ML18207A178
ML18207A178 | |
Person / Time | |
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Issue date: | 07/30/2018 |
From: | Steven Garry NRC/NRR/DRA/ARCB |
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Download: ML18207A178 (30) | |
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Accident-Range Gaseous Effluent Monitoring Calibration and Time-Dependent Instrument Response Factors Steve Garry, CHP Sr. Health Physicist Office of Nuclear Reactor Regulation U.S. Nuclear Regulatory Commission NEI HP Forum July 30, 2018 Naples, FL 1
- This presentation:
- shares basic information on calibration of accident-range gaseous effluent monitors
- reviews the regulatory basis and guidance for calibration of instruments
- is based in part on proposed guidance for calibration of accident-range effluent monitors given in HPPOS-001 and HPPOS-040
- Other calibration methods may be acceptable 2
TMI Accident Wednesday, March 28, 1979 3
Basic Issue (most detectors)
- Detectors were designed to measure dose, not activity, and most detectors are highly energy dependent
- Effluent monitors were initially calibrated to low-energy gammas from Xe-133
- During emergencies, a high-energy mix of noble gases could be released
- Calibrations based only on low energy gammas from Xe-133 are not representative of a mix of noble gases
- Effluent monitor response factors should be based on a mix of noble gases 4
5
- Footnote 9 Monitors should be capable of detecting and measuring radioactive gaseous effluent concentrations with compositions ranging from fresh equilibrium noble gas fission product mixtures to 10-day-old mixtures, with overall system accuracies within a factor of 2.
6
NUREG-0737 (November, 1980)
(NUREG-0660) 7
procedures or calculational methods to be used for converting instrument readings to release rates per unit time, based on exhaust air flow and considering radionuclide spectrum distribution as a function of time after shutdown (pg 3-96, section II.F.1-3) 8
HPPOS-001 NRR Guidance
- August 16, 1982, memo from NRR to Regional Administrators
- NRR proposed calibration guidance
- Now known as HPPOS-001 9
NEI 99-01 [Revision 6]
10
- Some EALs are based on pre-calculated effluent monitor values corresponding to EPA PAG doses for a 1 hr exposure 11
NEI 99-01, Rev 6 (endorsed by NRC)
- Unusual Event = 2x ODCM release rate limit
- 10 mrem TEDE, or
- 50 mrem CDE (thyroid)
- 100 mrem TEDE
- 500 mrem CDE (thyroid)
Dose Assessment Computer Codes
- Dose code input is in units of µCi/cc or Ci/sec of a mix of noble gases
- The dose assessment computer codes calculates the adjusted radionuclide mix based on decay of the T = 0 source term
- So the input needs to be Ci/sec or µCi/cc of the total MIX of noble gas radionuclides (not Xe-133) 13
cpm & mR/hr (HPPOS-001, pdf 17)
- cpm, or mR/hr, is not a good measure of activity or concentration because of detector energy dependence; i.e.,
different gamma energies and different gamma yields
- Example:
- 1 µCi of Xe-135 (250 keV) produces 7.6 times the dose as Xe-133
- 1 µCi of Kr-88 (~2 MeV) produces 48 times the dose as Xe-133 14
Instrument Response Factors
- Detectors do not measure the concentration of the mix,
- Detectors measure ionizations in cpm, or mR/hr
- An Instrument Response Factor is needed to convert from cpm or mR/hr into concentration uCi/cc or Ci/sec of a mix 15
Time Dependent Instrument Response Factors
- Vendors primary calibration is typically based on Xe-133
- Instrument Response Factors should be based on the calculated isotopic mix as function of time 16
Isotopic Mix
- The isotopic mix has a big effect on the instrument response factors (conventional detectors)
- Instruments calibrated only to Xe-133 will generally over-estimate the total µCi/cc of a mix
- Information on plant conditions and effluent monitor readings (exceeding EALs thresholds) are used to classify emergency conditions and determine if protective actions are needed
- Therefore, effluent monitor calibrations should be performed properly 17
GM Detectors
- GMs are energy compensated (e.g., lead shield)
- So GM detectors intentionally have a strong energy dependency so dose is measured +/- 20%
