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Forwards Confirmatory Surveys of Bldgs & Areas of Cintichem Facility Located in Tuxedo,Ny.Radionuclide Concentration in Bedrock Soil Samples & Orise Resrad Calculation,Encl
	ML20236S021
Person / Time
Site:	05000054, 07000687
Issue date:	06/02/1998
From:	Adams W; OAK RIDGE ASSOCIATED UNIVERSITIES
To:	Dragoun T; NRC OFFICE OF INSPECTION & ENFORCEMENT (IE REGION I)
Shared Package
ML20236S022	List: ML20236S021; ML20236S040; ML20236S052; ML20236S069; ML20236S081; ML20236S096;
References
	RFTA-96-17, NUDOCS 9807240086
	Download: ML20236S021 (31)
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/7 O ~ b Q Mr. Thomas Dragoun U.S. Nuclear Regulatory Commission Region I 475 AllendaleRoad KingofPrussia,PA 19406

SUBJECT:

ADDENDUM TO THE PHASE 5 CONFIRMATORY SURVEY REPORT-BEDROCK DOSE ASSESSMENT REPORT, CINTICHEM INCORPORATED, TUXEDO, NEW YORK (DOCKET NO.70-687; RFTA NO. 96-17)

Dear Mr. Dragoun:

The Cintichem facility, originally called the Union Carbide Nuclear Company (UCNC) Research Center, was originally designed and constructed to meet the joint needs of the Unien Carbide Nuclear and Ore Companies. The facility consisted primarily of a 5 MW pool-type reactor that was linked to a bank of five adjacent and intercell-conveyor-connected hot cells by a four-foot-wide by twelve-foot-deep water-filled canal. Shortly aAer going into operation, the facility operations expanded to provide various reactor based pmducts and services to a multitude of research, production, medical, and educational groups outside the Union Carbide organization.

In the late 1960's and early 1970's, the field of nuclear medicine grew and in 1978 the facility became the Medical Products Division of Union Carbide. Union Carbide operated the facility until 1985, when Cintichem, Inc., became owner under the parent company Medi-Physics, Inc.

The property was purchased in 1990 by the present parent company, Hoffmann-La Roche, Inc. In ;

1990, the facility shutdown because of two basic defects that rendered the plant functionally outmoded. Therefore, . it was determined that radiochemical processing operations be permanently terminated and decommissioning initiated (Cintichem 1996).

l The decommissioning projeet was divided into five phases by Cintichem. Phase 1 included the immediate exterior areas of Buildings 1 and 2 (HUT Excavation). Phase 2 included the l

decontamination and final status surveys of interior structural surfaces in the reactor building (Building 1), the tunnJ, and the pump room. Phase 3 included approximately 31 hectares (77 j acres) of unaffected land areas surrounding Buildings 1 and 2. Phase 4 included both affected i i

and unaffected land areas as well as concrete foundations associated with the exhaust stack. and an asphalt driveway and parking area. Phase 5 included the interior and exterior areas of the not laboratory building (Building 2), including the transfer canal, gamma pit, pit building, and the extemal shoring structures. This phase riso included land areas within and outside of the fonnerly fenced in Radiological Controlled Area (RCA), and the interior and exterior areas of the waste storage building, boiler house (Building 5), east and west butler buildings, and the 9907240086 980602 PDR I

ADOCK 05000054 [t iAx RioGE. itNNESLEE 378310117 W

PM Monos.d and operoi.d by ook u.og. Anocioe.d univ.,ui for ih. u s. o.porem.n, of En.,gy h i(l{ ;

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engineering builiEng (B6ilding 3).LORISE submitted the draft report for the Phase 5 survey activities on March 11,1998 (ORISE 1998).

l During the characterization of the site, Cintichem detected the presence of residual concentrations of contammation within fissures and interstitial spaces of the . site bedrock.

Because of the configuration of the material within the bedrock matrix and due to the high cost of remediation and the fact that remediation efforts would undermine the integrity of the hill (Sterling Mountain), Cintichem petitioned the NRC for a dose-based volumetric criteria.

Therefore, the results of the bedrock characterization and the final survey data for soil were used by Cintichem to estimate the potential radiation doses that would result from three possible future site scenarios (on-site industrial intmder, off-site residential occupant, and on-site residential occupant). Cintichem perfomied a dose assessment using a RESRAD computer code and provided the results to the NRC for review (Cintichem 1997).

At the request of the U.S. Nuclear Regulatory Commission (NRC), Region I Office, the Environmental Survey and Site Assessment Program (ESSAP) of the Oak Ridge Institute for Science and Education (ORISE) was tasked with performing a separate dose assessment and analyzing 20 soil samples for the Bedrock Area. ORISE performed independent confirmatory analyses of bedrock soil sanples as provided to ORISE by the licensee. ORISE also performed a confirmatory dose assessment using the RESRAD Version 5.782 computer code for the Bedrock Area.

CONFIRMATORY ANALYSIS OF BEDROCK SAMPLES Cintichem employees submitted a total of 20 soil samples from the Bedrock Area to ORISE for confirmatory analysis. ORISE was tasked to analyze the samples by solid-state gamma spectroscopy for Sb-125, Co-60, Ag-110m, Cs-134, Cs-137, Ce-144, and Eu-152 and compare the results with the licensee's analytical laboratory contractor, Teledyne.

