                               0.1            16.0 (4/4)              T-29, Lake Erie                             17.0 (2/2)          9.2 (2/2)      l       0 (14.4-18.4)              Intake                                     (15.5-18.4)         (4.6-13.8)     l j

1.5 mi NE Cs-137 0.054 (LLD - - (LLD 0 a I G8 = gross beta, GS = gama scan SS = suspended solids 05 = dissolved solids, TR = total residue. b LLD = nominal lower limit of detection based or. 4.66 sigma counting error for background sample. C Mean based upon detectable acasurements only. Fraction of detectable measurements at spectfled locations is indicated in parentheses. (F). . d '

     ' Locations are specified by station code (Tible 4.1) and distance (miles) and direction relative to reactor site.

Non-routine results are those which exceed ten times the control station value. I Two results (<0.053 and <0.020) have been excluded in the determination of the LLD for gross beta in airborne particulates. The elevated L 9 )LDs f resulted f rom low volame.4arterly composites of all samples fron indicator locations and all samples from control locations were gama scanned to location with the highest annual mean cannot be identified. h Six results (<0.16, <0.23, <0.58, <0.15, <0.17, and <0.14) have been excluded in the determination of the LLD of airbcrne iodine-131. i-

      ' (The elevated LLDs resulted from apparent ramp malfunction or low volume.)iarterly composites of two control locatinns and two indicator location cannot be identified.

i I, e 9

                                                                                ~
5. 0 REFERENCES ,

Arnold, J. R. and H. A. Al-Salih. 1955. Beryllium-7 Produced by Cosmic Rays. Science 121: 451-453. Gold, S., H. W. Barkhau, B. Shlein, and B. Kahn. 1964. Measurement of Naturally Occurring Radionuclides in Air, in the Natural Radiation Environment, University of Chicago Press, Chicago, Illinois, 369-382. Hazleton Environmental Sciences, 1979. Operational Environmental Radio-logical Monitoring for the Davis-Besse Nuclear Power Station, Oak Harbor, Ohio, Annual Report, January-December 1978. , 1980. Operational Environmental Radiological Monitoring for the Davis-Besse Nuclear Power Station, Oak Harbor, Ohio, Annual Report, January-December 1979. 1981. Operational Environmental Radiological Monitoiing for the Davis-Besse Nuclear Power Station Unit No.1, Oak Harbor', Ohio, Final Report - Part II, Data Tabulations and Analyses. January-December 1980. 1982. Operational Environmental Radiological Monitoring for the Davis-Besse Nuclear Power Station Unit No. 1, Oak Harbor, Ohio, Final Report - Part II, Data Tabulations and Analyses. January-December 1981. 1983. Operational Environmental Radiological Monitoring for the Davis-Besse Nuclear Power Station Unit No.1, Oak Harbor, Ohio, Final Report - Part II, Data Tabulations and' Analyses. January-December 1982. Industrial BIO-TEST Laboratories, Inc. 1976. Pre' operational and Operational ' Monitoring for the Davis-Besse Nuclear Power Station, Oak Harbor,' Ohio, Annual Report, January - December 1975. NALC0 Environmental Sciences. 1977. Preoperational and Operational Ridio-logical Monitoring for the Davis-Besse Nuclear Power Station, Oak Harbor, Ohio, Annual Report. January-December 1976. 3.2-31 l a _.

4

                    . 1978. Preoperational and Operational Radiological Monitoring for the Davis-Besse Nuclear Power Station, Oak Harbor, Ohio, Annual Report, January - December 1977.

National Center for Radiological Health. 1968. Section 1. Milk and Food. Radiological Health Data and Reports. Vol. 9, November 12, 730-746. National Council on Radiation Protection and Measurements. 1975. Natural Radiation Background in the United States. NCRP Report No. 45, pp. 71 and 108. Teledyne Isotopes Midwest Laboratory. 1984. Operational Environmental Radiological Monitoring for the Davis-Besse Nuclear Power Station Unit No.1, Oak Harbor, Ohio, Final Report - Part II, Data Tabulations and Analyses. January-December 1983.

                    . 1985. Operational Environmental Radiological Monitoring for the Davis-Besse Nuclear Power Station Unit No.1, Oak Harbor, Ohio, Final Report - Part II, Data Tabulations and Analyses.      January - December 1984.
                    . 1986. Operational Environmental Radiological Monitoring for the Davis-Besse Nuclear Power Station Unit No.1, Oak Harbor Ohio, Final Report - Part II, Data Tabulations and Analyses.      January - December 1985.

Wilson , D. W. , G. M. Ward, and J. E. Johnson. 1969. In: Environmental Contamination by Radioactive Materials, International Atomic Energy Agency, p.125. s O , 3.2-32

                             ,-2
                                                      ~.       ,

e.

