ML20247M395
| ML20247M395 | |
| Person / Time | |
|---|---|
| Site: | Peach Bottom  |
| Issue date: | 12/31/1988 |
| From: | Danni Smith PECO ENERGY CO., (FORMERLY PHILADELPHIA ELECTRIC |
| To: | NRC OFFICE OF INFORMATION RESOURCES MANAGEMENT (IRM) |
| References | |
| NUDOCS 8906050035 | |
| Download: ML20247M395 (191) | |
Text
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CCN-89-14079 PIIILADELPIIIA ELECTRIC COMPANY PEACII BOTTOM ATOMIC POWER STATION R. D.1, Box 208
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Delta, h nnsylvania 17314 rucu sormu-run rois ra or ExctLLewct (717)456 7014 D. M. Smith Vice President I
May 26, 1989 Docket Nos. 50-277 50-278 U.S. Nuclear Regulatory Commission Document Control Desk Washington, DC 20555
SUBJECT:
Peach Bottom Atomic Power Station 1988 Annual Radiological Environmental Operating Report No. 46.
Gentlemen:
Enclosed is a copy of the Peach Bottom Atomic Power Station 1988 Annual Radiological Environmental Operating Report No. 46. It was prepared in compliance with Appendix A to the Peach Bottom Atomic Power Station Operating License, Technical Specifications, Section 6.9.2.
If you have any questions or concerns almut this report, please do not hesitate to call.
Sincerel,
WnT6 DMS/ C/MJB: cme Enclosure cc:
J.T. Boettger, Public Service Electric & Gas T.M. Gerusky, Commonwealth of Pennsylvania T.P. Johnson, USNRC Senior Rcsident Inspector T.E. Magette, State of Maryland W.T. Russell., Administrator, Region I, USNRC H.C. Schwemm, Atlantic Electric J. Urban, Delmarva Power 8906050035 881231 PDR ADDCK 05000277 R
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PEACH BOTTOM ATOMIC POWER STATION l
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i UNITS 2 and 3
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ANNUAL RADIOLOGICAL ENVIRONMENTAL OPERATING REPORT i
l Prepared by PHILADELPHIA ELECTRIC COMPANY 2301 Market Street Philadelphia, Pennsylvania 19101 Radiological Analyses by CLEAN HARBORS ANALYTICAL SERVICES, INC.
325 Wood Road Braintree, Massachusetts 02184 And TELEDYNEISOTOPES 50 Van Buren Avenue Westwood, New Jersey 07675
I Docket No:
50-277 50-278 I
PEACH BOTTOM ATOMIC POWER STATION Units 2 and 3 I
Annual Radiological Environmental Operating Report Report #46 1 January 1988 through 31 December 1988 I
Prepared By Philadelphia Electric Company I
2301 Market Street Philadelphia, Pennsylvania 19101 1
Radiological Analyses Performed I
By Clean Harbors Analytical Services, Inc.
I 325 Wood Road Braintree, Massachusetts 02184 And I
Teledyne Isotopes 50 Van Buren Avenue l
Westwood, New Jersey 07675 lI i
May 1989 I
TABLE OF CONTENTS I
I.
Summary and Conclusions..........................................
1 II.
Introduction.....................................................
3 A.
Objectives..................................................
3 B.
Implementation..............................................
4 III.
Program Description..............................................
5 A.
S ampl e C ol l e ct i o n...........................................
5 B.
Data Interpretation.........................................
7 C.
Program Changes.............................................
7 D.
Program Exceptions..........................................
7 IV. Results and Discussion...........................................
9 A.
Aquatic Environment.........................................
9 1.
Surface Water..........................................
9 2.
Drinking Water........................................
10 3.
Fish..................................................
11 4.
Sediment 11
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Atmospheric Environment....................................
12 1.
Airborne..............................................
12
- a. Air Particulate 12
- b. Airborne Iodine 13 2.
Terrestrial 13 a.
Milk................................................
13
- b. Well Water.........................................
14
- c. Vegetation.........................................
15
- d. Soil 16 C.
Ambient Gamma Radiation....................................
16 V.
References......................................................
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I Appendix A -
Radiological Environmental Monitoring Report Summary Appendix B -
Sample Designation and Locations Appendix C -
Data Tables and Figures-Primary Laboratory Appendix D -
Data Tables and Figures-Comparison Laboratory Appendix E -
Synopsis of Analytical Procedures Section 1 - Collection Methods Section 2 - Analytical Methods and Calculations Appendix F -
Quality Control - EPA Crosscheck Appendix G -
PBAPS Survey I.
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SUMMARY
AND CONCLUSIONS I
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Summary and Conclusions This report on the Radiological Environmental Monitoring Program (REMP) conducted at the Peach Bottom Atomic Power Station (PBAPS) by Phila-delphia Electric Company (PECo) covers the period 1 January 1988 through 31 j
i December 1988. This report combines the results of the programs conducted j
by Teledyne Isotopes (TI) and Clean Harbors (CH) Laboratories. During this q
period 3,329 analyses were performed on 2,279 samples.
Surface water and drinking (potable) water samples were analyzed for concentrations of gross alpha, gross beta, gamma spectrometry, and tritium.
Additionally, drinking water samples were analyzed for concentrations of 1
Results of these analyses showed no significant differences be-tween control locations and potentially-affected stations. The values ob-served were within the ranges noted in the preoperational report.
The remaining sample media representing the aquatic environment in-cluded fish and sediment samples. Fish samples were analyzed for concentra-tions of gamn emitters and Strontium-89 and Strontium-90. Gross alpha, I
gross beta, and gamma spectrometry analyses were performed on sediment samples. As in previous years the program detected plant related activity at low levels in fish and sediment samples in Conowingo Pond. Cs-137 and i
Cs-134 were found in fish samples from off-site locations. Slightly higher concentrations of these nuclides and Co-60 and Zn-65 were found in samples from the plant water discharge system.
Sediment samples at indicator loca-tions showed Cs-137, Cs-134, Co-60 and Zn-65. Ce-141 was found at one loca-I tien. The resulting doses to the maximum exposed individual were less than 1% of 10CFR50 Appendix I design objectives. All results from these analyses were comparable to those of previous years.
The atmospheric environment was divided into two parts for examina-tion: airborne and terrestrial. Sample media for determining airborne ef-fects include air particulate and air iodine samples. Analyses performed on air particulate samples included gross beta and gamma spectrometry. The results from both analyses were generally consistent with results from the previous years.
Furthermore, no notable differences among results from on-I site, intermediate, and distant locations in either analysis were observed.
These findings indicate no measurable effects from the operation of PBAPS.
High sensitivity Iodine-131 analyses were performed on weekly air I
samples. All results were less than the minimum detectable level.
Examination of the terrestrial environment was accomplished by analyz-I ing milk, vegetation, soil, and well water samples. Milk samples were ana-lyzed for concentrations of Strontium-89, Strontium-90, Cesium-134, Cesium-137, and Iodine-131. Results from all analyses were consistent with those from previous years and no indication of PBAPS effect.
Analyses performed on well water samples included gross alpha, gross beta, gamma spectrometry, and uranium. Results from these analyses were generally comparable to those of previous years.
Results from the indicator and control locations were similar indicating no PBAPS effect..
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Analyses performed on vegetation samples included Strontium-89 and Strontium-90 and gamma spectrometry. Higher concentrations of Strontium-90 were detected in wild vegetation than cultivated crops, possibly due to the longer growing season. resulting in a greater accumulation of fallout.
These results were comparable to previous years. Gamma spectrometry results l
were similar to those seen in previous years. No notable difference was ob-3 served between indicator and control locations.
Analyses performed on soil samples included gross beta, Strontium-89 and Strontium-90, and gamma spectrometry. Results from gross beta, strontium analyses, and gamma spectrometry were comparable to those of pre-vious years. No notable difference was observed between indicator and con-trol locations.
Ambient gamma radiation levels were measured monthly and quarterly throughout the year. Most monthly and all quarterly measurements were below 10 mR/std. month. These results were consistent with those from previous years.
Except for fish and sediment samples, no measurable amounts of radioactivity were found off-site by the REMP which could be attributed to the operation of PBAPS.
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INTRODUCTION I
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1 II.
Introduction a
Peach Bottom Atomic Power Station (PBAPS) is located along the 5
Susquehanna River between Holtwood and Conowingo nams in Peach Bottom Town-ship, York County, Pennsylvania. The initial loading of fuel into Unit 1, a 40 MWe (net) high temperature, gas-cooled reactor, began on 5 February 1966, I
and initial criticality was achieved on 3 March 1966. Shutdown of Peach Bottom Unit I for decommissioning was on 31 October 1974.
For the purposes of the monitoring program, the beginning of the operational period for Unit 1 was considered to be 5 February 1966. A summary of the Unis,
preopera-I tional monitoring program was presented in a previous report i ?.
PBAPS l
Units 2 and 3 are boiling water reactors each with a power output of approx-imately 1050 MWe (net). The first fuel was loaded into Peach Bottom Unit 2 I
on 9 August 1973, criticality was achieved on 16 September 1973, and full power was reached on 16 June 1974. The first fuel was loaded into Peach Bottom Unit 3 on 5 July 1974, and full powp )y ; first reached on 21 Decem-ber 1974. Preoperational summary reports for Units 2 and 3 have been I
previously issued and summarize the results of all analyses performed on samples collected from 5 February 1966 through 8 August 1973.
I The Teledyne Isotopes (TI) program complements an existing program being conducted by Clean Harbors (CH) which has been carried out since 1960.
Analysis of the media was conducted by both laboratories as follows:
TI was the primary analytical laboratory for surface and drinking water, air iodine, and TLD samples, and the comparison laboratory for air particulate.
CH was the primary analytical laboratory for air particulate, fish, I
sediment, soil, well water, and vegetation, and the secondary laboratory for surface and drinking water.
Responsibility was shared for milk samples, with TI primary for I-131 analysis and CH primary for Cs-134 and Cs-137.
The total PBAPS REMP exceeds the requirements of the Radiological En-I.
vironmental Technical Specifications both in media sampled and analyses per-formed.
A.
Objectives The objectives of the REMP are:
1.
To identify, measure, and evaluate existing radionuclides in the environs of PBAPS site and any fluctuations in radioac-tivity levels which may occur.
l 2.
To monitor and evaluate ambient radiation levels.
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To determine within the scope of the program, any measurable
,I quantity of radioactivity introduced to the environment by the operation of PBAPS.
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B.
Implementation Implementation of the stated objectives is accomplished by identi-fying significant exposure pathways, establishing baseline radiological data of media within those pathways, and monitoring 6
those media during plant operation to assess plant effects (if 3
any) on man and the environment.
In order to achieve the stated objectives, the current programs l
include the following analyses on samples collected:
1.
Concentrations of tritium in surface water, drinking water, and well water.
2.
Concentrations of alpha emitters in surface water, drinking water, well water, and sediment.
3.
Concentrations of beta emitters in surface water, drinking water, well water, air particulate, soil, and sediment.
4.
Concentrations of Strontium-89 and Strontium-90 in milk, vegetation, and fish.
5.
Concentrations of gamma emitters in surface water, drinking water, well water, air particulate, milk, vegetation, soil, sediment, and fish.
6.
Concentrations of Iodine-131 in drinking water, air, and milk.
(Vegetation only if milk samples were not collected.)
7.
Ambient gamma radiation levels at various site environs.
8.
Concentrations of uranium in well water.
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PROGRAM DESCRIPTION I
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E III. Program Description A.
Sample Collection i
This section describes the basic collection methods used to obtain environmental samples. For a more detailed account, including I
equipment used, refer to Appendix E, Section 1: Synopsis of Pro-cedures - Collection Methods.
Aauatic Environment The aquatic environment was examined by analyzing samples of sur-face water, drinking water, fish, and sediment. Surface water N
from two locations (itt and iMM) and drinking water from two loca-W tions (4L and 61) were collected weekly from a tank at each loca-tion ar.d were composited into a monthly sample for analysis. Two additional surface water locations (13A and 13B) were collected as I
grab samples. Control locations were ILL and 61.
Fish samples from two groups, catfish (bottom feeder) and I
smallmouth bass (predator) were collected quarterly at five loca-tions: 1X, IEE, 41, and 4J (indicators) and 6 (control).
Sediment samples composed of recently deposited substrate were I
collected at six locations semiannually:
1X, IBB, 4J, 4D, and 4T (indicators) and 6F (control).
Atmospheric Environment The atmospheric environment was examined by analyzing airborne and I
terrestrial samples. These consisted of air particulate, air-borne iodine, milk, well water, vegetation, and soil samples. Air particulate samples were collected and analyzed weekly from six-teen locations (IA, IB, 2, 3A, 4B, 5, 6B,12A,120,14,15,17, I
31, 32, 33A, and 38). Control locations were 48, 6B, 12A, and 120. Air iodine samples were collected from eight locations (IB, 1Z, 2, 3A, 5, 6B, 12D, and 14). Control locations were 6B and I
120. Air particulate and air iodine samples were obtained using a vacuum sampler, glass fiber and charcoal filters, respectively.
The filters were replaced weekly and sent to the appropriate laboratory for analysis. The vacuum samplers were run continuous-ly at approximately 1 cubic foot per minute.
Milk samples were collected from six locations (A, B, G, 0, J, I
and N) monthly from December through March and biweekly during the grazing season (April through November). Additionally, samples from four locations (C, E, L, and M) were collected quarterly.
Locations A, B, C, and E were controls.
Well water samples were collected from four locations (1U, IV, 7, and 40) quarterly. The control location was 7.
Vegetation samples were collected three times a year from seven l
locations (1, 3A, 4N, 5, 6D, 8, and 23). Stems, leaves, and fruit I E
I were collected; foods whenever possible. Control locations were 4N, 60, and 8.
Soil samples from six locations (IAA, 2, 3A, 4N, 5, and 6G) were collected and analyzed semiannually. Control locations were 4N and 6G.
Ambient Gamma Radiation Direct radiation measurements were made using thermoluminescent dosimeters (TLDs) consisting of calcium sulfate (CaSO ) doped with 4
dyprosium (Dy). Samples were collected from forty-seven loca-tions. The TLD locations were placed on and around the PBAPS site 3.
using a "three ring concept":
3 A site boundary ring consisting of thirteen locations (IB,1C, ID, IE, IF, IG, 1H, IJ, IL, IM, INN, 2, and 40) near and within the site perimeter, representing fencepost doses (i.e., at locations where the doses will be greater than maximum annut1 off-site doses) from PBAPS releases; A middle ring consisting of twenty-five locations (3A, 4K, 5, 6B, 14, 15, 17, 22, 23, 26, 27, 31, 32, 33A, 38, 42, 43, 44, 45, 46, 47, 48, 49, 50, and 51) extending to approximately ten miles from l
the site, designed to measure possible exposures to close-in popu-lation; An outer ring consisting of seven locations (12B, 16, 18, 19, 20, 21B, and 24) extending from approximately 10 to 60 miles from the site, and considered to be unaffected by station releases.
Two on-site locations (1A and II), designated as plant complex locations, are not included in any of the three rings.
The specific TLD locations were determined by the following criteria:
1.
The presence of relatively dense population; 2.
Site meterological data taking into account distance and elevation for each of the 36 ten-degree sectors around the site, where estimated annual dose from PBAPS, if any, would be more significant; 3.
On hills free from local obstructions and within sight of the vents (where practical);
4.
Near the dwelling closest to the main stack in the prevailing down wind direction.
A TLD set was placed at each location in a locked formica E
" birdhouse" or polyethylene jar located approximately six feet E)
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4 above ground level. The TLD sets were exchanged monthly and quarterly, then sent to the laboratory for analysis. 1 o
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B.
Data Interpretation Several factors are important for interpretation of the data pre-sented in this report. These factors are discussed here to avoid unnecessary repetition in the discussion of the results.
The minimum detectable level (MDL) was defined as the two sigma counting statistic.
It represents the range of values into which I
95% of repeated counts of the same aliquot would fall. For all analyses an activity that was greater than or equal to the MDL was reported as " activity plus/minus the MDL value'. When an activity was less than the MDL, the result was reported as the "<MDL
- I val ue". Data received from the laboratories were reported using the convention of rounding the result to the same number of sig-nificant places as the first significant digit in the error term (e.g., 3.62 1 1.24 rounds to 4 1 1).
Results for each type of sample were grouped according to the analyses performed. Means and standard deviations of these results were calculated. These standard deviations represent the variability of measured results for different samples rather than single analysis uncertainty. For these calculations, all results I
below the MDL were considered to be at the MDL. As a result, the means were biased high, and the standard deviations were generally biased low.
C.
Program Changes A review of the ongoing REMP program resulted in no changes to the program.
D.
Program Exceptions For 1988 the PBAPS REMP had a sample collection recovery rate of approximately 98%. The exceptions to this program are listed be-low:
1.
Surface water sampler at location ILL was out of service from 01/08/88 to 01/15/88, 05/13/88 to 05/20/88, 05/27/88 to I
06/03/88, 08/19/88 to 09/16/88 and 11/25/88 to 12/02/88.
Daily grab samples were collected instead.
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Surface water sampler at locaticn IMM was out of service from B
o5/27/88 to 07/29/88 and 08/19/88 to 09/09/88. Daily grab samples were collected instead.
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Analysis of surface water sample from location 13A collected 04/30/88 was not reported due to laboratory contamination.
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Drinking water sampler at location 4L was out of service from g
01/09/88 to 01/16/88, 04/16/88 to 04/23/88 and 10/22/88 to 10/29/88 due to pump malfunction.
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Drinking water sampler at location 61 was out of service from 04/30/88 to 05/07/88, 05/28/88 to 06/04/88, 07/02/88 to l
07/09/88 and 08/06/88 to 08/20/88 due to pump malfunction.
6.
No smallmouth bass were available from locations 1EE or IX throughout the year and no catfish were available from loca-tion IEE for the fourth quarter due to unavailability of fish. Strontium results from location 6 for smallmouth bass collected in the fourth quarter were lost in analysis.
7.
Air particulate and air iodine samples were not available from the following locations due to out-of-service equipment:
3 3A from 03/05/88 to 03/12/88 and 1Z from 10/01/88 to 10/08/88.
3 8.
Air particulate samples were not available from the following locations due to out-of-service equipment: 4B from 12/24/88 to 12/31/88 and 4A from 06/26/88 to 07/09/88. Air particu-late samples from locations 12A and 12D for the period 09/19/88 to 09/26/88 were lost in the laboratory.
9.
Air iodine samples for the period 06/26/88 to 07/02/88 were lost in the mail along with the air particulate filter from 1Z for the same period.
- 10. Strontium results from milk farm N for the 09/05/88 collec-tion were lost in analysis. Strontium analyses of milk farm J for the period 11/14/88 were not completed by the secondary laboratory.
- 11. Strontium results for vegetation samples collected at loca-tion 60 from 07/16/88 and location 23 from 09/17/88 were lost in analysis.
Each program exception was reviewed to understand the causes of the program exception.
Sampling and maintenance errors were reviewed with the personnel involved to prevent a recurrence. Oc-3 casional equipment breakdowns and power outages were unavoidable.
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The overall sample recovery rate indicates that the appropriate procedures and equipment are in place to assure reliable program implementation.
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I RESULTS AND DISCUSSION I
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I-IV.
Results and Discussion A.
Aquatic Environment 1.
Surface Water Samples were collected from four locations monthly (ILL, IMM,13A and138).
ILL served as the control location. The following analyses were performed.
Gross Aloha Samples from all locations were analyzed for concentrations of
- I gross alpha in both soluble and insoluble fractions (Table C-I.1 and C-I.2).
Detectable activity was observed in the soluble frac-l tion in five of forty-seven samples. The data ranged from <.3 to 5
3 pCi/1. Activity was observed in the insoluble fraction, ranging from <.03 to 6 pC1/1.
In comparing the insoluble data from pre-vious years with that of 1988, no notable differences were ob-served. Comparison of the control and indicator locations I
presents no notable difference. The similarity of results when comparing preoperational and 1988 data, as well as indicator to control locations, suggests no increased effects in receiving water bodies due to the operation of PBAPS.
Gross Beta Samples from all locations were analyzed for concentrations of gross beta in both soluble and insoluble fractions (Table C-I.1 and C-I.2 and Figures C-1 and C-2).
The results for the soluble I'
fraction ranged from.9 to 5 pCi/1. The mean for the three in-dicator locations was 3.1 pCi/1, compared to the mean value of 2.9 pCi/1 from the control location. The results from analysis of the insoluble portion of all samples from the surface water locations I
ranged from <.4 to 10 pCi/1. The value of 10 pCi/1 (13B, February 1988) was due to an increased level of solids at that location.
The gamma analysis of that sample showed activity of all nuclides l-below MDL. Excluding this value the mean of the indicator loca-tions and control locations were 1.5 pC1/1 and.8 pCi/1, respec-tively.
Tritium Samples from three locations (ILL, IMM,13A) were analyzed for concentrations of aqueous tritium (Table C-I.1 and C-I.2).
Results ranged from 60 to 220 pC1/1 and were within the range found during the preoperational period. Means from indicator and I
control locations compared well, with values of 111 pCi/1 and 135 pCi/1, respectively.
Gamma Spectrometry Samples from all it, cations were analyzed for concentrations of gamma emitters (Tatne C-I.3 and C-I.4).
The nuclides searched for
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I were below the minimum detectable level with the exception of nat-urally occurring K-40 and Th-228. Potassium-40 was found at all locations and ranged from <4 to <20 pCi/1. Thcrium-228 was found R'
in one sample from station 138 (.8 pCi/1, April 1988).
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Drinkina (Potable) Water I
Samples were collected from two locations monthly (4L and 61). 61 served as the control location. The following analyses were per-formed.
Gross Aloha Samples from both locations were analyzed for concentrations of l
gross alpha activity in soluble and insoluble fractions (Table C-II.1). Gross alpha activity for the soluble fraction ranged from <.3 to 1.2 pCi/1. Analysis of the insoluble fraction for E
both locations showed results ranging from <.03 to 1.7 pCi/1.
5 These values were consistent with those seen in the preoperational period.
Gross Beta Samples from both locations were analyzed for concentrations of gross beta activity in soluble and insoluble fractions (Table C-II.1 and figures C-3 and C-4).
Positive beta activity was detected in all soluble fraction samples from both locations rang-a ing from 1 to 6 pCi/1. The values from the insoluble fraction 5
ranged from <.5 to 2.9 pCi/1. Only slight differences were ob-served between the means of the control and indicator stations.
The values were generally below those seen in the preoperational l
period.
Iritium Samples from both locations were analyzed for tritium concentra-tion quarterly (Table C-II.1). Results from both indicator and control locations indicate positive tritium activity, with no notable difference between the two locations. The indicator loca-tion values ranged from <90 to 130 pCi/1 with a mean of 100 pCi/1.
Control location values ranged from <40 to 250 pCi/1 with a mean 3
of 150 pCi/1. The concentrations were within the range found dur-a ing the preoperational period.
Iodine-131 Samples from both locations were analyzed monthly for I-131 con-centrations (Table C-II.1). Results from both the indicator and l
control locations were all less than MDL.
W Gamma Spectrometry Samples from both locations were analyzed for concentrations of gamma emitters (Table C-II.2). The nuclides searched for were be-E I
I low the minimum detectable level, except for Th-228 which was found in one sample at the control location 61 (1.5 i.8 pCi/1, May 1988).
3.
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Samples were collected from five locations quarterly (IEE, IX, 4I, 4J, and 6). The control location was 6.
The following analyses were performed.
Strontium-89 and Strontium-90 Samples from all locations were analyzed for concentrations of Sr-I 89 and Sr-90 (Table C-III.1 and Figure C-5). All Sr-89 values were at or less than MDL. Positive concentrations of Sr-90 were detected at all indicator and control locations. Results ranged from.0070 to.068 pCi/g (wet) at indicator locations and from I
.022 to.081 pCi/g (wet) at the control location. The indicator and control location results did not show notable differences.
Gamma Spectrometry Positive activity was observed for the nuclides Be-7, K-40, Zn-65, I
Cs-134, and Cs-137 (Table C-III.2). Data for Zn-65 ranged from
<.01 to.14 pCi/g (wet). Data for Cs-134 ranged from <.004 to.13 pCi/g (wet) and values for Cs-137 ranged from <.006 to.27 pCi/g (wet).
In addition to these nuclides, several others (Co-60, Nb-I 95, Cs-136, Ce-141, Ra-226 and Th-228) were found at their respec-tive MDL values and may be the result of counting statistics.
Figure C-6 illustrates the Cs-137 activity for indicator and con-I trol locations from the beginning of the operational period through the present. The maximum dose calculated using the USNRC Regulatory Guide 1.109 Model and assumptions is 1.06E-01 mrem to a teenager'; liver. The actual dose due to PBAPS operations was I
less, since the maximum concentrations of radionuclides were as-sumed to exist all year.
In addition, no credit was taken for Cs-137 from sources other than PBAPS. The calculated dose was 0.53%
of the 10CFR50 Appendix I design objectives.
4.
Sediment Samples were collected from six locations semiannually (IBB, IX, 4D, 4J, 4T, and 6F). The control location was 6F. The following analyses were performed.
Gross Aloha I
Samples from all locations were analyzed for concentrations of gross alpha (Table C-IV.1). Results from indicator locations ranged from 1.0 to 5 pCi/g (dry). The mean value was 2.0 pC1/g (dry) for the control location, and 3.9 pCi/g (dry) for the in-I-
dicator locations.
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Gross Beta Samples from all locations were analyzed for concentrations of gross beta (Table C-IV.1).
Results from indicator locations ranged from.8 to 3.8 pCi/g (dry) with a mean of 2.5 pCi/g (dry).
The control location mean was 2.2 pCi/g (dry). These concentra-tions were consistent with those found in the preoperational peri-od.
Gamma Spectrometry Samples from all locations were analyzed for concentrations of a
gamma emitters (Table C-IV.1).
Positive values of naturally-g occuring K-40 were found at all locations. Co-60 was found at three indicator locations and ranged from <.01 to.33 pCi/g (dry).
Location 4J had the highest average concentration of Co-60 (.30 E
pCi/g (dry)).
Ra-226 and Th-228 activity was found at all loca-E tions and Cs-137 was found at all locations except IX. Positive In-65 activity was found at locations 4D and 4J.
Concentrations a
of Cs-134 were found at location IBB, 4D and 4J ranging from <.009 g
to.24 pCi/g (dry).
In addition to these nuclides, Be-7, I-131 and Ce-141 were found at their respective MDL values in samples from Holtwood Pond, Conowingo Pond, and the plant water discharge system. The results were consistent with those from previous years.
Figure C-6 illustrates the comparison of activities of Cs-137 detected at the control location and two indicator locations a
from the preoperational period through the present.
If it is as-3 sumed that all cesium, Co-60 and 2n-65 found at off-site indicator locations was due to PBAPS releases, a dose calculation using the USNRC Regulatory Guide 1.109 model and assumptions results in a calculated dose of 2.41 E-02 mrem to a teenager's skin. This cal-culation conservatively assumes that the teenager was exposed to the maximum concentrations found for the entire period. The cal-E culated dose was 0.12% of the 10CFR50 Appendix I design objec-E tives.
B.
Atmospheric Environment l
1.
Airborne a.
Air Particulate Samples were collected from 16 locations (IA, IB, 2, 3A, 4B, 5, 6B, 12A, 12D, 14, 15, 17, 31, 32, 33A, and 38). Control locations were 4B, 6B, 12A, and 120. The following analyses were performed.
E Gross Beta W
~
Samples from all locations were analyzed for concentrations 3
of gross beta (Tables C-V.1 and C-V.2 and Figures C-8 and C-9).
g Air particulate locations are divided into three groups:
E I,
l
)
Group I, consisting of 1A,18, and 2, located on site at PBAPS; Group II, comprised of 3A, 4B, 5, 6B,14,15,17, 31, 32, 33A and 38, located at intermediate distances from PBAPS; l
and Group III, consisting of 12A and 12D, located at remote distances from PBAPS. Comparison of results among these three groups aids in determining the effects, if any, result-tion samples ranged from 9 to 57 E-3 pCi/m}ts from site loca-ing from the operation of PBAPS. The resu
, with a mean of k
3 28 E-3 pCi/m. The results fr m intermediate locations rangegfrom<4to67E-3pCi/m,withameanof28E-3 l,
pCi/m. The es s from d stant locad ong rang d kom 9 to 3
Comparison of 48 E-3 pCi/m, with a mean of 24 E-3 pCi/m.
the mean values indicate no notable difference among the t
three groups suggesting no effects from operation of PBAPS.
Gamma Spectrometry Samples from all locations were analyzed monthly for the presence of gamma emitters (Tables C-V.3 and C-V.4).
Natu-rally occuring Be-7 was found in most samples as has been the s
case in the past. Other nuclides, including K-40, Cs-136, Cs-137, Ra-226 and Th-228 were found at or slightly above the detection limit in a few samples. Due to the wide dispersal r
of the nuclides and their extremely low level, no PBAPS con-tribution is indicated.
b.
Airborne lodi_n_g Continuous air samples were collected weekly at eight loca-tions and analyzed for I-131 (Table C-VI.1). All results were less than the minimum detectable level.
2.
Terrestrial a.
lii.lk Samples were collected from ten locations (A, B, C, E, G, J, L, M, N, and 0).
Farms A, B, C, and E were control loca-tions. The following analyses were performed.
Strontium-89 and Strontium-90 L
Samples from all locations were analyzed quarterly for con-centrations of Sr-89 and Sr-90 (Table C-VII.1). A positive value of Sr-89 was observed at the detection limit in one i
sample from February at Farm C.
All samples indicated posi-tive Sr-90 activity with results ranging from 1.2 to 8.1 pCi/1. Sr-90 activities of samples from the nearby farms (G, 1
J, and 0) and intermediate farms (L, M, and N) were slightly higher than the activities detected in samples from the dis-tant farms (A, B, C, and E). Comparing Sr-90 means from the three groups: nearby farms had a mean for all samples of 2.8 pCi/1, intermediate farms had a mean of 3.0 pCi/1, and the 1 i
_.--___m--m_
I distant farms had a mean of 2.0 pCi/1. The trend for detect-ing higher activity at the nearby and intermediate farms is consistent with results from both the preoperational and op-I erational periods. The preoperational/ operational mean
{
ratios were similar and therefore the higher Sr-90 radioac-tivity concentrations observed are not due to PBAPS opera-g tion.
gj l
Cesium-134 and Cesium-137 Samples from all locations were analyzed quarterly for con-centrations for Cs-134 and Cs-137 (Table C-VII.1 and Figure C-10). Positive concentrations of Cs-137 were detected in some samples # rom most farms, with positive values ranging from 3 to 5 % t/2 and was attributed to atmospheric nuclear testing. Os '34 activity at the detection limit (3 1 3), was observed in tw sample from Farm N.
The absence, in general, l
of Cs-134 and the declining levels of Cs-137 over the past several years supports the nuclear testing assumption.
Iodine-131 Sampbs from all locations were analyzed for concentrations of I-131 (Tables C-VII.2 and C-VII.3). All results from all analyses were less than the minimum detectable level.
b.
Well Water Samples from four locations (10, IV, 40, and 7) were col-lected quarterly. Location 7 was the control. The following g
analyses were performed.
g Gross Aloha Samples from all locations were analyzed for concentrations of gross alpha (Table C-VIII.1). Results from analysis of samples from all locations were similar and ranged for <.2 to 1.7 pCi/1. The results for well water samples were similar to the results of previous years.
Gross Beta Samples from all locations were analyzed for concentrations of gross beta (Table C-VIII.1). Results ranged from <.7 to 4 pCi/1. Results from the control location were slightly higher than those from the indicator locations.
Results were within the range found in the PBAPS preoperational period.
Tritium j
Samples from all locations were analyzed for concentrations E
of aqueoud tritium (Table C-VIII.1). Values ranged from <40 5
to 170 pCi/1. There was no notable difference, between these results and those from previous years. B-
l(
Uranium Samples from all locations were analyzed for concentrations of uranium (Table C-VIII.1).
