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Annual Radiological Environ Rept for Period Jan-Dec 1997
	ML20217J039
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Site:	Cooper
Issue date:	12/31/1997
From:	Latham A; TELEDYNE BROWN ENGINEERING CO.
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Cooper Nuclear Station Annual Radiological Environmental Report s

Radiological Environmental Monitoring Program January 1,1997 - December 31,1997 USNRC Docket Number 50-298 Nebraskagubt H ower District Prepared by TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES l

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G40604 DSF

Cooper Nuclear Station Annual Radiological Environmental Report Radiaogical Environmental Monitoring Program January 1,1997 - December 31,1997 1

USNRC Docket Number 50-298 H

Nebraskagl[c Pow District Prepared by TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES l~

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f bR A KOO 298 R ,; , PDR G40604.DSF

l ATTACHMENT 3 LIST OF NRC COMMITMENTS l

Correspondence No: NLS990060 The following table identifies those actions committed to by the District in this document.

Any other actions discussed in the submittal represent intended or planned actions by the District. They are described to the NRC for the NRC's information and are not rer'*latory commitments. Please notify the NL&S Manager at Cooper Nuclear Station of any qu(,

ns regarding this document or any associated regul.g ory commitments.

COMMITTED DATE COMMITMENT OR OUTAGE None N/A l

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I l FROCEDURE NUMBER 0.42 l REVISION NUMBER 6 l PAGE B OF 13 l

W TELEDYNE BROWN ENGINEERING Environmental Services REPORT TO NEBRASKA PUBLIC POWER DISTRICT COLUMBUS, NEBRASKA

, RADIATION ENVIRONMENTAL MONITORING PROGRAM 3 COOPER NUCLEAR STATION

, NEMAHA COUNTY, NEBRASKA

\

ANNUAL REPORT JANUARY 1 TO DECEMBER 31,1997 i

PREPARED BY TELEDYNE BROWN ENGINEERING ENVIRONMENTAL SERVICES 50 VAN BUREN AVENUE WES'IWOOD, NEW JERSEY 07675-1235 i

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REPORT APPROVED BY: / .~7 R. LATHAM,

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MANAGER ENVIRONMENTAL ANALYSIS DEPARTMENT

PREFACE This report covers the period of January 1 through December 31,

, 1997. All sample collections were made by personnel of the Nebraska Public Power District. Analyses were performed and reports of analyses were prepared by Teledyne Brown Engineering - Environmental Services and forwarded to Nebraska Public Power District.

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TABLE OF CONTENTS PAGE Prefare......................................................................................................................... 11 IJstofTaNem.............................................................................................................. vi

. IJst of F1 gusts.. . . . . . ... . . . . .. . . . . . . .. . . . .. . . . . . . . .. . . . . . . ... ... . . . . .. . . . . . . .. . .. . . . .... ..... . . . .. . . .. .. .. . . . . . . .. . . . . . .. vii I. I n tro d u c ti o n .. .. .. .. .. .. . .. . . .... .. .. .. .. . .. .. .. .. .. .. . . .. . .. .. .. .. .. .. .... . .. .... .. .. .. .. .. ......... .. .... .. . .. .. .. .. .... .. 1 II. Summary.......................................................................................................................2 III. Sampling and Analyses Program, Stations and Maps .................................. 3 IV. Disc u s sion ... . .. . .. .. .. .. ... .. .. ... .. . .. .. .. . .. ... .. .. .. . . . .. ... ..... .. .. .. . .. .. .. . .. .. . .. .. ..... . ... ... .. . .... .. . .. .. .. . .. . 1 1 1 A. Program Objectives and Data Interpretation 11 Atmospheric Nuclear Detonations V. Radiological Environmental Monitoring Program Summary Table 3...12 REMPS TABLE 3 ANNUAL

SUMMARY

OF ALL SI'ATIONS OF THE ............13 ISOTOPES OF INTEREST WI'IE YEARLY AVERAGE ACTIVITY, NUMBER OF DETECTIONS PER 'IDTAL STATION WITH HIGHEST AVERAGE ACTIVITY, AVERAGE OF CONTROL STATION AND INCLUSIVE DATES OF ANALYSES VI.

DISCUSSION, IMPACT ON THE ENVIRONMENT, GRAPHS OF .................. 25

. RESULTS AND STATISTICAL TABLES FOR EACH QUARTER A and B. AIR PARTICULATES - GROSS BETA - GROSS ALPHA .................... 26 1

I C C HARC OAL FI LTER. I - 13 1 ............ ...... .......................... ................ ....... ..... 41 l

D. COMPOSITE OF AIR PARTICULATE FILTERS - GAMMA .............. 49 )

E. FISH.....................................................................................................................57 !

F. MILK - NEAREST PRODU CER ................................................................. 63 G. MILK - OTHER PRODUCERS ................................................................72 111

TABLE OF CONTENTS

. PAGE H. GROUNDWATER ....................................................................................81 I. RIVER WATER ............................................................................................87 J. THERMOLUMINESCENT DOSIMETERS ..........................................96

. K. FOOD - BROADI .EAF VEGETATIO M ......................................................104 i

L SHO RE LI NE SEDI MENT ........................................................ .................. 1 10 {

I vu . C OMPtErE DATA TiB tES . . .......................................................................... 115 i A.B,C. AIR PARTICULATE FILTERS - GROSS ALPHA. .........................116 GROSS BETA. I-131 D. COMPOSITE - AIR PARTICULATE FILTERS ...............................137 E. FISH.....................................................................................................148 F. MILK - NEAREST PRODUCER .......................................................... 151 G. MILK - OTHER PRODUCERS ............................................................ 158 H. G ROU NDWATER .................. ................................................................. 161 1

I . RIVER WATE R . .... .. ... . ... ... .. . .. . ............... .. ...... . .. .... ... .. ...... . ... ... .. . ... .. . .. .. . .. .. 1 M I i

i J. THERMOLUMINESCENT DOSIMETERS .....................................171 :

K. FOOD - BROADLEAF VEGETATION .................................................176 l

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L SHO RELINE SEDIMENT ..................................................................... 189 i a

REFERENCES.. . . .. . .... .... . . . . ... . .. .. . . .. .... .. . . . .. .. . . . . . . . .. ..... .. .... . . . .. .. . .. . . .. ..... . .. .. . .. ... ... . .. .. .. ... . . .. .. . . 191 1V

TABLE OF CONTENTS PAGE VIII. Appendix A. LAND U S E C E NS U S ................................ ................... ................. .......... ...A- 1 B INTERLABORATORY COMPARISON PROGRAM ...........................B-1 C STATI STI CAL NOTE S ............... ..............................................................C- 1 L$. NOTIFI CATI O N LEVE LS ............................................................ ............D- 1 E. C O NVE NTI O N S .. . .. .. .. .. ... .. . .. ... ... . ... .. . .. .. ... . .. . .... . .. . .. ... .. . .. . .. . .. .. . ... .. .. ... .. . . .. .E- 1 F. DETECITON CAPABIIJI1ES.......... ............. ..... .................. . .. ......... ........F- 1 G. SAMPLE STATION LOCATION AND SAMPLE TYPES................G-1 H.

SUMMARY

OF DOSES TO A MEMBER OF THE PUBLIC...........H-1 OFF-SITE I. NON-REMP ANALYSES.. .. .. .. .. .. .... .. ... . ... .. .. .. .. .. .. .. .. .. .. . . .. .. .. . . . ... .. .. ... .... .. .. ..I- 1 1

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12ST OF TABIES TABLES TITLE PAGE 1 Sampling schedule and analysis. 5 1997. Cooper Nuclear Station 2 Sample Station Iocation with 7 Distance and Direction from the Elevated Release Point (ERP) l I

3 Summary of Radiological Monitoring 13 Program A to L Statistical Summary Tables - Section VI pages25-114 By Sample Type A to L Data Tables - Section VII pages 115-190 By Sample Type and Station e

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LIST OF FIGURES E94 Init EAEC

1. Maps of sampling stations, Cooper Nuclear Station.............................. 9.10 A-1 Air Particulate, Gross Beta - CNS....................................... 28,29,30.50,51,52 A-2 Air Particulates, Gross Beta - ERAMS........................................... 31,32,53,54 B-1 Air Particulates, Gross Alpha - CNS.................................. 28,29,30,50,51,52 C-1 Airborne - Iodine, CNS. . . ..... ... .. ........... . . . .. .. . . ... . . . . .. . . . ... . . . .. . . . . ... . . .. . .. . .. . . . . .. . . . 42,43,44 D-1 Air Particulates - Ce-144 - CNS........................................... 28,29,30,50,51,52 D-2 Air Particulates Ce-144 - EML ......................................... ............. ......... 50,51,52 E-1 Fish, Gross Beta, K-40, Sr-90 and Cs-137 - All locations.......... 58,59, 60 F-1 Milk - Nearest Producer, K-40, I-131 and Cs-137........................ 64,65,66 F-2 Milk - Nearest Producer, Sr-89, Sr-90 and Elem. Ca................... 67,68,69 G-1 Milk - Commercial Producers, K-40, I-131 and Cs-137.............. 73,74,75 G-2 Milk - Commercial Producers, Sr-89, Sr-90 and Elem. Ca......... 76,77,78 H-1 Groundwater - All Locations, Gross Alpha, Beta and H-3............. 82,83,84 1 l

I-1 River Water - All locations, Gross Alpha, Beta................................. 88,89,90 I-2 River Water - All Imcations, Sr-89, Sr-90 and H-3........................ 91,92,93

, J-1 'Ihermoluminescent Dosimetry - All locations............................... 97,98,99 K-1 Food - Broadleaf Vegetation - All locations........................................105,106 !