                                                                         -h
                                        \                    s Appendix A Interlaboratory Comparison Program Results k

m t

                                                                              's A-1

V Aopendix A Interlaboratory Comparison Prooram Results Teledyne Isotopes Midwest Laboratory (formerly Hazleton Environmental Sciences)  ! has participated in interlaboratory comparison (crosscheck) programs since the formulation of its quality control program in December 1971. These programs are operated by agencies which supply environmental-type samples (e.g., milk or water) containing concentrations of radionuclides known to the issuing agency but not to participant laboratories. The , purpose of such a program is to provide an independent check on the laboratory's analytical procedures and to alert it to any possible problems. Participant laboratories measure the concentrations of specified radionuclides and report them to the issuing agency. Several months later, the agency reports the known values to the partic.ipant laboratories and specifies control limits. Results consistently higher or lower than the known values or outside the control limits indicate a need to check the instruments or procedures used. The results in Table A-1 were obtained through participation in the environ-O mental sample crosscheck program for milk, water, air filters, and food samples during the period 1982 through October 1985. This program has been conducted by the U. S. Environmental Protection Agency Intercomparison and Calibration Section, Quality Assurance Branch, Environmental Monitoring and Support Laboratory, Las Vegas, Nevada. The results in Table A-2 were obtained for thermoluminescent dosimeters (TLD's) during the period 1976, 1977, 1979, 1980, and 1981 through parti-cipation in the Second, Third, Fourth, and Fif th International Intercomparison of Environmental Dosimeters under the sponsorships listed in Table A-2. A-2

[ U Table A-1. U.S. Environmental Protection Agency's crosscheck program, com-parison of EPA and Teledyne Isotopes Midwest Laboratory results for milk, water, air filters, and food samples,1982 througn 1985.a Concentration in pCi/lb Lab Sample Date TIML Result EPA Result Code Type Collected Analysis i2ac 3c, n=1d STW-270 Water Jan. 1982 Sr-89 24.312.0 21.0t5.0 Sr-90 9.410.5 12.011.5 STW-273 Water Jan. 1982 I-131 8.610.6 8.4tl.5 STW-275 Water Feb. 1982 H-3 1580*147 1820t342 STW-276 Water Feb. 1982 Cr-51 <61 0 Co-60 26.0t3.7 20i5 Zn-65 <13 1515 Ru-106 <46 20t5 Cs-134 26.810.7 22i5 Cs-137 29.7tl.4 23i5 STW-277 Water Mar. 1982 Ra-226 11.9 1.9 11.6tl.7 STW-278 Water Mar. 1982 Gross alpha 15.6 1.9 1915 Gross beta 19.210.4 1915 STW-280 Water Apr. 1982 H-3 2690180 28601360 STW-281 Water Apr. 1982 Gross alpha 75i7.9 85t21 Gross beta 114.li5.9 106t5.3 Sr-89 17.411.8 2415 Sr-90 10.5 0.6 12il.5 Ra-226 11.412.0 10.911.5 Co-60 <4.6 0 STW-284 Water May 1982 Gross alpha 31.516.5 27. 5t7 Gross beta 25.9t3.4 29 5 STW-285 Water June 1982 H-3 1970 1408 1830i340 STW-286 Water June 1982 Ra-226 12.611.5 13.413.5 Ra-228 11.li2.5 8.7t2.3 STW-287 Water June 1982 I-131 6.510.3 4.410.7 STW-290 Water Aug. 1982 H-3 32101140 28901619 O A-3

1 O Table A-1. (continued) Concentration in pCi/lb Lab Sample Date TIML Result EPA Result Code Type Collected Analysis 12cc i3o, n=ld STW-291 Water Aug. 1982 I-131 94.6t2.5 87t15 STW-292 Water Sept. 1982 Sr-89 22.7t3.8 24.5i8.7 Sr-90 10.9i0.3 14.Si2.6 STW-296 Water Oct. 1982 Co-60 20.011.0 20i8.7 Zn-65 32.315.1 24i8.7 Cs-134 15.3tl.5 19.0i8.7 Cs-137 21.0il.7 20.0i8.7 STW-297 Water Oct. 1982 H-3 2470i20 25601612 STW-298 Water Oct. 1982 Gross alpha 32i30 55124 Gross beta 81.716.1 8118.7 Sr-89 <2 0 Sr-90 14.110.9 17.212.6 Cs-134 <2 1.8t8.7 22.7i0.6 20t8.7 O Cs-137 Ra-226 Ra-228 13.6i0.3 3.9tl.0 12.Si3.2 3.610.9 STW-301 Water Nov. 1982 Gross alpha 12.0il.0 19.018.7 Gross beta 34.0i2.7 24.018.7 STW-302 Water Dec. 1982 I-131 40.010.0 37.0i10 STW-303 Water Dec. 1982 H-3 1940i20 1990i345 STW-304 Water Dec. 1982 Ra-226 11.7*0.6 11.0il.7 ' 0 Ra-228 <3 l STW-306 Water Jan. 1983 Sr-89 20.0i8.7 29.2i5 Sr-90 21.7i8.4 17.2il.5 STW-307 Water Jan. 1983 Gross alpha 29.014.09 29.0 13 Gross beta 29.3t0.6 31.0i8.7 STM-309 Milk Feb. 1983 Sr-89 35i2.0 37i8.7 Sr-90 13.7i0.6 18t2.6 I-131 55.7t3.2 55i10.4 Cs-137 2911.0 26t8.7 Ba-140 <27 0 K-40 1637i5.8 1512i131 O. A-4

