ML20042A808

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Environ Rept 31,Jul-Dec 1981.
ML20042A808
Person / Time
Site: West Valley Demonstration Project
Issue date: 02/25/1982
From: Smokowksi R, Wilcox D
NUCLEAR FUEL SERVICES, INC.
To:
Shared Package
ML20042A806 List:
References
NUDOCS 8203240118
Download: ML20042A808 (26)


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) NUCLEAR FUEL SERVICES, INC.

1 West Valley, New York ENVIRONMENTAL REPORT NO. 31 i July - December 1981 ,

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D. P. Wilcox 4 'R. T. Smokowski i

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i i-TABLE OF CONTENTS _

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! 1.0 - INTRODUCTION . ..... . . . . . . . ... . . 1 i

2.0

SUMMARY

OF-RESULTS . . . . . . . . . . . . 6 i

3.0 LIQUID EFFLUEllTS - . . . . . . . . . . . . . . 7 1

I i 4.0 GASE0US EFFLUEllTS . . . . . . . . . . . . 12

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! 5.0 ENVIRONMEllTAL MEASUREMEllTS . . .-. . . . 15 4

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LIST OF TABLES AND FIGURES Paae Table 1-1 NFS Environmental Sampling Prooram Western New York Nuclear Services Center . . . . . . . . 3-4 Figure 1-1 Location of the Fixed Environmental Samplina Stations of Western New York Nuclear Service Center . . . . . . . . 5 Table 3-1 Liquid Discharges (Monthly Composite Data) . . . . . . . . 9 Table 3-2 Liquid Discharges (Quarterly Composite Data) . . . . . . . 10 Table 3-3 Buttermil k Creek Silt Activity . . . . . . . . . . . . . . 10 Table 3-4 Buttermilk Creek Water Activity ............. 11 Table 4-1 Gaseous Activity Released from Plant Stack . . . . . . . . 13 Table 4-2 Gaseous Activity Released from Plant Stack (Quarterly Composite Data) . . . . . . . . . . . . . . . . 14 Table 5-1 Perimeter Air Activi ty . . . . . . . . . . . . . . . . . . 17 Table 5-2 Monthly Accrued Background Near Site Perimeter . . . . . . 18 Table 5-3 Radioactivity in Cattaraugus Creek (Weekly Samples) ... 19 Table 5-4 Radioactivity in Cattaraugus Creek (Monthly Composites) . 20 Table 5-5 Fish Samples from Cattaraugus Creek (3rd Quarter 1981) . . 21 Table 5-6 Deer Sampl e Da ta . . . . . . . . . . . . . . . . . . . . . 22 Table 5-7 Mil k Sampl e Data . . . . . . . . . . . . . . . . . . . . . 23 l

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' 1.0 INTRODUCTI0ft .'

The Nuclear Fuel Services, Inc. spent fuel reprocessing plant is located at the Western New York Nuclear Service Center, a 3,345-acre site located cpproximately 30 ' miles southeast of Buffalo in Cattaraugus County in western New York. , ,

s The purpose of th'is plant was to recover the reusable uranium and

plutonium contained in spent nuclear power plant fuels. This recovery
  1. was accomplished by the mechanical separati6n of the fuel materials 7, y from their associated hardware, followed by the chemical. separation of

, the uranium and plutonium from the associate 1 fission product elements-l

' in the fuel materials. The recovered uranium and pihtonium was shipped

/off site. Reprocessing operations were suspended' March,1972. The

t , plant is maintained in a safe shutdown condition. ' ' \

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,i' Since the plant startup in 1966, monitoring of the environment by:

, NFS and cognizant government agencies ,has shown that ex9c ures to radiation of the gener.al. population in the vicinity of the plant-are f

not significantly different from those received in other portions of the state. The exposure levels that'do exist in the aretc are attributed

? + to natural background radiation and northern hemisphere falloit from

) past weapons testing. a

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s Nuclear Fuel Services mai'n tains an extensive environmental pr nram to assesss the imact of the reprocessing plant on the surroundino 4 '

environreent. This is' augmented by comoletely indeperdent environment'alJ a w

,i monitoring prograns carried out on a. routine basis by the New York State Department of Environmental Conservation.