Positive concentrations of uranium were detected in all locations. Values ranged from
<.05 ug/l to.54 ug/1. Results were generally lower than recent years. Uranium is naturally occuring in most rocks and is not of plant origin.
Gamma Spectrometry Samples from all locations were analyzed for concentrations of gamma emitters semiannually (Table C-VIII.2).
Positive concentrations of Ra-226 and Th-228 were detected in several samples. The Ra-226 activity was determined by the presence I
of Pb-214 and Bi-214, two short-lived daughter products of Rn-222.
It was assumed that they were in equilibrium with Ra-226; however, after comparing these results with the cor-responding gross alpha data, it was determined that activity I
would best be attributed to the presence of Rn-222. Cesium-134 and Nb-95 activity at the detection limit (313 and 5 i 3, respectively) was observed at station IV and lu, respec-I tively. No differences were observed between indicator and control locations.
c.
Veoetation 5.
Samples from seven locations (1, 3A, 4N, 5, 6D, 8, and 23) were collected and analyzed. The control locations were 4N, 6D, and 8.
The following analyses were performed.
Strontium-89 and Strontium-90 Samples from all locations were analyzed for concentrations of Sr-89 and Sr-90 (Table C-IX.1).
Positive activities of Sr-90 were detected at all locations ranging from.0070 to I
.580 pCi/g (wet). These results were comparable to those of the previous year, as well as, preoperational data. Positive concentrations of Sr-89 were detected in four samples at or I
slightly above the detection limit, with no notable dif-ference between positive values at control and indicator locations.
Gamma Spectrometry Samples from all locations were analyzed for concentrations I
of gamma emitters (Table C-IX.2).
Positive concentrations of Be-7 and K-40 were detected in most samples with Be-7 ac-tivity ranging from <.06 to.52 pCi/g (wet) and K-40 activity ranging from 1.4 to 8.1 pCi/g (wet). Cs-137, Ra-226, and I
Th-228 were found in several samples and may be due to soil contamination. Other instances of positive activities of the l I
E E
remaining nuclides searched for were at or slightly above the detection limit and therefore are not considered significant.
l No notable difference between the indicator and control loca-tions was evident.
d.
Egfl Samples were collected from six locations (IAA, 2, 3A, 4N, 5, and 6G) semi-annually. Control locations were 4N and 6G.
m The following analyses were performed.
g Gross Beta Samples from all locations were analyzed for concentrations of gross beta (Table C-X.1).
Positive values were detected in all samples ranging from 1.5 to 5.4 pCi/g (dry). Results from indicator and control locations were not notably dif-ferent.
1988 results were within the range of PBAPS preoperational data.
Strontium-89 and Strontium-90 Samples from all locations were analyzed for concentrations a
of Sr-89 and Sr-90 (Table C-X.1).
Positive values of Sr-90 g
were detected in all samples with activities ranging from
.050 to.260 pCi/g (dry). The highest activities were found at location 3A, with a mean of.171 pCi/g (dry). Sr-89 con-l centration was slightly above the detection limit in one a
sample, probably due to counting statistics. There was no notable difference between the 1988 Sr-89 and Sr-90 results and those of previous years.
Gamma Spectrometry Samples from all locations were analyzed for concentrations of gamma emitters (Table C-X.1).. Positive concentrations of K-40, Cs-137, Ra-226, and TF-228 were detected at all loca-E tions. Concentrations of Be 7, Cs-134 and Ce-131 at or 5l slightly above the detection limit were found at several i
locations. There was no notable difference between the 1988 lI cesium results and those of previous years.
C.
Ambient Gamma Radiation Ambient gamma radiation levels were measured at forty-seven loca-j tions (as described in the program description section) using
]
CaSO :Dy thermoluminescent dosimeters (Tables C-XI.1 through C-g' 4
XI.4 and Figures C-11 and C-12). Most monthly and all quarterly g
TLD readings were below 10 mR/std. month with a range of 3.0 to 12.3 mR/std. month for the monthly's and 2.7 to 7.5 mR/std. month for the quarterly's. No notable differences were observed among E
site-boundary, middle, and outer ring measurements. Tht. data in-E dicated that operation of PBAPS did not affect the existing am-j bient gamma radiation levels.
g 3
- t-
- I I
I-
-I REFERENCES E
I 1
I I
8 I
I I
$ I I
I 3
l
'I V.
References 1.
Preoperational Environs Radioactivity Survey Summary Report, March, 1960 through January, 1966.
(September 1967).
2.
Interex Corporation, Peach Bottom Atomic Power Station Regional Environs Radiation Monitoring Program Preoperational Summary Report, Units 2 and 3, 5 February 1966 through 8 August 1973, June 1977, Natick, Massachusetts.
3.
Radiation Management Corporation Publication, Peach Bottom Atomic Power Station Preoperational Radiological Monitoring Report for lI Unit 2 and 3, January, 1974, Philadelphia, Pennsylvania.
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APPENDIX B: SAMPLE DESIGNATION AND LOCATIONS LIST.OF TABLES AND FIGURES TABLES TABLE B-I:
Sample Collection and Analysis Program for the Radiological I
Environmental Monitoring Program, Peach Bottom Atomic Power Station, 1988 FIGURES FIGURE B-1:
Environmental Sampling Locaticns on site or near the Peach Bottom Atomic Power Station FIGURE B-2:
Environmental Sampling Locations at Intermediate Distances from the Peach Bottom Atomic Power Station FIGURE B-3:
Environmental Sampling Locations at Remote Distances from the Peach Bottom Atomic Power Station I
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i DATA TABLES AND FIGURES PRIMARY LABORATORY I
I I
E.
I il I
I I
I
d L
APPENDIX C:-
DATA TABLES AND FIGURES - PRIMARY LABORATORY TABLES Table C-I.1 Analytical Data for Surface Water Grab Samples Col-I lected in the Vicinity of PBAPS, 1988.
Table C-I.2 Analytical Data for Surface Water Composite Samples j
Collected in the Vicinity of PBAPS, 1988.
Table C-I.3 Concentrations of Gamma Emitters in Surface Water i
Grab Samples Collected in the Vicinity of PBAPS,
-I_
1988.
Table C-I.4 Concentrations of Gamma Emitters in Surface Water I
Composite Samples Collected in the Vicinity of 1
PBAPS, 1988.
Table C-II.1 Analytical Data for Drinking Water Composite Samples I
Collected in the Vicinity of PBAPS, 1988.
Table C-II.2 Concentrations of Gamma Emitters in Drinking Water I
Composite Samples Collected in the Vicinity of PBAPS, 1988.
Table C-III.1 Concentrations of Sr-89 and Sr-90 in Fish Samples I_
Collected in the Vicinity of PBAPS, 1988.
Table C-III.2 Concentrations of Gamma Emitters in Fish Samples Collected in the Vicinity of PBAPS, 1988.
Table C-IV.1 Analytical Data for Silt Samples Collected in the Vicinity of PBAPS, 1988.
Table C-V.1 Concentrations of Gross Beta Radioactivity in Air Particulate Samples Collected in the Vicinity of
'I PBAPS, 1988.
Table C-V.2 Monthly Mean Values of Gross Beta Concentrations 8
(E-3 pCi/cu. meter) in Air Particulate Sampics Col-1ected in the Vicinity of PBAPS,1988.
'g fable C-V.3 Concentrations of Gama Emitters in Air Particulate g
Samples Collected in the Vir.inity of PBAPS,1988.
1 I
Table C-V.4 Additional Gamma Emittin9 Wuclides Found in Air Par-I ticulate Samples Collected in the Vicinity of PBAPS, 1988.
Table C-VI.1 Concentrations of I-131 in Air Iodine Samplet Col-lected in the Vicinity of PBAPS, 1988.
I I
I Table C-VII.1 Analytical Data for Milk Samples Collected in the Vicinity of PBAPS, 1988.
Table C-VII.2 Average Concentrations of I-131 in Milk Samples Col-lected in the Vicinity of PBAPS, 1988.
Table C-VII.3 Concentrations of I-131 in Milk Samples Collected in Vicinity of PBAPS, 1988.
Table C-VIII.1 Analytical Data for Well Water Samples Collected in 3
the Vicinity of PBAPS, 1988.
5 Table C-VIII.2 Concentrations of Gamma Emitters in Well Water a
Samples Collected in the Vicinity of PBAPS,1988.
g Table C-IX.1 Concentrations of Sr-89 and Sr-90 in Vege.tation Samples Collected in the Vicinity of PBAPS, 1988.
Table C-IX.2 Concentrations of Gamma Emitters in Vegetation Samples Collected in the Vicinity of PBAPS, 1988.
Table C-IX.3 Additional Gamma Emitting Nuclides Found in Vegeta-tion Samples Collected in the Vicinity of PBAPS, 1988.
Table C-X.1 Analytical Data for Soil Samples Collected in the Vicinity of PBAPS, 1988.
Table C-XI.1 Monthly TLD Results for Peach Bottom Atomic Power Station, 1988.
Table C-XI.2 Quarterly TLD Results for Peach Bottom Atomic Power Station, 1988.
Table C-XI.3 1988 Mean TLD Results from Peach Bottom Atomic Power Station for the Site Boundary, Middle, and Outer Rings.
Table C-XI.4 Summary of the 1988 Ambient Dosimetry Program for Peach Bottom Atomic Power Station.
Tat,le C-XII.1 Summary of Collection Dates for Samples Collected in the Vicinity of PBAPS, 1988.
-tioures Figure C-1 Monthly Insoluble Grcss Beta Concentrations in Sur-ll face Water Samples Collected in the Vicinity of a
PBAPS, 1988.
Figure C-2 Monthly Soluble Gross Beta Concentrations in Surface Water Samples Cnilected in the Vicinity of PBAPS, l
1988.
E
i I
Figure C-3 Monthly Insoluble Grcss ~ Beta Concentrations in Drinking Water Samples Collected in the Vicinity of PBAPS,-1988.
Figure C-4 Monthly Soluble Gross Beta Concentrations in Drink-I ing Water Samples Collected in the Vicinity of PBAPS, 1988.
'I Figure C-5 Mean Annual Sr-90 Concentrations in Fish Samples Collected in the Vicinity of PBAPS, 1971-1988.
Figure C-6 Mean Annual Cs-137 Concentrations in Fish Samples I
Collected in the Vicinity of PBAPS, 1971-1988.
Figure C-7 Mean Annual Cs-137 Concentrations in Silt Samples Collected in the Vicinity of PBAPS, 1971-1988.
Figure C-8 Mean Weekly Gross Beta Concentrations in Air Partic-ulate Samples Collected in the Vicinity of PBAPS, I
1988.
Figure C-9 Mean Monthly Gross Beta Concentrations in Air Par-I ticulate Samples Collected in the Vicinity of PBAPS, 1970-1988.
Figure C-?0 Mean Annual Cs-137 Concentrations in Milk Samples I_
Collected in the Vicinity of PBAPS, 1971-1988.
Figure C-11 Mean Monthly Ambient Gamma Radiation Levels (TLD) in the Vicinity of PBAPS, 1988.
Figure C-12 Mean Quarterly Ambient Gamma Radiation Levels (TLD) in the Vicinity of PBAPS, 1973-1988.
I I
.I g
I:
I I
l TABLE C.I.1 ANALYTICAL DATA FOR SURFACE HATER GRAB SAMPLES COLLECTED IN THE VICINITY OF f'DAPS,1988 RESULTS D4 LA4ITS OF PCI/ LITER i 2 SIGMA COLLECTIO4 GROSS ALPHA CROSS ALPHA GROSS BETA GROSS BETA AQUEOUS H3 STATIO4 DATE SOLtJOLE INSOLUDLE SOLUBLE INSOLUDLE TOTAL I
13A 01/30/OS
<.3
.3 1.1 2.6 1.0 1.3 1.4 0 U27/80
< 7
.12 1.07 2
11
<.4 04/02/06
<.4
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04/30/S8 (1)
(1) 3.2 1.7 1.8 2.5 05/28/60 C 4 4
i.2 3.5 1.9 1.2 i.6 06/06/06
< 9 00 $.07 3
11
<.6 04/30 06/26/06 60 1 40 I
07/30/60
< 1
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11
(
4 09/03/00
< 9 05 1.06 5
11
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,9 1.7
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11
.6 i.4 07/30-09/30/06 C 100 11/05/06
< 1
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11
< 5 1 U04/68
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<.7
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11
< 5 11/05 12/31/86 140 2 50 5-ME#4
.7 1.5
.31 1 1.14 1.3 1 2.1 1.2 1 2.6 93 1 72 13D 01/29/0S
< 5 6
12 3.5 i.9 5.2 i.7 CU26/88
< 6 2
11 3
11 10 11 03/10/06
< 3
<.05 2.7 1.9 C 4 8
04/28/06
< 6
<.04 2.8 i.9
<.6 05/26/88
< 5
.6 i.3 2.7 1.9
<.6 06/17/88
<.6 4
12 2.8 i.9 4.0 1.9 07/2 USS
<.7
.2 1.1 4
11
.7 i.4 08/26/06
<.6
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11 4.3 i.6 5
09/23/00 2 11 15 1.00 3
11 9
2.4 10/20/00 C 9
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11
< 5 11/18/80
< 7
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11 1.2 i.5 12/09/00 C 5 1.0 i.4 1.9 i.9 6.1 1.9 MEAN 7
1.9 1.3 1 3.7 3.2 1 1.7 2.9 i 6.1 I
(1) SEE PROGRAM EXCEPTIQ45 SECTIO 4 FOR EXPLANATION E
I 8
4 1
I l
8 1
j
TABLE C-I.2 AtMLYTICAL DATA FOR SURFACE HATER COMPOSITE SAMPLES i
COLLECTED IN THE VICINITY OF PBAPS, 1900 l
RESULTS IH LA4ITS OF PCI/ LITER 1 2 SIGMA
- COLLECTION GROSS ALPHA GROSS ALPHA GROSS BETA GROSS BETA AQUEOUS H3 STATION PERIOD SOLUDLE IIISOLUDLE SOLUDLE INSOLUDLE TOTAL
.......c.....
tLL 01/01 01/29/08
<.5 4
1.2 2.9 1.6 1.4 1.4 01/29 02/26/08
< 6 13 1.08 2
21 5
1.5 02/26 04/01/06 C.7
.3 1.1 2.3 i.9
.6 2.4 01/01 04/01/80 210 1 60 04/01 04/29/08
<.3 2
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i.5 04/29 05/27/08
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1.6 05/27 06/24/86
< 7 4
i.2 2.0 i.9
<.6 04/01 06/24/06 110 1 50 06/24 07/29/06 3 12 5
1.2 5
i1 1.1 i.5 07/29 09/02/0S
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11 1.5 i,5 i
09/02 09/30/00
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11
<.5 11/04 11/25/0S
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< 5 06 1.05 1.4 i.9 6
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MEAN.9 1 1.6
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.6 1.7 135 i 101 1rti 01/01 01/29/88 C 5 1%
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04/01 04/29/88
<.3
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<.5 1.4 1.6 2.7 i.6 4.6 1.6 05/27 06/24/80 C.6 12 1.07 1.9 i.6
<.6 0*/01 06/24/00 70 1 30 06/24 07/29/00 2
1.1 4
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<.7 09 i.07 4
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< 90 09/30 11/04/06 3 11
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<.5 13 1.09 2.6 i.9 1.2 i.5 12/02-1 U30/08
<.4
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l TABLE C.II.1 ANALYTICAL DATA FOR DRDKDE NATER COMK$ITE SAMPLES COLLECTED IN THf VICD4ITY OF PBAPS,1906 RESULTS IN LHITS OF PCI/ LITER 1 2 SIGMA COLLECTION GROSS ALPHA GROSS ALPHA GROSS BETA GROSS BETA I.131 ASJEOUS H3 STATION PERIOD SOLUBLE INSOLUBLE SOLL2LE INSOLL2LE TOTAL TCTTAL I
4L 01/01 0?/30/08 C.6
.14 2.00 3.0 t.8 1.0 2.4 01/23 01/30/C6 C 06 01/30.C U27/86 C.4
.2 1.1 2
11 6
1.5 02/20 02/27/06 C. 05 I
02/27 04/0t/88 C 4 14 1.09 1.6 i.6 7
1.4 03/26 04/02/BS C 99 01/01 04/02/88 90 1 80 04/02 04/30/86 C.3
.4 1.t 2.4 1.6 1.5 1.5 04/30/06 C 04 I
04/30 05/28/00.6 2.6 15 t.09 3.1 1.9 C.6 05/t1 05/ttVDo C.1 05/26 06/26/06 C 6
.3 1.1 2.0 t.9 C.6 OW16 0VtV66 C 06 04/02 06/26/88 90 2 50 5
0UtdL.07/30/Se
< 5 12 2.06 6
11 2.9 i.6 07/22 07/30/06 C 06 07/30 09/03/06 C 1
.2 1.1 4
11 9
1.5 08/27 09/03/86 C*
09/03 09/30/85 1.2 1.9 13 1.0S 3
11 6
1.4 I
09/t3 09/30/80 C.07 06/26 09/30/88 C 90 09/30 11/05/08 C.6 C 1 5
11 C 5 10/29 11/05/86 C.05 8
11/05 12/04/08 C 4 C.06 4
11 1.5 2.5 11/26 1 U O4/BS C.09 1UO4.t u31/SS C 4 C.03 1.4 2.9 C 5 12/24 12/31/SS C 05 09/30 12/31/65 130 1 40 MEN 4.6 1.5
.16 1.20 3.2 1 2.7 1.0 1 1.4 C 07 100 1 40 62 01/02 01/30/56 C.5 11 1.07 3.5 1.9 1.1 1.4 01/23 01/30/06 C 06 I
01/30 0 Ut7/05 C.5 6
i.t 1
11 1.2 1.5 CU20 0U27/06 C.07 O U27 04/0Use C.6 1.0 1.6 2.6 1.9 2.3 1.6 03/26 04/0 VOS C 00 01/02 04/02/06 250 t 60 04/02 04/30/08.7 1.5 1.7
- .4 2.5 1.7 1.9 1.5 04/23.04/30/ce
<.05 04/30 05/26/D6 C 5 5
1.2 3.9 1.9 2.3 1.7 05/21 05/28/68 C.1 05/t6 06/t6/06 C.7 12 t.00 4
11
(
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06/19 0U26/De C 05 04/02 06/26/86 C 40 06/t6-07/30/88 C.6
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11 9
2.5 07/24 07/30/06 C.
07 I
07/30 09/03/SS 1 11 7
1.2 5
11 1.2 1.5 OS/27 09/03/86 C 1 09/03 10/01/06 C.7 11 1.06 2.9 2.9 5
1.4 09/24 10/01/06 C 00 D Vt6 10/01/DS 150 t 90 1
10/01 11/05/0e 1
C.06 4
21 C 5 10/29 11/05/ee C.07 11/ f.2/04/BB C 5
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11 9
i.5 11/. e.12/04/85 C.07 12/04 12/31/B0.7 1.6 C.07 1.4 i.9 C 5 5
12/24 12/31/88 C.05 10/01 12/31/08 160 1 50 MEAN.7 1.4 45 1 1.00 3.3 1 2.5 1.2 1 1.3 C.07 150 1 172 I
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TABLE C.III.1 COCDRRATIONS OF SR-09 AND.90 IN FISH SAMPLES COLLfCTED IN THE VICINITY OF PBAPSe 1966 l
l l
PCI/ GRAM (ASH)
PCI/ GRAM (MET) l t t SIONA 1 2 SIGPtA i
COLLECTION I
STATION MEDIA DATE SR-69 SR.90 SR-69 3R.90 1EE CATFISH 04/05/68 C.2 59 1.06 C.01
.029 1.004 l
06/01/86 C.2
.60 1.07 C.02 051 1.005 09/06/86 C 1 1.3 2.1 C 06 066 1.005 l
ME.AN C 5
.90 t.73 C.43 049 1.039 1X CATFISH 04/05/86 e.1
.60 2.05 C 007 033 1.003 06/01/06 C 3 44 2.06 C.01 020 2.003 I
09/06/06 C.3 46 2.07 C 02 023 1.003 11/03/06 C.3
,. 95 1.05 C.02 057 1.003 MEAN C.3
.61 1.47 C.014
.033 2.034 I
4I CATFISH 03/30/06 C 4 1.1 2.2 C.01
.030 t.005 06/15/06 C 4
.6 2.2 C 02
.036 1.006 09/23/80 C.3
.76 2.00 C.01 045 1.005 10/1 W06 C 4
.7 2.1 C.02
.033 1.005 NEAN
< 4
.e5 1.35 C.02
.037 2.013 SN BASS 03/24/08 C.3 34 2.07 C.02 019 1.004 06/15/SS C 2 43 *.06 C 006
.020 t.003 3
09/07/06 C 4
.22 1.09 C.01 000 2.003 i
10/1 FSS C.7
.3 1.1 C.03
.011 *.004 MEAN C 4 32 1.17 C 017 015 2.012
- I 4J CATFISH 04/06/86 C 4 62 1.07 C 01 026 1.003 06/15/06 C.3
.6 2.1 C 01
.036 1.005 09/14/06 C.6 1.0
- .4 C
03 05 1.02 10/18/80 C.2
.74 2.09 C.01 034 1.004 NE.AH C 4 79 1.32 C 02 037 1.020 SM BASS 04/0b/83 C.6
.2 1.2 C.02 007 1.005 06/15/06 C.2 4
2.1 C 01 021 *.005 09/06/06 C.3 41 1.05 C.01
.010 t.002 5
10/18/60 C 5 5
2.1
< 02
.021 1.006 MEAN C 4
.36 1.25 C.02
.017 1.013 6
CATFISH CVte/SS C 7 60 t.09 C 03 070 2.004 I
06/10/06 C.2 47 2.08 C.006 022 2.004 09/20/06 C 6 1.38 1.00 C 03 001 *.005 10/24/06 C.6 61 1.06 C.03 020 2.004 5
MEAN
<.5 77 1.63 C 025 040 t.055 SM BASS 03/26/06 C 3
.7 1.1
( 01 025 1.004 06/20/85 C 1 47 1.06 C 006
.029 1.004 09/20/B6
.3 1.2 5
1.1 01 1.01 022 t.005 (1) 10/24/88 MEAN
.2 1.2 56 1.25 009 1.002 025 1.007 MEAN CATFISH C 4
.78 2.54 C.019 039 1.033 I
SM BASS 4
1.4 41 2.26 014 2.014 018 i.014 (1) SEE PROGRAM EXC.EFTICNS SECTION FOR EXPLANATION I
I I
I TABLE C.III.2 CacDtrRATIGHS OF GAMMA EMITTERS IN FISH SAMPLES COLLECTED IN THE VICINITY OF PBA G. 1965 W
RESULTS IN LHITS OF PCI/ GRAM (HET) t 1 SIGMA STATION COLLECTIO4 CODC DATE MEDIA BE.7 K.40 h 54 CO.56 FE.59 1EE 04/11 CATFISH C.07 1.6 1.2 C 000 C.006 C.02 06/01 CATFISH C 1 3.0 t.3 C.01 C.01 C 04 09/06 CATFISH 13 1.09 3.1 1.3 C.009 C.01 C.03 MEAN CATFISH
.10 t.06 2.9 1 1.0 C 009 C.009 C 03 1X 04/13 CATFISH C 04 1.8 1.1 C.004 C 004 C.91 06/01 CATFISH C 1 3.6
- .3 C 01 C.01 C.03 09/06 CATFISH C 07 2.3 2.2 C.007 C 000 C.02 11/03 CATFISH C.06 1.3 1.2 C.006 C 007 C 02 MEAN CATFISH C 07 2.5 2 1.5 C.007 C.007 C 02 41 03/24 SN BASS C 06 2.4 i.2 C 007 C.006 C.02 03/30 CATFISH
.07 1.06 1.0 t.2 C 007 C.000 C 02 06/15 CATFISH C 09 2.6
- .3 C 009 C 01 C 03 SN BASS C 08 3.2 1.3
- 009 C.009 C.03 09/07
$N BASS C 00 3.3 1.2 C 009 C.009 C.05 09/23 CATFISH C.09 3.1 1.3 C 009 C.01 C 03 10/10 CATFISH C.09 2.6 1.2 C 008 C.01 C.03 SN BASS C,08 3.3 1.2 C 000 C 009 C.02 i
MEAN CATFISH
.09 2.02 2.6 1 1.1 C 000 C 010 C 03 SN BASS C.06 3.1 1.9 C 000 C 009 C.03 4J 04/05 SN BASS C.04 1.5 t.1 C 005 C.005 C.01 04/06 CATFISH C.05 1.3 1.2 C 006 C.007 C.02 06/15 CATFISH C.08 2.5 1.2 C 006 C 000 C.02 SN BASS C.07 2.0 1.2 C 007 C.007 C.02 09/06 SN BASS C.07 3.7 1.2 C 007 C.000 C 02 09/14 CATFISH C.05 1.9 1.2 C 006 C.006 C.02 10/16 CATFISH C.2 5.7
- .5 C 02 C.02 C.06 SN BASS C.06 3.4 1.2 C 007 C.000 C.02 I
MEAN CATFISH C.10 2.9 2 3.9 C 010 C 010 C 03 SN BASS C.06 2.7 1 2.1 C 007 C 007 C.02 6
0F2B CATFISH C 08 1.8 i.2 C.006 C.009 C 08 SN BASS C.07 1.0
- .2 C.007 C 000 C 02 06/20 CATFISH C 08 4.0 t.3 C 009 C 01 C.03 SN BASS C.07 3.1 1.2 C.00S C.009 C 02 09/20. SM BASS C.05 2.2 1.2 C 006 C 006 C 02 09/20 CATFISH C 09 3.0 1.2 C 009 C 01 C 05 10/24 CATFISH C 07 2.6
- .2 C.009 C.009 C 02 3
SN BASS C 06 3.0 t.2 C.006 C.007 C.02 MEAN CATFISH C 00 2.9 1 1.6 C 009 C.010 C.03 SN BASS C 06 2.5 1 1.3 C.007 C.006 C 02 MEAN ALL STATIONS CATFISH 06 1.07 2.7 1 2.1 C 009 C 009 C.03 SN BASS C 07 2.7 1 1.4 C.007 C.000 C 02 E
l I
E E'
l l
7.
j ~
I TABLE C.III.2 C04CENTRATIO43 OF GArt1A DiITTERS IN FISH SAMPLES COLLECTED IN THE VICINITY OF PBAPS,19%
RESULTS IN WITS OF PCI/ GRAM (WET) 1 2 SIGNA STATION COLLECTICH CODE DATE MEDIA CO.60 ZN-65 IB.95 CS.134 C5 136 1EE 04/11 CATFISH
< 009
<.02
< 01
< 000 C.02 I
06/01 CATFISH
<.01 06 2.03 C.02 04 2.01
< 05 09/06 CATFISH 10 t.01
.14 1.03
<.01
.13 1.01
< 03 MEAN CATFISH 040 1.105 07 1.12
< 01 059 1.127 C.03 I
1X 04/13 CATFISH
< 005 C 01
< 005 C 004 C 006 06/01 CATFISH
< 01
<.02
<.01
< 01
< 04 09/06 CATFISH
< 009
<.02
< 009 C.006
< 02 11/03 CATFISH
<.000 C 02
< 007 000 t.007
<.01 I
MEAN CATFISH
< 006 C 02
< 006
.000 t.005 C.020 4I 03/24 SN BASS C.000 C 02
< 01 007 1.007 C 03 5
03/30 CATFISH
<.009
<.02
<.009
<.007 C 02 06/15 CATFISH
< 01
<.02 C
11
< 009 4
<.04 SN BASS
< 01
< 02 C.01
<.009
< 03 09/07 SN BASS
< 01
< 02
< 01
<.006
< 03 09/23 CATFISH
< 01
< 02 C.01
< 009
< 05 3
10/13 CATFISH
< 010 C 02
< 010
.009 1.003
< 04 SN BASS
< 009 C.02
<.01
< 000 C 03 MEAN CATFISH
< 009
< 02
< 010
.009 1.003 C 04 SN BASS
< 009
< 02
< 01 000 t.002
<.03 I
4J 04/05 SM BASS
< 006 C 01
<.005 C 005 C 01 04/06 CATFISH
<.007 C 02
< 006
< 006 C 02 06/15 CATFISH
<.009
.02 1.02
< 01
< 000 C.02 i
SN BASS
< 000
< 02
< 009 006 1.006
< 03 09/06 SN BASS C 009 C.02
< 01 011 2.006
<.02 09/14 CATFISH
<.007
< 01
<.007 C 007
<.02 10/10 CATFISH
<.02
<.05 C 03
< 02
< 06 SM BASS C 000
< 02
.01 2.01
< 007 C.03 I.
MEAN CATFISH
< 011
.03 i.03
< 014
< 010 C 04 SN BASS
<.000 C 02 009 i.005 007 1.005 C.02 5
6 03/26 CATFISH
<.009 C.02
<.01
<.006
< 03 SM BASS
<.000 C.02
< 009 C 007
< 02 06/20 CATFISH
<.01
<.02
< 01
(
009
.03 2.03 SM BASS
<.009
<.02 C.01
< 000 C 02 09/20 SM BASS
<.007 C 01
< 006 C 006 C 01 I
09/20 CATFISH
<.01
< 02
<.01
<.006
< 05 10/24 CATFISH
< 01
< 02
< 01
<.000
< 02 SM BASS
<.000 C.02
<.000
<.007
< 01 MEAN CATFISH
<.010
< 02
<.01
<.006 03 i.03 5
SM BASS
<.005 C 02
<.006
<.007
< 02 NEAN ALL STATIONS CATFISH 014 1.042
.03 1.06 C 011 017 i.057 032 2.036 SM BASS
<.005 C 02 009 2.003 007 1.003 C 02 I
I l
8
_______________J
I:
TABLE C.III.2 CONCDURATIOt45 OF GArt% EMITTERS IN FISH SAMPLES COLLECTED IN THE VICINITY OF PBAPS,1960 W
RESULTS IN ANITS OF FCI/ GRAM (HET) 1 2 SIGr%
i STATION COLLECTION CODE CATE MEDIA CS-137 CE-141 RA.226 TH-226 1EE 04/11 CATFISH
< 009 C 01
<.02
<.02
{
06/01 CATFISH
.10 t.01
< 02 07 1.02 05 1.03 09/06 CATFISH
.27 1.02 C 02
< 02 C 0L MEAN CATFISH 126 1.265 C 02
.04 1.06 03 1.03 1X 04/13 CATFISH 010 t.005 C.006 C 009 C 01
=
06/01 CATFISH
< 01
< 02 03 1.02
< 0'l i
09/06 CATFISH
<.006
< 01
(.02 C.01 11/03 CATFISH 017 1.006 C 01
<. 'd l C 0.2 MEAN CATFISH 011 1.006 C 012 017 1.020
- 01 4I 03/24 SM BASS 019 2.007 C 01
<.01
<.02 05/30 CATFISH 008 1.000 C 01
<.01
< 02 06/15 CATFISH
.011 2.009 C.02
<.02
< 05 SN BA$$
.012 2.009
< 01
< 02
< 05 09/07 SN BASS 016 2.009 C 02
< 02
<. 0,!
09/23 CATFISH
.01 1.01
< 02
<.02 0'l 10/18 CATFISH 023 1.009 C 02 C.02 C 0;!
SN BASS 013 2.009 C 02
< 02 0.!
MEAN CATFISH 014 i.014 C.02
<.02 C 08 SM BASS
.015 1.006 C.02
<.02 0,1 4J 04/05 SM BASS
.016 i.005
<.007
<.01
< 01 04/06 CATFISH
.009 2.006 C 01
<.01 0,!
06/15 CATFISH 015 1.009
< 01 02 i.02 03 1.02 SM BASS 013 2.007
< 01
<.01 0.2 09/06 SN BASS 027 2.006
< 01
<.02
< 0;t i
09/14 CATFISH 017 2.006
< 01
<.01
< 0l!
