ML20155G186

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Environ Radiological Monitoring Rept for Louisiana Power & Light Waterford Steam Electric Station,Unit 3,1985
ML20155G186
Person / Time
Site: Waterford Entergy icon.png
Issue date: 12/31/1985
From: Cook K
LOUISIANA POWER & LIGHT CO.
To: Martin R
NRC OFFICE OF INSPECTION & ENFORCEMENT (IE REGION IV)
References
W3P86-0078, W3P86-78, NUDOCS 8605050048
Download: ML20155G186 (172)


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ENVIRONMENTAL RADIOLOGICAL MONITORING REPORT FOR THE LOUISIANA POWER AND LIGHT WATERFORD STEAM ELECTRIC STATION, UNIT 3 JANUARY 1 THROUGH DECEMBER 31, 1985 4

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ENVIRONMENTAL RADIOLOGICAL MONITORING REPORT FOR THE LOUISIANA POWER AND LIGHT WATERFORD STEAM ELECTRIC STATION, UNIT 3 JANUARY l THROUGH DECEMBER 31, 1985 PREPARED BY:

w V' 29 Y86 H. C. '% DATE L'esaQ REVIEWE BY:

E. M. llins '

Y S $k

' DATE Radia n Control Unit Coordinator APPROVED BY:-/ A 2 [> [ f K. R. Iyengar DATE Nuclear Support Manager

ABSTRACT This report is issued pursuant to Waterford 3 SES Technical Specification 6.9.1.7. Its purpose is to discuss the Waterford 3 SES Radiological Environmental Monitoring Program (REMP), present the results of the program for the year of 1985, and to evaluate the radiological impact on the environment resulting from plant operation. The Waterford 3 SES REMP collected data on environmental radio-activity levels around the Waterford 3 SES nuclear power plant. These levels were determined by analyzing samples of air, water, shoreline soil, fish, vegetation, and milk from various locations around the facility. Based on the evaluation of these analyses, the operation of Waterford 3 SES exhibited no discernable impact on the levels of radioactivity in the environment during 1985. i l l l

TABLE OF CONTENTS PAGE ABSTRACT . . . . . . . . . . . . . . . . . . . . . . . . . . 11 TABLE OF CONTENTS . . . . . . . . . . . . . . . . . . . . . iii LIST OF TABLES . . . . . . . . . . . . . . . . . . . . . . . V

                                                                                                               )

LIST OF FIGURES . . . . . . . . . . . . . . . . . . . . . . vii

1.0 INTRODUCTION

.       . . . . . . . . . . . . . . . . . . . . .                         1 1.1 Program and Report Objectives              . . . . . . . . . . .                 1 1.2 Plant and Site Description .              . . . . . . . . . . .                  1 2.0 PROGRAM DESCRIPTION          . . . . . . . . . . . . . . . . . .                       3 2.1 History and Development .            . . . . . . . . . . . . .                   3 2.2 Sample Collection and Handling Procedures .                       . . . .        3 2.2.1 Direct Radiation Exposure. Pathway Samples     . . . . . . . . . . . . . . . . . .                       4 2.2.2 Airborne Exposure Pathway Samples . . . . .                              4 2.2.3 Waterborne Exposure Pathway Samples . . . .                              5 2.2.4 Ingestion Exposure Pathway Samples . . . . .                             6 2.3 Analytical Procedures . . . .            . . . . . . . . . . .                   7 2.4 Laboratory Quality Assurance               . . . . . . . . . . .                 7 3.0 DISCUSSION OF RESULTS             . . . . . . . . . . . . . . . . .                 23 3.1 Direct Radiation Exposure Pathway . . . . . . . . .                           23 3.2 Airborne Exposure Pathway . . . . . . . . . . . . .                           24 3.2.1 Airborne Particulates . . . . . . . . . . .                           24 3.2.2 Airborne Iodine . . . . . . . . . . . . . .                           24 3.3 Waterborne Exposure Pathway .              . . . . . . . . . . .              24 3.3.1 Drinking / Surface Water .            . . . . . . . . . .             24 3.3.2 Groundwater . . . . . . . . . . . . . . . .                           26 3.3.3 Shoreline Soil . . . . . . . . . . . . . . .                          26 3.4 Ingestion Exposure Pathway              . . . . . . . . . . . .               27 3.4.1 Milk . . . . . . . . . . . . . . . . . . . .                          27 3.4.2 Fish . . . . . . . . . . . . . . . . . . . .                          28 3.4.3 Broad Leaf Vegetation . . . . . . . . . . .                           28 3.4.4 Food / Garden Crops          . . . . . . . . . . . . .                29 3.5 Deviations from the REMP             . . . . . . . . . . . . .                29 3.5.1 Unavailable Samples             . . . . . . . . . . . .               29 3.5.2 Missed Lower Limits of Detection .                    . . . . .       30 3.5.3 Changes to the REMP             . . . . . . . . . . . .               30 3.6 Annual Land Use Census Results                . . . . . . . . . .             31 1

4.0 CONCLUSION

S . . . . . . . . . . . . . . . . . . . . . . 34  ; iii .

TABLE OF CONTENTS (CONTINUED) PAGE APPENDIX A REMP DATA

SUMMARY

.                                             . . . . . . . . . . . . . . .                                                   35 APPENDIX B REMP DATA                                       . . . . . . . . . . . . . . . . . . .                                                           41 APPENDIX C 

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED l LOWER LIMITS OF DETECTION . . . . . . . . . . . . . . . 138 APPENDIX D

SUMMARY

OF INTERLABORATORY COMPARISONS . . . . . 144 APPENDIX E SYNOPSES OF ANALYTICAL PROCEDURES . . . . . . . . 150 E-1.0 ANALYSIS OF SAMPLES FOR GROSS BETA ACTIVITY . . . 151 E-1.1 Air Particulates . . . . . . . . . . . . . . 151 E-1.1 Water . . . . . . . . . . . . . . . . . . . 151 E-2.0 ANALYSIS OF WATER SAMPLES FOR TRITIUM . . . . . . 151 E-3.0 ANALYSIS OF SAMPLES FOR IODINE-131 . . . . . . . 151 E-3.1 Milk and Water . . . . . . . . . . . . . . . 151 E-3.2 Broad Leaf Vegetation . . . . . . . . . . . 152 E-4.0 GAMMA SPECTROSCOPY ANALYSIS . . . . . . . . . . . 152 E-4.1 Milk and Water . . . . . . . . . . . . . . . 152 E-4.2 Vegetation, Food and Garden Crops,

and Fish . . . . . . . . . . . . . . . . . . 152 E-4.3 Soils and Sediment . . . . . . . . . . . . . 153 E-4.4 Charcoal Cartridges (Air Iodine) . . . . . . 153 E-4.5 Air Particulates . . . . . . . . . . . . . . 153 E-4.6 Computer Software . . . . . . . . . . . . . 153 1

E-5.0 ENVIRONMENTAL DOSIMETRY . . . . . . . . . . . . . 154 ! APPENDIX F STATISTICAL ANALYSES . . . . . . . . . . . . . . 155 ' F-1.0 CALCULATION OF MEAN AND STANDARD DEVIATION . . . 156 F-2.0 COMPARING TWO SAE LE POPULATION MEANS . . . . . . 156 F-3.0 TLD MEASUREMENTS . . . . . . . . . . . . . . . . 158 F-4.0 GROSS BETA ACTIVITY ON AIR PARTICULATE FILTERS . . . . . . . . . . . . . . . . . . . . 158 F-5.0 GROSS BETA ACTIVITY IN McNTHLY DRINKING WATER COMPOSITES . . . . . . . . . . . . . . . . 158 I I i iv

 . . . . _ _ _ . _ . _ _ _ _ . . . _ _ . .     - . _ , . . .                 . , .    . _ _ , , . .            .._ _ _ _ _.. _ ._ .._._ _ ._.._, ,,. . _ ._._ -                         _..,.....r_    , . _ . , , . , . . . - ,

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                                                                  -LIST OF TABLES
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PAGE TABLE 2.1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM (REMP)

SUMMARY

. . . . . . . . . . . . . . . . . . . .                                                                                                     9 TABLE 

2.2 DESCRIPTION

OF REMP SAMPLING STATION

 ,                LOCATIONS . . . . . . . . . . . . . . . . . . . . . . .                                                                                                  10 TABLE 2.3 DETECTION CAPABILITIES FOR ENVIRONMENTAL SAMPLE j                ANALYSIS, LOWER LIMIT OF DETECTION (LLD) . . . . . . .                                                                                                    19
;           TABLE 3.1 1985 DIRECT PADIATION, DATA ORGANIZED BY COMPASS j                DIRECTION AND DISTANCE FROM WATERFORD 3 SES . . . . . .                                                                                                  32 TABLE 3.2 1985 ANNUAL, LAND USE CENSUS RESULTS                                                                  . . . . . . .                                 33 TABLE A-1 RADIOLOGICAL ENVIRONMENTAL MONITORING PROGRAM 

SUMMARY

.                            . . . . . . . . . . . . . . . . . . .                                                                       36 TABLE B-1 QUARTERLY TLD EXPOSURES                                                                . . . .. . . . . . . . . .                                   42 TABLE B-2 AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES:

GROSS BETA AND IODINE-131 ANALYSES . . . . . . . . . . 44 TABLE B-3 AIR PARTICULATE FILTERS: GAMMA ISOTOPIC ANALYSIS OF QUARTERLY COMPOSITES . . . . . . . . . . . . . . . . 64 TABLE B-4 DRINKING WATER: IODINE-131 ANALYSIS . . . . . . . 69 TABLE B-5 DRINKING WATER: GROSS BETA AND GAMMA ISOTOPIC ) ANALYSES ON MONTHLY COMPOSITES . . . . . . . . . . . . 71 l 4 TABLE B-6 DRINKING WATER: TRITIUM ANALYSIS ON QUARTERLY COMPOSITES AND, GAMMA ISOTOPIC ANALYSIS ON FILTERS . . . 83 i TABLE B-7 SURFACE NATER: GAMMA ISOTOPIC ANALYSIS ON MONTHLY COMPOSITES . . . . . . . . . . . . . . . . . . 86 1 TABLE B-8 SURFACE WATER: TRITIUM ANALYSIS ON QUARTERLY COMPOSITES AND GAMMA ISOTOPIC ANALYSIS ON FILTERS . . . 98 TABLE B-.9 GROUNDWATER: TRITIUM AND GAMMA ISOTOPIC ANALYSES . . . . . . . . . . . . . . . . . . . . . . . 101 i TABLE B-10 SHORELINE SOIL: GAMMA ISOTOPIC ANALYSIS . . . . . 102 i TABLE B-11 MILK: IODINE-131 AND GAMMA ISOTOPIC ANALYSES . . 104 i ,* l TABLE B-12 FISH: GAMMA ISOTOPIC ANALYSIS . . . . . . . . . 122 4 s

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   - . -- ,   .     . . , _ _ _     , . . _ . , _ , , _ . . ,   ,,,..-..,-,,,..,__,,,,__m__,...,_,,,m,..__.-                             . . _ _. , ~ . _ -_ _,__. _.-

LIST OF TABLES (CONTINUED) PAGE TABLE B-13 BAOAD LEAF VEGETATION: IODINE-131 AND GAMMA ISOTOPIC ANALYSES . . . . . . . . . . . . . . . . . . . 126 TABLE B-14 FOOD / GARDEN CROPS: IODINE-131 AND GAMMA ISOTOPIC ANALYSES . . . . . . . . . . . . . . . . . . . 137 TABLE C-1

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF JANUARY 1 TO MARCH 31, 1986 . . . . . . . . . . . . . . . . . . . . 139 , TABLE C-2

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF APRIL 1 TO JUNE 30, 1985 . . . . . . . . . . . . . . . . . . . . . 140

' TABLE C-3 

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS OF DETECTION DURING THE PERIOD OF JULY l TO SEPTEMBER 30, 1985 . . . . . . . . . . . . . . . . . . 141 TABLE C-4

SUMMARY

OF UNAVAILABLE SAMPLES AND MISSED LOWER

'      LIMITS OF DETECTION DURING THE PERIOD OF OCTOBER 1 TO DECEMBER 31, 1985 . . . . . . . . . . . . . . . . . . .                                                                                                 142 TABLE C-5 

SUMMARY

OF UNAVAILABLE TLD MEASUREMENTS FOR THE PERIOD OF JANUARY l TO DECEMBER 31, 1985 . . . . . 143 TABLE D-1 US EPA CROSS-CHECK PROGRAM RESULTS FOR 1985 . . . 145 TABLE D-2 SEVENTH INTERNATIONAL INTERCOMPARISON OF ENVIRON-MENTAL DOSIMETER RESULTS . . . . . . . . . . . . . . . 149 TABLE F-1 STATISTICAL COMPARISON OF TLD MEASUREMENTS FROM i STATIONS GROUPED BY DISTANCE FROM WATERFORD 3 SES . . . 160 TABLE F-2 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY ON AIR PARTICULATE FILTERS FOR 1985 .. . . . . . . . . . 161 TABLE F-3 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY IN MONTHLY DRINKING WATER COMPOSITES FOR 1985 . . . . . . 162 TABLE F-4 STATISTICAL COMPARISON OF GROSS BETA ACTIVITY IN MONTHLY DRINKING WATER COMPOSITES FOR 1984 AND 1985 . . 163 8 vi l I

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LIST OF FIGURES PAGE FIGURE 2.1 REMP SAMPLE LOCATIONS WITHIN 2 MILES OF WATERFORD 3 SES . . . . . .... ... . .. . . . . . 20 FIGURE 2.2 REMP SAMPLE LOCATIONS WITHIN 10 MILES OF WATERFORD 3 SES . . . . . . ... . .. . .... . . . 21 FIGURE 2.3 REMP SAMPLE LOCATIONS WITHIN 50 MILES OF WATERI?ORD 3 SES . . . . . ....... ........ 22 I e i vii

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l.0 INTRODUCTION , This report describes the Radiological Environmental Monitoring Program (REMP) for the Waterford 3 SES nuclear power plant and discusses the results obtained during the calendar year 1985. The results discussed within this report were used to evaluate the radiological environmental impact resulting from the opera-tion of Waterford 3 SES. The submission of this report to the Nuclear Regulatory Commission fulfills the requirements pursuant to Waterford 3 SES Technical Specification 6.9.1.7. 1.1 Procram and Renort Obiectives The overall objective of the monitoring program was to l evaluate the radiological environmental impact of the plant. The evaluation included an assessment of actual or potential exposures of humans to radioactive materials or radiation resulting from plant operation. In order to conduct this evaluation, the data analyses and interpreta-tions contained in this report fulfilled the following specific objectives:

a. identify if any radioactive materials or radiation in the environment was associated with plant operation;
b. compare the results obtained during the reporting period with past operational and preoperational data, when appropriate, to identify any trends or accumulation of radioactivity in the environment;
c. estimate the maximum exposure to a member of the general public from any environmental data which indicates the presence of plant related radioac-tivity; and i
d. verify compliance, when appropriate, with relevant federal requirements.

1.2 Plant and Site Descrintion The Louisiana Power and Light Company, Waterford Steam Electric Station, Unit No. 3 employs a pressurized water reactor for the production of approximately 1153 gross (1104 net) megawatts of electricity. The station uses a once through flow of water obtained from and discharged to the i Mississippi River for condenser cooling. During the period covered by this report, on March 4, 1985, the unit achieved initial criticality. t I 1 I .- . . - _ . ._ . - .

Waterford 3 SES is located on the west bank of the Missis-sippi River at River Mile 129.6 between Baton Rouge and New Orleans, Louisiana. The site is in the northwestern section of St. Charles Parish approximately 3 miles southeast of the St. John the Baptist Parish boundary near the towns of Killona and Taft. The Mississippi River is the closest prominent natural feature while others include Lac des Allemands, about 5.5 miles southwest of the site, and Lake Ponchartrain, about 7 miles northeast of the site. Most of the man-made features are located on the narrow strip of dry land between the Mississippi River and the wet-lands. Near the Waterford SES site are several large industrial facilities, including Waterford 1 and 2 Steam Electric Stations (0.4 miles northwest of the site), Little Gypsy Steam Electric Station (0.8 miles north northwest of the site, across the river from Waterford 3 SES), Beker Industries, a fertilizer manufacturer (0.6 miles east southeast), Occidental Chemical company (0.8 miles east southeast), and Union Carbide, a chemical manufacturer (1.2 miles east southeast). Louisiana Power and Light Company owns and operates the above mentioned steam electric stations. Major urban centers in the region of the site include New Orleans (approximately 25 miles east of the site) and Baton Rouge (approximately 50 miles west northwest) . Communities in St. Charles Parish near the site include Killona (0.9

;   miles west northwest), Montz (1.0 miles north), Norco (1.9 2

miles east) , Hahnville (3.7 miles east southeast) , and Destrahan (6.3 miles east southeast). Laplace (4.7 miles north) is located in St. John the Baptist Parish. i e 2

l I i i 2.0 PROGRAM DESCRIPTION , A general summary of the REMP is given in Table 2.1. Brief descriptions of the sampling stations and their locations are given in Table 2.2. The locations of the sampling stations with i respect to the Waterford 3 SES site are illustrated in Figures 2.1 through 2.3. A more detailed description of the overall REMP 4 is discussed in the following chapter. 2.1 History and Develonnent The Waterford 3 SES REMP was initiated in April of 1983. The program evolved from the Preoperational Environmental

Radiological Surveillance (PERS) Program which was conducted from 1978 through 1982. The equipment, procedures, tech-niques, and many of the same sampling locations used during the preoperational survey were incorporated into the operational program. The environmental data collected during the first two years of the REMP (1983 and 1984), when Waterford 3 SES had not yet achieved initial critical-ity, were used to supplement the baseline data obtained i during the PERS Program.

LP&L personnel were responsible for the proper implementa-tion of the REMP and insuring that the program complied with

                      . federal regulatory requirements and Technical Specification requirements. Specific responsibilities of LP&L personnel included collecting (with the exception of fish samples),

i preparing, and shipping of environmental samples; conducting environmental dosimetry measurements; reviewing analytical results reports; and preparing and submitting the annual Environmental Radiological Monitoring Report as well as any other relevant report to the Nuclear Regulatory Commission. The primary contractor, Teledyne Isotopes, Inc., located in Westwood, New Jersey, was responsibile for performing radiological analyses; conducting the initial data review;  ; preparing quarterly and annual results reports; and over-i seeing laboratory quality assurance and control. A separate , contractor, Dames and Moore, was responsible for the I collection, and delivery to LP&L, of fish samples. l , 2.2 Samole Collection and Handlina Procedures i The types of samples collected, the analyses performed, the sample collection frequencies, and the location of the sampling stations are summarized in Tables 2.1 and-2.2. The information contained in these tables is based on the , 1 t t

i requirements in Table 3.12-1 of Waterford 3 SES Technical Specification 3.12.1. The locations of the sampling 4 stations with respect to the Waterford 3 SES site are illustrated in Figures 2.1 through 2.3. Any deviations from the REMP (i.e., unavailable samples and missed lower limits . of detection) observed during 1985 are discussed in Section  ! 3.5. Changes made to the REMP during 1985 as a result of  ! the annual land use census are also discussed in Section i 3.5.

,                           The environmental samples collected were classified into four general categories according to exposure pathways:

direct radiation, airborne, waterborne, and ingestion. The collection and handling procedures used to obtain these samples are described in the following sections. The descriptions are intended to provide a concise overview of what was done rather than to be step-by-step procedures. 2.2.1 Direct Radiation Ernosure Pathway Samples Integrated external gamma exposures were dstermined ) using thermoluminescent dosimeters (TLDs). Multi-ele- i ment TLDs manufactured by Panasonic were placed at thirty-one locations as follows:

a. an inner ring of stations, one in each of the  !

sixteen meteorological sectors in the general l area of the site boundary,

b. an outer ring of stations, one in ten of the meteorological sectors in the six to eight kilometer range from the site, and
c. the balance placed in areas of special interest (e.g., population centers, schools, ,

i etc.) with one area serving as a control. l I 1 The TLDs were exchanged and analyzed quarterly by LP&L l personnel. l 2.2.2 Airborne Ernosure Pathway Samnles I Samples of airborne particulates and radiciodines were collected at five locations. The locations included i four indicator stations (APP-1, APQ-1, APG-1, APC-1) and one control station (APE-30). The samples were collected using low-volume air sampling devices. The i devices were designed to sample air on a continuous 1 - 4 1 . 6 l l

i i i i basis and record the volume of air sampled. The pump and metering device were housed inside a weatherproof l shelter. i 1 i' Airborne particulate samples were obtained by passing l air through a particulate filter using the device 4 described above. The filters were collected weekly by LP&L personnel and sent to the contract laboratory for gross beta analysis. These filters were composited by the contract laboratory on a quarterly basis for analysis by gamma spectroscopy. Airborne iodine sampling was done in conjunction with air particulate sampling. After the air passed through the particulate filter, it passed through a charcoal cartridge to collect airborne iodine. The cartridges were collected weekly by LP&L personnel and sent to the contract laboratory for iodine-131 analysis by gamma spectroscopy. 2.2.3 Waterborne Ernosure Pathway Samoles The Mississippi River is the major source of drinking water in the vicinity of Waterford 3 SES and it is also the surface water into which the plant discharges. Therefore, water samples taken from the Mississippi River were designated as both drinking water and

,                surface water samples.                                                                              I composite drinking / surface water samples were obtained                                             !

from the Mississippi River using automatic composite samplers placed at one upstream (DWP-7) and two downstream (DWG-2, DWE-5) locations from the plant. ' These composite water samples were collected biweekly by LP&L personnel. LP&L personnel acidified the samples with hydrochloric acid and added sodium bisulfite (to prevent protein binding of iodine) prior to shipment to the contract laboratory. The contract laboratory analyzed the biweekly samples for

!               iodine-131. The biweekly samples were composited on a monthly basis by the contract laboratory for gross beta and gamma spectroscopy analyses. The samples were i

also composited on a quarterly basis for tritium analysis.

'               Due to the high water table resulting from shallow aquifers in the vicinity of the site, groundwater discharge could be sampled from a drainage canal.                                                     !

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'               Groundwater samples were obtained quarterly by LP&L personnel from one sampling location (GWJ-1) using a 5

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grab sampling technique. The samples were acidified with hydrochloric acid and had sodium bisulfite added prior to shipment to the contract laboratory for tritium and gamma spectroscopy analyses. Shoreline soil samples were obtained semi-annually by LP&L personnel from two sampling stations. One station was located on the shoreline of the Mississippi River ' (SHWE-3) and the other was located on the shoreline of the 40-Arpent canal (SHWJ-1). Station SHWJ-1 was not added to the REMP until the second half of 1985 and therefore only one sample was obtained. The samples collected were shipped to the contract laboratory without further processing. 2.2.4 Incestion Fxcosure Pathway Samnles Milk samples vece collected semi-monthly by LP&L personnel. Control samples were obtained through

,             Louisiana Nuclear Energy Division personnel from the Louisiana State University Department of Agriculture (MKQ-50) located in Baton Rouge, Louisiana. Indicator samples were collected locally from two stations (MKQ-5, MKE-4). All samples had sodium bisulfite added (to inhibit protein binding of iodine) prior to shipment to the contract laboratory for iodine-131 and gamma spectroscopy analyses.

Fish samples were collected upstream (FH-1) and

downstream (FH-2) from the plant by a contractor. The fish were obtained by netting. The contractor seg-1 regated the samples by species and location sampled prior to delivery to LP&L. The samples were shipped frozen to the contract laboratory for analysis by j gamma spectroscopy.
LP&L personnel collected broad leaf vegetation samples monthly by obtaining cuttings taken at least one inch above the ground. Samples were collected from two indicator locations (BLB-1, BLQ-1) and from one of two control locations (BLH-10, BLK-15). The samples i

were shipped to the contract laboratory without further ) processing. A food / garden crop sample (soybeans) was collected by i LP&L personnel from one location (FPP-1). The sample was collected by normal harvesting techniques at the time of harvest. The sample was sent to the contract , laboratory without further processing for iodine-131 l and gamma spectroscopy analyses. l 6

          ~. __                           __                                                              _. -      __             _ _ _

2.3 Analytical Procedures Brief synopses of the analytical procedures used by Teledyne Isotopes and LP&L are given in Appendix E. These synopses are intended to provide an overview of what was done rather than to be step-by-step procedures. The minimum sensitivities for the analytical procedures used in the REMP are reflected by the Lower Limits of Detection (LLD) values presented in Table 2.3. These values are the same as the ones given in Table 4.12-1 of Waterford 3 SES Technical Specification 4.12.1. The LLD's are a nriori estimates based on assumed sample volumes, counting times, detector efficiencies, etc. These values reflect the lower levels of detection that were to be attained for the majority of the analyses performed. Deviations from ! the assumptions used in calculating these estimates (i.e., different sample volumes, counting times, etc.) caused some actual values to be higher than the ones given in Table 2.3. All analyses that could not achieve these lower limits of detection are discussed in Section 3.5. 2.4 Laboratorv Quality Assurance Teledyne Isotopes performed a variety of quality assurance analyses. The types consisted of spiked and blank samples 1 prepared in-house; spiked samples sent by customers or by a

;            second laboratory under contract to a customer; and EPA and l

NRC samples sent by the originator to customers and then sent to Teledyne Isotopes. Also certain customers have either 5% or lot of their samples analyzed in duplicate. It has been estimated that at Teledyne Isotopes, 5% of all analyses are for quality assurance purposes. Teledyne Isotopes also participates in the EPA radiological interlaboratory comparison (cross-check) program. Parti-

. cipation in this program involves a number of analyses on i various sample media as found in most REMP's. As a result j of participation in the program, an objective measure of analytical precision, accuracy, and an estimation of bias can be obtained. In the event that any results obtained by Teledyne Isotopes were not within control limits, as speci-
fled by the EPA, an investigation was conducted to determine j

the cause and corrective action was taken to prevent a recurrence. Appendix D lists the 1985 results of Teledyne Isotopes participation in the crosscheck program. In 1984 and 1985, LP&L participated in the Seventh and Eighth International Environmental Dosimeter Intercomparison Project sponsored jointly by the Department of Energy, the . 7

Nuclear Regulatory Commission, and the Environmental Protection Agency. Results of LP&L's participation in this comparison program for 1984 are presented in Appendix D. The results for 1985 will not be available until some time during 1986. These results will be presented and discussed in the 1986 Environmental Radiological Monitoring Report. i l 8

TABLE 2.1 1

  • RADIOLOGICAL ENVIRONMENTAL g ITORING PROGRAM (REMP) SUP9tARY Sample Type Location Analysis Frequency a

i Direct A-2, B-1, C-1, D-2, E-1, TLD gamma Quarterly Radiation F-2, G-2, H-2, J-2, K-1, , L-1, M-1, N-1, P-1, Q-1, R-1, A-5, B-4, D-5, E-5,

;                                          F-4, G-4,.H-6, P-6, Q-5, R-6, F-9, G-9, E-15, J-15, E-30 1

Radiciodine and APP-1, APQ-1, APG-1, Gross beta, I-131 Weekly Particulates APC-1, APE-30 y isotopic Quarterly composite Drinking Water DWG-2, DWE-5, DWP-7 H-3 Quarterly composite Gross beta, y isotopic Monthly composite I-131 Bi-weekly composite Surface Water SWG-2, SWE-5, SWP-7 H-3 Quarterly composite

y isotopic Monthly composite I

Ground Water GWJ-1 y isotopic, H-3 Quarterly j Shoreline Sediment SHWE-3, SHWJ-1 y isotopic Semi-annually i Milk MKE-4, MKQ-5, MKQ-50, y isotopic, I-131 Semi-monthly / monthly MKQ-1 Fish FH-1, FH-2 y isotopic In season or semi-annually 1 Food Products FPP-1 y isotopic At harvest time Broad Leaf BLQ-1, BLB-1, BLH-10, BLK-15 y isotopic, I-131 Monthly When milk samples not collected

a. Based on requirements in Table 3.12-1 of Waterford 3 SES Technical Specification 3.12.1.
b. Drinking and surface water samples are identical.

1

TABLE

2.2 DESCRIPTION

OF REMP SAMPLING STATION LOCATIONS l LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION Direct Radiation (TLD) 1 A-2 (Eastbank) On fence enclosure 1.1 N surrounding water tower west of Little Gypsy opposite Etienne St. Access from River Road (LA 628). The TLD's are located on the (S)

fence opposite the entrance gate j to the water tower.

B-1 (Eastbank) On fence enclosing the - 0.8 NNE transmission tower 0.3 miles west ' (up-river) from Little Gypsy. Access from River Road (LA 628). TLD's are located at SW corner of fence enclosure.

 !                         C-1                   (Eastbank) On fence enclosing the                                                                       0.8    NE i

Little Gypsy Cooling Water Intake. ' Access is from River Road (LA 628) across from Little Gypsy Power Station entrance. TLD's are on the south side (inside) of the Cooling Water Intake fence enclosure, I directly opposite the entrance gate. D-2 (Eastbank) Located at USGS Witness 1.1 ENE Post Survey Marker approximately l' 0.3 miles east of Little Gypsy Power Station. Access from River Road j (LA 628) near the west end of the Bonne Carre Spillway. TLD's are on the back of the Survey Marker l Sign (located on levee). 1 E-1 (Westbank) Located on utility pole 0.2 E along River Road (LA 18) approxi-sately 0.3 miles east of Waterford

)                                             3 plant entrance. Access from LA
18. TLD's are on the third utility pole east of the construction entrance road.
1 L

i i i 10

     ,                           TABLE 2.2 (CONTINUED)

LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION F-2 (Westbank) Located on fence 1.1 ESE enclosure surrounding the LP&L substation on LA 3142. Access from LA 3142 approximately 0.2 miles south of LA 18. TLD's are on the southeast corner of the fence enclosure. G-2 (Westbank) Located on utility pole 1.2 SE on East side of LA 3142 near Witco entrance gate (Next to Union Carbide Star Plant Gate 3). Access from LA 3142 approximately 0.2 miles north of railroad overpass. H-2 (Westbank) Located on fence enclosure 1.2 SSE to shell road off of LA 3142. Access from LA 3142 south of railroad overpass I on east side of LA 3142. TLD's are on the south side of the gate for shell road. (Just south of Texaco pipeline station) J-2 (Westbank) Located on northeast 1.3 S corner of fence enclosing Texaco valve station south of LA 3127. Access from LA 3127, approximately 0.6 miles west of LA 3127/3142 intersection. , K-1 (Westbank) Located behind " Private 1.0 SSW . Road" sign at Gate 8 entrance off of LA 3127. Access from LA 3127, approximately 1.3 miles west of

                                                                       )

LA 3127/3142 intersection. (Gate t 8 is the access to the Waterford 3 l switchyard station) L-1 (Westbank) located behind " Private 1.0 SW Road" sign at LP&L Gate 9 entrance off of LA 3127, approximately 1.6 miles west of LA 3127/3142 inter- , section. (Gate 9 is an access road for Waterford 3) 11 l i l t

4 TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION M-1 (Westbank) Located on south gate 0.7 WSW into the Waterford 1 and 2 fuel oil storage tank enclosure. Access is either thru LP&L Gate 8, Gate 9 off of LA 3127, the shell access road from LA 18 between Waterford 3, or thru the Waterford 1 and 2 access road. i N-1 (Westbank) Located behind the "No 0.9 W j Trespassing" sign off on Short Street, in Killona, just south of i the entrance to Killona Elementary i School. l P-1 (Westbank) Located behind "No 0.8 WNW Trespassing" sign on Short Street, in Killona, approximately 0.1 miles south of air sample station. Q-1 (Westbank) Located on fence 0.8 NW enclosing air sample station approximately 0.5 miles west of Waterford 1 and 2 on River Road (LA 18). R-1 (Westbank) Located on fence 0.5 NNW enclosure for Waterford 1 and 2 Cooling Water Intake Structure. Access is from River Road (LA 18) opposite Waterford 1 and 2.

                    ,                 TLD's are on the southwest corner of fence.

i l A-5 (Eastbank) Located on utility 4.5 N pole just east of the Shady Nook j Trailer Park on Hwy 61 in Laplace. l TLD's are on second utility pole east of trailer park on north side of Hwy 61 (eastern end of La Place). I 12

TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION B-4 (Eastbank) Located on utility pole 3.8 NNE just east of shell access road to South Central Bell transmission tower on south side of Hwy 61. Transmission tower is just east of Weigh Station at St. John /St. Charles Parish line. TLD's are on first utility pole east of access road. D-5 (Eastbank) Located on fence gate 4.2 ENE on shell access road to Big 3 Chemical Plant. Shell access road

is approximately 0.1 miles west of Hwy 61/48 intersection (at black and yellow gate). TLD's are on fence gate 0.1 miles north on i

shell access road from Hwy 61. E-5 (Eastbank) Located on the Norco 4.2 E Substation fence enclosure. Access from River Road (LA 48) onto Wesco St. (adjacent to Norco Shell Chemical Plant), take Wesco St. to the dead end. TLD's are located on sixth fence post south of the north subst:Lton gate. F-4 (Westbank) Located on utility pole 3.5 ESE i behind blonde brick house on , Aquarius St. in Hahnville. Access from River Road (LA 18) and turn

    .                onto Oak St. Follow Oak St. to Hickory St. , turn right on Hickory St. and follow to Aquarius St. and turn left.             Blonde brick house is second house on right (west) side of Aquarius St. heading south.