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The NFS environmental monitoring prog',am provides a measure of tihcdrrentenvironmentalbackground'~surroundinpthereprocessing

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plant. Samples collected at points where r:ncentrations of effluents

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in the environment are expected 'to he the greatest are compared, where a possible,withsamplescollectedatpointsunaffectedbyplantoperationsj

[ t The latter samples provide background measurements as a basis for

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distinguishing radioactivity introduced into the environment by the operation of the plant from that due to other sources. The samplina schedule assures that potentially significant changes in the environ-mental radioactivity are sampled most frequently. Those which are less affected by transient changes but may show long-term accumulations are sampled less frequently.

The NFS environment program at the Service Center began in July, 1963 with a preoperational monitoring program of the background gross alpha, beta and gamma activity at and near the Center. This program has since been extensively expanded to obtain the most significant data. The present UFS environmental program outlined in Table 1-1 provides for over 1,000 analyses per year. The location of the fixed sampling stations operated by NFS at the Center are shown in Figure 1-1.

9 Table 1-1 -.

f4FS EtNIRONMENTAL SA*4PLING PROGRAM .

WESTERN NEW YORK NUCLEAR SERVICE CENTER Sample Location Sample Type Sample Frecuency Analysis Buttemilk Creek (at Silt Quarterly Gross Alpha, Gross Beta, Gamma Scan Thomas Corners Bridge)

Water Quarterly Gross Alpha, Gross Beta, H-3 Cattaraugus Creek 9 Fish Second, Third Otrs Flesh of each for Cs-134, Cs-137, Sr-90 (between Buttermilk (6" Long) Skeleton of each for Sr-90 Creek & Springville Dam)

Cattaraugus Creek Water Weekly Gross Alpha, Gross Beta, H-3 (Felton Bridge)

Water Monthly Composite Gross Alpha, Gross Beta, Sr-90, *I-129 Flow Monthly Flow in Creek for Month b Plant Liquid Water Daily when Gross Alpha, Gross Beta, H-3, Cs-134, Effluent Discharging Lagoon Cs-137 Water Monthly Composite Gross Alpha, Gross Beta, H-3, Sr-90 Ru- 106, Rh-106, I-129 Cs-134, Cs-137 Water Quarterly Composite U Isotopic, Pu Isotopic Flow Monthly Discharge Volume for Month On-site, North of Deer Once/ Year (Fall) Flesh Cs-137, Cs-134, Sr-90 Plant Skeleton Sr-89, Sr-90 Perimeter Farms Milk August I-129, Sr-90, Cs-134, Cs-137 Northeast & Northwest c

Table 1-1 (Contd.)

Sample location Samole Type Samole Frecuency Analysis Perimeter Stations Air Continuous Sample Gross Alpha, Gross Beta Analyzed Weekly Direct Radiation Monthly Millirat. per Standard Month Gaseous Effluent Air Continuous Sample Gross Alpha, Gross Beta

. Analyzed Weekly Continuous Sample I-129 Analyzed Quarterly.

Quarterly Leaching Sr-90, Ru-106, Cs-134, Cs-137 i of Weekly Continu-ous Sample ,

=

, oCalculated based on dilution

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(A) NFS PERIMETER AIR (C)CATTARAUGUSCREEKCONTIriUGUS -

SAMPLER (D) !!FS E:: VIRO::MD:TAL 00SIMETERS

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LOCATIO?! 0F THE FIXE 0 ENVIR07:'!E!:TAL SAMPLING STATIONS OF THE WESTERN MEW YORK flUCLEAR SERVICE CEliTER l Fig 1-1

2.0

SUMMARY

OF RESULTS During the last half of 1981, over 800 seoarate analyses of air, water, fish, deer, milk, and silt were performed. These analyses indicated the concentrations of radioactivity in the environmental media are less than the applicable limits of the U. S. fluclear Regulatory Commission.

The concentration of radionuclides in Cattarauaus Creek during the last six months of 1981 average 0.39% of MPC with a maximum observed concentration of 0.49% of MPC.

The concentration of radionuclides in the stack during the last six months of 1981 average 0.07% of the Technical Specification limit with the maximum observed at 0.13%.

The concentration of radionuclides in perimeter air decreased to levels determined for the second half of 1980. The direct radiation from the environment remained stable at the 1980 determined average.