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- L-1 Shoreline Sediment - K-40, I-131, Cs-134 and Cs-137...............111,112 {

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L INTRODUCTION This report contains a complete tabulation of data collected during the period January through December 1997, for the operational Radiological Environmental Monitoring Program performed for the Cooper Nuclear Station (CNS) of the Nebraska Public Power District (NPPD) by Teledyne Brown Engineering - Environmental Services.

Cooper Nuclear Station is located in Nemaha County in the southeast corner of Nebraska on the Missouri River. A portion of the site extends into Missouri. The reactor is a 778 megawatt boiling water reactor. Initial criticality was attained on February 21, 1974. The reactor reached 50%

power on June 25,1974 and 100% power on November 20,1974.

Radiological environmental monitoring began in 1971 before the plant became operational and has continued to the present. The program monitors radiation levels in air, terrestrial and aquatic environments. Most samples are collected by NPPD personnel. All are shipped for analysis to a contrector's laboratory where there exists special facilities required for meamrements of extremely low levels of radioactivity. From 1971 through 1976 the contractor was Teledyne Isotopes, Westwood, New Jersey. NALCO Environmental Sciences assumed responsibility for the analyses effective January 1,1977.

On November 1,1978 Hazelton Environmental Sciences Corporation (HESC) assumed responsibility for the program. Prior to November 1,1978 Hazelton Environmental Sciences operated as NALCO Environmental

. Sciences. Teledyne Isotopes (now trading as Teledyne Brown Engineering -

Environmental Services) again assumed responsibility for the analyses effective January 1,1979 through December 31,1997.

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H.

SUMMARY

Presented in this report are summaries and discussions of the data generated for the Radiological Environmental Monitoring Program (REMP) .

for the Cooper Nuclear Station (CNS) of the Nebraska Public Power District (NPPD) for 1997.

Part V, Table 3 presents the yearly summary of the program with the total number of samples of each type analyzed, the yearly average for all samples, the number of detections per tc,tal number of samples, the station with the highest average, the average of the control station, and the inclusive dates of the analyses.

Part VI is a discussion of each type of sample analyzed and its impact, if any, on the environment. Included also is a graph of the isotopes of interest since 1977 and the statistical results for each quarter of the year. This is followed by a complete tabulation of the data by sample type and station number.

l The 1997 radiological environmental measurements for CNS indicates that there has been no residual fallout resulting from the explosion and fire at the Chernobyl Reactor in the Soviet Union which occurred on April 26, 1986. It may be conchtded from all measurements taken that the operations of CNS had no detectable impact on the environment in the vicinity of CNS.

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III. SAMPLING AND ANALYBES PROGRAM. STATIONS AND MAPS The 1997 sampling and analysis program is described in Table 1.

Teledyne Brown Engineering - Environmental Services has a comprehensive quality assurance / quality control program designed to assure the reliability of data obtained. The results for the 1997 Intercomparison Program conducted by the EPA Environmental Monitoring Systems L,aboratory in Las Vegas, Nevada and Analytic *s, Inc., are contained in Appendix B.

.. Sampling locations are summarized in Table 2. 'Ihe type or status of each location and its distance and direction from the reactor elevated re-lease point are specified. A map of locadons follows (Figure 1). Complete

. descriptions of active sampling locations are given in Appendix G.

The annual land use census for 1997 is described in Appendix A.

There were no milk animals found within three miles of CNS in 1997 and no evidence of potable water use from the river. The nearest garden to CNS is in sector M,12 miles from CNS. Gardens were found in 9 sectors during 1996 and in 1997. The nearest resident to CNS is in sector Q, 0.9 miles from CNS.

All of the required 1997 environmental monitoring. including sam-pling and analysis, was conducted as specified in Table 3.21.F.1 of the CNS Technical Specifications, except as noted below:

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COLLECTION STATION PATHWAY SAMPLE PERIOD REASON 03 Airborne Air Particulate & 04/08-04/15 Flooding.

Charcoal Filters 03 ~ Airborne Air Particulate & 04/15-04/22 Flooding.

Charcoal Filters 07 Airborne Charcoal Filter 04/15-04/22 Inadvertently sent in blank.

03 Airborne Air Particulate & 04/22-04/29 Flooding.

Charcoal Filter 07 Airborne Charcoal Filter 04/22-04/29 Human error.

03 Airborne Air Particulate & 04/28-05/06 Flooding.

Charcoal Filter 03 Airborne Air Particulate & 05/06-05/13 Flooding.

Charcoal Filter 03 Airborne Air Particulate & 5/13-05/20 Flooding.

Charcoal 3

COLLECTION STATION PA*IEWAY SAMPLE PERIOD REASON 02 Airborne Air Particulate & 09/16-09/23 Pump failure.

Charcoal 28 Aquatic Sediment /Sil 05/06 Flooding 28 Waterborne River Water 05/13 Flooding: sample taken

from expanded confines of river.

28 Waterborne River Water 6/2 Flooding; sample taken from expanded confines of river.

28 Aquatic Fish 6/24 High water conditions; mid-top species not available.

35 Aquatic Fish 6/24 High water conditions; mid-top species not available.

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TABIE 1 NEBRASKA PUBLIC POWER DISTRICT COOPER NUCLEAR STATION i

ENVIRONMENTAL RADIATION SURVEILLANCE PROGRAM SAMPLING SCHEDULE AND ANALYSIS

. I ONCE PER 7 DAYS l I

Sample Tyne Station Nos. Analyses Airborne - Particulate 1 - 10 Gross alpha, beta. Gam- !

ma isotopic on quarterly composite of each sta-tion and on each sample I in which gross beta ac- l tivity is > 10 times the yearly mean of control samples Airborne - Iodine 1-10 I-131 l ONCE PER 15 DAYS l Samnle Tyne Station Nos. Analyses Milk - Nearest Producer 61 1-131 (low level)

(gggk pasture only) Gamma isotopic Sr-89, Sr-90, Elem. I Ca. on monthly composite l ONCE PER 31 DAYS l 1 Samnle Tyne Station Nos. Analyses River Water 12,28 Gross alpha - sus and dis l Gross beta - sus and l dis, Sr-89, Sr-90, Gamma isotopic Tritium on quarterly connosite !

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TABIE 1 NEBRASKA PUBLIC POWER DISTRICT COOPER NUCLEAR STATION ENVIRONMENTAL RADIATION SURVEILLANCE PROGRAM SAMPLING SCHEDULE AND ANALYSIS l ONCE PER 31 DAYS -l Samnle Tyne Station Nos. Analyses Milk - Nearest Producer 61 1-131 (low level)

(non-peak pasture Sr-89, Sr-90 season)

Elem. Ca Gamma isotopic Food Products - Broad- 28,96,101, I-131 leaf Vegetation (when Gamma isotopic available) l ONCE PER 92 DAYS l Samole Tyne Station Not Analyses Background Radiation 1 - 10, 20, 44, 'ILD Readout 56,58,59,66, (gamma dose) 67, 71, 79 - 91, 94 -

Groundwater 11,47 Gross alpha, beta Gamma isotopic Tritium Milk - Commercial and 99, 100 I-131 (low level)

Other Milk Producers Sr-89, Sr-90 ,

Elem. Ca Gamma isotopic

[ l 2 TIMES / YEAR l Samnle Tyne Station Nos. Analyses Fish (Summer and Fall) 28,35 Gross beta Sr-89, Sr-90 Gamma isotopic Shoreline Sediment 28 Gamma isotopic 6

TABIJC 2 NEBRASKA PUBLIC POWER DISTRICT COOPER NUCLEAR STATION BROWNVILLE, NEBRASKA DISTANCE AND DIRECTION FROM THE ELEVATED RELEASE POINT (ERP)

TO THE SAMPLE STATION LOCATIONS 4 STATION" DISTANCED DIRECTION D SAMPLEa NUMBER (MILES) (DEGREES) CLASSIFICATION C TYPES 1 0.10 225 IND AP,C,TL 2 0.75 225 IND AP,C,TL 3 2.5 338 IND AP,C,TL 4 3.0 43 IND AP,C,TL 5 3.5 102 IND AP,C,TL l 6 3.0 165 IND AP,C,TL 7 2.5 230 IND AP,C,TL 8 2.5 260 IND AP,C,TL 9 7.3 335 IND AP,C,TL l 10 10.0 160 IND AP,C TL l 11 0.15 225 IND WG 12 0.10 360 CON WR 20 0.96 315 IND TL 28 1.8 150 IND WR, FI, SH, VT 35 2.0 350 CON FI 44 10.3 270 CON TL 47 25.8 154 IND WG 56 1.9 118 IND TL 58 1.1 219 IND TL 59 1.0 189 IND TL !