G-4 (Westbank) Located on railroad sign 3.2 SE i northwest side of LA 3160/ railroad track intersection. Access from either LA 3127 or River Road (LA 18) , j onto LA 3160. I l l 13

TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION H-6 (Westbank) Located on a construction 5.7 SSE sign on the southwest side of the second canal bridge east of LA 3160 along LA 3127. P-6 (Westbank) Located on utility pole 5.5 WNW at southwest corner of LA 640/ railroad track intersection. Utility pole is just west of LA 640 and east of radio transmission tower. Q-5 (Westbank) located on fence post 5.0 NW surrounding (green) river marker on levee just east of Edgard. Fence post is located along River Road (LA 18) across from the Webre's house. R-6 (Eastbank) Located on fence 5.3 NNW enclosing LP&L Laydown Yard on LA 3223 in Laplace. Access from Hwy 61 onto Elm St. (LA 3223), take Elm St. to the northeast corner of LA 3223/ railroad inter-section. TLD's are located on the southeast corner of fence enclosure. F-9 (Eastbank) Located on entrance 8.2 ESE gate to Destrehan Substation Access from River Road (LA 48), approximately 0.3 miles east of Luling-Destrehan Ferry, onto Destrehan Road (west of Bunge Corp. Grain Elevator), and l proceed to substation gate. G-9 (Westbank) Located on back fence 8.1 SE of LP&L District Office in Luling. Access via Ellington St. from either River Road (LA 18); or Second or Third St. from Paul Mallard Rd. (LA 52) to Ellington ' St. l l l i 14 l l

a -_ TABLE 2.2 (CONTINUED) i LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION E-15 (Eastbank) Located on Kenner 11.8 E Substation fence enclosure. Access frcs either River Road (LA 43) or Hwy 61, turn onto Alliance Ave. TLD's are located on the north side of the fence enclosure, near a light pole. J-15 (Westbank) Located on fence 12.0 S enclosure surrounding LP&L switchyard at LA 631/ Hwy 90 intersection in Des Allemands. TLD's are on the northwest corner of fence. Access from LA 631 via shell road. 1 E-30* (Westbank) Located on fence at 27.0 E LP&L General Office on Delaronde St. in Algiers. TLD's are on the fence, facing the Mississippi River, in the passageway to the transformer shop. . Airborne

APP-1 (Westbank) Located in soybean 0.8 WNW
field at northwest corner of Short St. in Killona.

APQ-1 (Westbank) Located at northwest 0.8 NW ! corner of soybean field on east )

  • side of Killona. Access from River Road (LA 18) approximately j

0.6 miles east of LA 18/3141 intersection. I APG-1 (Westbank) Located at the north 0.5 SE side of the Secondary Meteorology Tower. j 15 4

TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION APC-1 (Eastbank) Located inside the 0.8 NE Little Gypsy Cooling Water Intake Structure fence enclosure. APE-30* (Westbank) Located on the roof of 27.0 E the LP&L General Office building on Delaronde St. in Algiers. Waterborne DWG-2 (Westbank) Located at the Union 2.0 ESE SWG-2 Carbide drinking water canal. Access from LA 3142 through Gate 28. DWE-5 (Eastbank) Located at the 4.5 E SWE-5 St. Charles Parish Waterworks off of River Road (LA 48) near New Sarpy. DWP-7* (Westbank) Located at the St. 6.5 NW SWP-7* John Parish Waterworks off of LA 18 in Edgard. SHWE-3 (Westbank) Located at the Foot 3.0 E Ferry Landing off of LA 18 in Taft. SHWJ-1 (Westbank) Located at 40 Arpent 0.3 S Canal South of the Plant. Access from LA 3127 through LP&L Gate 8. The canal is northwest of the shell access road / railroad track intersection. GWJ-1 (Westbank) Located at 40 Arpent 0.3 S Canal south of the plant. Access from LA 3127 through LP&L Gate 8. The canal is northwest of the shell access road / railroad track inter-section. 16

TABLE 2.2 (CONTINUED) LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION Ingestion Milk MKE-4 (Westbank) Located .8 miles west 4.0 E of the Time Saver in Hahnville off of River Road. MKQ-1 (Westbank) 1.0 miles west of 1.0 NW Waterford 3 at the corner of River Road and Post Street in Killona. MKQ-5 (Westbank) Located at the Webre's 5.0 NW house, just across LA 18 from river marker, at the eastern end of Edgard. MKQ-50* (Eastbank) Located at the LSU Dairy 52 NW in Baton Rouge. Fish , FH-1* Upstream of the plant intake i structure. FH-2 Downstress of the plant intake structure. Broad Leaf BLQ-1 (Westbank) Located between LA 18 0.8 NW

       .          and soybean field on eastern edge of Killona, near air sample station APQ-1.

BLB-1 (Eastbank) Located at wooded area 0.8 NNE at the southwestern corner of the LP&L Little Gypsy plant along River Road. 17

TABLE 2.2 (CONTINUED) I LOCATION LOCATION MILES FROM SECTOR NUMBER DESCRIPTION PLANT DIRECTION 4 BLH-10* (Westbank) Located under overhead 9.5 SSE transmission lines along LA 633. BLK-15* (Westbank) Located 3.5 miles SSW 15 SSW of Des Allemands on Hwy. 90. Food Products FPP-1 (Westbank) Located in soybean 0.8 WNW field on eastern edge of Killona,- between air sample stations APP-1 and APQ-1.

  • DENOTES CONTROL LOCATION 18 i

i l 1 TABLE 2.3 DETECTION CAPABILITIES FOR ENVIRONMENTAL SAMPLE ANALYSIS LOWER LIMIT OF DETECTION (LLD)(*} WATER FISH MILK FOOD PRODUCTS ( ) SEDIMENT ANALYSIS (pCi/2) AIRBORNEPARTICp)TE OR GAS (pCi/a (pCi/kg, wet) (pCi/2) (pCi/kg, wet) (pCi/kg. dry) gross beta 4 0.01 H-3 2000 Mn-54 15 130 Fe-59 30 260 Co-58,60 15 130 Zn-65 30 260 Zr-Nb-95 15 d I-131 I 0.07 1 60 Cs-134 15 0.05 130 15 60 150 Cs-137 18 0.06 150 18 80 180 Ba-La-140 15 15

a. From Table 4.12-1 of Waterford 3 SES Technical Specification 12.4.1.
b. Applicable to broad leaf vegetation.

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i 3.0 DISCUSSION OF RESULTS i Analytical results for the year 1985 are discussed in this section by exposure pathway, type of sample, and analysis i performed. The analytical results of the REMP are summarized in i Appendix A and data for the individual analyses are presented in the tables of Appendix B. The radioactivity values summarized in Appendix A do not include any from naturally occurring radioac-tivity. i 1 i 3.1 Qigact Radiation Ernosure Pathway

The average exposures on both control and indicator Thermo-i luminescent Dosimeters (TLDs) were 16, 19, 16, and 15 mram per standard quarter (90 days) for the first, second, third, and fourth quarters of 1985, respectively. The average of j 112 TLD exposures for all of the indicator locations j was 17 ares / standard quarter compared to 21 aren/ standard quarter for the average of four exposures at the control t location. The lowest and highest individual exposures were i

13 and 27 area per standard quarter for all locations. Note

that the exposure for station J-2 during the first quarter

! of 1985 was 32 arem per standard quarter. Upon investiga-tion it was found that radiography was performed in the 1 } vicinity of station J-2 by the company which owns the property on which the TLD is located. The results obtained i from this TLD were deemed to have been affected by the j radiography and therefore the datum was not included in the

evaluation.

! Table 3.1 compares the TLD results by direction and distance , from the facility. The average exposure rate from TLD's located within two miles from the plant was statistically ! lower than the avera'e g exposure from stations located i more than five miles from the plant using the standard "t" test (see Appendix F). The average exposure rate from TLD's located between two and five miles from the plant was i statistically the same as the average exposure rate from ) stations located more than five miles from the plant.

  • Therefore, Waterford 3 SES operation did not have a detect-l able impact on direct radiation exposures from gamma radiation.

i, t , i 1 I I i l 23 i i

j 3.2 Airborne Ernosure Pathway i  ! { 3.2.1 Airborne Particulates Gross beta activity ranged from 0.0034 to 0.083 l l pCi/ cubic meter with an average of 0.021 pCi/ cubic j i meter for 253 measurements from all five sampling loca- t tions. The average gross beta activity for the control ! location, APE-30, was 0.022 pCi/ cubic meter compared to  ! l 0.021 pCi/ cubic meter for the four indicator locations ' ! (APP-1, APQ-1, APG-1, APC-1). The control station  : average is statistically the same as the average from 4 ! each indicator station using the standard statistical "t" test (see Appendix F). ! The gross beta activity results obtained during 1985 l i are consistent with those from the preoperational program. During the preoperational survey, in periods ' not significantly influenced by nuclear weapons detonations, the gross beta activity ranged between 0.02 and 0.04 pCi/ cubic meter. During the first two years of the REMP prior to Waterford 3 SES operation, i the average gross beta activity for all stations was j 0.021 pCi/ cubic meter with a range of 0.006 to 0.5

pCi/ cubic meter.

l Gamma spectroscopy results indicated detectable levels of cosmogenically produced beryllium-7 and potas-I sium-40 in the twenty quarterly composites. No i man-made radionuclides were detected above their respective lower limits of detection. 3.2.2 Airborna Iodine All of the 255 airborne iodine-131 results were below j the lower limit of detection which ranged from 0.01 to 0.6 pCi/ cubic meter. The variability of the lower ! limit of detection was due primarily to the difference ,

between air sample volumes. '

I. i

  • i
3.3 Waterborne Ernosure Pathway t j 3.3.1 Drinkina/ surface Water j As mentioned previously, drinking water is considered f synonymous with surface water. Results obtained from '

i j samples collected and analyzed as drinking water can be designated " surface water results". Therefore, i the results of the monthly and quarterly gamma spectral j 24 l 1 i ! i i 1

i  : l analyses as well as the quarterly tritium analysis ! reported as drinking water results are the same as for ! those reported as surface water results. Seventy-six composite drinking / surface water samples were analyzed by a radiochemical procedure for

iodine-131. All measurements were below the lower

! limits of detection. The samples were composited on a l monthly basis and analyzed by gamma spectroscopy. Only j naturally occurring potassium-40 was detected. No

man-made gamma emitters were detected above their i

respective icwor limits of detection. j The monthly composites were then filtered through a i Whatman number 54 filter and a gross beta analysis ' j performad on the filtrate. Gross beta activity was

detected in all of the thirty-six composites with an

! average activity of 6.2 pCi/ liter. The average activity for the control location was 5.7 pCi/ liter, compared to the averages of 7.9 and 5.0 pCi/ liter for indicator stations DWG-2 and DWE-5, respectively. The average gross beta activity detected at indicator station DWE-5 is statistically the same as that of the control station DNP-7 using the standard "t" test (see Appendix F). The average gross beta activity at station DWG-2, two miles downstream, is statistically larger than the control station average using the same statistical test. However, the difference between gross beta results for stations DWG-2 and DWP-7 was i also observed prior to Waterford 3 SES operation during ] 1984. Therefore the difference in measurements between ' j stations DWG-2 and DNP-7 appears to be the result of Jj some factor other than Waterford 3 SES operation. l In order to test this assumption, the numerical differences between control and indicator station l monthly gross beta results were calculated and compared for the years 1984 and 1985. A detailed discussion of this comparison is presented in Appendix F. Based on the results of this comparison, the difference ! , in gross beta activity between control station DWP-7 and indicator station DWG-2 were deemed to be unrelated

;           to the operation of Waterford 3 SES.

i Drinking / surface water samples were also composited j quarterly and analyzed for tritium. All measurements were below the respective lower limits of detection. j Although not required in the REMP the filters obtained e from the gross beta analysis were composited quarterly I and analyzed by gassa spectroscopy. No man-made gamaq l 25 i l l I

\ I emitters were detected above their respective lower limits of detection. 1 l i t

3.3.2 Groundwater Four groundwater samples were collected from one sampling location, GWJ-1, and analyzed for tritium and gamma ray emitters. All measurements were below the lower limits of detection.

l { 3.3.3 Shoreline Soil i Three shoreline soil samples were collected from two } sampling locations: two samples from the Mississippi River shoreline downriver of the plant (SNWE-3) and one ', sample from the shoreline of a drainage canal into which turbine buildin'g sumps are discharged (SHWJ-1). The latter location was added to the REMP during the second half of 1985. Naturally occurring potassium-40, radium-226, and thorium-228 were detected in all of the samples. 1 ' Man-made radioactivity, cesium-137, was detected in the sample obtained from station SNWJ-1 at a concentra-tion of 99 pCi/kg(dry). No other man-made radio-nuclides were detected in any of the samples. l

Radioactive. release permits for the year 1985 show that

{ no cesium-137 was discharge into the drainage canal l from which the sample came. Therefore, the presence of j the cesium-137 is most likely attributable to fallout i from past nuclear weapons detonations. This assumption ! is consistent with observations made during the { preoperational survey for soil samples collected from i the shoreline of the Mississippi River. During the ) preoperational program, cesium-137 was detected in 13 i of 18 soil samples at concentrations ranging between 30 ' l , and 890 PCi/kg(dry) with an average concentration of I 1 138 pCi/kg(dry) . 1 However, conservatively assuming that all of the i j cesium-137 activity detected in the shoreline soil at station SHWJ-1 originated from the plant, the maximum l dose to a member of the general public was calcu-lated. The methodology and assumptions used to calculate the maximum dose were based on the guidance i i provided in Regulatory Guide 1.109 (10/77). The dose \  : 26 1 - 1

 ~---_,,__._.____._.-_.-m.,_,,.                ..-_. ,_ , _ _ , _ _ . . . . , . - - . . ~ - _ .               _ . , . _ , _ _ . . - - , . . . - , -               . _ . . ,  ,

to the maximum exposed individual, a teenager, was calculated by the following equation: (1) R = (40) (C) (U) (D) where: R is the annual dose to the skin or the total , body in area / year; ' 40 is the area-mass conversion factor given in Appendix A of Regulatory Guide 1.109 in kg/ square meter; C is the radionuclide concentration in the shoreline soil sample in pCi/kg;

;                                             U          is the maximum exposure time given in Table E-5 of Regulatory Guide 1.109; 67 hours for a teenager; and D         L7 the external dose conversion factor for standing on contaminated ground given in
' Table E-6 of Regulatory Guide 1.109; the values for exposures resulting from cesium-137 to the skin and total body are 4.9E-09 and 4.2E-09 aren/hr per pCi/ square meter, respectively.

Using Equation (1), the maximum annual dose to a teenager spending 67 hours at the shoreline of the canal was calculated to be approximately 0.001 ares /yr i t to the skin and to the total body. Therefore, any radiological impacts to the general public resulting from cesium-137 detected in the shoreline soil are infinitesimal. i

3.4 Incestion Ernosure Pathway 3.4.1 Hilk Fifty milk samples were collected from three sampling locations and analyzed by a radiochemical procedure for iodine-131. All measurements were below the lower limits of detection. The samples were also analyzed by j gamma spectroscopy. Naturally occurring potassium-40 was detected in all samples. All man-made gamma 27

3

  .w

!^ emitters were below their respective lower limits of detection.

3.4.2 Zinh Twelve fish samples, five upstream and seven downstream of f;he plant, were collected and the edible portions analyzed by gamma spectroscopy. Naturally occurring '

pottssium-40 was detected in all samples. No man-made gamma emitters were detected above their respective ~

,                                                          lower limits of detection.

3.4.3 Broad Leaf Vecetation Waterford 3 SES Technical Specification 3.12.1 requires broad leaf vegetation to be sampled in the event milk , samples are unavailable. Since milk samples could be ' collected reliably from only one sampling location within five miles of Waterford 3 SES, broad loa. , vegetation was sampled monthly at two indicator  ; locations. Broad leaf vegetation was also collected from one of two control locations when milk from a l control location was. unavailable.  ; Twenty-seven broad leaf vegetation samples were 3 collected and analyzed by a radiochemical procedure for iodine-131. All measurements were below the lower limits of detection. The samples were also analyzed by . gamma spectroscopy. Naturally occurring radionuclides were detected in all of the samples. Cesium-137 was i detected in two of the control samples at an average ' concentration of 33 pCi/kg(wat). This man-made activity is most likely attributable to fallout from past nuclear weapons detonations. The cesium-137 concentrations detected in the control samples are consistent with preoperational results. 1 During the preoperational program, cesium-137 was

                                       , ,               occasionally detected at concentration ranging between 27 and 140 PCi/kg(wet) with an average concentration of 70 pCi/kg. No dose calculations were performed for
                                    ,                    these results since the activity was detected at a control location and could not attributed to Waterford 3 SES operation.

28 4 l 4

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3.4.4 Food / Garden Croos one food / garden crop sample was collected and analyzed ' by a radiochemical procedure for iodine-131. Iodine-131 was below the lower limit of detection. The sample was also analyzed by gamma spectroscopy. Naturally occur-ring potassium-40 was the only radionuclide detected. ' All man-made gamma emitters were below their respective  ! lower limits of detection. i i 1

                                                                                                                                                                          'i
3.5 Deviations from the REMP 3.5.1 Unavailable Samolen During 1985 deviations from the REMP sampling schedule All of the deviations (with the exception 1 occurred.  !
;                                                   of those associated with TLDs) were either the result of equipment malfunctions or the result of natural events beyond the control of LP&L.                                               With respect to equipment malfunctions, the causes leading to the                                                                       !

malfunction were identified and maintenance or replace-ment performed to prevent recurrence of the event. Deviations from the REMP associated with TLDs were beyond the control of LP&L and resulted from theft of a few of the dosimeters placed in the field. When a dosimeter was discovered missing during a monthly inspection, the TLD was replaced and the deviation noted. A listing of all unavailable samples for 1985 along with associated explanations of why the samples were not collected is given in Appendix C. A more detailed explanation for milk and vegetation sample unavailability is discussed below. Milk samples were not available on a regular basis from , the animal owner at station MKE-4 due to the small l volume of milk produced by the animals. With the absence of milk samples at this station, broad leaf

                       ,                           vegetation sampling was performed. One control location sample, MKQ-50, was unavailable from Louisiana Nuclear Energy Division personnel due to participation of the state in the Annual Emergency Planning Exercise conducted in September of 1985. Broad leaf vegetation was sampled at a control location during this month in lieu of the milk sample.

Broad leaf vegetation was not sampled at a control location during the months of January through May,

1985, since milk samples were available from the

, 29

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                                                               .,.,,..._-,.,-,_,m__-_._-___,.__._,.,,x_.,_m-,_,_m_,..,___                    ..,.o.-___m..__,.,--_

i I i control location. However, beginning in June of 1985, broad leaf vegetation was sampled even when control milk samples sere available in order to accumulate baseline data for future comparisons. I

 ,                                                   3.5.2 Missed Lower Limits of Detection A listing of all analyses                                                that could not attain the lower limits of detection                                                specified in Table 4.12-2 of Waterford 3 SES Technical                                                Specification 4.12.1 is presented in Appendix C.                                                 With the exception of one drinking / surface water sample, the LLDs were not attained due to insufficient sample size resulting from equipment malfunction. In all of these cases the equipment was repaired or replaced to prevent recur-i rence.

The LLD for barium-140/ lanthanum-140 could not be attained for one drinking / surface water sample. The missed LLD resulted from the gamma spectroscopy analysis being delayed. The delay was caused by the contract laboratory postponing the analysis while i awaiting arrival of a biweekly sample necessary to form a monthly composite. However, the biweekly sample was never collected due to equipment malfunction and miscommunication regarding the unavailable sample delayed analysis, i 3.5.3 Chances to the REMP During 1985, one new milk station, MKQ-1, was added to  ! the REMP as a result of the 1985 Annual Land Use ' census. However, no samples were available from the new location during 1985 (see Section 3.6) . The location of the control broad leaf vegetation

                          ,                        station was changed during 1985 as a result of re-eval-unting site meteorological data. The location was changed from BLH-10 to BLK-15 such that the new sampling station was located in the compass sector coinciding with the least prevalent wind direction.

Shoreline soil sampling location SHWJ-l was added to the REMP during the second half of 1985. The new location was added to monitor shoreline soil from a drainage canal into which affluents from the turbine building sumps are discharged. 30 l 2 - - - -- _ - . .y m,,- ,,,i--., .r- - - --tw----mme-ym e-e-wraw-yy vw g---w-rww=- 9 fw-wyy y,--mgyewcm,egw,-y,wy wy "g my-wg,,w4em+ g g ww we pw w-mmew

3.6 Annual Land Use Census Results In compliance with Waterford 3 SES Technical Specification 4.12.2, the Annual Land Use census was conducted on July 10 and 11, 1985. The nearest residence, garden, and milking I animal in each sector within a five mile radius of the plant l were found by visual inspection and verbal inquiry. The results of the 1985 census are given in Table 3.2. A new milking cow was found in sector Q at a distance of 1.1 miles from the plant. As a result, a new milk sampling station (MKQ-1) was added to the REMP. The owner of the animal stated that the cow was nursing a calf and would not begin producing milk for human consumption until December 1985. The owner was contacted on a periodic basis to determine the status of obtaining samples. The owner of milking goats at location MEE-4 has sold all but one of his goats. The remaining goat does not produce enough milk for Waterford 3 SES to obtain samples as stated

 .         by the owner. However, the sampling station will remain as part of the REMP and the owner will be contacted period-ically to determine the status of obtaining samples.

d 31 l l . . _ _ _ __. . _ . . _ _ - - , m- . - -

TABLE 3.1 1985 DIRECT RADIATION DATA ORGANIZED BY COMPASS DIRECTION AND DISTANCE FROM WATERFORD 3 SES EY COMPASS DIRECTION SECTOR COMPASS AVERAGE STANDARD NUMBER DIRECTION EXPOSURE DEVIATION IN (mram/std qtr) (aren/std qtr) GROUP A N 18 3.6 8 B NNE 16 0.8 8 C NE 13 1.5 3 D ENE 18 3.7 6 E(a) E 16 2.0 12 F ESE 17 2.8 12 G SE 17 1.9 11 H SSE 16 4.5 7 J S 17 5.1 7 K SSW 16 1.3 4 L SW 15 0.5 4 M WSW 17 2.4 4 N W 21 4.9 2 P WNW 19 3.6 8 Q NW 16 2.0 8 R NNW 16 2.3 8 CONTROL E 21 4.1 4 BY DISTANCE FROM PLANT DISTANCE AVERAGE STANDARD NUMBER FROM PLANT EXPOSURE DEVIATION IN (miles) (aren/std qtr) (arem/std qtr) GROUP 0-2 16 1.6 58 2-5 17 3.0 26

   > 5(a)                  18             3.4                    28 CONTROL                21              4.1                        4
a. Does not include control station data 32

TABLE 3.2 1985 ANNUAL LAND USE CENSUS RESULTS SECTOR DIRECTION DISTANCE FROM THE PLANT (miles) MILK MILK VEGETABLE RESIDENCE COW GOAT GARDEN A N - - 1.1 0.8 B NNE - - 1.3 0.8 C NE - - 1.0 0.9 D ENE - - 0.9 0.9 E E - 3.3(a) 3.2 2.6 F ESE - - 2.3 3.4 G SE - - 2.3 3.9 H SSE - - - - J S - - 0.9 - K SSW - - 0.9 - L SW - - 0.9 - M WSW - - 0.9 - N W - - 1.1 1.3 P WNW - - 0.9 0.9 Q NW 1.1(b,c) - 0.9 0.9 R NNW - - 2.9 2.0 1 Means none found in sector within a 5 mile radius of Waterford 3 SES.

a. Goat was not producing enough milk for samples.
b. Milk cow was nursing calf and does not supply milk for human consumption. The owner will be contacted on a periodic basis to determine availability of samples.
c. Samples will also continue to be taken 4.4 miles (MKQ-5).

This is the only reliable milk sample within 5 miles of Waterford 3 SES. 33 l

   --- , -            -            -   , . - _ , -       ..,,-,,..._._,.-__..w         y,_, . . . _ - ,r.p-   - _ , - - . - - _ . - . - - - - , . .

4.0 CONCLUSION

S The radiological environmental data collected during 1985 are consistent with the data obtained during the Preoperation Environmental Radiological Surveillance (PERS) Program and during the first two years of the REMP prior to Waterford 3 SES initial criticality. The only man-made radionuclide detected out of all of the environmental samples analyzed during 1985 was cesium-137. Cesium-137 was detected in one shoreline soil sample and two control location broad leaf vegetation samples. The origin of this man-made radioactivity is most likely attributable to fallout from past nuclear weapons detonations and not Water-ford 3 SES operation. In conclusion, based on the evaluation of the REMP data collected during 1985 the operation of Waterford 3 SES had no observable radiological impact on the environment. j m ' 34 l I

m.: APPENDIX A REMP DATA

SUMMARY

35

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TABLE A-1 BaBlotacICAL auriacusertat unstieaans panoness senestav - mene of heility , _ ,_a i ene anchet me, wuz Leestsee of pacility st. Charles. Leutetene .las ery 1 to

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  ,                                                                                                            (-)

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    *Leuer Limite of potecties (LLD) for individual radienec11 des emelysed for by gesma spectroscopy are gives la Waterford 3 Technical                                                   a one,    Spec j    d i

1 Iso etnision teuer Limit of Detecties (LLa) defined to Waterford 3 Techeical Specifications. 1 l l 4 I L _-__ __ _ _ _ _ _ _ _ - _ _ __ _ _ _ _ _ --

APPENDIX B REMP DATA 41

TABLE B-1 QUARTERLY TLD EXPOSURES mRee/ standard 90 day quarter STATI0s FIRST QUARTER SECONO QUARTER INit0 QUARIER f ouu1N QUAR 1ER EUGISER 12/27/04-83/28/85 03/28/85-06/28/85 06/28/05-10/02/85 10/02/85-01/03/66 A-2 18 19 19 15 A-5 17 26 (d) 15 th 8-1 15 16 16 15

  ,    8-4                17                        17                            16 w                                                                                                 15 C-1                13 (a)                   14                             11 (b) 8-2                IS                       21                            19 (b) 8-5                (b)                      21 (d)                         13                13 i

E-1 17 (a) 19 16 15 j E-5 14 17 14 13 .; E-15 17 19 18 th E-38 27 (c) 20 19 13 F-2 15 15 15 14 F-4 18 21 19 15 F-9 17 23 16 15 j G-2 14 20 19 16 I G-4 17 (b) 14 14 , G-9 17 18 17 15 N-2 17 18 17 ' (b)

    . H-6                13                       25                            13                 12

( a) TLD vandallied; replaced 03/01/85. (b) It0 Vandallied (c) ILD Vandalized; replaced 03/08/85. (d) ILD Vandalized; replaced 05/03/85.

                                                                                  ~ _ _ .                                        _

TABLE B-1 (Cont.) QUARTERLY TLD EXPOSURES mRee/ standard 90 day quarter STAil0N FIRST QUAATER Seton 0 QUARTER sussett 12/27/84-03/28/85 03/28/85-06/28/85 THIRD QUAR 1Elt FOURIN QUART [k 06/28/85-10/02/85 10/02/85-01/03/86 J-2 32 (a) 16 14 13 J-15 15 28 16 15 K-1 16 17 16 14 L-1 15 15 16 15

c. M-1 15 20 w 15 16 u-l (b) 24 (c) 17 (b)

P-1 17 27 (d) la 15 P-6 19 20 18 17 Q-1 14 17 15 13 Q.5 17 19 la 16 A-1 14 17 14 13 R .'6 17 19 18 la J aJ R adlegr aphy la area db i TLS Vandallaed ic ) TLD vandallaed; replaced 06/08/85. Ldj TLS vandallaed; replaced 05/01/85. I

TABLE B-2 AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND 10 DINE-131 ANALYSES STATION NUNSER APC-1 1sst COLLECTIOS DATE STAST STOP MID COUNT A P FILTER MID COUNT CHAACOAL FILTES TIME GROSS SETA OATE DATE VOL UME UNITS DATE (pCl/Cu. M.) TIME I-131 DATE (pCi/Cu. M.) , 12/31 01/07 1.02E 04 CU. FT. 01/15 2.2 s 0.3 E-02 01/!! L.T. 4. E-02 01/07 01/14 1.02E 04 CU, FT. 01/25 2.4 2 0.4 E-02 01/16 L.T. 2. E-02 01/14 01/22 1.l?E 04 CU. FT. 01/30 s~ 2.1 2 0.3 E-02 01/24 L.T. 3. E-02 01/22 01/28 8.51E 03 CU. FT. 02/06 1.9 2 0.4 E-02 01/30 L.T. 3. E-02 01/28 02/04 I.0lt 04 CU. FT. 02/11 1.9 1 0.3 E-02 02/07 L.T. 5. E-02 02/04 02/11 9.94E 03 CU. FT. 02/21 3.4 2 0.4 E-02 02/13 L.T. 3. E-02 02/11 02/18 1.02E 04 CU. FT. 02/26 2.8 1 0.4 E-02 02/21 L.T. 3. E-02 02/18 02/25 1.02E 04 CU. FT. 03/05 1.5 t 0.3 E-02 02/27 L.T. 3. E-02 02/25 03/04 1.03E 04 CU. FT. 03/13 1.8 2 0.3 E-02 03/06 L.T. 3. E-02 03/04 03/11 1.03E 04 CU. FT. 03/20 2.1 2 0.3 E-02 03/13 L.T. 3. E-02 03/11 03/18 1.03E 04 CU. FT. 03/26 2.0 s 0.3 E-02 03/20 L.T. 3. E-02 03/18 03/25 1.03E 04 CU. FT. 03/29 1.3 1 0.3 E-02 03/28 L.T. 4 E-02 03/25 04/01 6.56E 03 CU. FT. 04/08 2.4 s 0.4 E-02 04/03 L.T. 6. E-02

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STAil0N NUMBER APC-1 Iyst COLLECil04 OATE MID COUni START STSP A P FILTER M10 COUNI CHARCOAL FILTEk TIME SA055 SETA ilME OATE OATE VOL UME UNii5 OAit (pCl/Cu. M.) l-131 DATE (pCl/Cu. M.) 04/01 04/09 1.16E 04 CU. FT. 04/16 2.0 a 0.3 E-02 04/11 L.T. 3. E-02 04/09 04/15 8.73E 03 CU. FT. 04/25 2.1 1 0.4 E-02 04/18 L.T. 4 E-02 04/15 04/22 1.02E 04 CU. FT. 05/01 1.8 1 0.3 E-02 ' 04/24 L.T. 3. E-02 04/22 04/30 1.20E 04 CU. FT. 05/24 2.1 s 0.3 E-02 05/01 L.I. 2. E-02 04/30 05/06 (a) 05/06 05/08 3.69E 03 CU. FT. 05/21 3.8 s 0.8 E-02 05/16 L.T. 2. E-Ul(b) l 05/08 05/20 (c) 05/20 05/27 1.02E 04 CU. FT. 06/06 2.1 1 0.3 E-02 1 05/30 L.I. 2. E-02 05/27 06/03 1.00E 04 CU. FT. 06/17 3.0 s 0.3 E-02 06/05 L.T. 3. E-02 06/03 06/10 1.00E 04 CU. Fi. 06/19 2.6 t 0.4 E-02 06/13 L.T. 3. E-02 06/10 06/17 1.01E 04 CU. FT. 07/02 1.3 s 0.3 E-02 06/19 L.T. 4. E-02 06/17 06/24 1.01E 04 CU. FT. 07/10 2.0 t 0.3 E-02 06/26 L.T. 3. E-U2 06/24 07/01 1.01E 04 CU. FT. 07/15 2.7 1 0.4 E-02 i 07/03 L.T. 4. E-02 ( a'l Sample not collected; pump not working. i (b.I Regelred LLO could not be met due to low air volume. (c) Power failure; sample not collected,

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CAR'lllIDGES: GROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APC-1 i l ITES 4 COLLECTION DATE MID COUNT A P FILTER

START STop MID COUNT CHARC0AL FILTER T I ME GROSS SETA TIME l-131 DATE DATE WOL UME UNITS DATE (pCl/Cu. M.) DATE (pct /Cu. h.)

j 07/01 07/03 3.95E 03 CU. FT. 07/17 3.5

  • 0.6 E-02 07/11 L.T. I. E-01(a) 07/09 07/15 4.80E 03 CU. FT. 07/22 2.3 2 0.4 E-02 07/17 L.T. 3. E-02 07/15 07/23 1.!!E 04 CU. FT. 07/26 1.9 2 0.3 E-02 07/24 L.T. 3. E-U2 07/23 07/29 9.22E 03 CU. FT. 04/07 1.8 2 0.3 E-02 07/31 L.T. 3. E-02 07/29 08/05 1.02E 04 CU. FT. 08/15 2.0 1 0.3 E-02 04/07 L.T. 3. E-02 08/05 08/12 1.0IE 04 CU. FT. 08/19 2.2 2 0.3 E-02 08/14 L.T. 3. E-02 I 08/12 08/19 1.02E 04 CU. FT. 08/29 1.5 1 0.3 E-02 08/22 L.T. 3. E-02 04/19 08/26 1.04E 04 CU. FT. 04/30 1.9 2 0.3 E-02 08/28 L.T. 3. E-U2 08/26 09/03 1.15E 04 CU. FT. 09/09 2.0 1 0.3 E-02 09/04 L.T. 2. E-U2
!                                         09/03            09/09      9.71E 03     CU. FT.      09/19     1.5 t 0.3 E-02   09/10    L.T. 3. E-02 09/09            09/16      1.02E 04     CU. FT.      09/23     2.1 a 0.3 E-02   09/17    L.T. 4. E-02 09/16            09/23      1.01E 04     CU. FT.      10/03     1.8 1 0.3 E-02 s

09/24 L.T. 2. E-02 09/23 0*/30 1.03E 04 CU. FT. 10/07 2.3 a 0.3 E-02 10/01 L.T. 2. E-02 f (a) Required LLO could not be met due to low air volume. I t

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CilARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STAil0N NUNSER APC-1 17s3 COLLECil04 SATE NID COUNT A P FILTER MID COUNI CHARCOAL FILTER START STOP TIME GROSS BETA ilNE OATE l-131 . l DATE VOLUME UNITS DATE (pCl/Cu. M.) DATE (pct /Cu. M.) 09/30 10/07 1.0lE 04 CU. FT. 10/11 1.9 a 0.3 E-U2 10/08 L.T. 3. E-02

10/07 10/14 1.02E 04 CU. FT. 10/22 2.3 t 0.3 E-02 10/16 L.T. 3. t-02 10/14 10/21 1.02E 04 CU. FT. 10/29 1.3 2 0.3 E-02 10/23 L.T. 2. E-02 10/21 10/28 1.02E 04 CU. FT. 11/13 2.1 2 0.3 E-02 10/30 L.T. 3. E-02 i 10/28  !!/04 1.Olt 04 CU. FT. 11/13 1.5 1 0.3 E-02 11/06 L.T. 3. E-02 11/04 11/11 1.0lt 04 CU. FT. 11/21 3.1 2 0.4 E-02 11/14 L.T. 3. E-02 11/11 11/14 (a) 11/18 11/25 (a) 11/25 12/02 1.00E 04 CU. FT. 12/09 7.2 a 3.3 E-03 12/04 L.T. 3. E-02 12/02 12/09 1.02E 04 CU. Fi. 12/18 3.1 1 0.4 E-02 12/11 L.T. 3. L-02 l 12/09 12/16 9.61E 03 CU. FT. 12/30 2.1 1 0.3 E-02 12/19 L.T. 3. E-02 12/16 12/23 9.96E 03 CU. FT. 01/03 3.5 2 0.4 E-02 12/27 L.T. 2. E-02 12/23 12/30 9.89E 03 CU. FT. 01/07 2.3 1 0.3 E-02 01/02 L.T. 3. E-02 1

( a) Pump malfunction; no sample available, i l

TABl.E B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND 10 DINE-131 ANALYSES STATION NUNSER APG-1 1555 COLLECT!08 SATE MID COUNT STAST STOP A P FILIER MIO COUNI CHARCOAL FILTES TIME GROS 5 BETA TIME DATE DATE VOL UME UNIIS DATE (pCl/Co. M.) l-131 DATE (pC1/Co. M.) 12/31 01/07 9. 7 9E 03 CU. FT. 01/15 2.2 2 0.3 E-02 01/11 4. L.T. E-02 01/07 01/14 9.88E 03 CU. FT. 01/25 I 2.6 2 0.4 E-02 01/16 L.T. 2. E-02 01/14 01/22 9.18E 03 CU. FT. 01/30 2.4 1 0.4 E-02 01/24 L.T. 4 E-02 g 01/22 01/28 8.34E 03 CU. FT. (a) 01/30 L.T. 3. E-02 01/28 02/04 9.89E 03 CU. FT. 02/ll 1.9 a 0.3 E-02 02/07 L.T. 5. E-02 02/04 02/11 9.86E 03 CU. FT. 02/21 3.3 2 0.4 E-02 02/13 L.T. 3. E-02 02/11 02/18 9.90E 03 CU. FT. 02/26 2.6 2 0.4 E-02 02/21 L.T. 3. E-02 02/18 02/25 9.96E 03 CU. Fi. 03/05 1.7 2 0.3 E-02 02/27 L.T. 3. E-02 02/25 03/04 9.97E 03 CU. FT. 03/13 1.5 t 0.3 E-02 03/06 L.T. 3. E-02 03/04 03/11 1.00E 04 CU. FT. 03/20 1.9 1 0.3 E-02 03/13 L.T. 3. E-02 03/11 03/18 9.98E 03 CU. ff. 03/26 1.9 2 0.3 E-02 03/20 L.T. 3. E-02 03/18 03/25 9.98E 03 CU. Fi. 03/29 1.7 2 0.3 E-02 03/28 L.T. 5. E-02 03/25 04/01 1.00E 04 CU. FT. 04/08 2.2 a 0.3 E-02 04/03 L.T. 3. E-02 ( a) Lost filter during collection. High winds blew filter onto puddle of water.