10/10 CATFISH
<.02
< 03
<.04
<.05 SM EASS 014 2.007 C.01
<.01
< 02 MEAN CATFISH 015 2.009
<.02 02 1.03 03 2.03 SM BASS
.016 1.013 C 009
<.01
< 02
'6 03/20 CATFISH
<.009 C 01
<.02
<.02 SN BASS
<.007
< 01
<.01
<.02 5
06/20 CATFIS9 01 1.01
< 02
.02 2.02
< 03 SM BASS C 000 C 01 02 1.02 C 02 09/20 SM BASS C 006
<.006
<.01
<.02 09/20 CATFISH
<.009
<.02
<.02
<.03 10/24 CATFISH 010 1.009
<.01
<.02 C 02 SM BASS C.007
.01 1.01 02 1.01
<.02 I,
MEAN CATFISH 010 t.001
<.02 02 1.00 C 03 SN BASS
< 007 010 t.002
.02 i.01
<.02 MEAN ALL STATIDHS CATFISH 030 2.123 C.015
.022 i.026 03 1.02 SN BASS 013 2.012 011 2.006
.02 2.01
< 02 I
I I
E
TABLE C.IV.1 ANALYTICAL DATA FOR SILT SAMPLES COLLECTED D4 THE VICD4ITY OF PBAPS,1966 RESULTS IN tktITS OF PCI/ GRAM (DRY) i 2 SIGMA I
COLLECTION STATION DATE GPOSS ALittA GROSS BETA BE.7 K-40 CO.60 ZN-65 W
186 06/22/88 4.1 i.9 1.6 ' i.3 C.3 to i1
< 05
< 09 09/19/86 1.0 t.3
.6 i.2
< 09 10.0 t.4 03 i.01
< 03 MEAN' 2.6 1 4.4 1.3 1 1.4 C 20 19.0 1 25.5 04 1.03 C 06 I
1X 06/22/08 4.3 i.5 2.5 i.3
<.2 24 11
< 03 C 06 09/19/86 5.0 t.6 2.3 1.3 C.1 16.9 1.5 C.01
<.03 MEAN 4.7 1 1.0 2.4 i.3 C.2 20.5 1 10.0
< 02
< 05 I
4D 06/22/08 3.9 i.9 1.6 i.3 C 3 27 11
.12 i.05
< 1 09/19/08 5 11 3.0 1.4
. < 2 21.0 t.9
.to 1.04 13 1.07 MEAN 4.5 1 1.6 2.4 1 1.7
<.3 24.0 1 6.5
.20 i.23 12 i.04 5
4J 06/22/80 5 11 2.3 1.3
< 6 20 12 33 1.06
<.1 09/19/80 2.2 1.7 2.5 i.3 4
i.3 22 11
.27 i.05
.00 t.07 MEAN 3.6 t 4.0 2.4 i.5
.4 i.0 21 13 30 t.00 09 1.03 4T 06/22/88 4 11 3.6 i.4 C 4 29 12
<.05 C 1 09/19/80 4 11 3.6 1.4 C 4 24 11
< 05 C 1 MEAN 4 10 3.6 i.0
<.4 27 17 C.05
<.1 I
6F 06/22/88 2.0 i.4 1.0 t.3
< 2 15.1 1.9
<.03 C 04 09/19/66 1.9 1.5 9
1.3 C.1 0.1 1.5 C.02
< 03 1
MEAN 2.0 i.1 1.0 1.1
<.2 11.6 i 9.9
<.03
<.05 MEAN ALL STATIONS 3.5 1 2.0 2.2 1 2.0
.26 i.25 20.4 1 13.5
.11 1.23 06 1.07 I
I I
I I
I I
~
I I
1 I
TABLE C-IV.1 ANALYTICAL DATA FOR SILT SAMPLES COLLECTED IN THE VICD4ITT OF PBAPS,1900 l
RESULTS IN Lt4ITS OF PCI/ GRAM (DRY) 2 2 SIGM4 STATION COLLECTICH CDDE PERIOD I.131 CS.134 CS-137 CE.141 RA-tt6 TH 226 158 06/22 C.06
.06 1.04
.10 t.M C.06 1.1 2.1 1.4 1.1 09/19 02 1.02 C.009
.03 1.01 C 02
.31 1.03 42 1.04 NEAN 04 t.06
.045 1.100 07 1.10 C.M
.71 1 1.12 91 1 1.39 1X 06/22 C.04 C.02 C 03 C.05
.70 t.c7 9
1.1 09/19 C 02 C.01 C 01 C.03 47 1.M 71 1.05 MEAN
<.03 C.02 C.02 C.M 59 1.33
.04 i.18 4D 06/22 C.07 14 1.04
.20 2.05 0E 2.07 1.3 2.1 1.3 2.2 3
09/19 C.06
.24 2.93 50 t.04
.09 1.05 1.24 2.09 1.3 2.1 MEAN C 07
.19 1.14
.35 2.42 09 2.01 1.27 1.06 1.3 2.0 4J 06/22 C.09
.14 1.06 62 1.08 C 06 1.4 1.2 1.3 1.2 09/19 C 05
.23 2.04 70 2.05 C.05 1.20 2.09 1.4 2.1 MEAN
<.07
.19 1.15
.66 2.11 C 07 1.30 t.26 1.4 2.1 4T 06/22 C.2 C.04 51
- .07 C.09 1.6 1.1 2.2 2.2 M
09/19 C 09 C.04 4Q t.06 C.06 1.4 1.1 f.7 1.2 NEAN
< 15 C.04 46 1.16 C.09 1.5 2.3 2.0 t.7 6F 06/22 C 0S C.02 C 03 07 1.06 1.20 2.09 1.2 2.1 09/19 C.03 C 01
.07 1.02 C 03
.62 1.05
.09 2.07 MEAN C 06 C 02
.05 2.06
.05 1.06 1.01 1.54 1.05 2.44 MEAN ALL STATIONS 07 1.10
.002 1.171
.27 1.52 06 2.05 1.06 1.60 1.23 2.92 I
I I
I E
I I'
I E
TABLE C-V.1 CollCENTRATICHS OF GROSS BETTA RADIOACTIVITY IN AIR PARTICULATE SAMPLES COLLECTED IN Ti1E VICINITY OF PBAPS,1966 RESULTS IN UNITS OF E-3 PCI/CU. METER 1 2 SIGMA GRO ?D I. PEACH DOTTON SITE b4EEK 1A 15 2
I 1 45 25 27 13 33 13 2 57 15 53 15 54 15 3 29 24 26 14 21 14 4 17 14 30 15 54 i7 I
5 26 14 24 14 26 15 j
6 32 15 36 15 30 15 7 27 13 24 13 23 23 0 24 13 21 13 21 13 I
9 23 14 to i4 27 14 10 22 13 to i3 23 13 il 16 13 17 13 10 14 12 22 13 26 23 26 13 13 to i4 22 14 21 14 5
14 20 23 19 13 to i3 15 10 13 9
13 9
i3 16 19 23 21 13 24 13 17 21 23 25 14 20 13 16 14 22 19 23 13 12 I
19 22 14 24 13 22 13 20 14 13 11 13 15 23 21 17 12 15 23 10 22 22 30 13 36 23 35 i3 E.
23 25
- 4 24 14 22 14 24 33 13 34 23 34 13 25 31 14 37 14 33 14 26 15 13 15 13 10 13 27 37 i3 32 13 30 23 I
to 41 14 39 13 30 13 29 to i4 20 15 25 14 30 36 23 34 23 33 13 31 25 13 25 13 27 23 32 29 13 26 13 26 23 I
33 29 13 27 13 25 13 34 30 13 29 13 31 13 35 37 i3 33 14 37 13 36 26 13 to 13 25 13 I
37 31 13 33 13 32 13 30 28 13 to 13 to i3 39 35 13 32 13 32 13 40 26 13 25 13 29 13 41 27 13 20 t3 to i3 I
42 32 13 30 13
- S
- 3 43 31 23 29 i3 to i3 44 40 13 36 13 33 13 45 34 14 to i3 27 i4 I
46 to 13 27 13 32 13 47 25 23 30 13 25 13 46 33 13 34 13 36 23 49 41 14 41 14 38 14 50 41 14 42 14 46 14 51 44 14 43 14 41 14 52 42 14 39 13 36 13 MEAH 29 i to to i 16 to i to I
i I
I 1
u
)
TABLE C-V.1 COCDfTRATIQ45 OF GROSS BETTA RADIOACTIVITY IN AIR PARTICULATE SAMPLES COLLECTED IN THE VICD4ITY OF PBAPS,1966 RESULTS IN LA4ITS OF E-3 PCI/CU. METER 1 2 SIGMA CROUP II. INTERMEDIATE DISTANCE LOCATIO43 NEEK W
3A 4B 5
65 14 1 to 23 24 13 23 1 3' 27 13 29 i3 2 47 25 48 15 51 15 53 15 56 16 3 22 24 21 14 23 14 23 23 24 25 4 32 15 34 14 27 25 26 20 32 25 5 25 14
' 25 15 26 24 27 i5 to 15 6 33 15 31 25 29 24 30 15 31 14 7 23 13 24 13 20 23 23 14 27 13 8 22 24 25 14 20 24 20 24 21 14 9 67 10 25 14 29 i4 31 14 38 24 10 (1) 24 13 to 13 26 13 30 14 11 12 15 14 14 14 24 15 14 15 14 12 23 14 16 13 23 13 20 14 26 23 13 19 i4 16 24 16 14 21 24 22 24 14 17 13 17 23 16 23 19 13 22 14 15 10 14
<4 0
14 12 14 10 24 16 24 13 22 13 to 13 19 13 21 13 17 21 14 21 14 25 14 17 i3 23 14 j
10 15 12 14 12 13 22 14 12 13 12 l
19 21 13 19 12 20 23 23 13 22 13 l
20 14 13 14 23 11 23 13 13 to 13 21 19 13 16 12 to 22 to i2 20 13 22 31 23 34 23 33 13 35 14 40 24 23 23 24 20 14 19 24 16 24 24 14 24 31 23 34 14 36 13 36 13 38 13 25 34 14 36 14 39 24 35 14 30 24 j
26 17 23 16 13 17 13 16 23 24 13 27 29 13 32 13 39 13 35 13 40 23 to 38 23 30 13 42 14 42 24 42 14 i
29 25 14 25 14 23 13 27 i3 30 13 30 31 23 32 13 41 14 42 14 44 14 31 27 13 31 13 30 13 36 24 29 23 32 22 23 25 23 32 13 34 13 33 13 33 25 23 20 13 35 13 36 13 32 14 34 27 23 32 23 24 13 29 13 32 13 35 36 13 34 13 23 23 27 13 30 23 36 23 13 27 13 21 23 21 13 20 13 37 34 13 33 13 26 13 32 13 27 13 30 27 23 29 23 26 23 22 13 29 23 39 30 23 36 13 34 13 34 13 57 16 40 27 13 24 13 23 i3 26 13 20 23 41 28 23 30 23 24 13 23 13 34 14 42 29 13 31 23 31 23 33 13 31 13 43 29 13 29 13 27 23 26 13 31 13 l
44 36 13 35 13 35 13 15 i3 40 13 l
45 27 13 to 13 26 13 20 14 20 13
(.
46 25 23 to i3 34 14 33 24 36 24 47 23 23 26 23 32 24 29 24 to 24 40 Ja i3 26 23 34 13 36 23 35 13 49 39 24 3S 24 35 14 42 25 44 25 50 43 14 40 14 43 14 40 tc 36 13 51 40 14 40 24 45 15 40 14 42 24 52 43 14 (1) 37 13 41 24 36 23 MEAN 20 1 20 27 1 17 27 1 16 20 t to 30 2 20 l
5' 1
(1) SEE PROGRAM EXCEPTIIO43 SECTIO 4 FOR EXPLAHATIO4 l
I' I
t
___.____O
TABLE C.V.1 Cot 4CDURATI0 tis OF GROSS BETTA RADIOACTIVITY IN AIR PARTICULATE I.
SAPtPLES COLLECTED D4 THE VICINITY OF PBAPS,1908 RESULTS IN LAiITS OF E 3 PCI/CU METER 1 2 SIONA GROUP II. DRERMEDIATE DISTANCE LOCATIONS 15 17 31 32 33A 3e I-1 27 13 28 13 27 i3 26 13 27 23 to i3 2 45 25 49 25 49 25 53 15 52 25 56 26 3 19 i5 25 15 21 14 23 14 21 14 30 15 4 22 14 31 25 29 14 31 15 27 14 31 15 I
5 25 15 26 15 29 24 to i5 25 14 26 15 6 35 14 25 14 to 14 30 24 31 14 39 i5 7 23 23 25 23 2/
13 24 13 to i3 27 13 8 20 14 23 14 22 13 20 13 22 13 24 24 9 34 14 29 i4 16 13 35 24 31 24 30 14 I
10 25 23 25 i3 24 13 27 23 25 23 22 14 11 13 14 16 24 17 13 16 i4 15 13 to 14 12 21 23 23 13 25 13 22 23 24 13 21 24 13 10 14 22 24 22 24 to 14 19 i4 21 14 14 22 23 17 i4 19 23 25 13 27 13 26 23 5
15 8 24 9
24 10.
t4 10 14 9
13 11 24 16 20 23 21 23 23 23 21 23 22 23 21 23 17 25 14 22 14 19 24 24 14 24 14 22 14 to 15 12 15 12 14 12 13 13 14 12 12 12 5
19 24 13 21 23 22 13 23 13 22 13 24 13 20 11 14 to 13 14 13 13 14 13 24 13 13 21 10 23 17 12 17 12 17 12 29 i5 17 12 22 35 14 32 23 31 23 33 14 37 i4 38 14 23 19 24 20 14 19 13 21 14 22 24 19 13 I
24 35 23 34 13 38 23 33 23 35 13 32 13 25 34 14 37 14 39 14 37 24 37 14 35 14 26 17 13 16 23 17 13 16 13 26 23 25 23 27 37 13 36 23 34 13 37 13 28 13 39 13 I
20 43 i4 45 14 40 13 42 14 46 14 42 13 29 29 13 16 13 22 13 27 13 27 13 27 23 30 43 14 41 14 41 14 47 24 47 15 41 14 31 33 13 35 23 35 13 to i3 30 13 31 23 32 31 23 29 14 30 13 31 23 30 13 32 13 I
33 33 23 30 13 33 13 34 13 31 13 41 14 34 33 13 32 23 31 23 31 23 33 23 31 13 35 26 23 24 23 27 13 to i3 27 13 30 23 36 19 23 19 13 to 23 20 23 19 23 24 13 37 33 23 27 23 25 23 31 23 32 13 24 13 I
30 19 13 29 13 27 23 25 23 27 13 31 13 39 32 13 34 23 30 13 33 13 34 23 36 14 40 22 t2 25 13 22 22 20 t2 20 t2 23 t2 41 to t3 24 23 25 13 31 23 33 13 29 23 5
42 31 13 to 13 30 13 30 13 31 14 30 23 43 25 23 29 23 29 23 26 23 to i3 32 13 44 33 14 36 23 38 13 37 13 37 23 34 13 45 31 24 ES i3 26 13 26 13 26 23 26 13 46 36 24
- '3 i4 37 24 35 24 36 24 35 24 I
47 29 23 29 t3 20 13 32 14 29 13 30 23 46 32 13 36 23 34 23 32 13 37 23 45 16 49 36 24 37 14 35 24 42 15 42 15 47 25 50 35 14 39 i3 40 23 37 13 41 24 42 14 I
51 31 24 43 15 47 15 41 14 30 24 43 25 52 36 13 32 23 36 23 36 13 39 23 40 13 MEAN 28 t 17 to i 17 26 1 17 26 i to 29 1 to 30 1 19 I
1 1
I I
I
I j
TABLE C.V.1 COCDITRATIO43 OF GROSS BETTA RADIOACTIVITY IN AIR PARTICULATE SAMPLES COLLECTED IN THE VICINITY OF PBAPS,1900 RESULTS IH LA4ITS OF E-3 PCI/CU. METER i 2 SIGMA GROUP 'III - DISTANT LOCATIO43 NEEK 12A 120 1 32 14 36 14 2 36 14 30 14 3 22 15 21 15 4 25 14 17.
14 5 30 15 24 15 6 26 23 26 23 7 23 13 23 13 8 21 23 19 13 j
9 26 13 20 23 10 24 13 23 23 11 15 13 to 13 12 21 22 20 t2 13 22 12 21 12 14 9 23 12 14 15 9 13 11 13 16 26 24 24 24 17 20 t4 20 14 15 19 i3 20 13 19 20 13 10 12 20 14 12 15 12 21 21 22 19 12 22 23 14 22 14 23 29 24 21 14 24 36 i3 39 23 25 27 14 30 14 26 14 12 14 12 27 38 24 30 14 I
2e 33 13 37 24 I
I 29 21 14 19 i4 30 38 13 35 13 l
31 24 24 22 14 32 19 23 22 13 33 21 23 21 13 34 23 13 22 13 35 19 12 10 12 36 23 23 23 13 i
37 21 23 23 i3 15 (1)
(1) g i
39 26 23 26 i3 40 17 22 17 12 41 21 23 20 23 42 16 22 14 12 43 21 13 25 13 44 22 12 23 13 45 to i3 21 13 46 26 23 20 14 47 27 23 22 13 4B 21 23 27 13 49 26 13 25 23 50 48 14 26 13 51 26 13 27 23 52 40 13 35 13 s
MEAN 24 1 15 23 2 13 I
(1) SEE PROGRAM EXCEPTIIO43 SECTION FOR EXPLAHATIQ1 I
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TABLE C V.3 CDCDRU.TICHS OF GAP 91A D1ITTERS IN AIR PARTICULATE SAMPLES COLLECTED IN THE VICINITY OF PBAPS.1956 RESULTS IN LHITS OF E-3 PCI/CU, METER 2 2 SIGMA GROUP I SITE LOCATICHS STATICH COLLECTION CODE PERIOD BE-7 K-40 CS-134 CS-137 RA-226 TH-226 i
1A JAH OS 140 1 70 200 1 100 C5 C5 10 1 10 C 10 FEB 06 130 2 50 200 t 100 C5 C5 C 10 C 10 MAR OS 160 1 70
< 100 C5 C5 C6 C 10 APR GC 170 1 70 100 1 100 C4 C5 C 9 C 10 MAY 88 130 1 60 200 1 100 C5 C5 C8 C 10
.AH 68 210 2 70 C 100 C4 C4 C 9 it i 10 JUL 80 60 1 60 C 100 C5 C5 C9 C 10
' AUG 08 160 1 60 C 100 C4 C5 C6 C 10 SEP 66 190 1 70 C 100 C6 C 6 C 10 C 20 OCT SS 120 1 60
< 100 C6 C6 C 10 C 10 POV OS 110 1 60
< 100 C4 6
25 C 10 C 10 DEC 66 160 1 60 100 1 100 C5 C6 C 10 C 10 MEAN 146 1 74 125 2 90 C5 5
21 9
12 11 26 1B JAN SS 170 1 70 C 100 C5 C 6 C 10 C 10 FEB Se i70 e 70
< 100 C5 C5 C 20 C 20 MAR SS 160 2 60 120 2 90 C5 C4 C 7 C 10 APR 68 80 1 60 200 1 100 C5 C5 C 8 C 10 MAY 06 60 1 70
< 100 C5 C6 C 10
< 10 M4 80 290 t 60 100 2 100 C4 C4 C6 C 10 JUL 68 190 1 00 C 200 C6 C5 C 10 C to AUG BS 100 2 6C C 100 C4 C5 C 10 C 10 SEP BS 120 1 60 200 1 100 C5 C5 C9 C 10 OCT e6 60 1 50 C 100 C5 C6 C 9 C to NOV 88 90 2 60 C 100 C4 C 5 C 9 C 10 CEC Bo 100 2 90 C 200 C6 C7 C to C to MEAN 140 1 130 140 2 100 C 5 C5 C 9 C to 2
JAH OS 110 1 70 200 1 100 C5 C5 C 10 C 10 FEO SS 110 2 70 C 100 C5 C6 C 10 C 20 MAR BS 100 1 50 200 1 100 C4 C 4 C 7 C 9 APR SS 130 1 80
< 100 C6 C5 C 10
< 10 MAY 88 110 2 50 200 1 100 C5 C5 Co C to
- 4 86 200 1 60 300 1 100 C 4 C4 C6 C 10 JUL BS 90 2 60
< 100 C5 C5 C 10
< 10 AUG BS 160 2 60
< 100 C4 C5 C 9 C 10 SEP So 170 1 70 C 100 C 6 C6 C 10 C to OCT OS 120 1 60 C 100 C5 C6 C 10 C 10 POV SS 130 2 60 200 2 100 C4 C4 C6 C 10 DEC OS 160 1 70 200 1 100 C5 C5 C 10 C to P1EAN 133 1 66 156 1 134 C5 C5 C9 C 12 MEAN GROUP I 140 2 90 140 1 110 C5 5
11 9
22 11 27 I
I I
I E
i l
E TABLE C.V.3 CONCENTRATICHS OF gar 914 EMITTERS IN AIR PARTICULATE SAMPLES COLLECTED IN
]
THE VICINITY OF PSAPS,1985 RESULTS IN LHITS OF E-3 PCI/QJ. METER 1 2 SIGMA GROUP II - HEAR SITE LOCATI0t45 STATION COLLECTICH CODE PERIOD BE.7 K.40 C3 134 CS-137 RA-226 TH-228 I.
3A JAN SC 160 1 70
< 100 C 5 C 6
< 10
< 10 FEB 88 110 1 70 200 1 100
< 5
<5 10 i to
< to MAR 88 110 1 90
< 200 C7 C6 C 10
< 20 APR 88 100 1 70
< 200 C6 C6 C 10
< 20 MAY 88
< 70
< 200
<6
<7 C 10
< 10 AN 88 210 1 60 200 1 100
<4 C4 C6
< 10 JUL 68 90 1 80
< 200 C6 C5
< 10
< 20 AUG 85 176 2 60
< 100
<5 C5
< 10
< 10 I
SEP BS 130 1 70
< 100
<5 C5 C9 C 10 OCT SS C 70
< 200 C6 C 6 C 10
< 20 tW 88 120 2 70
< 100 C5 C5
< 10
< 10 DEC 80 80 2 80
< 100
<6 C6 C9 C 20 MEAN 118 1 66 158 1 103 C6 C 6 10 11
< 14 48 JAN 88 110 t 60
< 100
<4 C4 C9 C 10 FES SS 110 1 70 200 2 200
< 6
<6
< 10
< 10 PRR Bo 190 1 60
< 100
<5 C 5 C 6 C 10 I
APR 80 70 1 60
< 100
<5
< 5 C 9
< 10 MAY 88 70 2 50 100 1 100
< 5 C5
< 9
< 10 JUN 80 210 1 70
< 100
<4 C5 C6 C 10 JJL 85 190 1 80
< 100
< 5
<6 C 10
< 10 I
AUG SS 190 1 60
< 100
<5
<5
< 9 C to SEP BS 170 1 80
< 200
<6
<6 C 10
< 20 OCT 88 80 1 60 100 1 100
<5
<5 C 9 10 1 10 TOV 88 170 1 6?
< 100
<4
<5
< 9 C 10 CEC 80 300 1 100
< 200 C 7 C 7 C to C 20 MEAN 155 2 138 125 1 90 C5 C5 C9 12 26 5
JAN 88 120 1 70
< 100 C5 C5 C 10
< 20 FEB SS 140 1 80
< 200 C6
<5 C 10
< 10 I
MAR 88 110 1 60
< 100
<5
<5 10 i9
< 10 APR 88 180 1 80
< 200
<6 C 6
< 10
< 10 MAY 88 110 1 70
< 200
<6 C 6
< 10
< 20 JUN SS 170 1 70
< 100 C 4 9
25 C 9 C 10 I
JUL 88 130 1 80
< 100
< 6
<6
< 10
< 20 AUG 85 130 2 60
< 10 0
< 4 C4
<8
< 10 SEP 88 80 1 70
< 200
<6 C 6
< 10
< 10 OCT 88 90 1 70
< 100
< 5
<5 C 10
< 10 tW 88 110 1 60
< 100
< 4
<5
<8 C 10 I
l DEC 80 120 1 70 200 1 100
<5 C6 C 10
< 10 MEAN 124 i 58 142 2 103 C5 6
12 10 22 C 13
, I 6B JAN SS 140 1 60 100 1 100
<5 C5
< 9
< 10 FEB SS 170 2 70 200 1 100
<5
<5 C6 C to MAR 80 140 1 60 300 1 100
<5
<4 C6 C 10 l
APR 80 130 2 80
< 200 C6 C 7 C 10
< 10 MAY 86 120 1 60
< 100
<5 C5 C 9 C 10 i
JUN BS 230 1 70 300 2 100 C4 C4
<8 C 10 JUL 80 100 1 60 200 1 100
<5
<5 C 10
< 10 AUG BS 200 1 70 100 1 100 C4
<5 C 10
< 200 C6
<7 C 10
< 20 OCT BS 130 2 60 200 1 100
<5 C5 C to
< to I
POV BS 130 1 70
< 100
<5 C4 C 9 C to DEC 88 120 i 90
< 200
<6 C 6 C 10
< 20 MEAN 148 1 74 183 1 144 C5
<5
<9 C 12 I
I I
I TABLE C-v.3 CD4CENTRATIDHS OF GArt% EMITTERS IN AIR PARTICULATE SM1PLES COLLECTED IH i
THE VICINITY OF PBAPS,1966 RESULTS IN LNITS OF E-3 PCI/CU. METER 1 2 SIGNA GROUP II - HEAR SITE LO::ATIQ4S STATIDH COLLECTIDH m
CODE PERIOD BE-7 K-40 CS-134 CS-137 RA-tt6 TH-2tB 14 JAN 08 160 1 70 C 100 C5 C5 C 10 C 20 FEB SS 140 1 70 C 100 C5 C5 C 10 C 10 MAR 60 150 1 60 100 1 100 C4 C4 C 7 C 10 APR 66 160 t 60 200 1 200 C6 C6 C 10 C 20 MAY So 150 1 70
< 100 C5 C5 C 9 C 10 JUN 06 210 t 60
< 100 C5 C5 C 9 to 2 to JUL SC 120 1 70
< 100 C 5 C5 C 10 C to AUG 88 130 2 60 C 100 C4 C4 C7 C 10 SEP BS 150 1 70 200 t 200 C 6 C6 C 10 C 20 DCT 60 100 2 60 C 200 C5 C6 C 10 C 20 NDV 68 60 2 60 150 t 90 C4 C4 C 7 C 10 DEC 66 200 1 100
< 200 C6 C7 C 10 C 20 MEAN 146 1 74 138 1 97 C5 C5 C 9 14 1 10 15 JAH SS 150 1 60 C 100 C 5 C5 C6 C 10 FED $8 160 1 70 10b i 100 C5 C5 C 10 C 10 W
PAR Se 140 1 60 300 1 100 C4 C4 C 7 C 10 APR SS 120 1 70 300 1 100 C5 C5 C 9 C to MAY 06 60 1 70 C 100 C 6 C6 C 10 C 20 JUN 88 210 1 70 C 100 C5 C5 10 19 C 10 JUL 66 120 1 70 C 100 C 6 C 6 C 10 C 20 AUG 68 130 1 60 C 90 C 4 C4 C6 C 10 SEP BS 120 1 60 C 200 C 6 C6 C 10 C 20 CCT 58 130 1 60 200 1 100 C 5 C 5 C6 C to FEh/ BS 110 1 50 200 2 100 C4 C4 C7 C 10 DEC 60 110 2 70 200 1 100 C5 C6 C 9 C 10 MEAN 132 1 64 166 1 157 C5 C5 9
22 C 13 17 JM4 OS 110 1 60 200 1 100 C 5 C5 C 9 C 10 FEB B6 190 1 70
< 100 C6 C6 C 10 C 20 M4P 68 150 1 60 C 100 C5 C5 C 9 C 10 APP OS 120 1 70 200 1 200 C 6 C 6 C 10 C 20 MAY BS 160 1 60 C 200 C6 C 6 C 10 C 20 JUN 08 100 2 60 200 1 100 C4 C4 C 7 C 10 JUL 66 130 1 60 C 100 C6 C 6 C 10 C 20 AUG 08 160 1 60
< 100 C 5 C4 C 9 C 10 SEP B6 190 1 70 C 100 C5 C5 C 9 C 10 DCT So C 50 200 2 100 C4 C5 C 9 C 10 HOV SS 120 1 50 200 1 100 C4 C4 C7 C 10 DEC 00 70 1 70 200 2 100 C 5 C5 C 9 C to MEAN 136 1 90 156 1 103 C 5 C5 C 9 C 13 31 JAN SS 120 2 70
< 100 C5 C6 C 10 C 20 W
FEB $6 160 2 70 C 100 C5 C6 C to C to MAR BS 190 1 70 C 100 C4 C5 C6 C 10 APR 68 160 2 70 C 100 C5 C5 C 9 C 10 MAY 68 240 1 60 C 100 C6 C5 C 10 C to JUN SS 150 2 60 C 90 C4 C4 C6 C 10 JUL 58 150 1 70 C 100 C 6 C 6 C 10 C 20 AUG So 200 1 70 C 100 C4 C5 C 9 C 10 SEP DS 140 2 70 200 1 200 C5 C6 C 10 C 20 DCT 68 70 2 60
< 100 C5 C6 C 10 C 10 tCN 06 90 1 50 100 1 90 C3 C4 C7 C 10 DEC 68 120 1 60 200 2 100 C5 C5 C6 C 10 MEAN 151 1 96 116 1 79 C5 C5 C 9 C 14 Il II E
TABLE C.V.3 COCENTRATIQ43 OF GArt1A EMITTERS IN AIR PARTICULATE SAMPLES COLLECTED IN THE VICINITY OF PDAPS,1908 RESULTS IN 04ITS OF E.3 PCI/CU. METER 1 2 SIGNA GROUP II. HEAR SITE LOCATIO4S STATION COLLECTIO4 CODE PERIOD BE.7 K.40 CS.134 CS.137 RA.226 TH.220 32 JAN BS 110 1 60
< 100
<4 C5
<9 C to FEB SS 110 1 60
< 100
< 6 C6 C 10
< 20 MAR OS 190 1 60
< 100
<4
<5 C6 C 10 APR OS 160 1 70
< 100 C6 C6 C 10
< 20 MAY BS 200 1 70
< 100 C5 C5 C 9
< 10 Jlk4 OS 220 1 70 100 1 100
<4
<4
<7 10 2 10 JUL OS 150 2 70
< 100
<5 C5
<9 C to AUG OS 150 1 60
< 100
<5 C5
<9 C 10 SEP BS 120 1 60
< 100 C5 C5 C 10
< 20 OCT So 110 1 60 200 1 100
<5 C5 C 9
< 10 ICV 66 100 1 60
< 100
<5
<4
< 9 C 10 DEC BS 170 2 90
< 200
<6 C6
< 10
< 20 MEM4 151 1 et 117 1 70
<5
<5
< 9 13 2 10 33A JM4 08 160 1 60
< 100
<5 C5 C to
< to FED OS 160 1 70
< 200 C 5 C6
< 10
< 20 MAR 68 130 1 70
< 100
<5
<5 C 9
< 10 APR OS 150 1 70
< 100 C 6 C6 C 10
< 20 2
MAY 08 110 1 90
< 200
< 7
<7 C 10
< 20 JLki SS 190 1 60
< 100 C 5
<5 C 9
< 10 JUL BS 190 2 60 100 1 100
< 5
<5
< 9
< 10 AUG OS 100 1 60
< 100
<5 C5 C 9
< 10 SEP 68 100 1 70
< 100 r5
<5
< 10
< 10 OCT BS
< 70
< 200
<6
<5
< 10
< 20 tCV 65 100 1 60 200 1 100
<4 4
14 C 6 C0 DEC OS 160 1 90 300 1 100 C6 C6 C 10
< 10 MEAN 142 1 79 150 1 135 C5 5
12
< 10
< 13 38 JAN 08 100 2 60
< 100 C 5 C5 C6 20 1 20 FEB BS 200 t 70 100 1 100
< 5 C5 C 9
< 10 MAR BS 150 1 60 100 1 100
< 4 C4 C7 C 10 APR OS 200 1 70 100 1 100
< 5 C5
<9
< 10 MAY 08 200 1 70 300 1 100
< 5 C5
<8
< 10 JUN OS 220 1 70
< 100 C 5
<5 C6 C 10 JUL 68 130 1 60
< 100
< 5
<4
<9 C 10 AUG 08 210 1 60
< C0
<4
<4
<7 C 10 SEP 08 130 1 70 200 2 100
<5 C5
<9
< 10 OCT BS
< 60 200 1 100
<5 C5 C7
< 10 tCV SS 50 1 40 100 1 100 C4
<4
<6
< 10 DEC BS 190 1 90
< 200
<6
<7
< 10
< 20 MEAN 160 2 115 140 1 136
<5
<5 CS 12 16 l
MEAN GROUP II 142 1 90 145 1 117 C5 5
12 9
12 13 19 l
l m'
d'
I TABLE C-V.3 COCDRRATIO45 OF GAP 9% EMITTERS D4 AIR PARTICULATE SAMPLES COLLECTED Di THE YICD4ITY OF PBAPS.1960 l
RESULTS IN LHITS OF E-3 PCI/CU. METER 1 2 SIGMA GROUP III - COUROL LOCATIG43 STATIQ4 COLLECTIO4 CODE PERIOD BE-7 K-40 CS-134 CS-137 RA-Et6 TH-226 12A JAN 88 180 1 60 -
C 100 C5 C5 C9 C to FEB OS 160 1 70 200 1 100 C5 C5-C 10 C 10 MAR 86 110 1 60 100 1 100 C4 C4 C6 C 10 APR OS 150 2 60 C 100 C5 C5 C9 C 10 MY OS 190 1 70 200 1 100 C5 C5 C9 C 10 i
JUN SS 160 1 60 100 1 100 C4 C4 C7 C to JUL 66 160 1 60
< 200 C6 C6 C 10 C 20 AUG OS 100 1 100 C 100 C6 C6 C 10 C 20 SEP 06 90 1 50 120 2 90 C4 C4 C6 C9 OCT 80 C 70 C 200 C6 C6 C 10 C 20 tm 85 100 1 60 100 1 100 C5 C5 C6 C 10 DEC 80 120 2 70 C 100 C4 C4 C9 C 10 MEAN 133 1 61 135 1 97 C5 C 5 C 9 C 12 12D JAN OS 170 1 70 C 100 C6 C5 C 10
< 10 FEB 88 170 1 70 C 200 C6 C 6 C 10 C 10 MR 68 200 1 80 200 2 100 C5 C4 Ce C 10 APR 65
~180 1 60 100 1 100 C5 C5 C 9 C 10 MAY BS 210 2 60 C 100 C5 C 6 C 10
< 10 JLH OS 150 1 70 C 100 C4 C4 10 19 C 10 JUL 86 250 2 60 100 1 100 C5 C6 C 10
< 10 AUG SS 170 1 90 C 100 C5 C5 C 9 C 10 SEP OS 100 1 50 100 1 100 C4 C 4 C 7 C 10 OCT 66 100 1 60 200 1 100 C 5 C5 C 9 C 10 im OS 130 1 00 C 200 C6 C6 10 1 10
< 20 DEC 00 140 1 70
< 100 C 5 C4 C0 C 10 MEAN 164 i SS 133 1 90 C 5 C5 9
22 C 11 m
MEAN GrJUP III 148 1 69 134 1 95 C5 C 5 9
22 C 12 I.
1I I
I I
I' I!