                                                                                                       . _,_--m         _. ~ _ . , , _ , . _ . . , . -     -,c.,

O Table A-1. (continued) , Concentration in pCi/lb Lab Sample Date TIML Result EPA Result Code Type Collected Analysis *2cc i3o,n=1d STW-310 Water Feb. 1983 H-3 2470i80 25601612 STW-311 Water March 1983 Ra-226 11.9tl.3 12.7i3.3 Ra-228 <2.7 0 STW-312 Water March 1983 Gross alpha 31.614.59 31i13.4 Gross beta 27.012.0 28i8.7 STW-313 Water April 1983 H-3 3240i80 3330t627 STW-316 Water May 1983 Gross alpha 9417 64i19.9 Gross beta 13315 149t12.4 Sr-89 1911 2418.7 4 Sr-90 1211 1312.6 Ra-226 7.9 0.4 8.512.25 Co-60 30t2 3018.7 Cs-134 27i2 33i8.7 Cs-137 2911 27t8.7 STW-317 Water May 1983 Sr-89 59.7i2.1 5718.7 Sr-90 33.7tl.5 38i3.3 i STW-318f Water May 1983 Gross alpha 12.8tl.5 1118.7 Gross beta 49.413.9 5718.7 STM-320 Milk June 1983 Sr-89 2010 2518.7 Sr-90 10t1 1612.6 I-131 3011 30t10.4 Cs-137 52 2 4718.7 K-40 1553t57 14861129 l STW-321 Water June 1983 H-3 1470i89 1529tS83 STW-322 Water June 1983 Ra-226 4.310.2 4.8tl.24 i Ra-228 <2.5 0 STW-323 Water July 1983 Gross alpha 3il 718.7 Gross beta 2110 22 8.7 STW-324 Water August 1983 I-131 13.3i0.6 14i10. 4 O A-5

i i (O) Table A-1. (continued) l

                                                                                                                                   )

Concentration in pCi/lb Lab Sample Date TIML Result EPA Result Code Type Collected Analysis t2ac 13o, n=1d  : STAF-326 Air August 1983 Gross beta 42i2 36t8.7 i Filter Sr-90 1412 1012.6 ) Cs-137 1911 15t8.7 ' STW-328 Water Sept. 1983 Gross alpha 2.310.6 518.7 Gross beta 10.7tl.2 9i8.7 STW-329 Water Sept. 1983 Ra-226 3.0i0.2 3.110.81 Ra-228 3.210.7 2.010.52 1 STW-331 Water Oct. 1983 H-3 1300130 1210i570 ] STW-335 Water Dec. 1983 I-131 19.6tl.9 20i10.4 i STW-336 Water Dec. 1983 H-3 2870i100 2389t608 STAF-337 Air Nov. 1983 Gross alpha 18.0t0.2 1918.7 Filter Gross beta 58.611.2 50i8.7 Sr-90 10.910.1 15t2.6 O Cs-137 30.li2.5 20i8.7 STW-339 Water Jan. 1984 Sr-89 47.2tl.9 3618.7 Sr-90 22.514.0 24i2.6 STW-343 Water Feb. 1984 H-3 2487 7,6 2383t607 STM-347 Milk March 1984 I-131 5.311.1 611.6 4.1 1.06 I STW-349 Water March 1984 Ra-226 4.0 0.2

Ra-228 3.610.3 2.0t0.52 ,

STW-350 Water March 1984 Gross alpha 3.811.1 518.7 Gross beta 24.212.0 20i8.7 STW-354 Water April 1984 H-3 3560t50 3508i630 STW-355 Water April 1984 Gross alpha 21.014.1 35t15.2 Gross beta 127.814.1 147i12.7 Sr-89 29.3t2.0 23i8.7 Sr-90 16.6i0.7 26i2.6 Ra-226 4.0il.0 4.0tl.04 Co-60 -32.3tl.4 30t8. 7 Cs-134 33.613.1 30i8.7 Cs-137 33.3t2.2 2618.7 l

O l

A-6

Table A-1. (continued) Concentration in pCi/lb Lab Sample Date TIML Result EPA Result Code Type Collected Analysis f2cc i3c, n=1d STW-358 Water May 1984 Gross alpha 3.010.6 3t8.7 Gross beta 6.711.2 618.7 STM-366 Milk June 1984 Sr-89 21i3.1 2518.7 Sr-90 13 2.0 1712.6 I-131 4615.3 43110.4 Cs-137 3814.0 35i8. 7 ' K-40 1577t172 1496t130 STW-368 Water July 1984 Gross alpha 5.lil.1 618.7 Gross beta 11.9 2.4 13t8.7 STW-369 Water August 1984 I-131 34.3i5.0 34.0i10. 4 STW-370 Water August 1984 H-3 3003t253 28171617 STF-371 Food July 1984 Sr-89 22.015.3 25.Oi8.7 Sr-90 14.7i3.1 20.0t2.6 39.0i10.4 O I-131 Cs-137 K-40