TABLE 8-2 (Cont.) AIR PARTICUIATE FILTERS AND CitaRCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APG l Isss COLLECTION SATE MID COUNT A P FILifR START STOP MID COUNI CHARCOAL FILTER Tine GROSS BETA TIME l-131 DATE DATE VOLUME UNITS DATE (pCl/Cu. M.) DATE (pCl/Cu. M.) 04/01 04/09 1.06E 04 CU. FT. (a) 04/11 L.T. 3. E-02 04/09 04/15 7.93E 03 CU. FT. 04/25 2.4

  • 0.4 E-02 04/18 L.T. 4. E-02 04/15 04/22 9.20E 03 CU. FT. 05/01 2.2 2 0.4 E-02 04/24 L.T. 3. E-02 04/22 04/29 9.13E 03 CU. FT. 05/24 2.0 t 0.4 E-02 05/01 L.T. 3. E-02 04/29 05/06 9.22E 03 CU. FT. 05/14 1.9 1 0.3 E-02 OC/08 L.T. 3. E-U2 05/06 05/13 9.23E 03 CU. FT. 05/21 2.3 2 0.4 E-02 05/16 L.T. 5. E-02 05/13 05/20 9.96E 03 CU. FT. 05/31 2.3 a 0.3 E-02 05/23 L.T. 4 E-02 05/20 05/27 9.95E 03 CU. FT. 06/06 2.0 t 0.3 E-02 05/30 L.T. 2. E-02 05/2T 06/03 9.93E 03 CU. FT. 06/17 2.7 2 0.3 E-02 06/05 L.T. 3. E-02 06/03 06/10 1.IIE 04 CU. FT. 06/19 4.2 2 2.0 E-03 06/13 L.T. 2. E-02 06/11 06/18 9.96E 03 CU. FT. 07/02 1.2 a 0.3 E-02 06/19 L.T. 4. E-02 06/18 06/24 1.14E 04 CU. FT. 07/10 3.4 1 1.9 E-03 06/26 L.T. 3. E-02 06/24 06/27 3.81E 03 CU. FT. 07/15 3.3 2 0.7 E-02 07/03 L.I. 1. E-Ul(b)

I a Sample not received; lost during collection. h Pump ealfunctlen; required LLO not met due to low air volume.

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CllARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STAi!ON NUMNER APG-1 1955 COLLECil0N DATE M10 COUNI A P FILIER 5 TART Mlu COUNT CHARC0AL FILTLu STOP Tint 6R055 NEIA IlhE l-131 OAIE DATE volume UNIIS DAIE (pct /Cu. M.) DATE (pct /Cu. M.) 07/01 07/02 I.75E 03 CU. FT. 07/17 5.1 2 1.2 E-02 07/11 L.T. 3, E-01(a) 07/08 07/13 7.78E 03 CU. FT. 07/22 2.4 1 0.4 E-02 07/17 L.T. 4. E-02 07/15 07/22 9.70E 03 CU. FT. 07/26 1.7 2 0.3 E-02 07/24 L.I. 3. L-02 o 07/22 07/29 9.40E 03 CU. FT. 08/07 1.9 2 0.3 E-02 07/31 L.T. 3. E-02 07/29 08/05 9.81E 03 CU. FT. 08/15 2.0 2 0.3 E-02 08/07 L.T. 3. E-02 04/05 08/12 9.28E 03 CU. FT. 08/19 2.1 a 0.3 E-02 08/14 L.I. 3. E-02 1 08/13 08/89 8.35E 03 Cu. FT. 08/29 1.4 1 0.4 E-02 08/22 I L.T. 4 E-uz 08/19 08/26 9.68E 03 CU. FT. 08/30 1.9 2 0.3 E-02 08/28 L.T. 3. L-02 08/26 09/03 1.13E 04 CU. FT. 09/09 2.0 t 0.3 E-02 09/04 L.T. 2. E-u2 09/03 09/09 8.35E 03 CU. FT. 09/19 1.9 t 0.4 E-02 09/10 L.I. 3. E-02 09/09 09/16 9.79E 03 CU. FT. 09/23 2.1 t 0.3 E-02 09/11 L.T. 4. E-02 09/16 09/23 9.97E 03 CU. FT. 10/03 2.1 1 0.3 E-02 09/24 L.T. 2. E-02 09/23 09/30 1.04E 04 CU. FT. 10/07 1.9 t 0.3 E-02 10/01 L.T. 2. E-02 (a) Required LLO could eat be met due to lov air voluee; pump salfunctioned.

      ~

l

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND 10 DINE-131 ANALYSES STATION NUNSER APG-1 15s3 COLLECitte DATE MID COUNT A P FILTER STAAT STOP hl0 COUNT CNAACOAL FILTER

IlmE GR055 SEIA Time I-131 OATE DATE WOLUNE Unli5 DATE (pC1/Cu. M.) OATE (pCi/Cu. M.)

09/30 10/07 9.63E 03 CU. FT. 10/11 1.9 s 0.3 E-02 10/08 L.T. 3. E-02 10/07 10/14 9.96E 03 CU. FT. 10/22 1.8 1 0.3 E-02 10/16 L.T. 3. E-02 g 10/14 10/21 9.92E 03 CU. Fi. 10/29 9.7 a 2.5 E-03 10/23 L.I. 3. E-02 } 10/21 10/28 9.88E 03 CU. FT. 11/13 1.3 1 0.3 E-02 10/30 L.T. 3. E-02 10/30 11/04 6.76E 03 CU. FT. 11/13 i 2.6

  • 0.5 E-02  !!/06 L.T. 4. E-02 j 11/04 11/11 9.SSE 03 CU. FT. 11/21 4.1 a 0.5 E-02 11/14 L.7, 3. E-02 11/11 11/18 9.86E 03 CU. FT. 11/25 1.5 2 0.3 E-02 11/22 L.T. 3. E-02 11/18 11/25 9.92E 03 CU. F1. 12/06 2.3 1 0.4 E-02 12/02 L.I. 4. E-02 4

11/25 12/02 9.ssf 03 CU. FT. 12/09 7.6 a 3.3 E-03 12/04 L.T. 3. E-02 12/02 12/09 1.00E 04 CU. FT. 12/18 3.4 1 0.4 E-02 12/11 L.T. 3. E-02 12/09 12/16 9.30E 03 CU. FT. 12/30 2.4 a 0.3 E-02 12/19 L.T. 3. E-02 12/16 12/23 9.70E 03 CU. FT. 01/03 3.3 a 0.4 E-02 12/27 L.T. 3. E-02 12/23 12/30 9.96E 03 CU. FT. 01/07 2.6 t 0.4 E-02 01/02 L.I. 3. E-02 1 e 4

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CilARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APP-1 1955 COLLECil64 DATE STAST STOP MID COUNT A P FILilR MID COUNI CHASCOAL FILTEk Tint GROSS BEIA ilME DATE DATE V0tDNE UNITS DATE (pCl/Co. M.) l-131 DATE (pC1/Cu. M.) 12/31 01/07 1.02E 04 CU. FT. 01/15 2.0 2 0.3 E-02 01/11 L.T. 4 E-02 01/07 01/14 4.70E 03 CU. FT. 01/25 2.5 t 0.4 E-02 ! 01/16 L.T. 2. E-02 01/14 01/22 1.17E 04 CU. FT. 01/30 1.9 1 0.3 E-02 01/24 L.T. 4 E-02 01/22 01/28 4.70E 03 CU. FT. 02/06 2.0 1 0.4 E-02 01/30 L.T. 3 E-02 01/28 02/04 1.03E 04 CU. FT. 02/11 2.0 2 0.3 E-02 02/07 L.T. 4 E-02 02/04 02/11 1.02E 04 CU FT. 02/21 3.4 a 0.4 E-02 02/13 L.T. 3. E-02 ] 02/11 02/18 1.0lf 64 CU. FI. 02/26 2.6 1 0.4 E-02 02/21 L.T. 3. E.02 02/18 02/25 1.03E 04 CU. FT. 03/05 1.5 1 0.3 E-02 02/27 L.T. 3. E-02 j 02/25 03/04 1.03E 04 CU. FT. 03/13 1.9 2 0.3 E-02 03/06 L.T. 3. E-02 03/04 03/11 1.03E 04 CU. Fi. 03/20 1.4 a 0.3 E-02 03/13 L.T. 3. E-02 j 03/11 03/18 1.03E 04 CU. FT. 03/26 2.0 1 0.3 E-02 03/20 L.T. 3. E-02 03/18 03/25 1.03E 04 CU. FT. 03/29 1.4 1 0.3 E-02 03/28 L.T. 4 E-02 03/25 04/01 1.03E 04 CU. FT. 04/08 2.1 s 0.3 E-02 04/03 L.T. 3. E-02 e. u 4 i

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND IODINE-131 ANALYSES stall 0N NUM8ER APP-1 1955 COLLECil0N DATE MID COUNT A P FILTER 4 START STOP MID COUNT CHARCOAL FILTER ilME Ga0$$ SEIA SATE DATE VOL UME UNIT 5 DATE (pCl/Cu. M.) 11ME l-131 DAlf (pCl/Cu. M.) 04/01 04/09 1.18E 04 Cu. FT. 04/16 1.8 1 0.3 E-02 04/11 L.T. 3 L-02 04/09 04/15 8.83E 03 CU, FT. 04/25 1.9 i 0.4 E-02 04/18 L.I. 4 E-02 04/15 04/22 1.02E 04 CU. FT. 05/01 2.5 1 0.4 E-02 04(24 L.I. 3. E-02 U 04/22 04/29 1.01E 04 CU. FT. 05/24 2.2 a 0.3 E-02 05/01 L.T. 3. E-02 . 04/29 05/06 1.olf 04 CU. FT. 05/14 2.0 1 0.3 E-02 05/08 L.T. 2. E-02 1 05/06 05/13 1.02E 04 CU. FT. 05/21 2.3 a 0.3 E-02 05/16 L.T. 4 E-02 05/13 05/20 1.03E 04 CU. FT. 05/31 2.1 a 0.3 E-02 05/23 L.T. 3. E-02 05/20 05/27 1.03E 04 CU. FT. 06/06 2.5 2 0.3 E-02 05/30 L.T. 2. E-02 05/27 06/03 1.00E 04 CU FT. 06/17 2.9 1 0.3 E-02 06/05 L.I. 3. E-02 4 06/03 06/10 1.04E 04 CU. ii. 06/19 3.1 0.4 E-02 06/13 L.T. 2. E-02 06/10 06/17 9.65E 03 CU. FT. 07/02 1.1 i 0.3 E-02 06/19 L.T. 5. E-02 06/17 06/24 1.0lt 04 CU. FT. 01/10 2.4 t 0.3 E-02 06/26 L.T. 3. E-02 06/24 07/01 9.94E 03 CU. fi, 07/15 2.7

  • 0.4 E-02 07/03 L.I. 4 E-02

]

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APP-1 Isss COLLECTION SATE MID COUNT START STOP - A P FILTER nib COUNT CHASC0AL FILith TINE GROSS SETA BATE DATE VOLUME 04I15 OATE (pct /Cu. M.) TEME l-131 DATE (pct /Cu, M.) 07/01 07/08 1.0lf 04 CU. FT. 07/11 1.7

  • 0.3 E-02 07/11 L.T. 3. E-02 07/08 07/15 9.99E 03 CU. FT. 07/22 2.4 s 0.3 E-02 07/17 L.T. 3. E-02 07/15 07/22 1.05E 04 CU. FT. 07/26 l'.5 1 0.3 E-02 07/24 L.T. 3. E-02
 $                            07/22                             07/29    9.53E 03      CU. FT. 08/07      1.7 1 0.3 E-02    07/31           L.T.         3. E-02 07/29                             08/05     1.00E 04      CU. FT. 08/15     1.7 2 0.3 E-02     04/07           L.T.         3. E-02 08/05                             08/12    9.96E 03       CU. FT. 08/19
 '                                                                                                           1.9 1 0.3 E-02     08/14          L.T.          3. E-02 08/12                             08/19    1.00E 04      CU. FT. 08/29      1.3 1 0.3 E-02     08/22          L.T.        3. E-02 08/19                             08/26    1.02E 04      CU. FT. 04/30      1.8 1 0.3 E-02     08/28          L.T.         3. E-02 08/26                             09/03    1.12E 04     CU. FT.      09/09      1.8 s 0.3 E-02     09/04          L.T.        2. E-02 5

09/03 09/09 8.53E 03 CU. FT. 09/19 1.3 2 0.3 E-02 09/10 L.T. 3. E-02 09/09 09/16 9.98E 03 CU. FT. 09/23 2.1 2 0.3 E-02 09/17 L.T. 4. E-02 09/16 09/23 9.9tf 03 CU. FT. 10/03 ' 2.0 s 0.3 E-02 09/24 L.T. 2. E-02 09/23 09/30 1.03E 04 CU. FT. 10/07 1.8 2 0.3 E-02 10/01 L.T. 2. E-02 1

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CilARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES

                                                                            $1A'l0e i    NUNGER APP-1 Ivus COLLECilee  0 ATE                             M10 C00mi START       STOP A P FILIER       MID COUni CHAkC0AL FILTER tine     GROSS SEIA         ilME BATE        BATE     WOL umE       UnlT$         SATE     (pCi/Co. M.)                     l-131 DATE    (pCS/Cu. M.)

09/30 10/07 9.64E 03 CU. FT. 10/11 2.1 1 0.3 E-02 10/08 L.T. 3. E-02 10/07 10/14 9.95E 03 10/22 CU. ft. 2.4 s 0.3 E-02 10/16 L.T. 3. E-02 10/14 10/2; 9.80E 03 CU. FT. 10/29 1.3 2 0.3 E-02 10/23 L.T. 3. E-02 g 10/21 10/28 9.97E 03 CU. FT. 11/13 1.4 2 0.3 E-02 10/30 L.T. 3. E-02 10/28 11/00  % 17E 03 CU. FI. 11/13 1.5 s 0.3 E-02  !!/06 L.T. 3. E-02 11/04 11/11 9. Dot 03 CU. FI. 11/21 3.4 2 0.4 E-02 11/14 L.T. 3. E-02 11/11 11/18 9.85E 03 CU. FT. 11/25 1.6 1 0.3 E-02  !!/22 L.T. 3. E-02 11/18 11/25 9.94E 03 CU. Fi. 12/06 2.5 t 0.4 E-02 12/02 L.I. 4. E-02 11/25 12/02 1.02E 04 CU. FT. 12/09 L.T. 5. E-03 12/04 L.f. 3. E-02 12/02 12/09 1. ole 04 CU. FT. 12/18 3.2 1 0.4 E-02 12/II L.T. 3. E-02 12/09 12/16 9.54E 03 CU FT. 12/30 2.1 a 0.3 E-02 12/19 L.T. 3. E-02 12/16 12/23 9.861 03 CU. FT. 01/03 3.8 a 0.4 E-02 12/27 L.I. 3. E-02 12/23 12/30 9.84E 03 CU. FT. 01/07 2.2 a 0.3 E-02 01/02 L.T. 3. E-02

i TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APQ-1 4 1955 ' COLLECil0N SATE N10 COUNT START STOP A P FILTER MIO COUNI CHAkC0AL FILTER 0 ATE ilNE GROSS BETA IINE l-131 DATE VOLUME Unlii OATE (pCl/Co. M.) 0 ATE (pct /Cu. M.) 12/31 01/07 3.04E 03 CU. FT. 01/15 2.3 2 0.4 E-02 01/!! L.T. 5. E-02 01/07 01/14 8.22E 03 CU. FT. 01/25 2.7 i 0.4 E-02 01/16 L.T. 3. E-02

              -01/14        01/22    8.90E 03      CU. FT.      01/30      2.4 a 0.4 E-02 01/24     ^L.T. 5. E-02 01/22        01/28   6.27E 03       CU. FT.      02/06      2.0 2 0.5 E-02   01/30      L.T. 4    E-02 01/28       02/04     7.49E 03      CU. FI.      02/11     2.2 1 0.4 E-02    02/07      L.T. 6. E-02 02/64       02/11    7.45E 03       CU. FT.      02/21 3.5 t 0.5 E-02   02/13       L.T. 4    E-02 02/11       02/18    7.41E 03       CU. FT. 02/26      2.6 2 0 4 E-02   02/21    '

L'T.

                                                                                                         . 4    E-02 02/13       02/25    7.47E 03       CU. FT. 03/05      1.7 1 0.4 E-02   02/27       L.I. 4    E-02 02/25       03/04    7.48E 03       CU. FT. 03/13      1.8 1 0.4 E-02   03/06      L.T. 4    E-02 j               03/05       03/11    a . 60E '03    CU. FT. 03/20      2.4 t 0.3 E-02   03/13      L.T. 3. E-02 03/11        03/18    1.01E 04       CU. FT. 03/26      2.0 1 0.2 E-02   03/20      L.T. 3    E-02 03/13        03/25    1.0lt 04       CU. FT. 03/29      3.0 t 0.4 E-02   03/28      L.T. 5. E-02 03/25        04/01    1.02E 04       CU. FT. 04/08      2.2 1 0.3 E-02   04/03      L.T. 3. E-02

) i

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND IODINE-131 ANALYSES STATION NUNSER APQ-1 isss COLLECTION SATE START STOP MID COUNT A P FILIER M10 COUNI CHARCOAL FILIEu 0 ATE TIME GROS 5 BLIA TIME 0 ATE VOL UME UNIIS DATE (pct /Cu. M.) l 131 DAll (pCI/Co. M.) 04/01 04/09 1.16E 04 CU. FT. 04/16 1.8 1 0.3 E-02 04/l! L.T. 3. E-U2 04/09 04/15 4.69E 03 CU. FT. 04/25 2.2 a 0.4 E-02 04/18 L.T. 4. L-02 04/15 04/22 1.02E 04 CU. FT. 05/01 2.0 a 0.3 E-02 04/24 L.T. 3. E-U2 04/22 04/29 1.03E 04 CU. FT. 05/24 2.1 1 0.3 E-02 05/0! L.T. 3. E-02 04/29 05/06 1.04E 04 CU. FT. 05/14 2.0 1 0.3 E-02 05/08 L.T. 2. E-02 05/06 05/13 1.04E 04 CU. Fi. 05/21 2.4 a 0.3 E-02 05/16 L.T. 4. E-02 05/13 05/20 1.03E 04 CU. FT. 05/31 2.3 2 0.3 E-02 05/23 L.T. 3. E uz 05/20 05/27 1.03E 04 CU. FT. 06/06 2.1 4 0.3 E-02 05/30 L.T. 2. E-U2 05/27 06/03 1.04E 04 CU. F T. 06/17 2.3 1 0.3 E-02 06/05 L.T. 3. E-02 06/03 06/10 1.09E 04 CU. FT. 06/19 2.9 2 0.3 E-02 06/13 L.I. 2. E-02 06/10 06/17 1.04E 04 CU. Fi. 07/02 1.2 2 0.3 E-02 06/19 L.T. 4. L-02 06/17 06/24 1.IIE 04 CU. FT. 07/10 2.1 a 0.3 E-02 06/26 L.T. 3. L-ur 06/24 07/01 1.04E.04 CU. FT. 07/15 2.6 1 0.3 E-02 07/03 L.T. 4 E u2 4 d

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND 10 DINE-131 ANALYSES i 51 A1104 NutISER APQ-1 i 1 ' ives COLLECiles OArt MID COUNT A P FILIER START STOP M10 COUNT CHAAC0AL FILTLk TIME GROSS BETA OATE DATE WOL U8tf UNITS DATE (pCl/Co. II. ) TIME I-131 DATE (pCl/Cu. ft.) 07/01 07/08 1.05E 04 CU. FT. 07/17 1.7 2 0.3 E-02 07/11 L.T. 3. E-02 07/08 07/15 1.03E 04 .CU. FT. 07/22 2.4 a 0.3 E-02 07/17 L.T. 2. E-02

07/15 07/22 1.10E 04 CU. FT. 07/26 1.9 i 0.3 E-02 07/24 L.T. 2. E-02
       $       07/22        07/29    1.00E 04     CU. FT.       08/07                    2.0 t 0.3 E-02                    07/31       L.T.        3. E-02 07/29       08/05     1.04E 04     CU. FT.       08/15                    2.1 a 0.3 E-02                    08/07       L.I.        3. E-02 i               08/05       08/12    1.03E 04      CU. FT.       08/19                    2.5 t 0.3 E-02                   08/14        L.T.       3. E-02 08/12       08/19    1.04E 04      CU. Fi.       08/29                    1.5 t 0.3 E-02                   08/22        L.T.       3. E-02 i-              0./it       08,2. i.05E 04      CU. Fi.       08/30                    2.0 t . 3 E-02                   08/2.        t.i.       3. E-02 08/26       09/03    1.15E 04      CU. FT.       09/09                    2.1 a 0.3 E-02 1                                                                                                                         09/04         L.T.       2. E-02 09/03       09/09    8.59E 03     CU. FT.        09/19                    1.4 t 0.3 E-02                 09/10         L.T.        3., E-02

! 09/09 09/16 1.01E 04 CU. FI. 09/23 1.7 2 0.3 E-02 09/17 L.I. 4. E-02 09/16 09/23 9.91E 03 CU. FT. 10/03 1.7 a 0.3 E-02 t 09/24 L.I. 2. E-02 1 09/23 09/30 1.02E 04 CU. Fi. 10/07 2.0 t 0.3 E-02 10/01 L.T. 2. E-02 ) i l i t

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CilARCOAL CARTRIDGES: GROSS BETA AND 10 DINE-131 ANALYSES STAil0m NUMSER APQ-1 its> COLLECilos DATE MID COUNT A P FILTER MID COUni CHARC0AL FILTER START STOP TIME GROSS BETA TIME I-131 DATE DATE VOL UME UNITS DATE (pCl/Cu. M.) DATE (pct /Cu. M.) 09/30 10/07 9.47E 03 CU. FT. 10/11 1.7 a 0.3 E-02 10/08 L.T. 3. E-02 10/07 10/14 9.80E 03 CU. FT. 10/22 2.3 1 0.3 E-02 10/16 L.T. 3. E-02 10/14 10/21 9.70E 03 CU. FT. 10/29 1.1 2 0.3 E-02 10/23 L.T. 3. E-02 10/21 10/28 S.SSE 03 CU. FT. 11/13 1.5 t 0.3 E-02 10/30 L.T. 3. E-02 . u 10/30 11/04 (a) e 11/04 11/11 1.02E 04 CU. FT. 11/21 3.1 2 0.4 E-02 11/14 L.T. 3. E-02 11/11 11/18 1.00E 04 CU. FT. 11/25 1.4 a 0.3 E-02 11/22 L.T. 3. E-02 11/18 11/25 1.02E 04 CU. FT. 12/06 2.4 1 0.4 E-02 12/02 L.T. 4. E-02 j 11/25 12/02 9.89E 03 CU. FT. 12/09 7.8 1 3.3 E-03 12/04 L.T. 3. E-02 12/02 12/09 1.04E 04 CU. FT. 12/18 3.4 2 0.4 E-02 12/11 L.T. 3. E-02 12/09 12/16 9.57E 03 CU. FT. 12/30 2.1 1 0.3 E-02 12/19 L.T. 3. E-02 i 12/16 12/23 9.96E 03 CU. F T. 01/03 3.6 2 0.4 E-02 12/27 L.T. 3. E-02 12/23 12/30 9.97E 03 CU. FT. 01/07 2.2 1 0.3 E-02 01/02 L.T. 3. E-02 (a) No sample evallable; untL being repaired. 1

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: CROSS BETA AND IODINE-131 ANALYSES STAil04 NUMBER APE-30 Iss3 COLLECil04 DATE . MID COUNT A P FILTER START STOP M10 COUNT CHARCOAL FILTER TIME GROSS SEIA TIME - 1 131 DATE DATE V0t uME UnlT5 DATE (pct /Cu. M.) DATE (pct /Cu. M.) 12/31 01/07 9.77E 03 CU. Fi. 01/15 2.4 a 0.3 E-02 01/11 L.T. 2. E-02 i 01/07 01/14 9.84E 03 CU. FT. 01/25 2.5 t 0.4 E-02 01/16 L.T. 1. E-U2 01/14 01/22 1.12E 04 CU. FT. 01/30 2.0 1 0.3 E-02 i e 01/24 L.T. 2. E-02 O 01/22 01/28 8.21E 03 CU. FT. 02/06 I.9 2 0.4 E-02 01/30 L.T. 3. E-02 01/28 02/04 9.68E 03 CU. FT. 02/11 2.2 a 0.4 E-02 02/07 L.T. 2. E-U2 02/04 02/11 9.69E 03 CU. FT. 02/21 3.2 t 0.4 E-02 02/13 L.T. 2. E-02 02/11 02/18 9.68E 03 CU. FT. 02/26 2.8 2 0.4 E-02 02/21 L.T. 2. E-U2 02/18 02/25 9.65E 03 CU. FT. 03/05 1.7 2 0.3 E-02 02/27 L.T. 2. E-02 02/25 03/04 9.83E 03 CU. FT. 03/13 1.7 1 0.3 E-02 03/06 L.T. 2. E-02 03/04 03/11 9.80E 03 CU. FT. 03/20 2.0 2 0.3 E-02 03/13 L.I. 2. E-02 03/11 03/18 9.84E 03 CU. FT. 03/26 1.9 i 0.3 E-02 03/20 L.T. 2. E-02 03/18 03/25 9.90E 03 CU. FT. 03/29 1.6 2 0.3 E-02 03/28 ' L.T. 2. E-02 03/25 03/29 9.89E 03 CU. FT. 04/08 2.2 a 0.3 E-02 04/03 L.I. 2. E-02 2

                                                         .                   TABLE B-2 (Cont.)

AIR PARTICU1 ATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STAil0m NUNSER APE-30 isas COLLECil0N DATE MID COUNT A P FILTER Mlu CUUNI START STOP CHAkC0AL FILTEN TIME 640$$ SETA TIME l-131 DATE 0 ATE VOL UME UNITS DATE (pCl/Cu. M.) DATE (pct /Co. M.) 04/01 04/09 1.!!E 04 CU. FT. 04/16 2.1 a 0.3 E-02 04/11 L.T. 2. E-02 04/09 04/15 8.43E 03 CU. ft. 04/25 2.4

  • 0.4 E-02 04/18 L.T. 2. E-02 04/15 04/22 9.87E 03 CU. FT. 05/01 2.3 1 0.3 E-02 04/24 L.T. 2. E-02 04/22 04/29 9.99E 03 CU. FT. 05/24 2.4 2 0.4 E-02 05/01 L.T. 2. E-02 O 04/29 05/06 9.88E 03 CU. FT. 05/14 1.9 1 0.3 E-02 05/08 L.T. 2. E-02 05/06 05/13 9.99E 03 CU. FT. 05/21 2.0 t 0.3 E-02 05/16 2.

L.T. E-02 05/13 05/20 9.95E 03 CU. FT. 05/31 2.0 2 0.3 E-02 05/23 3. L.T. L-02 05/20 05/27 1.00E 04 CU. FT. 06/06 2.5 1 0.3 E-02 05/30 L.T. 2. E-02 05/27 06/03 9.98E 03 CU. FT. 06/17 2.2 a 0.3 E-02 04/05 2. L.I. E-U2 06/03 06/10 9.82E 03 CU. FT. 06/19 2.6 s 0.4 E-02 06/13 2. L.T. E-02 06/10 06/17 9.94E 03 CU. FT. 07/02 1.6 2 0.3 E-02 06/19 2. L.T. E-02 06/17 06/24 1.02E 04 CU. FT. 07/10 2.0 t 0.3 E-02 06/26 2. L.T. L-U2 06/24 07/01 1.00E 04 07/15 07/15 2.5 2 0.3 E-02 07/03 2. L.I. E-U2

TABLE B-2 (Cont.) AIR PARTICULATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINE-131 ANALYSES STAil0N NUNSER APE-30 lyst COLLECTION SATE Mio COUNT A P FILTER M10 COUNT START STOP CHARC0AL FILIER TIME G8055 SETA TIME l-131 DATE DATE VOL UME UNIIS DATE (pct /Cu. M.) DATE (pct /Cu. M.) 07/01 07/08 9.93E 03 CU. FT. 07/17 1.7 1 0.3 E-02 07/11 L.T. 2. E-02 07/08 07/15 1.0lt 04 CU. FT. 07/22 2.2 1 0.3 E-02 07/17 L.T. 2. E-02 07/15 07/23 1.10E 04 CU. FT. 07/26 1.7 1 0.3 E-02 07/24 L.T. 2. E-02 07/23 07/29 8.91E 03 CU. FT. 08/07 1.8 1 0.3 E-02 07/11 L.T. 2. , E-02 07/29 08/05 1.00E 04 CU. FT. 08/15 1.7 s 0.3 E-02 08/07 2. L.T. E-02 08/05 08/12 9.96E 03 CU. FT. 08/19 1.9 2 0.3 E-02 08/14 2. L.T. E-02 08/12 08/19 1.00E 04 CU. FT. 08/29 1.5 t 8.3 E-02 08/22 L.T. 2. E-02 08/19 08/26 1.02E 04 CU. 6 8. 08/30 1.8 2 0.3 E-02 08/28 2. L.T. E-02 08/26 09/03 1.13E 04 CU. FT. 09/09 1.8 1 0.3 E-02 09/04 L.T. 1. E-02 09/03 09/09 8.45E 03 CU. FT. 09/19 1.3 1 0.3 E-02 09/10 L.T.

