ML062830443

From kanterella
Jump to navigation Jump to search
NAI Report Release, Calculation NAI-1149-001, Revision 0, Primary Coolant Source Term Determination for Palisades Dose Calculations
ML062830443
Person / Time
Site: Palisades Entergy icon.png
Issue date: 06/09/2005
From: George T, Harrell J, Thomasson S
Numerical Applications
To:
Office of Nuclear Reactor Regulation
References
NAI-1149-011, Rev 0
Download: ML062830443 (32)


Text

NAI Report Release Calculation Number: NAI-1149-011 Revision Number: 0

Title:

Primary Coolant Source Term Determination for Palisades Dose Calculations

==

Description:==

The purpose of this calculation is to develop the PCS source term for use in AST dose calculations for Palisades. This source term will meet the 1.0 l~CVgm Dose Equivalent 1-131 and 1001E-bar gross activity limits specified in the Palisades Technical Specifications. In addition, the secondary side source term equal to the Technical Specification limit of 0.1 yCilgm Dose Equivalent 1-131 will be determined.

A&

G. TL b lqor Author Date Steven G. Thomasson 6/=?io Date V James R. Harrell Tom George I

NAI Calculation Approval Calculation Number: NAI-1149-011 Revision Number: 0

Title:

Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation

Description:

The purpose of this calculation is to develop the PCS source term for use in AST dose calculations for Palisades. This source term will meet the 1.0 pCi/gm Dose Equivalent 1-131 and 100/E-bar gross activity limits specified in the Palisades Technical Specifications. In addition, the secondary side source term equal to the Technical Specification limit of 0.1 pCi/gm Dose Equivalent 1-131 will be determined.

A - L G.b clsloc Author Date Steven G. Thomasson

Scope of Review:

Review included:

o A general review of calculation methods was completed for consistency with plant-specific and generic regulatory requirements and guidance.

e ORIGEN computer qualification was verified as appropriate.

e Calc and code inputs and assumptions were verified against IAM document(s).

o References were verified as appropriate.

o Outputs from spreadsheets and utility programs were checked with hand calcs.

e Reported results were verified against computer outputs.

0 Results and conclusions were reviewed for reasonableness.

Design Verification Rev. 0 - See Attachment 1 1: (4 (05 Date James R. Harrell

Check items in the following lists to verify that project documentation and engineering calculations are complete. Mark any items that are not applicable with NIA notation.

Project Documentation Checklist:

o Project QA Plan.

o Project Organization.

o Project Work Scope and Design Plan.

o Project Calculation and Document Index.

o Project QA Requirements.

CI Project Engineer Training and Qualification Forms.

Project QA Training Certification Forms.

o Project Correspondence.

Engineering Calculations Checklist:

d Identification by subject, originator, reviewer, date and Project so that the calculation is retrievable.

Table of contents.

d Statement of the objective of the analysis.

d Analysis inputs and their sources.

d Assumptions and how they were developed or determined.

d Hand calculations.

d Identification of computer calculations, including computer type, computer program name and version, code input and output.

Conclusions.

Review summary.

Responses to review comments.

References.

Each page of the calculation shall be numbered and the first page shall indicate the total number of pages. The calculation pages may be numbered by sections with the first page of the section indicating the total number of pages in the section.

The Calculation Approval Sheet shall be signed and dated by the originator.

Numerical Applications Inc. Page 5 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Table of Contents

1.0 INTRODUCTION

............................................................................................................................ 7 2.0

SUMMARY

OF RESULTS............................................................................................................. 7 3.0 DESIGN INPUT............................................................................................................................... 7 4.0 ASSUMPTIONS............................................................................................................................... 7 5.0 COMPUTER CODES...................................................................................................................... 7 6.0 CALCULATIONS............................................................................................................................ 8 6.1 PRIMARY COOLANT SOURCE TERM................................................................................................. 8 6.2 SECONDARY SIDE SOURCE TERM.................................................................................................. 16

6.3 REFERENCES

................................................................................................................................. 17

Numerical Applications Inc. Page 6 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Attachments Comments on Revision 1...................................................................................... 18 Palisades PCS Activity Nuclide Inventory File (pal_pcs.nif)................................. 19 Tables Table 6-1 Unadjusted Primary Coolant Source Term................................................................... 8 Table 6-2 Primary System D.E. I-131 Determination.................................................................. 10 Table 6-3 Primary System Activities for D.E. I-131 = 1.0 Ci/gm............................................... 10 Table 6-4 Primary System Activities = 100/E-bar........................................................................ 12 Table 6-5 Adjusted Primary Coolant Source Term...................................................................... 15 Table 6-6 Secondary Side Source Term..................................................................................... 16

Numerical Applications Inc. Page 7 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 1.0 Introduction The purpose of this calculation is to develop the PCS source term for use in AST dose calculations for Palisades. This source term will meet the 1.0 Ci/gm Dose Equivalent I-131 and 100/E-bar gross activity limits specified in the Palisades Technical Specifications. In addition, the secondary side source term equal to the Technical Specification limit of 0.1 Ci/gm Dose Equivalent I-131 will be determined.

2.0 Summary of Results The Palisades primary coolant source term is provided in Table 6-5 and the secondary side source term is provided in Table 6-6. The RADTRAD-NAI nuclide inventory file is provided in.