The bedrock soil sample results are provided in Table 1. Confirmatory radionuclides soil concentrations were less than 0.1 pCi/g for Sb-125, less than 4.5 pCi/g for Ag-110m, less than 0.2 pCi/g for Eu-152, less than 0.5 pCi/g for Cs-134, less than 0.8 pCi/g for Ag-110m, less than 0.2 to 1.9 pCi/g for Cs-137, and less than 0.3 pCi/g for Co-60.

Cintichem's analytical results for the same soil samples, as provided in the Bedrock Dose Assessment Report, are all in relative agreement with the ORISE results, which indicate that radionuclides concentration's were mainly below the lower limit of detection for the analyses.

BEDROCK DOSE ASSESSMENT The Bedrock Dose Assessment inchided a review of the bedrock data and the licensee's l RESRAD Version 5.0 calculations. ORISE performed a separate RESRAD calculation and the results are included as Attachment A. All RESRAD settings were left as the default settings (which are based on either the national average or reasonable maximum values for a subsistence Cintichem ine.. Tuxedo, NY (693)- June 2.1998 2 essapuettenwngoun.021. doc i

farmer scenario) with the exception of those listed below-which ORISE derived from the Cintichem bedrock data (Cintichem 1997).

2 Area ofcontaminated zone (m ) = 4.057E+04 (total bedrock area)

Thickness ofcontaminated zone (m) = 3.100E-01 ..

Length parallel to aquifer flow (m) = 2.000E+02 Basic radiation dose limit (mrem /yr) = 2.500E+01 Initial principle radionuclides (pCi/g): Ag-108m = 1.238E-02 Initial principle radionuclides (pCi/g): Ce-144 = 7.200E-04 initial principle radionuclides (pCi/g): Co-60 = 7.290E-03 Initial principle radionuclides (pCi/g): Cs-134 = 7.410E-03 ,

Initial principle radionuclides (pCi/g): Cs-137 = 5.584E-01 I I

Initial principle radionuclides (pCi/g): Sb-125 = 3.560E-03 Initial principle radionuclides (pCi/g): Sr-90 = 2.539E-01 (Note: All based on the average concentrations for the five zones as reported by the i licensee (Cintichem 1997)] j Density of contaminated zone (g/cm') = 2.500E+00 Density of saturated zone (g/cm') = 2.500E+00

[ Note: Data reported by the licensee (Cintichem 1997)]

Summarv of Pathway Selections j The following pathways were active: extemal gamma, inhalation (w/o radon), plant ingestion, meat ingestion, milk ingestion, aquatic foods, drinking water, and soil ingestion. The radon i pathway was suppressed.

Total Dos 2 Comparisons

ORISE could not duplicate the licensee's RESRAD input parameters as this specific information l

was not provided in the licensee's report and due to modifications to the RESRAD code itself.

l Therefore, ORISE elected to take a conservative approach and used all the parameters. The maximum total dose with the initial soil concentrations as provided by Cintichem was 1.98 l

I mrem /yr at t = 0 years for all radionuclides-with Cs-137 being the major contributor to the dose (Refer to Attachment A, Pages 9 and 10),

time (vearsi

ORISE Dose (mrem /vr) 0 1.98 1 1.829 3 1.738 10 1.337 30 0.7357 100 0.1171 300 2.743E-04 1000 2.172E-12 3 essap\ letters \draroun 021 doc Cmtichem Inc.. Tuxedo, NY (693) - June 2.1998

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The ORISE results indicated that the primary exposure pathway is from direct radiation at 1.297 mrem / year (Refer to Attachment A, Page 10). The maximum groundwater pathway dose from drinking water was 1.93 E-2 mrem / year for all nuclides-with Ag-108m being the major contributor to the dom (Refer to Attachment A, Page 12 and Attachment B).

.. 1 The results of the ORISE RESRAD calculations indicate that the total dose levels that would result from the remaining radionuclides site inventory would be significantly below 25 mrem / year, i The ORISE RESRAD maximum dose results of 1.98 mrem / year compares favorably with the Cintichem RESRAD maximum dose results of 1.46 mrem / year. Therefore, both RESRAD calculations were well below the NRC/NYS DEC annual dose limit of 10 mrem / year (Cintichem 1997).

Please contact me at (423) 576-0065, Tim Vitkus at (423) 576-5073, or Eric Abelquist at (423) 576-3740 should you have any questions.

Sincerely, tJA ch Wade C. Adams Project Leader / Health Physicist Environmental Survey and Site Assessment Program WCA:dkh Enclosure cc: R. Uleck, NRC/NMSS/rWFN 7F27 J. IIalvorsen, NRC/NMSS/TWFN 8A23 W. Beck, ORISE/ESSAP E. Abelquist,ORISE/ESSAP T. Vitkus, ORISE/ESSAP D. Quayle, ORISE/ESSAP File /693 i

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' Cintichem ine.. Tuxedo. NY (693) . June 2,1998 4 essap\lettersidragoun 021. doc _

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REFERENCES Cintichem, Inc., (Cintichem). Final Status Survey Plan and Report. Cintichem, Inc., Tuxedo, New York; April 1996.

Cintichem,_ Inc. Bedrock Dose Assessment Report. Cintichem, Inc., -Tuxedo, New York; September 1997.

- Oak Ridge Institute for Science and Education (ORISE). Draft Report - Confumatory Survey for the Phase 5 Areas, Cintichem, Incorporated, Tuxedo, New York. Oak Ridge, Tennessee;

' March 11,1998.

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SUBJECT:

Dear Mr. Dragoun:

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