2. E-02 09/09 09/16 9.98E 03 CU. FT. 09/23 2.2 1 0.3 E-02 09/17 2.

L.I. E-02 09/16 09/23 9.82E 03 CU. FT. 10/03 1.6 1 0.3 E-02 09/24 L.T. 2. E-02 09/23 09/30 9.73E 03 CU. FT. 10/07 2.3 1 0.3 E-02 10/01 2. L.T. E-02

TABLE B-2 (Cont.) AIR PARTICUIATE FILTERS AND CHARCOAL CARTRIDGES: GROSS BETA AND IODINK-131 ANALYSES 5iAT104 NUNSER nPE-30 1v53 " COLLECTION DATE START M10 COUNT A P FILTER MID COUNT CHARCOAL FILTER STOP Tint GROS 5 SE TA ilhE l-131 DATE DATE VOLUME UnlTS DATE (pCl/fu. M.) DATE (pCl/Cu. M.) i a 09/30 10/07 1.00E 04 CU. FT. 10/11 1.6 a 0.3 E-02 10/08 L.T. 1. L-02 10/07 10/14 9.83E 03 CU. FT. 10/22 2.5 t 0.3 E-02 10/16 L.T. 2. E-02 10/14 10/21 9.88E 03 CU. FT. 10/29 1.2 2 0.3 1-02 10/23 L.T. 2. E-02

;    10/21          10/28      9.90E 03       CU. FT.     !!/13     9.9 a 2.7 E-03      10/30    L.T. 2. E-02
  $  10/28         11/04       9.82E 03      CU. FT.      11/13     2.1 1 0.3 E-02      11/06    L.T. 3. E-02 11/04         11/11       9.64E 03      CU, FT.      11/21     3.2 a 0.4 E-02      !!/14    L.T. 2. E-02 11/11         11/18       9. 7 9E 03    CU. FT.      11/25     1.5 1 0.3 E-02      11/22   L.T. 3. E-02 11/18         11/25       9.66E 03      CU. FT.      12/06     2.4 2 0.4 E-02      12/02   L.T. 4   E-02 11/25         12/02      9.77E 03       CU. FT.      12/09     L.T. 5. E-03   12/04   L.T. 2. E-02 12/02          12/09      4.46E 02       CU. FT.      12/18     8.2 & 3.1 E-02(a)   12/11   L.T. 2. E-Ul(b) 12/10          12/16      8.04E 03       CU. FT.      12/30     2.4 a 0.4 E-02 12/19    L.T. 3. E-02 12/16          12/23      9.33E 03       CU. FT. 01/03      3.6 1 0.4 E-02     12/27    L.T. 2. E-02 12/23          12/30      9.28E 03       CU. FT. 01/07      1.9 1 0.3 E-02     01/02 i                                                                                                L.T. 2. E-02 (a) Hi9h gross beta result due to low air volume.

t (b) Required LLO could not be met due to low air volume. 4 ] 4

TABLE B-3 AIR PARTICULATE FILTERS: CAttiA ISOTOPIC ANALYSIS ON QUARTERLY COMPOSITES (pCl/Cu.M.) STAil0N NUNGER APC-1 GAMMA SPECTRUM ANALV515 FIRST QUARTER SECouc QUARTER THIR0 QUANTER FOURIN QUAkiER 4 12/31-04/01 04/01-07/01 07/01-09/30 09/30-12/30 SE-7 8.863 0.95E-02 9.03 1.27E-02 8.044 0.80E-02 9.494 0.9hE-02 K-40 L.T. 1. E-02 L.T. 3. E-02 5.22 22.92E-03 1.02t 0.3sE-02

                  ,     Ma-54                                       L.T. 7. E-04          L.I. 1. E-03  L.T. 4. E-04 L.T. 7. E-04 C0-58                                       L.T. 8. E-04          L.T. 1. E-03   L.T. 5. E-04
                                                                                      ,                                           L.T. 8. E-04 FE-59                                       L.T. 2. E-03          L.T. 3. E-03   L.T. 1. E-03 s

L.I. 2. E-03 CD-60 L.T. 1. E-03 L.T. 1. E-03 L.T. 4 E-04 L.T. 9. E-04 25-65 L.T. 2. E-03 L.T. 3. E-03 L.1. 1. E-03 L.T. 1. E-03 2R-95/m8-95 L.T. 8. E-04 L.T. 1. E-03 L.T. 5. E-04 L.T. 4. E-04 RU-103 L.T. 1. E-03 L.T. 1. E-03 L.T. 6. E-04 L.T. 1. E-03 AU-106 L.T. 6. E-03 L.T. 8. E-03 L.T. 4. E-03 L.T. 6. E-03 I-131 L.T. 7. E-03 L.T. 7. E-03 L.T. 2. E-03 L.T. 5. E-03 C5-134 L.I. 8. E-04 L.T. 1. E-03 L.T. 5. E-04 L.I. 9. E-04 C5-137 L.T. 7. E-04 L.T. 1. E-04 L.T. 4. E - 04 L.I. 8. E-04 BA-140/LA-140 L.T. 3. E-03 L.T. 4 E-03 L.T. 1. E-03 L.T. 3. E-03 CE-141 L.T. 1. E-03 L.T. 2. E-03 L.T. 1. E-03 L.T. 1. E-03 CE-144 L.T. 3. E-03 L.T. 5. E-03 L.T. 3. E-03 L.T. 4. E-03 l RA-226 L.T. 1. E-02 L.T. 1. E-02 9. L.T. E-03 L.T. 1. E-02 TH-228 L.T. 1. E-03 L.I. 1. E-03 L.T. 9. E-04 L.I. 1. E-uj i

l

                             .                  TABLE B-3 (Cont.)

AIR PARTICUIATE FILTERS: CADelA ISOTOPIC ANALYSIS ON QUARTERLY COMPOSITES (pCl/Co.N.) STATION NUNSER APG-1 SANNA SPECTRUM ASALYSIS FIRST QUARTER SEC0e0 QUARTER THIRO QUARTER fuuRTH QUARTER 12/31-04/01 04/01-07/01 07/01-09/30 09/30-12/30 BE-7 9.614 1.41E-02 7.311 0.89E-02 8. 5 3 20. 7 9E -02 1.01 so.11E-01 K-40 1.864 0.92E-02 L.T. 9. E-03 L.T. 9. E-03 L.T. 3. E-02

   $ Ne-54                     L.T. 9. E-04         L.T. 5. E-04 L.T. 4. E-04  L.T. 1. E-03 C0-58                     L.T. 1. E-03         L.T. 6. E-04 L.T. 6. E-04  L.T. 1. E-03 i

FE-59 L.T. 3. E-03 L.T. 1. E-03 L.T. 1. E-03 L.T. 3. E-03 i CO-60 L.T. 1. E-03 L.T. 5. E-04 L.T. 5. E-04 L.T. 1. L 03 2n-65 L.T. 3. E-03 L.T. I. E-03 L.T. 1. E-03 L.T. 2. E-03 2R-95/es-95 L.T. 1. E-03 L.T. 6. E-04 L.T. 5. E-04 L.T. 1. E-U3 RU-103 L.T. 1. E-03 L.T. 8. E-04 L.T. 7. E-04 L.T. 1. E-03 RU-106 L.T. 9. E-03 L.T. 5. E-03 L.T. 4. E-03 8. L.T. E-03 1 131 L.T. 9. E-03 L.T. 8. E-03 L.T. 3. E-03 L.T. 6. E-03

;    C5-134                    L.T. 1. E-03         L.T. 6   E-04 L.T. 5. E-04          1.

L.T. E-03 C5-137 L.T. 1. E-03 L.T. 5. E-04 L.T. 6. E.04 L.T. 9. E-04 , BA-140/LA-140 L.T. 4. E-03 L.T. 4. E-03 L.T. 2. E-03 L.T. 3. E-03 CE-141 L.T. 2. E-03 L.T. 1. E-03 L.T. 1. E-03 L.I. 2. E-03 CE-144 L.T. 5. E-03 L.T. 3. E-03 3. E-03 L.T. L.T. 5. E-03 RA-226 L.I. 1. ,E-02 L.T. 9. E-03 L.I. 1. E-02 > L.T. 1. E-02 TH-228 L.I. 1. E-03 L.T. 9. E-04 L.I. 8. E 04 L.T. 1. E-03 l

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TABLE B-3 (Cont.) AIR PARTICULATE PILTERSI CAletA ISOTOPIC ANALYSIS Oli QUARTERLY COMPOSITES l (pCl/Cu.N.) STAil0N NUNSER APQ-1 I EANNA SPECTRUN ANAL V515 FIRST QUARTER SEC040 QUARTER THIRD QUARTER 12/31-04/01 04/01-07/01 FOURTH QUANIER 07/01-09/30 09/30-12/30 SE-7 8.62: 0.86E-02 8.71 0.97E-02 8.44 11.50E-02 9.358 0.94E-02 E-40 L.I. 1. E-02 L.T. 3. E-02 1.37 10.55E-02 9. L.T. E-03 Ne-54 L.T. 5. E-04 L.I. 9. E-04 L.T. 8. E-04 L.T. 4. L-04 CO-50 L.T. 6. E-04 L.I. 1. E-03 L.T. 8. E-04 5. L.T. L-04 i FE-59 L.T. 1. E-03 L.I. 3. E-03 L.T. 2. E-03 L.T. 1. E-03 CS-60 L.I. 5. E-04 L.I. 8. E-04 L.T. 7. E-04 L.T. h. E-04 2N-65 L.T. 1. g-03 L.I. 2. E-03 L.I. 2. E-03 1. L.T. E-03 2R-95/88-95 L.I. 6. E-04 1. E-03 L.I. L.T. 3. E-04 L.I. 6. E-04 RU-103 L.T. 6. E-04 1. L.T. E-03 L.T. 1. E-03 L.I. 6. L-04 R0-106 L.I. 4. E-03 L.T. 7. E-03 L.T. 7. E-03 L.T. 4. E-uj I-131 L.T. 5. E-03 6. E-03 L.T. L.T. 5. E-03 L.I. 3. E-03 C5-134 L.T. 5. E-04 L.T. 9. E-04 L.T. 9. E-04 5. L.I. E-b4 C5-137 L.T. 7. E-04 9. L.T. E-04 L.T. a. E-04 L.T. 6. E-04 B A-140/L A-140 L,T. 2. g-03 L.T. 3. E-03 L.T. 2. E-03 L.T. 2. E-03 CE-141 1. E-03 L.T. L.T. 1. E-03 L.I. 2. E-03 L.T. 1. E-oj CE-144 L.I. 3. E-03 L.T. 4. E-03 L.T. 5. E-03 L.T. 3, g-oj RA-226 L.T. 9. E-03 L.T. 1. E-02 L.I. 2. E-02 L.I. 8. L-uJ l TH-228 L.I. 1. E-03 L.I. 1. E-03 i t.I. 2. E-03 L.g. g, g-og a

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D s T. I. I. I. T. I. T. T. I. T. T. T. T. I. r e _ L L L L L L L L L L L L L L l p m a s o t e u _ , d e l b

             .                                                                                                                                                                 a l

_. i a 5 5 5 5 5 5 5 v 5 5 5 5 5 5 5 a _ 8 8 8 /8 / 8/ 8/ 8/ 8 / /8 /8 /8 /8/3 8 0 e 7/ /2 / 5 8 4 t t 0 2 9 8 1 5 9 7 0 4 8 e

                                         / /1 / /

1 0 1 0 1 2 1 2 1 2 8 s 2 / 2/ / / 3/ /4 / 4/ /4 / _ i T 1 A 3 5 5 6 6 7 e T 0 4 e 4 8 -8 8 8 -0 0 0- - - - l p S 4 5 5 5 5 5 5 5 5 5 5 5 5 5 m

                              -         8/ /87 /0 /               8/ 8/ 8/ 8          /    /0 /8 /8 /8/ 8/ 8 8                                                                S a

4 2 5 8 4 8 1 5 9 3 7 8 4 E 2 0 2 0 1 0 1 8 1 2 1 2 1 2 T A 2/ /1 / / /2 / 2/ /3 / 3/ /4 /4 4/ / 1

                                                                                                                                                                              )

S 5 5 6 6 a 1 0 0 s 0 8 8 8 S 0 4 8 4 0 ( t Iil i 2l  !, 1 )!j? j  !

                                                                                                                           '                           i1'                 !{        ,

Ili!i ll, j

TABLE B-4 (Cont.) DRINKING WATER: IODINE-131 ANALYSIS (pC1/1)

COLLEClies SATE STAlles SWG-2 sgE-5

! dup-7

;                                  G7/44/85-87/23/85                                L.I.      2. E-01                                              L.I. 2    E-01 j

t.T. 2 E-ul 07/23/85-88/05/85 L.T. 5. E-01 L.I. 5. E-01 L.T. 5. i E-ul 88/05/85-80/19/05 L.T. 4. E-81 L.I. 4. E-01 4. L.T. L-un 48/19/85-89/03/85 L.I. 3. E-01 L.T. 3. E-01 L.T. 5. j L-un 89/03/85-89/16/85 L.I. 4. E-01 L.I. 4. E-01 4.

                                            ~

49/16/85-89/30/85 L.I. E-ul L.I. 4. E-41 L.I. 3. E-01 a L.T. 5. L-01 i3.iu i.fi4i.5 t.i. 4. E-ei i' t.i. 3. E-.i 3. 30/14/85-10/28/85 t.I. E-ui L.T. 2. E-SI (a) L.T. 2. E-01 L.i. 2. L-ut 10/28/85-11/11/05 L.I. 3. E-01 L.T. 3. E-01 L.T. 4. g.cg 11/11/85-!!/25/85 L.T. 4. E-01 L.I. 4. E-01 4. 11/25/85-12/09/85 L.T. E-ul L.I. 2. E-01 (b) L.I. 2. E-01 L.T. 4. t-ul 12/18/85-12/23/05 L.I. 4. E-01 L.I. 4. E-01 L.T. 5, g.gg

a b

Collectiaa dates 10/15/85-10/28/05 Collectica dates 11/25/85-12/10/85 i 1 l -. i l i

0 1 1 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 1 1 0 0 0 O 0 0 0 0 0 0 0 u 0 E E E E E E E E E E E 1 E E E E E E E E

                            /        4 3                    .       .      .       .      .        .      .      .         .       .       .        .        .         .       .

N0 1 3 5 3 3 6 3 6 3 3 3 5 3 3 4 5 2 7 6 C - R8 i A1 . . . . . . . . . . . . . . . . . . N/ 3 2 0 9 T. L T L

                                                         . I. T.      T. I. I.          T.        T.       T.      T.

T

                                                                                                                                        .      I.      T.        T.      T.        T.

T L L L L L L L L L L L L L L L L 0 1 1 0 0 0 0 0 0 0 1 0 0 0 0 0 1  ! 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 O 0 8 E E E E E E E E E E E E E E E E 1 E [ E V/ 3 R2 . . . . . . . . . . . . . . . . . . A0 1 3 4 3 3 6 3 7 3 4 3 9 3 3 6 6 2 7 6 U-A2 2 S B2 . . . . . . . . . . . . . . . . . . E E/ 2 S F1 0 7 T. L T. L T. L T. L T. L T. L T. L I. T. T. T. I. T. T. T. T. T. T. Y L L L L L L L L L L L L A N A S 2 C E - I T G P I W R O S S E T O 5 T O P -

-  A   S  M     R B   W   I  O )   E 1

0 1 0 1 0 0 0 0 0 0 0 1 1 0 0 1 0 1 1 0 E G A C 1 S

            / N          2 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 E        E       E       E      E       E      E        E L  N       Y 1 U          2                          8 E      E          E      E       E        E        E          E      E         E         [

B A I K M A L Cp N V/ 2 7 T N G H T ( E A1 A0 0 4 2 3 4 9 3 7 0 U - 4 5 3 3 4 3 1 9 3 7 7 I N l N4 R D O i A2 1 D N M A J/

                                               . 7         .      .       .      .        .      .        .        .       .       .        .        .         .        .        .         .

A N T S 2 1 1 1 I. 1 T. T. T. T. T. T. T. T. I. T. T. T. T. T. T. I. L 9 L L L L L L L L A O L L L L L L L L T E B S S O R C

5
        .                      5        1 1        5 5        V V        L L        A A        S R        A
A S N E L u 0 T A a 4 C C i 5 1 E I C 9 L N E
                                                                                                  -                                                 A t     E         P                                                        s o     N         S                                                        e                                                  L
                                                                                                                                                    /

C C / 3 0 A 4 3 9 6 4 7 0 1 4 6 8 G 0 5 5 0 0 1 3 3 4 4 4 2 2 E 1 3 7 0 5 5 5 6 6 9 T 0 - N - 4 - - - 1 1 3 1 1 1 1 1 2 2 A I - - - - - 1 - - - - - - - A a A E - # O E O N R 0 0 - 5 5 A E E A H D R G G B E N C F C 2 2 2 3 l C C S C C R I

  ;                 i i'                  .i;                                             i                         .i

O e O

  • O =O OO OO OO OO OOO OO O==O =. O O O O O O O O ==

O O O O O N tad led ted nad nad tad led ned tad w

                                       %                                                                                                                             ted       tad      led      tea         w w w                             w         ud 4                'O e,g g                    s               e         .         .         .           .         .         .         .           .        .         .        .

S e =* M 9 M M N M 4

  • M DN 9 N M M W # M S e "3 N *e g . . . . . . . . . . .

ed. W De De om, e t=. em eu em. D= O De >= o= em

                                                           .              .          .        .                     .         .      e=.e         .           . to.          .     >=.         .           e          .         .

a-

                                                                                                                                                                                                                                                        >=

a .d .a a .a .e =d

                                                                                                                                         #        a                 -d           d       d      .d          .d         .d          d             A         a
                                                       ==

O == O O.=. O OO OO O O O O OO OO OO =. O O O OO OO OO O .= =. O N O O O N tad ind ned las nas nna med had ins ame tea and tas ned w tad w tea tad sa N n= O e . . . . . . . . . . . * . 4 e O M 4A M M e M e M w E in M S M M e N M e N

                                      ==               ee UI                     %                                  .         .         .         .           .         .         .         .           .        .

W w O a= (f) O . o=. o=. >=. s=. s=. e. >=. >=. e=. >=. e=. a=. s=. a=. n=. ==. =

               >e
                                                      .=             .d         .a .a .a .a .4                                         s      .d         .d        .a =a .d                    .4                               .a
                                                                                                                                                                                                          .d         .a                     a            e 3

U3 N

 ^

O M e M 6e W

   .   .. dh,   M        3 d.n  M       C     tra     &

C W Fe U V O H j g u O -. M O O O O O O O ==

@    U
                        ^ tas M e
                        %. E to
                                     ==.

O tad O O O O O O O O O O O OO OO OOO O O O =.OO tad tas had tad tad 5 led tad a i 2.4 >. ,4  % had tad has ned tee had nad led nad ned and

     ,             ,,,3     a   -d w g                          -O                4A.                  .          .        .         .           .         .         .         .

W . . 4 ga3 2 w gy 5 =* w 4A M M N T W w in M ao T w N e M Gn CO

  1. GC C e-4 Q 2 4 m ime W ==

In O e. N N. e=. .=. a=. e=. a=. a=

                                                                                                                                     .      ,=.        n=.

e=

                                                                                                                                                                    .      n=. e=. >=.                      .       ,=.        .=                    .=

a .4 .d .a .4 .a .d .4 a .4 .a .4 s .4 .d a a a w t/3 t!) O as O

                                             ..               lA
          ,                                 tA                ==

a= 4A. 3 4A. 3 d 4 8 4 S 3 tae -d 2

                                   *=      4                 e                                                                                                                                        O u       u                 s=                                                                            4A 9

ese ted =. W @ d E and e

                                   -d                        e.

e 4 O and 2 4A e d W y S  %

                                                                                                                                           %M                    99                 e        N        O           se         e eNe
                                           .G.

W O 9 O 4A em O e se M M e w w tas O 4A 4A N N O O. lA @ @ e M me N N N. , e e e . . S. . a.s .e s.e m.e e m.e m.e l 4 4 5 a g O O e e i O M WW med S tad E E 3 3 4 4A in 4 tad led 4 E ad a W te. W N N g g == y u e y u a e. e i 72 1

O aa

  • O O O O O O O O O O O O OO OOO OO O O== O- O o o3 as O

gm O ned O O O O O tes ned w w nad % and ena ned w w tad w ia nas ned se.s w w .a hh EO and e q e e m o in e . . . e e o s s . e . . . . e e

                                                   >= m b O               80 M m e m e m e N e m m e de m a                                                                                                                             %

g,, g . . . . . . . . e . . e e e en m 4%e tuo t== De em aus gum go se pen O e . . . s e een tem pm em. >= pm pun ame > e e . . e . . . s .

                                                                                  .a        a         .a         .,a       a         .,,o         a       .e        .d        .a        .,a       .a            d       a          .4           a s         a O

O == O O == OO OOO OO O O O O O O OO ** == O O O O = .= 0 m O O O O O O O O O tad led .md had led ned and ned ned had nad led emm % tad ted had ned tee had tes 44 @ f%d 30 e . . e e . . e o s e e o e o 63 e == m in M m  % m N w w m #"I m 9 N e e . . DM f%s N  %  % (pg 4N 90 g  % e . . . . e . . . . . . . . . M O 4 e== em p- t== pm tmo to be t== De

                        >e                                                          e         e        .           .      >=.          .      >=.          .          .        .       em. >=. po.                                          >=.
                                                                                                                                                                                                                                                      > .==

e a w e a .a .a s a .4 .a w

                                                                                                                                                                                                                                     .                  e         .

a d a a a .a .d i a o E e .. a. se s aJ M t#3 C M N b

             ~    Y n      b C,., i                      O              - - O O to   O                          e        m o

O O O O OO OO OO OO OO -O -oO OO O- O O - O -O OO O 8 3 H

                             >e
                             ,,3     QE w O ew te             in.       i.s      nas       end         nas nas            las        and       ins       ime        end      nas        ins       nas         ina        ime       w w g                             ==    >O                 .             .         .         .          .         *         *
  • e o e g g t= .a e == w e est set e e y
                                                                                                                                                                                        .         .          .          .          .         .         .         e E     O                  4     39                                                                                         h                    en        fut       f=3       g          m         ao          e ev                 %        %
                                          >=     "1 e%s Q    K                  nn          %

ee e s . e e e e . 4 @ W en* >= >= to >= to De se

                                                                                                                                                                    .        e          .         o          .          .          e         .         .         e O             e             e         e         o          e em        6         >=        ge         em        >=          pm        e-         se       e-o         e         o          e         e         e         o         e          o          e          e         o         e         e
                                                                                &        S         $         &           O        O         O         &          &         4         &         &          &         &           &          &         &        &

t#5 t#3 O as O ee e 8 to == i == to M M

                                                           >              -d
                                                           .ma            4 4               3 O              4
                                                     .. g e                     E tas    w               3
                                                    >=    4               as                                                                                                                                       O W     W               e-                                                                                                                                       e iA                                                            ase las   ==              W                                                                          @

a E sen e e e ins a. e 4 O 2 to S

                                                                                                                                                                                                                   .4 W      W                                                                                                                                                        %

O @ O S O IA

                                                                                                                                                     % m O99 G 48 e >= O                          a==        w e                 CO tad    en   a              pen       O         in in                la
                                                                                                                                                                                    ** m M                         W          W          W         N         N
                                                   >=     O     e              e        9          e e e S                          a=        as        a         a=        s-a        me         ao         ao        N         N e          e         e         e         a          e         e        a.

4 e a e 4 E 4 W D 5 O nad O E E 3 3 14 na 4 s 6 e e O E 48 Ea G nd E bD W N tad had 4 E na. N es a == W W e W W es *= 73 I

   , , _ _ _                     -        -    P                                                                                                                                                                                                                       . - -

3 == == O O 3 3 O O O OO OO O OO OO O == == O O 3 3 === == 3 m 2 3 O O 3 3 3 3 3 3N tad tad tad tad ens tad tas tad ted tad tad tad nad % ed nad ted end tee un M teh n 4

                                                        ==e e

W s e e s e o e o e o s e s e e e o e tre o T T .f G T @ T en T se T W 3 @ W as f') 3 3 tad N *e gg o e o e e e o e o e e o e e

                                         .-e           one               sua        se        >=        se           em        s=

o e e . me e e o em em n= e= em em s= em >= o. > o-e o e e o e e e N s o e e o e o e ed M M ed ed M ed M M M ed ed ed M ed ed $ ed O O ==. =e == O en O O O O O O sO O O s e O O O OO === O O O === O ==O O== c Oo == c a e O 3 XN tad tad ted ned nad led tag tad tad tad tad e tee tad ted tee tad one ed one ene 3 mo.%  % E te, == e e . . . e e * *

  • e e e .-e @ =.e  % e m o N .= e
                                                                                                                                                                                                                      -e          m o            =                     e me                                                                                                                          =e                   N             %         %                                 W           -.e       N ON                  e6 3%                                      e          e         e         e            e         .         e          e           e         o           e            o 1/3                                   @                 >=                   a=        e=                                                                                                      e         e           e            e          o         e M                      .O e==                               om        e=        n=        em           n=        e=         >=            s=        em        em          *=          e=          a=
                                                         .                 e          e         e         e            e         e         e          e           e         o om e            o        e cf3                                   e                 e.a       .4         .a        .e           M                   -d           d                              .a e           e            o          e         e a                             .d        -d                       -s          d         d         .a             d        .a        .a n

M

                    =
  • ee ao M U N u e

C M w 0 H 3 t.) O O w pe d"* M e e O == O O==O OO OO OO OO OO OO OO== O =* O OO OO OO O .-e == N O O O g g N N ned had led ted 1 2. > we W W nad ted tad tad ned les ned tad tad tad tad tad nad nas nas a M rs O ie. %

                    .J g   --     e .O=              e.                  .          e         e         .

M M w s= Oe == g e g m m e

                                                                                                                               .         .          .           .         e           .            e         .         .           .            .           .
  • 3 ( em O
                                                                                           #we                                                   g           en m                 we           m           g        e .=                    #=e         == m 4      w                 a=     Wm                 es a            en     O%
                                       @            e                 >

e se e e e o e e e e e e e e e . . e e

                                                                                           >= >=                  se        em        om        >=                     em                                 *=

N O e e o e e e e e s en= e e s== e em e e om e== se em a= en -s =a .A -e s e o e e d -s d -# -s .a M .a -a .d -a -d a a t/3 t/3 O 5 e ee e n6 a

                                               =*            tA to             >
                                               >              -e ad            4 l

4 3 5 4 eo q e E ten .d 3

                                    *=         4             5                                                                                                                                                     O W         W              s=                                                                                48 9

tas me W =e M E tag e e e

                                     ==#      tas            es                                                                                e                                                                   4 O         2              to                                                                                a                                                                   .3 W         Ad                                                                                                                                                                   %

O %M q W h O =*

  • e e 4 W W S O 4A te e e me m M

' ens == m E N O 4A 4A @ W W N N s= m o E e 9 in e e S se me ese me me ao me == N N e e e e o 4 4 e d tad e e e se e a e a e o a O e a 3 O lad O 3 e 3 3 e 44 44 4 tad tad ( E LS 42 e ad E W tee W N ete e W == W W e W W e *= d i ! 74

i

                                       -           O           - - O O O O O O O -. -= O O O O u          O           O O O O O O O O O O O O O O O                                                                                                                     - o O O                 O
                                       ,          nna          tad       tad       w        ena       w w w                     tad       w         med     tea     tea     ses      med      4.d      w O                                                                                                                                                                         .4        .a
                                       %          ao m             .            .          .        .        .         .       .        .         .        .         .       .       .       .        .

20 eq w =A m n N m e m tA m ua N m e e a m a a m *e q ,e . . . . . . . . . . . . . . . . 3% 3 e= o= em e= >= em e= e- m. a. a= >= N . . . . >=. . e=. . e=. e=. . >=. em O w .d a .,,a a .4 .J n .d a .J .d .J a e .d

                                                                                                                                                                                                                 .4 a                .d O            ==

O O O == O 0 O O O O O O == O O O O O O O O O O O O O O O O O == == c O O O . one w w tad tea w w w e

                                      .e.                                                                            6.d       and                 tas     nas     tea     tad      tas      w        tad       tas         d         -
                                  >%                                                                                                                                                                                                    ch gN             O.              .         .         .       .         .       .        .         .        .

s WO . . . . . . . 4 3s

                                                .=

m w m m e m e m e m e m m e N m N N e EN *e t/) eN . . * * . . . . . . 9 W 9 e= e= e= e a= em em e= e=

                                                                                                                                                                                      .        .         .        .         .          e m                      tas .%.
w. >=. . . e. >=. . . . e. >=. . . . . em.
                                                                                                                                                                                                     #=        s=         >=
                                                                                                                                                                                                                                       ,d p                           O         M               A          a         a    .J           a     .J      .J       .A         .J        w         a     .J      .J         a w a

s a S h t/5 (,) M d 8m8 ge e 3 3

m. . m w w 3
                                                                                                                                                                                                                                  - e-M                          O                                                                                                                                                                                                     a
                                                                                                                                                                                                                                   ==zs o.

C e o i e === a.n.e f,,) ^ a eae w e=e a .== O -. == O O =* O O O O == N O we eee

                       %. tes      e         O                                                                                                                         O == =* ** **                                  O        =e=

O U g e R w O O O O O O O O O O O 4 O O O O O O w

                                                                                                                                                                                                                                  . t. u I  F.           >         5 8".

O t.d had nad tad tne las naf had led ' taf tad ted tap ned tad led tee led tad w** m e=4 .3 y a >% -. w. yd e -. 3e th2 3 5 4O

                                                   .            .         .         .       .         .       .        .         .        .         .       .       .       .        .        .         .        .         .       e at ,a
 ]    44                     O   3e
                                                ==           in        =$      m w                 se       w       P=.      tA        N          m       me      w w             N        se       m e e                          C == C g                  ==  S9              *e                                                                                                                                                                               *9*

e= 4N . . . . . . . . *

  • e 4 3 %
  • e=
                                                                      >=                                    se ee      N             e           .          .

em e to. em. .

                                                                                                                    >=
                                                                                                                       . a=.       to.        en.

en em. e=. e= e= >=

                                                                                                                                                                                                             >=. e=.
                                                                                                                                                                                                                                  .oe 9 es  o w

to a'* w ad -d ed -d .J .J ad ed d .J .J

                                                                                                                                                                  .d      me      ed e

ed e . A .4 -d &W& 9 3 De 3 m D .9 = 9 Nem g N W a=

                                                                                                                                                                                                                                .% o m%

O*C o.O es 3 es 9 N w OOO

                                                                                                                                                                                                                                 %w%

me me m O eO g Ee E

  • o%o
t. O h mTw
                                                         ..                                                                                                                                                                          me
                                            *.         to                                                                                                                                                                       S eS to                                                                                                                                                                                     tp e
  • em "o=

t ey m e.

                                                        >                                                                                                                                                                                  y to.

D .d g, 6 g,

                                          =#           4 4            S                                                                                                                                                                       == o.a=me
                                                                                                                                                                                                                                == gn S           4                                                                                                                                                                          o o
                                     .e   4                                                                                                                                                                                      w as u y

S S tee a S ed S es l ** 4 m O == == W W e= W Ek eb to a=. AoG ted - W S

                                    .d    S            tas                                                                    e                                                  4 e                                             9 84 q     tes          e.                                                                   e                                                                                                    e e G     3            to                                                                   a                                                      d                                                 O W     W
  • e. M w N
                                                                                                                                                                                 %                                               o -s e S                                    e        W 9 O                                                    43                              O =* * ~ to                           G        2 me S ene   a=   m            N         O en              tA        en       t$

4A te G en O e se ao as m m ms.ew se ao w wse N N 0- S e e w e e ao N N e e e e e e se e e e e o e m*=.a.= 4 4 E 4 tad a g O tad O 3 5 3 3 4 e G e 48 e ad W W 4 64 44 had saf 4 E 94W la a ts. N N e a se W u e W u as e- == w 75

O == == c O OO OO OO OO O == O== O O == O .= 3 O O O O O O O w O O O O O O O N tad ned ned ned ned and and tad ned and and

                               %                                                                                                                         had      nas       had       ned         nad      ins       nas      a 4

sgg N. . e . . . . . . . me me w @ M M  % M  % w sn m N w m

                                                                                                                                                                                     =e e m h

SN

                          =S N              *e g                            .       .       .              .       .         .       .        .        .         .          .        .         .         .          .         .         .        .

c ram >= t= p= p= >= > > p= e= >= O . . . . >=. a=. a=. . e e . >=. . . >=. >=. e. . a= M e .a -n d .d .,a .d e a -s os .e .e -e .d .4 .6 -d O == == O O == O ==* O O == == O O == == == N -* O O O O O O O O O O O O O O O O O O O m N ind uma ned nas nas and ned has tad ina nas ins tea

                              %                                                                                                                        nais      ned                            ina      ned       a           d in         @
                          >O                 .             .       .       .              .       .         .       .        .        .         .          .        .        .         .           .         .         .        .