3.0 LIQUID EFFLUENTS Liquid wastes are collected in two interceptor tanks and discharged to holding ponds if activity is less than the technical specification limit. The holding ponds provide surge capacity prior to further treat-ment.

In May of 1971, a low level waste treatment plant was put into operation to reduce cesium and strontium concentration in the liouid wastes. Typically the plant removes 96% of the ces4m and 99% of the strontium from the liquid wastes.

Following treatment, the liquid wastes are collected batchwise in two small lagoons. The water in the lagoon is analyzed for gross beta, cesium-137, and cesium-134. If cesium-134 and cesium-137 are below their respective MPC, the lagoon is transferred to the number 3 storage lagoon.

The water which collects in the number 3 storage lagoon is discharged to the creek system through a calibrated weir. During times of discharge, daily grab samples are taken from the weir and analyzed for gross beta

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activity. These grab samples from the weir are composited, based on lagoon discharge volume, and analyzed monthly for specific radionuclides to determine activity released. A total of 14 samples were used to make up the one monthly composite. Table 3-1 sumarizes the monthly liouid discharges as determined by composite analyses and flow measurements.

In addition to the data presented in Table 3-1, a quarterly composite of weir samples is analyzed for specific alpha emitting radionuclides.

Table 3-2 shows the quarterly liquid discharges based on these analyses.

Buttermilk Creek is the first major on-site stream to receive liquid discharges from the lagoon system. A bottom silt sample of Buttermilk Creek is taken quarterly near the Thomas Corners Road Bridge and analyzed for gamma emitting radionuclides. Samples in the third and fourth quarters of 1981 indicated principle radionuclides present were cesium-137 and potassium-40. Table 3-3 shows gross alpha and gross beta results on

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j samples. Water samples taken from Buttermilk Creek during the third j- and fourth quarters of 1981 and analyzed for gross alpha, gross beta r

l and tritium are shown in Table ~3-4. j 3 .

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Table 3-1 LAGOON DISCHARGES (Curies)

Total Beta Cattaraugus Other Than Total Water Over Creek Flow Month H-3 Alpha H-3 Sr-90 the Weir Averace Ru-106 Rh-106 I-129 Cs-134 Cs-137 (Gals x 106) (GPM x 105)

Jul 1981 NO DISCHARGE THIS MONTH - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - 2.17 Aug 1981 NO DISCHARGE THIS MONTH - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - 1.96 Sep 1981 i NO DISCHARGE THIS MONTH - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - 2.03 Oct 1981 0.058 0.00034

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71.6 0.0041 0.0012 0.0012 0.00016 0.00033 0.0125 4.41 2.44 Nov 1981 NO DISCHARGE THIS MONTH - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - 2.39 Dec 1981 NO DISCHARGE THIS MONTH - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - 2.06

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4 Table 3-2 LIOUID DISCHARGES Alpha Emittina Components (Curies)

Quarter U-234 U-235 U-238 Pu-238 Pu-239 l 3rd/1981 NO DISCHARGE TilIS QUARTER - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - - -

-6 -5 -5 4th/1981 3.01 + 0.84 x 10-5 <2.17 x 10 3.01 + 0.84 x 10 1.20 + 0.75 x 10-5 1.32 + 0.80 x 10 l

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Table 3-3 BUTTERMILK CREEK SILT ACTIVITY (Microcuries per Gram) 1981 Ouarter Gross Alpha Gross Beta 3rd 2.1 + 0.8 x 10-5 1.7 + 0.3 x 10-5 4th 6.6 + 2.4 x 10-6 1.6 + 0.1 x 10-5

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Table 3-4 BUTTERMILK CREEK WATER ACTIVITY (Microcuries per Milliliter) 1 1981 Quarter Gross Alpha Gross Beta Tritium 3rd <5.97 x 10-10 2,08 .+. 0.82 x 10-8 2.12 + 0.23 x 10-6

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4th <7.33 x 10 2.82 1 0.62 x 10-8 2.5410.07 x 10 '

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l 4.0 GASE0US EFFLUENT Gaseous plant effluents are sampled in the plant stack. The stack sampler contains a filter to collect particulates and an impregnated charcoal filter to collect iodine. Samples are removed from the stack sampler at least once every seven days and analyzed.