3.0 Design Input The base Palisades primary coolant activities are provided in Table 2 of Reference 1.

4.0 Assumptions The following assumptions were applied to the PCS and secondary side source term determinations:

1. When scaling the total iodine activity to 1.0 Ci/gm D.E. I-131, the relative concentrations of the iodine isotopes are assumed to remain the same.
2. When scaling the non-iodine isotope activities to 100/E-bar, the relative concentrations of the non-iodine isotopes are assumed to remain the same.
3. The relative concentrations of the iodine isotopes on the secondary side are assumed to be the same as the relative concentrations on the primary side.

5.0 Computer Codes No computer codes were required for this calculation.

Numerical Applications Inc. Page 8 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 6.0 Calculations 6.1 Primary Coolant Source Term The primary coolant source term was derived from Table 2 of Reference 1.

The iodine activities from Reference 1 (listed below in Table 6-1) were adjusted to achieve the Technical Specification limit of 1.0 Ci/gm dose equivalent I-131 (see Table 6-3). The non-iodine species were adjusted to achieve the Technical Specification limit of 100/E-bar for non-iodine activities (see Table 6-4). Table 6-5 presents the final adjusted primary coolant source term.

Table 6-1 Unadjusted Primary Coolant Source Term Nuclide Ci/gm Nuclide Ci/gm Co-58 7.0E-03 Np-239 Co-60 8.0E-04 Pu-238 Cr-51 4.7E-03 Pu-239 Fe-55 1.8E-03 Pu-240 Fe-59 4.5E-04 Pu-241 Mn-54 2.4E-03 Am-241 Kr-85 5.3E-01 Cm-242 Kr-85m 1.2E+00 Cm-244 Kr-87 7.5E-01 I-130 1.1E-01 Kr-88 2.2E+00 Kr-83m 3.2E-01 Rb-86 1.5E-02 Xe-138 4.7E-01 Sr-89 5.4E-03 Xe-131m 4.5E-01 Sr-90 4.9E-04 Xe-133m 1.7E+00 Sr-91 1.5E-03 Xe-135m 4.8E-01 Sr-92 5.9E-04 Cs-138 7.0E-01 Y-90 6.4E-04 Cs-134m 4.6E-02 Y-91 1.8E-02 Rb-88 2.3E+00 Y-92 7.2E-04 Rb-89 5.8E-02 Y-93 4.4E-04 Sb-124 1.1E-03 Zr-95 1.2E-03 Sb-125 9.2E-03 Zr-97 4.9E-04 Sb-126 6.2E-04 Nb-95 1.2E-03 Te-131 1.5E-02 Mo-99 4.2E+00 Te-133 6.1E-03 Tc-99m 3.2E+00 Te-134 2.1E-02 Ru-103 1.2E-03 Te-125m 2.0E-03 Ru-105 1.4E-04 Te-133m 1.2E-02 Ru-106 5.3E-04 Ba-141 9.1E-05 Rh-105 5.5E-04 Ba-137m 2.5E+01 Sb-127 4.3E-02 Pd-109 Sb-129 2.4E-02 Rh-106 5.3E-04 Te-127 4.6E-02 Rh-103m 1.2E-03 Te-127m 7.2E-03 Tc-101 1.5E-02 Te-129 3.8E-02 Eu-154 Te-129m 2.2E-02 Eu-155 Te-131m 3.7E-02 Eu-156 Te-132 4.8E-01 La-143 1.1E-05

Numerical Applications Inc. Page 9 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Nuclide Ci/gm Nuclide Ci/gm I-131 5.2E+00 Nb-97 8.1E-05 I-132 1.2E+00 Nb-95m 8.5E-06 I-133 5.4E+00 Pm-147 1.2E-04 I-134 4.7E-01 Pm-148 1.7E-04 I-135 2.3E+00 Pm-149 3.0E-04 Xe-133 7.0E+01 Pm-151 8.3E-05 Xe-135 7.4E+00 Pm-148m 2.6E-05 Cs-134 4.9E+01 Pr-144 9.3E-04 Cs-136 4.3E+00 Pr-144m 1.6E-05 Cs-137 2.6E+01 Sm-153 Ba-139 4.3E-04 Y-94 1.4E-05 Ba-140 7.1E-03 Y-95 8.6E-06 La-140 3.4E-03 Y-91m 8.9E-04 La-141 2.4E-04 Br-82 2.5E-02 La-142 6.8E-05 Br-83 6.6E-02 Ce-141 1.1E-03 Br-84 2.7E-02 Ce-143 6.3E-04 Am-242 Ce-144 9.3E-04 Np-238 Pr-143 1.0E-03 Pu-243 Nd-147 4.3E-04 Per the Palisades Technical Specifications, the primary coolant activity limit is 1.0 /gm Dose Equivalent I-131 and 100/E-bar Ci/gm gross radioactivity.

The definition for DOSE EQUIVALENT I-131 in the current Technical Specifications states that:

DOSE EQUIVALENT I-131 shall be that concentration of I-131 (microcuries/gram) that alone would produce the same thyroid dose as the quantity and isotopic mixture of I-131, I-132, I-133, I-134, and I-135 actually present. The thyroid dose conversion factors used for this calculation shall be those listed in Table III of TID-14844, AEC, 1962, "Calculation of Distance Factors for Power and Test Reactor Sites."