4 e e sen 4 sn sn =e sn no e m S im sn N en e == ee w *= ==

                             ==           es g                     %                           .       .       .              .        .         .       .        .        .         .          .        .        .         .

W w s= e- > t= e- >= o= g C O. e *=. . . s. >=. e e=. e=. e >=. s=. s=. . >=. .

                                                                                                                                                                                                                   >=
                                                                                                                                                                                                                      .      ==.

p en a .d =4 -s -a -a -a d -d d -a s ed a s s e Q n e .. a. e s=8 3 M  % O C M les ' V j , ^ m O -= -e O O O O O O O == -e O O O O O O O O O O O O O O OO O O O O

                *8   ans                O                                                                                                                                                               -o        N
                %. e       en                                                                                                                                                                         O         O O

@ U we E ** tas has had tad las led I 2 >* o 3  % taf tea tad taa tad had les nne tad has ted had and a M 3 a -s e

                         == O          O.                .       .       .              .        .       .         .        .       .         .                   .

I*g N E E e =e w en w m m e m w w n N no w w n a m == m aI O.= e. 4 e. g C E w 4 8"9 w es b= 9* D= De D= [=s 4 e= 0 . . . . De. De. >=. . . em. D= pm. t=

                                                                                                                                                                         >=.

t= tm.

                                                                                                                                                                                                        >=
                                                                                                                                                                                                                  >=. .=.

A m . . . . a a a e a a a a e a a a a a a a a a (A (n O 5 sn sn. eu

          .                      **              W9 6A              >

6 4 4 8

                            .. k               .

tas .e 3 8= 4 m O W t= W end

                                 ==                                                                                     idt                                                       ase las                  W                                                                       9
                           .ms   E              tas                                                                      e                                                        4 e

a ens a. e .a O 2 en S  % W W  % w O w G S O en eft m te O O se M N M O w w e ao e eN e

                                 ==    S             N        O en                                                                                                                                                         N and                                                in             4A      @          W       9        a=       me        M          pe       me        me       me          es.       N         N t-    O      e              a w             e          e            e      e          e       e        e         e       se          e        e         e           a        e
  • 4 4 m 4 and a g O tas O 3 a 3 3 e en en 4 t

O m WW e ad a W te. W me N m a m. W W G tad W ts W 4 m >= 2 76

                                                                                                                                                  --w                        - , - - - - - - - - -

O ~ N O O .e O o O O - -. O O O - -e O N 3 O O 3 O O O O O O O O O 3 O O 3 O O 3 eM tea w w tid had tas tad gas w w had w tas has w w w ,,ma w tad % M SS O

                                         ==

e e e

                                                     * = w w == m e      .        .       .       e       e       e        o      e       e         e        o       e                        e           o       e has e p= M S e e e                          =e     m e at                     -e                  w              -e        e S. O            el tan g                         e      e        e      e        e       e       e       e       e       e       e       e         o       e        e                        .          .        .

tM S S >= 0== t== >* t=s t- De Dam 8= >= em t== >= tem pse se > >= O e e e e e e e o e e o e e o e e o e e w d .4 a a a d .d a -d -a w .A a w a w d .a O =* .=e O O O O O O O =e a O O O = m -e o O O O O O O O O O O O O O O O O O O O m o tea taa ned has tad had had nad had had nad had nad ted ted tad tad had nad amm % 44 9 w 30 e . . e o e o e e e e o e o e . . . e 43 e s.e w tot M M rum M e w w M N m e e me m e a 3m M (N *e

                              %                        e      e       e       e        o       e       e       o       e       e       o       e         e       e U                   e**                    >=     g=      gum     >=      Dum      em      p=      tue     *==     to      >=      to        >= >= >= >=

o e esa o n= e O M. . . e o e e e e m. p e a a a .4 a .a a e .a o a .4 e e a e a e a e a .a e e a e i A U N.e

 -       -   i
   . .. a. N Y

a S O

     "5   -      2*

s O O O O O e 330 O3333 O O O O O O O O O

                                                                                                                                                                                                         .e O O O

W N tad w nas nas w 8 U a nas ned tad taa nas tas saa had has les ned w tad las m M >J

             >    3,  O      ,%,,      ,

v == p= WO e e e e e e . e e e e e e e M =d e ** w aft M e S e Pan W tS M M M w s=e e e

                                                                                                                                                                      ** m e S o             e        e
 ,,J nd               4  3e g3          >- as N           ee vi     %                        .      .       .       .        .       .       .       .       .       .       .       .         .       .        .                     .             e        e p                           na        eme         gum    go      p.      pm              go                       g-     p.       g       g.      an.       g        p.            p.                   p.

go. go. go. we d o e e . . e . . . . . * . . e e 48I .md .u0 .md ed .u0 .m0 ed and .ma .m0 ed .md ed .sd .m0 .md .mf .me U. tA in O 5 1 et ee en

        ,                         en          me
                                   =*         tM en           De 3*          -d
                                   =d          4 4           8 e    k           .

tan .d 2 O

                            *=     4          m                                                                                                             w W     bp          >*                                                          til                                               es nas   ==          W                                                           S                                                   e ed    O           te#                                                           9                                               4
                            .nl   tee         b                                                           8                                                 .a G      2          to                                                          S                                                 %
                            %#    tap O                              W
                                                                                                          *== M           q@              w       e**       O        a=*        w                       e         50 G S O                   eft     tit     O e              me     M       M         W        e w                                N         N tae    ==   G          pm      O      eft      tA     aft      te      @       S       se      e.e      M      ese     sme       one      s=*       ==                       N         N 0-    S     e           e     W        e       e       e        a       e       a       e       e      me       e         e       e        e               e                  e         e 4     4    4          tas      0     g O             lad      O       3 5             3       3         0     44      44        4        had        tad                     EC        Z S     S    W      44  G       bd     E        W      te.      W       N       N 5             m == W W                          G        W          W                       5
  • e 77

O O O O O O m 3 3 3 O O 3 3 O O O O 3 3 3N nad med had had tad ted ad w ted W tad % and had tad tea w tad med =e .4 3N hfI g ,,,, . . . . . . . e . . . . . w e, = . . . W afe e e m w a m a w nie w N w w e .= w -.

  • nad W *#

3 .g =e >= e-e-

                                                                                                            >=

p=

                                                                                       >=.                                                                     e.         a=       a=                  a=         em          o=
                                                        .              .        .                   .          .      m. >=.                   n     e=.          .          .        .      e=.           .          .           .      .=. ==.

M M and .M .d M e .$ M -d M -d M -d M d M d O O == ==s O O -. OO O O O O O O O O O O- . = = == ** === O O -. O to e e O O O O O O O 3 O O O EN a e tad ted ted tad nad tad tad nad hee % had had tad tad ted nad had had had tad tee G.=.= e 3 . . . . . . . h.o e m . N m e e e N e N De e=e - ON 40 3% . . . . . . . . . . C#I 9 >= en em e.= em >= e= e== e= a= >= se bl .O. - * * * * *

  • em >= a= > s= ==

cf3 A e .a s =a e

                                                                                                                                                                                                         .          .           =         .            .
                                                                                                                               .d
              >                                                                                                        A                     a         e      .d        .d        -d          d          s       .d            d       .a            M e
n. .. a. oe e ab C

Y M C ($5 Pe i.e d 3 R R O g

                       .=. e      .

O a. O O

                                                                           ~

8OO O O O O O O O O O O O O O O O O - O O - - ~ - N tad had nad nas

                       %.,.e E   m%                                                            ned       had       ned        nad       tad        nad      t.e        ned       nad      ned       ned        tad         ned        tad          ned 8             >*        O M  M           e3        === tad O.

e to V sie Oe = g N  %  %

                                                                                                                                                                                                    =,.           .           .          .

W 4 >= O N m N g g seg  %  % N  % N y e.d om W #=e ge a en O% 9 a= em om >= a= N 0 O. >=. . om. em. s.=. e== em e.=. s=. o a= no a= e d .d .d -d .d

                                                                                                                             .4
                                                                                                                                .          .         .                    .        .                   .          .           .      a=.              .

e .d .d e .4 .d =s .d d .4 .d d t/5 1 t/s O 5

                                             ..            e 44             ==
           ,                                =              e in             D=

De me e.d 4 eg S a 4

                                     .. g e                      I tas     -d             3 a=       4             a                                                                                                                                        O W      W              >=                                                                                                                                       w
                                           ==                                                                                         td'b                                                         as tas                    LJ
                                    .d      E             tas S                                                             e as                    a.                                                                            e                                                          4 O

nas 3 e e e W 3  % tes  % q 4 w O 9 8"o w N O .* w d ep O ede tA O =e tad

                                   >=
                                           .G.

O m 3 5 me O een en en e e e .O =e .s'.s .M. w w w N N N N 4 4 5 e 4 e e e o e o e e .m e mo e e e e e e had e WO ned O 3 m 3 3 e a 48 la e ad E W te. W N N es a .e. en U W e M 4 tad W ned W 4 m >= 2 1 I t 78 1

TABLE R-5 (Cont.) ~ DRINKING liATER: GROSS BETA AND CApetA ISOTOPIC ANALYSES ON MOlmlLY COMPOSITES (pct /1) stall 04 NUNGER - SWP-7 JANUARV FEtauAAV SATE COLLECTES: MARCN 12/24-01/22 01/22 02/18 02/IS-03/10 RASIOCNENICAL ASAlv5I5: GR-S 5.2 a 1.1 E 00 6.7 e 1.3 E 00 8.1 1 1.3 E 00 SANNA SPECTEUN ANAL V515: SE 7 4. E 01 L.T. L.T. 4. E 01 L.T. 3. E 01 E-40 L.T. 6. f G1 L.1. 5. E 01 L.T. 4. E 01 me-54 L.T. 3. E 00 L.T. 4. E 00 L.T. 3. E 00 CO-53 L.I. 4. E 00 L.T. 4. E 00 L.T. 3. E 00 FE-59 L.I. 9. E 00 L.T. 7. E 00 L.I. 6. E 00 CO-60 4. E 04 L.T. L.1 4 E 00 L.T. 3. E 00 Zu-65 L.I. 7. E 00 L.T. 8. E 00 L.T. 6. E 00 ZR-95/48-95 L.T. 4. E 00 L.T. 4. E 00 L.I. 3. E 00 au-103 L.T. 5. E 00 5. L.I. E 00 L.T. 3. E 00 AU-106 L.I. 3. E 01 L.T. 3. E 01 L.I. 2. E 01 I-131 L .1. 3. E 01 L.T. 1. E 01 L.T. 5. E 00 C5-134 L.T. 4. E 80 L.T. 4. E 00 L.I. 3. E 00 C5-137 L.T. 4. E 00 L.T. 4. E 00 L.I. 3. E 00 SA-140/LA-140 L.I. 1. E 01 L.T. 3. E 00 L.T. 4. E 00 CE-141 1. E 01 L.T. L.T. 8. E 00 L.I. 6. E 00 ,CE-144 L.1. 3. E 01 L.1. 3. t 01 L.T. 2. E 01 RA-226 L.T. 1. E 02 8, L.T. t 01 L.T. 7 E 01 1H-228 L.I. 9. E 00 L.T. 7 E 00 L.I. 6. [ 00

w

                                                                               . . . .                                                                      .                                                                . =

gg tad had .nd had led nad nad ted tad nad nad les ned has tad led ind .ad

                                                       %                                                                                                                                                                                  ed N.

U. S, - w t,.. . e e ~ e

                                              .~                                                                                         w w e ~ e                                               e                  e                     ~
                                              ' "g
  • ed, .. - - - - -

9 a .4 .d a a d .d .d .A .d . m

                                                                                                                               .       3                   . . . . . . . . .

N tad ned nad had had tee ted had nad had med tad tad nad led ted had

                                                       %                                                                                                                                                                    t.d         ned
                                              .t.,,               .

se e w e e e

                                                                                                                                       ,.         w e e e
                                                                                                                                                                                                                  ~

E .=A. *e M  % . . . . . . . . . . . . . M w N - - -. - - - - -

                         ,m                            .                        .      .       .        .        .        .               .          .       .        .          .        .       .        .          .        .           .
                                                                                            ..                .d               .a      .A                                     .d      .e                s         .d        .d          .d b

4 U N s

        *          .. As  w           :

ad 3 i M e a ss- -  ; - - e

                                      - .te,         .
                                                                             . .           88                          8888                               .       88                          8.-.     . .

S E ' ' ' - M 3 OQ. a -a ,% N In3 F, V -. . . . . . . . . . . . . . . ee e en e w a w N e en e a w w m m e a m .e 6e  %  % g - 4- m 9  % . . . . . . . . . . M 8"I $1* 9 . $8 $1. $1 - 9 e-69

                                                     .          I'.I           .      .                .        .      De.       e    $m.           . De.      9e.       De.
                                                                                                                                                                                     $2      $*

9e

                                                                                                                                                                                                          .      em.

om e in -d .d a

                                                                                           .A                .a        .J     .a         a       .4       .d      .4         .a      .4       .a       .4            s       d            e u
31 h.

M t#3 O b

                                                            ..          apt 44 e                                  a            to t#9           >

S E ta .d S . a.d 4 e u u e= en w m. te# .* u 9 a E tee e W 4

                                                       #   ete          &                                                             e E            en                                                            a                                                      %

e u u  % q w . ae a e W 9 . In en e. e me h e e a.w w** e a's * .N e N e w. en en en . tad -= G h WS p. ao M a* a N N s= . e e e e e e e e.e e e

  • 4 e

4 a e WW tes e W .e tad .e 3 e 23 1" s 69 to 4 4 e tad e tad 4 t e as E u te. u N N as a == u u e w u as o= e 80

O O - O - O OO OO OO OO OO OO OO -O - O O O O

                                                                                                                                                                                                       = O O                                       _. 2 O                                                                                                                                                                            O O O O                                      Q asm                  had             ***       **8        ins        had          a        **8        ta8       tad         had     taa         tae ted%                                                                                                                                                       *=d         4.d       ens         and        tas        tad         .a
                                                   ~

10Q . t e t

                                                   -                                     .e                                                               4,6      e 4,9
                                                                                                                                                                                                                .e
                               . O 4.,                                      .         .          .          .           .         .         .          .

m.% - - - - - - - - - - - . . . . . . . . . . O N. . . . . . . . . .

                                                   .                                               .d                     .d                   -,
                                                                                                                                                         .d                  .d                     a a                   .d                     .d O                                    O O                              . O O O O               O O O O                                                                                                               O O                                                     ~

m O O O O O O O O O O O O O O O tad had nad tad ted led tee

                             -~                                                                                                    tai       had        tee      had        ted        led         tee        had        ted        t.d         ted        tad m.O.                    .
                                                                  ,,.9         .
4. O ~ ,,.9 6,.9 h,.t ~

O f=t -

                             <~.                  .e m                                                     -

M Q t m e .d

                                                                                          .,      .d
            >.                                                                         _                     .d                   .e         a                             _.                     _. a                                         _.         a
 -         o.d e

13, e .. a, m u C O. F m 7 e, d 8 E O

                     - .         n O              O O 8OO -                  O          88O O8-                                  O         O           8OO                   O O O O O
                                                                                                                                                                                                                        - - ~
                    ""%.         N              tad             has        tad       les        tad         tad i                 e$   5       %                                                                                     had       tai        tas       tad      les        tad         had        tee        tad         had        nad        nad        tad E    8"4                O       h              eft a.3       == >O                                     e                    .          .                     .

y >= me # m.e . . . . . . . aft P.e W eft eft G . e-e 4 Se tit Pan T T 4ft T s T = a

                         >= "t N m              e       s                                 .                   .          .            .         .

e w . . . . . . . .

                                                                                    ==. -. - e- -.

e . . . . O . e. e- - - p. a. - >- >- 4

                                                                             .                                                     e          e      o.          e          .           .           .         e a a e a e a a e a a e a e a a a                                                                                                                           .          .

a a tn tn O 5

                                                           .o
                                           .e             ntt q                ==
           .                             .#9=             t#t M                >
                                         >                .d
                                         .d               e4 4                5 S                et
                                **      4 e                           5                                                                                                                                                                                                       i 4*e       .s                2 t=        at               as                                                                                                                                               O 4.5       bd               me tad       ==

W til

                                                                                                                                         .                                                                .e                                                      i
                              .e        E                ime e

e

                              .d        too              e.                                                                              e                                                                as                                                      '

O a e a a W  % m  %

                                                                                                                                                                                    , m O                                        , e a                            i g

4 W O . 4g3 O eft til @ tas == on. O ngt tgt g g . .O. 9 N N s= S 9 .M. .Me .T N N 4 4 4 48 0 ans e WO e a e o e e t m.

                                                                                                                                                                        .            e          e          e           e          e          e          #

S es O O e ned O 3 et 3 3 e M t#9 4 tee tes eg 2 e ad E W te. W N N e S .* W W G W W at P= t 81

s a .= o e o o o e o o o o 3 3 3 O o 4 3N M tad med tad tad O O . O O O O O 3 o o Q o o o had had tas tad tad ned nas one had sad taf % had .a tad had u.s 8~ 6.,., W idt

                                                                                                                        . ~                        en g~                      ~
                                                         ~                ,
                                                                                .d                -                 a          .J
                                                                                                                                                   .d        .d      .4                a      .d                   -        .4       .d
                                  . in N tad ted      tad nad      had nad tad        tad       had       led 3 . .. . . . . .

ted tad nad and tad

                                                                                                                                                                                                         ....o had       end      had      ted ted .%.               ~

3 .

                                  ..                                                                                          ~                  ~ ~ ~ ~                                                -                          _..

rA ON *e g . . . . . . . . m a.% om - >= t=

          >                           -                 nn.             .        .      e.          .      >=. >=.               .

t-

                                                                                                                                           . e=. >=.              . a=. >=.

t=

                                                                                                                                                                                                        >=

ma

                                                                                                                                                                                                                          >=       e-nn                    .d        .d       .J                a                                 e              .d                .d
                                                                                                                                                                                             .A         .d        .d      .A       _d v

E

n. .. a.

s

             ~

a

      *g g            ~

3 8 4 en I - OE s o

                                                                     . . . .                              8                  888..8                                                         8-..o      .

4 l * . . .

             $se a          a   om .=           .N   %

tae nn nas nad tad had ted tes nas tad ned nas tad tas tad has nad nad tad tes

                 ,.,. .=

med

      -               .          -                                                                                           ~                  tA        -                                 ~                   -

M O - g M.s A 3 e u. %m

  @g     .g g                                         ..           pu.               e        p                  p-        se        en        n-        e.       se      p.

p.

                                                                                                                                                                                            >=
                                     .S                                      se.         .        .       De.       .          .         .         .         .
p. s= e. o.

g to .a .d .a .J -d e .d .a a a .4 a e .d a .d .d d tn t/s O 5

                            .\

l e.*

         ,                                        .th 44           en.

3

                                                  >            _d
                                                  .d           4 4            8 8            4
                                       .          g too 3
                                                  .d           3 pm            (           g                                                                                                                            .

ay u u e= tad == u t.a

                                    .4            3           tad 4

e s tes a. .a E en . .d t.d u  % 8 9 t$ . . .N

                                                 .                                   4F       . . .                        tA                                     .*

M. a e N tes == . M. . tA en en te tG t.e M s.t

                                                                                                                                                                          .e       .M       .e      .r.                 N
                                   >=            .                  0       49        e                   e                  e                  e                 as
                                                                                                                                                                                                      .        m.                N 4             4    .e           had       0       3        .e        ind      .e        W         .e        3         3 e

e e to e 4 e e e e 4 e 2 e as ta to . Ad E u te. W *=e N == U W . nad WW had

                                                                                                                                                                                                                                   =

1 82

I M + tad 76 a= m O =* O == 0 O O O O O O ae me O O3 O OO OO == 3 ON O O O O O O O O O O O O O 3 q% tas ted tas ins tad med med ens ned nas tes ted tea tad w SN and tad ena ed On,e O e o e e e e . . . e o e e e e . EO N ** "" ** *"* M ** N N N '"* N =* "o N * # M mo m N g: . . . e . . . . . . . . e e e . . g e

                                                                     -e - e - - -e - - - -e e                    o        e                   e          .          .

e e o e e *

  • e
                                                      .d             and       ed       .e         .J         .J        .d       ed         .J         ed        ad         ed        .J          ed       .J         .J          .J       ed         ed 4

m m me == =e ind e e O O O O O O O O OO O OO 9O O O O== 9 @ OO O OOO O O O ao C e- m e O e% tad med had ens tad tad med tad had tes tad tad tas had nad W 49 had tas tad 3@ O Oe e e e o e e e e e e e e o e e e e e e e ON N == -e a we m == N me N e N ** ae @ M e N N

5. g  % e e e e e o e e o e o e e e e e e EO e= e= >= a= >= e= e. e. s= em >= >= e=

e . e= e o e >=. e=. e e m=. . De. . . e e o em e e e a= a e a a a e e e a e a a e a e e a e a e b M e-4 Ca3 I/3 0 Q eJ'4 b o-d Cae x m == o O O O O O O .e Q O O O O O O O O O c e O OO OO O OO == m .e -e O O ee a gjy

                                     -e                            w O O mN in,s i.e      tad        med        tad       tas      w          tad        w         ts         ime        ins        tad        w tea               w w w m          N C/I            4%             O
   @     H    l-e e  3                e              o         e         e          e          e        o                   e          e
                     >e          g3  g              u              u                                                          ,e                                  e         e          e          e                   e           e e                mJ    m     3          e
                                                                            ,a       u u e m                                             m m g                           m u                   g         ,,o       g w                   ,e        ,e M                       s-e   O   Ge S ee             o              e         e        o          e          o         e         e         e          o          e         e          e gn3                     %,,,g  e  O%            a=              a=                                                                                                                             o         e         e           o         e         e em                  em         a=        >=       e=         e.         >                    e.

g um e . . s=. . e e e e o

e. >= em >= e. e= a= ==

g ,,, g g g nad O ed .a .d .A -d .a .d =d -d .d .a e

                                                                                                                                                                         .J e
                                                                                                                                                                                    .d e
                                                                                                                                                                                               .d e
                                                                                                                                                                                                         .4 e
                                                                                                                                                                                                                   .d e
                                                                                                                                                                                                                              =a e
                                                                                                                                                                                                                                         -s e         e hd   Q      e-4   V                                                                                                                                                                                                                          d 2           b           ==

M f4 O 4 cm e=e Fe >- Q tt3 Q 'n

             >*      In eJ      M m              ao       ae O O O O O O O E

en# 9

                                    *=a=

O O O O O O O O O O O O O OOq O q O O O O e .* O O O tas tad tas nas tad tea tad tad tad V, % ted tas had one les tad tad ned tes tad e.e 4m O p g CO e . . e * * *

  • e .

g Oe N == N as se N we m eo se

                                                                                                                                                      .                    .          .          .         e         e          e          e         e e                                                                                                                  amo       en          me        se         N         seg       me         mm e= N en %             e              o         e        e          e          e         e        e          e          e         o          e         e           e         e WN            e=              se      em        em        a=          >= -               em        em         en         e=

o e e e

                                    .e en            e              e         e        e          o          e         e        e          e          e         o De e
                                                                                                                                                                                   >= >=                e==       em        em         he        ==

ed e o e e e o e it. =d =# .d .d =a .J -d .d -d .4 =a .4 .d =s .d .a .a .a

  • se en aus en
                                                             .d 4

es 3 M 4 es e= e en E

                                         '.e  >              3 em   a             e                                                                                                                                           O u    4             e=                                                                         4A e

me ens

                                         .e W

4 u e e toe e. e 4 O a E en e d u 3 a  %

                                              ==            4                       e O                  S
                                                                                                                                       % m e                                      w          h          O == w                         @         e O in to O O                                        se         m          M          w w w                          N         N tad e=

De

                                              ==  M         3 a

h e e O en e 4A e en @ @ S s=e e-o m see se se ao se N N e e e e e e me e e a 4 m e e nos a WG tes O 5 W 3 3 M M e a e e O >= EW e ad E u e 4 tee naa 4 E te. W N N g g == u u e y u er s= l 83

                                                                                                                                                                                                                                                                            ]

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ad M M ed M M e.d M M ed M M ed ed mid ed M d (4 M to tJ3 M ^ > H ad w in to e C af w p Q 3 V V N A " 4 O M e h 3 H  % b 94 3 .* N O O e O O - O O e == N I M o >3 u O e O O O O O O O O O O O O O O O O O O e o,q F.e m. - N tad is.s w i.e w M A: o g v >=4 us a i.d med n.d i.e w w sad and i.e w t.d d led O g E > em D N ' E to oe e N N C4 Q -O N N N N e e e m N N N N N

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O e e * . e e e e e e e e e e e e . .

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                                *=        0  e       e    e    e    e       e    e    e     e  se     e    e      e     e      e    o    e 4   4   ted     e  E    O    taa   O      3     m 3       3      e  to to 4          tea     tad  4     E t

O M e M S u w U N N e m = U u e u u,s > 1 ! 96 \ t

ae == 3 O 3 O O 3 3 == ao gN M O O 3 o tad ted tad W O 3 O O O O O OO OO =*O OO==O==O 0o ad ted ins ned tee tad had ned nad tad tad % ned ned ned tes e goo S f.% e o e . . . e e e 6.s e w 4A w w e M N e nn M

                                                                                                                                                                  .           .           .           e           .           e            .          .

4dtA == w w == m M e a tad N O% e e o e o e e e a e o se > >= e a e o e t- >= >= se >= e- >= e- >= p= o e ao e o e e a e e e e e o e e-o

                                                                                                                                                                                                 >=  e
                                                                                                                                                                                                            >= > ==                              to
                                                   &          SO         &                                                                                                                                        o           e            a          e
                                                                                   .ad        an$       me         &          &           mid       &         ed          &           ed          S            ed         S           .O          ed
                                                 =*         s==        ame        O         O         me O                                                                O O O O                                    se         me          eo          se           O           O          we           3 nn                        O O O O O O O O O O O o                               e O O                      O           O          O            O WN                  tad        ted        tad       ted        had       tad        had        had e           e tea %                                                                                                      nad       tad       had         tad         led         tad          nad        nad         teJ         tad S ==

3e o e . . . e a e e o e e e e tas e am e

                                                           == e ==                          M         e5         N == N                           N         N           N           O ==                     M w

e == CN m% e o e o e e o e e e e O e o e o

                                                 >=        t==        e==        0==        >=        D==        0=         p=         >=         0=

e e e an o e e e e e e to >= Be p= a= >= >= s= o e o e e o e ed M o e o e

                                                                      .m$        M          ed        M          eIS        M          ed         ed        M           ed         M            M           .md         ed         .u$          end tO s=4  to

^ (A M e

           >e   N M        N 66   es        tn         e C   M      x            e.

Q M M 3 Q ~ N ***% M

                   ~

N 5 b"

                                                ==        -e
  • 3 O O O O O O O -e m

I M U O Fe N 3 O O-Ch. e N O w O O O O O O O O O O ==OQ O O O -= ~ == O O O O O O

    <     c        w em     m%

te.s 4.s 6.a w w tea w w w w w w w w w w M bl (4 4 t.a a g g e- eo.O tad e o e . . e e . e

                        &#1 Oe                  T        @           M         8"3         m         W         N e         .           e           .           .            .          e           e           .
                            *= O                                                                                          T           en         M         as         g           W           N           me          M          e            CO um O%                    e          e          o         e          e I                S              0=        t==        >=         De         t==

o

                                                                                                               >=

e e se e e e o e o e e o e Q O e o e e o 0== e e 0== e e t= e D= e De 9= >= B== t= p= e=

                                               .a                                                                                                                        o           e          e            e           o          e
                                                         .d             a      ed            #      .d         .J         =a          .4 e
                                                                                                                                                 .4          e           a        =a          a           ed            d           e           d e

es l#.9 mm M w 4 l S ' 4 O E tan 3

                              >=       5                                                                                                                                                    O W        >                                                                                 eft 9

tad 4.d ce d had S e

                              .e       e.                                                                                e e

( O M E .a W  % M 4 9 tG 9 N O == W @ W O e S O 4A tA O O eme M M W W W Red pe 3 P% 4A 4A 4A @ W 9 emo see M e=e me me N N E 8 @ e e e e a e e B se sue em N N 4 4 tee e W O tad u a 5 3 3 e e o e e e e O W G e M 4#9 4 tad tad 4 1 nd E W te. W N N S S =* u W G W W W >= 97

m .= == 3 M C O A t"4 I"t == .= == 3 C O 3 == 3 a.a i o O O t) O O U O 3 O (J 3 0 3 3 3 3 3 3 a= M gN i.4 a n.a e.a n.a ina w a and ina ea i.4 n.4 ia i.a w a a w 4% 2N g O. . . . . . . . . . . . . . . . . . . e N == == == .e est -e N N N -e N .me == N w a m N Eo mM gg . . . . . . . . . . . . . . . . . . .

                      $p                     e=    e=    em        em. e-         >=              em            e-               e     ==           .= .=

qq >=. . . e e=. . . >=. . a=. . e. . e >=. . . >=. . . in. J .a a a a a a a .a a w .a a .a .4 a .a a E m == == ** o O O O O O o -. O O O O O == c tas O o O O O o o O o o e o O O O O O O O Q

                      >- m                                 e u%           w        naa    w w w w               i.a  6.a   s.s   ia       64   i.a      w          ina   w w            a   i.a     w 4e 30 O.

a,e N .= e .= m

                                                                         -    N N

e N e .

                                                                                                                 -. .= e m ao N

N ON 5%

                      -e              .        .      .     .    .    .    .     .     .      .      .     .            .      .      .    .     .       .     .

s= e0 2 e=. a e. a

                                                   ==.

a w

                                                              .a m-
                                                                   .4
                                                                      . e=.
                                                                         .a
                                                                              >=
                                                                              .4 om a

a

                                                                                               . o=. e=.

a .4 e=

                                                                                                                  .a om
                                                                                                                             .d
                                                                                                                               .  >=.

a

e. . >.
                                                                                                                                         .4       a
                                                                                                                                                     .=

W U3 H M M W V3 H O 3

      %  ee f                            m O  2        N m
                                            .= .=. o O             O     O O        O     O == =* O O == O ==                                                c Q          e              O        O      O o o o o e o o e o o o o o O O o H           8
  • a g5 2 e= , w inn ina i.e w i.s i.e w w w w w w 6.a w i.s w w m.
  **              m   mN 4%

M U3 e 34 O. . . . . . . . . . . . . . . . . . . E M N >' @o N N ial N N e N w M M N M N N ame e N w eg. 8 H M m a e a < < M i.e e m s .e 3  %,,

  • O%

e= e= e= e= a= s=

                                                                                                                                                             ==

W .,.4 5 um s=. e=. e=. e=. e=. e=. a=. a=. e=. e=. a=. >=. a g g g g g E O .a a ma =a J .ma .a .a a a ad ama uma .4 .ma .a -s

                                                                                                                                                     .4      a 4  4   Q  M   V    a H  %      %

af. U3 O o. m M H e= 4 U2 03 O '" ~

      >e U2
  • A m .= == c o o e o o O == 0 o o O O -. -= O 4 m O o o o o o e o o e Q o O O O O O O 3 we E *===

5% i.e i.s 6.a i.e saa nas i.a ina i.e ina i.e i.e is i.a i.e i.a s.4 a m 4m N p g 30 o. . . . . . . . . . . . . . . . . . g Oe N ==e N ce me N se M ee -e .e its emo se N m me m ee w h= N N% . . . . . . . . . . . . . . . . . . . N e- sm= > em. e= em >= >. a= >= > 5 me

                      .m              .     >=.       . e=. e=. e=. a=. e.            . e=.        .     .            .      .     .     .     .       .   .=.

i .ima .ma .ma .ma sma e.a w .a .ma .ma a .ma a .d .a w .m. .na mb 1 i 1 I N.= 0 Q

s. j
                                        .a                                                                                                                        1 4
                                ..      3 N        4 N.

i.e D 3 O

                          >             3                                                                                         e 4    4        em                                          ist                                           .mo i3e  M                                                    @                                                s
                          .*   4        u.e i                                             e                                           4 a          e.                                          e                                                 a o    E        w's                                          a                                            %

u 3  % M w w N O == w e a3

                                =                        w e        S    e     ide  ist    e oo=         se                 M      e     W     e      N       N a se            N      O    idt  oft  iat   e     @    m      se            M        M.e a          se   a=     == ===       N o=   ==  M           e    e      e    e     e    e     e    e      e       e   e=            e      e      o     e     o       e    N.