                                                                                              <172 24.015.3 2503i132 25.0i8.7 26051226.0 l                       STAF-372      Air        August 1984         uross alpha            15.3tl.2                            1718.7
Filter Gross beta 56.0t0.0 5118.7 4 Sr-90 14.3 1.2 18t2.4 Cs-137 21.0 2.0 1518.7 STW-375 Water Sept. 1984 Ra-226 5.1 0.4 4.911.27 Ra-228 2.210.1 2.3i0.60 STW-377 Water Sept. 1984 Gross alpha 3.3 1.2 5.0i8.7 Gross beta 12.712.3 16.0i8.7 STW-379 Water Oct. 1984 H-3 2860t312 2810i356 STW-380 Water Oct. 1984 Cr-51 <36 4018.7 Co-60 20.311.2 2018.7 Zn-65 150i8.1 147 8.7 Ru-106 <30 4718.7 Cs-134 31.3t7.0 31i8.7 l Cs-137 26.711.2 2418.7
.O A-7

i Table A-1. (continued) Concentration in pCi/lb Lab Sanple Date TIML Result EPA Result l Code Type Collected Analysis *2 c i3 , n=1d

STM-382 Milk Oct. 1984 Sr-89 15.714.2 22i8.7 j Sr-90 12.7tl.2 1612.6 i I-131 41.7i3.1 42i10.4 i Cs-137 31.3 6.1 32i8.7 K-40 1447166 1517i131 STW-384 Water Oct. 1984 Gross alpha 9.711.2. 14tS. 7 (Blind) Sanple A Ra-226 3.310.2 3.0f0.8 U an um NA8 Sib 4 Samp'le B Gross beta 48.3t5.0 6418.7
Sr-89 10.714.6 1118.7 Sr-90 7.3il.2 12i2.6 Co-60 16.3tl.2 1418.7 Cs-134 <2 218.7 Cs-137 16.7tl.2 14i8.7 STAF-387 Air Nov. 1984 Gross alpha 18.7 1.2 15i8.7

-l O Filter Gross beta Sr-90 Cs-137 59.015.3 18.311.2 10.3*1.2 52 8.7 21*2.6 1018.7 STW-388 Water Dec. 1984 I-131 28.012.0 36110.4 STW-389 Water Dec. 1984 H-3 3583fl10 3182i624 i STW-391 Water Dec. 1984 Ra-226 8.4tl.7 8.612.2 Ra-228 3.110.2 4.lil.1 l

STW-392 Water Jan. 1985 Sr-89 <3.0 3.0i8.7 Sr-90 27.315.2 30.0i2.6 STW-393 Water Jan. 1985 Gross alpha 3.311.2 518.7 Gross beta 17.3i3.0 1518.7

{ STS-395 Food Jan. 1985 Sr-89 25.316.4 34.015.0 Sr-90 27.0i8.8 26.011.5 I-131 38.0i2.0 35.016.0 i Cs-137 32.7*2.4 29.015.0 K-40 14101212 13821120 i i i A-8 i I

                                         . _ . ~        _ . _ _ _ _ _ _ , _ . . . .       .,... __ _._.           . _ . _ _       _ _ _ . _ . _ . . _ . _ _ _

l Table A-1. (continued)

                                                                                                                                                                  ' ^ '

I_ Sample Date Concentration in pCi/lb TIML Result EPA Result Lab Code Type Collected Analysis *2cc i3o, n=1d STW-397 Water Feb. 1985 Cr-51 <29 48i8.7 Co-60 21.3i3.0 20i8.7 l Zn-65 53.7t5.0 55t8.7 Ru-106 <23 2518.7 Cs-134 32.3*1.2 35t8.7  ; 4 Cs-137 25.3i3.0 25i8.7 4 STW-398 Water Feb. 1985 H-3 3869i319 37961634 STM-400 Milk March 1985 I-131 7.312.4 9.010.9 STW-402 Water March 1985 Ra-226 4.6i0. 6 5.011.3 Ra-228 (0. 8 9.0i2. 3 Reanalysis Ra-228 9.0i0.4 STW-404 Water March 1985 Gross alpha 4. L? . . 6t8.7 Gross beta 11.311.2 15t8.7 STAF-405 Air March 1985 Gross alpha 9.311.0 10.0t8.7 Filter Gross beta 42.0il.1 36.0i8.7 Sr-90 13.3tl.0 15.0i2.6 Cs-137 6.311.0 6. 0i8. 7 STW-407 Water April 1985 I-131 8.0i0.0 7.5t1.3 STW-408 Water April 1985 H-3 3399tl50 35591630 STW-409 Water April 1985 a (Blind) Gross alpha 29.7tl.8 32.0t5.0 Sample A Ra-226 4.4i0.2 4.110.6 Ra-228 nae 6.210.9 Uranium nae 7.0t6.0 Sample B Gross beta 74.3111.8 72.0t5.0 Sr-89 12.3t7.6 10.0z5. 0 Sr-90 14.7*2.4 15.011.5 Co-60 14.7*2.4 15.015.0 Cs-134 12.0i2.0 15.0i5.0 Cs-137 14.0i2.0 12.0t5.0 l A-9 1 .

