Text

Rept on Preoperational Environ Survey in Vicinity of Con Ed Indian Point Nuclear Electric Generating Plant
	ML20031G069
Person / Time
Site:	Indian Point
Issue date:	11/30/1959
From:	Hilleboe H; NEW YORK, STATE OF
To:	;
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A PRE-OPERATIONAL ENVIRONMEiJTAL SURVEY IN THE VICINITY OF THE CONSOLIDATED EDISON COMPANY'S

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cocnerEn INDIAN POINT NUCLEAR ELECTRIC E

MAR 171971 * '-3

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GENERATING P!. ANT S'

T!?,ll2lllll77

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ratts of electricity.

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D gorintion of*linrvey i

The ConcolidatN1 Fdison pre-operational nurvey covered c:trapling ctations within a 25 nile radius of the renctor sito. Tho locations of the sampling citec for the various types of camplec are shown,n mapa within the report. A nore completo description of.the sampling stations an' the numbering cystem can be found in the appendix.

Gross beta counts were made on most of the samples collected in 1958. It was apparent, cince 1953, that fallout from nuclear weapons testing contributed a significant portion of the total radioactivity found in different phases of the environment.

In order to better deter.aine the concentraticn of biologically significant fission products, the Division of Laboratories and Reccarch developed a more sp3cific test knotm as "bota 3

bone seekers". This nethod involves the chenical ceparation of the alkaline earths which include. the fission products Sr 9, Sr90_y90, Ba140,,t3140 This 8

test is much less tine censuming than a specific isotopic analysis for Sr90, The beta bone seeker method was used for the radiological analysis of all sanples, except air samples and rabbit thgroids, collected after mid-January 1959, ilaturally occurring uraniun and thorium and their daughters will contribute to the natural rcdioactivity as well as Potassium 40, 0

Rubidiun 7 and others. The " beta bone seeker" method eliminatec most of the naturally occurrind radioclenents.

P.abbit thyroids are the onc xception uhere a cpecific isotopic analycia was nado for I1 31 by grunma counting. To date, there has been no analyses med3 for alpha activity in environnental samples, o

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i The re:ults as reported in the tabica are et the time of counting.

l Activities ucre not extrapolated to dato of collection except for a series of air particulato samplea collected in Juno 1950.

Analysis for some specific icotopes and Cross beta analysis is planned in 1950 for selected samples.' A noro complete description of the i

rr.ethods of anal'ysis used can be found in the appendix.

An aerial survey of the area surrounding Indian Point has been made. Since a prior report was made on the survey, it is et included in this report.

Air S m leas On July 18, 1953 cnd July 24, 1958, air particulato samples were collected by local rad state Health Departme-personnel from 14 and i

12 recpective stations. These samples were taken utilizing high volume air saq Mrs of approximately 50 cubic feet per minute capacity and an 8 inch by 10 inch class fibre filter. Since there were at leart three days between i

sarpling and cer.. ting, the cosults uero not indicative of radon or thoron cc acntntions. The major part of the beta activity recorded was, therefore, due to f.ssion products fron weapons tests.

The operatien and naintenan.o of air s,.cplers on daily basis was fotad to be time censuming and tras found to give only a little more q

information than a weekly continuous sampler. Since in an environmental d

survey of the type bcinc mcde average results are considered to be the most sicnificant, the decision was nade to collect weekly samples. Consequently, 1 cubic foot per r.inute positive displacenent "Gast" air pumps woro utilized uith a 2 inch di acter class fibro filter. Five air sampling stations wero established at locations around the reactor site (sco Map #1). These camplers ucre operated for a period of seven days, the filter removed and sent to the labort. tory for counting.

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Fallnut Six fallout nampling ntnLiono nero entablit.hnd (cee M1p M.
The in ': hot la weichted c.f. the Imttom inv! is lined ulth a double polyet.hylene bag. The baC is sent in with the sample and proccaced with the sample so i
that dust collected is also counted. Difficulty with cnow and ice hac been experienced and ;omo method of overcoming the problem of drifting snow is being considered.
i Rabbit Thyroids Thyroid samples from cottontail rabbits killed uithin a 12 mile radius were counted for I131 The rabbits were killed with a 22 calibre rifle, the thyroids extracted, and sent to the laboratory by the l
t' Ccnnervatien Department. The sampling areas were selected considering i
i rance of the animal and on the basis of being able to select future specimens from the same general area.
"lil Soil sar.ples ucre taken at the same location es vegetation r nples as choun on Map f4 and further described in the appendix. Coil ples were taken from the upper two inches using a 6-7/8 inch dier.cter core tool.
The normal prcccdure was to shake the soil loose from the overlying vocetation. All large stones uere also removed. To date, no soil camples have been analy cd. These sanples are stored 2.nd vill be available for analysis in the future if indicated.
_Vecn tation The vegetation nornally sanpled were laurel or planton although other types of samples have been obtained because of the lack of laurel or platten in the area being sampled. The censon of the year also influenced the type of vegetation obtained. The vegetative comples were analy::cd for beta bene cockers.
It is to be noted that those carples colIceted in 1958 vore not enalyzed until 1959; consequently, one nuct contider the ti.xe between collectior. and actusl counting in interpreting the recults.
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, Unter Samp1*2 Water campica wsro co11ceted from all public wster courcoa rithin a ten mile radius of Ind'an Point. Inaddition,somesurfaco waters wcro campicd even though they w. re not public. unter courcea. The campling locations are chown on Map 15. In all cr.cos, raw water sampics were obtained either by dipping from a lake or by 'sanpling the raw water tap. Some samples also have been taken from the Hudson River by the Conservation Dep'artment asing a "Kemmerer" sampler. These are reported und'er Hudson River samples. The United States Public Health Service has been obtaining Hudson River weekly grab samples at Poughkeepsie and analysing for dissolved and suspended beta radioactivity; results are shown in Table VI.
Water sanples on uhich gross beta counts were made are repccted with the counting error as shown in Table V.
The counting error reported represents a 95% confidence limit.
The New York State Health Departnent has obtained weekly conposites of daily sanples of the Hudson River at Waterford, Glen ont and of the Mohawk River at Cohoes. Waterford is on the Hudson above the confluence of 3
the Mohtuk and Hudson, and Glenment is below this conflucr.ce. Cohoes is en the !!chawk above the confluence of the Mohawk and Hudson Rivers.
l Hudson River _S,nples Hudson River sampics include water, bottom muds, plankton, and fish. The Cc.:cervation Department has obtained sanples of water, and bottom muds at Manitou Beach and Croton Point as shown on Map 15. A plankton net wra used to obtain plankton surples at loth points.
l Fish vere obtsined by screening.
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i
r Milk A few milk camplos have bexn ecllected to dato; however, this report will not include such renults because of the limited data available at this time. A supplementary report will'be nado covering milk sampics collected in ccnnection tiith this survey, and will include results of camples collected in the statewide Milk Surveillance Program for comparicon.
e 9
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Y f:vnin rit Ion cl' IfriI t. ' II:'ad The maximum allo.rdble concentrations (it.LC.) acccrding to state and federal recuintions are expressed in terr er nicro curios timen 10 to com negative.oxuonont, i.e. 7 x 10"y' pc/cl.
In orlor to reduce the possible error in reporting end transcribing results, the more convenient unit micro 'alcro curies ves c.depted.
The units used for reporting results aro listed as fo11cws:
Air - ppe/m3 micro-micro cu~ies per cubic meter of air Fallout - ppe/ft.2/ day-micro-microcuriespersquarefcctcf nrea por uay.
i Rabbit thyroid - p,uc - micro-micro curies por thyroid Vegotation - p'pc/gm - micro-mieri curies per (dried at 1030 C) gram of dry vegetation Water - ppc/.al - micro-micro curios por milliliter of water Mud, Plankton, Fish - ppc/gm - micro-C ;ro curios per crc cf dry relids (dried at 1030 C)
The results roperted in all tables cro at the tims of ecunting, except for tho hi h-volume air se;,les which are reported at the tino of c
collecticn.
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/100 1.22 A-2 6-24-58 s100 2.98 1103 A-1 6-18-58 60 1.30 A-2 6-24-58 v100 2.80 1105 A-1 6-18-58
~100 1.20 A-2 6-24-58 100 3.10 1302 A-1 6-18-58 y100 1.06 1307 t.-1 6-18-58 71 1.24 A-2 6-24-58
> 100 3.05 1401 A-1 6-18-58 44 1.15 A-2 6-24-58
.' 100 2.71 1402 A-1 6-18-58 82.
1.02 A-2 6-24-58
>100 2.72 2C02 A-1 6-18-53 76 1.38 A-2 6-24-58 n100 2,75 2101 A-1 6-1r-58 51 1.65 A-2 6-24-58
?100 3.00 2202 A-1 6-18-58 56 1.43 A-2 6-24-58 7100 2.85 2301 A-1 6-18-$3 96 1.60 A-2 6-24-58 7100 2.96 3302 A-1 6-1P-58 46 1.45 2204 A-1 6-1P-53 64 1.50 A-2 6-24-58
100 3.30 Re