W M e 4 e.a e 3 o i.a O E a 3 3 e w's are 4 i.a i.e 4 Z e e= 2 48 e ad S tua is. u N N N S == 4.3 U S U u E e= l

                                                                                                                                           .                      l l

l l 98 i l l l l

I

                                 .as w                m             ==

o o o o o o o o

                                 == m aN 4%

o o o o o o o o o o o o oo o o o o o o o o o oo , i.4 and i.a e i.a i.4 t.d w a M ina una ina n.a a oN a e . ano o. e . . . . . . . . . . . . . . gg N ame =e se a f. se .ig a.e me Ji N a =e g e- m N gug N .g as % og . . . . . . . . . . . . . . . . . . e- . e- e- o= p- n=

                                 .o g                .            .                          e.

p- s= p- e-

                                                                                                                                                                   =.

e= e. p- e- =.

                                                  .e
                                                                           .         .                     .         .           .         .         .       .                    .                     .         .          .       ==.

a a e a a .,a .a s .a -o .4 a a a .a .,a a s er M e -e o o o o o e o -. o o o o =. o o o o o oo

                                                                                                                                                                  =e we e- m o            o o o                         o o o o o o o o o                                                                                                                       =e a%                i.e          i.a      i.a       ns         ie         i.e       n.a       ina         n.s       ina      w ia                   a       n.a          a       sea
  • si a a oo o.
                               &a                                .        .         .           .         .         .           .         .         .       .        .           .          .          .         .         .          .
  • N N w N N w == vet N N == N N N e w .* m m oN
                               .m e                 .            .        .         .          .          .         .          .          .         .       .        .           .          .         .

r,f3 zo e. e- e e-

  • g g - e. =. . . e. e. e. =. e. =. o. . ==. . .. i. ..

g gg M s .a a a a a a a a s s s a a a .a .* .* ea M r.r3 Id e2 o. n M h.

m. >*
  • m o =* o eo oe o o o o oo oe oo=*e == o oo o e

a.: g-o as W 4 c6 W M M r./3 e i.e 2 a.s ia

                              == w o

n.a e o *e oo -o o o -o o i.a i.a is ins ina i.e n.a e.a w O te H >* in 88 N i.e i.e i.a i.a i.4 ina i.e y 4 ,,,1 m 4% g g e og o. . . . . . . . . . . . . . g ,,,, Oo N N es N N inn N m N M e m i get

    =

u B <

  • O e i.e o.

m .- . N N e in == m m g<a. E O & E o% m- > p. p-g C M V o m . o. e. o. . . e-

                                                                                                                  .                                              e.         e.         o.

e

                                                                                                                                                                                                             ==.

a ag L a .u.e o a a .,a .,a .,a .a a a

                                                                                                                                      .,a      .a
                                                                                                                                                        .a a        .a m

4 D M M N g g o a a a a a .* H M Q -

          >*  va         e-J N          4 e-wt M

o

                                                            =e                 o o o o o o o                                                                     =e        o o o o                                    -n          == c
                             .e.r w e* o o o o                         o o o o o o o o o                                                                            o o o o o                                             o O                                nos          n.a       ia       i.e        i.e       ia         and       i.e         ia        n.a        a ina            n.a         ses E%                                                                                                                                                                  i.4        i.e       i.a         sea         n.a be  z              4m M

p f oo o. e . e . . . e . . . e

                             @e                N            ego its           N N                              ey        g                     e,       ey N              ey g
                                                                                                                                                                                                              .         .           .             e e                                                               ist                              e s                                               N                    in        - m                     m e- N e4 %                 .            .        .         .          .          .         .         .           .         .       .        .          .           e         .         .                     .             .

N De e es. e- p- >=

                             .E. s m

M

                                                            .a
                                                               . e.
                                                                     =a e.

M e=. M .a M e e. M e. M e. M e. ma M

                                                                                                                                                                   .          .        e.
                                                                                                                                                                                       .a
e. >=. e.
                                                                                                                                                                                                            .a
                                                                                                                                                                                                                                  ..          e=
                                                                                                                                                                           .ma                   .ma                  ma          .us         ea 60
                                                       ==

Y

                                                       .a 4
                                            ..         3 4
                                    .. i.n.

i > o o e.ns

                                     *     .a          S                                                                                                                                        w W       4            >=                                                                           ide i.e     a            W                                                                            m ame e

a 4 a.4 e 4 M a. e o E e m  % a w  % m e o == wg e Ne

                                          .o                                                                                                  g isg N

g g 3 o ial ggt e m g g N i.e e-e= N o oft idt is" iG @ m =e det =e .m.e a=. == == N N

                                          ==   M                     e          e          e         e          e         e           e        e        e .=.               e           e         e         e         e           e            e 4       e     e      4   i.ee       e                  o                    o E                   m o o                        e        VI          M         4 aa                   a         4          2 o       e=   E       48  S         ad                  W         i.na
i. W *is N m a a. W u a w *W at s=

99

1 J l

                                                                                                                                                                                                                                                                               )

U ed M )

                                    ==M             Q                  ==

O O == c 3 O == 0 O O O -. o C O 3 o =.e 3 I 3N (% tea w sad O O 3 O o O o o O O o o o o o o ned had e 3N had had ted tas sad w w .ma med w w w w .d

                                    @.e e          C.                    .           .                      .            .           .            .

EO N =* "" a == N

  • N ==

e=m N EO N == -e a m a N N 6 ,% 3 . . . . . . . . OO 8.* ** e= e. >= e= >. e= m.

                                                                                                                                                                                >=

e= g

                                                   .4
                                                       .                 .          .           .           .           .       e.               .           .          .          .           .        e=. e.               >=. e.                 >=. .=.

e= d a d .4 w a a .a -d .4 .a d =a -d

                                                                                                                                                                                                                                         -d            A        .J        -d 28             M had C e- m 3                 ==

O 3==O OO OOO OO OO OO O O O O == O O0 OO O O OO oO == o o c ww w w ina w w w w w w w w we tad iaa w w sad had 44 ind 30 2e O. . . . . . . . e N == .= == == m == N ON us

                                                                                                                                                       == == m == == == e N nn                                                                               N          N t/s                  xO             .-                  = =

m. gaJ t/3 om

  • e e >. > >= e= N o e= e= >- e= om em e=

p gag a a -d d w ist e e .d d .a -d -d -d .4 -d d -a a -s -d C/3 Em O >J A w

    *       >     8 ad                        N                    m
        ..  =2    t/3                                             ==                     O O O O U

e Q g m H og W H e-a t/3 a in e e, a w

                                 == =

WN o w o wawo 6.A w w w o o o oO Oow Owow==o==o OowOo and had O O O ooooo w w w w w w O w d ad ,H.3 m <% g g ;g s e De O. . . . . . g @@ N N N == =e m .e O E m N N a.e N == N m m N m N so U Og 4 E U cd. w*M O" %' e= saa fa O w w 5 um e=. e= e=. s=. >=. e. om e= J M b 2 ted O

                                                  .                            .                                                        >=. e=.                    .        a=. e=.                    .       em. e=. e=.

em

                                                                                                                                                                                                                                                           >=.

om so m t/3 0 ** a ad A d d ed d ed -d a -d .A .J d d d 4 t/3 w H a a d ad H m

  • H A

8 _ 4 < k x M g g m we O == O O == O OOO O O O O O O O - O O O O O O O O O O O O O O O O O.=

                                                                                                                                                                                                                                               =e                  O p     g             >"=.8           had              tad         tad         nad        had         had         had         tad          led         tad        4.d M                                                                                                                                                                          ted         tad         ted        ted        had                   led Of.

M em nad had 4 DO O. H @e N

                                                                == N W                                                  == .= m == m == N ==                                                                           ide                     N          m m == w m
                               >= N tA %              e                 e          e           e          .            .          .

EN . e e . . . e o= . . . e . amm -e e=. . e=. e=. >=. >=. a=. e=. e=. ==. e=. em e em s= >. om te. =d .d A -J ed ad d a .d

                                                                                                                                                                                         .           .          .        >=. >=.                 .           .         .

a ed a -d -d ad e e.a .J e d .M

                                                           =

to 4

                                           ..             a 4
                                   .. to.

O to E tad > D

                                  >=      .d             S                                                                                                                                                              O u       4              em tad     S              U                                                                                         tdl m                                                                   .T 4              tad e

e

                                  .a                     e.                                                                                        e                                                                    W O       E              to E                                                                    a W       3                                                                                                                                                                            %
                                                                                                                                                   %           M          te                     w           N
                                          ==             4                             W          6 m O                                                                                                                O =*
  • e e ned
                                  >=      s=.

m M g a N e O en W tn la te e m == == tA nn O O ** M

                                                                                                                                                                                                == ==

M 9e .T

                                                                                                                                                                                                                                   =    ==

T N N N N 4 5 e ( tad e WO e e e e e e e me e o e e o e e O e= E e tad O E E 3 3 e 64 W .C tad led 4 Z la e ad E W ta. W N N g a == y u a y u a >= l . 100

A l N -o N h SIO M h 8'O M O 3 O O O 3 3 O O O O O 3 Oh h h ='. O O 59 3

                                                                                                                                                                                                                                                        .N 3

GH. 3 tas and & med tad ted ==s =ms w .ns tad ins tad t.d & ind w , a g 4,, 3 O. . . . . . . . . . . . . . . 3 ggg N edl M =A edt ame idt ame Jt @ g se 3 JD arl Pim ame g .m. suo

                                                       .O.

e . . . . . . . . . . . . . . . M AE . . . . M DS M. . . . M. M. M. M. M. M. M. DE De WW ed &

                                                                                                                                                         .                                        M.        M.        M.             .       M.           .           .

and M ed .E M M M M ed and M M .ud M & ed ed M == N O O == O -e O O O O O O O O O OO O O e =* O O O * == O N == O O O O O 3 O tas ned med ins ss e .ns tad and ins ned tas tad tas tad w w and =m# e N 3= e O. . . . . . . . . . . . . . . . e% f%e in N edt =A sue idt see @ me D em. d 4A @ en g .-e g =e "D O em. p. D= em. em. p= p . em. k. em. em. t= p. e= I ed

                                                                      .           .         .         .        .          . M.           .          .      De.       e=.            .           .         .      a=.            .         .          .

em. me ed & & & .$ $ ad ad & ed & ed & & & ad .ns U) M (n

                               >=

m .m. -e o O =e O == 0 0 .e O tes O O O O O O O O O O O Oe OOO OO OO O e N O O O and tes nas nas tad tas nas tes nas tad see las tad ted tea tmo nas ned

                                        .e    .am.a
                                                 .e Pm Q           e   m%                 O.              .         .         .         .         .        .         .          .         .

D'$ "D 49 N edt Fai. IA T og

                               &         2    46 ame                 me        tg         g g                  S           ep         @         q          p          q          see       *h Q *=. O                              .            e         .         .        .          .        .

3 M N $ D* mW. WW Di=

                                                                                                                                                       .         .         .           .           e         .         .          .          .         .          .
                                                                                                                                                              $3 O             b        %
                                   ==    E
                                                                    .         >=.          .         .     >=. e'=. e'=. >=.                           .        .
                                                                                                                                                                       $=

DB DB P= su=

                                                                                                                                                                                                                       .      e=.

em.

                                                                                                                                                                                                                                             .      e=.

e=

                                                                 -d                                                                                                                                                                                               .

M u O .J d ad as ed .J -d =A .J .md ad ad .d s d &

                                                                                                                                                                                                                                          .ms                  -d En2                         ==

4 .m.

                                    . >=

k s b - o as O m 0 == m O O = = , O O tad O O O O O O O OO OO O tes tad and

                                                                                                                                                                  == O O O O O O O O O O O                                                             N O
                                                                                                                                                                                                                                                               ==

O ned tad tad tes tad tas ans ted ted tea tad tad saa ned w M. . M qN 4% N ta ame in ta eo en

                                                                                                                                 .         .          .         .         e           .           e         .         .          .          .         .           .

3- .mo e en est e g g in p g me am N.e p aO 4 . . . . . . . . . . . . 7 n= >= >= e-

                                                                >=.                              a=. a=.                                                              e=                                 >=        e=         e=         >. >= ==
                                                                                .         .                             .        .     >=. e=. e=.                        .       a=. >=.                   .         .          .          .         .          .

and ed & .n$ & & & & & & & & & & & & end and ens f

                                                             ..          4/4 e

to ==

                                                           -             gpt 44             3 3            .s
                                                            =ms          4 4             m O            4 4

O E ted .a 3 8 4 m 0 u" u >= en W amo tea == ed E 4.) nos e e e 4 d tes & O 3 O e u u in a  % O 4 9 e O O 4A

                                                                                                                                                 %M                   e                      g em                 e          se         g          e e tae            ==            E    m       O         4A tA          O O ==                          M          M         9          9          9          N          N tA       4A         6        @         9          ase       se         M           en B=

4 O M E "e W e e e e e e e e sus e amo e eme e me e

                                                                                                                                                                                                                                        ==e s

N e N 4 e 4 ed e E O mesen. O E S 3 3 e O m X 4A e ad E u e 4#9 t#9 4 tad had 4 2 u me me a e == u u O u u a W T l i 101

TABLE B-10 SHORELINE SOII.: CA)04A ISOTOPIC ANALYSES (pCI/kg Dai) ST ATION NUNSER - SNWE-3 l MARCH OCTOBER DATE COLLECTE0: 03/06/85 10/08/85 GANNA SPECTRUN ANALYSI5; BE-F 4.00 11.76: 92 L.T. 4. E 02 K-40 1.13 t0.IIE 04 1.81 10.18E 04 5 w Ne-54 L.T. 3. E 01 L.T. 4. E 01 C0-58 L.T. 3. E 01 L.T. 4. E 01 FE-59 L.T. 6. E 01 L.T. 9. E 01 CO-60 3. E 01 L.I. L.T. 4. E 01 2N-65 L.I. 7. E' O'l L.T. 9. E 01 2R-95/NS-95 L.T. 4. E 01 5. L.T. E 01 30-103 L.I. 3. E 01 L.T. 5. E 01 AU-106 2. E 02 f.T. L.T. 4. E 02 I-131 L.T. 8. E 01 L.T. -1, E 02 C5-134 L.T. 3. E 01 L.T. 5. E 01 C5-137 3. E 01 L.T. L.T. 4. E 01 BA-140/LA-140 L.T. 5. E 01 L.T. 1. E 02 CE-141 L.T. 5. E 01 L.T. 8. E 01 CE-144 L.T. 2. E 02 L.T. 3. E 02 RA-226 4.18 to.5 3E 03 i 2.08 to.75E 03 IH-228 7.33 30.73E 02 1.94 10.19E 03 i

TABLE B-10 (Cont.) a.'ORELI.NE SOIL: CAlen ISOTOPIC ANALYSES (pCS/k9 Day) STAil0N NUNSER - SHNJ-1 GCTOBER OATE COLLECTf 0: 10/08 GA8MSA SPECTRUN ANALV5IS: SE-7 1.74 30.33E 03 E-40 1.88 20.19E 04 H NN-54 L.T. O 4. E 01 CO-58 L.T. 5. E 01 FE-59 1. L.I. E 02 C0-60 L.T. 4. E 01 2N-65 L.I. 1. E 02 2A-95/NS-95 L.T. 5. E 01 RU-103 L.T. 5. E 01 RU-106 L.I. 4 E 02 1-131 L.T. 2. E 02 C5-134 L.I. 5. E 01 CS-137 9.93 s3.61E 01 BA-140/LA-140 L.T. 4. E 01 CE-141 L.T. 7. E 01 CE-144 L.T. 2. E 02 RA-226 3.44 so.63E 03 IH-228 1.26 10.13E 03

TABLE B-11 MIlX: IODINE-131 AND CAP 9IA ISOTOPIC ANALYSES (pci/1) STATION NUMBER NKQ-5 JAtuARV JANUARY DATE COLLECTE0: 01/03 FEsauAay 01/23 02/05 RA010CNENICAL ARAlv515: I-131 L.T. 2. E-01 L.T. 4. E-01 L.T. 2. E-01 GAINGA SPECTRUN ANALYSIS: SE-7 L.T. 4. E 01 L.T. 3. E 01 L.T. 3. E 01 K-40 1.35 20.14E 03 1.18 20.12E 03 1.06 20. llE 03 Nu-54 i.T. 3. E 00 L.T. 3. E 00 L.I. 4 E 00 C0-58 L.T. 4. E 00 L.T. 3. E 00 L.T. 4 E 00 FE-59 L.T. E 00

9. L.T. 7. E 00 L.T. 8. E 00 C0-60 L.T. 4. E 00 L.T. 4. E 00 L.T. 4. E 00 ZN-65 L.T. E 01 I. L.T. 8. E 00 L.I. 9. E 00 28-95/58-95 L.T. 4. E 00 L.I. 3. E 00 L.l. 4. E 00 RU-103 L.T. 4 E 00 L.I. 4. E 00 L.I. 4. E 00 RU-106 L.T. 3. E 01 L.T. 3. E 01 L.T. 3. E 01 1 131 L.I. 7. E 00 L.T. 4. E 00 L.T. 5. E 00 C5-134 L.I. 4 E 00 L.T. 4. E 00 L.T. 4 E 00 C5-137 L.T. 4 E 00 L.I. 4. E 00 L.T. 4 E 00 SA-140/LA-140 L.T. 5. E 00 L.T. 4 E 00 L.T. 4 E 00 CE-141 L.T. 7 E 00 L.T. 5. [ 00 L.T. 7. E 00 CE-144 L.T. 3 E 01 L.T. 2. E 01 L.T. 3. E 01 RA-226 L.T. 8 E 01 L.T. 7 E 01 1.

L.T. L 02 TH-228 L.T. 8 E 00 L.T. 7. E 00 L.T. 9 t 00 _ __ ^^^ _ _ _ _ _ _ _ _ _ - _

ae ** M O O O O O O O O O O O O O O OO O ao O O O O O O O == N O e O O O O O O O w .na tad W tad ned W w N tas tea taa w tad has med =ms ans w w ES "* u s==o * * * * * * * . * * *

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                                                        ==s O O C O O O O O                                          O == c O                            O        O        O == .= c e                             O O O O O O O O                                                        O O O O                             O           O O O tale            %nd      haJ    had               tad had              tea      ted      had       had      nad      led      tad      had T                                                                                                         had      med        .ad     med ad
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had had had tad ned led led had tad had had had tad nad tad tad had W end M me er . . e e . . e e e e . e e e e . . . . ned O N M O T T == idt ** T T T S T to ed's O M == m EN *e 2@

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ed and M ed =d M ed M M ed ed M ed end and M and and ud E"* M m

        *=4 8

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W W  % M O T h O == T 4 # O .'" 4 Y G S O tA en O O ame M M T er T N N na.d

                                ==  M          S    M        O       tA      4A       tA       @       @        S        emo       se       M        se       se       me       one        one      N       N k      O              S      e      T        e        e        e       e        e        e        e         e      sue        e        e        e        e          e       e       e 4      4   8'e* 4          tad        0     W       O        tad      O       E        5        O 3                         W1       4A       4                                    Z Q      R e                                 ned        ned      4
                                    =* 48           e ed E                   W        ns.      W       N        N        m         5        == W W                     e        to u                E       >=

i 107

i

                                        =*            ~       M        o O O                     O      .-e          O O               =e O

e O O O O O O O O O O O O Oo o O o O == ~ o O O O O C had taJ tad ned saf tad nad had ted tad N nad ned nad tad had had d had W t= @ *=e wg e o e o e o e e e e o e e e e o e e e 3% M W O T T e T ==e 49  % T T T === T 9 tre e M S S 30 eg e e N . e o e e o e o e . . e e e e e e== >= N *= s= e= e== e= e= e- >= em e= e= e- >= >= >= >= e o e e e o e o e e o e e e o e e e e

                                        &            .O       **      ed      O         ed      ed      S          eb        eb       ad         ed       &        ad          &         S          ed                    old      =Es
                                       ==e          ==s      M       O O O O                           ==s       O O == O O O                                                 O          O ==

O N O e O O O O O O O O O O O O O O O O O O ned had taJ &nd ned had had nad tad tad ned tad had had had had had nad en tad

                                                             ==e
                         > .4             e            o       e       e        e        o       e        e           e        e         e         e        .         e          e         e          o                     e        e
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e a= o e e e e e e e e e o e e o e

            >e                                              in                         e==     >=      s=       to          >= >= >=                     e-                                       >=                   a=        >

to. J .a e

                                                            =*

e o e o e o e o e o e >=. >=. >=. e e e A .d .A .a d . -d ==d s -a ed d .4 s d .d a a O ^ m en e & e

&J        c         cr c         F*        M C         O
  • O m a a V ee t=e p4 w

N

               ***e e sed E                ==            **       M
  • m O 3 O O O O O O O O ==e O O O O O == == Q e"I E & B e O O O O O O O O O O O O O O O O O O

$ V tad ned ned ens tad ned ens tad a M ned ned ned ned nad nad tad had ned nad had g O ene g - N e e . e e e . e . . . e e e= >O M O e o e . . . et .a % T T T S T S T 4A er t== T T T Pam M W W es a= 3 Pam H en 3 0 e e e e e o e e e o e e-4 e e e e e e e o e= em N >= e= >= >= >= >= pg e e o e t= em e- >= >= >= to > e= g -d .d a=8 ed o S e o e e o e e e e e=. e e e amd .J .d .J .4 ed =4 ed .d -d d d d =a .d i M 2.e: Q Q

        >.4 es ee           en a                            to            ==
                                ==            to to            >
                                >             ad
                                -d            4 4             E S             4 es og O                 E tad .s            3 t=   4             m                                                                                                                           o W    W             >=                                                                                                                          W 4A                                                           ==e ned  ==            W                                                              S                                                               e
                            -d  3             had                                                              a                                                          4 e,

O d had 2 to e .4 W  %,e E  % s's  % e=0 W W ** O =8 W @ e W O S O en 4A O O me M M T N N tad O. m M pg O in na en e e T e- O === 0 W e g3 3 ese ame m me ame ,te me one N N e e e e e e e me e e e e 6 4 4 e 4 ned a 3 O t t O M es G tad O 3 m 3 3 e to to .C tad tad eC Z S ad % W nao u N N m e == W W e W W m >* a t 108

                                                  =*              ==         M O                                    O O == O                                  ==         O O ==                         4         O O                  O e             O O O O O O O                                                            O O O O O O                                                    O
                                                                                                                                                                                                                     == == N -

O O O O had tad tsJ had had ned ted tad ned nad nad tad led N N tad ted had med tad .ma tad N =* goe #. . . . . . . . . . g% =e in O to en me nad S

                                                                                                                      @         ce         tA        N         ta       me          @          d         N          ==           .P                    -.

98

                                >= O e,                  .
                                                                    . N                  .         .          .          .        .          .
                                                 >=                                                                                                    .          .        .          .          .         .

nad es. >= >= e-w . . N. e==. >=. e. a=. e. o= em a= e. >= we ese se .d ed

                                                                                                              .          .                                                 .          .       e=.          .           .            .      >=,        s=,

ens ad ad -d .d -d -a -d -d .J d ad eJ .4 me me M Q O 0 p. O a=e O O == O O O O == == N O O O O O O O O O O O O O O

                                                                                                                                                                                                                                                     ==

e O O O O E tad nad tad tad led ted had ted had had nad ted had had the N ned tad tad med end ST *=0 30 . . . . . . . . . . . ned % N to O 4A en me

                             >= 9                                                                                  tG         as        tA        e         6A         N         e e e                           .e M               a. O ee                                                                                                                                                 T          -.

BB in.s . . N . . . . . h N h'= p M. M. N. M. M. b.

                                                                                                                              $=
                                                                                                                                                            >=.                             D=                   $=          W           e.e a            uma       -e         .J        .a
                                                                                                         .d
                                                                                                                                .       M.        M.                   N.        b.            .      M.            .            .          .

mes

                                                                                                                   .4         .0        .A        .d        e.d         d        -d         .a        e.d          a         .d          a E

a u w

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e b U C O O m u v sn m had

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w '.*=e.

                 .      O                    -4               ==        M OO OO O            O O       O ==     O OO OO O==OO OO OO OO g                      2                     O                                                                                                                                                                 O == == O O        O a=             .       g
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O O O O b3 >= 4A N . . . mJ . . . . 4 O% d=9 T O

                        >=  OW                                                     T         T          S         T         se        T          T         T         h          T          T         6A        N            M tA                                                et                                                                                                                                                             C          C 30 3

' 4 . . te . . . . . . g . . . . . . . e- #='t e= . . . a=. e. >=. e. a=. a=. a= se >= >= e- ==

                                                                                                                                                                                                                                       .=,. >=.

em0 and M em0 ed

                                                                                                                                                  .          .       e=. e.                  .         .          .            e em0          0       ed        and       am0        .d        ed        emi        d         ed         eJ          and         d i                                                                                                                                                                                                                                    ese a         4 O

M

                                        ..             en e                                 tA              em.
                                       ==              we tA              3=

3= w

                                       =d              4 4               3 5               4
                                .. eg O                       E tad    a                O em     4               W                                                                                                                                            O W      W               >=                                                                                                                                           W had    =               W                                                                              4A                                                            s=e ad     E               tas S                                                              e e
                               .md    nee             e.                                                                             e                                                             4 O      2               to 3                                                             .d W      W                                                                                              %         M O    ** 4                                                                                                          43                   T          N         O ==                   T           @          e W         G S O                           4A        tA        O         G          se        M          M tad     ==   M          M    N          O          tA        4A                   tG                                                                                 T         T            er          N          N
                              >=      O    me         S      e        T           e to                    tG        S         a=e       s=e        M         ene        se        se        ==          *e           N          N e          e         e 4       4                                                                                     e         e         e         e         me         e e         4    tad         a         3         C         tad        O E                  E         O         O e         e          e           e           e          s O       M    ==         O    S          ad E                 W                    W e        tA         WS        4         ted          Gad         4          E na.                   N         Pte       a         5 ==                 W          W         m         W            W           at         e=

109

t a a* M O O O O O O O

                                                 =ma e

O w w mw O O O O O O O OO ==O 0 OO OO O O O O O == -. 3 C 3 3 n tad w w ned w w tad w w 6d med w tad w nace

  • O e e . . . e E% N M C w w e w a w w w
                                                                                                                      .         .          .        .        .              .          e         e         e                   .                 . . .

nas =e *I .a w w w a m 00 00

                              >==

0 . e e . e . . . . 3 I= D= em t= tm >= >=

                                                 .4
                                                    .                .      N.         .      >=.          .         .          .        >=.        .

tm

                                                                                                                                                                         >=

p.e em

                                                                                                                                                                                                        >=. >.                              .= no        a=
                                                                  -d       ==       .4        .J        M         -d a        .d       .J       M               a          s         a       .d                   a                .d     -s   ed 9
                                              ==                ==e O                 O O       m O O =* O ** O O                                                              =e            O         O O                   O == .= N ==

e O O O O O O O O O O O O O O O O tid ned m nad ned ted med tad tes ned w nas ned ned ned ned A .ad med ==* m m tad =A . . . . . e == m in 0% O*e wd ta == e ** e e in N e e e == til == ** (4 u.O. a= . . w . . . . kB O e- . . . . . . . . . . .

  • e >=. m. e. >=. e=. t= t=

s=. a=. e=. t= t= e-(4 e a == =d

                                                                                                                  .           .                                          .      s=. >=.                 .       >=.                                >=. ==.
           >*                                                                               .J        -d          a        .d        .J        -s .d                   .J          a       =a           a       .d                         .4
                                                                                                                                                                                                                                                   -d   -d e

U

  • n e

M e Se ad M C O H ind Q ^ e w .. M 3 ** M g N

                <ed 3

E O e

                                                              ==

O nas OmeseOO OO OO OO O O O O OO =* O OO OO OO O O OO == =* O O O O

      ,g tad               ted 8   A                E                                                  w led       ned       nad         had       ned       nad      ned          led        ned        ned A                w   O    E                                                e          .

med had med had tad

                    -    ine ==                .                .         .       .         .
                    *=   eO                 N M                    4    0%                                   w Oes w w e e a w w w

.J *= *= 0 N w w e N m a e m 44 *= . . en . . O >= t= M >* D= e t= sm. e= tm >= to to p= 6 e e . . e t= a= p. >= a= p'= M .d M M ed .d

                                                                                                                .                     e        .         .             e        e          e          e         .                           .       e      e M                                                                                                    ed         M         ed        M         M         M            M          M            e       ad                       ed         ed    .'8 M

1 M 5 8

                                      ..               tpt t#l               ==
                                     ==                t#9 t#1               >
                                     >                 .d
                                     -d                4 4                 3 S                 4
                             ..      et e                          E nas p=

3 4 m O u u 8= v tad - W nft == ed E ned m e

                                                      &                                                                            3
                            -d O

ens E t#1 e ( d W W 3  % C =* e e m Q 4A

                                                                                                                                  %mW                                        w          N         O == w e #

tad ==

                                         .m.               N           O       tA       4A        eft        e e 4 e en OmeO                                  =e             m          M                   w w                                  N      N 8=       O     =

O w e e e e e.o m me se .e.e .mo =e N N 4 4 0 4 tad 3 e e ao O 5 == e I WO ned O E E 3 3 W e e t#t e e a 9 e e ad X W 4 4 E ne. W N N e s == u u e u u a 4>'* ned I had

                                         \                                      110 s

l 1 I i

                                           ==             a O              O O m O 3 OO O 3 O=*                                     O O O O O O 3 =* 3O oO 3 33 3o o                                                                                      =a         N 3             1 g

s ned 2 o a ' had tad tad had ned tad ned tad 44 tad ted tel tad tad N te. ted and ed e. E .O. . . *".* . . . . . . . . . . W% N O Y Y N T M T Y M WN 4e N Y Y d N N W M had om e . e e e e . . . . e . . . . p= > o= > a= e == a= e. a= == == N. e= == p-e.d

                                             *              .                     .        e         .           e        .      e=.           .            e          .          .              .        e          .           o     >=.
                                                                                                                                                                                                                                                    .=

e.$ 8"o ed e.J u.0 a.d eJ ed .nd and e.e .J e e .J .4 -d a ; i i ne ** m O O O O =e O O en O e O O O O O O O O O O O O OO O O O O O O == O N 3 C Q led ned led had led tad had tad led M had led had had Lee ned N t.d end tad tad tad s=e SM e . e . . e . . . . 3O M M Q T T S tA me W W M 4A T

                                                                                                                                                                                 .            e          .          e          .         .           e C/)         tad %                                      es                                                                                                                    T          T          P%         M          ==          @

ga3 m W t.d N. b O n= s= >. > e= > e= N. e. e= en eI

                                                        =d e

8'O

                                                                                .                  .           e                   .      e.           >=.            e         e            .       e=. e.                a=. e. .                  .

eO and =d gni ed -J m.$ med a.d ed ad e$ e.d d ed ad i U ^ b d e

&J O        cr l=e      w C           Q       R O          V3    m U           M     M  N v                 %, nas
        -        ~

M i 3 eg ,l O - , O O O O O O O O O O O O O O O O O O O O OO OO O O .= - ~ = O O O m E a a 6 4.0 4., t., led 4., t., t.d 4., t., t 4.d 4.d 4.d 44 - te., - - O 64 .m g g == ee e . . . . e . . 3 '- E N

  • O *e* * * * *
  • 4 e-taa '%"'

m en 4A m a w w e e w e en O e= N M M >

                                          .              e       4A           .         e         e          e         e         e          e            .          .          e            .          .         .           .

m e-e=. em. e=. *e=. e=. e=. em. p. en e4 =a

                                                      =a
                                                         .       N.

me a a =A .a

                                                                                                                                                         .          .       e=. e=. >=. >=.                              e=

e= s= l a =d a a a -d .J -d .a .d .a -d Di2 2e". O O M O .. h3 E

                                  ==             We 4M             >
                                  >                e and            4 4               8 8 '

ag 4 O E ted .s 3 a= 4 W O W W e= W 4A tee - W S s-. s E ted 4 e

                           =.d m     led            &                                                                                                                                                  4 O     E              to S                                                                     ed W     W                                                                                           M                                                                     %
                                                                                                                             %          M            @                     w            on.        O =* w                          4           00 0    **                                  W         G         S          O         4A        4A         O O                                             M          W 1.s   ==   M                         O         4A                  en ame         M                                 W          T          N           N e-    O    me 8't                            4A                   @         @         O          e=e         se         m           amo          s=o        a.o       are        ==         N           N e         9          e         e          e         e         e         e          e            e        me           e            e 4     4     e        4    had         e        E O                            O         E e          e         e          a            e e     m    == W           e                                        ted                            E          O            3          e          to to 4                           tad        had        4           2 ad E                W         t          W         N         N          5            m         em          W W e                             W          44         m *=

s 111 <

w. ,- --y a-g- w pr----+-

w- -

TABLE B-11 (Cont.) Mll.K: n-IODINE-131 AND CMetA ISOTOPIC ANALYSES

s. (pCi/1) '
                                                                                                                                               \

s

                                                                "                          STATION NUNSER NKE-4 (a) 1 N

MARCH (b) NAACH i s 4 Of f COLLECTE0: 03/04 03/19 N ADIOCNENICAL ANAL YSIS: 1-131 2. E-01

                   .                                                                              L.I.                    L.T. 3. E-01 GANNA SPECTRUM ANALYSIS:                                                      ~

SE-7 L.T. 4. E 01 L.T. 4. E 01 K-40 1.27 20.13E 03 1.35 20.14E 03 NN-54 4. E 00 L.T. L.T. 4. E 00 C0-58 4. E 00 L.T. L.T. 4. E 00 FE-59 L.T. 9. E 00 L.T. 9. E 00 CO-60 L.T. 4 E 00 L.T. 4. E 00 ZN-65 L.T. 9. E 00 L.T. 9. E 00 2R-95/NS-95 L.T. 4. E 00 i ' L.T. 4. E 00 , RU-103 L.T. 4. E 00 L.T. 4. E 00 RU-I D6 L.T. 4. E 04

L.T. 3. E 01 l-131 L.T. 8. E 00 i

L.T. 8 E 00 C5-134 L.T. 4. E 00 L.T. 4. E 00 4 C5-137 L.T. 4 E 00 i L.T. 4. E 00 SA-140/LA-140 L.T. 6. E 00

 !                                                                                                                       L.T. 6. E 00
 ;                                                  CE-141                                       L.T. 9. E 00        L.T. 9.    ,E 00 CE-144                                       L.T. 3. E 01        L.T. 3. E 01
  • RA-226 L.I. 1. E 02 L.T. 1. E 02 TH-228 9. E 00 L.I. L.T. 9. E 00 (a) New station added to program.

l (b) No saeples were available prior to March since goats were not lactating.