61 3.5 326 IND M (Nearest) !

66 4.5 200 IND TL 67 4.8 325 IND TL 4 71 4.3 71 IND TL IND 79 0.85 299 TL 80 0.75 284 IND TL

. 81 0.80 265 IND TL l 82 0.80 176 IND TL 83 4.4 189 IND TL 84 4.4 297 IND TL 85 3.1 3 IND TL 86 4.6 16 IND TL 87 1.75 20 IND TL 88 1.75 63 IND TL 89 2.0 86 IND TL 90 2.25 134 IND TL 91 6.9 54 IND TL 7

TABIE2 NEBRASKA PUBLIC POWER DISTRICT COOPER NUCLEAR STATION BROWNVILLE, NEBRASKA DISTANCE AND DIRECTION FROM THE ELEVATED RELEASE POINT (ERP)

TO THE SAMPLE STATION LOCATIONS STATIONa DISTANCE D

DIRECTION D SAMPLEd k NUMBER (MILES) (DEGREES) CLASSIFICATION C TYPES 94 3.6 108 IND TL 96 1.25 334 IND VT 99 10.5 189 IND M (Other) 100 11.5 197 IND M (Other) 101 13.3 73 IND VT a Only currently active Sample Stations are listed. Sample Station numbers missing from the sequence are for inactive or discontinued locations.

b Approximate distance and direction are specified with respect to the re-actor Elevated Release Point (ERP).

C Classification codes: IND = indicator: CON = control.

d Environmental sample type codes: AP = air particulate filters: C = char-coal cartridges: FI = fish; M = milk; SH = shoreline sediment TL = envi-ronmental thermoluminescent dosimeters: VT = broadleaf vegetation: WG

= groundwater: WR = river water.

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I.

IV. DISCUSSION A. Proaram Obiectives and Data Interoretation The objective of the monitoring program is to detect and assess the im-pact of possible releases to the environs of radionuclides from the operations of the Cooper Nuclear Station. This objective requires measurements of low levels of radioactivity equal to or lower than pre-determined limits of detec-tion. 'In addition the source of the environmental radiation must be estab-lished. Sources of environmental radiation include:

l (1) Natural background radiation from cosmic rays (Be-7).

(2) Terrestrial, primordial radionuclides from the environment (K-40,

, Ra-226, Th-228).

(3) Fallout from atmospheric nuclear tests such as the September 1977 detonation by the Peoples' Republ!c of China and the atmospheric weapons test of October 16,1980 (fission products and fusion prod-ucts).

i (4) Releases from nuclear power plants such as CNS (fission products

! and neutron activation products).

(5) Fallout from the Chernobyl Nuclear Reactor Accident.

Radiation levels measured in the vicinity of an operating power station are compared with preoperational measurements at the same locations to distinguish power plant effects from other sources. Also, results of the moni-toring program are related to events known to cause elevated levels of radia-tion in the environment, e.g., atmospheric nuclear detonations or abnormal plant releases.

11 Atmosoheric Nuclear Tests Three atmospheric nuclear detonations in the People's Republic of China

influenced program results significantly in late 1976 and in 1977. Two of these detonations occurred in late 1976 (September 26 and November 17) and one in late 1977 (September 17). As a consequence of these tests ele-vated activities of gross beta in air particulate filters and I-131 in milk were observed throughout most of the United States.

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! No atmospheric nuclear tests have been conducted since 1977, thus no short-lived fission products were detected in air particulate samples. Also no I-131 was detected from radiogases from any sources.

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On April 26,1986 the fire and explosion of Chernobyl Reactor No. 4 in

. the Soviet Union resulted in the release of fission products to the atmo-sphere and worldwide fallout. Following the explosion, elevated levels of gross beta activities in air particulates and 1-131 in charcoal filters and milk samples were measured. Additionally, in 1986, Cs-137 and the short-lived isotopes I-131, Ru-106, and Cs-134 were detected in broadleaf vegetation.

Similar results occurred in other areas of the United States and the entire Northern Hemisphere.

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V. RADIOLOGICAL ENVIRONmNTAL MONITORING PROGRAM TA_ntra Presented in Table 3 are the radiological environmental monitoring pro- -

gram summaries (RP,MPS) generated from the reports of analyses performed during 1997 for the NPPD sampling and analyses program. The REMPS ta-bles conform to the requirements of Table 1 in Regulatory Guide 4.8 (Reference 6).

The average activity le v-1 for all samples collected for the year for each sample type are summarizu bi this table. The mean, range and fraction of detections to total samples asoayed are presented. The station location and .

station number with the highest annual mean is also tabulated. If a control station is specified the comparable results of the control are listed.

From the REMPS table it is possible to determine the total number of each type of sample analyzed and the average activity of all samples from all l stations of each nuclide. If there were no positive detections the maximum of the lowest levels of detection is listed. The station having the highest level of activity is specified. From this data it is possible to determine any high levels of activity and the source. The dose impact on the population can thus be evaluated.

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1 TABLE 3 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM SUMMARIES (REMP) 1997 O

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I VI. DISCUSSION, IMPACT ON THE ENVIRONMENT GRAPHS OF RESULTS FROM 1977 - 1997 AND l

l STATISTICAL TABLES EACH QUARTER l

l l

I l

l f

O t

f 25

A and B. AIR PARTICULATE SAMPLES - GROSS BETA AND GROSS ALPHA ISee Tables A A-4. B B-4)

STATIONS 01 to 10 Air particulates were collected on membrane filters at ten locations (01-10). The filters were changed weekly and analyzed for gross beta and gross alpha activities. Quarterly composites are analyzed for gamma emitting iso-topes. .

The average gross beta activity of all stations for each quarter of 1996 and 1997 is summarized below: .

1996 First Quarter 0.025 pC1/Cu. M.

Second Quarter 0.017 pCi/Cu. M.

'Ihird Quarter 0.023 pCi/Cu. M.

Fourth Quarter 0.025 pCi/Cu. M.

Average 1996 0.022 pC1/Cu. M.

1997 First Quarter 0.020 pCi/Cu. M.

Second Quarter 0.015 pCi/Cu. M.

Third Quarter 0.025 pCi/Cu. M.

Fourth Quarter 0.025 pCi/Cu. M.

Average 1997 0.021 pCi/Cu. M.

The level of beta activity was at normal environmental levels in 1997 showing the natural seasonal variations. There was a slight decrease in the level of gross beta activity during the first quarter; the second quarter of 1996 was slightly higher than 1997 and there was a slight increase from the third quarter of 1996; the fourth quarter was the same as 1996 as shown in Table A-4. The increase and decline in activity often occurs and is attributed to natural phenomena.

The gross alpha activity continued low and close to the limits of detec- ~

tion. Gross alpha activity is probably due to the alpha emitters found in soil and particulates drawn into the filters.

No effect attributable to the Cooper Nuclear Station was observed in the .

results of monitoring air particulates.

26 j

1 A and B. AIR PARTICULATE SAMPrRS - GROSS BETA AND GROSS ALPHA ISee Tables A A-4. B B-4)

STATIONS 01 to 10

, Figure A1, B1 shows the gross beta, gross alpha and Ce-144 activity in the environs of CNS. The results for 1986 through 1997 are on the second

, and third pages of Figure A-1, B-1. The gross beta activity in 1997 was simi-lar to previous years in which there were no nuclear atmospheric weapons tests or nuclear accidents. 'Ihe gross alpha activity remained low and near

, the normal detection level. Cesium-144 was below the level of detection.

Figure A-2 shows the gross beta activity in air samples through April 1989 at Jefferson City. Missouri as reported by the Environmental Radiation Monitoring System (ERAMS) of the US Environmental Protection Agency.

No more recent data was available. This data was taken from Environmental l Radiation Data distributed by the Eastern Environmental Radiation Facility, Montgomery Alabama. The measurements by ERAMS were made after a waiting period which may explain the somewhat lower results because of decay of the isotopes having a shorter half-life. Measurements of Ce-144 l were no longer reported because the activity has approached the limit of de-tection by the analytical techniques now used.

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C AIR RADIOIODINE - CHARCOAL FILTERS (See Tables C-1 through C-4)

STATIONS 01 TO 10 Charcoal filters used in series with air particulate filters were collected weekly during 1997 at stations 01 through 10 and monitored for radiciodine.

9 Tables C-1 through C-4 show the average monthly and quarterly results

. for each station and the average of all 10 stations. Airborne I-131 levels were below the limits of detection for all of 1997.

- Figure C-1 plots the results of I-131 as monitored in charcoal filters and summarized monthly in 1997 compared with previous years. Results for 1997 were below the normal limits of detection indicating no atmospheric effect from the operations of CNS.