3 Table A-1. (continued) l Concentration in pCi/lb i Lab Sample Date TIML Result EPA Result Code Type Collected Analysis f2 c t3 ,n=1d STW-413 Water May 1985 Sr-89 36.0112.4 39.015.0 Sr-90 14.3i4.2 15.0tl.5 STW-414 Water May 1985 Gross alpha 8.3i4.1 12.0i5.0 Gross 'seta 8.711.2 11.0i5.0 STW-416 Water June 1985 Cr-51 44.7i6.0 44. 0t5. 0 Co-60 14.3tl.2 14.0*5. 0 i Zn-65 50.3i7.0 47. 0t5. 0 Ru-106 55.3i5.8 62.015.0 Cs-134 32.711.2 35.0t5. 0 Cs-137 22.7i2.4 20.0i5.0 STW-418 Water June 1985 H-3 2446i132 2416t351 STM-421 Milk June 1985 Sr-89 10.3 4.6 11.Di8.7 Sr-90 9.012.0 11.0t2.6 ) ! I-131 11.7tl.2 11.0i10.4 ' Cs-137 12.711.2 11.018.7 K-40 1512i62 1525tl32 STW-423 Water July 1985 Gross alpha 5.0 0.0 11.0i8.7 Gross beta 5. 0i2. 0 8.018.7 i STW-425 Water August 1985 I-131 25.7t3.0 33.0i10.4 STW-426 Water August 1985 H-3 4363i83 4480t776 STAF-427 Air August 1985 Gross alpha 11.310.6 13.0i8.7 Filter Gross beta 46.0il.0 44.0i8.7 Sr-90 17.7i0.6 18.0t2.6

                                                                      - Cs-137                               10.3i0.6                                 8. 0i8. 7 STW-429                Water            Sept. 1985               Sr-89                        15.7i0.6                                20.018.7 Sr-90                          7. 0i0. 0                              7.012.6 STW-430                Water            Sept. 1985               Ra-226                         8.210.3                                8.9t2.3 Ra-228                         4. li0. 3                              4.6t1.2 STW-431                Water           Sept. 1985               Gross alpha                    4.7 0.6                                8. 0i8. 7 Gross beta                     4.711.2                                8.0t8.7 i

O A-10

                                     . .._-                          ._                              - ._      - --                 . - - - _ .                       _=                                            ..   . - . -

i t

\ Table A-1. (continued)

Concentration in pCi/lb i Lab Sanple Date TIML Result EPA Result Code Type Collected Analysis f2cc i3o, n=1d 4 STW-433 Water Oct. 1985 Cr-51 <13 21.0f8.7 Co-60 19.30.6 20.0i8.7 Zn-65 19.710.6 19.0i8.7 Ru-106 <19 20.018.7 Cs-134 17.011.0 20.018,7 4 Cs-137 19.3tl.2 20.018.7 STW-435 Water Oct. 1985 H-3 1957tSO 1974i598 l a Results obtained by Teledyne Isotopes Midwest Laboratory as a participant l in the environmental sample crosscheck program operated by the Intercom-l parison and Calibration Section, Quality Assurance Branch, Environmental i Monitoring and Support Laboratory, U.S. Environmental Protection Agency,

b (EPA),

All results Las Vegas, are in Nevada. pCi/1, except for elemental potassium (K) data, which are in mg/1; air filter samples, which are in pCi/ filter; and food, which is in pCi/kg. 4 O c Unless otherwise indicated, the TIML results are given as the mean 12 standard deviations for three determinations. l' d USEPA results are presented as the known values i control limits of 3a for n = 1. e NA = Not analyzed. f Analyzed but not reported to the EPA. 9 Results af ter calculations corrected (error in calculations when reported to

EPA).

j l f t A-11 i

   , , . _ . . . , . . , . _ , , _          _ _ , _ _ _ . _ , _ .       , , , . ,,__,,,.,.<~,,,_y         . , , , . , .       . , .             .,,..y. _ . . , . .      , _ _ . ,,_,,_,,,,,.,,..__.,-._,,,,,,3.,.,_..,

O O O

                                                                                                  ~

Table A-2. Cros: check program results, thermoluminescent dosimeters (TLDs). mR Teledyne Average 12o d-Lab TLD Result Known (4 I Code Type Measurement 12aa Value participants) 2nd International Intercomparisonb 115-2b CaF2:Mn Gansna-Field 17.011.9 17.lc 16.417.7 Bulb Gansna-Lab 20.814.1 21.3C 18.817.6 3rd International Interconparisone 115-3e CaF :Mn Gama-Field 30.713.2 34.914.Gf 31.513.0

    ?              Bu b M                            Gama-Lab                 89.616.4                    91.7114.6f 86.2124.0 4th International Intercomparison9 115-49      CaF :Mn        Gama-Field               14.111'1                    14.lil.4f  16.019.0 i                   Bu b Gamma-Lab (Low)           9.311.3                    12.212.4f  12.017.6 l                                 Gansna-Lab (High)        40.411.4                    45.819.2f  43.9113.2 5th International Intercosparisonh