TABLE B-11 (Cont.) MILK: IODINE-131 AND GM9E ISOTOPIC ANALYSES (pC1/1) STATION NUNSER NKE-4 NAT DATE COLLECTE0: 05/07 BASIOCNENICAL ANALYSIS: 1-131 L.T. 3. E-01 GANNA SPECTRUM ANALYSIS: 8E-1 L.T. 4 E 01 K-40 1.23 20.12E 03 NN-54 L.I. 5. E 00 CO-58 L.I. 4. E 00 w [ FE-59 L.T. 1. E 01 C0-60 L.T. 5. E 00 2N-65 L.T. 1. E 01 FR-95/us-95 L.T. 5. E 00 AU-103 L.T. 5. E 00 AU-106 L.I. 4. E 01 1-131 L.T. 6. E 00 C5-134 L.T. 5. E 00 C5-137 L.T. 5. E 00 BA-140/LA-140 L.T. 5. E 00 CE-141 L.T. 8. E 00 CE-144 L.T. 4. L 01 RA.226 L.T. 1. E 02 IH-228 L.T. 1. L 01 d

'_ _ _ _ _ _ _ _ - - _ _ _ _ _ _ . . _ _ _ _ _ _ _ _ _ _ _ _ _ _ - . _ _ _ - _ _ _ _ _ ~ _ _ _ _ _ - _ _

s's s=e M O O O O O O O O me O O O O O e taif O O O O O O O O O O O O O 3 O e. O O O O med nad les nad ted had ted ned nef led W 'A tad tad tad see tea tait eind had We ag O e e e e e e e e o e . . e e e 3% 9 M C e 9 e e a w w M e e e e SN *e 4A e v en  % M e % SO tad *

  • N e * * *
                                                          >                                                                                  *         *           *          *           *         *
  • e e e h

e

                                                                          >= w                 t=       em          >=        e-         >= >=                  e=         t=         e=         t=         >=          t=        e-          >= >

a= e o e o e e e e e e o e o e e e e e

                                                          =J              -d        s==        .J           8       -J           d       .J         .J          ad         and        .J         .d         d           .d        .J          .d            e      .J
                                                        -a              -e         8"o O O O O O O O                                                               ao O

e O O O O O O O O O O O O OO O O O O O == == c O O O O end tad had nad ted led led nad tad had tad tad had led had ted tad M had had De e=e MN e e o e e e e o e g e e o e 4N M w O w w e e e a e e e e U 3% *e 4A 6A 4A w Pe w to te e M m e S a== M 40 e e e e e . .

                 >e            e=3                      e.              p.                   m.        p.                   p.

e e e e e o e e e e - e

e. a. p. p. p. p. a. p. p.

e . N. . . . . . . e e e . e o a. e me ,. p. em$ end 8'e e e e end .O emI d. and and .A .u0 .d ed and and en0 d ed and U M O A A to

  • O O'
  &d            H e

U o 8 n=4 M V m

                    %    tad ee       we   e esed Q    E                            n=e              ==       M es OO OO O            O OO OO OO OO===                                 O OO OO O                       O OO O ghe 3                             O                                                                                                                                                                       O           ==         N ==

m 1 e=e E w E ' O O O O O a "' '*' "' 'd '** "' M O m- ,M''''''' e a=3

                         ==

e= me e o e o e e . . e e 4O N . . e e e e e e e 4 3% w O gew w m na m w in w e w w to e e a=e == e= 3 ene

              ,.g        M   40                          e               o      M             e         o          e         e          o                     e m              '"4                      >=

e

                                                                       >=       4A         >= >=                e=        a=         t=e        e==

e

                                                                                                                                                          >=          p.

e

                                                                                                                                                                                 >=

e p. e e. e em e

                                                                                                                                                                                                                              >=

e om e e= e a= e 4 e e e e e e . e e e o e g -d s ** e e . . - e.d .d .d s .A .J .s .d a .d .d -d es d M d -e 2l ee Q O w.e

                                                 ..              m
        ,                                       44               ==

a= M to se

                                                >                ad ad               4 4                 3 3                4
e. ag O E nad -,A 3
                                 >*            4                E                                                                                                                                                 O tid           e=f              >=                                                                             tA w

led == W 9 a=e

                                 -d            E                tad                                                                             e e

a ned a. e 4 C 2 M a .,e W W  % M O w m.e wOw == O w w e e N

                                                    *==

lad == M Pe O w W S S tA en O O me seg rg N 4A tA GA te @ S a=e ao a=e se

                                >              O    **                 e e                 e         e          e         e          e          e         a           e d=e se e=o        se         ==          N          N 4              4      e         4    led                                                                                                                     o         e           e          3           e          e O              E a         g O                 tad        O          E          E         3           3           e          M         to 4                              tad         4          2 e
                                                    == 48            e ad a W                                 W          W          N          N         N                                  W had 5 ==                             W           GW                    W           M
  • i 114 i
                                                                                                                                                            " ~
                                                   =e                 =e 0                  O O mO O          O        O =O 3O O==                      O O O O -.                   O O O
                                                                                                                                                                          .= 0 OO O3 ==                                        O m          N ==

e 3 3 3 ned thi had had had of nad tad taf had had W Gad nad taJ tad tad and ud w uE ,O,o e e 3% M 9 3 @ @ . . . . . . . . 4m me @ s=e @ @ ta s=e @ @ D == == es in s=e EO

                                                       .                 .      N           .         .          .         .           .         .         .         .          .           .            .          .

M. W >= P= N. O. N. . M. M. M. N. D= M N %I= e'= D=

                                                  <u.d               e.0       8'e       d         d          ed 0        M         ed
                                                                                                                                                                     .          .       M.               e          e       b.             o         . .

euid s u.0 e.0 ed and end ed e.O d me amo m O O me O s-e O O s-e e-o O e had O O las O O O O O O O O O O OO O O == == == O O N -. O O had led nad had Gad led tad

                                                                              @                                                             had       naif      ned                   led           had       had          had        tad       ens       lied ET WO                    .                  .      a'.s        .         .          .         .           .         .         .         .

5% N @ O @ @ ** @ == N WM 4e @ kH as @ @ ao ame ga a.e ce U3 EO W . . S . . . . . . . . . . . . . t/3, . . . p >=. >=. M. e=. a=. e=. e=. e=. a=. >=. t= p= >= >= g .J s ao s e.s a w

                                                                                                                                                                   .       >=. >=.                    .      >=.              .       e.          .     >=.

s .4 a a a e.d a .J -d a a a I 4 O O m *

m. m a 4, C E O

O ^ m V .. N sW tes

                      %n O p.e                  w  E                     ==

m y G == m O O == O .= 0 O a-o me a I sd E y E 3 O e tas O O O tea na nas ned O O O O O O O O OO OOO O == == O O N == O O W > a=i sm.s tea tad nas nas naa ins ned gas led tea tad 4.s =ad sad O ge M == qw e . as , 4 M CO M @ O N N 4 e= SN g% 4e

                                                                                                          ==        N           N         N          e        @         ao          N            N          e           ce          nn        N         ==

g W wN .

  • N . . . . .

g hO >= . . . . . .

                                                                            ==. >=            >= >=

D= . . . . .

                                                  .
  • a=. >=. >=. tu > > em >= >=
                                               &                  O         Y
                                                                                                  .         .                                         .       a=.          .      .=.               .          .        >=.            .      *=.
                                                                                                                                                                                                                                                        *=

nad & O & ed ed ed & & & i mid =d ed mid e.d M E w Q C w e

                                                                                                                                                                                                                                                                 .D =

O e

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                                          **              M                                                                                                                                                                                                       >

N =S g

                                         .=               to                                                                                                                                                                                                      g to               D
                                         >                -d                                                                                                                                                                                                     .gs ed               4 4                3                                                                                                                                                                                                       ..

3 4 6

                                  **     4                                                                                                                                                                                                                         .e
                                 &                        E                                                                                                                                                                                                       g nas       e              3                                                                                                                                                                                                     ==

em 4 S O W W *= 9 9 las - W 48 a.e S e

                                .4      E                tad s

e CL

                                .d      les              e.                                                                              e                                                                 4                                                      sk O        E                to 3                                                                 a                                                    ==

W W  % 2

                                     - O     8'*         4                          9         O
                                                                                                                                         %         M         q                     W            Pi.        O           ame         e         @         g        th
                                        =    M           g                                              S O                   tA         4A        O O .=                          M            M          9                       W tad                               N         O        4A        tA        tA         @           @         D         ene       se        M          ao T                     N         N e=       Q    *=e         a        e        9         e         e         s - e                  e         e         e                  s=8 a=e        se          ==          me        N         N 4        4                                                                                                                     a                     e            e          e 0         4    ' ned         e       S O                 ned        O           3         5         3 e           e         e         s       ==.

O e " W G 3 0 th to 4 W EW wW *e N m a == W W e W has nad W 4 2 as >= w 9 l 115

1 1 3 0 0 0 0 1 0 0 0 0 0 0 0 00 000 0 0 0 0 1 E

                                                   -           0 0 0 0 0 E        E         E          E          E          E          E 0 0                      1 0 0 0 1         0 4                                                                E            E          [          E           E          E          E            E          E           L        t 6                                    1 V0                 .            .         .         .         .           .         .           .          .                      .

A/ N5 2 4 o 4 4 9 5 1 4 4 4 5 4 5 5 t 8 3 9 9 0

                                                                 . 2                 .         .          .          .           .          .           .          .          .           .          .          .

4 . . . . T. T. T. T. T. T. T. T. L L 1 T. T. T. T. T. T. T. I

                                                                                                                                                                                                                                         .       T.       T.

L L L L L L L L L L L L L L L L 1 1 3 0 0 1 1 1 0 0 0 0 0 0 0 0 0 0 0 0 00 00 0 00 0 1 0 0 1 2 1

                                                -                                                                                                                                                                        0          0 0 0 E              E        E         E         E          E          E           E 3                                                                E          E           E          E           E          E          E            E           E           E        E 1

L5 . . . . . . . . . I1 3 . . . . . . 5 0 5 5 1 6 . . . . S R/ 1 1 5 6 5 S 5 6 6 9 4 1 1 E P4 S A0 .

                                                               . 0                .          .          .          .           .          .           .          .          .           .

Y T. T. 3 . . . . . . L T. T. T. T. T. T. T. T. T. T. T. L L T. T. T. T. T. A 1 L L L L L, L L L L L L L L L N L L A

   )

C 0 I

      .        P      5 t          O      Q n          T      K o          O      N C           S  )

(  : I 1 R E 1 l l A

                  /

i S N 1 i t cp U 1 1 3 0 0 1 0 e 0 0 0 00 0 0 0 00 000 00 0 0 1 1 0 B

    -     M A

l ( N E

                                              -            0 0 E         E 0

E 0 E E E 1 1 0 0 0 2 0 G N E E E E E E E E E O 3 E E E E I 1 L D T L1 I0 B N A R/ 1 4 o 4 4 1 5 1 4 5 4 9 4 5 6 A A T P4 t 1 4 1 9 T S A0 . . 6 . . . . . 1 2 3 T. T. T. T. T. T. T. T. T. 1 L L 1 L E T. T. T. T. T. T. T. T

                                                                                                                                                                                                                                                .      I.

L L L L L L L L L

                -                                                                                                                                                                                        L            L          L           L         1 E

N I D O I

S
            .                         S               I I               S S               V Y               L L               A A               N S               A

_  : A 0 N E L U T A R 0 C C T 4 E I C 5 1 L N E 9 - L E P - A O N S 8 L C C s / O 1 A / 3 6 4 7 0 1 4 6 E 4 0 9 0 5 5 0 0 8 I 3 N  ? 0 5 5 5 6 6 9 1 3 3 3 4 4 4 2 2 T D 1 N - 4 - - - - - - 1 1 1 1 1 1 1 2 2 A A - A E

                                                                                                                                                -           -        1             -          -          -            -          -           -         -

D G G

                                                                    - e 0                        E           0 5 R                            U           U            -         5          5          A                                    A 1               D         K         N         C         F           C          2          2          R           R E          E                     M 1            C C B                             C          C           R         T i                       ' i. i,                                           i                              'j          l                     j4{                               }l*               :'              j                      I                      i>

l

                                                    *
  • M O O O O O O O O O =* O O O O O a N O e

O O O O O O O O O O O O O O O O 3 tad ted ted led had nad tad ned had nee tad had had and ted had ted ted t.d 9 r== 8==e gag . . . . . . . . . . . . . . . . . . . 3% M T C T T S T S 4A en T 9 T T @ @ W == @ O@ *e 70 . . @ . . . . . . . . . . . . . . . . e- >= e- >= >= se p= a= a= o=

                                                       .                  e   M. a=.       e     >=. >=.          e=.          .        e       .    >=. >=.          e=.          e    >=.           e             .        e ed                 M      M      .d     M        M      .d        M            d        d    M       -d         d     .d       M        M          e.$    .O                 0 m                  =*     M      Q O O O O O O == 0 O                                                                 O        O O                                                                                                                                       O -. == 0 e

O O O O O O O O O O O O O O O O O O had tad tad Led led led had had ted led tad ned led had had led ned tad and M s.e rue . . . . . . . . . . . . . . . . . . . tad O N M O 9 9 S T S T T T @ T tA en N M f01 E% +e O O M @@ gjy =3 0 . . M . . . . . . . . . . . . . . . . p om D= > D= >* >= p= em > >= g . . M. e. >=. >=. >=. . . . em. . >=. e=. . . a. . . a .a == a .d d a .d a .4 a .d a a a .4 s e .4 0

  • M
m. m ,

4.8 CF C M C E O ^ w .. M M M

                   %.  **8 d             M   E                          ==*

N =* M O O == O ==. O O ** ==. O O 8 s"I E 9sa 3 a O O O O O O O O O O O O O O O O

                                                                                                                                                                                          -. ==

O O N O O

                                                                                                                                                                                                                             ==

e M V ned tas ned has and nas nad and nad 6ad nas tad nas ned tad E 4A te s 64 tad had g O m a = e- >N O N O 4A en == 4 4% ge Pan ==s @ N 4A em @ @ e == 9 == ==

                       >=        E to H                 to             O              .                  . S         .      .        .       .

M D= p= >= m >= M

                                                  >=.                   . T.        .   >=. e.              .    >=.           . e=. e=. >=         .
                                                                                                                                                              >=

o=

                                                                                                                                                                                    . e=.
                                                                                                                                                                                                    >=

o= a=

                                                  -6                 ed     m         d   .a       .d     .a           e     .a        .a      .h      .A      .A       =o          A     .a           a       ,o            .d l

M lE.e n Q O w 1 I 1 to t.o. )

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                                            >              -d
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had == u 9 e ed E ned 4 (

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u u  % M 49 9 r== O == 9 @

                                                 == 4                                                                                                                                                                        c0 9      G S             O        4A        tA       O        g       se     M        M        g ned
                                     >=

O.

                                            =

G M

                                                 ==e g        Pts     O en          4A      4A      @        @         S        s.e      e-. M      se       one      em T

am. T me N N N N a e 9 e e e e e e e . == * *

  • 4 4 8 4 tad a 3 O ins O 3 m O O to 44 4 4

e m == W e e ned tad 3 ad E u te. W N N g a == u u e u u eg >= Y l i 117

                                                                                                 -                                                                                                                                  l

e

                                                     .4           =*           M O                                O O O O O O O * O O O O O == =*                                                                                                               O had e          O O O had          had    had O O O O O O O O O O O O O O tad O

he8 tad had ted ted ned ted had had ted N had tad ud med tus en =8 mO e . . . . . . . . . . . e . . e 3% M 9 . . . gg Oes e e e e e en e e a en e e e M e e ] 1 20 ' m o e en e e e e o e . . e e . . . . e o e- >= >= >= >= se se e . ==. e. e a=. e=. >=. e e >=. e e em e e-e

                                                                                                                                                                                                     =

e >=. e=

                                                                                                                                                                                                                                     >=

e l and =4 emme .J ,,3 ,,3 d d .J .J .g ,,3 .g .g i

                                                                                                                                                                                           .A       ,,3      ,,3       .3            d
                                                    ==           ==          M O

e O O O OO OO O O O O O==O OO 0 O O==O 0O O O O O == tJ

                                                                                                                                                                                                            == O0 O                       O had          led        had      had    Gad    had         ned      had W                                                    had      hh8      tad      had     led        tad       had       had     tad        had           had s
p. en.
                                     .                                      m'e E                 d%                  M
                                                       .            .                  e g

e o e . . . e e e e e . . . M T O T S 43 se g gn g e nn en g tn 3 run *e N #we e e

                                '9 0 y                                       e             e       en         o      e      .             e      e        e        o         e y                                     t=           tm                 a=            t=           tm.              >=        em e       .           e        o        e         e         e            e
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                                                      .            .        M.         .             .             .    >=.        .        e      >=. >=.            .        e=.          . e=.          e em o

p= e ed em0 WO ed ed and em0 M emf and and and and em0 .J .m0 ed .d ed O O m ese nn e Se ' u

  • e M C

O ^ m v .. M M w

                    *me    e M                   M
 ~         ~         y,      l E                                       .e                      M        O O           .e 4                  y y                     O O O O O O O O O O O O O OO OO O O O .= O O                               e                                  .mo                =. ~

O ea O O w M e= w wN and w w w w w w w w w 6.s w w w ie. tad y s= se

                             >=

N . . . . . . . . . . . .

                                >O                 M            N          O        Pt.           N
                                                                                                                                                             .                   .         e        .        .          .            .

en ed % 4e h N N Pam 9 N N mW -e a=e @ N == g SA O "5 0 e e e o e e . e e e e o e e e e e e e d t= e=e >= >= e=

                                                   >=.             .          .       . e=.               a=.

t= e=. em >=

                                                                                                                                                                   >=.
                                                                                                                                                                              >=                                    s=            s=

I -d =d o'* =d

                                                                                                    .                    .        .                  .       .                   e      e=. =.            e=.          .             .

M .J ed -d -d .d ed -d -s -d -8 .d e sus .d =d lE pus Q O pue e. j e ** to a ==

                                        ==                  en en                  3=
                                        >                   a es                  4 4                   S S                  4
e. eg e 5 tad ed 3 em 4 e e SmA 4p 8= w ta se nas == W e
                                   =d   E                  tad                                                                 5 e

w one sk 4 O 2 in e aus W W 3  % O s'*  % M te e P=. O e-o e e e O nn*enW en e gO geng en O O tad == sue M s's sue w w ,ew N N one ese m ese ,M e es, N N em 3 aus e e e e e e p me

                                   <    =          a       =    w                   a UO w na. O aWe Na aN a        3        a                         a           e         4        e        e         e             e e e == eW a wW.= ew W                                   w =W z e

O 5 == W e - ad S ,5 t= s 1 I i 118

l l TABLE B-11 (Cont.) MILK: 10 DINE-131 AND CAlelA ISOTOPIC ANALYSES (PCi/1) i STAil0N NUNSER NKQ-50 AUGUST SEPTEMSER DATE COLLECTES: 04/19 SEPTEM0Ek 09/04 09/16 BASIOCNENICAL ANALYSIS: I-131 3. E-01

                                                                                                ~

L.T. L.T. 2. E-01 L.T. 2. E-01 GANNA SPECTRON ANAL YSIS: i SE-7 L.T. 4. E 01 L.T. 4 E O! L.T. 4 E 01 K-40 1.14 20.llE 03 I 1.34 1 0.13 03 1.30 so.13E 03 e Na-54 L.T. 4. E 00 L.T. 4 E 00 i e" L.T. 4 E 00 j CO-53 L.I. 4. E 00 L.I. 3. E 00 L.T. 4 E 00 FE-59 1. E 01 L.I. L.T. 8. E 00 L.T. 1. E O! CO-60 L.T. 4. E 00 g L.T. 4 E 04 L.I. 4 E 00 2n-65 L.T. 1. E 01 L

                                                                                                            '.I. 9. E 00  L.I. 1. E 01 2R-95/e8-95                                    L.T. 4. E 00              L.T.

i 4 E 00 L.T. 4 E 00 l RU-103 L.T. 5. E 00 L.I. 4 E 00 L.T. 4 E 00 $ RU-106 L.T. 4 E 01 L.I. 3. E 01 L.T. 4 E 01 1 131 L.T. 9. E 00 L.T. 5. E 00 L.T. s. E 00 C5-134 L.T. 4 E 00 L.I. 4. [ 00 L.T. 4. E 00 i C5-137 4 ., E 00 L.I. L.T. 4 E 00 L.T. 4 E 00 BA-140/LA-140 L.T. 6 E 00 L.T. 4 E 00 L.T. 5. E 00 4 CE-141 L.T. 9. E 00 L.I. 7 E 00 L.T. 8 E 00

             ..CE-144                                                       L.T.         E 01 4                      L.T. 3. E 01  L.I. 3. E o!

RA-226 L.T. E 02

l. L.T. 1. E 02 L.I. 9. E ol l

TH-228 9. E 00 E.T. E.I. 8. ( 00 L.I. 8 E ou 4

             -                                                                                                       i                                                                                                 -

1 1 3 0 0 0 0 0 0 0 0 0 0 0 0 0 0 00 000 00 0 0 0 0 02 1 0 1 0 E

                                               -             0 D 0 E       E       E         E        E         E         E         E 0

R 3 E E E E E E E E E L E4 1 B0 . . . . . . . . . . . N/ 3 4 o 4 4 9 4 9 4 5 4 6 4 5 5 9 E1 s 4 1 9 v1 o . . 7 . . . . . . m 2 T. T. T. T. T. T. T. T. T. T T. T, L L 1 L L L

                                                                                                                                                    .              T.        T.                  T.             T.       T.          T.

L L L L L L L L L L L L L 1 3 0 1 0 0 1 0 1 0 0 1 0 0 0 0 0 E

                                             -             0 0 E        E 0

E 0E 0E 0 0 0 0 0 0 0 0 0 0 0 02 1 0 0 E E E E E E E E E E E 2 E E R 1 E4 . . . . . . . . 01 . . . . . . . 2 5 0 5 5 1 7 S 0/ 3 1 6 6 4 7 6 6 6 9 4 1 9 E T0 S C1 . . 4 . . . . . Y O 2 L T. T. T. T. T. T. T. T. T. T. T. T. L T. T. T. T. T. T. A L 1 L. L L L L L L L L L L L L L L N L A C 0

  )                 I
     .              P    5 t                O    Q n                T     K o                O    N C                S  )

(  : I 1 R K / E S l L A i N l I M C U

   -      M        M   P N B                A  (

G N E O R L D I E1 . B N T A t0 ) A A T o/ a T i0 ( S C1 1 D 3 1 . E l N l I i D r O d I y c n e g r e m e

5 e S I l
               -                   I                S                                                                                                                                                                                       b S                Y                                                                                                                                                                                        a Y                L                                                                                                                                                                                      l L                A                                                                                                                                                                                      i A                B                                                                                                                                                                                        a G                A                                                                                                                                                                                        v
A a 0 N E L U 0

e T A R l _ C C T 5 4 p E I C 1 m L N E 9 - a E - A s - L P s O N S m L C C 0 / 3 6 4 7

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0 o 1 A 4 0 9 0 5 5 0 0 1 3 3 1 4 6 8 N E 1 3 I 7 0 5 5 5 4 4 4 2 2 T 0 1 M - - 6 6 9 1 1 3 1 1 1 1 1 2 2 A - 8 4 - - - - - - - 1 - - - - - A A E - e O E O - - ) S R 1 G S K N C F C 5 R U u - 5 5 A E E A M a 2 2 B a l C C B C C R T (

p. w 4l ,! i1 1  !;l: i tj
                                                   =*                   =*        M       O O O O

a O O O O O O 3O OO OOO OO OO O O O O 3 o .. O o o o o c had tad had tad nad ned tad led and de nad ted tad E N nad had nad had and .ad t "* tad ,tae o e e e e 3% and N N f*1 O

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S est e e o T e T e T e te o in e T e tot e 3 e 8"t e e o

                                                                                                                                                                                                                                           @t e

U,,, se g e e idt e e e e e e e e >= e== a= p.= e.= t== to p= to t-o

                                                                                                                                                          >= >=

e t-e

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e se e e-e e

                                                                                                                                                                                                                       >= >=

o e e e o e e e e e e e e= e o e e o e o e M M M .d M =$ M e d =d M M M d .5 d M M .d M

                                                  ==                  ==       M O

e O O O O OO OO OOO OO OO O O O=*O O O O O O O O == O

                                                                                                                                                                                                                   .=  O OO           O ned                 ned      ned      nad      had                tad E                                                                           ned                had      tad       led      ted       too       and       led       ted        med       had       had 9                                                                                                                                                         one tad                                              **

e e e e o e e o e o e e e R est O N f*t O T T S T S T T P9 o e o e e e tad % ge T T T T @ 8"I O O WN and o o e o T e e e e e o e o e e e M O t== to pe 0= to o e e e e T. 9== >= De B= >e >=. >= >=.

                                                    .                    .                e        e      Be.          e       e      De.       >=.         e         e         e ime       t-d                    a .=             a        e         d         d     .5         d          e        a         a a         a        d           a      .d       =d          d O       O m          m       e o        b         o U

C C Cr te w 0 C E U fn ^ w ee H E

      -     d          d a s=4   e=4 Q   3 E         Q. E                     ==                    =*       M        O O
  • O -e O O -e 8 w O O O O O O
                                                                                                                                                                   -e       O O O                            =          e     N          --

g E O el e O O O O O O O O O O O O O has tad

                         ==                                                   and      nas nas e had               nad      tad      led       ted      tas       and      tas O                  >

lad 88 889 and nad ned and ned had m 4 E s-e e e e e e e e o e e

                         *=  tad %             v"t                                                                                                        e         o         e         e         e          e         e         o        e to  ze e-o                                 tn O en                     ids      se       tst ==             iA        e        T        .=e       e in                #%         .=         T                  .=

es o=4 O e.8 m E

  • e me o e o e e e e e e e e e e e e e B= >= >= >= p= t=

P,=0 e. e= a= >= >= >= >= e e M. . . . e=. e=. e a=. e e e=. e e-e e g .i.s a =e a a M a a d d e d a M d d e a e d X e-e Q O w es qvy e en me

                                          ==              gn GM              Da De              .d
                                          -d              4                                                                                                                                                                                     \

4 m S 4 '

                                   .. eg                                                                                                                                                                                                    I O                       E                                                                                                                                                                                     i i

tes -d 2 O e= 4 es U W em T in e-o ted == W S

                                 .d      E               tes                                                                         e                                                        4 e
                                  .4     tan             e.                                                                         e O       E               wt                                                                         S                                                         %

a W V %M 9 G *= 9 S S O 99 >== O ** T @ CO e= M 8% tA to

  • O W me M Pt T T T N N tad
                                 >=      g    a=                     g O eng to g estg teg te g S g

a a.e se sus ame a=e a=s N N 4 4 g e g .fut e e e e g g s e 8 4 tee 0 3 O ted O 3 5 3 3 t#9 t#9 4 O AB *= 48 G nd E W te. W N 0 tad tad 4 E N 5 m =* W W e W W m >= f 1 121

3 3 p

  • 3 =* 3 3 == == 3 0 e O O' 3 W "3 U 3-U 3 3 e e.o y e.,

g

                                               =            =8       w 3 u o                            3           3          m a o e
                                                                              =as      ins       ies      W              =ad       sad       nas      w         and          ins       =ad                    w saa                       a          a      w M                      M Net                 e     N           .         e         e          .            .         e         e        e         o            e         e         o 3 emp             4                                                                                                                                                   e          o e     N        N         N        N               N        N          O        d         N            N         N         .=

e e

                                          %                         3                                                                                                                                        ame        art       ==         ee are ind                    es os
  • w e e e e s e e e e e o e e a N ae == em = e= e. e.= = = s= e= s= == == = =

e o e 3 e e e e e o e o e o e o e o e d N ed =6 ed ad =8 e e

                                                                                                                                  .mn       =6           6      4            =0        e        ad          ed         a          ed         -e N        M        se       ame      me        ano             me       ans       me        N        .mo          em                  .mo 3 3 O ame                   ame        N          N         mie O O O O O O 3                                                            f3           O         O         3            3         3          3         3 tad     tea       w        tea      tea       tad             w        and       las      ans                                                                          w had          nad      esa        i.s         .ma        in,                  w Pam                       feb OE
  • M e e o e o e e e e e e e e e e
                                        %3                N
  • N N 9 N 9 N N se @ N N #st fug .e M e

ad9 5 O #wn OS se e som e o e e e e e e o e e e e e o e em N 3-m a= e== >= e== De em De De e- == De 0- De p= e o e o e a e o e o a= e e e e e e e e em0 M ed am0 em$ em0 and au0 ame ed =d f ==8 and d and d d M p-e (f3

d -

N

    -           w .

I *e Ua ime IER 2: >* Cf3 A* In3 md O* A  % H%-

  • a .me m O O me O - O O o O O O O O O e O O O O O OO O O eme u 5 m e N .mo
                 & O                        -                                                                                                                                                                        O O                  O e=         las          ins     taa      las      amo       ted       tas            tad      nas       had       ned nad               ins em          ese                  g'*                                                                                                               tad       tea         and        end        tea       t-s 4     N4                        #8e b*      OW iw
                                                           *
  • e
  • e e e W  % e O te rum N N N N s%
                                                                                                                                  *         *        *         *            *
  • e * * * *
                                       @3                         %                                                                                e N e                           f%        =e         e=e         ef't      == ==

OO

                                            .a             e     O           e        e        e         e              *         *         *        *         *            *         *
  • e ed >= w p. p= >= a= p= >= e= e. e= a= s= s= e.
                                                                                                                                                                                                                    >=         e=

e e= e tas e e o e e e e e e o e e o e e e o M eld M ed ed e em0 emE euf ed =0 ed euO and ed am0 em0 ed ed ed i l l l e e. e M ed 1 a 4 l se 1 tas 3 s= a O u e= idt T me een U O e ed tne e auf & 4 O t#9 O ed u S  %

                                                                                                                              %         M         te                 w            N         O          me          e         @

i T O S O el tad N O eft eft edt O O me M M @ W W N N tdt eft 49 43 S suo see M amo og me se e= e 9 s e e e e sue N N e e e me e e e e 4 tad e WO tad O E S W e e e O O ad E u 3 3 e W 4 tad nad 4 2 to nas u N N e m == u u e u u a == i l l i I 122 1 __ _.. - _ _ , _ _ _ , . - - - - , . . ---- -- ~ -- - - ~ ' '

1 l l l i

                                                     == m O O                                O              O                 e     == g O                                                    N 3            O O O O O O O                                          @       O O O O O                                 O O O O O m            nas     nas    ins      ins             w tas          W               W       W
                                        ==                   me and                            nas                      nas nas          w            tad      w w w es O e=                 . m. .               .       .       .      .       .       .       .       .       .         .       .            .
                                   %4                S       O   S S N 4 N                                  S       =e      @       S e >=                    M
                                   =* u                      *e                                                                                                            N        4 N **

sue ina . O . . . . . . . . . . . . . . . 3 == a= to a =. . >=. a=. . e. >=. a=. e=. to. . >=. e=. t-

                                                                                                                                                                           >=.

a= e-. a=

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                                                                                                                                                                           -d         a w

a US 1

  '          N t/1 a        >*              ==
       . A                e u                      a         3           =.      M                        **             == O                    == =*                             =* == ==

g a w e O O O O O N =* e- == O O O O O O O ins a w tas nas nas nas nas w ins and one and and ins 3 tas s= en ans nas ins nas nas V ** U e e4 nas E N e S Ow . m. . . . N &n b a 3  % in O tA e N en

                                                                                                   =e e4  p-e         %      S     s=* 3                     40 em      pm. 9       to to te                  N            me       w          me     ==

g b == =* O g u a =# . e . . . . . . . . . .