: alta of U.S.P.H.S.
tilhany, :1.Y.
6-18-58
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/100 4.05 Ilartford, Conn.
6-18-58 7100 0.(4 6-24-g
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(Wookly Gn::t Air Pump Unntile) 4 D, ton Colicetcq Groreget.a Sernie C tet ion.hbor St.nrt Stori Dntn~Countml
_g 7501 3-26-59 4-6-59 4-14-59 4.1 II.D. A., Pauling,
4-6-59 4-13-59 4-19-59 5.4 Datebcas County 4-13-59 4-20-59 5-5-59 6.4 4-20-59 4-27-59 5-5-59 7.2 4-27-59 5-9-59 5-17-59 3.8 5-9-59 5-18-59 5-30-59 3.8 5218-59 5-25-59 6-5-59
?.9 5-25-59 6-1-59 7-3-59 4.6 6-1-59 6-9-59 7-15-59 2.6 6-9-59 6-1B-59 7-26-59 2.1 6-18-59 7-13-59 8-7-59 1.1 7-13-59 7-23-59 8-17-59 0.4 7-21-59 7-27-59 8-17-59 0.6 4401 3-26-59 4-2-59 4-14-59 6.2 Unicn Ctrbide, Tuxedo, 4-2-59 4-16-59 5-5-59 4.9 Oran c County 4-16-59 4-23-59 5-5-59 7.6 4-23-59 4-33-59 5-5-59 6.2 4-30-59 5-11-59 5-17-59 5.1 5-11-59 5-13.,9 5-30-59 3.5 5-1S-59 5-25-59 5-30-59 3.4 5-25-59 6-1-59 7-3-59 5.7 6-1-59 6- 0-59 7-15-59 2.9 6-8-59 6-15-59 7-26-59 2.6
'6-15-59 6-22-59 7-29-59 2.3 6-30-59 7-6-59 6-7-59 1.L 7-6-59 7-20-59 8-17-59 0.9 2003 3-27-59 4-3-59 4-14-59 5.2 Terkins Cove, 4-3-59 4-10-59 4-19-59 6.9 Roi: lend County 4-10-59 4-17-59 5-5-59 7.0 4-17-59 4-24-39 5-5-59 7.4 L-24-59 5-1-59 5-5-59 6.3 5-1-59 5-P-59 5-17-59 4.9 5-C-59 5-15-59 5-22-59
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'-14-59 5.6 4-3-59 4-10-59 l-19-59 5.8 4-10-59 4-16-59 5-5-59 5.0 4-16-59 4-24-59 5-5-59 6.6 I
4-24-59 4-30-59 5-5-59 5.6 4-30 59 5-7-59 5-17-59 3.8 5-7-59 5-21-59 5-22-59 6.1 5-21-59 5-29-59 7-3-59 4.6 5-28-59 6-4-59 7-15-59 2.3 6-4-59 6-11-59 7-26-59 2.9 6-11-59 6-18-59 7-26-59 2.0 6-18-59 6-26-59 E-3-59 1.7 6-26-59 7-2-59 P-3-59 0.6 7-2-59 7-9-59 8-7-59 1.8 7-9-59 7-17 59 E-13-59 0.7 7-17-59 7-24-59 e-17-59 0.4 1307 3-12-59 3-19-59 3-27-59 3.9 0:sining, Westehcoter 3-19 59 3-26-59 4-5-59 7.0 County 3-26-59 4-3-59 4-14-59 5.7 4-3-59 4-10-59 5-30-59 3.7
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Tfl1LM IT-A FLTTCUT ~ Dota Dono Station Collection Period Late Gross Deta Geek,ers flumber SM GA Coimted uncht./dny uncht. /laz. 1103 Camp J ' c.-5 0 10-?5-58 11-9-58 515 Smith 10-25-50 11-10-58 11-20-58 1200 11-10-58 11-24-58' 12-15-58 '212 11-24-58 12-17-58 1-6-59 210 1-6-59 1-22-59 2-16-59 408 1-22-59 2-I-59 2-27-59 1LL7 2-4-59 2-20-59 3-10-59 290 2-20-59 3-5-59 3-27-59 150 3-5-59 3-19-59 4-5-59 274 3-19-59 4-3-59 4-19-59 355 4-3-59 4-16-59 5-2-59 140 l 4-16-59 4-30-59 5-17-59 206 4-30-59 5-14-59 5-30-59 118 5-14-59 5-28-59 7-15-59 43 5-28-59 6-12-59 7-26-59 48 6-12-59 6-26-59 8-10-59 122 6-26-59 7-9-59 8-7-59 19 7-9-59 7-27-59 8-7-59 34 7-27-59 8-6-59 P-28-59 33 8-6-59 8-20-59 9-2-59 10 6-20-59 9-3-59 9-22-59 9 9-3-59 9-17-59 9-28-59 4 -1105 10- 9-58 10-25-58 11-9-58 485 Peekskill 10-25-58 11-10-58 11-20-58 590 11-10-58 11-24-58 12-15-58 200 11-24-58 12-17-58 1-16-59 172 1-6-59 1-22-59 2-16-59 480 1-22-59 2-4-59 2-27-59 122 4-4-59 2-20-59 3-14-59 205 2-20-59 3-5-59 3-27-59 ~156 3-5-59 3-19-59 4-5-59 103 3-19-59 4-3-59 4-19-59 452 4-3-59 4-16-59 5-2-59 159 4-16-59 4-30-59 5-17-59 314 i-30-59 5-14-59 5-30-59 78 5-14-59 5-28-59 7-15-59 56 5-28-59 6-12-59 7-26-59 40 6-12-59 6-26-59 8-10-59 117 6-26-59 7 "-59 8-7-59 18 7-9-59 7-27 '9 8-16-59 21 7-27-59 F-6-59 P-28-59 36 E-6-59 8-20-59 9-2-59 12 8-20-59 9-3-59 9-2?-59 5 9-3-59 9-17-59 9-28-59 3 12 +3
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P: Plasto.i 0.L.= Oak Innf S.C.= Ukunk Cnbbago E= r:vergreen II.it.:: llenlock Couch S= Spru :o F=. Fern C= Cedor IM!ullen Plant
- Ir. ir.urci !..U.= l!oney Suckle 0= Gracs 7p flot $ dor.tifled I =. Ivy We 4.la 19 4 - g S -s v '-~e. 'e~-e,-+, -,,,, _, -
TMifFl TV En' h,.n t..c OgJ..n 4 ) Pw:n 2 l a 3 mpin Dato Iki t.o Type or p;:e/crnn hl.m-Qur_td b~,tnod yogoman Pa t.c ttare hot c 1202 V-1 7-18-58 9-16-59 P 12 V-2 11-25-58 8-25-59 P 106 V-3 4-3-59 9-2-59 F 150 i V-4 5-27-59 9-13-59 P 37 [ 1301 V-1 7-22-58 9-16-59 P 26 1 1 V-2 11-28-58 8-25-59 P 115 V-3 4-1-59 9-2-59 F 1El V-4 6-4-59 9-13-59 P .27 1302 V-1 7-18-58 9-16-59 P 14 V-2 11-28-58 8-25-59 t4 23 V-3 4-6-59 9-2-59 E 95 V-4 5-25-59 9-73-59 P 26 t 1303 V-1 8-14-58 9-16-59 P 16 V-2 12-1-58 8-25-59 P 70 V-3 4-2-59 9-2-59 E 78 V-4 5-26-59 9-13-59 P 68 1304 V-1 7-21-58 9-16-59 P 35 V-2 12-1 -58 8-25-59 F 13 V-3 4-1-59 9-2-59 F 124 V-4 5-26-59 9-13-59 P 37 1 1305 V-1 7-21-58 9-16 59 P 3!. V-2 12-1-58 8-25-59 P 14 i V-3 4-1-59 9-2-59 P 109 V-4 5-25-59 9-13-59 P 41 1306 V-1 7-22-58 9-16-59 P 20 V-2 12-2-58 8-25-59 P 17 V-3 3-T6-59 9-2-59 E 89 Y-4 5-27-59 9-13-59 P 50 1307 V-1 6-30-58 9-16-59 P 21 V-2 11-24-58 E-25-59 P /,3 V-3 /,- 2-59 9- ?-59 P 55 V-4 5-26-59 13-59 P 32 l 1308 V-1 7-22-58 9-16-59 P 22 V r2 12-2-58 8-25-59 P 107 V 4-1-59 9-2-59 0 76 V-4 5-27-59 9-13-59 P 44 j J 20 i 7
l TAPfR TV tfantr bonter County (Con't 1 Pogo 3
eple Dnto Dato Tyve of ppc/genm grier Coltalted' hn,innd Varn',etion Datn linno Soakor 1309 V-1 7-22-58 9-16-59 P
27 V-2 12-2-58 8-25-59 'P 67 V-3 4-7-59 9-2 0 71 V-4 5-29-59 9-16-59 P 40 1310,V-1 7-21-58 9-16=59 P 25 V-2 12-9-58 8-25-59 L 10 V-3 4-6-59 9-2-59 P 166 V-4 5-25-59 9-16-59 P 164 1401 V -I 7-22-58 9-22-59 P 5 V-2 12-9-58 8-25-59 M 110 V-3 4-7-59 9-2-59 W 168 V-4 5-22-59 9-16-59 P 37 1402 V-1 7-23-58 9-22-59 P 5 V-2 12-11-58 8-25-59 7 ri V-3 4 /.-59 ? 2-59 F 74 V-4 5-29-59 9-16-59 P 41 11.03 V-1 7-23-58 9-22-59 P. 16 V-2 12-11-58 8-25-59 E 21 V-3 4-8-59 9-2-59 L 72 Y-4 5-25-59 9-16-59 L $6 1404 V-1 6-30-53 9-22-59 P 5 V-2 12-12-58 8-25-59 H 9 V-3 4-6-59 9-2-59 E 32 I V-4 6-21-59 9-16-59 P 28 1405 V-1 7-22-58 9-22-59 P~ 7 V-2 12-12-58 8-25-59 E 47 l V-3 4-9 59 9-2-59 E 62 V-4 6-2-59 9-16-59 P 39 14C6 V-1 7-20-58 9-2.2-59 P 21 V-1 12-12-58 ' 8-25-59 P 107 G-25-59 !!.S. 39 V-3 4 3-59 1407 V-1 7-28-58 9-22-59 P 7 V-2 12-17-58 8-25-59 P 72 V-3 4-P-59 9-2-59 F 100 V-4 6-4-59 9 16-59 P 16 1408 V-1 7-23-58 9-72 -59 P 11 V-2 12-5-58 8-25-59 P 59 l V-3 4-F-59 9-2 59 S.C. 141 i V-4 6-2-59 9-16-59 P 58 21 s e i
r-l Telii): IV $$ clin: tor Cwmtv (C<in't-) Pnco 4 Un plo Date Date Type of ppe/syom ilual r Collected Evc M ned -
V crMdgn Deta 13nna I'no%g 1409 V-1 8-14-58 9-22-59 P
4 V-2 12-18-58 8-25-59 F 49 V-3 4-7-59 9-2-59 L 120 V-4 5p5-59 9-16-59 P E6 1410 V-1 7-28-58 9-22-59 P 7 .V-2 12-19-58 8-25-59 F 47 V-3 4-9-59 9-2-59 F 319 V-4 6-2-59 9-16-59 P 64 1 1411 V-l' 7-20-58 9-22-59 P ~ 39 V-2 12-19-58 8-25-59 S 11 V-3 4-9 59 9-2-59 5 86 V-4 6-2-59 9-16-59 P 162 1412 V-1. 7-28-58 9-22-59 P 14 V-2 12-19-58 8-25-59 E 17 V-3 4-E-59 9-2-59 F 9 V-4 6-2-59 9-16-59 P 49 e e f e d 9 22
~ T/11ti:]V, VKtEgitvi nr. 9' int a 3 1JgMm f:::li>rry lim.>plo Dt.to Dato Tyin of Jpe/;;rren flimbor Con no t art Fvrmined Vormtrit T on l'ot n 1 ano :tne%r 2001 V-1 10-30-58 9-22-59 L' 45 V-2 6-19-59 9-2-59 L 13 V-3 9-13-59 10- 5-59 L 11 2002 V-1 10-30-58 9-22-59 L 78 V-2 6-l')-59 9-2-59 -L 34 V-3 9-18-59 10- 5-59 L 34 2101 V-1. 10-30-58 9-22-59 0.L. 68 V-2 6-19-59 9-2-59 L 35 i V-3 9-18-59 10- 5-59 L 28 l 2102 V-1 10-30-58 8-25-59 L 55 S-2 6-19-59 9-2-59 L 51 V-3 9-18-59 10- 5-59 L 29 2103 V-1 10-30-58 8-25-59 L 13 V-2 3-5-59 8-25-59 I 31 V-3 6-19-59 9 59 L 20 V-4 9-18-59 10-14-59 L 13 2201 V-1 10-30-58 8-25-59 'L 93 V-2 6-19-59 9-2-59 L 20 V-3 9-18-59 10-14-59 L 10 2202 V-1 10-30-58 8-25-59 L 43 V-2 6-19-59 9-2-59 L 29 V-3 9-18-59 10 % L 4 2301 V-1 10-3W58 8-25-59 L 23 V-2 3-5-59 8-25-59 L 30 V-3 6-19-59 9-2-59 L 45 V-4 9-18-59 10-24-59 L 35 2302 V-1 10-30-58 8-25-59 ? 46 V-2 3-5-59 8-25-59 L 27 V-3 6-19-59 9-2-59 L 26 V-4 9-18 59 10-14-59 L 14 23
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TM11F. TV VECF, TAT {NI S AMPIES 6rnns'n County Ocelo %to Date Type of p;tc/gran N rlsr Collonted_ Ewined bpjMgD "at" Pena Um +n r i 4203 V-1 10- 9-58 9-15-59 P 24 4301 V-1 10- 9-58 9-16-59 F 26 4302 V-1 10- 9-58 9-16-59 L 9 V-2 4-3-59 9-16-59 L 66 1 Datn,m Co'mtr l i 3201 V-1 10- E-58 9-16-59 P 15 V-2 5-8-59 9-16-59 P 105 l 3302 V-1 10- E-58 9-16-59 P 29 3401 V-1 10- 8-58 9-16-59 P 21 V-2 5-8-59 9-16-59 P 36 k 7 i I t i i 24