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Air Part1Eulate Filters, which were collected weekly, were composited for each station for a quarterly gamma spectral analysis during the four quar- ;

ters of 1997.

Bery111um-7, a naturally occurring cosmogenic nuclide, was detected in 40 of 40 samples at a level of 0.12 pCi per cubic meter which is similar to the levels of past years. Potassium-40, also a naturally occurring nuclide, was not detected in any of the 40 samples.

Figure D-1 graphs the gross beta, gross alpha and Ce-144 activity as measured on air particulate filters collected weekly at CNS. (This is the same as Figure A-1, B-1). The plot illustrates that there were no detections of Ce-144 above the normal level of detection as measured by the quarterly gamma scan of samples from CNS.

Figure D-2 shows that measurements of Ce-144 are no longer reported by the Environmental Measurements Laboratory of the US Department of Energy because the artificial nuclides such as Ce-144, have reached the lim-its of detection by the analytical techniques now used.

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E. FISH (See Tables E-1. E-2)

STATIONS 28. 35 Fish samples were collected during the summer and fall at the above

. stations and analyzed for gross beta, Sr-89, Sr-90, and gamma emitting iso-topes. An attempt was made to collect a middle-top feeding fish (carp) and a bottom feeding fish (catfish). Only the bottom feeding fish (catfish) was collected during the summer but both types of fish were collected in the fall sampling period.

The gross beta and Sr-90 activities were similar to the levels of previous years. Strontium-90 was below the normal level of detection. '1here were no detections of Sr-89. Naturally occurring K-40 was detected in all samples at an average level of 3.21 pCi/gm, wet. 'Ihere were no detections of Cs-137 during 1997.

Plotted in Figure E-1 are the radionuclides gross beta, K-40, Sr-90 and Cs-137 monitored in fish samples which show no appreciable change from 1977 through 1997. The plot of the nuclides shows that most of the gross beta activity is due to the terrestrial nuclide K-40.

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F. MILK (See Tables F-1. F-2)

STATION 61 (NEAREST PRODUCER) i Milk samples from the nearest producer Station 61, 3.5 miles, 326 degrees from the elevated release point of CNS were collected once every 15

days in peak pasture season and once every 31 days the rest of the year.

The monthly samples collected January through May and October through

, December were analyzed for I-131 by chemical separation, for elemental calcium and strontium 89 and 90. In addition they were analyzed for gamma emitting isotopes on a high resolution gamma spectrometer. The samples 1 collected every 15 days during peak pasture season were analyzed upon re-ceipt for I-131 and gamma emitting isotopes. A monthly composite was prepared and analyzed as described above.

There were no detections of I-131 in the twenty-two samples analyzed by chemical separation. 'Ihere were no detections of Sr-89 in the samples analyzed. Strontium-90 was detected at an average level of 1.3 pC1/ liter, which is a normal environmental level. Elemental calcium was found at an average level of 1.3 mg/ liter. Potassium-40, a naturally occurring isotope, was detected at an average level of 1180 pCi/ liter.

Cesium-137 was not detected in any of the samples analyzed. There was no indication of an effect on the milk of the producer nearest the plant from the operations of CNS.

Shown in Figure F-1 and F-2 are the plots of radionuclides monitored from 1977 through 1997 in milk samples from producers nearest the reac-tor. The levels of K-40, elemental calcium and Sr-90 remained stable.

There were no detections of I-131, Sr-89 or Cs-137. 'Ihis indicates no effect on milk samples from the operations of CNS.

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G. MILK (SEE TABLES G-1. G-21 STATIONS 99.100 (OTHER PRODUCERS)

Milk samples were collected quarterly from other producers, Station 99, 10.5 miles from the plant and Station 100 which is 11.5 miles from the plant. The samples were analyzed for I-131 by chemical separation, for ele- ~

mental calcium, for Sr-89 and 90 and for gamma emitting isotopes. There were no detections of I-131 in the eight samples monitored. .

There were no detections of Sr-89. Strontium-90 was found at an aver-age level of 1.3 pCi/ liter. There were 1.5 mg of calcium per liter of milk. .

Potassium-40 was detected at an average level of 1360. pCi/ liter. The stron-tium-90, K-40 and elemental calcium were at normal environmental levels and were similar to the results obtained from analyses of milk from the near-est producer. There were no detections of Cs-137 in the samples collected.

It can be concluded that the operations of CNS had no effect on milk samples and thus no dose impact on the population.

The levels of radioactivities of the nuclides K-40, I-131 and Cs-137 are plotted on Figure G-1. Potassium-40 was at normal environmental levels as in previous years. There were no detections of I-131 or Cs-137. Figure G-2 shows that Sr-90 and elemental calcium are at a level comparable to previous years and there were no detections of Sr-89. These graphs indicate that there was no appreciable difference between the levels of activity of the nearest producer and the commercial producers. This indicated no effect on

{ milk samples from the operations of CNS.

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l H. GROUNDWATER (See Tables H-1 and H-2)

STATIONS 11. 47 Groundwater was collected from two stations quarterly and analyzed for gross beta and gross alpha activity, for tritium and for gamma emitting ra-dionuclides. Station 11 is 0.15 miles from the plant and station 47 is 25.8

. miles from the plant.

The gross beta activity averaged 8.5 pCi/ liter which is statistically similar l . to past y ars. There was no detection of gross alpha above the normal level of detection There were no detections of gamma emitters above the normal level of detection. The tritium level averaged 100 pCi/ liter for the year which is the normal environmental level.

There was no difference in levels of beta activity or tritium for the sta-tion close to the plant as compared with the more distant station. It may be concluded that there was no impact from the operations of CNS on the envi-ronment as shown by measurements of radionuclides in groundwater.

Shown in Figure H-1 are the gross alpha, gross beta and tritium levels in groundwater. The levels of these activities have remained essentially un-changed.

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I. RIVER WATER (See Table 1-1 and I-2)

STATIONS 12. 28 River water was collected monthly and monitored for gross beta and gross alpha, suspended and dissolved, Sr-89 and Sr-90 plus gamma emitting isotopes. A quarterly composite was measured for tritium.

There were no detections of potassium-40 above the normal level of de-tection and no detections of Sr-89. Strontium-90 was detected in one sample at Station 28 at a level of 0.34 pCi/l.

The average gross alpha and gross beta readings were similar to previous years as indicated in the summary of 1996 and 1997 averages below:

1996 1997 Average pCi/ liter Average pC1/ liter Gross Alpha 3.7 3.1 (dissolved)

Gross Alpha 4.8 1.7 (suspended)

Gross Beta 11.0 9.8 (dissolved)

Gross Beta 11.6 4.6 (suspended)

Figure I-1. which follows, is a plot of the gross alpha and gross beta of suspended and dissolved particles. The levels of activity continued to rise and fall within statistical limits depending on water levels and turbulence and were probably due to naturally occurring isotopes. No fission or reactor activation products were detected. Figure I-2 illustrates the level of activity for tritium, Sr-89 and Sr-90.

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J. AMBIENT RADIATION - THERMOLUMINESCENT DOSIMETERS fTLDs - See Tables J-1 AND J-2)

STATIONS 01-10. 20. 44. 56. 58. 59. 66. 67. 71. 79-91. 94 Ambient radiation was monitored at 32 locations within a 10 mile ra-dius of CNS and collected quarterly. The quarterly averages for all stations of ambient net gamma radiation ranged from 13.1 milliroentgen / quarter to 20.0 milliroentgen / quarter. The highest exposure during each of the four

quarters was at Station 84 (4.4 miles, 297 degrees) and averaged 20.0 mR/ quarter. The lowest exposure was at Station 03 (2.5 miles, 338 degrees)

averaging 15.7 milliroentgen / quarter.

The radiation at station 44, (10.5 miles, 270 degrees) which is the control station, was an average of 19.6 mR/ quarter. 'Ihis was similar to other stations and to the average of all stations which was 17.6 mR/ quarter.

The average total exposure for the year was 70.6 mR which is consid-erably below the 125 millirems per quarter specified in 10 CFR 20.105 for an unrestricted area. The relationship between milliroentgen (mR) and millirems (mr) is approximately one for the exposure conditions encoun-tered. No plant effect from CNS was indicated.

The gamma exposures monitored by thermoluminescent dosimeters from 1977 through 1997 are plotted on Figure J-1. 'Ihe data from year to year is in good agreement and indicates no adverse changes in radiation ex-posure to the population near CNS.

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K. VEGETATION. BROADmAF (See Tables K-1 and K-2)

STATIONS 28. 96. 101 Broadleaf vegetation was collected each month from May through October. Three samples were collected each month from each station plus a quality control sample. The samples were tested for I-131 by chemical sepa- -

ration and for gamma emitting isotopes by high resolution spectrometry.

The naturally occurring isotopes Be-7, K-40, and Th-228 were de- -

tected in the samples at normal environmental levels. Radium-226 was

detected in one sample with an average of 0.34 pCi/g wet. No 1-131 was de-tected in any of the 60 samples. No Cs-137 was detected. Cesium-137 is detected in other areas of the United States and is attributed to fallout from ,

previous atomic weapons testing.