In addition to the stack sampler, a stack monitor is used to continuously determine the particulate radioactivity in the stack air and to alert operators if pre-set limits are approached. The filter paper on the particulate monitor is advanced daily and will alarm if the accumulation of particulate radioactivity over a four-hour period exceeds that.which would occur if particulates were being discharged over the same time period at the limit set by Technical Specifications.

The particulate radioactivity in the stack and the relationship to the Technical Specification limit are shown on Table 4-1. The curies of radioactivity released from the plant stack as determined on a quarterly combined sample is shown on Table 4-2.

Table 4-1 -

PARTICULATE RADI0 ACTIVITY RELEASED FROM PLANT STACK 1981 Alpha Beta  % of Tech Month (Curies) (Curies) Socc Limitl Jul 7.16 x 10-7 3.37 x 10-5 0.01 Aug 8.19 x 10-7 7.71 x 10-5 0.03

-6 -4 Sep 2.05 x 10 3.15 x 10 0.13 1.41 x 10-6

-4 9ct 1.04 x 10 0.03 Nov 8.18 x 10-7 2.48 x 10-4 0.10 Dec 8.53 x 10-6 2.66 x 10-4 0.11 1 Particulate release limit 0.1 microcurie per second

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! Table 4-2 RADI0 ACTIVITY RELEASED FR0!! PLANT STACK QUARTERLY DATA 1981 CURIES Quarter Sr-90 Ru-106 I-129 Cs-134 Cs-137 3rd 3.12 + 0.10 x 10 -5

<5.94 x 10-6 <2.68 x 10~0 1.59 _+ 0.79 x 10-6 1.83 .+_ 0.05 x 10-4 ,

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4th -5 -0 -5 -3 9.91 1 0.50 x 10 <1.29 x 10-5 <8.42 x 10 1.34 1 0.15 x 10 1.39 1 0.05 x 10 7 4

5.0 EflVIR0flMEflTAL MEASUREMENTS In the first half of 1981, the average concentrations of gross radioactivity and the average concentration of specific radionuclides in environmental samples of air, water, milk, fish and silt continued to be less than applicable limits of the U. S. Nuclear Regulatory Coninission.

5.1 AIR M0!!ITORIflG Particulate air activity is continuously sampled at three perimeter sampling statfor.s. The Fox Valley sampler is located two miles south-east of the plant, Route 240 sampler is 1-1/2 miles northeast of the plant, and Thomas Corners sampler is 2-1/2 miles north-northwest of the plant. A total of 78 weekly samples were collected during the last half of 1981 and analyzed for gross alpha and gross beta particulate radioactivity. To allow for decay of naturally occurring short lived radioisotopes such as lead-212, lead-214, and their daughter products, the air samples are stored for one week prior to counting. Following this decay period, the long lived activity from natural occurring radionuclides and fallout can be determined. The results of these analyses appear in Table 5-1.

5.2 BACKGROUf!D RADIATIOff Radiation background measurements around the site are determined by using energy corrected CaSO4 :Tm TLDs at 16 locations around the flFS site perimeter. These dosimeters are changed and evaluated monthly.

Data obtained for July through December 1981 are shown in Table 5-2.

5.3 CATTARAUGUS CREEK Samples of water from Cattaraugus Creek are taken with a continuous sampler located about one-half mile downstream from the confluence of Cattaraugus Creek and Buttermilk Creek. These samples are collected weekly and analyzed for gross alpha, gross beta and tritium. The results of these analyses are shown in Table 5-3. The 26 weekly samples were composited based on creek flow and analyzed for gross

alpha, gross beta and Strontium-90. The Iodine-129 was calculated from the Lagoon 3 composite. Data is shown in Table 5-4.

5.4 FISH During the second and third quarters of each year, NFS takes fish samples from Cattaraugus Creek between the point of discharge of Buttermilk Creek and the Springville hydroelectric dam, two miles downstream. The results of analysis on the fish samples collected for the third quarter of 1981 are shown in Table 5-5.

5.5 DEER Deer samples were obtained during October,1981. Results of these samples appear in Table 5-6.

. 5.6 MILK Milk samples from two farms located near the site boundary to the northeast and northwest of the piant are taken yearly in August. Results of these samples appear in Table 5-7.