I I
t 1
I M
0 1
6 A
2 1-
_ M 1
9 0
5
_ M 0
1 3
0 5
0 M
4 9
A 3
- i
- i 3
0 4
4 1
M 0
9 1
1 3
0 9
M 0
0 7
9 5
3 7
- i
- - i 1
- i 1
7 9
0 0
5 3
M 2
6 E
5 1
i T
1 A8 R
2 6
M L 0 U9 G
C1 I
I S
T 0
RS 2
D i
1 M
I O T
RP 0
I R
4 AF E
E DY H 0
T 3
M 1DI I
J B
- i - -
0D Q 6
0C
/
0 FI I
3 V
C S
P RE 0
EH 3
0 TT 2
M T
E I4 0
1 MD F
4 E
O 0
D 0
ME S
2 T
T tt C I
4 AE M
A GL
(
6 L
LO 1
2 i
RC D
4 6
OS S
IE T
TL L
M IP U
DM S
4 DA E
G AS R
I D 6
0 8
6 80 S
S 0
08S 6
S 8
TO 0
6 8
0 00 O
O 0
68O 8
O 6
CI 4
4 4
ER T
G G
4 T B
BR4 B
G 4
LE W
C U
U MC E
A M
EP E
U L
A A
4 LP J
O A
A JO F
J J
FAJ F
A J
L L
M O
V C
C E
N t
t D
3 0
9 1
6 0
0 1
E I
7 8
5 5
0 1
2 3
3 4
4 4
L L
5 5
9 9
1 1
1 1
1 1
1 B
C 1
A J
O 0 R
o U G
E I
S A
A E
M 8
T C
0 Z
t R
A T
C
'D L
C 1
M M
i
Illl i
E TABLE C.VI.1 ANALYTICAL DATA POR AIR 200D4E SAMPLES SAMPLES COLLECTED IN THE VICD4ITY OF PBAPS,1900 RLSULTS IH LHIT1 0F PCI/CU. METER 1 2 SIONA GROUP I GROUP II GROUP III HEgx 1
0 16 1Z t
3A 5
60 14 120 1
C 01 C.01 C 01 C.01 C 000 C.01 C 009 C 02 2
C.01 C 01 C 01 C 01 C 01 C.St C 01 C 02 l
3 C.01 C.01 C 01 C 01 C 009 C 03 C 03 C 02 4
C 01 C 01 C 02 C 01 C 006 C 01 C 006 C 02 5
C.03 C 07 C 03 C.03 C 02 C 02 C 02 C 01 6
C 01 C 61 C 01 C.01 C 007 C 01 C.009 C 01 7
C.01 C 01 C.01 C.01 C 01 C.02 C.02 C 01 0
C.01 C.01 C 01 C 01 C 006 C 01 C 01
(
01 9
C 02 C 02 C 02 C 05 C 02 C.02 C.02 C 01 10 C 03 C 03 C 03 (1)
C.St C 03 C.03 C 0 00 11 C 02 C.02 C 02 C 02 C 01 C 01 C.01
(.02 12 C 01 C.01 C 01 C 02 C 009 C.01 C.01 C 02 13 C 01 C 01 C.01 C.01 C 009 C.01
<.009 C.01 14 C.006 C 01 C.01 C.01 C 02 C 02 C 009 C 02 15 C 02 C 02 C.02 C 02 C 01 C 01 C.01 C 006 16 C 01 C 01 C 01 C 01
< 01 C 01
<.01 C 02 17 C 01 C.01 C 01 C 01 C.009 C 01 C 01 C.005 l
1C C 02 C 02 C 02 C.02 C.01
< 02 C 02 C 006 19 C 02 C.02 C 02 C 02 C 01 C 01 C
01
(.02 20 C.02 C
02 C 02 C.02 C 01 C.02 C.01 C.01 21 C.01 C 01 C 01
(
01 C 006 C 01 C.006 C 01 I
22 C 01 C.01 C 01 C 01 C 01 C.02 C 02 C 01 23 C 02 C.02 C.02 C.02 C 01 C.01 C 01 C 01 24 C 01 C.01 C.01 C.01 C 006 C.0 06 C 000 C 02 25 C 01 C.01 C.02 C.02 C 007 C.01 C 02 C 01 26 (1)
(1)
(1)
(1)
(1)
(1)
(1)
C 02 27 C 009 C 007 C 009 C.009 C 01 C 02 C 02 C.02 to C 02 C.02 C 02 C 02 C 01 C 02 C 02 C.02 29 C.02 C 02 C.02 C.02 C 01
< 01 C 007 C 02 30 C.01 C 01 C 01 C.01 C 01 C.03 C 02 C
000 31 C.01 C
01 C.01 C
01 C 009 C 02 C 01 C 009 32 C.02 C.02 C
02 C 02 C 01 C.01 C 007 C 01 33 C.01 C.01 C 01 C 01 C 01 C
01 C 009 C.0 06 34 C.01 C 01 C 01 C 01 C 009 C 009 C.01 C 01 35 C 01
< 01 C.01 C 02 C 009 C 01 C 01 C 01 36 C 02 C.02 C.02 C 02 C.01 C 02 C 01 C 01 37 C.02 C
02 C 02 C.02 C.01 C.01 C 009 C.01 36 C.02 C 02 C.02 C.02 C 01 C 01 C 006 C 000 39 C 01 C 02 C.01 C.01 C 01 C 01
< 02 C 02 40 C 02 (1)
C 02 C.02 C 01 C 01 C 009 C 02 41 C 02 C.02 C.02 C.02 C.01 C.02 C.02 C.02 42 C.01 C.01 C 01 C 01 C 009 C 02 C 01 C.C2 43 C 01 C 01
(
01 C.01
(
007 C 01 C 01 C 01 44 C 01 C.01 C 01 C.02 C.009 C.01 C 01 C.01 45 C 01 C 01 C.01 C 01
< 009 C 02 C.02 C 01 46 e C 009 C 009 C.0 06 C 01 C 005 C 01 C 01 C 01 47 C 01 C 01 C 01 C 01 C 009 C 02 C 01 C 02 46 C 01 C 01 C 01 C 01 C 007 C.01 C 006 C 005 49 C 02 C 02 C 02 C.02 C 01 C.02 C 01 C 000 50 C 02 C 02 C 02 C 02 C.000 C.01 C 01 C 02 51 C 02 C 02 C 02 C.02 C 01 C 0D6 C 007 C 01 52 C.01 C.01 C.009 C.01 C 005 C 01 C.007 C.01 MEAN C.014 C 014 C 015 C.015 C 010 C 014 C 012 C.013 (1) SEE PROGRAM EXCEPTIONS SECTIDH FOR EXPLANATICH ll ll 11
. I-TABLE C.VII.1 AtuLYTICAL DATA FOR MILX SAMPLES COLLECTED IN THE VICINITY OF PD4PS,1906 RESULTS IH UNITS OF PCI/ LITER 2 2 SIGPM COLLECTION STATION DATE SR-69 SR.90 CS-134 CS.137 I
G CU15/06 C2 3.8 i.4 C3 4
13 05/30/06 C2 3.3
.t. 6
<4 5
23 09/05/06
<2 2.5 1.6 C 3
<3 11/14/68 C2 4.5 2.5 C3 3
13 MEAN
<2 3.5 1 1.7
<3 4
22 J
CU15/05
<1 2.2 2.3 C 3 C 2 05/30/08
< 1 2.6 1.3 C6
<5 I
09/05/06
< 1 1.6 1.7
<2
<2 11/14/06
< 1 2.6 1.4 C4
<3 NEAN
< 1 2.3 i.6 C4
<3 I
O CU15/08
< 1 1.9 1.3
<9 C8 i
05/30/88 C.6 1.7 1.3
<7 C6 l
09/05/06
< 1 1.7 1.5 C4
<3 11/14/80
< 1 5.4 2.3 C4
<I i
MEAN
<.9 2.7 2 3.6 C 6 C5 MEAN NEARBY FARMS
< 1.3 2.6 1 2.4
<4 4
24 L
CU15/08
< 1 3.5 1.4
< 3 3
12 05/30/08
<.7 2.3 1.3 C4
<4 I
09/05/08
< 2 3.5 i.6 C 3 C 3 11/14/88
< 3 3.3 1.7 C3 C3 MEAN
< 1.7 3.2 2 1.1
<3 3
11 I
M CU15/86
< 1 3.6 1.3 C 3
<2 05/30/06
< 2 5.4 i,6
<4 C3 09/05/08
< 1 2.0 2.4
<3 5
23 11/14/88 C 1 2.6 1.4 C4 5
13 MEAN
< 1 3.4 1 3.0
<4 4
13 H
CU15/00
< 1 2.0 t.3 3
13 C2 05/30/08
<3 2.5 1.6 C4 C 3 I
09/05/88 (1)
(1)
<3 3-12 11/14/86
<2 2.6 i.3 C 3
<2 NEAN
<2 2.4 1.6 3
11 3
11 MEAN INTERMEDIATE FARMS
< 1. 6 3.0 1 2.0 3
11 3
12 (1) SEE PROGRAM EXCEPTIONS SECTICH FOR EXPLANATION
. I I
I I
1
F
~
TABLE C-VII.1 ANALYTICAL DATA FOR MILK SAMPLES COLLECTED D4 THE VICD4rTY OF P8APS,1988 RESULTS D1 UNITS OF PCI/ LITER 1 2 SIGNA
.{
COLLECTION STATICH DATE SR.89 SR.90 C3 134 C3 137 A
CU15/88 C2 1.5 1.3
<3 C3 g L 05/30/88 C 3 3.4 i.6
<5 C4 j
09/05/88
< 1 1.3 i.4 C3 C3 11/14/88 C 9 1.2 i.4
<3 3
12 I
MEAN
< 1.7 1.9 1 2.1
<4 3
11 B
DU15/88
<.6 1.2 i.2
<7 C5 05/30/88
< 1 1.2 i.5 C3 C 3 09/05/88
< 1 1.2 i.7 C5 C4 11/14/88 C 2 1.6 i.4
<4 C3 MEAN
< 1.2 1.3 i.4 C5 C4 C
CU15/88 1 11 1.4 i.3 a3 3
05/30/08
< 1 2.7 i.4
< 2
< 2 09/05/88
< 2 1.2 i.7 C 3
< 3 11/14/88
< 1 8.1 i.5 C 3
< 3 MEAN 1 11 3.3 1 6.5 C 3
< 3
=
E Ou15/88
< 1 1.3 i.4
<4
< 3 l
05/30/88
<.7 1.3 1.4
<4
<3 09/05/88
<2 1.8 i.6
<3 C 3 g
11/14/88 C 1 2.3 i.5
<3 3
13 MEAN
< 1.2 1.7 1 1.0
<4 3
10 MEAN DISTAtC FARMS 1.3 1 1.3 2.0 1 3.5
<4 3
11 I
OVERALL MEANS HEAR 8Y FARMS DU15/88
< 1 2.6 1 2.0
<5 5
16 05/30/88
< 1.2 2.5 1 1.6 C6 5
i1 09/05/88
< 1 2.0 2.9
< 3
<3 11/14/08 C 1 4.2 1 2.9
<4 3
10 INTERMEDIATE FARMS l
CU15/88 C 1 3.0 1 1.8 3
iO 2
11 05/30/88 C 1.9 3.4 1 3.5 e4 C3 09/05/88 C2 2.8 1 2.1
<3 4
12 11/14/88
< 2 2.8 i.8 C 3 3
13 DISTANT FARMS CU15/88 1.2 1 1.2 1.4 1.3 C 4
<3 05/30/88 C 1.4 2.1 1 2.1
<4
<3 09/05/88 C 2 1.4 i.6 C4 C 3 11/14/88
< 1.2 3.3 1 6.5
<3 3
10 MEAN ALL FARMS 1.4 1 1.4 2.6 1 2.9 4
13 3
12 I.
I I.
TABLE C.VII.2 AVERAGE CONCENTRATE 0H? 0F I-131 IN MILK SAMPLES COLLfGED IN THE VICINITY OF PBAPS 1986 RESULTS IN LHITS OF PCI/ LITER i 2 SIGMA COLLECTION NEARBY FARM INTERMEDIATE FARMS DISTANT FARMS DATE (G,J.0)
( D. L.M.N)
(A,5,C.E)
ALL FARMS 01/18/88 C.05 C.06 C 06 C 05 I
02/15/06 C.06 C 06 C 06 C 06 05/21/06 C.05 C 04 C.05 C 05 04/04/66 C.06 C 05 C.06 C 06 04/18/06 C.05 C 04 C 05 C.05 05/02/0C C.04 C.05 C 05 C 04 I
05/16/80 C 05 C.04 C 05 C 05 05/30/80 C.05 C 06 C.06 C.06 06/13/06 C.04 C 04 C.04 C 04 C 6/27/80 C.04 C 03 C.04 C.04 I
07/11/06 C.05 C.04 C 05 C 05 07/25/88 C.06 C 06 C.06 C 06 06/08/06 C 05 C 05 C 06 C 05 06/22/88 C.04 C.04 C.04 C 04 09/05/88 C.05 C 00 C 08 C 06 I
09/19/S6 C 04 C 04 C 05 C 04 10/03/00 C.04 C.03 C.04 C 04 10/17/88 C.05 C.04 C 06 C 05 10/31/86 C 06 C 05 C 0S C 07 11/14/88 C.05 C 04 C.06 C 05 I
12/12/60 C.04 C.03 C 05 C 04 I
I I
I I
I I
I I
m
1 l
l T ABLE C.VII.3 CONCENTRATIONS OF I.131 IN MILK SAMPLES COLLECTED IN THE YZCINITY OF PDAPS,1906 RESULTS IN LNITS OF PC1/LITEL t
- 31Gr14 W LLECTION l
DATE A
B C
E G
J L
M N
O
'91/16/06 C.05 C 06 C.05 C.M C 06 C 06 12/15/06 C.05 C 06 C.04 C.07 C.06 C.05 C.07 C 07 C.05 C.06 0Ft1/SS C 05 C 05 C.05
<.05 C.M C.05 l
D4/04/06 C.M C.05 C 07 C.t5 C 05 C 05 M/18/06 C 05 C.M C.05 C.05 C.M C 05 05/02/88 C 07 C.03 C.M C.M C 03 C 03 05/16/06 C 05 C.04 C.05 C.05 C.M C.M 95/30/06 C 06 C.06 C 05 C.05 C.05 C.05 C.M C 06 C 05 C 06 06/$ #D0 C 04 C.03 C.M C.05 C.M C.M 06/27/06 C.M C 03 C.M C.M C 03 '
C.04 07/11/88 C 05 C.05 C.05 C.05 C.M C 05 07/25/E8 C 06 C 05 C.M C.M C 66 C.05 06/08/80 C.06 C 05 C.45 C.05 C.05 C 06 06/22/06 C 04 C 04 C.04 C.M C 04 C 04 09/05/06 C.06 C 07 C.00 C.07 C.1 C 00 C.07 C 06 C.06 C.07 09/19/05 C 06 C.04 C.03 C.03 C.M C.05 10/03/06 C 05 C.03 C.M C.M C.03 C 03 10/17/06 C 06 C 04 C 05 C.06 C 04 C 04 1
10/31/86 C 1 C 06 C.07 C.07 C 05 C.05 i
11/14/68 C 00 C 05 C 05 C.06 C.05 C 05 C 05 C 03 C.05 C.06 12/12/06 C 06 C.04 C.M C.05 C 03 C 04 MEAN
< 06 C.05 C
06 C.M C 05 C.05 C.06 C.M C.04 C 05 I
I I
I I
I I
I I
~
I I
I I
TABLE CLEAN C.VIII.1 At4ALYTICAL DATA FOR WELL HATER SAMPLES COLLECTED IN THE VICINITY OF PSAPS,1906 RESULTS IN uiITS OF PCI/ LITER 2 2 SIGMA STATIQ4 DATE N GROS $ ALPHA GROSS BETA UlWilut(A)
A9JEOUS H3 I
1U CU27/06
.6 1.3 C.9 C.5 60 1 50 04/30/60
.7 1.4 2.0 1.6 05 60 1 46 06/26/OS C 7 1.1 1.7
.25 C 50 10/01/06 5 2.4 1.5 1.6
.35 90 2 50 MEAN
.6 1.2 1.4 1 1.0
.30 t.35 65 1 35 1V CU27/06
.6 1.6 C.7 C.6 C 50 04/30/80 5 2.3 2.1 1,7
.13 170 2 50 I
06/26/88 C 6 2.0 2.7 C.05 C 50 10/01/06 C.2 1.1 2.7
.20 80 1 40 MEAN 5 1.5 1.5 1 1.4 25 g.49 66 1 114 I
7 C U27/06 C.3 4
11 C 5 C 50 04/30/88 5 1.3 2.5 1.6 08 C 50 06/26/06 C 1 3.0 t.0 C 05 C 50 09/30/08 C.3 2.3 1.6
.15 50 1 50 MEAN 5 t.7 3.0 1 1.5
.20 t.42 50 10 40 C U27/86 C.3 1.9 2.9 C 3 C 40 l
04/30/S5 1.7 1.7 2.1 1.6 54 50 1 40 06/26/00 C 5 2.0 1.6 C 05 C 40 09/30/80 C 4 2.1 2.6 C 05 60 2 40 i
MEAN
.7 1 1.3 2.0 2.2
.24 1.47 46 1 19 MEAN ALL STATIO4S
.6 1.7 2.0 1 1.6
.21 1.36 63
- 63 1 I IOTE8 (A) URANIui C04CDRRATIO4 IN UMLITER I
I I
1 I I
)
i I
1 I
o
lIill l!l l
1l{lil Il i!
3 3
1 1
i i
5 3
33 3
33 3
33 3
9-C e
t 5
4 3
5 55 r
55 5
55 5 55 S
5 9- << < << < <<
C RZ 5
66 6
66 4
66 6
66 6
6 6
4D U
0 33 3
33 3
33 3
33 3
3 6
t<
<C O
C SEL 9
77 7
77 7
77 7
77 7
7 P
5 N
( <
C c
U A
E S
F R
ETAH A
L0 N
L0 G
E9 I
8 33 3
33 3
33 3
33 3
3 N1 S
5 4
2 D
DS C
P U
SA i
R3 1 EF T
R TF E
1O T
1 I
DY L
T U 9
22 2
32 3
22 2
33 3
2 U
AI 5
1 t C
C rD P
t 4
t AC t
GI F
V O FOE S
H T
3T I
0 6
0 4
5 4
4 5
2 6
1 1
G4 FL ID i0 1
00 0
01 i
00 0
i 4
T 0
5 55 5
5 55 5
AD D
4 RE
< < c <
TT S
K I
C T
0 0
0 5
4 DE L
7 6
6 5
5 CL U
l L S
aO E
1 CC R
Q 4
t 4
4 3
ID 76 M
76 s
76 N
76 M
t TO 22 E
22 E
22 E
22 E
G 2
CI U/ H U6 N U6 H U6 N I
/
/
/
ER 6
T I
LE C0 O0 O0 O0 A
I LP T
I O
S V
C L
C 4
L Q
A U
E IE L
TD 4
D AU M
A TC U
V 0
E T
S 1
I 7
4 N
U.
O llIl lll
~l(i[t
l TABLE C-VIII.E CorDfrRATICHS OF Gk91A EMITTERS IN HELL HATER SAMPLES COLLECTED IN THE VIC2HITT OF PBAPS, 1968 RESULTS IN L24ITS OF PCI/ LITER 2 2 SIEMA I
l STATIO4 COLLECTICH (1)
CODE PERIOD CS-134 CS-137 BA-140 LA-140 RA-226 TH-226 1U 02/27 C2 C3 C 20 C6 56 17 9
27 I
06/26 C 2 C3 C to C6 41 26 C7 MEAN
<2 C3 C 20 C6 49 2 21 8
13 1V 02/27 C 3 C 3 C to C7 57 27 C7 06/26 3
23 C3 C to C6 50 27 C7 NEAN 3 10 C 3 C to C7 54 2 to C7 I
7 02/27 C 2 C 2 C to C6 15 26 C 7 06/26 C2 C 3 C to C6 35 26 C 7 MEAN
< 2 C 3 C to C6 25 1 to C 7 I
40 Cu27 -
C 3 C 3 C 20 C 6 75 27 9
27 06/26 C 3 C 3 C 20 C5 69 18 C6 MEAN
<3 C3 e to C6 of 2 to 9
21 I
MEAN ALL STATIONS 3 11 C 3 C 20 C6 52 2 46 8
22 I
(1) RA-226 ACTIVITY HAS DETECTED FROM PD-214 #43 BI-213, THE DAUGHTER PRODUCTS OF RN-222.
6412CH WERE ASStkiED TO BE IN ESJILIBRIlti.
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5 TABLE C.IX.1 CONCENTRATIONS OF SR.69 AND.90 IN VEGETATICH SAMPLES COLLECTED IN THE VICINITY OF PBAPS,1986 PCI/SRAM (ASH)
PCI/ GRAM (HET) 2 2 Sit ~ A
& 2 SIem COLLECTICH STATION DATE MEDIA SR-69 SR.90 SR.09 SR.90 1
07/1 U56 BROCCOLI C.1
.75
&.04 C 004
.032 2.002 CDRH C.6 2.4 1.5 C 006 023 1.0M OUSU86 BROC(X)LI C2 5.4 2.5 C 03 002 2.006 CORN C.3 2.6 2.1 C 007 076 2.0M 09/17/06 COIN C3 3.0 t.4 C 04 046 1.007 STRING BEAMS C4 C.3 C 05 C.004 MEAN
< 1.7 2.44 2 3.65 C.023 044.t'.062 3A 07/1 ues MILD VEG
<2 29.6 1.6 C.02~
.331 2.007 06/06/06 NILD VEG C 20 76.3 2.6 C 2 560 t.006 09/17/06 NILD VEG 2
22 21.6 2.7 02 1.02
.221 t.007 MEAH 6
2 21 42.5 2 59.1 06 i.21
.377 1.366 4H 07/16/06 WILD VEG P
12 5.5 1.2
.M i.03
.092 1.004 05/06/80 WILD VEG C4 10.9 1.2 C 06
.174 2.004 09/17/06 WILD VEG C2 3.6 1.3 C.03 049 1.0M MEAN 3
22 6.7 1 7.6 04 1.03
.105 2.127 5
07/16/06 REET TOPS C 3 5.0 t.1 C.009
.135 1.004 STRING BEAN PLT
.2 2.2 2.22 2.05 009 2.006.106 2.003 05/06/06 BEETS C.3 1.27 1.06 C.009 041 1.002 CARROT TOPS C.2 2.47 1.07 C.006 099 i.003 09/17/86 BEETS C.2
.60 2.06 C.004 016 1.002 CARROTS C 1 2.3 2.2 C 05 006 2.000 MEAN 4
2.4 2.31 2 3.00
.015 i.035.061 2.006 6D 07/16/86 PEA PLANTS (1)
STRING BEAN PLT C.3 2.7 1.1 C.009 076 2.004 06/0 UO6 BEAN VINES C.3 7.7 1.2 C.01
.217 1.005 CDRH
<.2
.6 2.1 C 006
.016 1.003 09/17/66 LDM BEANS C 1 6.0 t.1 C.03 171 2.003 STRING BEANS C.3 5.4 1.1 C.006 145 1.003 MEAN
< 4 4.9 2 6.4 C 013
.126.2.157 6
07/1 US6 L*ROCCOLI C.9 6.7 1.1 C.02 160 t.003 STRIH3 BEAN PLT 2 21 12.5 1.2
.M i.02
.216 1.003 OUO6/06 BEANS C 2 5.5 1.2 C.1
.259 1.007 BROCCOLI C 5 9.6 2.2 C.02 440 t.007 09/17/06 GREEN PEPPERS C to 12 13 C.06 06 1.02-TURNIPS C.2 2.52 2.05 C. 01
.173 1.004 I
MEAN 2.6 1 7.4 6.5 1 7.7
.05 2.07
.221 1.246 23 07/16/06 APPLES C.6 6.0 t.2 C 007
.067 1.002 PEACHES C2 5.7 1.4 C 02 064 1.004 De/06/06 APPLES C1 2.2 1.5 C 0M 007 2.002 PEACHES C.3 6.7 1.2 C 0M
.107 2.0M 99/17/06 APPLES (1)
PEACHES C3 27.1 1.3 C.07 753 2.007 MEAN C 1.4 9.5 1 19.9 C.021
.200 t.623 MEAN ALL STATICHS 2.0 1 7.4 6.6 2 27.7
.03 2.06 152 2.327 (1) SEE PROGRAM EXCEPTIONS SECTION FOR EXPLMTICH L-_-_-________--_-_-__
TABLE C.IX.2 CO4CENTRATIQ4S OF GAtt1A EMITTERS IN VEGETATION SAMPLES COLLECTED Di THE VICINITY OF PBAPS,1966 RESULTS IN LA4ITS OF PCI/ GRAM (NET) 1 2 SIGMA STATIO4 COLLECTIQ4 CODE PERIOD MEDIA CS.137 BA.140 RA.226 TH.228 1
07/16 BROCCOLI C.01
<.06 C 02 C 03 CORN
<.01 C 06 C.02 C 03 06/06 BROCCOLI
- .01
< 07 C 02 05 1.03 CORH
<.009 C 07 C 02
<.02 09/17 CORN
< 01
(
06 C 03 C 04 STRD4G BE.M4S C 02 C 09 C.03
<.04 MEM4
< 012
< 07 C 02
.04 1.02 3A 07/16 HILD VEG C 009 C 04 C 02 C 02 06/06 HILO VEG. GRAPE
< 01 C.07 C 02 C 03 09/17 F' s VEG 011 i.000 C 06 C 02 C 02 NEAN 010 1.002
< 06 C 02
< 02
- H 07/16 HILD VEG
<.01 C.05 03 i.03 C 04 05/06 WILD VEG C 01
< 06 C
0" C 03 09/17 NILD VEG C 01
<.1 C.03
< 04 MEM4
< 01
< 07
.03 2.01
< 04 5
07/16 BEET TOPS
< 02 C 1
< 03 05 i.04 STRD4G BEAN PLT C 01
< 07 C 03
.06 1.04 DVQ6 BEETS
< 006
< 06 02 t.01
< 02 CARROT TOPS
< 009 C 07 02 i.02 C 02 09/17 BEETS C 01
<.06 03 i.02
<.03 CARROTS 01 i.01
< 05 02 2.02 C 03 ML44
.011 i.009
<.07 03 1.01 04 i.05 6D 07/16 PEA PLANTS C 02 C 09 C 03 C 05 STRING BE44 PLT C 01
< 06 C 02 05 1.03 08/06 DEAN VINES C.009
< 03 C 02 04 i.02 CORH C 007 C 03 C 01
<.02 09/17 LIMA BEANS C 009 C 07 02 1.02 03 i.02 STRING BEANS 02 i.01 C.07 C 02 04 1.04 MEAN 013 1.012
< 06 02 1.01 04 2.02 6
67/16 BROCCOLI C 00S
< 05 C 02 C.02 STRD4G BEM4 PLT C 009 C 05 C 02
< 02 06/06 BE44S C 006 C 06 04 i.02 03 2.02 BPOCCOLI 019 i.006.04 1.04 06 1.01 00 t.02 09/17 GREEN PEPPERS C 01
< 05 C.02 C 03 1URNIPS C 01 C.06
.03 2.02 06 2.03 MEAN 011 1.006 05 1.02 03 1.03 04 i.05 23 07/16 APPLES C 01
< 06
.03 i.02
<.03 PEACHS C.01
< 07
< 03
<.04 06/06 APPLES C 009
< 04 C 0t
< 02 PEACHES C 01
< 07 C.02 C.03 09/17 APPLES C.01 C 06
< 02
<.03 l
PEACHS C.02 C 1
<.03 C 05 MEAN
< 012
< 07 03 2.01
< 03 NEM4 ALL STATIO4S 011 2.006
.06 i.04
.02 2.02 04 1.03
TABLE C.X.1 AtMLYTICAL DATA FOR SOIL SAMPLES COLLECTED IN THE VICINITY OF PBAPS,1900 RESULTS D4 Lk4ITS OF PCI/ GRAM (DRY) 1 2 SIGMA STATIQ4 COLLECTION CODE PERIOD GROSS BETA SR.69 SR.90 SE.7 K.40 1AA 06/04 2.7 1.4
< 02
.077 1.004
.3
. 1.3 19 11 11/12 2.1 2.5 C.01 027 2.005
< 5 25 12 MEAN 2.4 i.6 C 02
.052 i.071
.4 1.3 22 t' 6 2
06/04 1.7 2.3 C 04 07 i.02
.3 i.3 to i1 I
11/12 5.4 1.5 C.1
.21 i.02 C.7 30 12 W
MEAN 3.6 1 5.2 C 07
.14 1 20
.5 1.6 24 2 17 3A 06/04 1.9 1.3.