See Figure K-1 for the levels of activities in food samples as repre-sented in broadleaf vegetation in 1997.

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L SHORELINE SEDIMENT STATION 28 Shoreline sediment samples were collected in the spring and fall from Station 28,1.8 miles,150 degrees downstream of the release point of CNS.

They were analyzed for gamma emitters by means of a high resolution ganuna spectrometer. In the samples collected the naturally occurring isotopes Be-7, K-40, Ra-226 and Th-228 were detected at normal environmental levels. .

Cesium-137, a fission product, was detected at an average level of 0.065 -

pCi/gm dry.

Potassium-40 was detected at 16.8 pCi/gm, dry in the second quarter -

and 0.38 pCi/gm, dry in the fourth quarter. Radium-226 was detected at about the same level in the fourth as in the second quarter. Thorium-228 had an average level of 0.67 pC1/gm dry for the year. Beryllium-7 was detected at a level of 0.22 pCi/gm, dry in the second quarter but was below the detection limit in the fourth quarter. The average manganese-54, an activation product, was detected at a level of 0.014 pCi/gm, dry. All other nuclides were below the detection limit for both the spring and fall.

Presented in Figure L-1 are the plots of the radionuclides K-40,1-131, Cs-134 and Cs-137 in shoreline sediment since 1985. No detections of 1-l 131 nor Cs-134 were seen and K-40 was at a normal environmental level.

The Cs-137 was at a low level which is found in many areas and media. Since sediment tends to trap and retain any elements in the water pathway, it acts as a good indicator of the effects on the water pathway of any reactor efflu-ents.

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SECTION VII COMPLETE DATA TABLES O

O

. I 4

1 i

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l REFERENCES

1. Nebraska Public Power District, Cooper Nuclear Station Environmental Radiation Monitoring Program, Annual Report, January 1, 1982-

. December 31,1982 (prepared by Teledyne Isotopes).

2. Nebraska Public Power District, Cooper Nuclear Station Environmental

, , Radiation Monitoring Program, Annual Report, January 1, 1983-December 31,1983 (prepared by Teledyne Isotopes).

3. Nebraska Public Power District Cooper Nuclear Station Environmental

, Monitoring Program, Annual Report, January 1,1984 to December 31, 1984. (Prepared by Teledyne Isotopes).

4. U.S. Department of Energy; EML 440 March 1985; EML-444 April 1989; Environmental Measurements Laboratory, US Department of Energy, New York, New York 10014.

5. U.S. Environmental Protection Agency; Environmental Radiation Data, Report 35. July -- September 1983, Report 39, July -- September 1985; Report 40. October -- December 1984; Report 41, January -- March 1985. Report 42 April -- June 1985; Report 43, July-September 1985, Report 44-45. October-March 1986; Report 46, April-June 1986; Report 47, July-September 1986; Report 48, October-December 1986; Report 49, January-March 1987. Environmental Radiation Facility, Montgomery, Alabama.

6. U.S. Department of Energy; EML 460, October 1,1986; Environmental Measurements Laboratory, US Department of Energy, New York, New York 10014.

7. U.S. Nuclear Regulatory Commission,1975. Regulatory Guide 4.8, Environmental Technical Specifications for Nuclear Power Plants.

O 191

APPENDIX e

e e

'A

't.

O e

4 0

APPENDIX A LAND USE CENSUS O

e 9

4 e

A-1

CNS ANNUAL LAND USE CENSUS June 23,1997 -

0-3 Miles Cooper Nuclear Station (CNS) Radiological Effluent Technical Specifications (RETS) requires that an annual land use census be conducted. This census identifies the location of the nearest garden that is greater than 500 square feet in area and yields leafy green vegetables, the nearest milk animal, and the location of the nearest resident in each of the 16 meteorological sectors ,

within three miles of CNS.

In accordance with CNS RETS, a land use census was performed on June 23,1997. The nearest residence to CNS is in sector 'Q',0.9 miles from CNS, and the nearest garden to CNS is in sector 'M',1.2 miles from CNS.

No milk animals were found within 3 miles of CNS in 1997, and there was no evidence of potable water use noted from the Missouri River within three miles downstream of CNS.

l l

e I

A-2 L -- _ _ - _ _ _-___ - ____-__________-________________________ _ __________ ____

CNS ANNUAL LAND USE CENSUS June 23.1997 0-3 Miles 1

SECTOR NEAREST RESIDENT DIRECTION NEAREST GARDEN DIRECTION MILK ANIMAL e

A 3.0 Miles 1.0 J.0 Miles '1.0 NONE B 2.7 Miles 13.0 NONE --

NONE C NONE --

NONE --

4- NONE D 1.7 Miles 62.0 NONE --

MNE E 1.8 Miles 94.0 1.8 Miles 94.0 NONE F 2.4 Miles 112.0 2.4 Miles 112.0 NONE G 2.9 Miles 138.0 NONE --

NONE H NONE -- NONE --

NONE J NONE --

NONE --

NONE K 2.0 Miles 208.0 NONE --

NONE L 1.3 Miles 221.0 1.3 Miles 221.0 NONE M 1.2 Miles 251.0 1.2 Miles 251.0 NONE N 1.0 Miles 266.5 2.9 Miles 272.0 NONE P 1.6 Miles 294.0 2.3 Miles 295.0 NONE Q- 0.9 Miles 307.0 2.8 Miles 322.0 NONE R 1.8 Miles 331.0 1.8 Miles 331.0 NONE A-3

APPENDIX B INTERLABORATORY COMPARISON PROGRAM 9

0 0

I 1

l 1

i l

2 8

O e

B-1

1997

)

l A summary of the Results of the Analyses by Teledyne Brown Engineering -

Environmental Services of the EPA and Analytics, Inc. Cross Check Samples Compared with the Known Activity as reported by the Environmental .

Monitoring Systems Laboratory, Las Vegas, Nevada and Analytics, Inc.

All results which exceed three sigma deviation from the known are ap-pended with a note giving the possible cause of the deviation and corrective action taken.

O e

B-2

EPAINTERLABORATORY COMPARISON PROGRAM 1997 Environmental Teledyne Brown Collection Engineering Result (b) Deviation (c)

Media Nuclide EPA Result (a)

Date 5.0 10.00 i 1.00 -0.69 Water Sr-89 12.0 t 0.00 01/17/97 25.0 5.0 25.00 1.00 Sr-90 8.10 i 0.89 1.00 Gross Alpha 5.2 i 5.0 0.10 01/31/97 Water 5.0 15.00 i 1.00 Gross Beta 14.7 i 9.0 106.00 1 4.36 3.85 (d)

Water I-131 86.0 i 02/07/97 5.27 0.23 -1.22 Ra 226 5.9 1 0.9 0.16 02/14/97 W ater 8.2 i 2.1 8.40 i 0.30 Ra-228 7366.67 i 378.59 -1.17 Water H-3 7900.0 1 790.0 03/07/97 103.33 i 5.77 0.14 Gr-Beta 102.1 i 15.3 -0.35 04/15/97 Water 5.0 23.00 i 1.00 Sr-89 24.0 1.15 -0.12 13.0 i 5.0 12.67 Sr 90 22.67 i 0.58 0.58 Co-60 21.0 i 5.0 -0.81 5.0 28.67 i 0.58 Cs-134 31.0 i 1.53 0.92 22.0i 5.0 24.67 Cs-137 54.67 1.53 0.96 Gr-Alpha 48.0 i 12.0 0.00 2.0 13.00 i 1.00 Ra-226 13.0 0.12 3.82 (e) i 3.1 i O.8 4.87 Ra-228 19.00 i 0.00 0.35 Co-60 18.0 i 5.0 -0.12 06/06/97 W ater 10.0 99.33 i 1.15 Zn-65 100.0 i 1.15 -1.15 22.0 1 5.0 18.67 Cs-134 48.67 i 0.58 -0.12 Cs-137 49.0 1 5.0 -0.92 5.0 22.33 i 2.52 Ba-133 25.0 i 3.43 1 0.49 1.50 ,

Ra-226 3.0 1 0.5 0.72 06/13/97 Water 0.8 3.43 1 0.23 Ra-228 3.1 2.93 0.25 -0.06 Gr-Alpha 3.1 i 5.0 0.38 06/18/97 Water 5.0 14.00 i 1.00 Gr-Beta 15.1 1 38.33 i 1.53 -1.96 Sr-89 44.0 i 5.0 3.12 (f) 07/11/97 Water 5.0 25.00 t 0.00 Sr-90 16.0 0.00 1.56 11010 1101.0 12000.00 Water H-3 08/08/97 20.00 t 1.73 0.00 Ra-226 20.0 i 3.0 -0.52 09/12/97 Water 2.0 7.40 0.17 Ra-228 8.0 1 11.00 i 0.00 0.29 1-131 10.0 i 6.0 09/19/97 Water

Footnotes are located at end of table.