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1 Table 5-1 PERIMETER AIR ACTIVITY (Curies per Cubic Meter) 1981 Alpha Beta Month Max. Avo. Max. Avg.

FOX VALLEY 6.41 x 10 -I4 July 2.90 x 10-16 -6 1.76 x 10 9.85 x 10-I4 August 4.59 x 10 -16 2.30 x 10 -16 4.63 x 10-14 3.12 x 10-14 September 3.95 x 10 -16 2.10 x 10-16 2.49 x 10-14 1.50 x 10-14 October 5.98 x 10-I6 3.65 x 10 -16 2.55 x 10 -I4 1.42 x 10-I4 November 3.20 x 10 -16 1.84 x 10-16 1.71 x 10-I4 1.17 x 10-14 December 2.91 x 10 -16 1.76 x 10 -16 2.23 x 10-14 1.50 x 10 -I4 ROUTE 240 July 2.17 x 10-16 1.58 x 10-16 9.75 x 10-14 7.51 x 10-14 August 7.28 x 10-16 4.54 x 10-16 5.05 x 10-14 3.63 x 10-14 September 7.28 x 10-16 5.65 x 10-16 3.42 x 10 -14 1.44 x 10-I4 October 5.09 x 10-10 3.19 x 10-16 2.44 x 10 -14 1.32 x 10-I4 November 3.96 x 10-16 2.03 x 10 -I0 1.51 x 10-14 1.18 x 10-14

-14 December 6.83 x 10-16 3.26 x 10-16 2.49 x 10 1.81 x 10-14 Tl10 MAS CORNERS July 3.85 x 10-16 2.03 x 10 -16 8.57 x 10-14 6.39 x 10-14 August 5.88 x 10-16 3.40 x 10-16 3.40 x 10-14 2.78 x 10-I#

-16 September 4.47 x 10-16 2.90 x 10 2.09 x 10-14 1.26 x 10-14 October 5.12 x 10-16 2.63 x 10-16 3.92 x 10-14 2.08 x 10-I4 November 8.69 x 10-16 3.57 x 10-16 1.91 x 10-14 1.39 x 10-14 December 3.07 x 10-16 2.25 x 10 -16 2.32 x 10-14 1.78 x 10-14

Table 5-2 MONTHLY ACCRUED BACKGROUND NEAR SITE PERIMETER Location flillirad per Standard Month - 1981 Direction F at From Plant (Miles) July Auoust September October November Decenber SSW 1.3 6.18 1 0.32 6.05 1 0.64 6.69 1 0.66 6.41 1 0.35 7.13 1 0.82 5.98 1 0.72 S 2.3 6.55 1 0.58 6.69 1 0.63 6.55 i 1.02 6.50 1 1.26 7.04 1 0.32 6.35 1 0.53 SSE 1.8 6.40 1 0.37 5.63 1 0.69 6.59 1 0.56 5.86 1 0.86 6.54 1 1.20 5.72 1 0.67 SE 1.7 6.66 1 0.29 5.62 1 0.44 6.05 1 0.51 6.7510.46 6.56 1 0.17 6.0610.45 ESE 1.5 6.33 1 1.12 6.14 1 0.45 6.43 1 0.96 6.30 1 0.76 6.51 1 0.30 6.34 1 0.53 1.6 '

E 6.33 1 0.58 5.70 1 0.95 6.28 1 0.47 6.03 1 0.99 6.32 1 1.11 6.09 1 0.51 ENE 1.2 5.78 1 0.94 5.30 1 0.41 6.09 1 0.63 5.90 1 0.37 6.16 1 0.29 5.83 1 0.69 5 NE 1.6 5.53 1 0.98 5.67 1 0.47 5.30 1 1.34 6.47 1 1.02 6.31 1 0.23 5.91 1 0.39 NNE 2.1 6.3410.46 5.70 1 1.15 6.08 1 0.94 6.15 1 0.68 6.4510.69 7.06 1 0.92 N 1.5 6.16 1 0.80 5.5510.46 5.87 1 0.72 6.48 1 0.93 6.34 1 0.76 5.66 1 0.92 NNW 2.4 6.68 1 0.92 7.06 1 0.11 6.15 1 0.67 7.n6 1 1.45 7.19 1 0.97 7.01 1 0.16 NW 1.4 6.37 1 0.34 5.61 1 0.47 6.02 1 0.19 6.51 1 0.74 5.92 1 0.59 6.12 1 1.18 WNW 0.8 7.08 1 0.63 7.20 1 0.77 6.4510.85 7.2210.40 7.81 1 0.48 6.67 1 0.50 W 1.2 6.4510.86 6.44 1 0.59 6.77 1 0.70 6.44 1 0.49 6.33 1 1.37 5.92 1 0.68 WSW 1.4 6.32 1 0.79 5.88 1 0.49 6.54 1 0.72 6.46 1 1.47 7.17 1 0.72 6.15 1 0.34 SW 1.5 5.20 1 0.51 4.89 1 0.48 5.26 1 0.64 6.85 1 1.24 5.68 1 1.09 5.49 1 0.37