<.02 062 1.009
<.3 22 11 11/12 3.1 2.5
< 03
.260 2.009 C 4 19 21 MEAN 2.5 1 1.7
< 03
.171 i.252 4 4 21 14 4N 06/04 1.5 1.2 03 i.03 05 i.01
<.2 9.7 1.5 11/12 2.1 1.3 (1)
(1)
<.4 12 11 MEAN 1.6 i.6
.03 i.00
.05 i.00
<.3 10.9 i 3.3 5
06/04 2.7 1.3
<.02 05 i.01
<.3 30 11 11/12 2.3 2.3
< 1 00 t.06
<.2 19.3 2.6 MW4 2.5 2.6
<.06 07 i.04
<.3 24.7 1 15.1 6G 06/04 3.2 1.4
<.03
.214 1.009
.3 i.3 19 21 11/12 3.1 2.4 C.05 25 2.01
<.2 12.5 i.7 MEAN 3.2 2 1
<.04
.232 2.051 3
i.1 15.6 2 9.2 MEAN ALL STATIONS 2.7 2 2.1 04 1.06
.125 t.176
.3 1.3 19.6 2 12.9 (1) SEE PROGRAM EXCEPTIQ43 SECTIO 4 FOR EXPLAtaTIG4 I
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.l 1
TABLE C.X.1 ANALYTICAL DATA FOR SOIL SAMPLES COLLECTED IN 1NE VICINITY OF PBAPS, 1906 RESULTS IN LHITS OF PCI/ GRAM (DRY) 1 2 SIGMA
' STATION COLLECTION CODE PERIOD.
CS.134
,CS.137 CE.141 RA.226 1N.220 1AA 06/04
< 03 40 i.05
< 06.
.76 i.09 9
1.1 11/12
<.06 1.1-.1.1
< 1 1.4 2.2 -
1.7 2.2 MEAN
<.05
.75 i.99 C 06
'1.06 i.91 1.3 1 1.1 2
06/04 C 03 62 1.05 C 06 1.21 2.09 1.5 1.1 11/12
<.06 3.0 t.2
<.1 1.6 i.2 2.1 1
.3'
-MEAN
<.05 1,81 2 3.37
<.06 :
1.41 1.55 1.6
- .6 3A 06/04 C 03 68 1.05
< 06 1.3 i.1 1.4.
i.1 11/12
< 04 1.4 1.1
< 09
.9 2.1 -
1.1 1.2 NEAN
< 04 1.04 1 1.02
<.06 1.1 1.6 1.3 i.4 4H 06/04 ~
'C 01
.12 ~ t.02 '
< 04
.70 2.05 05 i.07 11/12
<.04
.46 2.06
'<.09 1.3 2.1 1.3 i.2 MEAN
< 03
.29 1.46
<.07 1.00 t.85 1.06 1.64 5
06/04
< 03
.36 i.04
<.06 1.01 2.09 1.5 2.1 11/12
< 02
.16 i.03
<.04 71 1.06 1.00 t.09 MEAN
<. 03
.27 1.25 C 05 66 2.42 1.25 1.71 60 06/04 C 03 79 1.06 07 1.06 1.1 1.1 1.3 1.1 11/12
.03 i.02 40 t.04 C 05
.66 1.06
.92 1.06 NEAN
.03 1.00
.60 i.55 06 i.03
.88 1 '.62 1.11 i.54 MEAN ALL STATIONS 03 i.03 79 1 1.57 07 i.04 1.05 1.63 1.30 1.75 f
1 i
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1 6
6 3
6 8 0
7 7
1 I
E 6
5 6
7 6
5 7
7 6
7 5
7 7
6 7
6 7
6 7
7 6
7 7
X H2 C
N O
E I E 9
0 6
2 3
4 6
7 1
2 A
6 0
2 3
4 5
6 7
6 9
0 1
L TD 1
2 1
2 2
2 2
2 3
3 3
3 4
4 4
4 4
4 4
4 4
5 5
B AO 2
3 A
TC T
S.
F f
TABLE C.XI.2 GUARTERLY TLD RESULTS FOR PEACH 60TTOM ATOMIC PG4ER STATION.1966 l
RESULTS IN LHITS OF MILLI.ROENTEDFSTD. 70. 2 2 S.D.
STATION MEAN 2 JAN-MAR APR.AH JUL.SEP OCT.DEC CODE 2 S.D.-(1) 1A 5.72.3 5.5 1 1.1 5.71.6 5.6 1.4 5.6 1.5 to 5.5 1 2.4 4.7 1.1 5.0 t.3 5.2 1.3 7.3 2.4 1C 6.0 t.4 5.6 &.4 6.0 t.5 6.0 t.5
' 6.3 &.5 1D 5.6 1.6 5.41.3 5.71.3 5.92.3 6.1 &.4 1E 5.6 1.6 5.2 1.4 5.31.4 5.7 1.3 6.1 1.1-1F 6.3 i.9 6.41.6-5.6 1.4 6.9 1.5 6.1 1.6 1G 4.4 i.7 4.0 2.2 4.4 1.1 4.3 1.2 4.6 &.3 1H 5.511.0 5.72.4 4.91.3 6.0 2.4 5.3 1.3 11 4.9 1.6 4.5 1.2 5.0 t.9 4.9 1.2 5.2 1.4 1J 6.3 1.9 6.5 2.5 5.6 1.4 6.6 2.4 6.2 i.5 il 3.6 2 1.4 3.32.3 3.4 1.1 4.6 1.4 3.5 1.2 1M 3.0 1.6 3.2 i.1 2.72.0 3.3 1.1 2.72.2 1HN 5.9 2 2.0 6.3 1.5 5.9 2.5 6.9 2.6 4.5 i.2 2
5.7 1.6 5.4 1.4 5.4 2.6 5.6 2.4 6.2 1.5 3A 4.5 1 1.4 3.9 1.2 4.5 t.4 4.2 1.3 5.5 2.4 4K 4.2 1.6 3.9 2.2 4.2 2.7 4.0 1.3 4.6 2.9 5
5.5 1.6 5.3 1.2 5.3 2.3 5.62.2 5.6 1 1.3 66 4.9 1 1.1 4.6 i.2 4.6 2.7 4.6 1.2 5.7 1.5 14 6.0 t.9 5.6 1.4 5.7 1.6 6.1 1.5 6.6 1.9 1 28 5.721.3 5.4 1.2 6.2 i.5 4.91.2 6.3 1.4 15 6.0 2.5 5.7 t '.4 6.0 t.4 6.1 2.3 6.3 2.3 16 6.3 1 1.0 5.6 1.4 6.5 1.5 6.2 1.5 6.7 1.6 17 6.6 2.6 6.4 1.3 6.9 1.6 7.02.4 7.1 2 1.0 16 6.31.7 5.92.4 6.0 1.4 6.4 1.4 6.7 1.2
- 1. MEAN AND TWO TIMES THE STANDARD DEVIATION OF THE GUARTERLY RESULTS.
i l
I f
. TABLE C.XI.2 QUARTERLY TLD RESULTS FOR PEACH DOTTOM ATOMIC PONER STATION,1906 RESULTS D4 (NITS OF MILLI-RotNTGEWSTO. MO.12 S.D.
STATION MEAN i JAN-MAR APR.JI.H JUL.SEP OCT.DEC CODE 2 S.D. (1).
19 6.1 1 1.1 5.5 1.3 5.6 i.6 6.5 i.4 6.7 i.6 20 5.1 i.6 4.72.2 5.2 1.2 5.3 2.4 5.3 i.5 21B 5.9 2.6 5.6 1.1 5.6 1.3 5.91.2' 6.4 i.2 22 6.3 2 1.1 5.7 1.4 6.2 1 1.2 6.3 2.6.
7.0 1.6 23-6.5 1.6 6.0 i.4 6.7 i.9 6.6 i.3 6.91.5 24.
4.3 2.6 4.4 1.2 4.0 t.4 4.8 i.1 4.0 i.1 26 6.7 i.8
'6.1 i.3 6.8 i.3 6.8 i.6 7.1 1.6 27 6.3 2.6 5.8 i.5 6.1 i.4 6.7 i.4 6.5 i.3 31 5.0 t.6 5.4 2.3 6.0 t.4 6.0 i.4 5.9 i.7 32 6.6 i 1.2 5.6 2.4 6.7 i.6 6.72.4.
7.2 i.9 33A 4.1 1.6 4.1 i.2 3.9 i.1 4.7 1.2 3.9 2.2 36 6.3 i.9 5.7 i.4 6.3 i.4 -
6.5 i.4 6,6 1.4 40 6.92.6 6.4 i.3 6.0 t.4 7.2 1.3 7.2 1.2 42 6.0 1 1.0 6.0 2.4 6.5 i.3 7.4 2.4 6.3 1.4 43 6.2 2 1.1 6.1 2.4 5.91.4 7.0 2.4 5.92.2 44 5.2 1 1.0 5.3 i.3 4.8 i.3 5.9 i.2 4.0 t.1 45 5.6 1 1.0 5.8 i.4 5.5 2.4 6.6 2.5 5.5 i.6 46 5.6 i.9 5.21.5 5.71.3 6.0 i.*.
6.2 i.3
. 47 7.0 i.9 6.6 i.5 6.71.3 7.3 i.5 7.5 i.4 48 5.5 i.5 5.5 i.3 5.3 i.2 6.1 1.4 5.0 t.2 49 5.4 i.7 5.21.2 5.5 2.3 5.0 2.4 5.0 t.4 50 7.0 1 6.5 1.5 6.71.9 7.2 2.3 7.5 1.5 51 5.7 i.9 5.7 i.3 5.3 i.6 6.3 1.4 5.5 2.3
- 1. MEAN AND TW3 TIMES THE STANDARD DEVIATION OF THE QUARTERLY RESULTS.
l l
}-
t
L.
TABLE C.XI.3 MEAN TLD RESULTS FOR THE PEACH BOTTOM ATOMIC POWER STATION
' SITE BOWDARY, MIDDLE, AND CUTER RDGS,1966 RESULTS IN WITS OF MILLI.ROENTGEWSTD. MO. - 2 2 STANDARD DEVIATIONS OF THE STATION DATA SAMPLE EXPOSURE SITE HIDDLE RING OUTER RING TYPE PERIOD MONTHLT JAN 1966 5.9 1 2.0 6.221.3 6.1 2 1.0' FEB 1966 5.8 1-2.2 6.211.6 5.711.0 MAR 1965 5.7 1 2.3 6.1 1 1.6 5.6 1 1.1 APR 1968 6.2 1 2.4 6.7 1 1.6 6.311.2 MAY 1966 7.0 1 3.4 6.6 2 4.5 7.1 1 1.4 JUN 1988 6.6 1 2.6 7.0 1 2.0 6.4 1 1.3 JUL 1988 6.4 1 2.7 7.0 1 1.8 6.711.2 AUG 1908 5.2 1 2.4 5.711.6 5.4 2 1.0 SEP 1966 6.4 1 2.6 6.911.8 6.6 1 1.3 OCT 1966 6.1 1 2.6 6.711.6 6.4 2 1.4 NOV 1900 6,0 1 2.6 6.4 2 1.7 6.2 i 1.3 DEC 1968 7.6 1 2.6 6.4 2 1.5 7.6 1 2.2 QUARTERLY JAN. MAR 1968 5.3 1 2.3 5.5 2 1.5 5.3 2 1.1 APR.JUN 1906 5.2 1 2.2 5.0 1 1.7 5.6 1 1.7-JUL.SEP 1968 5.6 1 2.3 6.1.1 1.6.
5.7 1 1.4 OCT.DEC 1908 5.6 1 2.7 6.1 1 1.9 6.0 1 2.0 TABLE C.XI.4 SumARY OF THE AreIENT DOSIMETRY PROGRAM FOR PE/CH BOTTON ATOMIC POWER STATION, 1966 RESULTS D4 WITS OP MILLI.ROENTGEWSTD MO.
PERIOD PRE.OP SAMPLE No. OF SAMPLES PERIOD PERIOD
. MEAN MEAN TYPE LOCATION
- 4ALYZED MD4DijM MAXDitt i 2 S.D. ' i 2 S.D. (1)
MONTHLY SITE 156 3.0 11.6 6.3 1 2.8 5.3 1 2.2 MIDDLE RING 300 3.3 12.3 6.6 2 2.7 6.0 1 2.0 CUTER RD4G 64 4.6 9.4 6.4 1 1.7 6.2 1 1.4 QUARTERLY SITE 52 2.7 7.3 5.4 1 2.4 5.4 1 1.7 MIDDLE RD4G 100 3.9 7.5 5.9 i-1.6 5.311.3 OUTER RING to 4.0 6.7 5.7 2 1.6 5.7 1 1.6 (1) THE PRE. OPERATIONAL MEAN WAS CALCULATED FROM TLD READDMS 1/07/73 TO EV05/73. STATIG43 1M, 31 #4D 32 WERE ADDED TO THE PROGRAM 7/06/73 AND STATIONS 33A AND 36 WERE M3T IN THE PRE. OPERATIONAL PROGRAM.
STATIONS 1m AND 40 THROUGH 51 WERE ADDED TO THE PROGRAM CN 07/12/60 1
SITE BOLNDARY RING STATIONS.18,1C,1D,1E,1F,1Ge 1H, 1J, 1L.
k 1M,1M4, 2, AND 40.
MIDDLE RING STATIONS 3A, 4K, 5, 68, 14, 15, 17, 22, 23, 26, 27, 31, 32, 33A, 36, 42, 43, 44, 45, 46, 47, 46, 49, 50, 51.
OUTER RDG STATIONS 125, 16, 16, 19, 20, 218, 24 t
i Ig TABLE C-MII.1 Surt1ARY OF COLLECTION DATES FOR SAMPLES COLLECTED IN THE VICINITY OF PBAPSe 1966 AIR PARTICULATE C AIR IODINE 3
GROUP I - SITE BOL.HDARY LOCATIONS
-WEEK #
1 OR 1A 15 1Z 2
j MTH. COr1P.
{
--------------==------------ --------------
1 1'
01/01-01/09/06 01/01-01/09/86 01/01-01/09/08 01/01-01/09/86 2
01/09-01/16/06 01/09-01/16/06 01/09-01/16/06 Of/09-01/16/06 3
01/16 01/23/80 01/16-01/23/86 01/16-01/23/88 01/16-01/23/86 4
01/23-01/30/06 01/23-01/30/06 01/23-01/30/86 01/23-01/30/06 JAN 66 01/01-01/30/06 01/01-01/30/06 01/01-01/30/88 5
01/30-0 U06/06 01/30-0 UO6/86 01/30 0 U 0 V86 01/30-0 U O6/86 6'
Cu06-0U13/06 02/06-02/13/06 02/06-0U1V86 02/06-02/1V86
.7 02/13-0U20/06 02/13 02/20/06 02/13-0U20/88 Oul3-0U20/06 6
0U20-0U27/86 0Ut0-02/27/86 Out0-02/t7/86 02/20 02/27/06 FEB 86 Ci/30-0 U27/86 01/30-0 U27/86 01/30-0U27/06 9
0U27-03/05/06 0U27-03/05/86 0U27-DV05/86 02/21-03/05/66 10 03/05-03/1U86 03/05-03/12/86 03/05-03/1USS OV05-03/12/06 11 03/12-03/19/06 03/12-0V19/06 OV12-0V19/06 03/12-03/19/06 12 03/19-03/26/06 03/19-03/26/06 03/19-0 V26/06 03/19-0 V26/06 13 03/26-04/02/86 03/26-04/02/06 03/26-04/02/06 03/26-04/0U86 MAR 86 CU27-04/0U60 02/27-04/0U68 0U27-04/02/06 14 04/02-04/09/06 04/02-04/09/06 04/02-04/09/06 04/02-04/09/06 15 04/09 04/16/06 04/09-04/16/06 04/09-04/16/86 04/09-04/16/86 l
16 04/16 04/23/86 04/16-04/23/06 04/16-04/23/06 04/16-04/23/86 17 04/23 04/30/06 04/23-04/30/66 04/23-04/30/86 04/23-04/30/86 APR 66 04/02-04/30,'86 04/02-04/30/06 04/02-04/30/06 to 04/30-05/07/66 04/30-05/07/86 04/30-05/07/86 04/30-05/07/06 19 05/07-05/14/08 05/07-05/14/86 05/07-05/14/86 05/07-05/14/86 20 05/14-05/21/86 05/14-05/21/06 05/14-05/21/86 05/14 05/21/86 21 05/21-05/26/06 05/21-07/26/06 05/21-05/26/06 05/21-05/26/86 MAY 86 04/30-05/26/86 04/30-05/26/06 04/30-05/26/86 22 05/26-06/04/86 05/26-06/04/86 05/20-06/04/06 05/26-06/04/66 23 06/04-06/10/66 06/04-06/10/66 06/04-06/10/86 06/04-06/10/06 24 06/10-06/1 U86 06/10-06/16/86 06/10-06/16/06 06/10-06/16/06 25 06/16-06/26/88 06/16-06/26/06 06/16-06/26/06 06/16-06/26/06 26 06/26-07/0 U86 06/26-07/0 V86 06/26-07/02/86 JLJ4 80 05/20-07/02/06 05/26-07/02/06
. 05/20-07/02/06 27 07/02-07/09/06 07/02-07/09/86 07/02-07/09/06 07/02-07/09/86 26 07/09-07/16/86 07/09-0 U16/86 07/09 07/16/86 07/09-07/16/86 29 07/16-07/22/86 07/16-07/22/86 07/16-07/2U06 07/16 0U2U86 30 07/22-07/30/86 07/22-07/30/86 07/22-0 U30/06 07/22 07/30/86 JUL 66 07/02-07/30/86 07/02-07/30/06 07/02-07/30/06 31 07/30-06/06/86 07/30-00/06/06 07/30-06/06/06 0U30-06/06/80 32 06/06-06/12/06 06/06-06/12/86 Oc/06-06/12/86 06/06-06/12/86 33 06/12-06/f0/86 06/12-06/20/86 06/12-06/20/86 06/12-06/20/86 34 06/20-06/07/06 08/20-06/2 U66 06/20 06/2 U66 C6/20-00/27/86 35 06/27-09/03/06 06/27-09/03/86 06/27-09/03/86 06/27-09/03/06 AUG 86 0 U30-09/03/66 07/30-09/0 V86 07/30-09/03/06 36 09/03-09/10/66 09/03-09/10/06 09/03-09/10/86 09/03-09/10/86 37 09/10-09/17/86 09/10-09/17/06 09/10-09/17/86 09/10-09/1U66 36 09/17-09/23/86 09/17-09/23/86 09/17-09/2 V86 09/17-09/23/06 39 09/23-10/41/86 09/23-10/01/86 09/23-10/01/06 09/23-10/01/06 f
- SEP 86 06/27-10/01/06 06/27 10/01/86 06/27-10/01/86 40 10/01-10/06/06 10/01-10/06/06 10/01-10/0US$ 10/01-10/06/86 41 10/06-10/15/86 10/06-10/15/86 10/06-10/15/06 10/06-10/15/86 42 10/15-10/12/06 10/15-10/22/86 10/15 10/22/06 10/15-10/2 uS6 l
43 10/22-10/29/06 10/22-10/29/06 10/22-10/29/06 10/22-iO/29/86 l
OCT 86 -
10/01-10/29/06 10/01-10/29/06 10/01-10/29/86 I
44 10/29-11/05/06 10/29-11/05/06 10/29-11/05/06 10/29-11/05/86 45 11/05-11/1 U66 11/05-11/12/86 11/05-11/12/86 11/05-11/12/06 46 11/11-11/19/8611/12-11/19/0611/12-11/19/0611/f t-11/19/06 i
47 11/19-11/26/06 11/19-11/26/06 11/19-11/26/06 11/19-11/26/06
~
46 11/26-12/04/86 11/26-12/04/86 11/26-12/04/06 11/26-12/04/06 HW OS 10/29-12/04/86 10/29-12/04/06 10/P9-12/04/86 49 12/04-12/10/06 12/04-12/10/86 12/04-12/10/06 12/C4-12/10/86 50 1 U10-1 U17/06 1 U10-12/17/06 1 Ut o-1 U17/86 1 U10-12/17/06 51 12/17-1 U24/06 1 U17-12/24/06 1 U17 1 U24/86 1 U17-1 U24/06 52 12/24-12/31/06 12/24-12/31/86 12/24-12/31/06 1 U24-12/31/86 DEC SS 12/04-12/31/86 1 U04-12/31/06 12/04-12./31/86
TABLE C-XII.1 SUtt1ARY CF COLLECTICH DATES FOR MP1PLES COLLECTED IN THE VICINITY OF PDAPS 1968 AIR PARTICULATE C AIR IODINE GROUP II - INTERP1EDIATE DISTANCE UX%TIONS WEEK #
OR 3A 4B 5
6B 14 MTH. COMP.
1 01/01-01/09/88 01/01-01/09/06 01/02-01/10/86 01/02-01/10/861U31-01/10/66 2
01/09-01/16/68 01/09-01/16/88 01/10-01/16/06 01/10-01/16/06 01/10-01/16/OS 3
01/16-01/23/88 01/16-01/23/08 01/16-01/23/06 01/16-01/26/08 01/16-01/23/e8 4
01/23-01/30/88 01/23-01/30/06 01/23-01/30/06 01/26-01/30/06 01/23-01/30/06 JAN SS 01/01-01/30/88 01/01-01/3 U68 01/02-01/3 USS 01/02-01/30/08 12/31-01/30/06 5
01/30-0UO6/86 01/30-0UO6/88 01/30-02/06/88 01/30-02/06/06 01/30-02/06/06 6
CUO6-0U13/88 CUO6-0U13/00 02/06-02/14/SS OUO6-0U14/06 02/06 02/14/80 7
02/13-0U20/88 02/13-02/20/88 02/14-02/2WSS CU14-0U20/06 02/14-02/20/06 8
02/20-0U27/80 CU20-02/27/80 02/20-02/27/06 02/20-02/27/06 02/20-02/27/86 FEB 80 01/30-02/27/08 01/30-0U27/88 01/30-02/27/06 01/30-0U27/06 01/30-0U27/86 9
02/27-03/05/06 0U27-03'05/88 02/27-03/05/06 02/27-03/05/08 CU27-03/05/86 10 03/05-03/1U80 03/05-03/1USS 03/05-03/12/06 03/05-03/1USS 11 03/12-03/19/00 03/12-03/19/06 03/12-03/19/06 03/12-03/19/06 O V12-03/19/06 12 03/19-03/26/06 03/19-03/26/06 03/19-03/26/06 03/19-03/26/06 03/19-03/26/06 13 03/26-04/0USS CV26-04/0USS 03/26-04/0U8S 03/26-04/02/0S 03/26-04/02/80 MAR OS 02/27-04/02/80 02/27-04/02/SS 02/27-04/02/60 02/27-04/0U68 02/27-04/02/06 14 04/02-04/09/00 04/02-04/09/88 04/02-04/09/88 04/02-04/09/06 04/02-04/09/80 15 04/09-04/16/06 04/09-04/16/06 04/09-04/16/86 04/09-04/16/80 04/09-04/16/06 16 04/16-04/23/88 04/16-04/23/88 04/16-04/23/06 04/16-04/23/86 04/16-04/23/80 17 04/23-04/30/8S 04/23-04/30/86 04/23-04/30/68 04/23-04/30/06 04/23-04/30/88 APR SS 04/02-04/30/88 04/02-04/30/06 04/02-04/3 U86 04/02-04/30/06 04/02-04/30/88 10 04/30-05/07/88 04/30-05/07/86 04/30-05/07/88 04/30-05/07/88 04/30-05/07/0S 19 05/07-05/14/86 05/07-05/14/88 05/07-05/14/86 05/07-05/14/06 05/07-05/14/88 20 05/14-05/21/88 05/14-05/21/06 05/14-05/21/06 05/14-05/21/88 05/14-05/21/88 21 05/21-05/28/03 05/21-05/28/88 05/21-05/28/88 05/21-05/28/88 05/21 05/28/86 MAY SS 04/30-05/28/86 04/30-05/28/86 04/30-05/2W88 04/30-05/28/88 04/30-05/28/88 22 05/28-06/04/85 05/26-06/04/83 05/20-06/04/80 05/28-06/04/06 05/26-06/04/86 23 06/04-06/10/80 06/04-06/10/06 06/04-06/11/86 06/04-06/11/06 06/04-06/11/88 24 06/10-06/18/88 06/10-06/1C/68 06/11-06/19/06 06/11-06/19/06 06/11-06/19/88 25 06/18-06/26/88 06/18-06/26/88 06/19-06/26/OS 06/19-06/26/06 06/19-06/26/88 26 06/26-07/02/06 06/26-07/02/86 06/26-07/02/06 06/26-01/0U80 06/tb-07/0U80 JLN 88 05/26-07/0 USS 05/28-07/0 U86 05/28-07/02/86 05/20 07/0 USS 05/20-07/02/06 27 07/02-07/09/06 07/02-07/09/88 07/02-07/09/88 07/02-07/09/06 07/02-07/09/88 to 07/09-07/16/06 07/09-07/16/06 07/09-07/16/83 07/09-07/16/08 07/09-07/16/06 29 07/16-07/22/8S 07/16-07/2 U SS 07/16-07/24/80 07/16-07/24/88 07/16-07/24/06 30 07/22-07/30/88 07/22-07/30/86 07/24-07/30/08 07/24-07/30/86 07/24-07/30/06 JUL 80 07/02-07/30/OS 07/02-07/30/SS 07/02-07/30/86 07/02-07/30/80 07/02-07/30/89 31 07/30-08/06/08 07/30-08/06/88 07/30-06/06/08 07/30-08/06/88 07/30-00/06/08 32 03/06-00/12/00 08/06-06/12/88 06/06-06/13/08 OS/06-08/13/88 08/06-06/13/06 33 05/12-06/20/08 08/12-0S/20/88 08/13-08/20/06 08/13-08/20/06 08/13-06/20/06 34 08/20-06/27/06 06/20-08/27/68 06/20-06/27/80 06/20-06/27/68 06/20-06/27/86 35 06/27-09/03/88 O V 27-09/03/SS OS/27-09/03/SS 06/27-09/03/88 05/27-09/03/06 AUG 80 07/30-09/03/88 07/30-09/03/0S 07/30-09/03/06 07/30-09/03A38 07/30-09/03/86 36 09/03-09/10/88 09/03-09/10/86 09/03-09/10/0S 09/03-09/10/8C 09/03-09/10/88 37 09/10-09/17/08 09/10-09/17/80 09/10-09/17/06 09/10-09/17/06 09/10-09/17/80 38 09/17-09/23/68 0?/17-09/23/88 09/17-09/24/80 09/17-09/24/06 09/17-09/24/80 39 09/23-10/01/80 09/23-09/30/06 09/24-10/01/06 09/24-10/01/88 09/24-09/30/SS
{
??P SS 06/27-10/01/88 08/27-09/30/86 05/27-10/01/88 08/27-10/01/88 06/27-09/30/88 40 10/01-10/06/86 09/30-10/05/88 10/01-10/09/06 10/01-10/09/06 09/30-10/09/06 41 10/08-10/15/68 10/06-10/15/06 10/09-10/15/06 10/09-10/15/86 10/09-10/15/88 42 10/15-10/22/06 10/15-10/22/80 10/15-10/22/BS 10/15-10/22/88 10/15-10/21/06 43 10/22-10/29/66 10/22-10/29/06 10/22-10/29/80 10/22-10/29/06 10/22-10/29/88 OCT SS 10/01-10/29/88 09/30-10/29/SS 10/01-10/29/85 10/01-10/29/80 09/30-10/29/86
(
44 10/29-11/05/86 10/29-11/05/88 10/29-11/05/86 10/29 11/05/06 10/29-11/05/06 45 11/05-11/1 USS 11/05-11/12/06 11/05-11/12/88 11/05-11/12/86 11/05-11/12/06 46 11/12-11/19/80 11/12-11/19/06 11/12-11/19/06 11/12-11/19/06 11/12-11/19/OS l
47 11/19-11/26/86 11/19-11/26/88 11/19-11/26/08 11/19-11/26/88 11/19-11/26/06 46 11/26-12/04/88 11/26-12/04/86 11/26-1 UO4/80 11/26-1 UO4/88 11/26-1 UO4/SS HW 08 10/29-12/04/86 10/29-1UO4/SS 10/29-1UD4/SS 10/29-12/04/88 10/29-12/04/88 49 1 UO4-1 U10/8S 1 UO4-12/10/88 12/04-1 U10/08 1 UO4-1 U10/06 1 U64-1 U10/06 50 12/10-1U17/881U10-12/17/SS 1U10-1U18/861U10-12/10/031U10-12/16/OS 51 12/17-tu24/BS 12/17-1U24/80 1U18-12/24/BS 12/18-1U24/86 1U16-1U24/06 52 12/24-1 U31/SS 12/24-12/31/06 1 U24-1 U31/06 12/24-1 U31/06 DEC OS 1 UC4-1 U31/SS 12/04-1 U31/08 t uo4-12/31/88 1 UO4-12/31/80 1 UO4-1 U31/85
/
h k
TABLE C-XII.1 SuttARY OF COLLECTION DATES POR SAMPLt3 i
COLLECTED Di THE VICINITY OF PSAPS,1986 AIR PARTICULATE C AIR IODINE I
880UP II. ImtfritDIATE DISTANCE LOCATIONS HttK 8 OR 15 17 31 32 33A 36 MTH. COMP.