B-3

EPA INTERLABORATORY COMPARISON PROGRAM 1997 Environmental Teledyne Brown Collection Engineering Result (b) Deviation (c)

Media Nuclide EPA Result (a)

Date 21.5 136.67 i 5.77 -0.54 Water Gr-Beta 143.4 i 0.00 10/21/97 36.0 5.0 36.00 i 1.00 Sr-89 2.08 -0.12 Sr-90 22.0 i 5.0 21.67 5.0 10.67 1 0.58 0.23 Co-60 10.0 i 0.12 41.0 5.0 41.33 i 0.58 -

Cs-134 0.69 Cs-137 34.0 i 5.0 36.00 i 1.00 49.9 i 12.5 45.67 i 1.15 -0.59 Gr-Alpha 0.10 1.95 5.01 0.8 5.90 .

Ra-226 0.12 -0.98 5.0 i 1.3 4.27 Ra-228 5.0 19.67 1.53 1.72 Water Gr-Alpha 14.7 10/31/97 48.9 5.0 50.67 3.51 0.61 I Gr-Beta 5.0 25.00 1 1.00 -0.69 Water Co-60 27.0i 11/07/97 8.0 71.00 i 3.61 -0.87 Zn-65 75.0 t 0.23 10.0 5.0 10.67 0.58 Cs-134 1.00 0.69 Cs-137 74.O i 5.0 76.00 i 10.0 78.67 i 0.58 -3.52 (g) i Ba-133 99.0 i I

Footnotes:

I (a)

EPA Results-Expected laboratory precision (1 sigma). Units are pC1/ liter for water and milk except K is in mg/ liter. Units are total pCi for air p. rticulate filters.

(b) Teledyne Results - Average i one sigma. Units are pCi/ liter for water and milk except K is in mg/ liter. Units are total pCi for air particulate filters.

l I

l (c) Normalized deviation from the known.

(d)

Erroneously high reading of the stable iodine content by ton specific electrode occurred.

causing an erroneously low chemical yield. If the electrode reading is ignored, the average i-131 result becomes 90 pCi/1, in good agreement with the given value. An erroneous electrode reading can be caused by certain chemical species in the sample, such as sulfide. We will investigate suspiciously high electrode readings by performing a gravimetric yield on the

sample without the addition oflodide carrier or the I-131 content of active samples can also be verifled by perfonning a gamma spectral analysis.

(e) An investigation discovered a low chemical yield on one sample and the loss of another during analysis. In the future we will repeat analyses of samples with yields less than 85%. ,

(f) Error apparently caused by insufficient training. The strontium separation chemistry was performed on 7/22/97 by a summer employee. Initial results for the three samples did not agree well, so all were remilked by a senior analyst. This was insufficient to correct the There will be problem. In-house QC samples showed satisfactory results at this time.

additional qualification of analysts according to performance on in-house blanks and spikes.

(g) An investigation is being conducted; results will be available shortly.

1 B-4

ANALYTICS CROSS CHECK COMPARISON PROGRAM 1997 Teledyne Brown Analytics Sample ID Media Nuclide Engineering Result (a) Result Ratio (b)

E0975-396 Milk I-131 18 i 1 20 i 1 0.90 T1#41238 Cc-141 L.T.1. 2321 12 ---

03/20/97 Cr-51 381 38 387 i 19 0.98 Cs-134 132 13 143 i 7 0.92 Cs-137 128 13 114 i - 6 1.12

Co-58 89 i 9 79d 4 1.13 Mn-54 195 i 20 176i 9 1.11 Fe-59 161 i 16 144i 7 1.12

. Zn-65 171 17 1651 8 1.04 CO-60 179 18 176 9 1.02 EO976-396 Milk Sr-89 13 i 3 25 i 1 0.52 (c)

TI#41239 Sr-90 16 i 1 19 i 1 0.84 03/20/97 E1092-396 Air Filter Ce-141 143 8 1321 7 1.08 TI #49899-901 Cr-51 229 17 198 i 10 1.16 Cs-134 74 i 4 81 4 0.91 06/19/97 115i 6 1.24 Cs-137 143i 8 Co-58 89 5 77 i 4 1.16 Mn-54 1021 6 84 1 4 1.21 Fe-59 98 i 6 75 i 4 1.31 Zn 65 188 i 11 1391 7 1.35 Co-60 1131 7 1041 5 1.09 Cartridge I-131 106i 6 88 4 1.20 E1093-396 TI #49902-04 06/19/97 Elli94-396 Air Filter Sr-90 88 i 5 96 i 5 0.92 T1 #49893-95 06/19/97 E1095-396 Air Filter Gross Alpha 103 i 6 93 i 5 1.11 Gross Beta 210 6 1931 10 1.09 ,

11 #49896-98

. 06/19/97 10 87 i 4 1.11 E1204-396 Milk I-131 97 i 77 4 1.08

'Il#57520 Ce-141 83 1 8 Cr-51 323 i 40 304i 15 1.06 ;

09/18/97 10 1021 5 0.96 i Cs-134 98 1 !

117 12 1071 5 1.09 Cs-137 6 60 i 3 1.07 !

Co-58 64 i 99 i 10 88 i 4 1.13 Mn-54 132 13 119i 6 1.11 Fe-59 218 i 22 196i 10 1.11 Zn 65 209 i 21 197 10 1.06 Co-60 B-5

ANALYTICS CROSS CHECK COMPARISON PROGRAM 1997 Teledyne Brown Analyucs Sample ID Media Nuclide Engineering Result (a) Result Ratio (b)

E1203-396 Milk Sr-89 14 1 1 15 i 1 0.93 .

"Il#57517 Sr-90 18 1 1 14 i 1 1.29 09/18/97 Footnotes:

(a) Teledyne Results - counting error is two standard deviations. Units are pCi/ liter for water and milk. For gamma results, if two standard deviations are less than 10%. then a 10% error is reported. Units are total pCi for air particulate filters.

(b) Ratio of Teledyne Brown Engineering to Analytics results.

(c) Caused by incorrect rinsing of the strontium extraction column. Additional training was conducted on 9/5/97 and was documented in the analyst's training file. Subsequent tests on two milk samples spiked with Sr-89 produced good results.

Note: Ce-141 was identified by gamma spectrometry system (232123 pC1/1) for the 3/20/97 milk sample. but was not reported to Analytics.

I 1

O l

B-6

x r s APPENDIX C STATISTICAL NOTES

1. Each activity is reported in one of two forms:

x

s or

<L, '

where l

x = value of measurement; .

s = counting error at the 95%

confidence level (2 sigma error); .

L = detection limit based on 4.66 sigma error for counter background

2. All activities are corrected to collection time except for gross alpha and gross beta.

3. Computation of means:

(a) In any statistical table, the values are entered as 7 s or <L where x = sample mean = Ix; n

n = number of data points averaged; s = average of the 2 sigma counting errors = Is n

(b) For gross beta and gross alpha results in air particulates, averaging ;

includes values which are less than the lower limits of detection. -

i The detection limit is used as the sample activity in these cases.

{

(c) In all cases, if all values in an averaging group are below detec-tion limits, the highest of the detection limits is reported as a "less than" value without an associated tolerance. If some values are above detection limits and some are below, then:

l l C-1

l

\

l l

APPENDIX C STATISTICAL NOTES l 8 O

l l

l t

i O

I

l l

____________._________________._________.____.____.___J

(1) The mean of the positive results is reported and the number of positives is listed in parentheses.

(d) Means are reported on a quarterly basis except for air particulate and airborne iodine data which are reported monthly. For air particulate and charcoal filters, data for samples collected on the 1st, 2nd, and 3rd day of a month are assigned to the previous month.

, (e) In rounding off, numbers followed by a 5 or higher digit are rounded upwards.

e 4

4 C-2 I

1 1

1 l

l 1

1 L

Appendix 0

. Notification Levels l

l l

t i

l l

\ .

1 i

S 4

1 I

l 1

NEBRASEA FUBLIC F0VER DISTRICT C00FER NUCLEAR STATION ENVIRONMENTAL RADIATION SURVEILIANCE FROGRAM NOTIFICATION LEVELS Media and Nuclide Notification Level Air 3

Cross Alpha . . . . . . . . . . . ... ... . . . . 0.1 pCi/m 3

Gross Beta. . . . . . . . . . . . ... .... . .. 1.0 pCi/m I-131 . . . .. . . . . . . . . . ... ... . . .. 0.31 pCi/m 3 .