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TAlt!.M V W'u f( ~ EiWEtl.7c C..!'utX Ectn 1 n:m Danple Date Date ' Orena Data Ue n'<"ra nir+or co11oetog ' inn t n~1 ge/rei _ggfj_1_._ 1001 U-1 8-12-58 12-1-58 O.007* 0.005 W-2 11-20-58 1-12-59 0.015 t 0.002 W-3 4-7-59 6-29-59 0.019 U-4 6-9-59 7-15-59 0.009 1101 W-1 8-12-58 12-6-58 0.015 0.006 W-2 11-20-58 1-12-59 0.077 1 0.005 U-3 4-7-59 6-22-59 0.035 W-4 6-9-59 7-26-59 0.025 1102 W-1 8-12-58 12-3-58 0.004 t 0.005 W-2 11-20-58 1-12-59 0.009.1 0.002 d-3 4-7-59 6-2-59 O.021 U-4 6-9-59 7-15-59 0.0C9 1103 W '. 8-14-58 12-6-58 0.002 i 0.006 U-J 11-25-58 1-12-59 0.007 + 0.002 W-3 4-7-59 6-22-59 0.012 ~ U-4 6-9-59 7-15-59 0.005 1104 U-1 P-12-58 32-3 -58 0.006 i 0.006 U-2 11-26-58 1-12-59 0.025 + 0.002 W-3 4-7-59 6-29-59 0.0C8 W-4 6-9-59 7-1J-59 0.001 1105 W-1 8-12-58 12-6-58 0.005 0.006 U-2 11-25-58 0.004
0.002 U-3 4-7-59 6 "9-59 0.013 W-4 6-9-59 7-26-59 0.006 1201 W1 2-13-58 12-6-58 0.015 i 0.006 U-2 11-26-58 1-12-59 0.040 1 0.003 i
U-3 4-7-59 6-22-59 0.C25 W-4 6-9-59 7-15-59 0.016 4 1301 J-1 8-12-58 12-6-58 0.023 i 0.006 W-2 11-28-58 1-12-59 0.018 i 0.C02 U-3 4-7-59 6-22-59
o.C25 W4 6-9-59 7'26-59
" 014 1302 W-1 8-13-58 12-3 -58 v 009 1 0.005 W-2 11-28-58 1-12-59 0.009 1 0.002 W-3 /.- H-59 6-2?-59 0.c09 W-4 6-9-59 7-26-59 0.041 26 - ~
Tlli!M V or t.ch.gt cr Coim t v2 ( onMpigd Pnro 2 Deta lloro 3.mplo Doto Dato crosn Deta Gork as fl inly;n Colk cM F'xy,ined gnph1 pc hl __ 13 03 U-1 P.14-SS 12-6 -58 0.008 0.006 V-2 12-1-58 1-12-59 0.049 i 0.004 U-3 4-7-59 (-22-59 0.017 U-4 6-9-59 7-26-59 0.017 1304. U-1 8-13-58 12-3-58 0.010
0.005 U-2 12-1158 1-12-59 0.027 1 0.002 U-3 4- ~<-59 6-29-59 0.017 W-4 6-9-59 7-15-59 0.001 1305 U-1 2-13-58 11-30-58 0.009 t 0.0C5
'ef-2 12-1-58 1-12-59 0.018
0.002 l
"3 4- /-59 6-22-59 0.012 W-4 6-9-59 7-26-59 0.011 13C6 U-1 8-13-58 12-3-58 0.005 0.005 U-2 12-2-58 1-12-59 0.014 0.002 W-3 4-7-59 6:2-59 0.017 U-4 6-9-59 7-15-59 0.009 1307 U-1 6-13-58 12-3-59 0.007 0.005 U-2 11-24-58 1-12-59 0.016 t 0.CO2 U-3 4-7-59 6-29-59 0.014 "-4 6-9-59 7-15-59 0.011 1308 U-1 8-12-58 12-6-58 0.002 t 0.006 G* U-2 12-2-58 1-12-59 0.002 0.002 U-3 4-8-59 6-29-59 0.002 W-4 6-10-59 7-26-59 0.001 1309 U-1 6-14-58 11-30-58 0.004
0.006 U-2 12-2-58 1-12-59 0.023 0.002 U-3 4-E-59 6-29-59 0.025 d-4 6-10-59 7-15-59 0.010 1310
'!-1 2-14-58 1?- 6-58 0.03 1 0.c07 U-2 12-2-58 1-12-59 0.005
0.002 U-3 4-8-59 6-22-59 0.005 W-4 6-10-59 7-26-59 0.010 1401 W-1 6-12-58 11-30-58 0.009 0.006 U-2 12-9-58 1-12-59 0.012 i 0.002 U-3 4-6 59 6-22-59 0.013 W-4 6-10-59 7-26-59 0.010
"(G-croani water supply) 27
'fADIE k o Uo;2dgf or County _
g}yyl Pugn 3 Pota Dono Unnplo Dato Dato Gro.Ja Eota Oeckern
!!o-ba_g CnJ 1octori Fy,H nerl 4;pcEL_ -p;c/"I 1402 '1-1 F-3.7-58 11-30-58 0.008 0.006 U-2 12-11-58 1-12-59 0.006 i O.002 U-3 4-8-59 6-22-59 0.006 31-4 6-10-59 7-15-59 0.009 1404 '<!-1 F-14-58 12-3-58 0.005 i 0.006
G U-2 12-12-58 1-12-59 0.004 i 0.002 U-3 4-E 59 6-29-59 0.c00 U-4 6-10-59 7-15-59 0.001 1405 U-1 8-12-58 11-28-58 0.015 0.006 U-2 12-12-58 1-12-59 0.011 t 0.002 W-3 4-6-59 6-29-59 0.013 W-4 6-9-59 7-15-59 0.014 14C6 "1
6-12-58 11-2 %58 0.002 0.005 U-2 12-12-58 1-12-59 0.061 0.004 U-3 4-6-59 7-3-59 0.061 U-4 6-9-59 7-26-59 0.020 1407 "1 2-12-58 11-28-58 0.009 0.005 U-2 1?-17-58 1-12-59 0.005 0.002 P-3 4-6-59 6-29-59 0.008 U-4 6-10-59 7-15-59 0.012 1A03 U-1 8-18-58 11-2P-58 0.010 0.005 W-2 12-18-58 1-12-59 0.018 t 0.002 4-25-59 6-29-59 0.011 1. 6-9-59 7-26-59 0.012 1409 W-1 2-14-58 12-6-58 0.012 i 0.006 W-2 12-1S58 1-2-59 0.012 t 0.002 U-3 4-2-59 6-22-59 0.023 U-4 6-9-59 7-15-59 0.015 1410 U-l F-1?-53 11-29-58 0.025 i 0.006 U-2 12-19-58 1-12-59 0.008 0.002 U-3 4-N59 6-22-59 0.012. U-4 6-- 9-59 7-15-59 0.010 1412 U-1 "-]P-58 12-3-58 0.018 i 0.005 U-2 1:?-19-58 1-12-59 0.028 0.003 U-3 4-C-59 6-29-59 0.0?1 U-4 6-9-59 7-15-59
0. 01')
(C-cround water nupoly) w
T41'TF. V (C<dt,J DrCKT. 'UD CO l;rTY. Data Dono Ormplo Dat,c Date Gro.w Deta' 1.,ckerc tb n-bo r-Colle c trel F.minrel upc/,1 _ppc/')_, 2110 W-1 8-19-58 11-22-58 0.007 0.005 W-2 11-18-58 12-12-58 0.009 0.002 G* W-3 3-20-59 4-14-59 0.003 W-4 6-26-59 8-3-59 0.002 2210 U-1 8-19-58 11-26-58 0.001 0.006 U-2 11-17-58 12-12-58 0.000 0.001 G* W-3 3-20-59 '4-19-59 0.001 W-4 6-26-59 7-29-59 0.000 2211 U-1 8-19-58 11-26-58 0.003 i 0.006 U-2 11-17-58 12-12-58 0.001
0.001 G5 U-3 3-20-59 4-2;-59 0.001 U-4 6-26-59 8-3-59 0.000 2212 U-1 8-19-58 10-26-58 0.005 0.002 U-2 11-17-58 12-12-58 0.010 0.CO2 U-3 3-20-59 4-14-59 0.008 U-4 6-26-59 7-29-59 0.003 2213 W-1 8-19-58 10-26-38 0.006 0 003 U-2 11-ir-58 12-6-58 0.005 i 0.006 G*
W-3 3-20-59 4 i4-59 0.001 U-4 6-26-59 8-J-59 0.000 2310 U F-19-58 11-26-58 0.015
0. 0'. 9 U-2 11-19-58 12-8-58 0.020 1 0.005 U-3 3-20-59 4-14-59 0.014 U-.4 6-26-59 7-29-59 c.013 2311 U-1 8-19-58 11-26-58 0.000 0.005 G4 M-2 11-17-58 1?-12-58 0.001 0.001 2312 U-1 C-19-58 31-26-58 0.000 1 0.006 U-2 11-19-58 32-12-58 0.001 0.001 G*
W-3 3-20-59 4-14-59 0.001 U-4 6-26-59 8-3-59 0.001 2313 U-1 8-19-58 11.26-58 0.001
0.006 Wa2 11-19-58 12-12-58 0.005 0.002 G"
W-3 3-?O-59 4-16-59 0.C01 W-4 6-26-59 8-3-59 0.000
(G-crcund water aupply) i 29
3.nn: y IWnxin CW "Y (cog t) Pm;c 2 e Dcta Dono Gre ple Dato Dato GrDas Bota Sockcro tr Sqn Collget21 Ermineri m /n1 ,;tlic/,1 2314 U-1 0-19-58 11-26-58 0,002 0.006 G" U-2 11-19-58 12 58 0.005.'. 0.007 2315 W-1. 8-18-58 11-23-58 0.014 1 0.006 W-2 5-18-59 6-29-59 0.02 0 U-3 7-29-59 8-20-59 0.008 2316 U-1 E-21-58 13-26-58 0.005 t 0.005 W2 5 -] C-59 429-59 0.027 W-3 7-29-59 0-20-59 0.009 2317 U-1 3-20-59 /.-14-59 0.020 '4-2 6-26-59 6-3-59 0.039 2318 1 3-20-59 4-14-59 0.013 W-2 6-26-59 8-3-59 0.007 2319 U-1 3-20-59 4-14 -59 0.023 ~4-2 6-26-59 C-3-59 0.022 2410 U-1 8-19-58 10-26-58 0.001 t 0.001 U-2 11-19-58 12-6-58 0.001 0.0C6 G* U-3 3-2.0-59 4-14-59 0.001 U-4 6-23-59 C-3-59 0.001 2411 U-1 8-19-58 11-26-58 0.009 t 0.C05 L2 11-19-58 1?-1?-58 0.012 A 0.002 3 3-20.59 l -1/,-59 0.G19 U-4 6-26-59 8-3-59
0. 08 2/.12 W-1 2-19-58 0.001 0.008 U-2 11-19-58 12-12-58 0.009 0.002 G*
U-3 3-20-59 4-14-59 0.002 U-4 6-26-59 C-- 3-59 0'.C01 ?413 U-1 8-36-58 11-2"-58 0.009 0.005 W-2 5-18-59 C-29-59 0.017 E-3 7-27-59 C-20-59 0 #06
(G-cmumi vat = cupply) 30
Tfi'.T J : V _{g, g'M y m/,flCE CoII: fry De ' t: lione Sor:plc Data Dato Grona Data S%kers __g c/_g3 grbl ilm-b;;g CM i cct.v1 E;rimined 2 4?10 W-1 3E1-58 12-0-58 0.026 0.006 U-2 5-18-59 6-29-59 0.013 'i-3 7-29-59 8-20-59 0.005 4310 U-l 10- 9-58 11-28-58 0.004 t 0.005 U-2 4-10-59 5-2-59 0.034 U-3 7-21-59 8-16-59 0.005 i 4311 U-1 1-19-59 1-29-59 0.015 t 0.C0 U-2 3-12-59 4-14 -59 0.014 il-3 4-15-59 5-11-59. 0.006 W-4 7-21-59 Ca20-59 0.004 4312' U-1 0-18-58 11-2C-58 0.008 i 0.: 35 U-2 5-10-59 6-29-59 0.011 U-3 7-29-59 L20-59 0.006 4313 U-l C-21-58 11-2F-58 0.008 i 0.005 W-2 5-17-59 6-29-59 0.064 W-3 7-29-59 E-20-59 0.C08 4314 U-1 S-13-56 10-25-58 0.009 0.002 U-2 5-1S-59 6-29-59 0.017 W-3 7-29-59 8-20-59 0.006 4315 W-1 1-26-59 2-16-59 0.025
0.002 U-2 3-19-59 4-14-59 0.034 W-3 7-22-59 E-16 -59 0.006
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G 4411 U-1 1-19-59 1-29 ',9 0.014 i 0.C02 U-2 4-15-59 5-11 '9 0.017 W-3 7-21-59 0-20-59 0.010 4412 U-1 0-13-58 10-26-58 0.007 i 0.002 Y-2 5-Id-59 6-29-59 0.017 M-3 7-29-59 C-20-59 0.005 4413 t!-1 1-26-59
?-13-59 0.001 0.001 W-2 3-17-59 4-1!.-59 0.000
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(G-cround mter supply) 31
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-TNilf:_Vf UpIYMiilIVI:ll1A"I'im tril(!-l Afirrof!. P1:lli. tJATI'It At Crot.nn Point Dota-Dono Bo ta-Don.' Gronn Date Dato .Ucchcro Cechcra T :ta Typn On-,1n D, nth-ft. Cc.11ce tm] Cottntod ppc/m _ppe/r 1 ,itpc / 1 1hd 23'(f12 Bou 9-4-58 9-22-59 4 10 f(!!-Cove)y) 4 10' 5-25-59 9 30' 5 Plankton 9-4-58 9-22-59 20 10' 5-25-59 30 Fish crth Cove 9-4-58 9-22-59 0.7 5-25-59 0.9 Water 12 ' in 23 ' 9-4-58 12-12-58 0.038 6 ' i n 10 ' 9-4-58 0.025 0.5' 4 7-59 6-22-59 0.012 ) 15 ' in 30 ' 5-25-59 6-29-59 0.006 6' in 10' 5-25-59 6-29-59 0.005 0.5' 6-10-59 7-15-59 0.007 At f+ nitnu Bench !bd 5 9-4-58 9-22-59 5 80 4 5-25-59 39 9-27-59 52 Plankton 10-4-58 9-22-59 16 75 5-25-59 26 Fish 9-14-59 9-22-59' 1.0 5-25-59 1.0 River Unter 50 in 50 9-5-58 12-12-58 0.019 33