Table 5-3 RADI0 ACTIVITY IN CATTARAUGUS CREEK - WEEKLY SAMPLES (Microcuries per Milliliter)

Date Gross Alpha Gross Beta Tritium 7/07/81 <2.98 x 10-10 1.05 + 0.51 x 10-8 2.22 + 0.21 x 10-6 7/14/81 <3.36 x 10-10 3.94 + 3.89 x 10 -9 2.80 + 0.22 x 10

-6 7/21/81 <3.27 x 10 -10 1.77 + 0.51 x 10 -8 2.25 + 0.21 x 10-6

-6 7/28/81 <4.07 x 10-10 1.63 + 0.65 x 10 -9 1.32 + 0.20 x 10

-6 8/04/81 <3.48 x 10-10 1.05 + 0.36 x 10 -8 1.60 + 0.21 x 10 8/11/81 <3.15 x 10-10 5.92 + 4.75 x 10-9 1.12 + 0.21 x 10-6

-8 8/18/81 <5.16 x 10-10 1.40 + 0.48 x 10 1.02 + 0.19 x 10-6 8/25/81 <3.15 x 10 -10 7.00 + 4.25 x 10-9 1.46 + 0.20 x 10 -6

-8 9/01/81 <4.02 x 10-10 1.34 + 0.50 x 10 8.56 + 1.86 x 10-7 9/08/81 <4.13 x 10-10 4.51 + 4.50 x 10 -9 1.28 + 0.20 x 10

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-6 9/15/81 <5.22 x 10-10 1.41 + 0.43 x 10-8 1.22 + 0.21 x 10 9/22/81 <2.78 x 10-10 1.14 + 0.43 x 10 -8 1.86 + 0.21 x 10 -6

-8 9/29/81 <2.98 x 10-10 1.17 + 0.45 x 10 1.74 + 0.20 x 10 -6 10/06/81 6.66 + 5.74 x 10-10 1.94 + 0.54 x 10 -8 7.20 + 1.84 x 10~7 10/13/81 6.97[5.12x10-10 2.98 2.92'x 10-9 1.25 0.19 x 10-6 10/20/81 <4.02 x 10-10 8.10 1 3.95 x 10~9 5.74 1 0.27 x 10-6

-6 10/27/81 7.76 1 6.14 x 10-10 9.92 1 4.84 x 10~9 7.08 1 0.30 x 10

-10 -6 11/03/81 6.31 1 6.08 x 10 9.27 1 4.46 x 10~9 4.65 1 0.26 x 10 11/10/81 <3.94 x 10-10 2.06 1 0.31 x 10-8 1.44 0.22 x 10-6

-7 11/17/81 <3.48 x 10-10 1.5610.44 x 10-9 8.12 1 1.89 x 10

-6 11/24/81 <3.03 x 10-10 1.50 + 0.42 x 10-8 1.44 + 0.20 x 10 6.91 + 4.33 x 10 -9

-7 12/01/81 <4.60 x 10-10 2.08 + 1.79 x 10

-8 0.21 x 10-6

, 12/08/81 <3.77 x 10-10 1.48 0.44 x 10 1.37

-8 12/15/81 <4.42 x 10-10 1.06 1 0.35 x 10 9.39 1 1.67 x 10-7

-7 12/22/81 <4.60 x 10-10 7.18 1 2.71 x 10-9 9.14 1 1.85 x 10 12/29/81 <4.52 x 10-10 1.24 1 0.36 x 10-8 3.63 1 1.72 x 10-7

t Table 5-4 RADIOACTIVITY IN CATTARAUGUS CREEK - COMPOSITE SAMPLES (Microcuries per Milliliter)