Cs-134 . . . . . . . . . . . . .... ... . . . . 3.3 pci/m 33 Cs-137 . . . .. . . . . . . . . .. . . .. . . . . 6.7 pCi/m Milk I-131 (low level) . . . . . . . . ... . ... . . . 1.09 pCi/1 Sr-89 . .. . . . . . . . . . . . ... .... . .. 6.04 pCi/1 Sr-90 . . . . . . . . . . . . . .... ... . . . . 14.82 pCi/1 Cs-134 .. . . . . . . . . . . . ... ..... .. 20.0 pCi/1 Cs-137 . . . . . . . . . . . . . ....... . .. 23.0 pci/1 Croundwater Cross Alpha . . . . . . . . . . . .... ... . . . 12.0 pci/1 Cross Beta. . . . . . . . . . . . ....... . . . 33.8 pCi/1 H-3 . . . . . . . . . . . . . . . ... . . .. . . . 6700 pci/1 Mn-54 . .. .. . . . . . . . . . ..... . . . . . 330 pCi/1 Fe-59 . . . . . . . . . . . . . . ... . . . . . . 130 pCi/1 Co-58 . .. . . . . . . . . . . . .... . . . . . 330 pCi/1 Co-60 . .. . . . . . . . . . . . ... .. . .. .. 100 pCi/1 2n-65 . . . .. . . . . . . . . . .... .. . . . . 100 pci/1 Zr-Nb-95 . . . . . . . . . . . . ... . .. .. . . 67 pCi/1 1-131 . .. ... .. . . . . . . . ... .. . . .. 0.67 pci/1 Cs-134 .. ... . . . . . . . . ........ .. 10 pci/1 Cs-137 . . . . . . . . . . . . . .... ... . .. 17 pCi/1 Ba-La-140 . .... . . . . . . . ... . ... . .. 67 pC1/1 Food Products .

I-131 . . . .. . . . . . . . . . ... . . .. . .. 0.1 pCi/g vet Cs-134 Cs-137

. . ... . . . . . . . . .... ... . .. 0.33 pCi/g vet -

.. .. . . . . . . . . . .. .... . . .. 0.66 pCi/g wet .

Fish Cross Beta. .. . . . . . . . . . .... ... . . .

10.8 pCi/g vet Sr-89 . . . ... . . . . . . . . .... ... ...

3.3 pCi/g vet Sr-90 . . . . . . . . . . . . . . .... ... . . . 1.2 pCi/g wet Mn-54 . . . .. . . . . . . . . . ... . . . . ... 10 pCi/g vet D-1

l l

l Media and Nuclide Notification Level Fish (Continued)

Fe-59 . . . . . . . . . . . . . . .. . ... . . . . 3.3 pCi/g vet Co-58 . . . . . . . . . . . . . . . . . . .. . . . . 10 pC1/g vet Co-60 . . . . . . . . . . . .. . . . . . . . . . . . 3.3 pCi/g vet 2n-65 . . . . . . . . . . . .. . . . . . .. . . . . 6.7 pCi/g vet Cs-134 . . . . . . . . . . . . . . . . . . . . . . . 0.33 pCi/g vet

, Cs-137 . . . . . . . . . . ... . . . .. . . . . a, 0.67 pCi/g vet River Water Gross Aipha sus . . . . . . .. . ... . . . . . . . 22.0 pci/1 Gross Alpha Dis . . . . . . .. . . . . .. . . . . . 27.6 pCi/1 Cross Beta Sus. . . . . . . .. . . . . . . . . . . . 58.8 pC1/1 Cross Beta Dis. . . . . . . . . . . . . .. . . . . . 88.6 pCi/1 Sr-89 . . . . . . . . . . . . . . . . . . . . . . . . 1000.0 pCi/1 Sr-90 . . . . . . . . . . . . . . .. . . . . . . . . 100.0 pCi/1 H-3 . . .. . . . . . . . . . . . . . . . . .s . . . . 6700 pCi/1 Mn-54 . . . .. . . . . . . .. .. . . . . . . . . . 330 pCi/1 Fe-59 . . . . . . . . . . . . . . . . . . . .. . . . 130 pCi/1 Co-58 . .. . . . . . . . . . . . . . . . . .. . . . 330 pCi/1 Co-60 . . . . . . . . . . . .. . . . . . . . . . . . 100 pCi/1 Zn-65 . . . . . . . . . . . . . . . . . . . . . . . . 100 pci/1 Zr-Nb-95 . .. . . . . . . . . . . .. . . . . . . . 67 pCi/1 1-131 . . . . . . . . . . . .. . . . . . . . . . . . 0.67 pCi/1 Cs-134 . . .. . . . .. . . . . . . . .. . . . . . 10 pCi/1 Cs-137 . . .. . . . . . . .. . . .. .. . . . . . 17 pCi/1 Ba-La-140 . .. . . . . . . . . . . . . . . . . . . . 67 pC1/1 Shoreline Sediment Co-60 . . . . . . . . . . . . .. . . . .. . . . . . 0.1 pCi/g dry Cs-134 Cs-137

.. . . . . . . . . . . . . . . . . .. . . . 0.75 pCi/g dry

. . .. . . . . . . .. . . . . . . . . . . . 0.75 pCi/g dry O

D-2

e i

I l

~

APPENDIX E CONVENTIONS USED IN DATA TREND GRAPHS

/

1 1

1 e

l a

. l I

l

APPENDIX E Conventions used in Data Trend Graphs

1. The data trend plots are based on statistical summaries of Section VI. .

2. Monthly or quarterly averages are plotted.

3. The conventions used to determine if a "less than" (<) value or detectable result is plotted are those given in Appendix C. .

4. Iowest levels of detection (LLD) are noted by a straight line on the graphs.

5. A typicalless-than value arising from delayed counting of short-lived isotopes (such as 1-131 or Ba-140) or reduced sample size are omitted.

e e

E-1

1 I

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I O

AFFENDIX F 1 DETECTION CAPABILITIES l

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n s o dq .

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l l yw do e r c rt emaahnt l d

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_ Q A 'o $ Q A S S Q I H Lfo eThTTLi I

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LLD = lower limit of detection based on 4.66sb ; & where sb is the standard deviation.of the background counting rate or of

the counting rate of a blank sample as apprdbriate (as counts per minute) . The LLD is at counting time and must be corrected to collection time. The LLDs given above are based on the quantities indicated and the background count rate in the absence of any radionuclides in the sample. In

'

calculating the LLD for a radionuclide determined by gamma-ray spectrometry, the background shall include the typical contributions of other radio-nuclides normally present in the samples (e.g. , potassium-40 in milk samples) .

occasionally background fluctuations, unavoidably small sample sizes, the presence of interfering nuclides, or other uncontrollable circumstances may render these LLD's unachlevable. In such cases, the contributing factors will be identified and described in the Environmental Radiation Monitoring Program Annual Report.

Note:All LLD's which we require are listed in this table for Ge(Li) Gamma Spectroscopy. If any nuclide is detected, it shall be reported quantitatively whether or not it is one of the 20 nuclides listed above.

i W

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APPENDIX G SAMPLE STATION LOCATIONS AND SAMPLE TYPES G

G O

4 e

COOPER NUCLEAR STATION LIST OF ACTIVE SAMPLE STATIONS 1997 Sample Station

Sample Description -- Type and Location No. 1 Types (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry .

Location: Outside the northwest edge of fence, east of the gate to the LLRW storage pad on the CNS site, NW%, S32, T5N, R16E, Nemaha County, Nebraska. ,

No. 2 Type: (1) Air Parciculate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry Location: North side of county road access to the south portion of CNS site approximately 275 feet west of the former Jefferson Broady farmstead, SWM, S32, TSN, R16E, Nemaha County, NE.

No. 3 Type: (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry Location: Located on the north side of the Brownville State Recreation Park access road near water gauging station, SE%, .S18, T5N, R16E, Nemaha County, Nebraska.

No. 4 Types (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry Location: Located % mile south of Phelps City, Missouri, on west side of Highway "U", NE%, S2, T64N, R42W, Atchison County, Missouri.

No. 5 Type: (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry Location: Located % mile south and % mile east of Langdon, Missouri, on north side of road, west of railroad tracks, SW%, S18, T64N, R41W, Atchison County, Missouri.

No. 6 Type: (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry Location: One mile west of the end of Missouri State Highway "U", south ,

side of road, SW corner of the intersection, NW%, S34, T64N, R42W, Atchison County, Missouri.

No. 7 Type: (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry .

Location: 300 yards east of Highway 67 on north side of road, west of Nemaha elevator, SW%, S6, T4N, R16E, Nemaha County, Nebraska.

G-2

Scmple

. Station Samole Descriotion -- Tvoe and Location No.'8 Types (1) Air Particulate and Charcoal Filters (2) Environmental Thermoluminescent Dosimetry Location: % mile north, % mile west and % mile north of Nemaha, on west-

' side of road adjacent to Mark T. Moore Transmission Line, NE%,

S35, TSN, R15E, Nemaha County, Nebraska.

4 No. 9 Types (1) Air Particulate and Charcoal. Filters (2) Environmental.Thermoluminescent Dosimetry a

Location: Four miles north of Highway 136, on Highway 67. Then 1 mile-

, east of Highway 67 and % ndle north on west side of road, SWM, S26,.T6N, R15E, Nemaha County, Nebraska.

No. 10 Type .(1) Air Particulate and Charcoal Filters (2) Environmental Thenmoluminescent Dosimetry Location; One mile north of Barada, Nebraska, in SW corner of intersection, NEM, S14, T3N, R16E, Richardson County, NE.

No. 11 Type: (1) Water - Ground Location: Plant well water supply header at well pits, NW%, S32, T5N, R16E, Nemaha County,-Nebraska.