' tiliF, V TI f fffftCnil it iVM:t %Ttt R*' *tlittf. L 1%Tf.D f4Y 't.:1. I'.fl.!;. /.T I.ls. '. Pl i.T. POM!KI:'.1:: TE Dato Dato ~ Gro s Thta Cnimt - mig /r.1 Sollected Ceunted Suc.nnnded i nnoly.cd_ Tot 1 h D 6-9-58 6'16-58 6-16-58 6-20-58 0.007 0.021 0.028 0.002 0.025 0.027 6-23-58 6-30-58 0.004 0.002 0.006 6-30-58 7-9-58 0.009 0.024 0.013 7-7-58 7-11-58 0.001 0.008
0. 0. ' 9 7-14-58 7-23-58 0.003 0.m n 0,013 7.21-58 E-1-58 0.000 0.004 0.004 L
7-2 E-38 E-7-58 0.004 0.087 0.091 8-11-58 E-20-58 0.001 0.014 0.015 E-18-58 E-29-58 0.000 0.009 0.009 g 8-25-58 9-2-58 "0.005 0.028 0.033. 9-2-58 9-11-58 0.006 0.017 0.017 9-8-58 9-16-58 0.002 0.'016 0.018 10- 6-58 10-15-58 0.002 0.021 0.023 10-20-58 10-2C-58 0.000 0.010 0.010 10-27-58 1-5-53 0.017 0.054 0.071 11-3-58 11-14-58 0.156 0.100 0.256 11-26-58 0.110 0.075 0.185 12-2-58 0.103 0.073 0.176 12 -58 0.089 0.0 73 0.162 12-16-58 0.075 0.0/A 0.121 11-10-58 11-21-58 0.033 0.044 0.057 11-17-58 11-J-58 0.003 0.033 0.036 11-24-58 12-9-58 0.027 0.028 0.055 12-1-58 7-12-58 0.005 0.015 0.020 12-E-58 12-23-58 0.046 0.021 0.067 12-15-58 12-24-58 0.008 0.022 0.030 12-22-58 1 59 0.004 0.032 0.03 6 12-29-58 1-14-59 0.008 0.016 0.024 1-5-59 1-22-59 0.000 0.008 0.008 1-1;:-59 ~1-20-59 0.001 0.019 0.020 1-21-59 2-?- 59 0.000 0.010 0.010 1-28-59 2-11-59 0.033 0.066 0.099 P- /. -5 9 2-l'*-5 9 0.177 0.085 0.262 2-9-59 2-27-59 0.051 0.04 9 0.300 2-16-59 3-5-59 0.029 0.046 0.075 2-?5-59 3-11-54 0.r/,4 0.066 0.110 3-4-5') 3-16-59 0.036 0.069 0.107 3-9-59 3-20-59 0.0/,4 0.056 0.100 3-16-59 3-27-59 0.068 0.009 0.157 3-25-59 4-3-59 0.079 0.093 0.172 4-1-59 4-13-59 0.016 0.034 0.050 4- (,-59 4-20-59 0.036 0.043 0.079 4-13-59 4-27-59 0.026 0.078 0.104 /.-20-59 !.-30-59 0,076 0.021 0.097 34
~. 6 Tr.lti,{}. VTT ("on't) ~ I liflD;IfW RTV:dil '!/iT::li it.'.;;:ll..; P!;1MITrn UT 'l:)'all.0. 1.T 3.It. ? !. ILI.:JIT, WT)G"l;:l;. TG l a Dato Dato g/y,1 - B, O mg E ".".I d Co+ m t< il 9iins.ninct pinao yl,d Tn+n1 /.-27-59 5-12-59, 0.006 0.009 0.015 5-6-59 5-21-59 0.000-0.000 0.000 5-13-59 5-25-59 0.118 0.143 0.261 j 5-20-59 6-1-59 0.0J/ 0.034 0.041 5-27-59 6-1-59 0.043 0.030 0.073 6-1-59 6-16-59 0.017 0.049 0.066 1 6-F-59 6-19-59 0.005 0.009 0.014 6-15-59 7-7r-59 0.010 0.029 0.03 9 6-22-59 7-9-59 0.C07 0.052 0.059 6-29-59 7-12-59 0.000 0.001 0.001 7-6-59 8-6-59 0.015 0.003 0.01 8 7-13-59 8-7-59 0.000 0.009 0.009 7-20-59 8-7-59 0.007 O. col 0.008 3 7-29-59 P-10-59 0.002 0.009 0.011 F-5-59 E-11-59 0.006 0.016 0.032 E-12-59 E-20-59 0.C04 0.0; 3 0.022 C-19-59 S-31-59 0.000 0.000 0.000 G-26-59 9-3-59 0.012 0.005 0.017 9-9-59 9-21-59 0.003 0.011 0.014 1 9-2?-59 10- 5-59 0.001
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i FIGURE I AIR, FALLOUT, V...GETATION, and V!ATER GrOns Beta cod Oc.a Bono Scohors BY THREE t.'r3MTH PERIODS FROM JUNE 350 i g i,, a r < r r a,,,,,,,,,, a r - a i r r a rr r r r i r i s i s e s < < i, y
59 -
AIR (5 Stations) Gross Deto 2 j u !>>>>>>,,,,rririr>>>rri pp c/ cu. m. f f e i f i 1 O I 2 3 4 5 6 ,d,,, c.~rrrn rii ,,,,<<<<iaz. ,. i 1,111 i r i i i s i i i i i i i i i i s, u i i r i u i i s i in 4 FALLOUT / Gross' Beto (6 Stations) f f 7 ,59 - ,ul''''''' Bato Banc Scchcts 2 pJi c / 3q.f t./ day L f f i e l-1 O 150 300 450 600 750 gehy 'IiiEiIf ' ;3. ~3 ~~ / i/J ! I i///I' 'i ~ 4 VEGETA'.lON U 2 I" CCUU OUU!CIU f T (45 Stations) e 1 11_i f_ / / / / 1 f ] t 1 / / / 1 1 / / /1 1J f r ?_ / r i t r_t r o o r t s 1 1 t ' jty C / gm L t e f a l 0 25 50 75 (00 t //// / / I!!I istii11 // ///// f / SUSEACE Y/bIEO / / / / / i i i / / / / / / / / ' / / / i i <' Gross 00to ff11ill) 'gg _2./ ( <?! Stationc) _h_ l [ /_u./. 'J.> / / / r e Octo Cono S0chers >> ! !! LLU.LLLU t f I / U.UJ.J.LU p)1 C / mi b _L_ l _-._1 I O .003 .010 .013 .020 .G3 3 030M:lD V!".TEi! T / /rrirr rcc - C :io 4 L:T.EllD /rrti r\\. '59 (15 Sicilca') a m ::.;.- '53-3 AljG,02P,CCT /'- p p c / :.:1 ^ ';3., i:OV,C2C,J.^.) ~~ ~ b U!.J 'CD-1 FEU,t.).'.::,T"a 'g < _. a t.:J.Y, J U :!, J U L g l>
-i i t) R (20) FALLOUT 9 300 g
,,v,,,,,,,,
' '.:. '4 l
2.
e s s____; ,,,,,,,,,,,,,s,' l -200 g El I e i s 8 I , a i i i i,, i < <, E --J LEGEND / -10 0 s o Average of Camp Smith, Pockskill, $____ __ _) i Oasining, Stony Pt., Hoverstrow, '77<<,,,,,, I 2 d and Echo Loko --- Albany '5 5 7, D J O JAN FEB f.1Al1 APR MAY JUN JUL FIGURES 2a and 2b i FALLOUT cad /ua (Grc33 Co?a and Octa Scno Scchors ) CO:.i3OLID.TTED FD;SCM STATIOMS cad ALCANY (F m Jan'59) 9 _g 4 ,t /t (2b) GCOSS EITA \\ It /\\ / / \\ / \\ ACTIVITY OF / b \\l \\ ~ I -7 1 /\\ / v i PARTICU LATES / 1 \\l \\ \\ \\ IN AIR d -6 f\\ / I/ ) \\ \\l 0 I \\ l \\' N i \\, -S \\ u
s.
~ /\\ ~. \\/\\ -4 \\ .2 \\ LEGEi!D \\ ,si a \\ fl A:::.: : ci P.:. ' :lli, C.rining, To::cdo, s s 2.) -2 f.: :liac, cat! To..);tiac C;vo \\' \\., 'N / \\ --- Albc.1y ( U.'. l1J i' x!;c) s \\ -l \\,,- L __.--I i i N.:1 17:.:J f.;.:
/..'.Y JU. I JUL
e c U.o.m-3 i m FALLnU i ( C...o ~ r, r...a .,,! n e _, C,,, e,,.. ~.... eJ s t.i m. ...-ma.... - CONSOLIDATED EDiSC?! GTETIC:'.3 !9:D STAT 21!iDZ CITi3S R om Oct.1533 1000 I I M ~ / ~ ~ / i 5'J) / / / j'M O ) vg a a 1-n r'rrr a f 'Ii iI T' d / f A-a y aa aeer, ) t I- - T r- - - i / L _ _J t__j j -- 3 6e iI i! / 100 / ) / / ~ Ii liff / 50 j / ~ / s / / LEGEND / i, < <,,, Avercy of 'omp Emith, Pcohchill, L___./ Occining,Gicn."i., Mcvorciravi, /, j and Echo Lohn j 10, ~ ~ ~ ~ A./crcco of Albany, C!achamton, Loc' : ort, j"" Plottsburg, Schenectady, C Sy.ccuca I N5 Cross Cota C0to E'ano Sach're a 6) N o*( -g J i a i i I OCT NOV DZC l.'TN FED t.1^.;; f '. i.'...'/ JUN D AUG 1C33 1:uD
o c FIGUI'E 4a ~ DETA DONE SEEKER ACTlVITY / LBANY TREATED WATER - FrOm July 1958 .01 ] .000 ~ f W. a I E ~ o
n A
J L- ,o g; _ AUr, i SCP-OCT, fl0V-DEC. JAN-FED. fiAR-A'3R, MAY jtIM,.1UJ.- o'JP i i r. r; il FIGU..E 4b 1 l ^ I :' 11 BETA BOME SEEKER ACTF '!TY' i .C s - I m 3 I !.y 1 HUDSON cad MC:U.'#K RNLM WATER l I i, \\ a ~ i From Jan 1959 ~ i: g e I:
1' l's -
sl 11 c \\f, t i <\\. * \\ cd .\\ 1 1 \\ li V. s g.i ,'[k,5!' l Ie I '.s ~ \\ I 'Oi !- ',/ t / ,j ^ \\_. / LEG _ EtID
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s g .005- -- Gl:nment (!!udon R.-S.of f thony) ', i Viaterford (M2dson R.-N. of and ~ above Mchowh R. confluence) --- Cohoca ( Mohorth R. '//. of and abova i,1 ~ Hudson R. conflucree ) (/ .0 01-t i i i i i i JAN-FED MAR ~APH MAY-JUN JU'. AUG SEP-0CT s
r i i FIGURE. 5 GROSS BETA ACTIVITY HUDSCN RIVER V/KIER AT POUGHl(EEPCIE FROM JULY 1958 ' i US?HS ANALYSIS 3 ~ ~ 1 03 l I N o gC1-g-/ } \\/ 1 2 \\ ~ ~ 3 03 Ua { ~ g is 1 .01 i i .005 \\ 'k
==. - ! .0 01 1 8 JUL-AUG SEP 0CT NOV-DEC JAN-FED MAR-APR MAY-JUN JUL-AUG 1950 1959 f
Di n. ur.ni nn or Rx_ul t2 b In evaluating the recults containe.d in this report, it is apparent that fission products in the atmocphero as a result of nuclear weapons testing contributo a larCe portion of the r;dioactivity found in all surfaco camples. As an overall p.eans of comparison, Figure 1 has been prepared which graphically illustrates the aver:ge results for three menth increments for air, fallout, unter and vcGetative samples. The caries of nuclear weapons tests in October of 1958 account for the marked increr in the radioactivity of samples collected during the fourth period of 1953 and the first period of 1959. The decline of radioactivity in the cceend period of 1959 is a recult of cessatien of weepens testing. Data now being co11cated, but not included in this report, shew a further decline to the l' point w'ere it is becening difficult to detect the low levels of radioaativity 1 present. A nore careful analysis of the data indicates high levcis of activity in the latter part of October and c: 'ly Novenber of 1956 uith c:me decline in Decer.ber 1958 an early January 1959. About nid-Emunry, an increcsing trend in radioactivity was noted. About this same tico, I 31 l was found in rabbit thyroids although previous th:, cid sonples indicated no [ 31 Becauce of the lack of informaticn concerning the amounts of,.or behavior of ficsion prcducts deposited in the ctratocphere from weapons tectin;, it is difficult to accesa tho variatienc noted in resulta Letween October 1958 and the Spring of 1959. Air Cor.parison of the data obtained at the d.erent air campling locations indic..tes no cignificant differences Letueen the stations. The 41 s