! 115-5Ah CaF2:Mn Gansna-Field 31.411.8 30.016.01 30.2114.6 Gansna-Lab 77.415.8 . 75.217.61 75.8140.4 at beginning Gansna-Lab 96.615.8 88.418.81 90.7131.2 at the end l

O O O Table A-2. Crosscheck progran results, thermoluminescent dosimeters (TLD5). mR

     ~

Teledyne Average 120 d Lab TLD Result Known (all Code Type Measurement 12aa Value participants) 2nd International Intercomparisonb 115-2b CaF2:Mn Gansna-Field 17.011.9 17.lc 16.417.7 ] Bulb Gamma-Lab 20.814.1 21.3c 18.817.6 3rd International Intercomparisone 115-3e CaF :Mn Gansna-Field 30.713.2 34.914.8f 31.513.0 89.616.4 91.7114.6f 86.2124.0 w Gamma-Lab 4th International Intercomparison9 115-49 CaF2:Mn Gansna-Field 14.111.1 14.lil.4f 16.019.0 BuTb Gansna-Lab (Low) 9.311 3 12.212.4f 12.017.6 Gansna-Lab (High) 40.411.4 45.819.2f 43.9113.2 1 5th International Intercomparisonh CaF :Mn Gansna-Field 31.411.8 30.016.01 30.2114.6 115-5Ah Bu b Gansna-Lab 77.415.8 75.217.61 75.8140.4 at beginning Gaassa-Lab 96.6 5.8 88.418.81 90.7131.2 < at the end

O O O Table A-2. (Continued) i mR Teledyne Average i 20 d Lab TLD Result Known (all Code Type Measurement 12ba Value participants) 115-5Bh LiF-100 Gansna-Field 30.314.8 30.0161 30.2114.6 Chips Gamma-Lab 81.117.4 75.217.61 75.8140.4 at beginning 3 Gamma-Lab 85.4111.7 88.418.8I 90.7131.2 at the end j y a Lab result given is the mean 12 standard deviations of three determinations. i g b Second International Intercomparison of Environmental Dosimeters conducted in April of 1976 by the Health and Safety Laboratory (GASL), New York, New York, and the School of Public Health of the University of Texas, Houston, Texas. c Value determined by sponsor of the intercomparison using continuc,usly operated pressurized ion chas er. d Mean 12 standard deviations of results obtained by all laboratories participating in the program. e Third International Intercomparison of Environmental Dosimeters conducted in summer of 1977 by Oak Ridge National Laboratory and the School of Public Health of the University of Texas, Houston, Texas. i f Value 12 standard deviations as determined by sponsor of the intercomparison using continuously operated pressurized ion chamber. 9 Fourth International Intercouparison of Environmental Dosimeters conducted in senener of 1979 by the School of Public Health of the University of Texas, Houston, Texas. h Fifth International Intercomparison of Environmental Dosimeter conducted in fall of 1980 at Idaho Falls, Idaho and sponsored by the School of Public Health of the University of Texas, Houston, Texas and Environmental Measurements Laboratory, New York, New York, U.S. Department of Energy. I Value determined by sponsor of the intercomparison using continuously operated pressurized icn chaser.

i i i l 1 f i i i i } i 1985 Land-Use and Milk Animal Census { Toledo Edison Company 1 i Davis-Besse Nuclear Power Station l 1

Prepared By
Jane Branum, Environmental Monitoring Group

{ June, 1985 i Reviewed By: A. Gephart J. Scott-Wasilk 4 D. Briden i R. Scott G. Downing 1 1 4 l. J ! I i , g 8 - I l i l l l

~ - - - _                           __ - - . _ . . - - . - - _ _                                                                 _. ... - .                        . - . -. ,.- , -    .-

1985 LAND-USE AND MILK ANIMAL CENSUS O)

 \

v Background and Methods Appendix I, to 10 CFR 50, states "The licensee shall establish an appropri-ate surveillance and monitoring program for evaluating doses to individu-als from principal pathways of exposure." Appendix B, Section 3.2, to the , Davis-Besse Technical Specifications states "an annual census of animals l producing milk for human consumption shall be conducted at the start of ' the grazing season to determine their location and number with respect to the site." Pathways are defined as any means by which radionuclides can i get into the human food chain. Pathways recorded in the Land-Use and Milk Animal Census are residences, vegetable gardens, milk animals, and beef i animals. All the pathway locations must be determined within a five-mile radius of the station vent. All dairy goats within a fifteen-mile radius of the station vent must also be located. The 1985 Land-Use and Milk Animal Census was done on May 22, 23 and 28, 1985. Local agencies, such as the Northwest Ohio Goat Dairyman Associa-tion, and the Ottawa County, Sandusky County, ana Lucas County Cooperative Extension Agencies provided information on dairy goat owners in their areas. l The Ottawa County Cooperative Extension Agency confirmed the presence of ! all beef cattle, milk cows, and milk goats reported within the five-mile radius of the station. The pathway distances listed below are measured l i (Q v j from the station vent. i I The following changes were recorded in the 1985 census: l N Sector - A vegetable garden pathway at 890 meters which was present l last year was not observed at the time of the census.  ; Since no major change had occurred in the area and the l census was taken in early spring, it was assumed that the garden would be planted at a later date and was included in the census. NNE Sector - The vegetable garden pathway at 900 meters which was ! present last year was not observed at the time of the l census. For the same reason as stated above, it was included in the census. ESE Sector - A dairy goat pathway was added at 21,240 meters (13.2 miles). SE Sector - A dairy goat pathway at 18,170 meters (11.3 miles) was deleted since it did not appear on the 1985 dairy goat listing. SSE Sector - The vegetable garden pathway at 2,230 meters was changed to 2,680 meters. A new dairy goat pathway was also added at 23,500 meters (14.6 miles).