However, a revision is being proposed to this Technical Specification definition that will change the referenced thyroid dose conversion factors to the effective dose conversion factors provided in Table 2.1 of Federal Guidance Report No. 11.

The Tech. Spec. definition of Dose Equivalent I-131 (D.E. I-131) can be represented by the following equation:

D.E. I-131 (Ci/gm) = (ai x DCFi) / DCFI-131 where: ai

= activity of individual isotope (Ci/gm)

DCFi

= effective dose conversion factor for the individual isotope (Table 2.1 of FGR 11, Reference 3)

DCFI-131 = effective dose conversion factor for I-131

Numerical Applications Inc. Page 10 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Table 6-2 provides the determination of the D.E. I-131 for the Table 6-1 iodine activities:

Table 6-2 Primary System D.E. I-131 Determination Isotope Table 6-1 Activity (Ci/gm)

DCFi Activity*DCF I-131 5.20E+00 8.89E-09 4.6228E-08 I-132 1.20E+00 1.03E-10 1.2360E-10 I-133 5.40E+00 1.58E-09 8.5320E-09 I-134 4.70E-01 3.55E-11 1.6685E-11 I-135 2.30E+00 3.32E-10 7.6360E-10 Total 5.5664E-08 D.E. I-131 Total / DCFI-131

=

6.26140 Ci/gm*

  • the numbers in the table are rounded, the actual computation of DE I-131 is performed in a spreadsheet.

Assuming that the relative iodine concentrations would remain the same, the Table 6-2 activities were adjusted by dividing the activities by 6.26140. This gives a D.E. I-131 of 1.0 Ci/gm:

Table 6-3 Primary System Activities for D.E. I-131 = 1.0 Ci/gm Isotope (Table 6-2 Activity / 6.26140)

(Ci/gm)

DCFi Activity*DCF I-131 0.8305 8.89E-09 7.3830E-09 I-132 0.1917 1.03E-10 1.9740E-11 I-133 0.8624 1.58E-09 1.3626E-09 I-134 0.0751 3.55E-11 2.6647E-12 I-135 0.3673 3.32E-10 1.2195E-10 Total 8.8900E-09 DE I-131 Total / DCFI-131

=

1.00 Ci/gm The remaining isotopes in Table 6-1 were adjusted to achieve the Tech. Spec. limit of 100/E-bar microcuries per gram of gross activity. The Tech. Spec. definition of E-bar, Average Disintegration Energy, is:

shall be the average (weighted in proportion to the concentration of each radionuclide in the primary coolant at the time of sampling) of the sum of the average beta and gamma energies per disintegration (in MeV) for isotopes, other than iodines, with half lives > 15 minutes, making up at least 95% of the total noniodine activity in the coolant.

The Tech. Spec. definition of E-bar can be represented by the following equation:

E-bar = [(E i + E I) x ai] / ai where: ai

= activity of individual isotope (Ci/gm)

E i

= average beta emission energy (MeV/dis)

E i

= average gamma emission energy (MeV/dis)

Numerical Applications Inc. Page 11 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Table 6-4 presents the calculations performed to adjust the activities to equal 100/E-bar. In this table, the initial activities were multiplied by a common factor (0.734) so that the total activity equaled 100/E-bar. Values for E i and E I were obtained from Table A.1 of Reference 4.

Isotopes with half lives less than 15 minutes were deleted from the 100/E-bar calculation.

Numerical Applications Inc. Page 12 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Table 6-4 Primary System Activities = 100/E-bar Activity Adjusted Nuclide uCi/gm E-beta E-gamma (E