~ n raco results of the fico dr empling ntat.iona chou a high valuo or 7.0 micro nicrocuries por cubic noter "or the latter part of April 1959 and a low value of 0,5 during the latter part of July 1999. Figure 2b graphically illustrates the average values for the fivo ctations and for the wechly averages of the l'nited Stntes Public Health Service reaults at Albany. Doth plottings follow each othc/ closely. Fallout results have also been plotted in Figuro 2a for comparison purpcses. Since radon and thoron daughters were not being measured,.n, conclusions can be nado as to the natural radioactivity in the air at the sampling stations. It does appear, however, that thero will be no significant difference betueen senpling stations for fission product contaminaticn originating from nuclear.wcapons testing. F-11out Figure 3 cenpares the average nonthly values of fallout at the six sanglir.g LLations with the riverage results of fallout fron six cities lecated in varicus geographical arans of the Stato. A tabular conparison has also been made in Table II B. The amount and frequency of precipi;ation, heavy snoufall, and differences totucen time of sanpling and counting are sone facte s uhich influence the results. Considering these factors, there nppears to be no apprec$ able difference between the results of fallout obtained in the Lower Hudson Valley and other areas in Neu York State on the basis of sampling for relatively long periods of time. Sono variations, uithin relatively short canpling periods have been noted and continuation of a limited nunber of stations is desirablo, Rebb4 t Thyroids The only sanples chouing 1131 were 4 samples collected in the latter half of January 1959. This coincided uith an increase of racioactivity in air, Hudnon River water and fallout. 42 e /
~ h of.nt.lon Reference la mento to Fir,oro 1 for a comp:n imn or ":.ul tn of vegetativo rmmples. 't he r u.ulto are niedlar to other t.ypec of c,mplen in th tt they reflect the influence of nuclear weaponc cesting and sub..cquent concation of theco terta. An import nt factor wbich doec not mke for a Cood valid comparicon is the long tic.o between c. Icetion.nd ccunt. int;. for thoco canplea collected in 1958 It would appear that more frequent s:u.pling of vecetation f"on the sane arca will give a better indication of the influence of fallout, thter The craphical cenparis n of Figure 1 clearly indicates the influence of fallout fron nuclear bonb tests on curface water canples. The ground water rc.;ults, as would be enpected, do not chow this influence. l Except for the Hudcon River, nost of the surface water canples come fren lakes or recorvoirs of various inpounding capacities. Results of grocs beta on Hudacn River water at Feuchkeepri.e 1 are plotted in Figure 5. Becauco cf direct : an-off, cne treuld expect a fairly ir.: :diate rise of rad] activity in the water follouin;; a heavy fallout. The Ceneral trend of a rice in rr.licactivity in early Fovenber 1958 folletred by a decline in Dececber 1958 and a subsequent riso a;;ain in the latter part of hnuary 1959 was apparent. The radicactivity alco renained seneuhat olevated as late as the end of th:,1959. Ficuro ha chcus beta bone seeker results on Albany treated rater. This has been presented becau.ic it is the only water cupply on 1:hich the teta bene seeker nnalycis was n.ede previous to 1959. The effect of fauout is conciderably dampened because of the riorace capacity of the Alcove Rect cvoir. Thic supply is locnted approximtely 15 miles couthwest of Albany. Ficut 5b chow: typical beta bone cceker recults of waters of the h)
!!oltwk anil... inon Rivern in the Anany Are t. Ar, for t.hn thul::on 11 ver.tt. Poughlwep::io, t.ho re::ulta did not nt.trt a :mbstantia_1 Icc11no until iby of 197). b %n itivor 0,rgTg To dato there has not been cufficient d:ita ebtained on r.ud, plankton and fich cumples to draw any conclusions as to how fallout nicht influence the resulta. The informatien given in Tablo VI will, of cour:c, be of value in future canIding. The !!udson River water nar.ples reported in tap.e VI are in general agreement with results reported by the United States Public IIcalth Scr'vice at Pouchkeepsie. ) Igly
I 9 A PTY.H1 0 X A ('t'ivi.TD ATi'D i'D T:WI l'tM Ol*'IGT TGIAT. ::f f4VRY CAMi'i.it:0 GTATT0l"SW i. fly --l i l U..rtchesterjRockland l Putnars Orange I Tctn1 i t C nnty County l County l County 'all Cona*,1cn i Carling ' 3 Par i ed.1.tn.. 'i...m.. _. int,.. :h.._na..q,8 ph.. 3 rrn, S,t, i..{ gen,; S tm n. L-m i. Itm n 7 Ac 3-% 59 l 2 46 1 17 1 13 5" 89" i to u 7-30-59 ' ?~ l i j 'Fellout 10-9-58 i 3 64 '2 47 I 1 16 6 127 J,.' i ~r to g I a 1 9-29-59 Echbits 9.8-58 1 14 20 l9 10 2 4 13 4 27 38 i to i l 9-8-59 l i t 1 10-58 j 31 124 9 35 1 3 6 3 6 46 171 ,p
Soil 4
t I e j/ to 4 9-10-59 o 1 I I i i 6-30-58 31 123 9 30 i3 5 l3 4' s :'{ 46 162 i
V.re-to t
i fs ltatien l 9-12-59 I i-I W l
~
,Unter to 4 i 15: 52 js 'Cround 8-12-58 ' 3 12 10 36 l2 W i 7-29-59 l I S irSco. 8-12-58;24 8 24 9 28 41 148 '?ater i to l i j l7-29-59I l Sr cen R.I I l j 4 Fi::h 9-4-5B l1 2 1 2 2 4 l to j 5-25-59 ; I I l l i ! !bl 4-58 i 1 4 1 4 I 2 8 l to s j ! 5-25-59 ! l I I l i F1:,nktva 9-4-58 1 2 1 2 2 4_ l to j 5-2!-59. i i l i I 3 hter 9-4-58 to l (- 10-59 ' 1 6 1 1 2 7 l i 2. 'Inclu ba.13 n!r cunplen from 1 canplina station in Dutchoss County 4'$
e /I FilfrIX A ([gd1 f.,,NPIE :'T/,'[i CI $Y s All stath n noil,cru wJll ecnaint c ' four di;;Jta: The thouncnda <lf git utll,refei to the county or crecini rarca in vLich the station in located. T".000htDS CCUNTY CR LOCATION 1 Uuctchester County 2_ Rockland County 3_ Putnam County 4_ Orange C.'inty 5.__ Above alto en 1:udson 6_ _ _ Balcw cite en Hudson 7_ Special simples + -Tv o h*rt cds sly,it uill refer to apecific di::tance acetors from the site. 0.__ _ w'1: te,steticna within 2 miles. c __1 between 2 cn3 4 miles. 4 and 6 miles. 2 _._3_._ 6 and 10 miles. __4__ 10 and 20 milca. The t<>ns & units digits will be arbitrarily assigicd to stationc within the c cific county on1 distance.metors in order to distinguish Individual stations. Th.;a, an exampics, tl:c sta'icn at Camp Smith will be nunbered: 1101 The firnt arbitrary etntion # Ucstchester County s
>2 mi.
at this distance in Vect. Co. ( 4 mi. .t'nd th7 station at Pookakill vill bo Wentchouter Ceunty 1102 Second nrbitrary ctation # 2 mi.'
4 ni.
New Croton Racervoir: Ucotchentor Ccunty I?O2 Seccnd staticn In area j
4 mi.
Is(> _i
m glTEMI)TX _ A _ f *nntl nned Urntebder Cmmty Station _ tit"d2. Inm:i6Fl" filrv - U"Sc"I ilSH L I JI rber 1301 L1 -18'-10" 75 -50'-45" 445' Mohegan Lake in 0 V, SU, S southwest area 1302 A,V,SW,S 41 -15'-00" 73 -50'-10" 220' Sarnoff residence 0 located on llunter Rd. ~ 'ast of Croton huservoir 4 1303 V, UJ, S 41 -13'-00" 73 -51'-45" 320' tiewbury Pond at 0 intercection of f Ossining Rd. and Otmker Ridge hoad 1304 V, N, S 410-17'-C0" 73 -48r-30" 460' Lake Mchannic at 0 south end uhcro Mohancic Ave crosses the lako 1305 V, :P.1, 3 41 -15'-10" 73 -45'-15" 170' Croton Rerervoir at intersection of Toconic ParLvay and i Hunterville Dan Read 1306 73 -48'-10" 420J Lako Osecola at north 0 V, UJ, S 41'-20'-10" shoro 1307 A, F, V, S'cl, S 41 -11'-30" 73 -51'-50" 220' Iulian Brook Recora 0 voir at south enat end 1308 V, GJ, S 41 -20'-00" 730-50'-00" 420' Chrub Cak UcIla north of Jeffercon Valley Ikl. and weat of the high cchool 1309 V, N, 3 410-18'-30" 73"-47'-10" 500' Spark 1c lake at north eact end 40
t P gis:'OtX_ A. f:c3,'.hir.cJ ',l %: t.e li ::I r Pgpiit.y Stat r on I 3;gt Tj;t.i t.sylo pn
i.o.!g,
- [1.C.L. I:ltriid hD. l 1 L: U10 V, S'i, S 41 -118-15" 730-48'-15" 340' Echo Lake ut north-ond i 1401
f., V ' W, S 41 178-15" 73 -45'-30" 400' A.a>alk R o:.rvoir at l