i 1
12/31 01/10/06 01/02-01/10/86 01/02 01/10/86 12/31 01/10/06 12/31-01/10/06 12/31-01/10/06 2
f t/10-01/1ue6 01/10-01/tuS6 01/10-01/1U88 01/10-01/f ue6 01/10 01/tuS8 Ol/10-01/1UO6 3
01/16 01/23/06 01/16-0t/23/06 01/te-01/t V86 01/16 01/23/86 01/16 01/tV86 01/16 01/23/06 4
01/23 01/30/06 01/23-01n0/06 01/23-01/30/06 01/13-01n0/86 01/23-01n0/06 01/t3-01/30/86 I
JAN 86 12/31-01/30/06 01/02-01/30/06 01/02-01/30/06 12/31-01/30/96 12/31 01n0/06 1U31 01/30/06 5
01/30-Of/DU86 01/30-02/06/86 01/30-02/06/06 01/30-Ot/ DUBS 01/30 02/06/06 01/30-02/ sus 6 6
02/06 02/14/06 02/06 02/14/06 02/06-02/14/96 St/06-of /1&B6 02/06-02/14/06 Of/06 02/14/06 7
02/14-02/20/86 St/14-02/tuS6 02/14 0Ute/86 02/14-01 '20/96 02/14 02/20/96 02/14-02/20/06 8
8 02/20-02/27/86 02/20-02/27/06 02/20-0Ut7/06 02/20 0227/06 02/20-02/27/06 02/20 02/27/86 FEB 86 01/30-0t/t7/88 01/30-02/27/86 01/30-tutF/06 01/30-0t/27/06 01n0-02/2746 01/30-0Ut7/80 9
Ot/27-SV05/06 St/27 0V05/06 02/27 0F05/86 02/27-03/05/86 02/27-0F05/06 St/27 0F05/06 10 03/05-0W12/06 OV05-0Vit/06 DV05-0V12/96 0F05-0V12/06 OV05-0V12/06 03/05-03/12/06 11 03/12-03/19/86 SVit-03/19/06 OW12-0Vt9/86 03/12-03/19/88 03/12-03/19/86 OVit-0V19/06 8
12 03/19 03/26/88 03/19-0V26/06 03/19-03/26/06 OW19 03/26/06 OV19-03/tuo6 03/19-03/tue6 13 03/26-04/02/06 03/26 04/02/06 DVt6-04/02/88 OW26-04/02/06 03/26-WOf/06 03/26-04/02/06 MAR e6 Out7-04/Ouee 02/27-04/02/06 02/27-04/02/83 02/27-cuat/86 02/27-04/02/06 Out7-04/02/06 14 04/02-04/09/06 04/02 04/09/06 04/02 04/09/06 04/02-04/09/06 WO2-DV09/06 04/02-04/09/06 15 04/09 04/16/06 04/09-04/16/06 04/09-04/tuS6 04/09-04/16/06 04/09-04/f uS6 04/09 04/16/86 I
16 04/16-04/23/06 04/16-04/23/06 04/16-04/23/06 04/16-04/23/06 04/16-04/23/06 04/16-04/23/06 17 04/23-04/30/06 04/23-04/30/86 04/23-W30/06 04/23-04 30/86 04/23-04/3U66 04/23-W30/06 APR 66 04/02 04/30/06 04/02 04/30/06 04/02-04/30/06 04/02-W 30/06 04/02-04/30/06 04/02-04/30/06 16 04/30-05/07/06 04/30-05/07/96 04/30-05/07/06 04/30-05/07/06 04/30-05/07/86 04/30-05/07/06 19 05/07-05/14/06 05/07-09/14/06 05/07-05/14/06 05/07-05/14/06 05/07-05/14/06 05/07 05/14/96 1
20 05/14-05/21/06 05/14-05/21/86 05/14-05/21/06 05/14-05/21/86 05/14-05/21/86 05/14-05/21/86 21 05/21-05/26/06 05/21-05/26/06 05/11-05/26/06 05/tt-05/2 W86 05/tt-05/tW86 05/21-05/26/06 NAY 86 04/30-05/26/06 04/30-05/26/06 04/30-05/26/06 04/30-05/tW86 04/30-05/26/06 04/30-05/26/06 22 05/26-06/04/06 05/26 0V04/06 05/26-0U04/06 05/26-0U04/06 05/26-06/04/86 65/26-0U04/06 23 06/M-0U11/06 0u04-06/11/86 OU04-06/t t/86 06/M-06/11/86 OuG4-06/11/86 06/04-0Vit/86 I
24 06/11-06/19/86 06/11-06/19/06 0U11-06/19/06 06/11-0U19/06 0 U11-0U19/06 0 U11 0U19/06 25 0U19-Ou2U86 06/19-06/26/86 06/19-Out6/86 Out9-06/26/96 06/19-OutuS6 0U19 06/tuS6 26 06/ts-07/0t/06 0Ut6-07/02/06 0Utb 07/0V06 06/ts-07/02/06 06/tb-07/0V66 0Uts-07/0t/86 JLN SS C5/26 07/0US6 05/26-07/0U86 05/26-07/02/86 05/26-07/02/86 05/26-07/6f/86 05/26 07/0U66 27 07/02-07/09/06 07/02-07/09/06 07/02-07/09/06 07/02-07/09/86 07/02-07/09/06 07/02-07/09/06 to 07/09 07/f uS6 07/09 07/1U86 07/09-07/1U66 07/09-07/tv86 07/09-0U16/86 07/09 07/luS6 29 07/16-07/24/06 07/16-07/24/86 07/16-07/24/06 0U16-07/24/06 0Uf 6-0U24/06 07/16-07/24/06 30 07/24-07/30/06 07/24-07/30/06 07/24-0U30/86 0Ut4-07/30/06 07/24-07/30/06 07/24-07/30/86 JUL 66 0UO2-0U30/06 07/02-0W30/06 07/02-07/30/86 07/02-07/30/06 0U02-07/30/06 07/02-0U30/06 11 07/30-WouS6 07/30-06/0U86 07/30-06/ sus 6 07/30-06/0uS6 07/30-06/0uS6 07/30-OvouB6 32 OWO6 0W13/06 06/06-0W1 W86 OWO6-06/13/06 OW O4-0W1 W86 06/06-0W13/06 06/06-06/1 W86 33 06/13-06/10/06 DW13-0W20/06 06/13-06/20/06 OW13-0W20/06 DW13-06/20/06 06/13-0W20/06 34 06/20-06/27/06 06/20-06/27/06 06/20-06/27/06 06/20-0W27/86 06/20-0W27/06 OW20 06/tT/06 35 06/27 09/0F86 GW27-09/03/06 06/27-09/0V86 OW17-09/0F66 OW27-09/03/06 06/27-09/03/86 i
AUG 86 07/30-09/0F86 07/30 09/0F06 07/30-09/0W86 07/30-09/03/86 07/30-09/0V86 07/30-09/03/06 36 09/03-09/10/06 09/03-29/10/96 09/03-09/10/06 09/03-09/18/06 09/03-09/10/06 09/03-09/10/06 37 09/10-09/17/06 09/10-09/17/06 09/10-09/17/06 09/10-09/17/06 09/10-09/17/86 09/10-09/17/86 36 09/17 09/24/06 09/17-09/24/96 09/17-09/24/86 09/t7-09/24/06 09/f 7-09/24/06 09/17-09/24/06 39 09/24-69/30/06 09/24-18/01/88 09/te-18/01/D6 09/24-09/30/06 09/24-09/30/06 09/24-09/30/06 i
StP 86 06/27 09/30/86 OW27-18/01/88 OW 27-18/01/86 06/27-09/30/06 OW27 09/30/86 06/27-09/30/06 40 09/30-18/09/M61W91-16/09/9618/01-10/09/06 09/30-18/0940 09/30-10/99/86 09/30 18/99/06 41 10/09 18/15/86 10/09 18/15/86 10/09-18/15/86 1 W99-10/15/86 10/09-t W1548 18/99-10/15/06 42 10/15-10/22/96 10/15-10/22/86 10/15-18/tt/86 10/15 10/tt/S6 18/15-1 Ftt/88 10/15 10/22/06 43 10/22-18/29/80 t Wit-10/29/86 10/12-10/19/86 10/22-10/t9/06 10/22-18/89/06 18/tt=1 W29/06 OCT 86 09/30-10/t9/8818/01-10/29/8618/01-10/29/96 09/30-10/19/96 09/30-tW29/06 09/30-f W29/06 44 10/29-11/05/86 10/t 9-11/05/86 10/29 11/05/86 1 F29 11/05/86 10/29-11/05/86 10/29-11/05/06 45 11/05-11/12/06 11/05-11/12/06 11/05-11/12/06 11/05-11/12/06 11/05 11/12/86 1 t/05-11/12/06 46 11/12-11/19/06 11/12-11/19/88 11/12-11/19/86 11/12-11/19/96 11/12-11/19/06 11/12-11/19/86 47 11/1911/tuS611/19-11/tuS611/19-11/tuS611/19-11/ tub 611/1911/tuS6 f t/19.t t/ tub 6 I
to 11/26-12/04/b6 11/26-1UD4/06 f t/26-12/04/06 11/26-i t/W86 11/26-12/04/86 11/26-12/04/96 MN 06 10/19-1 f/04/06 10/29-12/04/86 10/29 12/M/86 10/29-12/04/86 10/29-12/04/06 10/29-12/04/06 l
49 12/04-12/10/88 12/04-12/10/06 12/04-12/10/06 12/04-12/10/86 12/04-12/10/06 12/04-12/10/06 50 f t/10-1 U16/06 12/10-12/16/06 12/10-12/16/06 1 U10-12/16/06 12/10-12/16/06 i t/10-It/1W86 51 12/16-If/24/86 If/16-1t/24/061U16-12/24/06 f t/16-it/24/0612/16-12/24/0612/16-12/24/06 52 it/24-12/31/8612/2412/31/0612/24-12/31/0612/2412/31/8C 12/24-12/31/0612/24-12/31/06 OtC OS 12/04-12/31/06 12/04-12/31/86 f t/M-12/31/86 12/04-12/3t/86 1UD4-12/31/06 it/M-S t/31/86 i
TABLE C-XII,1 SLt91ARY OF COLLECTION DATES FOR SAMPLES COLLECTED IN THE VICINITY OF PBAPS 1906 iI AIR PARTICULATE C AIR IODINE GROUP III - DISTAtR LOCATIONS WEEK #
OR 12A 12D HTH, COMP, 1
01/04 01/11/06 01/04-01/11/60 2
01/11-01/18/66 01/11-01/19/86 3
01/16-01/25/00 01/19-01/25/86 4
01/25-02/01/80 01/25-02/01/80 JAN OS 1U29 02/01/061U29-02/01/60 5
02/01-0 UCS/06 0 UQ1-02/0W D6 6
0U06-0U16/06 CU0S-02/16/06 7
0U16-02/2U60 CU16 02/2U80 8
Q U22 02/29/86 02/22-0 U29/06 FEB 68 02/01-02/29/06 02/01-0 U29/06 9
02/29 03/07/88 02/29 0 V07/88 10 03/07-03/14/66 03/07-03/14/06 11 03/14 03/21/80 03/14-03/21/08 12 03/21-03/28/88 OV21-03/28/B0 13 03/25 04/04/06 C V20-04/04/88 MAR 68 CU29 04/04/86 07/29-04/04/06 14 04/04-04/11/86 04/04-04/11/85 15 04/11-04/18/08 04/11-04/16/88 16 04/18-04/25/06 04/16-04/25/06 17 04/25-05/02/06 04/25-05/02/06 APR 68 04/04-05/0 USS 04/04-05/02/08 10 05/02-05/09/00 05/02-05/09/88 19 05/09-05/16/06 05/09-05/16/00 20 05/16-05/23/08 05/16 05/23/06 21 05/23-05/31/08 05/23-05/31/88 MAY BS 05/02-05/31/88 05/02-05/31/80 22 05/31-06/06/06 05/31-06/06/06 23 06/06-06/13/08 06/06-06/13/00 24 06/13-06/20/80 06/13-06/20/80 25 06/20-06/27/06 06/20-06/27/66 l
26 06/27-07/05/06 06/27-07/05/86 JL.N 88 05/31-07/05/88 05/31-07/05/88 27 07/05-07/11/88 07/05-07/11/88 20 07/11-07/16/88 07/11-07/18/86 29 07/18 07/25/88 07/16-07/25/00 30 07/25 08/01/88 07/25-06/01/86 JUL 80 07/05-0S/01/86 07/05 08/01/06 31 08/01-08/08/08 08/01-0V08/88 32 08/06-06/15/86 0S/05-06/15/06 33 05/15-00/2USS 08/15-06/22/06 34 0S/22-05/29/08 06/22-06/29/80 AUG 64 06/01-00/29/08 05/01-08/29/88 35 08/29-09/06/80 06/29-09/06/06 36 09/06-09/1USS 09/06-09/1U66
]
37 09/12-09/19/8S 09/12-09/19/06 4
30 J
39 09/26-10/0 F06 09/26-10/0 V60 1
SEP OS 08/29-10/03/00 06/29-10/03/06
]
40 10/03-10/11/80 10/03-10/11/88 j
41 10/11-10/17/88 10/11-10/17/80-42 10/17-10/24/86 10/17-10/24/66 43 10/24-10/31/06 10/24-10/31/06
'l OCT 88 10/03-10/31/88 10/03-10/31/88 44 10/31-11/05/86 10/31-11/06/06 45 11/06-11/14/88 11/06-11/14/86 1
46 11/14 11/21/86 11/14-11/21/86 47 11/21-11/28/86 11/21-11/26/88 tm 86 10/31-11/28/06 10/31-11/26/06 48 11/26-12/05/88 11/26-12/05/60 I
49 1 UC5-12/12/88 12/05-1 U1 USS 50 1 U12-12/19/06 1 U12-1 U19/88 51 12/19 1 U27/88 1U19 12/27/SS 52 12/P 7-01/03/89 12/27-01/03/09 DEC BS 11/26-01/03/69 11/26-01/03/09 Il I:
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t TABLE C-XII.1. SuttARY OF COLLECTION DATES FOR SAMPLES CDLLECTED 3H THE YZCINITY OF PBAPSe 1900 TLD - ElutRTERLY
- ^.,
JAN-MAR APR-JLN.
JUL-SEP OCT-SEC STATION 1906
'1986 9986 1986 CODE 1A ' 01/01-04/02 04/02-0 Ut6 Out6-10/01 10/01-12/31
- l~
16 01/01-W 02 04/02-0Ut6 Out6-10/01 10/01-12/31 1C 12/31-W 02 W 02-06/26 GU16-10/01 10/01-12/31 10 01/01 W 92 04/02-06/26 $Ut6-10/01 1 U01-18/31-it 12/31-04/02 W OR-Oute tut 4-0 U30 09/30-12/31 1F 12/31 04/02 W et=0Ut6 W 16-1 U01 10/01-12/31-1G 01/01-04/02 W et-O ut6 0Ut6-10/01 10/01-12/31 1H 01/01-04/02 W0t=0Ute tut 6-10/01 10/01-12/31 11 12/31=W02 WO2-0Ut6 0Ut6-10/01 10/St=1U31 1J 12/31 W O2 04/02-0 Ut6 $Ut6-10/01 10/01-12/31 1L-12/31-W 02 04/02-06/26 07/01-09/30 09/30 12/31
.1M 12/31-04/02 M/0t=06/26 $Ut6-09/30 09/30-12/31 1m 01/01-M/02 04/02-06/26 Out6-10/01 10/01-1F/31 2
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l DATA TABLES AND FIGURES COMPARISON LABORATORY
- I I
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5 I
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APPENDIX 0:
DATA TABLES AND FIGURES - COMPARISON LABORATORY Table Table D-I.1 Analytical Data for Surface Water Samples Collected in the Vicinity of PBAPS, 1988.
Table D-II.1 Analytical Data for Drinking Water Samples Collected in the Vicinity of PBAPS, 1988.
' Table D-III.1 Concentrations of_ Gross Beta Radioactivity in Air Particulate Samples Collected in the Vicinity of' PBAPS, 1988.
Table D-III.2 Concentrations of Gamma Emitters in Air Particulate Samples Collected in the Vicinity of PBAPS,1988.
Table D-IV.1 Analytical Data for Milk Samples Collected in the Vicinity of PBAPS, 1988.
Table D-V.1 Concentrations of Gross Beta Radioactivity in Well Water Samples Collected in the Vicinity of PBAPS, 1988.
Table D-VI.1 Summary of Collection Dates for Samples Collected in the Vicinity of PBAPS, 1988.
Fioures Figure D-1 Weekly Gross Beta Concentrations in Air Particulate Samples Collected from PBAPS Locations IA and IZ, 1988.
Figure D-2 Weekly Gross Beta Concentrations in Air Particulate Samples Collected from PBAPS Locations 4A and 4B, 1988.
I
)
1
]
i The. following section contains data and figures illustrating I
the analyses performed by the secondary laboratory.
Duplicate samples were obtained from several locations and media and split g
between Teledyne Isotopes (TI) and Clean Harbors (CH).
3i Comparison of the results for most media were within expected ranges, though occasional differences were seen:
iI!
1.
TI gross beta results in water were generally higher than CH.
However, CH K-40 results were generally g'
higher than TI results.
3 2.
CE results for gross beta in air particulate were consistently higher than thase obtained form TI..
I t.
was observed that the ratio between the two 3
laboratories remained relatively constant throughout 5
the year (Figures D-1 and D-2).
Inspection of the EPA g
results (see Appendix F) indicated a similar ratio.
The differences were accounted for by slightly different 3
calibration procedures used by the laboratoryles, g
respectively.
I I
E 8
E E
I I
I I
I
't TABLE D-I.1
- 1ALYTICAL DATA FOR SURFACE HATER SAMPLES COLLECTED IN THE VICD4ITY OF PBAPS,1986 I
RESULTS D4 lt4ITS OF PCI/ LITER 12 SIGMA COLLECTIO4 GROSS BETA GROSS BETA STATIQ4 DATE SOLUBLE DISOLUDLE DE-7 K-40 tt 4-54 CO-56 5
13A 01/30/88 1.6 i.4 9
2.1
< 30 C 50
<2
<3 92/27/08 2.7 1.5
.31 i.09 C 20
< 50
<2
<3 04/02/06 1.6 i.4
.C 1.1
< 20
< 50
<2
<3 (1) 0V30/SS 05/20/80 2.5 i.5 1.2 2.2
< 20
< 50
<2
<2 I
06/26/80 2.4 2.5 5
2.1
< 20
< 50
<2
<3 07/30/00 3.4 2.9
<.07
< 20
< 50
<2
<2 09/03/80 2.9 i.i
.21 1.00
< 20 140 1 60
<2
<3 09/30/60 3.2 1 sb
.26 i.09 C 20
< 50
<2
< 2 11/05/06 3.1 i.6
.10 t.09
< 30 60 1 50
<3 C 3 8
12/04/88 1.5 i.5 3.6 1.3
< 20
< 50
<2
< 3 12/31/00 2.0 t.5 4
1.3
< 20 C 60
<2
<3 MEAN 2.5 1 1.3
.77 2 2.00
< 22 62 2 55
<2
< 3 i
135 01/29/08 2.0 i.6 7.4 i.9 30 1 30
< 50
<2
< 3 CU26/oS 2.3 1.5 4.2 2.6
< 40
< 50
<2
<4 03/10/89 2.3 1.5 15 i.00
< 30 C 50
<2
<3 04/28/e8 i.9 2.5 09 i.07
< 30 60 t 60
<3
<3 1
05/26/80 1.7 i.4 1.6 1.2
< 20
< 50
<2
<2 06/17/08 2.0 t.5 5.4 1.6
< 20 60 1 60
<2
<3 1
07/22/06 2.6 i.6 5
1.1
< 20
< 50
<2
<3 08/26/00 2.7 i.5 9
1.1
< 30
< 50
<2
<3 09/23/08 3.0 1.5
.3 i.1
< 20
< 50
<2
<3 10/28/06 3.5 i.6 9
i.1
< 30
< 50
<3 C 3 11/10/00 2.2 i.5 1.5 t.2
< 30 90 1 60
<2
< 3 12/09/00 2.3
- .5 1.5 1.2
< 30 60 1 50
<2
< 3 MEAN 2.4 1 1.0 2.04 1 4.70 26 1 12 50 t 27 C2
< 3 1LL 01/01-01/29/00 2.4 1.5
.7 1.1
< 30
< 50
<3
< 3 01/29-0 U26/06 2.2 t.5 3
t.1
< 20
< 50
<2
< 3 02/26-04/01/88 3.1 1.5
.7 i.1
< 20
< 50
<2
< 3 5
04/01-04/29/08 1.9 1.5 6
1.1
< 20
< 50
<2
< 2 04/29-05/27/08 1.9 t.5
.O 2.1
< 20
< 60
<2
<2 05/27-06/24/06 1.3 i.5 8
2.1
< 20
< 50
<2
<3 06/24-07/29/00 3.7 1.9 9
2.1
< 20 C 50
<2 C 2 8
07/29-09/0USS 3.1 i.6 7
i.1
< 20
< 50
<2
<2 09/02-09/30/00 2.9 i.6 6
i.1
< 20
< 50
<2
<2 09/30-11/04/08 3.6 i.6 5
i.1
< 30
< 50
<2
<3 11/04-11/25/05 3.0 t.7 5
1.1
< 20
< 50
<2
<3 12/02-12/30/88 2.5 1.5
<.06 C 20 C 50
<2
<3 I
MEAN 2.6 1 1.5 60 1.46
< 22
< 51
<2
<3 trti 01/01-01/29/06 1.6 1.4 3
i.1
< 30
< 50
<2
<3 5
01/29-0U26/08 3.0 t.5
.7 i.1
< 2L
< 50
<2
<2 CU26-04/01/De 2.3 i.5 5
1.1
< 20
< 50
<2
<3 04/01-04/29/00 2.7 1.6 6
1.1
< 20
< 60
<2
<2 04/29-05/27/88 1.9 i.4 4.2 i.5 C 20
< 50
<2
<2 05/27-06/24/88 2.1 i.5 17 t.00
< 20
< 50
<2
<2 I
06/24-07/29/03 2.7 t.6 6
t.1
< 20
< 50
<2
< 2 07/29-09/02/05 3.5 i.6 4
i.1
< 20
< 50
<2
<3 09/02-09/30/00 2.8 1.5 5
2.1
< TO
< 50
<2
< 3 09/30-11/04/80 3.0 1.6 5
i.1
< 30
< 50
<3 C 3 11/04-1 UO 2/OS 2.7 i.5 7
1.1
< 20
< 50
<2
< 3 I
1 UC2-1 U30/08 2.0 2.5
.2 2.1
.< 20 90 2 60
<2
< 2 MEAN 2.5 i 1.1 60 1 2.18
< 22 54 1 23
<2
< 3 l
l (1) SEE PROGRAM EXCEPTIQ4S SECTION FOR EXPLMIATIQ4 I
I
_=
TABLE D.I.1 Ar4ALYTICAL DA1A FOR SURFACE HATER SAMPLES COLLECTED D4 THE VICD4ITY OF PDAPS,1988 RESULTS D4 LA4ITS OF PCI/ LITER i 2 SIGNA COLLECTIQ4 STATIQi DATE FE.59 CO.60 224 65 ZR-95 lB.95 CS.134
=
13A 01/30/88
<9
<3
. <6
<6
<4
<2 02/27/88 C 7 C 3 C6
<5 3
13 C2 04/0 uoB C 7
< 3 C6
<5 C3 C 2 (1) 04/30/88 05/28/88
<6
<3
<5
<4
<3 C2 06/26/08
<6
<3
<5 C5
<3
<2 07/30/08 C 6
<3
<5 C 4 C 2
<2 09/03/08
< 7 4 3
<6
< 5
< 3
<3 09/30/06
< 6
( 3
<6
< 5
< 3
<3 11/05/08
< 9
< 3
<6
< 6
<4 C 2 12/04/06
<7
< 3
<6
< 5 C 3
<2 t u31/08
< 7
< 3
<5 C5
< 3
<2 MEAN
< 7
<3
<6 C5 3
11
<2 130 01/29/06
< 9
< 3
<6
<6 4
i4
<2 Cu26/DS
< 10
< 3
<6
<7
< 7 C2 i
03/16/08 C 9
< 3 C6
<6
<5 C 2 04/20/08 C 10
< 3
<6
<6 C 5
< 2 05/26/06
< 6
< 3
<5
<4
<3
< 2 06/17/06
< B C 3
<6
<5
< 3
< 2 07/2uSB C 7
< 3
<5
<5
< 3
< 2 08/26/88
< 8
< 3 C6
<6 C4 C2 09/2 F08
< 7
< 3
<6
<5
<3
<2 10/28/08 C 9 4
13 C 6
<6
<4 C 2 11/18/88
< 9 C 3 C 6
<6
<4
<2 12/09/06
< 10
< 3
< 6
<6
<5
<2 MEAN
< 9 3
i1
<6
<6 4
12
< 2 1LL 01/01 01/29/85
< 9
< 3
< 6 C6 C4
<2 01/29 0U26/88
< 7 C 3
<5
<5
<3
<2 02/26 04/01/08
< 7
<3
<6
<5 C 3
<2 04/01 04/29/08
< 6
< 3
<5
<4
<3
< 2 04/29 05/27/88
< 6 C 3
<5
<4
<2
< 2 05/27 06/24/88
< 7
< 3 6
i6
<5
<3
<2 06/24 07/29/08
< 6
< 3
<6
<4
<3
<2 07/29 09/02/08
<6
< 3
<5
<4
<3
< 2 09/02 09/30/88
< 6
< 3
<6
<4 C3 C 2 09/30 11/04/08
<9
< 3
<6
<6 C4
< 2 11.'04 11/25/08
<7
< 3
<6
<5
<3
< 2 12/02 1 U30/06
< 7
< 3
<5
<4 C 3 C2 NEAN
<7
< 3 6
11
<5
<3
<2 1tti 01/01-01/29/68
< 9
< 3 C 6 C6 C 5 C 2 01/29 0u26/08 C 7 C 3
< 5
<5
< 3
< 2 02/26 04/01/88
< 7
< 3
< 6 C5
< 3
< 2 04/01 04/29/88
< 6
< 3
<5
<4
< 3 C2 04/29 05/27/08
< 6
< 3 C 5
<4 C 2
< 2 05/27 06/24/88 C6 C 3
<6
<4
< 3
<2 06/24-07/29/08
< 6
< 3
<5
<4
< 3
< 2 07/29 09/02/08
<6 C 3
< 6 C4 C 3
< 2 09/02 09/30/88
<6 C 3 C6 C4
< 3
< 2 09/30-11/04/88
<8
< 3 C6
<6
<4
<2 11/04 1uouS8
<7
< 3
<6
<5 C 3
< 2 12/02 12/30/88 C6
< 1
<5
<4
< 3 C 2 NEAti C 7
< 3
<6 C5
< 2 (1) SEE PROGRAM EXCEPTIQtS SECTIQi FOR EXPLAt4ATIQ1 I
E
TABLE D.I.1 ANALYTICAL DATA POR SURF' ACE MATER' SAMPLES COLLECTE0 IN THE VICD4ITY OF PBAPS,1966 RESULTS IN LHITS OF PCI/ LITER i 2 SIGMA COLLECTION, STATION DATE CS.137 BA.140 LA-140 CE.141 RA-226, TW228
..............................................~......................................
13A-01/30/86 C 2' C 50
< 20
_ <7 6~.
15 C 7.
02/27/06 C 2
'< to
<5
<4 C5
<1
~04/02/60
<3 C 20
<7
.<5-C5
- C 7'
- 11) 04/30/06 05/26/06~
<3 C 10
<4 C4-C5 C7 06/26/06 C t
. < 20 c'5
<5 C5
<7 07/30/80'
<2.
< 10
<3
<4 6
1 5-
.09/03/30
< 3
, < 20
<5 C5 C6
'7
. t7
<7 09/30/06 C 3'
< 20
<5
<5 C5'
-. < 7_
11/05/86
< 3 C 50
<20-
<6
<5
- c. 7.
12/04/80-
<3
< 20
<7' C5-7 i5-
<7:
12/31/06 C3
< 20
~ <5 C4
<5 C7 MEAN
.c3
< 24
<8 C5 5
i1 7
t0 138.
C1/29/06
<3
< 50
< 10
<7
<5
<7 02/26/06
<2
< 200
< 50
< 10
<5
<7 03/10/08 C 3
< 60
< 20
<7 7
15-
<7 04/20/06
. <2
< 60
< 20 6
i7 C5 C 7.
'05/26/06
<3 C 10
<4 C4 e5 C7 06/17/06
'<3
. < 30 C 9' C5 C 5 6
i7 07/2Uoo-
<3
< 20
<7 C4
< 5 C7 08/26/08
< 3 C 40
< 10
<6
< 5'
<7 09/23/06
<3 C 20
< 7-
<5
< 5
<7 10/28/06
<3-
< 50
< 20
<7
< 5
<7 11/18/06 C3
' < 50
' < 10
<7
< 5 1 C7 12/09/80
<3
< 70-
< 20
<8 C5
-C7-MEAN
~<3
< 55 C 16 7
14 5
11 7
1 1.
1LL 01/01 01/29/08 C 3
< 60
< 20
<7 C5
' <7 01/29 0 u26/08 C 3 C 20
<6
<4
't5 C7
- OU26 04/01/88 3 13
< 20
<7
<5
<5 9
t7 04/01 04/29/06
< 2
< 10 C4
<4
<5 9-t7 04/29 05/27/85
<3
< 10
<3 C3
<5 C7 05/27 06/24/06
< 3 C 20
<5 C4 CS
<7 06/24 07/29/00
< 2
< 10 C 3 C4
<5 C7 07/29 09/02/06
<3
< 10 C4 C5 C7 09/02 09/30/8S
< 2
< 10
' <5 C4 C5 C7 09/30 11/04/86-
.< 2
< 50 -
< 10
<6 C5
<7 11/04 11/25/08-
< 3
< 20
<5-
<5
<5-14 i7 12/02 12/30/86 C2
< 10
<5 C4
<5 C 7 MEAN 3 11
< 21
<6
<5 C5 6
14 Itti 01/01 01/29/06 C2 C 60
< 20
<7 C5
<7 01/29 02/26/00
<2
< 20
<5
<4-
<5
<7 02/26 04/01/08 3 13 C 20
<7
<5
<5
<7 04/01 04/29/08
<3
< 10
<4 C4
<7 04/29 05/27/80
<3
< 10
<3 C4 C 5
<7 05/27 06/24/OS C 3 C 10
<4 C4
<5 C 7 06/24 07/29/88
<3
< 10
<3
<4
<5
< 7 07/29 09/02/08
<3
< 10
<4
<4 C5
<7 09/02 0?/30/68 C 3 C 10
<4 C4 6
15
.<7 i
09/30 11/04/80
< 3 C 50
< 10 C 7 C5
<7 1
11/04 12/02/06 C3
< 20 C8'
< 5
< 7 l:
12/02 12/30/06 C 2
< 10
<5 C4
<5 C7 MEAN 3 11
< 20
<6
<5 5
i1
<7 (1) SEE PROGRArt EXCEPTIONS SECTION FOR EXPLANATION 1
5 665766655675 6
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4-i TABLE D.III.1 CONCENTRATIONS OF CROSS i: ETA RADIOACTIVITY.3H AIR PARTICULATE
. SAMPLES COLLECTED D4 THE VICINITY OF PBAPS,1906 RESULTS IN LNITS OF E.3 PCI/CU.. METER t 2 SIGMA' HEEK-
^1Z
-4A 1 26-13-25 i3 2 46 14 39 24 3 21 14 15
't3
.4 27 14 23 13 5 21 14 20-14 6 25
'i4-25 - 14 7 33-14 7
13 6 16 13 20 14 9 24 1.3 26-23
,10 13 -
.1 4 -
.13 14-11.11 13 11 23
.12 13 14 15
-24 13 9
.14 6
14 14 13 13 13
.i3 15 6 13' 6
i3 16 17 13
.to i3 17 12-13 10
't3 to 6
't3 7
13 19 10 14 14 14 20
< 2.
<3 21 10-13 5
23 22 21 24 17: 14 23 12
't 4 0
14 P4 17 13 23 14-25 15-13 36 i6 26 (1)
(1) 27 21 14 (1) to 26 14
'12 16
- 29 12
-14 8
i4
- 30 24 13 31 14
'31 12 14 17 24 32 13 14 12
.24 33 17 13
.15 13 34 21 14 21 14 35 24 24 25 14 36 15 i4
-15' i4
.37 17 24 20 24 38 16 i4 14 14 39 34 15 26 24 40 (1),
6 13 41 17
.24 17 i4 42 16 14 20-i4 43 20 14 19 24 44 24' i4 20 14 45 16 14 14 i4 46 17 i4 24 14 47 11 14 10 24 46 22 24 17 23 49 27 25 23 14 50 90 14 to 14 51 32 14 31 14 l
52 22 t4 20 t4
'l MEAN 19 1 16 17 1 17 (1) SEE PROGRAM EXCEPTIQ43 SECTIG4 FOR EXPLANATIQ4 y
i
l I
TABLE D-III.2 CulCb,T".1"D4S OF GAtt% EMITTERS IN AIR PARTICULATE SAMPLES COLLECTED IN THE VICD4ITY OF PDAPS,1900 REMJLTS Di LHITS OF PCI/0). METERS i 2 SIR 1A STATIG4 COLLECTIQ4 CODE PERIOD BE-7 K.40 CS-134 CS-137 TH-226
....... ~.........