i + E i) x ai Multiplier Activity (E

i + E i) x ai KR-83M 3.200E-01 0.039 0.003 1.344E-02 0.734 2.349E-01 9.865E-03 KR-85M 1.200E+00 0.255 0.158 4.956E-01 0.734 8.808E-01 3.638E-01 KR-85 5.300E-01 0.251 0.002 1.341E-01 0.734 3.890E-01 9.842E-02 KR-87 7.500E-01 1.324 0.793 1.588E+00 0.734 5.505E-01 1.165E+00 KR-88 2.200E+00 0.364 1.955 5.102E+00 0.734 1.615E+00 3.745E+00 XE-131M 4.500E-01 0.144 0.020 7.380E-02 0.734 3.303E-01 5.417E-02 XE-133M 1.700E+00 0.192 0.041 3.961E-01 0.734 1.248E+00 2.907E-01 XE-133 7.000E+01 0.136 0.046 1.274E+01 0.734 5.138E+01 9.351E+00 XE-135 7.400E+00 0.317 0.249 4.188E+00 0.734 5.432E+00 3.074E+00 BR-83 6.600E-02 0.321 0.008 2.171E-02 0.734 4.844E-02 1.594E-02 BR-84 2.700E-02 1.229 1.788 8.146E-02 0.734 1.982E-02 5.979E-02 RB-86 1.500E-02 0.668 0.095 1.145E-02 0.734 1.101E-02 8.401E-03 CS-134 4.900E+01 0.164 1.555 8.423E+01 0.734 3.597E+01 6.183E+01 CS-136 4.300E+00 0.139 2.166 9.912E+00 0.734 3.156E+00 7.275E+00 CS-137 2.600E+01 0.187 0.000 4.862E+00 0.734 1.908E+01 3.569E+00 CS-138 7.000E-01 1.207 2.361 2.498E+00 0.734 5.138E-01 1.833E+00 SR-89 5.400E-03 0.583 0.000 3.148E-03 0.734 3.964E-03 2.311E-03 SR-90 4.900E-04 0.196 0.000 9.604E-05 0.734 3.597E-04 7.049E-05 CR-51 4.700E-03 0.004 0.033 1.739E-04 0.734 3.450E-03 1.276E-04 FE-59 4.500E-04 0.118 1.189 5.882E-04 0.734 3.303E-04 4.317E-04 CO-60 8.000E-04 0.097 2.504 2.081E-03 0.734 5.872E-04 1.527E-03 SR-91 1.500E-03 0.656 0.697 2.030E-03 0.734 1.101E-03 1.490E-03 SR-92 5.900E-04 0.196 1.339 9.057E-04 0.734 4.331E-04 6.647E-04 Y-90 6.400E-04 0.935 0.000 5.984E-04 0.734 4.698E-04 4.392E-04 Y-91M 8.900E-04 0.027 0.530 4.957E-04 0.734 6.533E-04 3.639E-04 Y-91 1.800E-02 0.602 0.004 1.091E-02 0.734 1.321E-02 8.006E-03 Y-92 7.200E-04 1.446 0.252 1.223E-03 0.734 5.285E-04 8.974E-04 Y-93 4.400E-04 1.174 0.089 5.557E-04 0.734 3.230E-04 4.079E-04 ZR-95 1.200E-03 0.116 0.739 1.026E-03 0.734 8.808E-04 7.531E-04 NB-95 1.200E-03 0.044 0.766 9.720E-04 0.734 8.808E-04 7.134E-04

Numerical Applications Inc. Page 13 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Activity Adjusted Nuclide uCi/gm E-beta E-gamma (E

i + E i) x ai Multiplier Activity (E

i + E i) x ai MO-99 4.200E+00 0.392 0.150 2.276E+00 0.734 3.083E+00 1.671E+00 TC-99M 3.200E+00 0.016 0.126 4.544E-01 0.734 2.349E+00 3.335E-01 RU-103 1.200E-03 0.075 0.469 6.528E-04 0.734 8.808E-04 4.792E-04 RU-106 5.300E-04 0.010 0.000 5.300E-06 0.734 3.890E-04 3.890E-06 RH-103M 1.200E-03 0.038 0.002 4.800E-05 0.734 8.808E-04 3.523E-05 TE-125M 2.000E-03 0.109 0.036 2.900E-04 0.734 1.468E-03 2.129E-04 TE-127M 7.200E-03 0.082 0.011 6.696E-04 0.734 5.285E-03 4.915E-04 TE-127 4.600E-02 0.223 0.005 1.049E-02 0.734 3.376E-02 7.698E-03 TE-129M 2.200E-02 0.260 0.038 6.556E-03 0.734 1.615E-02 4.812E-03 TE-129 3.800E-02 0.544 0.059 2.291E-02 0.734 2.789E-02 1.682E-02 TE-131M 3.700E-02 0.202 1.425 6.020E-02 0.734 2.716E-02 4.419E-02 TE-132 4.800E-01 0.102 0.234 1.613E-01 0.734 3.523E-01 1.184E-01 TE-134 2.100E-02 0.300 0.886 2.491E-02 0.734 1.541E-02 1.828E-02 BA-140 7.100E-03 0.313 0.183 3.522E-03 0.734 5.211E-03 2.585E-03 LA-140 3.400E-03 0.537 2.315 9.697E-03 0.734 2.496E-03 7.117E-03 CE-141 1.100E-03 0.171 0.076 2.717E-04 0.734 8.074E-04 1.994E-04 CE-143 6.300E-04 0.433 0.282 4.505E-04 0.734 4.624E-04 3.306E-04 CE-144 9.300E-04 0.092 0.021 1.051E-04 0.734 6.826E-04 7.714E-05 PR-143 1.000E-03 0.314 0.000 3.140E-04 0.734 7.340E-04 2.305E-04 MN-54 2.400E-03 0.004 0.836 2.016E-03 0.734 1.762E-03 1.480E-03 FE-55 1.800E-03 0.004 0.002 1.080E-05 0.734 1.321E-03 7.927E-06 CO-58 7.000E-03 0.034 0.976 7.070E-03 0.734 5.138E-03 5.189E-03 ZR-97 4.900E-04 0.700 0.179 4.307E-04 0.734 3.597E-04 3.161E-04 RU-105 1.400E-04 0.400 0.784 1.658E-04 0.734 1.028E-04 1.217E-04 RH-105 5.500E-04 0.154 0.078 1.276E-04 0.734 4.037E-04 9.366E-05 SB-127 4.300E-02 0.316 0.688 4.317E-02 0.734 3.156E-02 3.169E-02 SB-129 2.400E-02 0.408 1.437 4.428E-02 0.734 1.762E-02 3.250E-02 XE-135M 4.800E-01 0.098 0.429 2.530E-01 0.734 3.523E-01 1.857E-01 CS-134M 4.600E-02 0.112 0.027 6.394E-03 0.734 3.376E-02 4.693E-03 RB-88 2.300E+00 2.066 0.629 6.199E+00 0.734 1.688E+00 4.550E+00 RB-89 5.800E-02 1.013 2.071 1.789E-01 0.734 4.257E-02 1.313E-01 SB-124 1.100E-03 0.387 1.817 2.424E-03 0.734 8.074E-04 1.780E-03