   ,O U

1

SSW Sector - The vegetable garden pathway was changed from 1,000 meters to 1,260 meters. SW Sector - The vegetable garden pathway at 990 meters was changed to

1,050 meters. New beef cattle were added to the sector, i changing the beef cattle pathway from 5,050 meters to

! 4,740 meters. WSW Sector - The vegetable garden pathway was changed from 2,590 meters to 1,640 meters. The beef cattle pathway changed from 8,560 meters to 8,100 meters. The dairy goat pathway also changed from 11,100 meters to 14,480 meters i (9.0 miles). This change occurred since a dairy goat at 11,100 meters did not appear in the 1985 dairy goat list. W Sector - The dairy goat pathway at 4,140 meters was eliminated

!                             since it did not appear on the 1985 dairy goat list.

t l WNW Sector - The vegetable garden pathway was changed from 1,730 meters to 2,880 meters. , NNW Sector - The vegetable garden pathway at 1,250 meters was changed to 1,330 meters. Results ] [ ss The results of the 1985 Land-Use and Milk Animal Census are presented in short form in Table 1. The detailed receptor list in Table 2 is used to

                                                                                                   )
                                                                                                   )

update the data file of the Semiannual Radioactive Effluent Release 1 Report. Table 7 is the updated table for Appendix B of the Offsite Dose Calculation Manual (0DCM). The ODCM describes the methodology and ., parameters used in calculating offsite doses due to radioactive liquid and gaseous effluents and in calculating liquid and gaseous effluent j monitoring instrumentation alarm / trip setpoints. The critical receptor

!            of the 1985 Census has not changed from the 1983 and 1984 reports. The
;            vegetable pathway at 900 meters in the NNE sector with X/Qr value of 1.27 E-6 i             and D/Q value of 1.39 E-8 is still the most critical receptor.

Acknowledgements Yvonne Leidorf and Pat McCloskey of the Environmental Monitoring Group assisted in the field work, i i DBP 4307F l

l TABII 1 l l 1 Pathway Identification ) 1 Sector Distance (meters) Receptor  !

\ l N 870 residence 893 residence, vegetable garden **

NNE 870 residence j 900 residence, vegetable garden **  ; NE 900 residence l ENE* - - E* - - ESE 21,240 residence, vegetable garden, dairy goat SE* l SSE 2,030 residence  !

,                                                                      2,680                                  residence, vegetable garden                                                                      !
4,000 residence, vegetable garden, beef cattle
!                                                                   23,500                                    residence, vegetable garden, dairy goat S                                  1,130                                 residence 1,430                                 residence, vegetable garden 4,420                                  residence, vegetable garden, beef cattle SSW                                1,000                                 residence 1,260                                 residence, vegetable garden 3,780                                  residence, vegetable garden, beef cattle SW                                          990                          residence 1,050                                 residence, vegetable garden                                                                      j

, 4,740 residence, beef cattle 11,910 residence, vegetable garden, dairy goat l WSW 1,640 residence, vegetable garden 4,250 residence, vegetable garden, dairy cow < 8,100 residence, beef cattle 14,480 residence, vegetable garden, dairy goat W 980 residence, vegetable garden 1,700 residence, vegetable garden, beef cattle

,                                    WNW                                1,730                                 residence 2,880                                  residence, vegetable garden 16,580                                   residence, vegetable garden, dairy goat NW                                 1,160                                 residence, vegetable garden NNW                                1,330                                 residence, vegetable garden
  • Sectors over Lake Erie and marsh areas.
                                     **The vegetable gardens were not observed at the time of the census. It was assumed that the garden would be planted at a later date and were therefore included in the census.

THE 2 4 Receptor Distance From Site (Meters) SECTOR 1 (N) 870 890* Inhalation 1 1 Contaminated Ground 1 1 l Vegetation 1 i l Cow Milk i { Goat Milk Meat Animal 1 i Plume Exposure 1 1 SECTOR 2 (NNE) 870 900* Inhalation 1 1 Contaminated Ground 1 1 Vegetation 1 Cow Milk Goat Milk Meat Animal Plume Exposure 1 1 ! SECTOR 3 (NE) 900 1

!                      Inhalation                       1                                                    *

! Contaminated Ground 1 Vegetation i Cow Milk j Goat Milk l Heat Animal

}

4 Plume Exposure 1

                       *The vegetable gardens were not observed at the time of the census. It was
assumed that the gardens would be planted at a later date and were therefore i included in the census.