I 1Z JN4 80 90 t to C8
< 0.4
< 0.4 C 0.6 FEB 00 100 i 10
<8 C 0.4
< 0.5 C 0.6 MAR OS 90 1 20
< 10
< 0.0
< 0.6 2
22 APR 88 100 1 10 30 1 10
< 0.5
< 0.5
< 0.7 MAY 08 90 1 10
<0
< 0.5
< 0.5
< 0.6 I
JUH 88 120 1 20 11 1 10
< 0.6
< 0.5 C 0.7 JUL 88 140 2 20
< 10
< 0.7-
< 0.7
< 1 AUG OS 110 1 10
<7
< 0.4
< 0.4 C 0.7 SEP BS 90 1 20
< 10
< 0.5 C 0.5 C 0.6 I
OCT 88 00 2 20 30 i 10
< 0.4
< b.7
< 1 im OS 50 16 C 4
< 0.2
< 0.2 C 0.3 DEC 88 100 1 30 C 40
< 1
<1
< 1 MEAN 96 1 45 15 1 23 C 0.6 C 0.5 0.0 1 0.9 5
4A JAN 08 70 1 10
< 10
< 0.5 C 0.6
< 0.6 FEB 08 80 1 20
< 10
< 0.5
< 0.5
< 0.8 MAR 68 130 1 20
<9
< 0.6
< 0.6
< 0.9 I
APR OS 90 1 10
< 10
< 0.5
< 0.5
< 0.7 MAY OS 60 1 20
<9 C 0.6
< 0.5
< 0.7 JUH 80 160 2 30 590 1 60
< 1
< 1
< 2 JUL BS 110 1 20
< 20
< 0.9
< 0.7
< 1 AUG 88 100 1 20
<9
< 0.5
< 0.4
< 0.6 i
SEP 68 100 1 20
< 10
- c. 0.5
< 0.6
< 0.0 OCT 00 00 1 20
< 10
< 0.6
< 0.4
< 0.6 tW OS 65 19
< 10
< 0.4
< 0.4
< 0.5 DEC OS 100 1 20
< 30
< 1.0
< 1.0
< 1 MEAH 97 i 54 61 2 334 C 0.6
< 0.6
< 0.9 I
I I
I I
I I
l l
l i
1l1
!ll,
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0.
4 t333 3
1 A
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4.
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4 0000 0
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04 0000 0
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I 0060 A
60680 M
8608 A
0000 M
A A_
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CT. 5054 N
501 54 N
5054 M
5054 N
C EA 1 301 1 31 01 1 301 1 30t LD
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TABLE D-V.1
' C0t4CEffTRATIC'tS OF' GROSS BETA RADIOACTIVITY IN HELL NATER
>^
SAMPLES COLLLCTED IN THE VICINITY OF PBAPS.- 1966 i
RESULTS IN LNITS OF PCULITER i 2 SIGMA
-COLLECTION STATICH DATE:
GROSS BETA 1U OU21/06 1.6 1.4 04/30/86 1.4 i.4 06/26/06 1.3 i.5 '
10/01/06 1.1 i.4 MEAN -1.4 i'.4 1V.:
O U27/88
- 1. 3 - ' 1.4 04/30/66.
<.3 06/26/86 2.1 i.5 ~
10/01/08.1.3 1.5 MEAN 1.3 1 1.5 7
.CU27/68 1.8 i.4 04/30/00~ 2.1 i.4 06/26/06 3.4 1.6 09/30/08. 2.0 1.5 MEAN 2.3 11.5-40 0U27/06 1.9 i.4 04/30/06 3.4 t'.5~
06/26/85 2.7 1.5 09/30/06 2.8 i.5 MEAN 2.7 11.2.
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$ttt1ARY O? COLLECTIOf DATES FOR SAMPLES COLLECTED TABLE D-VI.1 l
IN THE VICINITY OF PDAPS,1966 AIR PARTICULATE HEEK lt OR Knt. COMP.
,1Z 4A 1
01/01-01/09/80 01/01-01/09/06 2
01/09-01/16/86 01/09-01/16/86 3
01/16-01/2V08 01/16-01/23/85
'4
'01/23-01/30/Ce 01/23-01/30/06 JAH Oo 01/01-01/30/06 01/01-01/30/06 5'
01/30-02/06/80 01/30-02/06/08' 6
0 UO6-0 U13/06 02/06-02/13/88 7
02/13-02/20/08 02/13-02/20/06 8
02/20-02/27/88 0U20-02/27/80 FEB 60 01/30-02/27/06 01/30-0 U27/86 9
0 U27-03/05/06 02/27-03/05/80 10 03/05-03/1 UO6 03/05-03/1 U66 11 03/12-03/19/80 03/12-03/19/06 12 03/19-03/26/80 03/19-03/26/08 MAR SS 0U27-03/26/06 0U27-03/26/06 13 03 '26-04/0UO8 03/26-04/02/06 14 04'02-04/09/85 04/02-04/09/06 15 04/09-04/16/80 D4/09-04/16/06 16 04/16-04/23/06 04/16-04/23/06
.17 04/23-04/30/05 04/23-04/30/06 APR 68 03/26-04/30/08 03/26-04/30/88 18.
04/30-05/07/00 04/30-05/07/00 19 05/07-05/14/88 05/07-05/14/08 20 05/14-05/21/86~05/14-05/21/06 21 05/21-05/28/08 05/21-05/20/06 MAY 08 04/30-05/28/80 04/30-05/28/80 22 05/26-06/04/06 05/28-06/04/06 23 06/04-06/10/06 06/04-06/10/08 24 06/10-06/16/06 06/10-06/10/06-25 06/16-06/26/88 06/18-06/26/00 26 AR4 06 05/26 06/26/06 05/26-06/26/06 27 07/02-07/09/88 to 07/09-07/16/06 07/12-07/16/06 29 07/16-07/2UO6 07/16-07/22/06 30 07/22-07/30/08 07/22-07/30/06 JUL 88' 07/02-07/30/06 07/12-07/30/08 31 07/30-06/06/80 07/30-05/06/80 32 08/06-06/12/06 08/06-00/12/00 33 08/12-08/20/80 00/12-00/20/88 34 03/20-08/27/S0 08/20-06/27/S6 35 08/27-09/03/08 08/27 09/03/06 AUG 80 07/30-09/03/00 07/30-09/03/05 36 09/03-09/10/80 09/03-09/10/06 37 09/10-09/17/88 09/10-09/17/68 30 09/17-09/23/OS 09/17-09/23/88 39 09/23-10/01/88 09/23-09/30/06 j
SEP BS 09/03-10/01/06 09/03-09/30/00 40 09/30-10/05/88 I
41 10/06-10/15/65 10/00-10/15/06 42 10/15-10/2 USS 10/15-10/2 U66 43 10/22-10/29/06 10/22-10/29/0S OCT OS 10/06-10/29/05 09/30-10/29/00 44 10/29-11/05/80 10/29-11/05/00 45 11/05-11/1 USS 11/05-11/1 USS 46 11/12-11/19/06 11/12-11/19/06 47 11/19-11/26/SS 11/19-11/26/06 48 11/26-1 U O4/08 11/26-12/04/00 IKN 08 10/29-12/04/08 10/29-12/04/0S 49 12/04-1 U10/60 12/04-1 U10/00 50 1 U10-12/17/68 12/10-1 U17/06 51 12/17-12/24/08 12/17-1 U24/85 52 1U24-1U31/OS 12/24-1U31/08 DEC 80 1 UO4-1 U31/08 1 UO4-1 U31/68
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SYN 0PSIS OF ANALYTICAL PROCEDURES I
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w APPENDIX E:. SYNOPSIS. OF ANALYTICAL PROCEDURES The following appendix is comprised of two sections: ~ Section I describes the col-lection methods used to obtain samples for the REMP, and Section 2 describes the methods and formulas used by Teledyne Isotopes and C1can Harbors to' obtain the sample activities.
[
l 1
Section 1: Collection Methods Surface and Drinking Water Samples Surface and drinking water samples are composited over a one-month period at four
' locations (ILL, IMM, 4L, and 61). Water is continuously sampled at each location and col-lected in large tanks. Two quarts of water are removed from the tank each week and put into a clean two-gallon polyethylene bottle to form a monthly composite. At locations 13A and 13B a monthly grab sample is obtained.
Well Water Samples Prior to collection of well water samples, the well pump is run for several minutes to flush the line. Two gallon grab samples are then collected from the building faucets.
This sampling method is utilized at all four sampling locations.
Air Particulate and Air Iodine Samples Air particulate samples are obtained using.a system consisting of a pump, a glass fiber filter with a 35-mm diameter orifice, and a running time meter to indicate the total period of operation. At those locations where airborne iodine was also sampled, a char-coal filter was mounted behind the glass fiber filter. The volume sampled for the period if determined from the known flow rate and the running time. At the end of each weekly air particulate collection period, the air sampling unit is. stopped. The filter is then removed from the. holder and replaced with a clean filter, and the air sampling unit is returned to operation.
Soil Samples
. Collection of soil samples is accomplished by obtaining 3-inch plugs of soil 4 to 6 inches deep from a 4 square foot area and mixing them in a plastic bag. Approximately 1000 grams of the composite is then placed in a plastic bottle.
Sediment Samples Sediment samples are collected by one of two methods, determined by the depth from which the sediment is obtained. In water greater than 4-feet deep, sediment is collected by either a Ponar or Ekman Grab with a surface area of 81 square inches. In shallow water (1-4 feet), sediment is collected by scooping up mud with a plastic two gallon bucket.
Milk Samples Milk samples are obtained by removing two gallons from the dairyman's bulk tank.
The sample from each location is therefore a composite of all the milk from the dairy herd (from 1 to 3 milkings). The milk is scooped from the agitated bulk tank and placed in new plastic containers.
Vegetation Samples Samples of approximately 500 grams of cut grass and wild greens are placed in l
polyethylene bags and sealed for shipment. Crops are collected when available and shipped in plastic bottles.
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I Fish Samples
.l Fish samples are collected via several methods at Conowingo Pond locations; canal g-fish are caught by net trapping. Fish at other locations are caught by seine or elec-g troshocking techniques.
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l Section 2: Analytical Methods and Calculations DETERMINATION OF ~ GROSS ALPHA AND/OR BETA ACTIVITY IN WATER SAMPLES (TOTAL SUSPENDED AND DISSOLVED FRACTION)
Teledyne Isotopes This describes' the process used to measure the radioactivity of ' water samples-without identifying the radioactive species present. No chemical separation techniques are involved.
For well water samples a 1-liter aliquot is evaporated almost to dryness and then transferred to a 2-inch stainless steel planchet.
- For surface and drinking water samples, one liter of the sample is filtered under vacuum through a 0.45 micron Millipore filter. This filter represents the insoluble por-tion of the sample. The filter is dried and mounted on a planchet. The filter which represents the soluble portion of the sample is evaporated on a hotplate, and the residue is transferred and dried on another planchet.
The planchets are counted for 50 minutes in a icw-background gas flow proportional counter. Calculation of activity includes a self-absorption correction for counter ef-ficiency based on the weight of residue on each planchet.
Calculation of Sample Activity or of the MDL
~#
t i/ ) " 2.22(v)(E) i 2.22( v)( E)
Net Activity Counting Error where:
N
= total counts from sample (counts) t
= counting time for sample (min)
= background rate of counter (cpm) 2.22
= dpm per pCi v
= volume in liters E
- efficiency of the counter 2
= multiple of counting error The MDL is defined as that value equal to the two sigma counting error of the result.
- Less than MDL is reported as the result when this value is greater than the measured result defined above.
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- Clean ' Harbors '
This'. describes the process used to measure the overall radioactivity of-water.-
samples 'without. identifying the radioactive species present. No chemical l separation tech-niques are involved.
t For well water samples, a 1 liter aliquot is evaporated almost to dryness-in a beaker and then transferred to a 2-inch ringed planchet. It is then evaporated to dryness
~and counted using a gas flow proportional counter.
y
'For surface and drinking water samples,' the samples are first filtered through mem--
brane filters of 0.45 micron mean pore size. The filtrate'is treated as above. The fil-
~
ter papers are transferred to o pre-weighed planchet, ignited using acetone and a flame,
- and then put into a muffle furnace for final ashing. The ash is then counted using a gas
' flow proportional counter.
Calculation of the Sample Activity and 2 Sigma Error C,
C,
' C,
- C' 2
b e
t.
T~K A T,8 T
hpdi)*
b i
( 2.22)( E)(v)
( 2.22)( E)(v)
Net Activity Counting Error where:
C,
= total gross sample counts (counts)
T,
= sample count time (min)
C
= total background count (counts) b T
= background count time (min) b E
= counting efficiency based on CS-137 or uranium for the weight of planchetted sample v
= aliquot size in liters 2.22
= dpm per pCi 2
= multiple of counting error The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this va?ue is greater than the net activity.
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DETERMINATION'OF TRITIUM BY GAS. COUNTING Teledyne Isotopes
- A 2 ml aliquot is oxidized and the hydrogen gas is' collected in' an activated char-coal trap. The hydrogen is then transferred into a previously evacuated one liter propor-tional counter.. Non-tritiated hydrogen and ultra-high purity methane is added and then-counted.- Backgrounds and standards are counted in the same gas mixture as the samples.
Calculation of the Sample Activity or the MDL:
3.234 x tug x 'V 3.234 x tug x V, 3
CPMG x Vs
[ CPMc - BKG ] i CPMG x Vs
+"
Net Activity Counting Error where:
tun
= the tritium units of the standard V
= volume of the standard used to calibrate 3
the efficiency of the detector (psia)
V
= volume of-the sample loaded into the -
s detector (psia)
CPMn
= the cpm activity of the standard of volume V CPM :
= the gross activity of the sample of volume.V a
and the detector background BKG
=.the background of the detector in cpm-3.234
= conversion factor changing TU to pCi/l 2
= multiple of the counting error oG
= standard deviation of the gross activity of the sample and the detector background, in epm eB
= standard deviation of the background, in epm The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this value is greater than the net activity.
l.
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[.
,r DETERMINATION OF TRITIUM IN WATER BY ELECTROLYTIC:
ENRICHMENT AND LIQUID SCINTILLATION COUNTING I
Teledyne Isotopes
~
A 60 ml aliquot is distilled and collected in an Erlenmeyer flask. Approximately 55 g of the distillate is transferred into an electrolytic enrichment cell. 'One.ml of 30%
- sodium hydroxide solution is added to the cell. The sample is electrolyzed in a 10 C cooling water bath until the volume is 3-4 mis. CO is bubbled through the solution to 2
neutralize the sodium hydroxide. The sample is transferred to a collecting bottle at.
-80 C and weighed. It is then transferred into a liquid scintillation vial and 20 mis of cocktail is added.' The sample is counted for 100 minutes in a liquid scintillation counter,-
Determination of the Enrichment Factor-Aliquots of a tritium standard solution have been enriched to different final
~
volumes to provide a graph of the enrichment factor versus the final volume.
final volume) (' observed dpm/ml)
Entschment Factor = ((initial volume) (standard dpm/ml)
Calculation of the Sample Activity or of the MDL for Tritium
'(M1 - 0
~2 Y
b (tJ
.t,
2 t)
Net pCi "
unit vol.
2.22( v)( EF)( E) i 2.22( v)( EF)( E)
Net Activity Counting Error where:
N
= total counts from sample (counts) t
= counting time for sample (min)
S
= backe;ound rate of counter (cpm) dpm 2.22 I
=g.
= initial volume (in liters) before enrichment v
EF
= enrichment factor E
- efficiency of the counter tritium 2
= multiples of counting error The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this value is greater than the net activity.
DETERMINATION OF URANIUM ' ACTIVITY IN WELL WATER SAMPLES Clean Harbors Uranium is separated and purified by passing an aliquot of sample through' an ion. ex-change column. After eluting from the resin and concentrating,' an aliquot is evaporated onto a platiunum dish and fused with a NaF/LIF pellet. The uranium activity is determined by fluorescence.
Calculation of Uranium Activity Result (pg/l)' = R x CF,
where:
R
= fluorometer reading CF
= calibration factor from standard curve.
[
l
F DETERMINATION OF GROSS BETA ACTIVITY IN AIR PARTICULATE SAMPLES Teledyne Isotopes This describes the process;used to measure 'the overall beta activity of air particu--
late filters without identifying the radioactive species present. No chemical separation techniques are involved. Each air particulate filter is placed directly on a 2-inch'
. stainless steel planchet. The planchets are then counted for' beta activity in a low-
' background gas flow proportional counter. Calculation of activity includes an empirical
- self-absorption correction curve which allows for the change in effective counting ef-
. ficiency caused by 'the residue mass. Self-absorption is not considered in the case of air particulate filters because of the impracticality of accurately weighing the deposit and because the penetration depth of the deposit into the filter is unknown.
~#
b Res u t i
( pCi/m ) " - ( 2.22)( v)( E)(.02832).
(2.22)( v)( E)(.02832)
Net Activity Counting Error
,where:
N
= total counts from sample (counts) t
= counting time for sample (min)
= background rate of counter (cpm) 2.22
= dpm perc pCi y
=. volume of sample analyzed in cubic feet calculated from the elapsed time meter E
- efficiency of the counter 2
= multiple of counting error
.02832
= conversion from cubic feet to cubic meters The' MDL is defined as that value equal to the two sigma counting error of the' result.
Less than MDL is reported as the result when this value is greater than the net. activity.
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Clean Harbors Each filter paper is placed in a 2-inch diameter planchet and counted using a gas
~ flow proportional counter.-
Calculation of Sample Activity and 2 Sigma Error:
C C,
C' 2
b b
Res utt K~K
% T,2 +
T' b
8 (pCi/m ) " (2.22)(v)(E)(.02832) i ( 2.22)( v)( E)(.02832)
Net Activity Counting Error where:
C,
= total gross sample counts (counts)
T,
= sample count time (min).
C
= total background count (counts) b T
= background count time (min)
I b
E
= counting efficiency based on CS-137 v
= sample volume in cubic feet calculated from the elapsed time meter readings and the flow rate
.02832
- conversion to cubic meters 2.22
= dpm per pCi 2'
= multiple of the counting error The MDL is defined as that wilue equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this.value is greater than the net activity.
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DETERMINATION OF GROSS -ALPHA AND GROSS BETA ACTIVIT1ES IN SOIL : AND SEDIMENT SAMPLES -'
Clean Harbors To perform the analyses on both sample types, a 10 gram aliquot of dried sample is acid leached. The leachings are filtered and the filtrate diluted to 10 ml. A 2-ml quantity is plancheted, evaporated and counted using a gas flow proportional counter.
Calculation of the Sample Activity and 2 Sigma Error:
C,.
C C,
C 2
b b
e I
7K
$ T,8 T'
b pdi g)t- " (2.22)(E)( A) I (2.22)(E)( A)
Net Activity Counting Error where:
C,
= total gross sample counts (counts)
T,.
= sample count time (min)~
C
= total background count' time (counts) b T-
= background count time (min).
b E.
= counting efficiency based on CS-137 or uranium for the weight of plancheted sample A-
= aliquot analyzed (grams) 2.22'
= dpm per pCi 2
= multiple of counting error The MDL is defined as ' hat value equal to the two sigma counting error of the result.
t Less than MDL is reported as the result when this value is greater than the net activity.
)
l I
(
DETERMINATION OF I-131 IN MILK AND WATER SAMPLES BY RADIOCHEMISTRY AND LIQUID PHASE BETA ANALYSIS Teledyne Isotopes The following describes the radiochemical method for determining I-131 ectivity in milk and water samples by coincidence counting in the liquid phase.
Four liters of sample are first equilibrated with stable iodide carrier. A batch treatment with anion exchange resin is used to remove iodide from the sample. The iodine is then stripped from the resin with sodium hypochloride, reduced with hydroxylamines hydrochloride, and extracted into carbon tetrachloride as free iodine. It is then back-extracted as iodide into sodium bisulfite solution.
The iodide sample solution is oxidized to the free state using NANO reagent and l
2 is extracted several times into a total of 15 ml of toluene. A 200 microliter aliquot is taken for determining chemical yield by spectrophotometer. The decolonizing agent, 2-methyl-2-buttne is added to the toluene-iodine solution to form an inert molecule and to minimize liquid scintillation quenching. A toluene-based liquid scintillation counting solution is added to the sample, which is then analyzed by a beta-gated gamma-coincidence counting system.
Calculation of the Sample Activity and 2 Sigma Error:
t hp#
i
.22(v)(y)(DF)(E)
Ci )"
2.22( v)( y)( DF)( E) 2 Net Activity Counting Error where:
N
= total counts from sample (counts) t
= counting time for sample (min)
= background rate of counter (cpm) 2.22
= dpm per pCi v
= volume of sample analyzed (liters) y
= chemical yield of the amount of sample counted DF
= decay factor from the collection to the midcount I
time (eM*"O E
= efficiency of the counter for I-131 2
= multiple of the counting error NOTE: Efficiency is determined by counting an I-131 standard. Consequently, the branching intensity (abundance) of the I-131 gamma does not appear in the above equation.
The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this value is greater than the net activity.
Clean Harbors Analysis for determination of I-131 activity is performed by initially adding iodide carrier to an aliquot of sample. The iodide is concentrated by stirring with ion exchange resin, and then purified by extraction into chloroform and back extraction. The iodide is precipitated as palladium iodide for counting in a low-background beta counter or a beta-gamma coincidence counter.
Calculation of the Sample Activity and 2 Sigma Error:
C C
C C
2 e
b b
Result K,q
$ T,y + 3 Tb (pCi/1) " (2.22)( A)(E)(y)(DF) i (2.22)( A)(E)(y)(DF)
Net Activity Counting Error where:
C,
= total gross sample counts (counts)
T,
- sample count time (min)
C
= total background counts (counts) b T
= background count time (min) b E
= counting efficiency for 1-131 A
= aliquot analyzed (liters) y
= decay factor from time of sampling to the midpoint of the sample count (eO **'I) 2.22
= dpm per pCi 2
= nultiple of the counting error The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this value is greater than the net activity.
l 1
l
I I
l DETERMINATION OF STRONTIUM ACTIVITY Clean Harbors A description of the analytical methods, beginning with milk samples, used for each sa.nple 1ype is presented, followed by the general formula used for calculation of the sample activities.
To a one liter aliquot of milk sample, strontium and cesiam carriers are added.
After cesium removal, the liquid is made basic and the strontium is precipitated as oxa-late. After filtration, the oxalate is muffled and then dissolved. The strontium is purified by several precipitations as the nitrate. Possible interfering nuclides are removed by an iron hydroxide and then a barrium chromate scavenge. The Y-90 is separated I
as the hydroxide and then precipitated as the oxalate for counting in a low-background beta counter. Prior to precipitation, a known aliquot is taken for determination of the strontium yield by atomic absorption.
An aliquot of vegetation sample is wet ashed, and then dry ashed. The ash is then I
acid leached, followed by precipitation of strontium as the carbonate. The carbonate precipitate is dissolved and strontium is purified by several precipitations as the nitrate. The procedure for analysis of milk samples is followed from this point. Fish samples are analyzed by the same procedure as that for vegetation samples.
An aliquot of soil sample is sieved, followed by the addition of strontium and cesium carriers. The sample is then leached with HCI, filtered and silicates r.re removed.
Cesium is then collected, and the supernate is removed for strontium analysis. Strontium is separated from the supernate as strcntium oxalate, which is removed by filtration and I
then muffled. This procedure for analysis of milk samples is followed from this point.
Calculation of the Sample Activity and 2 Sigma Error for Sr-89 Routine:
C Qy b.
y (pCi/ unit
- - - C
C*
h.P + b.3+P+P Result C.-C.
y by s
y t,
1, 3
v o I u m e " (2.22)(E,)( A)(DF,)(Y,)( ABS,) i (2.22)(E,)( A)(DF,)( Y,)( ABS,)
or mass)
Net Activity Counting Error I
I I
I
e where:
C,
= gross Sr-89 counts (counts) t,.
- strontium count time (min)
C
- background counts of strontium counter (counts) bs
't
= background count time of strontium counter (min) bs 2.22
= dpm per. pCi '
E,
= Sr-89 counting efficiency -
A
= aliquot (in unit volume or mass)
DF,
- decay factor for Sr-89 from the sample time to the midpoint of the strontium count time (g-4131eT(days))
Y,
- ABS,
= Sr-89 absorption factor = [(.00125)(W,)+1.05]
where:
W, = weight of SrCO3 2
= multiple of counting error C,. - net counts due to Sr-90 (dpm)
"C C '
, f
,by, (E,') ( ABS,')
y (E )(GF )(DF )(y,)
y y
y C. = net counts due to Y-90 (dpm) y "C
C
[y - t (E ') (IG )
y y
by,
(E )(GF )(DF )(Y )
y y
y y
where:
C
= gross yttrium counts (counts) y t
= yttrium count time (min) y C
- backvound counts of yttrium counter (counts) by t
= background count time of yttrium counter (min) by E
= yttrium counter efficiency y
E,'
= Sr-90 counting efficiency E'
= yttrium efficiency in strontium counter y
precipitate wt Y
= yttrium yield = carrier weight y
ABS,'
= Sr-90 absorption factor = [(.004)(W,)+1.12]
= decay factor for Y-90 from the time of separation to l
y the midpoint of the count time (e'#1880TIh "))
GF
= grow-in factor for Y-90 into the purified Sr-90 from the y
time of the hydroxide scavenge to the time of yttrium precipitation (1-e'#IU880D ""))
IG
- ingrowth factor for Y-90 into the strontium mount from y
the milk time to mid-count time (1-e-A10830T(hours))
Calculation of the Sample Activity and 2 Sigma Error for SR-9Q (ph/ unit by
". (2.22)(E )( A)(DF )(GF )(Y )('Y,) i (2.22)(E )( A)(DF )(GF )(Y )(y,) :
V,o ImEs y
y y
y y
y y
y Net Activity Counting Error where:
C
= gross yttrium counts y
t
= yttrium count time y
C
= background counts of yttrium counter by t
= bac50und count time of strium counter by 2.22
= dpm per pCi E
= yttrium counter. efficiency y
A
= aliquot (in unit volume or mass) precipitate wt Y
=. yttrium yield = carrier weight y
Y,
= multiple of counting error -
= decay factor for Y-90 from the time of separation to y
the midpoint of the count time (e-m1 asMoun))
GF
= grow-in factor for Y-90 into the purified Sr-90 from the y
time of the hydroxide scavenge to the time of yttrium precipitation (l-e*#I#N ""))
The MDL is defined as that value equal to the two sigma counting error of the result.-
Less than MDL is reported as the result when this value is greater than the measured result defined above, l
r 1
DETERMINATION OF STRONTIUM ACTIVITY IN MILK SAMPLES Teledyne Isotopes To determine strontium activity, stable strontium carrier is added to a one liter aliquot of the sample, followed by the addition of tri-chloroacetic acid (TCA) to produce a curd. The curd is separated by filtration and discarded. An oxalate precipitation is performed on the filtrate and the precipitate is ashed in a muffle furnace. The ash is then leached in hydrochloric acid. Calcium and strontium are precipitated as phosphates, collected by vacuum filtration, then dissolved in nitric acid. Strontium is precipitated as Sr(NO )2 repeatedly using 90%, then 70% nitic acid. A barium chromate scavenge and 3
an iron (ferric hydroxide) scavenge are then performed. Stable yttrium carrier is added and the sample is allowed to stand for five days or longer for yttrium ingrowth. The yt-trium oxalate is mounted on a nylon planchet and counted in a low level beta counter to infer Sr-90 activity. Sr-89 activity is determined by precipitating SrCO from the s
sample after yttrium separation. The precipitate is mounted on a nylon planchet and cov-8 ered with an 80 mg/cm aluminum absorber for low level beta counting.
Calculation of the Sample Activity and 2 Sigma Error for Sr-89:
+ B, + BA
--N' -B
-B 2g pdi)" ( 2.22)( V)( Y,)( DF,)( E,) + ( 2.22)( V)( Y,)( DF,)( E,)
Net Activity Counting Error where:
N,
= total counts from sample (counts) t,
= counting time for sample (minutes)
B,
= background rate of Sr-89 counter (cpm)
B
= background addition from Sr-90 and ingrowth of Y-90 (see calculation below)
A 2.22 = dpm per pCi V
= volume analyzed (liters)
Y,
= chemical yield of strontium DF, = decay factor for Sr-89 from the mid collection date to counting date
.01:14T(days))
E,
= efficiency of the Sr-89 counter
)
l l
l l
l
I I
Calculation of Background Addition (B ) from Sr-90 Activity and from the Ingrowth of Y-92 A
NY-By
' K " (E )(IF )(DF )(Y )
y y
y y
'W where:
K
= dpm of Sr-90 on the strontium mount' I
N
= total Sr-90 counts (counts) y t
= counting time (min) y i
B
- background rate of Y-90 counter (cpm) y E
= efficiency of counter for Y-90 y
Y
- chemical yield of yttrium y
- the decay factor for Y-90 from the ' milk" time y
to the mid-count time [e-ci ssamoun)J IF
- ingrowth factor for Y-90 from scavenge time to y
milking time (1-e-ci ssamoun))
B
= 0.016( K) + ( K)( EyAss)(IG )
3 y
where:
I K
= dpm of Sr-90 on the strontium mount E
= the efficiency of counting Y-90 through a yABS No. 6 absorber I
0.016
= the efficiency of measuring Sr-90 through a No. 6 absorber IG
= the ingrowth factor for Y-90 into the strontium y
mount from the milk time to the mid-count I
time (1-e-41ase@un))
Calculation of Sample Activity and 2 Sigma Error for Sr-92 1l-B
-B 2
Pi )"
(2.22)(V)(Y )(Y,)(DF )(IF )(E ) i (2.22)(V)(Y )(Y,)(DF )(IF )(E )
y y
y y
y y
y y
Net Activity Counting Error where:
I N
= total counts from yttrium counter (counts) y B
= background rate of yttrium counter (cpm) y I
I
I t
- counting time for sample (minutes) '
y 2.22
= dpm per pCi V
= volume analyzed (liters)
Y
- chemical yield of yttrium g.
y Y,
= chemical yield of strontium E
= decay factor of yttrium from the milking time y
to the mideount time (e-41083&Mhoun)]
IF
- ingrowth factor for Y-90 from scavenge time to y
milking time (1-e-Al 83eyhoun)]
E
= efficiency of yttrium counter y
The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when the value is greater than the measured result
=
defined above.
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DETERM' NATION OF GAMMA EMITTING RADIOISOTOPES Teledyne Isotopes Gamma emitting radioisotopes are determined with the use of a lithium drifted l
germanium (GeLi) and high purity germanium detectors with high resolution spectrometry in specific media; such as, air particulate filters, charcoal filters, milk and water. Each sample to be assayed is prepared and counted in standard geometries such as one liter I
wrap-around Marinelli containers, 300 ml or 150 ml bottles, or 2-inch filter paper source geometries.
I Samples are counted on large (>55 cc volume) GeLi detectors connected to Nuclear Data 6620 data acquisition and computation systems. All resultant spectra are stored on magnetic tape.
The analysis of each sample consists of calculating the specific activities of all detected radionuclides or the detection limits from a standard list of nuclides. The GeLi systems are calibrated for each standard geometry using certified radionuclides standards traceable to the National Bureau of Standards.
Calculation of the Sample Activity and 2 Sigma Error:
Net pCi/
- 0) - B )
2%)+B) g g
vol. or mass, 2.22(V)(E ))(BI)(DF ))(t).-
2.22(V)(E ))(B1)(DF ))(t) g g
g g
Net Activity Counting Error where:
N)
= area, in counts, of a special region containing a g
gamma emission of the nuclide of interest NOTE-If the detector exhibits a peak in this region when counting a blank (i.e.,
from natural background (BB)(t) is subtracted from N before using the above -
equation. BB is the count rate of the blank, cpm, in the background peak.
B)
= background counts in the region of interest, calculated g
by fitting a straight line across the region connecting h
the two adjacent region.
E t
= counting interval of sample, minutes 2.22
= dpm per pCi V
= volume or mass of sample analyzed I
E)
- efficiency of counter at the energy region of interest g
BI
= branching intensity of the nuclide at the gamma emission energy under consideration I
DF )
= decay factor for nuclide j from sample collection time g
to midpoint of the counting interval (e#*"))
2
= multiple of counting error The MDL is defined as that value equal to the two sigma counting error of the result.
Less than MDL is reported as the result when this value is greater than the measured I
result defined above.
I
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Clean Harbors The procedure for detection of gamma emitting radioisotopes generates high resolu-tion gamma spectra which are used for quantitative determination and identification.