Numerical Applications Inc. Page 14 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Activity Adjusted Nuclide uCi/gm E-beta E-gamma (E

i + E i) x ai Multiplier Activity (E

i + E i) x ai SB-125 9.200E-03 0.100 0.431 4.885E-03 0.734 6.753E-03 3.586E-03 SB-126 6.200E-04 0.283 2.834 1.933E-03 0.734 4.551E-04 1.418E-03 TE-131 1.500E-02 0.719 0.420 1.709E-02 0.734 1.101E-02 1.254E-02 TE-133M 1.200E-02 0.705 2.313 3.622E-02 0.734 8.808E-03 2.658E-02 BA-141 9.100E-05 0.901 0.845 1.589E-04 0.734 6.679E-05 1.166E-04 BA-139 4.300E-04 0.898 0.043 4.046E-04 0.734 3.156E-04 2.970E-04 LA-141 2.400E-04 0.948 0.043 2.378E-04 0.734 1.762E-04 1.746E-04 LA-142 6.800E-05 0.846 2.753 2.447E-04 0.734 4.991E-05 1.796E-04 ND-147 4.300E-04 0.270 0.140 1.763E-04 0.734 3.156E-04 1.294E-04 NB-97 8.100E-05 0.468 0.655 9.096E-05 0.734 5.945E-05 6.677E-05 NB-95M 8.500E-06 0.166 0.068 1.989E-06 0.734 6.239E-06 1.460E-06 PM-147 1.200E-04 0.062 0.000 7.440E-06 0.734 8.808E-05 5.461E-06 PM-148 1.700E-04 0.724 0.575 2.208E-04 0.734 1.248E-04 1.621E-04 PM-149 3.000E-04 0.366 0.011 1.131E-04 0.734 2.202E-04 8.302E-05 PM-151 8.300E-05 0.306 0.321 5.204E-05 0.734 6.092E-05 3.820E-05 PM-148M 2.600E-05 0.170 2.000 5.642E-05 0.734 1.908E-05 4.141E-05 PR-144 9.300E-04 1.208 0.032 1.153E-03 0.734 6.826E-04 8.464E-04 Y-94 1.400E-05 1.675 1.110 3.899E-05 0.734 1.028E-05 2.862E-05 BR-82 2.500E-02 0.139 2.642 6.953E-02 0.734 1.835E-02 5.103E-02 Total 1.758E+02 1.363E+02 1.290E+02 1.000E+02 E-bar =

7.752E-01 7.752E-01 100/E-bar =

1.290E+02 1.290E+02

Numerical Applications Inc. Page 15 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Table 6-5 Adjusted Primary Coolant Source Term Nuclide Ci/gm Nuclide Ci/gm KR-83M 2.349E-01 BA-140 5.211E-03 KR-85M 8.808E-01 LA-140 2.496E-03 KR-85 3.890E-01 CE-141 8.074E-04 KR-87 5.505E-01 CE-143 4.624E-04 KR-88 1.615E+00 CE-144 6.826E-04 XE-131M 3.303E-01 PR-143 7.340E-04 XE-133M 1.248E+00 MN-54 1.762E-03 XE-133 5.138E+01 FE-55 1.321E-03 XE-135 5.432E+00 CO-58 5.138E-03 BR-83 4.844E-02 ZR-97 3.597E-04 BR-84 1.982E-02 RU-105 1.028E-04 RB-86 1.101E-02 RH-105 4.037E-04 CS-134 3.597E+01 SB-127 3.156E-02 CS-136 3.156E+00 SB-129 1.762E-02 CS-137 1.908E+01 XE-135M 3.523E-01 CS-138 5.138E-01 CS-134M 3.376E-02 SR-89 3.964E-03 RB-88 1.688E+00 SR-90 3.597E-04 RB-89 4.257E-02 CR-51 3.450E-03 SB-124 8.074E-04 FE-59 3.303E-04 SB-125 6.753E-03 CO-60 5.872E-04 SB-126 4.551E-04 SR-91 1.101E-03 TE-131 1.101E-02 SR-92 4.331E-04 TE-133M 8.808E-03 Y-90 4.698E-04 BA-141 6.679E-05 Y-91M 6.533E-04 BA-139 3.156E-04 Y-91 1.321E-02 LA-141 1.762E-04 Y-92 5.285E-04 LA-142 4.991E-05 Y-93 3.230E-04 ND-147 3.156E-04 ZR-95 8.808E-04 NB-97 5.945E-05 NB-95 8.808E-04 NB-95M 6.239E-06 MO-99 3.083E+00 PM-147 8.808E-05 TC-99M 2.349E+00 PM-148 1.248E-04 RU-103 8.808E-04 PM-149 2.202E-04 RU-106 3.890E-04 PM-151 6.092E-05 RH-103M 8.808E-04 PM-148M 1.908E-05 TE-125M 1.468E-03 PR-144 6.826E-04 TE-127M 5.285E-03 Y-94 1.028E-05 TE-127 3.376E-02 BR-82 1.835E-02 TE-129M 1.615E-02 I-131 0.8305 TE-129 2.789E-02 I-132 0.1917

Numerical Applications Inc. Page 16 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Nuclide Ci/gm Nuclide Ci/gm TE-131M 2.716E-02 I-133 0.8624 TE-132 3.523E-01 I-134 0.0751 TE-134 1.541E-02 I-135 0.3673 6.2 Secondary Side Source Term The secondary side source term is defined by Palisades Technical Specification LCO 3.7.17:

The specific activity of the secondary coolant shall be 0.10 Ci/gm DOSE EQUIVALENT I-131.