- GM detectors under-respond at low gamma energy
- GM readouts are in cpm // µCi/cc of Xe-133
- Should be adjusted to readout in terms of a mix of nuclides 18
Mid-Range (V)
Energy-Compensated GM Detector Regular size paper clip 19
Ion Chambers
- Measures electrical current (amps) caused by radiation exposure
- Detector output is electrical current (e.g. picoAmps);
- current is directly proportional to exposure rate
- Programmable microprocessor converts picoAmps to mR/hr or µCi/cc or Ci/sec 20
Instrument Response Factors
- At T = 0 (worst case), detectors calibrated to Xe-133 (81 keV gamma),
- GM detectors could over-respond by a factor ~30
- Ion Chambers could over-respond by a factor of ~ 10
- Cd/Te detectors could over-respond by a factor of ~ 5
- Flow-through ion chambers may be within factor of ~ 2 21
Time-Dependent Response
- GM response factors that are based only on Xe-133 could over-estimate the release: e.g.,
- 0 to 8 hours9.259259e-5 days <br />0.00222 hours <br />1.322751e-5 weeks <br />3.044e-6 months <br />
- Gas Gap - T = 0 high estimate by a factor of ~ 5
- Core Melt - T = 0 high estimate by a factor of ~ 30 12 hours1.388889e-4 days <br />0.00333 hours <br />1.984127e-5 weeks <br />4.566e-6 months <br />
- Gas Gap - T= 8 hrs, much better estimate
- Core Melt - T = 8 hrs, much better estimate
- > 24 hours2.777778e-4 days <br />0.00667 hours <br />3.968254e-5 weeks <br />9.132e-6 months <br /> - T > 24 hours2.777778e-4 days <br />0.00667 hours <br />3.968254e-5 weeks <br />9.132e-6 months <br />, under estimate 22
Example Calibration Process Step 1. Vendor Calibrations
- Step 1.1 Gas calibration
- Step 1.2 Linearity check
- Step 1.3 Transfer calibration
- Step 1.4 Detectors energy response characterization Step 2. Secondary Calibration check at Plant Step 3. Energy Response Factors Step 4. Instrument Response Factors 23
IP 71124.06 - Radioactive Gaseous and Liquid Effluent Treatment
- Inspection Objectives
- To ensure that the gaseous and liquid effluent processing systems are maintained so that radiological discharges are properly mitigated, monitored and evaluated with regards to public exposure.
- 02.04 Instrumentation and Equipment (1 Sample)
- (c) High-Range Effluent Monitoring Instrumentation
- Verify instruments are calibrated and available
- Review methodology for calculating EAL thresholds (e.g.
instrument response factor determination) associated with system modifications since the last inspection
- Verify licensee can collect and analyze high-range, post-accident iodine and particulate samples 24
IP 71124.06 - Inspector Guidance
- Guidance 03.04(c) :
- Refer to FSAR, technical specification requirements and NUREG-0737
- Since monitors are used for PARs, ensure regional EP staff is aware of monitoring issues that could impact the monitors function
- Interview personnel who perform calculations
- Detailed review of EAL threshold calculations not intended
- Focus on changes since last inspection
- Refer significant questions or issues to the program office for further guidance 25
Items to Consider
- Which plant departments are responsible for the effluent monitors?
- Radiation Protection, Chemistry, I&C, or EP?
- Is there good communication between departments?
- Calibration QA
- Typically required by T.S. commitment to RG 1.33 26
Plant Commitments
- Letters to NRC describing implementation of NUREG-0737 items
- Letters to NRC describing implementation of RG 1.97
- Documents that contain compliance-related commitments 27
Vendor Documents to Review during 71124.06 Inspections
- Equipment Design Documentation
- Technical manuals
- User manuals
- Vendor Calibration Documentation
- Initial gas calibration data
- Transfer calibration data
- Detector energy-dependence studies 28
Plant Calibration Procedures and Detector Energy Response Studies
- Plant Calibration Procedure(s)
- Plant Engineering Studies
- Programmed instrument calibration constants for converting detector output into source term
- cpm into Ci/sec or micro-Ci/cc
- mR/hr into Ci/sec or micro-Ci/cc
- Evaluation of instrument response to changing radionuclide mix
- Instrument response factors 29
Questions 30