couthee.nt end. 1402 A, V, SW, S 41 -14'-50" 73 -45'-15" 170' Croton Lek.. r. rth of 0 Lakeside Ee.ti und east 1 of laurelten Po> d - 1/.03 l A, V, G, 41 -11'-15" 730-44'-10" 280' Mo'mt Kisce Country _ l CLJb near catrance l s 1404 I V, G.7, S 41 -03'-00" 73 -48'-30" 240' Bricr liff "sner v! ells Diatrict - o.1 cc:st of i-well #3 .~! 1405 l V, SW, S 41 -19'-30" 73 -40'-00" 270'- Lake Purdr at south 0 cnd. 1406 V, SW, S 41o_17 -00" 73 J.388-45" 330' Lake Stenah at north! end j 1407 V, dd, S 41 -13'-15" 73 -40'-00" 320' Pond on httheus 11111 ] Ro.d t'.;cr+h end i 3408 V, SW, S 41 -09'-15" 73 -41'-30" 455' P;/rs: LcP-Fep IIouco 0 1409 V, ; 4, S 41 -07'-30" 73 -45'-00" 320' Wippcorwill lake' c 1410 i' ( V, Ud, S. 41 -17'-45" 73 -35'-00" 465' WaceaLuc Lake i .1411 ( - V, S, 41 -19'-10" 73 - 35'-30" 440' b rd Pcn1 R4! O E C I Eucervoir: 4 c L 1412 i V, UJ, S 45 -12'-00" 73 -35' 45" 480' Bluo Iferc.n t.ako near i. coutheast chorn line i, 49 l' t I< f, .J! + 6i
3PWi!D1X A ContitMel [h g1Q nl ('<unk Statlon O.03 E,I P[;.I.CD, (! q nl.,,- IitIt.wld Init" I f.'FI& IjjfL 2fX11 0 V, S 41 -16'-5G" 73 -57 '-!.0" 10' Dun <1enburg Moun' in at Jonen l'oint near abandon uchool 2002 A,F,V,S, 41 -15'-1)" 73 -598-34" 300' Euckburg "chool l t 2003 A 41 -15'-30" 73 -5?,8-45" 50' Roor or Cranco - 0 Focklar.d Utilition, I Lovett Plt.nt, Tonkins Cove. l 2101 A, V, S 41 -17'-56" 73 -59'-30" 310' Deodletv..n School 0 2102 V,3 41 -.14'-55" 73 -598-54" 260' 0.Occut C:m.p Bullowa c t Fancer's Horr.e 2103 V, S 41 -13'-50" 73'-59'-21" 180' North of HauM 210 6t intercoctton of* Jay 6t. cnd Orchard S. t 2110 0 G, .4 410-178-55" 74 -00r-15" 500' Iona Iolund Infiltration. Gallerien located near Doodletown P.W.S 2201 V, S, 41 -13'-10" 74 -01'-31" 420' Intersection of Willow Crovo Ed. and Lotchworth 101. at fl.Z.S. D toh.iorth Mental li.scrital i 2202 A, t', V, S /f -12'-Go" 73 -58'-00" C0' Haveratraw liigh o hool c 50
4 Al'IV. tile 1X A c...di g 4 4 I f ockton<l (but.y (Con't), j Ut.ation ibtrier ! d.1 ht.lo Dr1 turla F,jfqy, l'<vrqdt la c 2'!O4 A 41 -18'-40" 73 -59'-00" 2180' Palisadou Stato Park l' Adm. Duilding y i' h 2210 GI 41 -12'-35" 71 -00'-40" 320' N.Y. Water dervice- -f doll at Thiclls P.W.3. j-4 2211 1 G4 41 -12'-25" 73 -59'-25" 200' N.Y. '.iater Serv. ice. Woll at Garnerville-P.W.S. t 2212 SW 410-14'-30" '74 -01'-30" 220' N.Y. Water Service j o Ecocevcir et Rt. 210-P.U..;. i 2213 Gl 41 -12'-50" 73.-59'-10" 145' Gvnervillo Holding i Co. Well' P.H.S. j 1 3 2301 i A,V,S, 41c_11 -55" 74 -03'-45" 200' Call's-Hallow Road $n town of Haver-s'traw. j. ? 2302 1 V, S 41'-08'-50" 73 -55'-47" 180' Eact new York v.vo. 'l and south of Iske PA. 1 2310 SW 41 -12'-55" 74 -03'-30" 680' Intcivorth Villago-i- Recorvoir P.W.S. t i 2311 ' G.1 41"-11'-00" 71 -00'-20" 140' Wolla n.mr Luke Lue!11o !!achen9ack Water Co. P.W.C. j 2312 i 74 -01'-55" 225' Sum-it Park Lab. 0 0 Gi 41 -10'-15" Spring Valley Wo113,Worku, P.W.S. Water i 5 t l 51 i l c \\ 1 1-i.. s - -. -. -.. ~., -. - -.,, _, -L. .,--...e-v--.r, 7~ c.,, _-,,,.. ~, -,.. _, _,
API'dNDIX A _ tin ilni, tad (con't) Hnnk b,ryj, Cmne r S t.nt ion grim To ti t n,Jp_ Lovi ttvlo ljlm. Nrcrintloa 2313 41 -10'-00" '74 03'-40" 500' Hillaidc Ntatcc Well 0 C'.i Soring Vn11ey Water Workc, P.H.S. ~ 2314 220' Conger Realty Corp.' 0 C1 41 -07'-50" 73 -56'-15" Well, P.W.S. l 2315 SW 41 -12 8 35n 74o.,: -35" 10838 Break:wek Lako 0 F.W.S. P. J.. P. 2316 l SW 41"- 13'-40" 74 -04'-25" 1000' Lake Welch j P.*.S. P.I.P. i 2317 S4 41 - 08'-30" 73 _ 55'-30" 1608 Rockland Lake [ l' 2318 0 SW 41 -11'-00" 71 -00'-20" 140' Lako~ Lucille l 2319 I C SW 41 -08'-15" 73 -568-20" It 38 Congers Lake 1 2410 Cl 41"- 07'-40" 74"-05'-20" 600' W3 faro Ho.mo W11 Spring Valley Water Works, P.'.4.S. l-2411 S",1 ' 41 -06'-30" 73 -58'-00" S08 Lake DoForcet et Congers HacFc r,uck i Water Co., P.W.S. 2412 CW 41 -07'-20" 73 -56'-50" E0 ' Fullo Water Supply P.W.S. 1 2413 bW 41 -12'-55" 74 -07'-50" 'r/28 Sebago Lako P.W.S., P. l. P. " P.I.P.-Palis.ido' Int ratuto Park P.W.S.-Public Water Supply i 52 l .i 1
fI':Y.NulK,.,6 Cq.11ngd Iht nc-Cmmtg ^ Strtlen p n-Iv.t-I.n t. (p.,1n ym 1 f.udo Flav. Deom Int. ion 3?01 0 V, S, 41 -20'-20" 73 -53'-05" 280' Lake P'okakill roar of Corialo re.;ldenco 3302 l t., V, S 41 -21'-40" 73'-52'-10" 500 O.3 milen south of I Craft Corners, east j' side of Oscavana Lake Road at Ground Ob- 'I cerver Corp. Station 3401 V,~S 1 -20'-50" 73 -45'-15" 620'- Baldvin Flece Rail-read Statica ,0; c.3 Coanty j 4203 V, S 410-19'-30" 73 -598-25" 140' Intersecti:.n of Ft. MontConary Road and Route 97 4210 l i SU 41 -19'-40" 74 -01'-30" 460' Lako Quc-.; boro l P.W.S., P.I.P. i i 4301 F, V, 'I 410-16'-15" 75 -08'-10" 710' Echo Lake l 4302 V, S 41 -19'-15" 74 -5'-15" 960' Intoracction of " cutes 293 and 6 f. i 4310 j 41 -16'-7.0" 74 -00'-20" 709' Echo Lake, P.U.S. SU i i 4311 SW 41 -22'-35" 73 -59'-10" 560' Highland Fells, P.U.S. l 4312 f' 74 -03'-30"- 720' Silver Mine Lake 0 SW 410-17'-40" P.U.S., ?.I.P. i l / '13 - i Al 41 -18'-50" 740-05'-40" 1C67' Sumi t I<ito, P.W A.,. P.I.P. ~ 4314 SW 41 -16'-30" 74 -05'-20" 1032' Iake Tlorati, P.U.S. t P.I.P. 53
g lEMintX A ibutt p d I Utntlon I guahs Intibylo im Ibulo li] m Dmier 1 r ti en r: 4315 SW 41 -24'-25" 74*-C0'-55" 1000' Alce lfendow Ecaervoir F P.V.S. I 4401 A 41 -14'-15" 74 -128-42" 700 North westerly cide b of Long Su tmp Road I-approximetely mile south of Route 17A l i 4410 1 0 GW 41 -18'-40" 74 -08'-45" 540' Harriman Water Supply P.W.S. 4 i 4411 SW 41 -20'-45" 74 -08'-45" 743' Town Woodbury c well Lake, P.j rom-J.S. i 4412 SW 41 -14'-00" 74 -09'-50" 715' . Lake Stahahe, P.W.S., P.I.P. 4413 0 G4 41 -21'-15" 74 -08'-00" 800' Skyline ' trails Well j Supply, Highland j Mills -7501 l A 41 -35'-36" 73 -38'-57" 7608 Genierator Building of 0 N.D.A. Experimental j Laberatories north of i the intersection of routes 55 and 216 RAPBTT KTIL TU:ATTONS i 0 1030 41 -16'-00" 73 -56'-00" 20' South of Peekskill, N.E. of Duchonan i C 1031 41 -15'-45" 73 -57'-40" 100'
3. of Indian Point, H. of Verpl uck
^ 1032 410-15'-30" 73 -56'-20" 120' W. of Routo 9, N. of Montroso 1033 41 -15'-00" 73 -56'-00" 120' W. or Routo 9, S. of Mcntrono i $N .,-.e,- n--
~g;g.gg 3, egg,,3 Rid h.it Kl.11_ImnMuna, Wri't) Utntion gn[,,n Lnti g Ingstitwin Um pqnqt' pt icri 1130 41 -18'-30" 73 -56'-40"- 150' Corap Cm1th ? 1131 41 -17'-45" 73 -53'-00" 380' Dent Mt. Par kvay none Incust Av.nuo 1132 41 -18'-00" 73 -548-20" 4001 Bear Mt.' Parkway vest of Locust Avenue 1230 41 -19'-15" 73 -53'-00" 200' N.E. of Van Cortland-ville 1231 41 -13'-30" 73 -53'-20" 300' E. of Route 9, S. of Furnace Road 0 73 -54'-00" 300' N. of Peekskill 12.32 41 -188-00" Hallow Creek, W. of Cotskill Ac.uaduct 1233 410-17'-30" 73 -51'-00" 320' Dear Mt. Parkway near i road to !bheCan Lake l 1234' 41 -19'-45" 73 -52'-20" 200' S. of Putn n County, l g Ucstehester County Line, E. of Road to Putnan Valley 1330 41 -11'-00" 730-54'-00" 408 Croton Point Park i 1332 410-20-15" 73 -47'-20" 480' Route 6 cast of Reute i
61I, 2130 41 -13'-00" 73 -58'-20" 10' S.V. of Graasy Point 0
2131 41 -1/'-30" 73 -59'-40" 500' Pold :cdes P"rk, S. of Doodletown 2132 41 -18'-15" 73 -59'-20" 350' Palisades Paric, N.E. of Doodletown 2230 41 -13'-00" 74 -00'-00" 2008 W. of Wert Haver-0 0 straw, S. Willev Grove Road 2330 41 -08'-30" 74 -02'-00" 5408 E. of Route 45, S. of New IIc:npatend Road 0 2331 41 -11'-30" 74 -02'-00" 4208 N.E. c,0 Mount Ivy I ,55 e 6
s_ e. ~ p]T"?T!])f Contingd !!nlihIt VJ11 focationo Statien !Fi".he_r.,, Int i ttuj.2. lent itudn Elev. Dn.g r int 1on 2332 410-10'-30" 740-04'-00" 480' Route 306 N. of Pomona lloights 2333 41 -08'-45" 73 ~59'-00" 200' N.E. of Now City, W. of Browery Rond 1 2334 41 -10'-00" 73*-59'-20" 1408 S.E. of Int. of Route 304 and Zuror Road 3330 41 -22'-00" 730-54'-30" 700' E, of Routo 9 an1 S. of Fort Defiance Ilill 3331 41 -21'-00" 73 -51'-00" 400' S.W. of Int. of Krar. ors Road nad Church Road j-1 4330 41 -20'-30" 74 -06'-00" 700' E er C1ove Road, W. j of Lake rrederick ~ 4331 41 -21'-45" 74 -05'-00" 600' S. of Mineral Spring i Ercok, W. ' of Popo-4 lopen Lake 3 4332 4 ' -19 '-30" 74 -07'-20" 500' W. of Thruvoy, E. of [ Route 6, S. of Central Valley l! I' l l l e J 4 I i l I l r 56 i i i L