Thus, assuming that the relative concentrations of the iodine isotopes on the secondary side are the same as those on the primary side, the secondary side activity is 0.1 times the activity given in Table 6-3.

Table 6-6 Secondary Side Source Term Isotope Ci/gm I-131 0.0830 I-132 0.0192 I-133 0.0862 I-134 0.0075 I-135 0.0367

Numerical Applications Inc. Page 17 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 6.3 References

1. NAI Calculation Number NAI-1149-007 Rev. 0, Primary Coolant Activity for Palisades.
2. Palisades Technical Specifications, through Amendment 213.
3. Federal Guidance Report No. 11, Limiting Values of Radionuclide Intake and Air Concentration and Dose Conversion Factors for Inhalation, Submersion, and Ingestion, September 1988.
4. Federal Guidance Report No. 12, External Exposure to Radionuclides in Air, Water, and Soil, September 1993.

Numerical Applications Inc. Attachment 1 Page 18 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Comments on Revision 1 Comment 1 Please correct the title and calculation number in the header.

Response

Headers corrected.

Comment 2 Page 11, Second sentence - Should state that activities were multiplied by 0.734 versus increased.

Response

Fixed.

Numerical Applications Inc. Attachment 2 Page 19 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Palisades PCS Activity Nuclide Inventory File (pal_pcs.nif)

Nuclide Inventory Name:

Palisades PCS Source 1.0 uCi/gm DE131 and 100/E-bar Power Level:

0.1000E+01 Nuclides:

107 Nuclide 001:

Co-58 7

0.6117120000E+07 0.5800E+02 0.5138E-02 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 002:

Co-60 7

0.1663401096E+09 0.6000E+02 0.5872E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 003:

Kr-85 1

0.3382974720E+09 0.8500E+02 0.3890E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 004:

Kr-85m 1

0.1612800000E+05 0.8500E+02 0.8808E+00 Kr-85 0.2110E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 005:

Kr-87 1

0.4578000000E+04 0.8700E+02 0.5505E+00 Rb-87 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 006:

Kr-88 1

0.1022400000E+05 0.8800E+02 0.1615E+01 Rb-88 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 007:

Rb-86 3

0.1612224000E+07 0.8600E+02 0.1101E-01

Numerical Applications Inc. Attachment 2 Page 20 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 008:

Sr-89 5

0.4363200000E+07 0.8900E+02 0.3964E-02 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 009:

Sr-90 5

0.9189573120E+09 0.9000E+02 0.3597E-03 Y-90 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 010:

Sr-91 5

0.3420000000E+05 0.9100E+02 0.1101E-02 Y-91m 0.5780E+00 Y-91 0.4220E+00 none 0.0000E+00 Nuclide 011:

Sr-92 5

0.9756000000E+04 0.9200E+02 0.4331E-03 Y-92 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 012:

Y-90 9

0.2304000000E+06 0.9000E+02 0.4698E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 013:

Y-91 9

0.5055264000E+07 0.9100E+02 0.1321E-01 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 014:

Y-92 9

0.1274400000E+05 0.9200E+02 0.5285E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 015:

Y-93 9

0.3636000000E+05

Numerical Applications Inc. Attachment 2 Page 21 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 0.9300E+02 0.3230E-03 Zr-93 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 016:

Zr-95 9

0.5527872000E+07 0.9500E+02 0.8808E-03 Nb-95m 0.7000E-02 Nb-95 0.9930E+00 none 0.0000E+00 Nuclide 017:

Zr-97 9

0.6084000000E+05 0.9700E+02 0.3597E-03 Nb-97m 0.9470E+00 Nb-97 0.5300E-01 none 0.0000E+00 Nuclide 018:

Nb-95 9

0.3036960000E+07 0.9500E+02 0.8808E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 019:

Mo-99 7

0.2376000000E+06 0.9900E+02 0.3083E+01 Tc-99m 0.8760E+00 Tc-99 0.1240E+00 none 0.0000E+00 Nuclide 020:

Tc-99m 7

0.2167200000E+05 0.9900E+02 0.2349E+01 Tc-99 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 021:

Ru-103 7

0.3393792000E+07 0.1030E+03 0.8808E-03 Rh-103m 0.9970E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 022:

Ru-105 7

0.1598400000E+05 0.1050E+03 0.1028E-03 Rh-105 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 023:

Ru-106

Numerical Applications Inc. Attachment 2 Page 22 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 7

0.3181248000E+08 0.1060E+03 0.3890E-03 Rh-106 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 024:

Rh-105 7

0.1272960000E+06 0.1050E+03 0.4037E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 025:

Sb-127 4

0.3326400000E+06 0.1270E+03 0.3156E-01 Te-127m 0.1760E+00 Te-127 0.8240E+00 none 0.0000E+00 Nuclide 026:

Sb-129 4

0.1555200000E+05 0.1290E+03 0.1762E-01 Te-129m 0.2250E+00 Te-129 0.7750E+00 none 0.0000E+00 Nuclide 027:

Te-127 4

0.3366000000E+05 0.1270E+03 0.3376E-01 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 028:

Te-127m 4

0.9417600000E+07 0.1270E+03 0.5285E-02 Te-127 0.9760E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 029:

Te-129 4

0.4176000000E+04 0.1290E+03 0.2789E-01 I-129 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 030:

Te-129m 4

0.2903040000E+07 0.1290E+03 0.1615E-01 Te-129 0.6500E+00 I-129 0.3500E+00 none 0.0000E+00

Numerical Applications Inc. Attachment 2 Page 23 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Nuclide 031:

Te-131m 4

0.1080000000E+06 0.1310E+03 0.2716E-01 Te-131 0.2220E+00 I-131 0.7780E+00 none 0.0000E+00 Nuclide 032:

Te-132 4

0.2815200000E+06 0.1320E+03 0.3523E+00 I-132 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 033:

I-131 2

0.6946560000E+06 0.1310E+03 0.8305E+00 Xe-131m 0.1110E-01 none 0.0000E+00 none 0.0000E+00 Nuclide 034:

I-132 2

0.8280000000E+04 0.1320E+03 0.1917E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 035:

I-133 2

0.7488000000E+05 0.1330E+03 0.8624E+00 Xe-133m 0.2900E-01 Xe-133 0.9710E+00 none 0.0000E+00 Nuclide 036:

I-134 2

0.3156000000E+04 0.1340E+03 0.7510E-01 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 037:

I-135 2

0.2379600000E+05 0.1350E+03 0.3673E+00 Xe-135m 0.1540E+00 Xe-135 0.8460E+00 none 0.0000E+00 Nuclide 038:

Xe-133 1

0.4531680000E+06 0.1330E+03 0.5138E+02 none 0.0000E+00

Numerical Applications Inc. Attachment 2 Page 24 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 none 0.0000E+00 none 0.0000E+00 Nuclide 039:

Xe-135 1

0.3272400000E+05 0.1350E+03 0.5432E+01 Cs-135 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 040:

Cs-134 3

0.6507177120E+08 0.1340E+03 0.3597E+02 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 041:

Cs-136 3

0.1131840000E+07 0.1360E+03 0.3156E+01 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 042:

Cs-137 3

0.9467280000E+09 0.1370E+03 0.1908E+02 Ba-137m 0.9460E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 043:

Ba-139 6

0.4962000000E+04 0.1390E+03 0.3156E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 044:

Ba-140 6

0.1100736000E+07 0.1400E+03 0.5211E-02 La-140 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 045:

La-140 9

0.1449792000E+06 0.1400E+03 0.2496E-02 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 046:

La-141 9

0.1414800000E+05 0.1410E+03

Numerical Applications Inc. Attachment 2 Page 25 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 0.1762E-03 Ce-141 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 047:

La-142 9

0.5550000000E+04 0.1420E+03 0.4991E-04 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 048:

Ce-141 8

0.2808086400E+07 0.1410E+03 0.8074E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 049:

Ce-143 8

0.1188000000E+06 0.1430E+03 0.4624E-03 Pr-143 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 050:

Ce-144 8

0.2456352000E+08 0.1440E+03 0.6826E-03 Pr-144m 0.1780E-01 Pr-144 0.9822E+00 none 0.0000E+00 Nuclide 051:

Pr-143 9

0.1171584000E+07 0.1430E+03 0.7340E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 052:

Nd-147 9

0.9486720000E+06 0.1470E+03 0.3156E-03 Pm-147 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 053:

Np-239 8

0.2034720000E+06 0.2390E+03 0.0000E+00 Pu-239 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 054:

Pu-238 8

Numerical Applications Inc. Attachment 2 Page 26 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 0.2768863824E+10 0.2380E+03 0.0000E+00 U-234 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 055:

Pu-239 8

0.7594336440E+12 0.2390E+03 0.0000E+00 U-235 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 056:

Pu-240 8

0.2062920312E+12 0.2400E+03 0.0000E+00 U-236 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 057:

Pu-241 8

0.4544294400E+09 0.2410E+03 0.0000E+00 U-237 0.2450E-04 Am-241 0.1000E+01 none 0.0000E+00 Nuclide 058:

Am-241 9

0.1363919472E+11 0.2410E+03 0.0000E+00 Np-237 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 059:

Cm-242 9

0.1406592000E+08 0.2420E+03 0.0000E+00 Pu-238 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 060:

Cm-244 9

0.5715081360E+09 0.2440E+03 0.0000E+00 Pu-240 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 061:

I-130 2

0.4449600000E+05 0.1300E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 062:

Numerical Applications Inc. Attachment 2 Page 27 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Kr-83m 1

0.6588000000E+04 0.8300E+02 0.2349E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 063:

Xe-138 1

0.8502000000E+03 0.1380E+03 0.0000E+00 Cs-138 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 064:

Xe-131m 1

0.1028160000E+07 0.1310E+03 0.3303E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 065:

Xe-133m 1

0.1890432000E+06 0.1330E+03 0.1248E+01 Xe-133 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 066:

Xe-135m 1

0.9174000000E+03 0.1350E+03 0.3523E+00 Xe-135 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 067:

Cs-138 3

0.1932000000E+04 0.1380E+03 0.5138E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 068:

Cs-134m 3

0.1044000000E+05 0.1340E+03 0.3376E-01 Cs-134 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 069:

Rb-88 3

0.1068000000E+04 0.8800E+02 0.1688E+01 none 0.0000E+00 none 0.0000E+00

Numerical Applications Inc. Attachment 2 Page 28 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 none 0.0000E+00 Nuclide 070:

Rb-89 3

0.9120000000E+03 0.8900E+02 0.4257E-01 Sr-89 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 071:

Sb-124 4

0.5201280000E+07 0.1240E+03 0.8074E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 072:

Sb-125 4

0.8741455200E+08 0.1250E+03 0.6753E-02 Te-125m 0.2280E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 073:

Sb-126 4

0.1071360000E+07 0.1260E+03 0.4551E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 074:

Te-131 4

0.1500000000E+04 0.1310E+03 0.1101E-01 I-131 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 075:

Te-133 4

0.7470000000E+03 0.1330E+03 0.0000E+00 I-133 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 076:

Te-134 4

0.2508000000E+04 0.1340E+03 0.1541E-01 I-134 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 077:

Te-125m 4

0.5011200000E+07 0.1250E+03 0.1468E-02

Numerical Applications Inc. Attachment 2 Page 29 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 078:

Te-133m 4

0.3324000000E+04 0.1330E+03 0.8808E-02 I-133 0.8700E+00 Te-133 0.1300E+00 none 0.0000E+00 Nuclide 079:

Ba-141 6

0.1096200000E+04 0.1410E+03 0.6679E-04 La-141 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 080:

Ba-137m 6

0.1531200000E+03 0.1370E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 081:

Pd-109 7

0.4833720000E+05 0.1090E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 082:

Rh-106 7

0.2990000000E+02 0.1060E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 083:

Rh-103m 7

0.3367200000E+04 0.1030E+03 0.8808E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 084:

Tc-101 7

0.8520000000E+03 0.1010E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 085:

Eu-154 9

0.2777068800E+09

Numerical Applications Inc. Attachment 2 Page 30 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 0.1540E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 086:

Eu-155 9

0.1565256960E+09 0.1550E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 087:

Eu-156 9

0.1312416000E+07 0.1560E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 088:

La-143 9

0.8538000000E+03 0.1430E+03 0.0000E+00 Ce-143 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 089:

Nb-97 9

0.4326000000E+04 0.9700E+02 0.5945E-04 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 090:

Nb-95m 9

0.3117600000E+06 0.9500E+02 0.6239E-05 Nb-95 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 091:

Pm-147 9

0.8278820780E+08 0.1470E+03 0.8808E-04 Sm-147 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 092:

Pm-148 9

0.4639680000E+06 0.1480E+03 0.1248E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 093:

Pm-149

Numerical Applications Inc. Attachment 2 Page 31 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 9

0.1910880000E+06 0.1490E+03 0.2202E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 094:

Pm-151 9

0.1022400000E+06 0.1510E+03 0.6092E-04 Sm-151 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 095:

Pm-148m 9

0.3568320000E+07 0.1480E+03 0.1908E-04 Pm-148 0.4600E-01 none 0.0000E+00 none 0.0000E+00 Nuclide 096:

Pr-144 9

0.1036800000E+04 0.1440E+03 0.6826E-03 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 097:

Pr-144m 9

0.4320000000E+03 0.1440E+03 0.0000E+00 Pr-144 0.9990E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 098:

Sm-153 9

0.1681200000E+06 0.1530E+03 0.0000E+00 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 099:

Y-94 9

0.1146000000E+04 0.9400E+02 0.1028E-04 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 100:

Y-95 9

0.6420000000E+03 0.9500E+02 0.0000E+00 Zr-95 0.1000E+01 none 0.0000E+00 none 0.0000E+00

Numerical Applications Inc. Attachment 2 Page 32 of 32 Primary Coolant Source Term Determination for Palisades Dose Calculations Calculation Number: NAI-1149-011 Rev. 0 Nuclide 101:

Y-91m 9

0.2982600000E+04 0.9100E+02 0.6533E-03 Y-91 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 102:

Br-82 2

0.1270800000E+06 0.8200E+02 0.1835E-01 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 103:

Br-83 2

0.8604000000E+04 0.8300E+02 0.4844E-01 Kr-83m 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 104:

Br-84 2

0.1908000000E+04 0.8400E+02 0.1982E-01 none 0.0000E+00 none 0.0000E+00 none 0.0000E+00 Nuclide 105:

Am-242 9

0.5767200000E+05 0.2420E+03 0.0000E+00 Cm-242 0.8270E+00 Pu-242 0.1730E+00 none 0.0000E+00 Nuclide 106:

Np-238 8

0.1829088000E+06 0.2380E+03 0.0000E+00 Pu-238 0.1000E+01 none 0.0000E+00 none 0.0000E+00 Nuclide 107:

Pu-243 8

0.1784160000E+05 0.2430E+03 0.0000E+00 Am-243 0.1000E+01 none 0.0000E+00 none 0.0000E+00 End of Nuclear Inventory File