No. 12 Types (1) Water - River Location: Sample (1) is taken from the Missouri River immediately upstream from the Plant Intake Structure-(River Mile 532.5).

(During periods when unsafe conditions warrant, Station 35 nay be used as an alternate upstream collection site.)

No. 20 Types (1) Environmental.Thermoluminescent Dosimetry Location: On NNW boundary of NPPD property, approximately 20 yards east of county road, SE%, S30, T5N, R16E, Nemaha county, NE.

No. 28 Type: (1) Water - River (2) Fish (3) Sediment from Shoreline j- (4) Food Products - Broadleaf Vegetation

! I Location: Samples (1) and (3) are taken from the Missouri River or its '

j .* shore, below the Plant Discharge Flume near River Mile 530.

l- Sample (2) is taken from the Missouri River % to 3 miles ;

l downstream of the plant site. j No. 35 Type: (1) Fish I (2) Water - River (Alternate Site)

Location: Sample (1) is taken from the Missouri River about 1 to 3 miles

, above the CNS intake structure. Sample (2) is taken about M l mile south of the Brownville State Recreation Area in Sector A. During periods when unsafe cotiditions warrant, Station 35 may be used as an alternate to Station 12 for sample type (3).

1 G-3 l

Sample Station Sample Description -- Tvoe and Locatio_r1 No. 44 Types (1) Environmental Thermoluminescent Dosimetry Location: Two miles south of Auburn stoplight and % mile south of Auburn Country Club on Highway 75, then % mile east of Highway 75 at fence line north of county road, SEM, S27, T5N, R14E, Nemaha County, Nebraska.

No. 47 Type: (1) Water - Ground Location: At Falls City municipal water supply well south of Rulo, Nebraska, out of main header flow meter, SW%, S20, T1N, R18E, Richardson County, Nebraska.

No. 56 Type: (1) Environmental Thermoluminescent Dosimetry Location: 1-% miles SW of Langdon, Missouri, on Highway "U", on the

right side of the highway (Bill Gebheart farm), NW%, S23, T64N, R42W, Atchison County, Missouri.

No. 58 Type: (1) Environmental Thermoluminescent Dosimetry Location: Three miles south'of Bro'vnville, Nebraska, on county road, at the SE corner of the intersection with the farm road leading to Sample Station No. 2, SE%, S31, T5N, R16E, Nemaha County, Nebraska.

No. 59 Types (1) Environmental Thermoluminescent Dosimetry Location: One mile SSE of the CNS Elevated Release Point, 50 yards west of the levee at the south boundary of NPPD property, SEM, S32, TSN, R16E, Nemaha County, Nebraska.

No. 61 Type: (1) Milk - Nearest Producer Location: One mile west of Brownville, Nebraska, on Highway 136, then 1 mile north on the county road, turn right and proceed approximately % mile east, on south side of road (Raymond Gentert dairy), NW%, S13, T5N, R15E, Nemaha County, Nebraska.

No. 66 Type: (1) Environmental Thermoluminescent Dosimetry Location: Two miles south of Nemaha, Nebraska, on Highway 67 - east side j of road (Mrs. Lola Kennedy farm), NW%, S19, T4N, R16E, Nemaha l County, Nebraska.

No. 67 Type: (1) Environmental Thermoluminescent Dosimetry Location: 2 miles west of Brownville, Nebraska, on Highway 136, then ,

north 1-% miles on county road and east % mile, on north side of road (Walter Parkhurst farm), NE%, S11, T5N, R15E, Nemaha

County, Nebraska, No. 71 Type: (1) Environmental Thermoluminescent Dosimetry .

Location: Two miles east of Phelps City, Missouri, on Highway 136, then south 1-% miles on county road and west % mile (Tom Boatman farm), SE%, S6, T64N, R41W, Atchison County, Missouri.

G-4

Scmple Station Sample Descrintion -- Tyne and Location No. 79 Types (1) Environmental Thermoluminescent Dosimetry Location: 1-7/8 miles south of Brownville, NE, on east side of paved 1

road, NPPD property, SE%, S30 TSN, R16E, Nemaha County, NE.

No. 80 Type (1) Environmental Thermoluminescent Dosimetry

. Location: 2-1/8 miles south of Brownville, east side of paved road, NPPD property, NE%, S31, T5N, R16E, Nemaha County, Nebraska.

No. 81 Type: (1) Environmental Thermoluminescent Dosimetry l

Location: 2-3/8 miles south of Brownville, Nebraska, in the NE corner of the intersection of the paved county road and CNS access road, NPPD property, NE%, S31, T5N, R16E, Nemaha County, Nebraska.

No. 82 Type: (1) Environmental Thermoluminescent Dosimetry Location: 7/8 mile south of CNS in a field, on NPPD property, SW%, S32, T5N, R16E, Nemaha County, Nebraska. 1

)

No. 83 Type: (1) Environmental Thermoluminescent Dosimetry Location: 2-% miles south of Nemaha, Nebraska, on Highway 67, then east 1 mile to the junction of the driveway and county road (east side of drive, Leroy Kennedy), NE%, S19, T4N, R16E, Nemaha County, Nebraska.

No. 84 Type: (1) Environmental Thermoluminescent Dosimetry Location: 2-M miles west of Brownville, Nebraska, south side of Highway 136 west of Locust Grove School (Bruce L. Solie), NW%, S22, T5N, R15E, Nemaha County, Nebraska.

No. 85 Type: (1) Environmental Thermoluminescent Dosimetry Location: One mile east of Brownville, Nebraska, on Highway 136, then north % mile on the east side of the county road (Scott Leseburg), NE%, S33, T65N, R42W, Atchison County, Missouri.

No. 86 Type: (1) Environmental Thermoluminescent Dosimetry l

Location: One mile west of Phelps City, Missouri, on Highway 136, then north 1-% miles on Highway "D" on west side (Mrs. Olin e Harmes), SE%, S22, T65N, R43W, Atchison County, Missouri.

No. 87 Type: (1) Environmental Thermoluminescent Dosimetry l Location: One mile west of Phelps City, Missouri, on Highway 136, south

% mile on county road and % mile west on county road (to end of road, Robert Graf), SW%, S3, T64N, R42W, Atchison County, Missouri.

No. 88 Type: (1) Environmental Thermoluminescent Dosimetry Location: One mile west of Phelps City, Missouri, on Highway 136, then

.outh 2 miles at the end of the county road (David Meyerkorth), NW%, S11, T64N, R42W, Atchison County, Missouri. '

G-5

Samplo Station Samole Descriotion -- Tvoe and Location i

No. 89 Types (1) Environmental Thermoluminescent Dosimetry Location: 2-% miles south of Phelps City, Missouri, on Highway "U", then

% mile west in the SE corner of the county road intersection (Gertrude Rosenbohm), NE%, S14, T64N, R42W, Atchison County, Missouri.

No. 90 Type: (1) Environmental Thermoluminescent Dosimetry ,

Location: 1-% miles west and % mile south of Langdon, Missouri, on Highway "U*, then % mile west (Garth Green), SW%, S23, T64N, R42W, Atchison County, Missouri.

No. 91 Type: (1) Environmental Thermoluminescent Dosimetry Location: % mile west of Rock Port, Missouri, on the south side of the intersection of Hwy. 136 and Hwy. 275, at the water tower (Richard H. and Vicki Cook), NW%, S28, T65N, R41W, Atchison County, Missouri.

No. 94 Type: (1) Environmental Thermoluminescent Dosimetry Location: M mile south of Langdon, Missouri, on the west side of the road (Max Peeler), NEM, S24, T64N, R42W, Atchison County, Missouri.

No. 96 Type: (1) Food Products - Broadleaf Vegetation Location: Approximately 1 mile south of Brownville, Nebraska, along the paved road in the road ditch, in Sector R, SW%, S19, TSN, R16E, Nemaha County, Nebraska.

No. 99 Type: (1) Milk (other Producer)

Location: 1-% miles south of Shubert, Nebraska, west side of Hwy. 67 (James Zentner dairy), NE%, S24, T3N, R15E, Richardson County, Nebraska.

No. 100 Type: -(1) Milk (Other Producer)

Location: Two miles south and 1 mile west of Shubert, Nebraska (Dick James dairy), SWM, S23, T3N, R15E, Richardson County, Nebraska.

I No. 101 Types (1) Food Products - Broadleaf Vegetation

Location: 5% miles east and % mile north of Rock Port, Missouri, near the junction of Highway 136 and Highway 59, in Sector D, ,

encompasses portions of S19 and S30, T65N, R41W, Atchison County, Missouri.

NOTES:

Sample Station numbers missing from the sequence are inactive or discontinued Sample Stations.

l:

i G-6

APPENDIX H

SUMMARY

OF DOSES TO A MimtRR OF THE PUBLIC OFF-SITE t

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APPENDIX I One water sample from the LL Waste Pad location was collected in 1997 and analyzed for gross alpha and gross beta suspended and dissolved and by .

gamma spectroscopy. These analyses are not part of the REMP.

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