LI'IT"! dix D Dlvl::.lon of "~hort. tor kn nnd Rosenrch fl..w *iork O f '.t.. D.:litirl.m..n t, of II.. nit,h Du tt rmimit lon of I'. r.o -r..oh t og Ifwl !.1;i..l.iii.ori ln Hilk Tho cbjectivo of this proepduro in to preparo for low bcekground beta counting the bono-cooking activities including ctrent!um, celefum, barium, yttrinn, and lanthanum. Theso aro l carbonatos and exides prior to counting. No attempt is mado to 'j precipitatc<1 as a goup in the form of oralates und ignited to scparato individual isotopos frorr tho group. Reagents: l 1. HNO cene. (ACS g ade). 3 2. Strontium-yttrium carrier solution. To a mixtura of 12.7 grams of I 023 (A.D.?hekay,Inc. How York, 99.9% pure) water, 50 nl. of conc.7 6H O (AC$ grado), add 500 ml. of and 30.4 cruEs of SrC1 2 j 1101 and heat to dissolvo. Cool i and make up to 1 liter in a volumatric flack. The final solution centains 10 mg. of Sr++ and 10 mg. of Y+++per ml. l I'H CH cone. (2Ef>)(ACS grada). 3. 4 4. Dilt. a "H CH (1-1). 111x equal volumas of conc. UH CH and 4 4 distilled water. 5. Diluta UNO. D13"to 100 nl. of conc. IEIO3 to 1 liter with 3 distilled water. 6. Arc. onium cxalato. (ACS grado, powdcred). l 7. Armenium oxalate,1% colution.- 10 gr ma of (UH )2 2 4 ~ 00 4 H O p:r litor. 2 Preccdure s l l To 450 grama of :nilk, add with stirring 50 ml. of concen-trated 1C103 and 10 ml. of strontium-yttrium carrict colution. Doll i l the mixture for two hours after focming subsidco and maintain the volume by addit 3oa of distilled H O.nen nococcary. 2 Cool and filtor rapidly through 250 mm. retentivo.ctali-t>ttive paper (A.II. Thomac #5160 is sr.tisfactory). Unsh the fatty roniduc with diluto llNO. Add the wachings to the filtrato and 3 diccard the rociduo. l l Ucutralizo the acidity with cone. U!! GI, adding it clowly f and with stirring until the solution bucomes dliglitly cloudy. Adjust the pil to 3.0 with diluto HM03 or 1-1 NH Gl. A p!! motor with turpura-j t l turo compuncution control is required fot pH adjustment. i 57 9
AriMil TX n. ?Jnn'Q Hono-m L ing rndioicotr: pea Jn milk I Ad'l 20 grr c:a of peudor d remonium oxn!nte, b mt, to boll-ing and sinocr for ono hour. Allow to.:t.:;nd osvenicht befaro 4 filtoring throuch Uhatman #5 pnper (?40 t:n. dJacoter). Wash tho l precipitate on the filter with 1% amonium ox:lato colution. l Dry in en oven. Tran:;for the f31ter with the residuo to a pictinum dish. Char the paper by hcoting the dish gently over a " Mokur-type burner tt king care that the pnpor dcca not burn with a j flamo. Ignito in a mufflo furnaco at 6000C. - 70000. until the n'h is pura whito. Ono hour of heat,ing time is usually sufficient. s Transfer tho ash to a gluccino paper for volghing and J then to a 1" x r" stainless steel planchet for counting. Cover
~
the planchet with " Saran wrap"%nd count in the B:Ird-Atomic l-background anti-coincidence Golger type bata counter vs. a K gou 4 Cl i standard of equal eight. i
frocedure Sarun wrap seal for planchets 1.
Cut squaro of Saran wrap to siso and place on a picco of l cheesecloth. 2. Ueich semplo and put it la ple ahot. 3. Paint a Icycr of C ue around the outside of the planchet. l 4. Put Saran wrcp ever plcnchot and pull t.4.shtly cround the j bottom with a spinning motion in order te provide a taut film over the open face of the planchot. -5. Holding twisted cnds, rotate the planchot s1culy in a centlo. flow of steam fcr approximutely 10 seconds. 6. Let Unran wrap dry and trim off cxcess uith a razor blado. l l 58 t
e . - _ _ _. ~ j d!'Djil.OI.X.)I - 2_MEILN 111 a l n ; ort or int or rit orto: ital P morirch i ?!e w brk ;;l.oto l'epart. it of Ilonll.h Dot.orrif tistion of bono neokJng Radioinotopeu in Water and Ocwago } The objective of this procedure is to propara for automatic can flow thin window proportional counting of bone-seeking activities l inclu< ling stontium, yttrium, calcium, barium, end lanthonum. These are precipitated an a Group in the form of oxalatea and ignited to oxidea nnd ctrbonated prior to counting. No attempt is made to i 4 ,copnrato individual icotopca from the group. Reagonta: l 1. Ultric acid conc. (ACS grcie) 2. Strontium-yttrium-culcium carrier solution. To a mixture of 12.7 grams of Y 02 3 (A.D. F.ackay, Inc., New Ycrk, 99.9% Fure), 30.4 grans of Srcl.6 H O (ACS grado) and 36.8 grans j 2 of CaCl.2 H O (reagent grado)2 add 500 ml. of vator, 50 ml. 2 2 of cenc. hcl, and heat to dicaolve. Cool und make up to 1 liter in a volumetric flack. The finc1 calution contains 10 mg. of Sr++ and 10 mg. of Y+++per ml. I H CH cone. (25, ACS grade) 3. 4 4. Dilute 3 CH (1-1). Mix equc1 volumec of conc. NH CII and f 4 4 diatilled water. 5. Diluto H::C (10%). Add 100 m~ of cene. H:IO to 500 ml. f water a d make up to 1 lit w. l 6. Ammonium oxalate (ACS grade, poeder). 7. A nonium oxalate, in colution. Dissolvo 10 grams of C 0.H O (ACS grado) in water and make up to (ffd )2 24 2 g 1 liter l Proceduro: To two liters of samplo (if leas comple is availablo, i meacure the vol.ume to the nearent 100 ml.) add 50 ml. of conc. HtIO3 (100 ml. if th'o canplc in cowar:o) and 10 ml. of strontiun-yttrium-enicium carrier colution. Add a few Icflen boiling chios and virornualy boil the mixture for ona hour. Filter the colution t rapidly. through 250 mn. retentive qualitativo paper (A. H. Thomas //51/,0 is.naticf::ctory). Solution may be filtered while hot. i-( 59 i -y.
Dono-n, < l< 1ng ruliol:a t or a In A f1 r i.i_) I _X 1_1... _/dC._. n.._'_LJ uriter nerl. -un::" l>ut.rrilieu 1.l o co'lat.h n wi th c ne. lil'4.!I r.d'line: it alowly 8 awl vith atirring. Ilan w thyl ornur:0 na nn ia<!lenf.ur und n1+roor:h the endpaint frem.he olkt lira.Wlo. Chock i.ho p!! finally with a meter h:.ving a 's:npcroture co. :endator and udjunt to p'l 2.5-3.0 uaing dil tte l'UO3 and diluto Mi! CII solutiona for adjustment. 4 2!d 4 gn:ns of pcud: rad ann. onium oxalate and hoot to 0 boiling rugd 33rner for 1 hour at 90 0. Allow to stand overnight before filtering through Whattan (5 fil'er raper (240 rn. diameter). Ucch the precipitate on tio l filter with 1 por cent a::noniu:1 oxalnto solution. Dry in an oven. Trancfer the f lter with the residuo to a plati m dich. Char the y per by heating the dinh gently over a n l'cker type b trner, tekin'; care that th: paper de.?s not burat into j flare. (An i.f ired liu p may be used in placo of ovan drying). Ipnite in a taffle furnace at 60N/0000, until the r; h is puro I white. On. hour of heating is usunlly auiricient. i Trancrer the ash into a veighed 2-inch stainlaan stcol pl.mchot and raveigh. Cover the plan; hot with Saran urapNand count in tha 3aird Atenic automatic Cus flow proporticnal counter vs. a '%D1 standard cf cqual ucicht. 'Proccira Seran wrap ceal for planchets 1. Cut-squaro of Saran wrap to cice and place on a piece of checcccloth. 2 edrh scmplo and put it in p.7anchet. i 3. Pcint n Inycr of glue around the outside of the planchet. j 4. Put Cart.n wrap over pl.:~ het and pull tightly around the i.atten with a spinning n.stion in or:ler to provide a tcut l filn cycr the open face of the planchc'. 5. Holdin~ twicted cnic, rotato the plenchet slowly in a Cuntlo flow of steam for upproxicately 10 seconds. 6. Lot Sarar. urop :lry nnd trim off excesc wi th a razor blu-le. t 60 t