Month Gross Alpha Gross Beta Sr-90 I-129 Jul 1981 <3.27 x 10-10 -10 9.75 1 3.48 x 10-9 9.2714.0 x 10 ND Aug 1981 <3.27 x 10-10 7.59 1 3.98 x 10-9 6.66 1 3.0 x 10-19 ND Sep 1981 <3.32 x 10-10 -IO 1.19 1 0.32 x 10-8 6.39 1 2.9 x 10 ND

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Oct 1981 <5.74 x 10-10 8.15 1 2.68 x 10-9 3.79 x 10-12 7 5.44 1 3.6 x 10-10 Nov 1981 <4.57 x 10-10 8.90 1 2.78 x 10-9 <5.39 x 10-I0 ND Dec 1981 <3.52 x 10-10 7.55 1 2.93 x 10-9 6.63 1 3.0 x 10-10 ND ND - Not determined. No lagoon release this month.

4 Table 5-5 FISH SAMPLES FROM CATTARAUGUS CREEK - 3RD OUARTER 1981 (Microcuries per Gram)

Weight length Sample (grams) (inches) Bone Strontium-90 Flesh Strontium-90 Flesh Cesium-134 Flesh Cesium-137

-7 -8 -7 Dace #1 60 7.0 4.0 1 1.0 x 10 6.1 1 3.7 x 10 <2.6 x 10 <2.5 x 10-

-7 -7 -7 Dace #2 51 7.0 4.2 1 2.5 x 10-7 1.3 1 0.3 x 10 <2.3 x 10 <2.9 x 10

-8 Dace #3 57 7.0 4.7 1 1.4 x 10-7 7.1 1 1.9 x 10 <2.6 x 10-7 <2.6 x 10-7

-7 Date #4 45 6.5 6.0 1 2.7 x 10-7 3.6 1 2.1 x 10-8 <2.6 x 10 <3.6 x 10 -7 ,

-8 -7 Dace #5 34 6.25 4.6 1 1.7 x 10-7 3.2 1 2.6 x 10 3.013.0 x 10 <4.0 x 10-7 Dace #6 40 6.5 1.3 1 0.4 x 10

-6 a.9 2.6 x 10 -8 <3.4 x 10-7 <3.7 x 10-7

-8 Dace #7 37 6.25 <2.0 x 10-7 3.8 1 2.9 x 10 <3.1 x 10 -7 <4.0 x 10-7 Dace #8 37 6.5 <9.2 x 10 -8 <5.3 x 10 -8 <3.6 x 10 -7 <3.2 x 10 -7

-7 -7 Dace #9 40 6.25 2.0 1 1.4 x 10-7 4.0 1 3.5 x 10-8 <3.1 x 10 <3.5 x 10 3.65 x 10 -7 4.65 x 10 -8 2.9 x 10 -7 Median 3.36 x 10 Geometric Deviation 2.25 1.62 1.17 1.25

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t Table 5-6 DEER SAMPLE DATA (Microcuries per Kilogram)

Sample, Description, Date, Location Flesh Skeleton Cs-134 Cs-137 Sr-90 Sr-89 Sr-90 Deer, Female m 10/15/81 -5 -5 -5 East of P1 ant <1.0 x 10 -2 -2 9.5 i 1.4 x 10 2.6 1 0.7 x 10 <3.4 x 10 <1.2 x 10 Deer, Female 10/16/81 -4 -5 East of Plant <1.1 x 10-5 -3 1.3 1 0.2 x 10 6.410.9 x 10 <7.8 x 10-3 <2.7 x 10

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Table 5-7 MILK SAMPLE DATA (MicrocuriesperMilliliter)

Sample Date Sr-90 I-129 Cs-134 Cs-137 NE Farm August 1981 5.1 1 1.6 x 10-9 <1.7 x 10-9 ' <6.9 x 10-9 <7.8 x 10-9 NW Farm August 1981 3.8 1 1.5 x 10-9 <1.7 x 10 -9 <1.2 x 10 -8 1.4 1.4 x 10-9 l

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