i

f TME 2 i i j Receptor Distance From Site (Meters) 1 ] SECTOR 4 (ENE) - ! Inhalation ' 3 Contaminated Ground i l Vegetation i i Cow Milk ) I Goat Milk l i 1

;                                                       Meat Animal l

j Plume Exposure i SECTOR 5 (E) - Inhalation ! Contaminated Ground ! Vegetation m J Cow Milk Goat Milk

  • i Meat Animal j Plume Exposure i

SECTOR 6 (ESE) 21,240 1 Inhalation 1 1 't Contaminated Ground 1 I a Vegetation 1  ; Cow Milk l l i Goat Milk 1 4 Heat Animal 1 Plume Exposure 1 i

)
)

i i

TABLE 2 l l l Receptor Distance From Site (Meters) l; SECTOR 7 (SE)

!                      Inhalation 3

Contaminated Ground ' Vegetation Cow Milk

;                     Goat Milk                                                                                                                                        1

! Meat Animal Plume Exposure i I I i l SECTOR 8 (SSE) 2030 2680 4000 23,500 l s

                                                                                                                                                                       \

j Inhalation 1 1 1 1 i j Contaminated Ground 1 1 1 1 i j Vegetation 1 1 1 ! Cow Milk j Goat Milk 1 i l Meat Animal 1 j Plume Exposure 1 1 1 1 1 I i SECTOR 9 (S) 1130 1430 4420 i Inhalation 1 1 1

!                     Contaminated Ground                    1         1              1
,                     Vegetation                                       1               1 l

l Cow Milk i

Goat Milk i,

j Meat Animal 1

}                     Plume Exposure                         1         1               1 l

k i i l 4 d, l

TABLE 2 1 Receptor Distance From Site (Meters) SECTOR 10 (SSW) 1000 1260 3780 l Inhalation 1 1 1 i ! Contaminated Ground 1 1 1 Vegetation 1 .1 Cow Milk i I Goat Milk I Heat Animal 1

Plume Exposure 1 1 1 e

1 SECTOR 11 (SW) 990 1050 4740 11910 Inhalation 1 1 1 1 i Contaminated Ground 1 1 1 1 1 Vegetation 1 1 4 1 Cow Milk t Goat Milk 1 Heat Animal 1 Plusae Exposure 1 1 1 1 . i SECTOR 12 (WSW) 1640 4250 8100 14480 1 Inhalation 1 1 1 1 Contaminated Ground 1 1 1 1 Vegetation 1 1 1 Cow Milk 1 , Goat Milk 1 i Heat Animal 1 Plume Exposure 1 1 1 1 l l a i . I i

1 TABLE 2

Receptor Distance From Site (Meters) j 1

SECTOR 13 (W) 980 1700 Inhalation 1 1 i I Contaminated Ground 1 1 I Vegetation 1 1  ! Cow Milk Goat Milk , i Meat Animal 1 l i Plume Exposure 1 1 I i j SECTOR 14 (WNW) 1730 2880 16580 -l ! Inhalation 1 1 1 t

,                                Contaminated Ground                          1                        1        1 4

Vegetation 1 1 ( Cow Milk 1 l Goat Milk 1 1 Meat Animal I i Plume Exposure 1 1 1 SECTOR 15 (NW) 1160 ! Inhalation 1 Contaminated Ground 1 l Vegetation 1 l Cow Milk l 5 Goat Milk I Meat Animal I Plume Exposure 1 b i 4 1

TABLE 2 Receptor Distance From Site (Meters) SECTOR 16 (NNW) 1250 1330 Inhalation 1 1 Contaminated Ground 1 1 Vegetation 1 Cow Milk Goat Milk Meat Animal Plume Exposure 1 1

1 0FFSITE DOSE CALCULATIONS MANUAL TABLE 7, APPENDIX B Controlling Receptor Location Pathways and Atmospheric Dispersion Parameters Distance Sector (ueters) Pathways Age Group X/Qg D/Q N*** 890 vegetation child 8.76E-7 8.24E-9 NNE*** 900 vegetation child 1.19E-6 1.39E-8 NE 900 inhalation child 1.26E-6 1.58E-8 ENE* - - - - - E* - - - - - ESE** 8,000 goat / milk infant 3.65E-8 1.24E-10 SE* - - - - - SSE 2680 vegetation child 7.45E-8 9.38E-10 S 1,430 vegetation child 1.24E-7 2.51E-9 SSW 1,260 vegetation child 1.48E-7 3.27E-9 SW 1,050 vegetation child 2.92E-7 5.33E-9 WSW 4,250 cow / milk infant 5.74E-8 5.36E-10 W 980 vegetation child 6.21E-7 9.58E-9 WNW 2,880 vegetation child 7.25E-8 6.59E-10 NW 1,160 vegetation child 2.40E-7 2.04E-9 NNW 1,330 vegetation child 2.51E-7 1.57E-9 O *Since these sectors are located over Lake Erie, no ingestion pathways are present.

   ** Default value of 8000 meters is over water. This value is used since the actual receptor site of 21,240 meters can not be accurately extrapolated.
 ***The vegetable gardens were not observed at the time of the census. It was assumed the gardens would be planted at a later date and were there-fore included in the census.

1 DBP 4307F l}}