AjpCID TQ 8;,Jco,q ' t), { s i Diviaton of Iaborntoricc vnd tir centch i Il9u York Stato Nport:veat of !!calth i Dot <:rrdnntion of Ifr.no-sodin:: Fwliojcotopen in Vey tution, Tianov, Plankton, Fich i l The objactive of thin precedure is to prepare for rute s FJ' tic gn3 ficW thin WinflGW'!&oportion01 countlnN of bene-c00hing cchivJ tica ine.luding atrontium, yttrium, calcium, tar f un, cnd lenthr.num. The.a are precipitated as a group in the for:t er exa-1r;tes and Jeptited to oxid"a rnd corbenatcc prior to counting. lio attempt is made to copcrato judividual icotope.; from th: gro;p. Reagents: 3 cene. (ACS grado) 1. HNO rier solution. To a nirture of 12.7 2. St*cntium-yttrium grams of LO3 (A.D. Vn dev, Inc., Nov York, 99.6 rure) l end 30.4 gEs.s of SrCl,0 '(ACS grado) c.dd 500 ml. cfCoal j unter, 50 r1. of conc. hcl and heat to discolvo. ^ and take up to 1 liter in a volumetric fluck. Thc final s colution centsina 10 cc. of Cr++ and 10 mg. of I+'+rer.:1. t 3. Ird O!! conc. (20$)(ACS grado). 9 4 /,. Dilute NH CH (:.1). I'tx equal volunas of cono. NH Gi 4 cnl dictikled utor. {: z to 1 liter j 5 Dilyte HNO. Dilute 100 cl. of conc. 3:!03 3 i with distilled unter. 6. le cniu= oxalato (ACS grado, powdered). 7. A=cnium exalate,15 solution. 10 Crana c" (UM )2 2 4.H 6 C0 g 2 per liter. e .'i froccluro: - i; 1 If the physical stato of the cample in homogenacus, relect a ucll mixed pcrtien for ena!;nia, otherwise, put the senple thrcugh n Uorjng blen br for 5 minutoa. If tho vegotation cenple hos cen ~ y sidorchlc coil attnched to the roots, this chould be chaken cff. P_o pn!. t:~ h thn dirt err cince there is possibility thereby of loss of A littic distilled water l n :Livity clinging to tho : :. alka and leavec. in tho blender with the c:aaple aids in the disintegration prc:can. g Dry the homogenccuc material to conctnnt ucicht in nn cvon at 103 0 Trancfor a portion (10 - 20 grama) to n '.laring blender. l 0 Icave the avcr on Op: rote tho blender until sample is pulvorized. / thu blendor "or at lecct 5 minutoc to allow tho duct to ccttic. l f Ueich out 10 - 20 gramn of the pcudered cre.ple into a j porcelain dich cnd char it cerofully over a N ker-type burner taking 1 61 i i
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i.lsnt< ton, ri ch cure thnt it dot s not bu n uit.h et flor:vi. An inferred In:c.p n:ny be nubutituted for the ?khor burner. Trennfor to a cufflo furnaco end ignito at 600 -7'.'O')C until canpletely ached. Tre.ncfer the nah to an 200-ml. beaker, rdd nlowly 200 cl. of 10% IC!O) nnd 10 ml. of carrier colution. Cover the bortkcr and boil gentl for ono hour, nnint.aining the volume with dia-tilled H,30 Uce Teflon chips in the bankor to prever'. Funning. F11 tor t'ic colution while het through paper (A. H. Thanas / '!160, ' 15 cm. dic.ater is catiafactory). Wach the reciriue u' th 1::,'> nitric acid Ln:1 diccard the paper cud reciduo. I!cutr, lice the filtrate with 1-1 I!H 0H, edding it slowly 4 and with stirring. Une tc.e4'.yl oranga ac an indicator an1 npproach 11.o end point frca the alkaline aido. Adjuct the pH to 2.f-3.0 u;ing a pH :..ater with temp raturo cog ansation for final check. Add I. grans fo pcudered annonium oxalato, bring to a bai.1 nr.d cir.er at CO C. fcr eno h-ur. Allow to ct 4nd evarni::ht before filtiring through Whatzen h5 paper (240-nn, dic: ter). ( hch the precipitate on the filter with 1% ar.cnium ortlate r.clution. [ Dry in el cven. TroncNr tha filter with rcsiluo to a plet!"un dish, Chr r the paper by h.'a' g the dith ge n.~y over a l'h. burner, ttking cre that the par r decs not hur;t into flan: l An infered.n.ter nay be substituted for the even :r.1 lbk.r burner. [ I.; nite in a ruffle frnaco ct 6000-700cC..:ntil the sch is pure white. One hour cf hecting is usually cufficient. Trancrer tha och to n ucichrA ?" stainlecc ctoci planchot i c 1 revolch. Cevar the planchot uith Jaron urnp ind count in a h ird-Atomic autenatic gcc ficy propertional ecunter vs. u K40c1 l ct lari of. c:juul uci ht. C
Proceduro - Saran wrap coal for plcnchots 1.
Cut equare of 3 cran wrap to size and p1r.co en a piece of chec xoloth. l ?. Wah:h ca.! lo and put it in Idanchet. l i l 3. Paint a loyar of ;;1ua nround the outrido of tho pliac: hot. 4. Put, Saran wrap over plunchot and ru' ' tirbtly around the l'ott y, with a spinnin;; notion in or kr to provilo a tnut film over the open fcee of th^ planchet. 1 5. Ihlding twinted enda, retnto the pinneh t ulowly in u gent,lo f]os of.Acam for approxinatoly 10 ceconic. 6. Let Unran urnp dry and trim off exces: ui th a razor blado. 62
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,A l',11 : tii!.{ It l/,,(i..n ), ie lii v ia l on ol' l. il.or, t. >r l.,: . m. I li..:i. rir h Now brk ut:tto Duporttunt, ot' llimith Saran wr:.p ner.1 for planchota "' en the Gar,n vrap in brought near the top of the planchot, the sar.pl'. natorial in the p]- tehot w.y have a tendency to " fly m>" to neat the Jaron uran. To c2 inato loca of ca nple, tho Saran wrap 13 cut to si:.o and then pinced cn u cloth to retcovo static cluctricity. l Eccause of the narrow rin on core plancheta, and minor vari-l stiens in cist which nako th"n fit tightly in the counter, use of clue I is desirablo uhen covering planchets uith Saran wrap
To nako gluo, nix pcrtc of t<.nzano to 1 r rt of ethyleno dichlorido, and add poly-iso-butyl nothacrylate polymer to bring t' the conalstency
<ler' red. " Procedure: 1. Cut cqu re of Saran urap to nizo nnd place on a piecc of l cheececloth. I .I 2. Ucich ca:ple en1 put it in plunchot. i 3. ?cint a Icycr of cleo crotrA the outs $de of the plcnehet. 4. fut b rua urap over plon het and pu' tightly around tho bettan with a anInuing. motion in or; c to provido a tout i film over the open fato of the planchet. l 5. Holdin;; titicted on-In, rotote the planchot slowly in a cantle flow of steam for approxirately 10 scconds. 6. Lat Saran wrap dry and trin off exccas with a rczor blado. l l r l i i i l l I l l 4 63 l l ? l l 1
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,(r*.,n t, ) t Dlv ic ion of laber,.t...e l..a nn.1 hinn.rech Ucw York Ctato lia nctnoot, of flonJ th i R tdio3ccical eneminition of air particulates I The cot: plea to be ana2yzed l rive citLer bcen n 8 3-ch by l 1 10 inch or a 2 inch dimruter gloca fibre filter. The filtera cro cupplied by Mine Safety Applianco Congany of Pittchurgh, Pa. and coch The 2 inch pnebgo of 25 filter, t.carc the estalogue number CT. '.5428. diareter filterc ec precsed cut of the 8 inch by 10 inch cheats. l Uhen in the filter holder the effcetive arca of the 8" x 10" ] f))ter is reduced to 7 inches by 9 inches and the effectivo diameter of the 2 inch diorctor filter becomen 13/4 inchoc. At lenct six hourc are alleued to e3apec between the tino the campling 1 cried ended and the time of examination. The 8 inch by 10 inch filter (used on the Stcplex High-Vclune Samp3cr) is prepared for cct.ating in the following tanner. i 1. Meigh r 2" stain 1cco stcol planchet. f I 2. Cut 4 - 13/4 inch dio: cater disco from the expcsed pcrtion of the filtar cpceing tnca evenly along a dioconal. 3. Stach there 4 disco in the planch.;o with c:poced cido up. 4 4. Ucigh planchet and contents. 5. Cover plcnchet with caran vrap. The 2 inch dicceter filter (used in the Gast Sampler) is r i prepared for counting in the follouing tanner, i r 1. Weigh the 2" stainless atec1 planchot, i 2. Incert the 2" filter into the planchet with expeced cide up, t 3. Ucich planchot and contents. 4. Cover planchet with scran urcp. i The propacd canplec are then counted under a 2aird-Atonic The counta oro ctandcrdiced a'>tc.r ttic thin win le i r. oportional counter. by ecmportcon to KC1 nt.ind vdc of tho s a..a unicht, l'achcround is rtetcraj nod by counting; un eer.ty 2" ctainlenc nteci planchot covered with ceran wrap. P.ich cumple ta cou.tted nt least tuice for 900 counts If obrarvation indle itco chart-lived icotopec are percut, cach tino. further atudy is required. l f 64 ) 1
i 1 Mr M AITFhDIX 13 ') (Coa't) r Divicien of Laboratorica and lleccarch !!w York Stato Dop trt,nont of IIcolth Radiological camin:1 tion of air particulntos I no efficiency of the countinr; tee' Jque is found by Since c"1culating an efficiency. factor for vr.rious weight stend rde. tl.9 Cecactry is conatant, the efficiency for canples is aucuned to be the cono u; that obt?ined for equal volght standards. Ia crder to calcuJate the activity in ppe per noter cubed the following fceters nust also to known: 1. Length of canpling period. 2, Averc3e air flow. Ratio of area of filter to area of sanple. 3. 4 I i t 1 l s i 65 -i __.}}

ML20031G069

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