Standard geometries have been established to maximize efficiency, for all sample types; primarily air particulate filters, water, vegetation, soil, sediment, and fish.
A description of the analytical methods, beginning with air particulate used for 5
each sample type is presented, followed by the general formula used for calculation of the WI sample activities.
Air particulate samples from each location are placed in a petri dish and counted on GeLi detectors connected to a multichannel analyzer and micro-computer. Spectra are stored first on floppy disk, then on magnetic tape.
Water samples are placed into the appropriate sized container, depending on the volume of sample available. The preferred volume is 3.5 liters. The samples are counted and spectra are stored as with air particulate samples.
Vegetation samples are packed tightly in a tared container and weighed. Samples that contain excess liquid due to preservatives or decomposition are drained before weigh-l ing, and then returned to the container for counting. Samples such as grass are air dryed W
to remove surface moisture before weighing and counting. Samples are counted and spectra stored as with air particulate samples.
Soil and sediment samples are dried prior to weighing. An aliquot of dried sample is placed in a marinelli beaker and counted and spectra stored as with air particule samples.
Fish samples from each location are placed into marinelli beakers for counting. The aliquot size may vary, depending on availability of sample, up to 4 liters. The samples are counted and spectra stored as for air particulate samples.
t E
E l.
E' l
1
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1 Calculation of the Sample Activity and 2 Sigma Error:
{P ) + B )] (M)(E ) (G)(.06)
[P ) - B )] (M)(E ))(G)(.06) 2g g
g g
g g
g i
( A)(T)[DF ))
( A)(T){DF )]
g g
where:
P)
= number of gross counts in peak channels g
for nuclide j B)
= number of background counts in peak channels l
g for nuclide j M
= relative GeLi efficiency (GeLi 1-1)
E)
= pCi/ cpm for nuclide j U
G
= geometry factor for deviation from I liter in volume A
= aliquot size in unit volume (varies according to I
sample type)
T
= time counted in kiloseconds c
.06
= conversion to minutes DF )
= decay factor for nuclide j from time of sampling g
to time of counting (eMd*"I) 2
= multiple of counting error The MDL is defined as that value equal to the two sigma counting error of the result.
I Less than MDL is reported as the result when this value is greater than the measured result defined above.
I 1
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I
.Il DETERMINATION OF Cs-134 AND Cs-137 ACTIVITY IN MILK SAMPLES Clean Harbors Cesium carrier is added to an aliquot of sample, which is ashed with acid, then i
muffled. The ash is extracted with acid, cesium is collected onto ammonium molyb-i diphosphate by stirring and the supernate is removed for other strontium analysis. The cesium is pur'ified as cesium cobaltinitrite and finally precipitated as the chloroplatinate for mounting and counting. The samples are then counted on a GeLi detec-tor connected to a multi-channel analyzer and micro-computer. Spectra are stored first on floppy disks then on magnetic tape.
The Cs-134 and Cs-137 are calculated using the 796 kev peak for Cs-134 and the 662 l
kev peak for Cs-137.
E Calculation of the Sample Activity and 2 Sigma Error:
[P ) - B )](M)(E ))(G)(.06) 2g {P ) + B )](M)(E )(G)(.06) g g
g g
g g
( A)(T)[DF )]
( A)(T)[DF )]
g g
where:
P)
= number of gross counts in peak channels g
for nuclide j B)
= number of background counts in peak channels g
for nuclide j M
= relative GeLi efficiency (GeLi !=1)
E)
= pCi/ cpm for nuclide j g
G
= geometry factor for deviation from I liter in volume g
A
= aliquot size in unit volume (varies according g
to sample type)
T
= time counted in kiloseconds
.06
= conversion to minutes DF )
= decay factor for nuclide j from time of sampling g
to time of counting (e#*"))
2
= multiple of counting error I
I I
I
ENVIRONMENTAL DOSIMETRY Teledyne Isotopes dosimeters are rectangular teflon wafers impregnated with 25%
CaSO,:Dy phosphor. They are annealed in a hot air oven prior to use and are inserted into black polyethylene pouches. The filled pouches are labelled and placed in rec-tangular holders which contain copper shielding to filter out low energy radiation. After exposure in the environment, four separate areas of the dosimeter are read in a Teledyne Isotopes model 8300 TLD reader. The dosimeter is then re-irradiated by a standardized Cs-137 source and the four areas are read again. Calculation of the environmental exposure is performed by computer, using the re-irradiation readings to determine the sensitivity of each area of the dosimeter. The reading of control dosimeters are subtracted to allow for transit dose and system background.
A.
For any given area of the dosimeter, the dose mR is calculated by the formula:
Dose = R ( #h8') - avcontrol where:
R
= initial reading of the area RR
= second reading of the area (after re-irradiation) redose
= re-irradiation dose in mR avcontrol
= average of control values calculated as explained below. If no controls are used, avcontrol = 0 and gross exposures result B.
Each area of each control is calculated by the formula-cdose = cr ( CT d $ )
err where:
cdose
= control area dose in mR cr
= initial reading of the control area crr
= second reading of the control area (after re-irradation) credose
= re-irradiation dose of the control dosimeter in mR The average of control values is then calculated from all four areas of all controls by the formula-4N Ecdose 2
avcontrol =
4N N
= total number of control dosimeters
}
B.
A I
C.
The average and standard deviation of the area readings for each dosimeter are calcu-lated by standard methods, gg)
D.
Using the criteria that if one standard deviation is greater than 10% of the average of the four readings and that if the value of one area is outside the range of 3 g
standard deviations of the average of the other three areas, then that area will be g
eliminated and the results will be based on the remaining areas.
I I
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E 4
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~. - - - -
r-
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QUALITY CONTROL 1
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APPENDIX F:
INTER-LABORATORY COMPARISON PROGRAM
.TI and CH participate'in the EPA Radiological Inter-laboratory comparison (cross check) Program.
This-participation includes analyses on various sample media as found in the Peach Bottom REMP.
This participation provides an objective measurement of analytical precision and accuracy.as well as a bias estimation of the results are obtained.
Examination of the data shows that the vast majority were within the EPA control limits.
Each case of exceeding the control limits was investigated.
There is no evidence to suggest systematic errors.
For CH the results.from participation in the EPA progata are the basis for continued certification by the Commonwealth of Massachusetts in radiological analysis.
1
)
)
I Table F-1 EPA Intercomparison Samples Clean F. arbors Analytical Service I
Page 1 of 18 Gross Alpha and Beta Sample No.
Sample Date Sample Tyne Gross Alpha Gross Beta 37158 1/22/88 Water (a) 4 10 4
9
,gg 1
2 Lab Avg.
4(1) 9(1)
EPA Known 4(5,9,0).
8(5,9,0)
EPA Gr. Avg.
4(2,0) 8(2,0) 8803216 3/18/88 Water (a) 6 8
5 10 I
h 10 Lab Avg.
6(1) 9(1)
EPA Known 6(5,9,0) 13(5,9,1)
EPA Gr. Avg.
6(2,0) 13(2,-1) 8803297 3/25/88 Air Filter (b) 60 65 I
(Note 1) 58 65 51 kh Lab Avg.
60(3) 65(1)
EPA Known 20(5,9,14) 50(5,9,5)
EPA Gr. Avg.
23(5,13) 53(6,4) 8804184 4/24/88 Water (a) 48 I
8804252 45 kl Lab Avg.
47(2)
EPA Known 46(11,19,0) i EPA Gr. Avg.
45(12,0) 8804204 4/24/88 Water (a) 65 I.
8804253 59 kh Lab Avg.
63(3)
EPA Known 57(5,9,2)
I EPA Gr. Avg.
58(6,2)
B I
I I
8 I
3 I,'
Table F-1 EPA Intercomparison Samples Clean Harbors Analytical Service l;
Page 2 of 18 g
Gross Alpha and Beta Samole No.
Samole Date Samole Tvoe Gross AIDha Gro.np Beta 8805233 5/20/88 Water (a) 7 13 7
12 Z.
10 Lab Avg.
7(0) 12(2)
EPA Known 11(5,9,-1) 11(5,9,0) g EPA Gr. Avg.
9(3 -1) 12(2,0) g 8807192 7/22/88 Vater (a) 14 5
l 14 5
11 A
E Lab Avg.
13(2) 5(0)
EPA Known 15(5,9,-1) 4(5,9,0) g EPA Gr. Avg.
12(3,0) 6(2,0) g 8808301 8/26/88 Air Filter (b) 9 1010 (Note 10) 8 970 2
1222 Lab Avg.
9(1) 990(20)
EPA Known 8(5,9,0) 29(5,9,334) g EPA Gr. Avg.
9(2,0) 29(4,331) g 8809241 9/23/88 Water (a) 7 10 9
12 2
12 Lab Avg.
8(1) 11(1)
EPA Known 8(5,9,0) 10(5,9,0)
EPA Gr. Avg.
8(2,0) 10(2,0) 8810192 10/18/88 Water (a) 43 ag 43
$.6 Lab Avg.
44(2)
EPA Known 41(10,17,1) l EPA Gr. Avg.
39(9,1)
W I
1 I
I
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I Table F-1 EPA Intercomparison Samples Clean Harbors Analytical Service
'I Page 3 of 18 Gross Alpha and Beta Sample No.
Sample Date Sample Tvoe Gror,s Aloha Gross Beta 8*10193 10/18/88 Water (a) 54 I
53 kl Lab Avg.
53(1)
EPA Known 54(5,9,0) 8811281 11/25/88 Water (a) 8 7
10 9
I 2
S Lab Avg.
9(1) 8(1)
EPA Known 9(5,9,0) 9(5,9,0) i EPA Gr. Avg.
9(2,0) 10(2,0)
Note: (a) pCi/l (b) pCi/ filter The parenthesis next to the " Lab Avg." is the experienced 1 SD, 1 determination. A parenthesis next to a lab result means that the 1 SD of the procedure is greater than the EPA decreed SD. The first number in the parenthesis I
after the " EPA Known" value is the EPA decreed 1 SD, 1 determination. The next value is 3 SD, 3 determinations, i.e.
the EPA control limit. A value in parenthesis next to the " EPA Gr. Avg." is the experienced 1 SD where it is significantly different from the EPA value.
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Table F-1 EPA Intercomparison Samples Clean Harbors Analytical Service Page 4 of 18 Gamma Sample No.
Sample Date Sample Tvoq
'l 8802093 2/5/88 Water (Note 2)
=
Nuclide (pCi/1) 72*
Nuclide (pci/1) 60*
3 Cs-137 82 Cp-50 64.
g 21 E
Lab Avg.
77*(5*)
Lab Avg.
60*(4*)
EPA Known 94(5,9,-6*)
EPA Known 69(5,9,3*)
l EPA Gr. Avg.
94(6,-6)
EPA Gr. Avg.
69(5,-4)
W>
Nuclide (pCi/1) 82*
Nuclide (pci/1) 49(50**)
2n-65 88 Rm106 88(52**)
21 42J52**)
Lab Avg.
81*(8*)
Lab Avg.
60(25)
~
EPA Known 94(9,16,-3*)
EPA Known 105(11,19,-7)
EPA Gr. Avg.
96(7.-4)
EPA Gr. Avg.
100(13,-7)
I Nuclide (pCi/1) 43*
Cs-134 60 E
Lab Avg.
53*(9*)
EPA Known 64(5,9,-4*)
EPA Gr. Avg.
61(5,-3)
I Note:
- - These values reflect our recalculated values not our reported values.
- - Two sigma standard deviations.
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I Table F-1 i
EPA Intercomparison Samples Clean Harbors Analytical Service Page 5 of 18 Gamma I
Sample No.
Samole Date Sample Tvon l
37164 1/29/88 Food (Note 8)
Nuclide (pci/kg) 91 Nuclide (pCi/kg) 90 I-131 106 Cs-137 103 I
lE 19.0 Lab Avg.
105(15)
Lab Avg.
98(7)
EPA Known 102(10,17,1)
EPA Known 91(5,9,2)
EPA Gr. Avg.
99(8,1)
EPA Gr. Avg.
91(7,2)
Nuclide (mg/kg) 1586 E-4Q 1563 I
16E Lab Avg.
1523(90)
EPA Kncwn 1230(62,107,8)
EPA Gr. Avg.
1218(122,9) 8803297 3/25/88 Air Filter Nuclide (pCi/ filter)
C s - 13 */
18 I
20 E
Lab Avg.
19(1)
I-EPA Known 16(5,9,1)
EPA Gr. Avg.
18(3,1) 8804204 4/24/88 Water 8804253
.l Nuclide (pC1/1) 52 Nuclide (pCi/1) 6 W
Co-60 54 Cs-134 7
11 1
Lab Avg.
52(2)
Lab Avg.
6(1)
I EPA Known 50(5,9,1)
EPA Known 7(5,9,0)
EPA Gr. Avg.
51(4,1)
EPA Gr. Avg.
7(2,0)
I Nuclide (pCi/1)
Cs-137 7
7 i
I Lab Avg.
7(1)
EPA Known 7(5,9,0)
EPA Gr. Avg.
8(2,0)
I
', %
- z
.~
o.
l-f Table F-1
,e EPA Intercomparison Samples.
g:
~
clean Harbors Analytical Service.
+
Page 6 of 18 Camma Samole No.
Samole Date
- Samole Tvoe 8806033 6/3/88 Water (Note 4).
'Nuclide-(pCi/1) 294 Nuclide (pCi/1) 15 Cr-51 249 Co-60 15 222
~11
. Lab Avg.
271(23)
Lab Avg.
15(0)
H EPA Known 302(30,52,-2)
EPA Known 15(5,9,0)
EPA Gr.' Avg.
205(32,-2)
EPA Gr. Avg.
16(2,0)
L.
V Nuclide-(pCi/1) 92 Nuclide (pci/1) 160 Zn-65
~
97 Ey.-l.0.J.
169 21 114 Lab Avg.
95(3)
Lab Avg.
161(8)
' EPA'Known 101(10,17,-1).
EPA Known 195(20,35,-3)
EPA Gr. Avg.
103(7 -1)
EPA Gr. Avg.
191(16,-3)
.Nuclide (pci/1) 15 Nuclide (pC1/1) 22 Cs-134
'15 Cs-137 25 16.
21 Lab Avg.
15(1)
Lab Avg.
23(2)
EPA Known 20(5,9,-2)
EPA Known 25(5,9,-1)~
EPA Gr. Avg.
19(2,-1)
EPA Gr. Avg.
26(3,-1)
- 8806257 6/24/88 Milk-Nuclide (pCi/1) 46 Nuclide (mg/1) 1537 Cs-137 54 E. _4.9 1615 i
4 il 153 1 Lab Avg.
52(6)
Lab Avg.
1606(65)
EPA Known 51(5,9,0)
EPA Known 1600(80,139,0) j EPA Gr. Avg.
52(4,0)
EPA Gr. Avg.
1589(138,0)
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I LI Table F-1 I
EPA Intercomparison Samples Clean Harbors Analytical Service Page 7 of 18 Gamma 1
l' Sample No.
Samole Date Samole Tyne 8808028 7/29/88 Food Nuclide(pCi/kg) 96 Nuclide(pCi/kg) 47 I-131 86 Cs-137 45 10]
g l
Lab Avg.
95(9)
Lab Avg.
45(3)
EPA Known 107(11,19,-2)
EPA Known 49(5,9,-2)
EPA Gr. Avg.
108(8,3)
EPA Gr. Avg.
48(3,-2)
Nuclide(mg/kg) 1258 I
K-40 1267 129.1 Lab Avg.
1243(34)
EPA Known 1240(62,107,0)
EPA Gr. Avg.
1225(50,1) 8808301 8/26/88 Air Filter Nuclide pCi/ filter 16 l
Cs-137 19 22 I
Lab Avg.
19(3)
EPA Known 12(5,9,2)
EPA Gr. Avg.
13(3,2)
I I
I I
I I
I a
L L
l Table F-1 EPA Intercomparison Samples clean' Harbors Analytical Service Page 8 of 18 Gamma Sample No.
Samole Date-Samole Tyne 8810082 10/07/88 Water (Note 11)
Nuclide (pCi/1) 186 Nuclide(pci/1 22 Cr-51 201 Co-60 22 122 21 Lab Avg.
195(8)
Lab Avg.
23(2)
EPA Known 251(25,43,-4)
EPA Known 25(5,9,-1)
EPA Gr. Avg.
249(24,-4)
EPA Gr. Avg.
26(2,-1)
Nuclide (pC1/1) 135 Nuclide (pCi/l) 113 Zn-65 132 Ru-106 104 1M D1 Lab Avg.
134(2)
Lab Avg.
116(14)
EPA Known 151(15,26,-2)
EPA Known 152(15,26,-4)
EPA Gr. Avg.
152(9,-2)
EPA Gr. Avg.
144(18,-3)
Nuclide (pci/1) 20 Nuclide (pci/1) 12 Cs-134 2C Cs 137 13 20 14 Lab Avg.
20(0)
Lab Avg.
13(1)
EPA Known 25(5,9,-2)
EPA Known 15(5.9,-1)
EPA Gr. Avg.
24(2,-1)
EPA Gr. Avg.
16(2,-l)
I
{
l
{
5('
y.-
Table F-1.
EPA ~Intercomparison Samples Clean Harbors Analytical Service Page~ 9 of.18 Gamma.
. Sample No.
Sample Date-Sample Type 8810193 10/18/88 Water NuclidA(pci/1)-
13 Nuclide(pCi/1) 13 Cs-134' 11 Cs-137 13 11
- 14. '
Lab Avg.
12(1)
Lab. Avg.
13(1)
EPA Known, 15(5,9,-1)
EPA Known 15(5,9,-1)
EPA Gr. Avg.
- 14'( 2, - 1)
EPA Gr. Avg.
. 16(2,-1)
. 8810261-10/28/88-M11*n
'(Note'15)
Nuclide(pci/1) 40 Nuclide(ag/1) 1610-
- Cs-137 42 E-4_Q 1510.-
44' 1692 Lab Avg.
42(2)-
Lab Avg.
1570(60)
EPA Known 50(5,9,-3)
EPA Known 1600(80,140,-1)
EPA Gr. Avg.
S0(4,-3)
EPA Gr. Avg.
'1620(100,-1).
I-L j
u
I Table F-1 EPA Intercomparison Samples Clean Harbors Analytical Service Page 10 of 18 I-131 (pCi/1)
Samole No.
Sample Date Samole Tvoe I-131 8802312 2/26/88 Milk 4
Lab Avg.
4(0)-
EPA Known' 4(0,1,0)
EPA Gr. Avg.
4(1,-1) 8804070 3/8/88 Water 8-9 2
Lab Avg.
9(1)
EPA Known 8(1,2,3)
EPA Gr. Avg.
8(1,3) 8806257 6/24/88 Milk 107 (Note 5) 106 106 Lab Avg.
106(1)
EPA Known 94(9,16,2) i EPA Gr. Avg.
96(9,2) 8808087 8/05/88 Water 83-(Note 12) 88 R1 Lab Avg.
85(3)
EPA Known 76(8,14,2)
EPA Gr. Avg.
77(8,2) 8810261 10/28/88 Milk 66 (Note 16) 69 l
12 Lab Avg.
66(4)
EPA Known 91(9,16,-5) i l
EPA Gr. Avg.
90(8,-5) 8812089 12/09/88 Water 97 (Note 17) 91 l
El Lab Avg.
91(6)
EPA Known 115(12,21,-3)
EPA Gr. Avg.
116(14,-3) i
= _ - _ - - _,
i Table F-1
-EPA Intercomparison Samples Clean Harbors Analytical Service'.
Psgs 11 of 18
'Ra 226 and Ra-228(pCi/1)'
Samole No.
@ ele Date Samole T g Ra-226
'Ra-228-
- 8803127 '
3/11/88 Cater-6.0 9. '6 4.1 7.6 M.
M Lab Avg'.
6.1(2.0).
8.5(1.0).
EPA Known 7.6(1,1,2.0,2.3).
7. 7 (l'. 2,2. 0.1. 2 )
- EPA Gr. Avg.
7.2(1.1,-1.7) 7.6(1;7,124) 8804184 4/24/88 Water 3.0 3.9 8804252
.3. 9 4.2 (Note 6)
M M-Lab Avg.
3.7( 6) 4.5(.7)~
-EPA Known 6.4(1.0,1.7,-4.9) 5.6(.8,1.5, 2.3)-
EPA Gr. Avg.
6.0(.9,-4.2) 5.7(1.2,-2.5)
~8806194 6/17/88 Water 11.2 14.6' (Note 7) 10.1 17.5 M
1M Lab Avg.
-10.3(.8) 14.7(2.8)
EPA Known 10.0(1.5,2.6,.4) 12.4(1.9,3.2,2.1)
EPA Gr. Avg.
9.8(1.5,.6) 11.6(2.3,2.9) 8809178.
9/16/88 Water 4.5 8.1 (Note 13) 4.5 14.6 4.9 M
Lab Avg.
4.6(.2) 12.2(3.6)
EPA Known 8.4(1.3,2.3,-5.0) 5.4(.8,1.4,14.8).
EPA Gr. Avg.
7.8(1.4,-4.2) 5.6(1.2,14.2) 8810192 10/18/88 Water 4.2 2.9
-(Note 18) 3.3 2.9 M
M Lab Avg.
.'3. 8 (. 5) 2.9(0.0)
EPA Known 5.0(.8,1.4,-2.7) 5.2(.8,1.4,-5.0)
EPA Gr. Avg.
4.9(.5,-2.4) 5.3(.9,-5.3) 1[
8812143 12/16/88 Water 2.0 13.1
-(Note 19) 1.6 14.1 l.J 1M Lab Avg.
1.6(.4) 14.4(1.4)
EPA Known 3.5(.9,1.6) 10.3(2.6,4.5)
\\
l
Table F-1 EPA Intercomparison Samples Clean Harbors Analytical Service Page 12 of 18 Sr-89 and Sr-90 Sample No.
Sample Date Sample Type Sr-89 Sr-90 37164 1/29/88 Food (c) 52 53 (Note 8) 38 60 si ll Lab Avg.
45(5) 50(12)
EPA Known 46(5,9,0) 55(3,5,-3)
EPA Gr. Avg.
42(12,1) 5?(6,-2) 8801055 1/8/88 Water (a) 33 13 36 15 22 11 Lab Avg.
36(3) 14(1)
EPA Known 30(5,9,2) 15(2,3,-1)
EPA Gr. Avg.
28(6,3) 14(2,0) 8803297 3/25/88 Air Filter (b) 23 (Note 9) 16 21 Lab Avg.
21(5)
EPA Known 17(2,3,5)
EPA Gr. Avg.
17(2,5) 8804204 4/24/88 Water (a) 6 5
8804253 5
6 s
i Lab Avg.
5(1) 6(1)
EPA Known 5(5,9,0) 5(2,3,1)
EPA Gr. Avg.
6(2,0) 5(1,1) 8805104 5/6/88 Water (a) 30 22 27 21 22 22 Lab Avg.
26(5) 22(1)
EPA Known 20(5,9,2) 20(2,3,2)
EPA Gr. Avg.
19(6,2) 18(4,4) 8806257 6/24/88 Milk (a) 39 62 I
(Note 3) 41 11 Lab Avg.
44(6) 64(2)
EPA Known 40(5,9,-1) 60(3,5,2)
EPA Gr. Avg.
34(12) 56(10)
I l
!L -
LI Table F-1
'!l EPA Intercomparison Samples e
Clean Harbors Analytical Service Page 13 of 18 Sr-89 and Sr-90 Samole No.
Sample Date Sample Tvoe Sr-89 Sr-90 l
8808028 7/29j@C Food (c) 45 36 m
(Note 14) 26 44 M
4.1 Lab Avg.
35(10) 42(6)
I EPA Known 33(5,9,1) 34(2,3,7)
EPA Gr. Avg.
26(11,3) 31(6,9) 8808301' 8/26/88 Air Filter (b) 7 a
Lab Avg.
7(1)
I EPA Known 8(2,3,-1)
EPA Gr. Avg.
8(2,-1)
I 8810193 10/18/88 Water (a) 14 13 (Note 20) 15 11 12 12 I
Lab Avg.
14(2) 12(1)
EPA Known 11(5,9,1) 10(2,3,2)
EPA Gr. Avg.
10(3,1) 9(1,3) 8810261 10/28/88 Milk (a) 69 77 (Note 21) 74 66 Il 12 I
Lab Avg.
73(3) 67(9)
EPA Known 40(5,9,11) 60(3,5,4)
EPA Gr. Avg.
32(12,14) 56(6,7)
I Note:
(a) pCi/1
.l (b) pCi/ filter W-(c) pCi/kg I-I I.
I I
I-Table F-1 EPA Intercomparison Samples Clean Harbors Analytical Service Page 14 of 18 Triitium Samole No.
Sample Date Sample Tyne Tritium (nCi/1) 8802152 2/12/88 Water 3430 3540 1Z19 Lab Avg.
3570(160)
EPA Known 3330(360,630,1)
EPA Gr. Avg.
3360(340,1) 8806108 6/10/88 Water 5100 4900 1QDOQ Lab Avg.
5000(100)
EPA Known 5570(560,960,-2)
EPA Gr. Avg.
5390(500,1) 8810142 10/14/88 Water 2080 2010 2.Q1Q Lab Avg.
2030(40)
EPA Known 2320(350,610,-1)
EPA Gr. Avg.
2320(240,-1)
{
I i
l
I
'I Table F-1 EPA Intercomparison Samples I
Clean Harbors Analytical Service Page 15 of 18 Uranium (pCi/1)
Samole No.
Sample Date Samole Type Uranium I
8804184 4/24/88 Water 3
8804252 3
1 Lab Avg.
3(0)
I EPA Known 6(6,10,0)
EPA Cr. Avg.
6(2,-1) 8810192 10/18/88 Water 5
I 1
ig Lab Avg.
5(0)
EPA Known 5(6,10,0) g EPA Cr. Avg.
6(2,0) lI lI ls I
I I
I 5
l I
I
EPA Intercomparison Samples Clean Harbors Analytical Service Page 16 of 18 NOTES
- 1. The air filter results were outside the acceptance criteria for alpha and beta.
The raw data was checked and recalculated' for the alpha and the beta finding all inputs correct.
The beta rerun shows data concurring with the original data.
The results for alpha and beta were outside the acceptance criteria for no apparent reason.
- 2. The water Geli (2/5/88) was outside the acceptance criteria for all the nuclides, however, when 8802093A was recalculated, only Cs-134, Cs-137 and Ru-106 were out of acceptance.
The Cs values were out for no apparent reason but the problem is not generic.
The Ru-106 values were consistant with each other and if included ( ) our error, would be within the EPA results.
- 3. Table Of Results Sr-89 Sr-90 1 5 60 3
EPA 40 CHAS Reported 103 45 CHAS Reported 119 50 CHAS Reported Not Reported 55 880625701AR 119 6
28.6 i.7 880625701B 103 1 4 28.3 i.7 880625701C 21 3
29 4 i.8 880625701D 39 1 11 62 1 2 Recalculated C 48 7
65 2
Sample 8806257-01C recalculated and 880625701D were acceptable results.
However, samples AR and B were not acceptable and review of the raw data, calculations and counting data indicated no problems.
- 4. Ru-106 was recalculated with the Ru 106 correction factor (See Note 11): 208 219 2.0 0Q 1.ab Avg.
209 19 **
Recalculated results are within two standard deviations of the EPA result.
(
i
- 5. The raw data, calculations and counting data indicated no problems.
- two sigma standard deviation
{
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I E
EPA Intercomparison Samples I
Clean Harbors Analytical Service Page 17 of 18 NOTES I
- 6. Ra-226 result was low in comparison with the true result.
The Ra-226 results will be watched for a trend in low spike recoveries.
The new data calculations and counting data for Ra-228 indicated no problems.
- 7. The raw data, calculations and counting data for Ra-228 indicated no problems.
Sr-90 had yield problems due to the sample typ.
R-40 was biased high
,l l
due to non-homogeneous sample.
A letter was sent to the EPA asking how jW best to deal with this type of sample, food.
3
- 9. Low Sr chemical yields appear to be responsible for reported Sr-90 values g
which were outside the acceptance criteria. A different type of filter from that used for contract samples was used which may have contributed to the low Sr yield.
ll
<W
- 10. The air filters were out for beta because of a problem with the dateflex calculation program. The program converted the aliquot for air particules
, g from ft3 3 which is correct for contract samples.
The program was to m g.
changed so that if the sample type is AP and aliquot - 1, then the aliquot will not be converted.
The air filters were recalculated on the old Apple beta program and on the corrected data flex program with the I
following results:
Apple 28.6 1.5 IBM 28.6 1.5 Basic 27.4 1.4 Data flex 27.4 i 1.4 28 2
28 2
11.
The water geli was out for Ru-106 and Cr-51.
Because Ru-106 has been consistently low, a DI spiked with Ru-106 was run.
From this result and I.
previous EPA results, a correction factor for Ru-106 was calculated.
Water geli (10-07-88) was recalculated using the Ru-106 correction tactor to give the following results:
I Nuclide 146 34 **
Ru-106 134 1 34 **
119 t.h **
Avg. - 150 37 I
Recalibration of the Geli is underway and Cr-51 is being investigated.
I
- two sigma standard deviation I
I I.
D&
-t k
- r EPA Intercomparison Samples L
Clean Harbors Analytical Service
.Page 18lof 18 NOTES ~
12.
I-131"was checked for error.-
Results were recalculated with new efficiencies 'from LLB calibration.
Recalculated results are within-two
, standard deviations of the EPA known.
'Nuclide (pCi/1) 70~
I-131 72 l.9 Avg. - 70 1 3 **
- two sigma standard deviation.
13.
The results were outside the' acceptance criteria for both Ra-226 and Ra-.
.228.
Review of counting data and calculations indicated no problem. An investigation into possible problems in chemistry is underway.
14.
Food results were outside the acceptance criteria for Sr-90.
A review of the -- raw data,. counting data, and calculations. indicated no problems -
other then possible non-homogeneity of this sample type.
15.
Cs-137 was checked for error.
A review:of'the counting data and calculations indicated no problems.
l'
. 16.
Low I-131 results are currently under investigation.
Calibration for I-l 131 on the low level beta counters will be rerun.
17.
Low I-131 results are currently under investigation..The calibration for I-131 on the low level beta counters will be rerun.
18 Ra-226 was checked for error. Review of raw data, counting data, and calculations indicated no problems. Ra-228 is outside the ' acceptance criteria. Raw data, counting data, and calculations were reviewed and no y
problems were found. Ra-228's will be counted for 900 minutes to improve the counting statistics.
l
- 19. Because of. computer problems at EPA, statistics for 8812143 are not available at this time.
I l:
20.
Check of raw data, counting data, and calculations indicated no problems.
')
- 21. Sr-89 ' and Sr-90 were outside the acceptance limits because of possible
{
problems in chemistry and' low Sr yields.
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PBAPS SURVEY I
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M APPENDIX G:
PBAPS SURVEYS A Land Use Census around the Peach Bottom Atomic Power Station (PBAPS) was conducted by RMC Environmental Services for Philadelphia Electric Company to comply with Section 3/4.8.E.2 of PBAPS's Technical Specifications.
The survey was conducted during the May to October 1988 growing season.
The results of this survey are summarized in Table ~G-1.
There were no changes required to the PBAPS REMP as a result of this. survey.
4 1
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e9 TABLE G-1 LOCATION OF THE NEAREST MILK FARM WITHIN A FIVE MILE RADIUS OF PBAPS, 1988 DISTANCE (FT.)
SECTOR
'FROM VENT N
18,500 NNE' 15,600 NE 11,200 ENE 14,000 E
19,700 ESE 17,000
^
SE.
24,700 SSE S
6,900 SSW 6,900 SW~
11,600 WSW 12,400 W
6,000 WNW 8,400 NW 17,900
'j NNW INDICATES NO MILK FARM LOCATED
_ _ = _ - _ _ _. = _ _ _ _. _ _ _ _. _ _ _ _ - - _ _ _ _ - _ _ _ - - _ -