                      & O              w           to             >=       t-      >=      t-                             >=      e=
                     =mp   ==         ene             . e.        e        .       .       .    >=. >=.

em. > p= >= >= t= t- >= O'" e . e e . N M w N ed ens .ms . =a ema e.# ed aus gma e.s 4 ems .as ed -d -s d e n= M Y

                                             ==

M es e 4 S 4 S tas S 3

                                >=          m                                                                                                              O W           >=                                                           nn e

las W s.e

                                =s 9                                                  e tas                                                           e
                                 -8         en                                                                                                             4 O           M                                                            e                                                 =s W                                                                        S                                                 %

W G

                                                                                                         %       M       e               9        8*.      O           so       w        @         ee i                                                                            e S O             tA     te                      sus     M        M        9           W        sqP      N         N tes Pm 4

O T 4A 0 tA 8 tA 8 t$ 4

                                                                                                  @      S       .e mo     see     M       sme      se       se          =e       ame      N         N 4                                                                  4      4       4       8      as        t        9       8            8        8         4       6 O

led 8 E O Las O E 5 3 3 8 M M 4 las nas 4 E ta e ad E u te. W N pe g g me u y a u u a >= 123 1 1 -- - - - ' -' ~ ~ ~ ~ '

N M .e -e .= -* -e 3 O

                                                                                                                                               .e           .= s                                e          e         se 3 O 3 O O O 3 3                                                                                   3         0 m o a o o o e        .y        .y tA                tes        tad        nas         tea          tad         .ad          med         ted          nas en                                                                                                                            ned        ind        tea         and         .d          w w                      a         .d 4                            e he                       e       M              e           e            o          e             o          e            e           e O                    N
  • N N 9 N 9 N N N e e e e e e e .
                                    %O                               O                                                                                                            9         N           fnd         M            gr         as         e v 4A tad                            *e gg                       e        e            *
  • e e e e e o e e e o= >= e e e e
                                         ==                          in                     e=           >= >= >=                             e=           >=                                                                                                        e g                   e          e          o            e           e           e            e a=         e-         >=          em          e.           e-         >=        e=           n e            e          e          o          e          o                                   e
                                         >=                  a       M          .4           .J           -d
                                                                                                                                                                                                                       .           .                     e           e in
                                                                                                                     .J           .J          d            .4         .d         .e        .J           .J          =a           .J         -J        d              a
                                                         **         M           3 O                     s=e        O o O O O O O O O O OO O O O OOO O e                               me          =e                      O                    s=e          ao        N O O                              3 O
                                                                                                                                                                                                                                                                ==e E                 '  '"'   "           
                                   ~.                               e OO                       e       N
  • e o e e e e e e e o e
                                   %                     in            e      64                                                                                                                                                 e          o         e            e tse ned                         O to          .=e         e me e te w                                                 me        ta e                     N         s=e          w **                   a-o O ps                             se me                 e       e             e            e           e          e            e            e            o         e           o         e           e           e            o          e 3               >= S                  e=          a=           e=         >=           km          a=            e=        a=          >         a=          >=          e-e            e 3                  e          e          *           *            *
  • e
                                                                                                                                                                                                                            >=           >e        **          e=

e e e e o e o e =

  • d N e .J .a a a .d
                                                                                                                                                         .J        .J          =a        .J          =s              a      =6           .J        -d              a g                                      ao         M          O O O O O O O O O $

ame m x e=e Q O O em O O suo s=e me N a-o U N e We

                                       ==

O O O O O O O O O O O A e M E tem tee tad led tee tais led led led tai had tee led led tad tad led had had siJ = m N e= , M > 04 e M e o e e C O g a %u e O e e N N e e N 4 e Ob e fee o N e e e 9 S ** N te N == e e e e e U e'** e las ee V ** U m e 3 3 e e e e o e o e e o e e 3 >= se o e o e e M M  % S

                                      -e e                  o M

e

                                                                                         >=          a=         a=          om           a=            em        >=          to        to          >= >=                  em           e=        a=

o e= N M b == M e e o e e e e o e e e o e e e e e-e N u a .d .a .d as .a ed -d .J -e .d .J .J =e .d me =a .e l b & O g w

                         ==

M N 4 we n 4 H U M O O O e O O O O O O O O O O O O O OO O O O O O e me 3 .,e N e e O O

                                     =e              tad        tad        had         nad          tad        bd          had          had           nad taa               tad tan e=

e tes tea tee led led led tad M Ng e e e o e e e e . e Ou te O @ @ N N == te

                                                                                                                                                                   .                     e           e           e          e            e         e           e
                                 %                               es h         4A          N e to ==                                    ao           its       == =*

W5 3 OO e e e e e e e e e e e n= e o e e

                                     .J e

e 4A e o= o a= e e= o= ee >= a= e= e= a= e- >= >=e >= o= e

                                                                                                                                                                                                                                                            >=

e e o e e e o e o taf $ N e e o e e 0 $ 0 ed e.d e.J

                                     >                                                                                         $                                ed          d         5.0        e$              e       e.0          e.0       ed          .J             e e

ce M

                                              ==

W ed 4 3 4 S E tas S i e= es O 4 u >= 4A e les u s.e

                               .d                                                                                                      et                                                                     e has e
                               -d           &                                                                                          S                                                                    4                                                                 i O             We E                                                                     .J                                                          .

l u  % M te

                                                                                                                                                                                                            %                                                           e    i W                             W          G            S O                    4A            4A          O O                     pe 9

M h M O me W 9 to G tad Paa O 4A in in te e m we a=e M == 9 N N a= e e e e me s=e e == N N 4 e o e o e e ee e O tea e WO tad O 3 a 3 3 e W e a e e e e e .= u u e u u aW 48 e ks e 4A 4A qad tad X E u nas u N N e= i 124

N m =* me .= == m

                                                                                                                                                                    .                        -e 3                  0 3 O                                                                                                               N .=                                                      N         N e                                                      O 3 3 3                                       3
  .                                                             ==                 tad       tes        tea            ina        w         ted         .ed         es 3 3 O 3 3 3 O c o o 1                                                              g.,                          Je                                                                                   had        tad       es            tea         ud        tea       es                    w and                  w
                                                                >=

gag . m. . . . . . gy =e c e == m ame N .* N me

                                                            %                                *e                                                                                              se                     ==                     e m ==                          N         N
                                                            == ned 3                     . a                   .            .          .         .           .           .             .          .

a >= w e- >= e= e- >= >= >= e- >= a= a * * * * * * * * * *

  • e-a=- >* >= =
                                                                                  .d        fut         .4            .4         w         .A             a        .d               '
                                                                                                                                                                                            .J        .d            .4             a      .J        .d          -.a       .J            a n

4 3 m = m O O == O == 0 == == == O O == == =* N == w a a ena w etas o atad o o a a o a e a o a a a a e= 4 tea tea med w w w tad ned nas ins tea ts i.s i.4 e4 oW . m. . . . . . . . . . .

                                                           %                    e O                 N                                    e                                                                                       .         .         .           .
                                                           -. 3                            ee
                                                                                                                    # N                              N          e =* e                              N            N            N         N         N          A          a          =*
                                                           =* O
                                                              .d                           -e            .             .          .         .           .           .             .          .

w . . . . . . . . D e- to e-w . e. . >=. a=. e=. . . =. e. >=. e= e.

                                                                                                                                                                                                                                        >=
e. >= >= n=
m. .a m .a .a a .4 .4 .a .ms .s .a
                                                                                                                                                                                                                 .a           .a        .4        .4         -a         .4        s M

M N rn e m >s 2 e o w 4.a e= g w e O 3 tad U e so .. U ,m S"

C M  % e n m 6 .=
                                                                              .* m o a                                                  o == o o
                                                                                                                                                   * * * * * *e o* * * * *N
  • w N -. .* =e g

I b N "& w E

                                                   ==                         * * * * * *nas ans i.e        ned       tea            tea        tea
                                                   >=                                    tab tad            tea        tes       tea          tes           nas      tad        w         t.#        tas       .ma W                                  4 e

e3 OR . e%.s . . m %S e e ce N N N e N as e O .= e N N e m N e == == se g

                                                                                 . m                 .               .          .         .           .          .              .          .         .            .            .         .         .

em >= >= . . .

                                                                                                                                                                            >=         0          em
                                                                                 .       T.          .            >=.          .       a=. e.                >=.                .         .          .        e.
                                                                                                                                                                                                                            >=

a=

e. >=.
                                                                                                                                                                                                                                                                      > >=
                                                                              .d         N        .d              .d         e.a                                                       .a
                                                                                                                                                                                                                                         .                               .         e and         em0        ed             aus                     a a                    aid       .mus         a       e.d        ed        a N

3=

                                                                     .d 4

3 8 i t 4 1 O 1 w N W

                                                                    .I
                                                                    >=

i idt e les W S

                                                        .a          tes                                                                                                                                                               e e

w e. e 4 O 4W"l 3 a W  %

                                                                                                                                                            %             889                               e              N         e 9               e S S                            til       til           G e *.* M te 9

ao W e e e ted N O eft 889 9 N N til til 44 49 S se ame m em 1 ese n= see sue N a 9 e e e o e o e e se ese N 4 tee e g O nas O S e e e e e a e e e o e 3 3 s M M 4 nas tes 4 3 ad a W te. W N N e W ** W W S W W et >= 1

                                                                                                                                                                                                                   +*
\

i 125 i I I

. TABLE B-13 BROAD LEAF VECETATION: IODINE-131 AND GMetA ISO'IUPIC ANALYSES (pCl/kg WET) STATION NUNSER BLS-1 NAACM NARCN DATE COLLECTES: 03/04 03/26 BASIOCNENICAL ASALYSI5:

l-131 L.T. 5. E 00 L.T. 3. E 00 GAsueA SPECTRUN ANALYSIS

SE-7 6.39 0.72E 02 3.931 0.97E 02 K-40 5.40s 0.54E 03 5.264 0.53E 03 sen-54 L.T. 7. E 00 L.T. 9. E 00 C0-58 L.T. 8. E 00 L.T. 9. E 00 FE-59 L.T. 2. E 01 L.T. 2. E 01 o C0-60 L.T. 7. E 00 L.I. 1. E 01 Zu-65 2. E 01 L.T. L.T. 2. E 01 2A-95/98-95 L.T. S. E 00 L.T. 9. E 00 RU-Is3 L.T. 8. E 00 L.I. 9. E 00 A0-106 L.T. 6. E 01 L.T. 8. E 01 ! l-131 L.I. 1. E 01 L.T. 1. E 01 C5-134 L.I. 8. E 00 L.I. 1. E 01 i C5-137 L.T. 7. E DO L.I. 1. E 01 1 BA-140/LA-140 L.T. 1. E 01 L.1. 9. E 00 CE-141 L.I. 1. E 01 . L.1. 2. E 01 CE-144 4. E 01 L.T. L.T. 7 E 01 RA-226 L.I. 1. E 02 L.T. 2. E 02 IH-228 L.I. 1. E 01 L.I. 2. L 01

l l

                                           =               N O                                                    O = O                          =e         O O =* = O                                        O             .ie        ==

O O O O O O O O O O O O O O O e N == O c Q tad w wM w w w w w ame tad .ad and tais w ned ud w w w w* g . N. e. . . . . . . .. . . ind N we Q O N . . . . 5% N NW N W S N N W N as N @ N N 3 es 40 g . e N . . . . . . . . . . . s= S > >= >= a= e. a= n= n= e= n= e= e e M. . . . n=. . . . e e e n=. >=. e=. s== M N N ed M M ad ed M e . . mid ed ed ed M - eud and ed ed mus me N M se see suo eo se e-o O O s=o N s-e me sme =e me N N ==. O O O O O O O O O O O O O O O O O w tea te,s led w w tad is.s w w w tes d til ned ned nad had nad e w M 9 8

                         >N                 ,           0%.

M (% me me O suo g M Ed see N g me N es g sue N N M m M M g O

                                                         *
  • s.e
n. . . . . . . . . . .

e.- . . . .

                                                                                             >=      >= >=                                                                                                                                 .                             .
                                            .           e.       e.               e.            .         .          e     e=. n=. >..                     n=. o=.            >=

o.

                                                                                                                                                                                            .         >=. ==. e=.                                            .=

ens O O sum 0 M ed ad em0 aus ed M and ed ad gud ed eu0 ud ed E m o O.s

          >        =*

e e-( & e U H m a C M au - o S

              - e w

e e n .s M "> d M  %'

              .= 3 l

I b W E O M M .e we

    $          & 5                     O               O O O                               O me        me         ==        me        me         N         se                  s-e          me         me                      N                 -=

M uns 3 w O

                   ===

tad O O O O O O O O O O O O O O a a e= tais les nas M ned led tad w w and and ned led ned tes tais tas e <

                             ==                       .m had                          ans 4                   W
                        >O                e               . N.                  .         .          .

N 4% Se v O O ce N M as M N N we oft N M N M e-o M e M M S M o * *e

         #=4
                                          .           N        ==                   .         e         e          .         .          .         .         .         .         .
                                       >=.                                       >.        M.                             D=        a=

em. .= .= >= g N. M. . . n=. >=. . . . . . em a= em a= em >= hl -8 ** * . . . . .

                                                                                 -8        =8        -8         =*        -d        -d         -8                    d 5
                                                                                                                                                         ==8                    8      -8           -8         ed
  • d -d 8

o-

                                   ..            M M              ==

a em e M > 9= =# ed 4 4 5 5 4

                            .. g S                     E nas      d            2
                           ==    4              S                                                                                                                                                 O W     W              e=                                                                                                                                                9 taf   ==                                                                                                til                                                           me W                                                                                  G ens   E              tas                                                                                                                                                 e
                           .ns   tes            a.                                                                                 e e

( G 2 e a e W nd  % M G *e W W 9 O 99 9 N O me W W e ted am M mm O ngg eft tft tft O O se M M @ W T N N a= O ** tag @ q S se ame M sus sus a-o e W e e e e e o e

                                                                                                                                                                                                              .mo          ao         N N 4      4     e        4    ned        e W G e        amo        e         e            e           e           e          e                 e S      e    .* W                                                          and        O S                 E          3 3                  e        M         M          4            tad                     4            E e ad E W                                       en.        W         N         N e m == u u e W had W          m >=

127

_ _ _ . _ . _ _ - - . - _ _ = . - . . _ - . ._- .- - . - _ _ _ _ . . _ _ _ _ _ _ TABLE B-13 (Cont.) BROAD LEAF VECETATION: IODINE-131 AND GAISIA ISOTOPIC ANALYSES (pCl/kg uti) STATION - BLS-1

JULY AUGUST OATE COLLECTES
SEPTEh8ER 07/31 08/28 09/24 R ADIOCNENICAL AGALVSIS:

1-131 L.I. 7. E 00 L.T. 4 E 00 'L.T. 5. E 00 SANetA SPECTRUN ANALV515: j 3E-7 2.27 0.24E 03 1.47 20.15E 03 4.69 20.klE 02 K-40 4.28: 0.43E 03 i 6.03 to.60E 03 3.94 20.40E U3 885-54 L.T. 2. E 01 L.I. 1. E 01 L.I. 8. E 00 C0-58 2. E 01 L.T. L.T. 1. E 01 L.T. 9. E 00 j [ FE-59 5. E 01 L.T. 4 m L.T. 3. E 01 L.T. 2. E 01 CO-60 2. E 01 L.T. L.T. 1. E 01 L.T. 1. E 01 25-65 L.T. 5. E 01 L.T. 3. E 01 L.T. 2. E 01 2R-95/58-95 L.T. 3. E 01 L.T. 1. E 01 L.T. 9. E 00 au-103 L.T. 3. E 01 1.

,                                                                                                                      L.T.        E 01  L.T.                                               1.                E 01

] RU-106 2. E 02 L.T. L.T. 1. E 02 L.T. 8. E 01

l-131 L.T. 4 E 01 L.T. 3. E 01 2.

L.T. E 01 C5-134 L.T. 3. E 01 L.I. 1. E 01 L.I. 9. E 00 C5-137 3. E 01 L.T. L.T. 1. E 01 L.T. 9. E 00 SA-140/LA-140 L.I. 4 E 01 L.T. 2. E 01 L.T. 1. E 01 CE-141 L.T. 5. E 01 3. L.T. E 01 L.T. 2. E 01 CE-144 L.I. 2. E 02 L.T. 1. E 02 L.T. 7. E O!

                        ..RA-226                                            L.I. 5. E 02                          L.T. 3. E 02   L.T.                                            2.                   E 02 TH-228                                            L.T. 5. E 01                          L.T. 3. E 01   L.I.                                           2.                    L U1 i

i

o N m O me me == -e me se s.e m o me se == O O o o o o O o o o oN o eo e e w O O O O O O w w tad ine nad w nea w g N -N te.s ned ind w w nad ina w ind w tad me S W e e e e e e e o t es% T O O 9 s=* N ee 8"5 a=e s=8 9 N s-e e o me e e e e taa N et *e s=e N e N N Wee gna S e S e e e e e o e a em s.e se he one em em em e.m >= o e se e e e e e o e y e N. . e e e o e e e.m em aus >= eum em em e e o e e e e e eh & Y e o

                                                                                                    &         &          md        &         &          &          &          &         ad         &          e.$         nad       &                &          &         e.O Q                N          fut         see       e-o         one      .mo       e.e         me         me         N        me          se         s=e        sus O                O          O                                                                                                                                            a=e           N             N         s-e es O O O O o o O o O O O O O                                                                                                                      O Q                     Q gna               n.e        w           and       ses sea nas ned                                       nas w                                     w had @                                           s=s ned                            ned         tes                   ins        ned          w              naa      ses C/)

153 IN% tes se en o e edl e o e o e e e o e *

  • e e o e e

(#3 as == f*l o N N @ MW M f"5 N @ M 8"9 M @ N e

                                                                                                                                                                                                                                                              @         tA y                   o                                               M g                   a                      .               . m                     .         e          e         e         e -         e         e          o         e          e           e          o         e e.-

e

                                                                           >- o >-o >-

o e e

                                                                                                                       >- e
                                                                                                                                 >  e m-o e-e
                                                                                                                                                                 >- >- e                          > >                  e.         e=           e=

e e-e e e e e e e o ed e.d d e e ed ens ed e.d ed ens & a.d ed ed u.O $ e.O ems aus & se X U C o=*

m. >=4 Se ad I-* O .e C M N -e e O H Q >= m u W m g &

m O O , ., e e e - e N I o e

                                                                                                                                                                                                                                             ~ ~ -

M

             $ne d

u == O tea o o o o o o o o o o o e o o O o o o Q a e- .i.e

                                                                           .e i.a e           and       inn         ins      ans sea               tad        ins        ned      ins         sea       and         ins        e.s        w                         i.,

la3 m.J w 4 E 9

 ,,,3 g
                               >     wo                     .            8'.l          e           e         .          .         .         e           e         e to gm               e                  o o                       e      me          m        me        m .= N e

m

                                                                                                                                                                                       .                      e N m e          e eo              mm e        e e- o                                 *e         es W                       u se                   e            e.e        @              e         .          .                              e M

8 m"4 o s= N e= a= a=

                                                                                                                                         >= >=

e e o e e o e e e e M e o. e e e e .>=. e e p= e

                                                                                                                                                                          >= >=

e e e= o e- >= e- e= e= e=

                                                      .a                 8"t        w              a      .a            a      .s e           o         e              e            e       ..

t I # d e s .s a a a a & .e a p., 8 e.

              *                                  **                %A 44                 a.m me                 sn to                 am 3"                 ed ad                 4 4                  S ee o

g 4 o 3 tes -d 3

                                        >=      4                 m                                                                                                                                                 O W       W                  e=

4A ans == W me

                                        .e     E                  ime 9                                                                  e e
                                        .d     tes                a.                                                                                                                                                4 o       3                  to                                                                               et as a

W W %M eg W N O W a=* W G S o 4A en o e me seg m g me e e Ne tee a=

                                               *=

0 M a=s N o g tA en tA @ tG S s=* s=0 M s=8 s=8 ** ** g g a=o N N N e e a e o e e e e ese 4 4 e 4 tes e o e e e e e o e o e == W e ad u 4Ad e S E 3 3 e M 44 4 and led 4 2 enn u N N e e me u u e W w a >= , I i 129

a ~ M a a - a a a e a a a a a a a a e aa aoa a- a a a~ a e o tea w w naa w w w w w w naa w tes w w w 3.

                                                  ~
                                                   ..   .,                                                                                          taa                     w w um               .                 .                        .      .      .                              .

4M M a o ~ - ~ -

                                                                                                                                                            ~ ~ ~ ~

ma .

                                       .               ~          .       .        .      .      .      .       .       .      .        .      .

a . - .

e. -
       .                                                      s a s
                                                                                              .4 s

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       .J m   o M
a. C.
  .=   a.          .

e M >* O C -a o - = o a a

  • u
           -                       *             * *
  • I-o = * * - * * * * - * -* o* o* -* -= -= ~= -=

n h 3 w ggw w w w w w w w w w w w w w w w

            . -       z.                         .. .

M as 5 Wo . . . . l b  % S 8% eS a a G G N O N g .d2 ** 4M O O h N O @ e.e om. sn N o g Q W

            & a W   Sa                         es es g        w ==*
                                      .         e e             .       .        .      .      .      .       .       .      .        .      .       .
  • J Q . . .
                                                             >=. >=          >=                                                                                                      .

88 a= e=. e. h. . . >=. e=. >=. t= a=. p=

                                                                                                                                           >=.
e. - >=

4 q 4 .a a w .a a a .a .a .a a .a

                                                                                                                                   .a
                                                                                                                                      .              .       . e=. e.             .

I.m e a e w .a -a .a W9 . N M O M 1 W 2 e 8

                               ..          tv W D          m.t wg W9            >
                              >            ad
                              .a           4 3

4 S

                          .. 1
  • 5 w .4 2
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tes a. W @ af E ted 9 e y w tw E

e. e 4
                                                                                                                                                 -a en                                                       S W    tal                                                                                                                 N S    **                                                               %M             t@              w       h      a         e     w e e W        W       G       a en          tA     O       W       me      est            9               W tad
                        >=
                             ==

S M me N a tA tA tA te @ S eme ame M me .M.e me .e N N N N e W 4 e e o e e e t me e

                                                                                                                                                                 .=.

4 e 4 m 8

                                  ==      48 tes e ad e     W E

aW tea w w a 5 m 3 3 a W9 a WS 4 e e ene e nas 4 e 3 e N N e m == W W e W W m e= l 130 l

m N M O O 3 me O me O me =a me O O == -o == N W O O O O w w w O O O O O O O O O O O O O O e

                                                                                     =e ed e

ned nas w w ind ned w ned ned w w ia w w N e . M. e e . . . e . . e e == O O e e N S N S =* N N 3 e ned N s.e N e N N m% en ee 30 e o m e e e o e o e e . e e e e e

                                     =3 e                      e,                    4                >=              e=         to         a=       em         se        >=        em
m. e e . e e e e . s=.

e= e a= e. e- >. n=

                                                               -J                   M         M           d
                                                                                                                                                                                                                          .                                  .                   .          o a          a       .J           d      es        .J         -d        .a            e            s          d         .id        ed                    a       .a se                   N         sul     ame            se          me                             ce O                    O O ame      ame                  me        N         as         amo          see        ame          me          ena           N .=

O O O O O O O O O O O O O O O O had ned ina w ned nas w nas and naa nas W ned nas ned nas w w est ned a e m N a- N e e e e e e e e . t/3 aC % . e . e e . e Ca3 3 68% a=* me O .** == w N T we N se 9 ** N N m ** M e M m O w a p e e e e e e e e e e e e . e e d t= w e= >= >= e- >= to to >= a= t= a= o e . . e e T. e e e o 0

                                                                                                                                                                                                                                             >=,        >=

a e e e e e . o e n=. n=. e N a a a a a a a a a a a a a a . a a E U ""

     ^       C      M
  • M Ge a a H O e c H a O H< Q *= e U Ca3 us nas tan v 3 e M

m b r.E

                        %                                  O                      ~        s.9 1
                        = m                                o                                       O O .* O =* O                                                          e                   e       O O                      .e                                  ~ .=

N u O

                         & =*

O O O O O O O O O O O O O O O O O O tad C&3 M w e= had edt nas 49 ned ned tad w tad tad had nad sad ned ted ned nas had nas has

     .2                       4         ==                                        ee g             .c.       a=    >O                          e                           e.

4 q M {% ist O O N e N e o e e N e e e

                                                                                                                                                                       .e e         e e m as a e          .            .          e            .

e H C O , .

                                                                                                                                                                                                                              .e          N                      N                   ==

ed M N M

                                                               .                 N        et          .              .          e           .        e          .         e        e         e e=                                                                                                                                           .             .          .            e v4                                          e M

e 49 >= e e-e

                                                                                                                              >= e e e         o
                                                                                                                                                  >= e
                                                                                                                                                            >= e
                                                                                                                                                                      >=e >=o >=e                    em            a=         e'=         em          a=

e n= e

                                                                                                                                                                                                                                                                                     ==

e l ad te e ed .J me =# .A .J .J o e e o e . e Ca3 s e .J -d as # es .J .J E N Q C w

                                                 ..                   M e                                    M                      m.

em mA M >

                                                >                     a
                                               .J                     4 44                     8 8                      as
                                       ..      eg e                               5 tes      .d                     3 s=       4                     m                                                                                                                                                       O W        u                     em                                                                                     eft 9

nas a. W see

                                      .d       E                     lad 9                                                                 e a                                                               4
                                      .e      nas                    a.                                                                                     e O         3                     to                                                                                                                                                      .a u        w                                                                                                             a                                                                %

O *= w O m O efe

                                                                                                                                                            %M eft q                   w           s==

O =* w e e w - e N O e me M T w w N N 0- O a.te e O est

                                                                                          @        e e e e e e e           e se        se        sus       . set e         ce           ==         me           no         N                   N

( 4 e 4 nas e WO tad e O 3 e 3 O o e 3 e se e t#t M e e e e e s SW == m e ad E W na. WN N e EE led had *C E e e == W W G u u a e-5 1 131 i I

                                                                                                         , _ _ - _                    _                                                                        - ,                       - -                     - ~ , - . - - -              , - _ , - - -

O N M s=e O ** O == se == me se == -e O O O O O O O O O O O O O O

                                                                                                                                                                                                                                       .e         N O O O O                              :3 m              and            nas w w                  ned       nas w w w                              tas       ins      w w w w ens                            O       N                                                                                                                        tas          a w                a g                        P%       N                                                                                                                                           e

' t age e . e e e e o e e e e g o e e o e o e e ens % N Oge O se G N e N a- a ==e =e e N se s.e == N N N

                                                              &O te                                                                                                                                          .,.ee nas
  • M N e e . . . . . . e e . .

to e= 889 h e= to t= em 0- e= >=

                                                                                                                                                                                                                                .         . 3                e e                                                                                                        >         De       p.e      e.e     I.=      em         %        0.e as            W o

N e o e e e e o e a=. e e o e e e e e

                                                                                                             .J      .d        -d                                                                  .a
                                                                                                                                          .4        -d        .J      .J       .J           s                  s       d     .a           s      N        w O             M         M       ** =.*           me          == ==                  e    ==e      N         s.e                == ==

O e e N N .e O O O O 3 O O O O O O O O O O O O O em G ins ins 8% ned til w w w taa nas naa w nas ins nas ned nas w ins w tas 14 N N G*e 3% e e e e . . e e o e e o e e f#3 OO tA O O s=e se M me M po me me #=t ** s=e N M e me e e e 3O ge se M est 4

                            >3 e

e% e e. e-e s= e D. e

                                                                                                                                        >=

o e.e e

                                                                                                                                                          ' >= e
                                                                                                                                                                   == >.

e e o.e e e-. e e e.e e e e= e em e

                                                                                                                                                                                                                                                        >=

N 8"t e i .J =J a .ns .e .e -d .d .a .d .A .d .d .d -s .d 4 1 ee X U

                ^

e O M M b W W .e 4 s.u. 9 Bue @ g * .s fe, m as O N M S O -e O e O O .* == c S l b  %

  • g O O O O O O O O O O O O O O
                                                                                                                                                                                      .e                          -e O O O O O
                                                                                                                                                                                                                           -e       ==         N           e W        ==                           w             imp w             tas ins w                   ins        ins       w M                     & >*                                                                                                                          ins      w tas              nas       ins     nas      6a       w          tas      nas
                       .3           -                            -e St n         .ee ed          O                 4.e e             De d't           e               e       o       e       e         e          .         e         .       e        e         e

} N .d % W O O G e . . . e o e I Sh P% N S N G W @ a=e s=8 G a=e N @ N N

                                                            *1 O                         es        to g                                                 e           e O                 .       .         e          e         .         .       .        e         .         .        .

P1 >=

e. ee e=. o= o= e- p- e. e. s= e=

e= s= o=

                                                                                                                                                                                                                                                        ==

a e se e e o e e s=. . e e a=. a=. e e e e

                           '$'8                                                                           -d         a         s       os         .a        .d     .d        .a       .d       .a        .a       .4         a      .a         -J       .d E

M i 4 8 M i e se es ' to .spg

                                                                      =           m N            D De          .d
                                                                      .e          4 3

ee 4 e 3 nas -d 3 e e= 4 e W W == e tA ** tas == W e e ad 3 tas e 4

                                                                .e   tes          &                                                                        a                                                     .a O     2            t/t 3                                                     %

4.# W  % M S 9 8% O ** W 4 S S =* T S e O eft eft O me M M @ T W N N tas == M N O eft te aft O e e me .S e M se se as we e N N 9.e O em 0 9 0 0 $ 0 0 0 $ $ sue G $ 9 0 4 4 0 0 0 e led 8 O O has O E S 3 3 M 4 e s == W e ad E W te. W N N S e == 9 WW t#3 GWW nad nad 4 5 2

                                                                                                                                                                                                                                                       >=

1 132

1. _ _.,.___ _ _ _ _ _ . _ - - - . _ _ - . - - --~- - - - - - - - - - --- - - - - - ~ ~ - ~ ~~

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  • e M"e s= N amo s= >= >= em >= e=

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                                                             >=               .=.e                       e        9            e est           s=e           ao          en       ee        en       N       N i                                                             e      S            e                     w e        e     e       e         e       e         e          ama              e             e          e       e         e        e       e
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                                                                                                                                                                                                                                                                                 ==

+ I i i 133 i (

i i i TABLE B-13 (Cont.) BROAD LEAF VECETATION: 10 DINE-131 AND GAISIA ISOTOPIC ANALYSES (pct /kg WET) STATION buRSER SLN-10 1 JUNE DATE C04LECTED: 04/26 BASIOCNENICAL ANALV5IS: I-131 L.T. 1. E 01 GANNA SPECTRUN ANALV515:

SE-7 7.20s 0.72E 02 K-40 5.03
0.50E 03 Na-54 L.T. 6. E 00 l E$

s- C0-58 L.T. 6. E 00 i FE-59 L.I. 2. E 01 CO-60 L.T. 7. E 00 1 Zu-65 L.T. 1. E 01 la-95/me-95 L.I. 6. E 00 s 38-103 L.I. 7. E 00 RU-106 L.T. 5. E 01 1-131 L.T. 1. E 01 C5-134 L.T. 6. E 80 C5-137 1.35: 0.50E 01 SA-140/LA-140 L.T. S. E 00 CE-141 L.T. 1. E 01 CE-144 L.I. 4. E 01 I RA-226 L.T. 1. E 02 TH-228 L.T. 1. E 01

TABLE B-13 (Cont.) 1

  • BROAD LEAF VEGETATION:

IODINE-131 AND GAMIA ISOTOPIC AllALYSES { (pCl/kg WET) STAil04 - SLN-10 JULY AUGUST BATE COLLECTES: 07/31 SEP TENSER 08/28 09/24 R ASIOCNE NIC AL AGALYSIS: 1-131 5. E 00 L.I. L.T. 4. E 00 L.T. 7. E 00 SANNA SPECTRUN ANALYSIS: SE-7 1.012 0.14E 03 1.39 av.16E 03 1.28 AO.14E 03 K-40 7.31 0.73E 03 5.71 20.57E 03 6.79 so.68E 03 Ne-54 L.T. 1. E 01 L.T. 1. E 01 L.T. 2. E 01 CO-53 L.T. 1. E 01 L.I. 2. E 01 L.T. 2. E 01 [ w FE-59 L.T. 3. E 01 L.T. 4 E 01 L.I. 4. E 01 l CO-60 L.T. 2. E 01 L.I. 2 E 01 L.T. 2. E 01 25-65 L.T. 4. E 01 L.T. 4 E 01 L.T. 4 E O! - 23-95/ma-95 L.T. 2. E 01 L.T. 2. E 01 L.T. 2. E 01 RU-103 2. E 01 L.I. L.T. 2. E 01 L.T. 2. E 01 au-106 L.T. 1. E 02 i L.T. 1. E 02 L.T. I. E 02 1-133 L.I. 3. E 01 L.I. 4 E 01 L.I. 3. E 01 i CS-134 L.I. 2. E 01 L.T. 2. E 01 L.T. 2. E 01 C5-137 L.T. 2. E 01 L.T. 2. E 01 L.T. 2. E 01 BA-140/LA-140 L.T. 1. E 01 L.T. 2. E 01 L.I. 2. E 01 CE-141 L.T. 3. E 01 L.T. 3. E 01 L.T. 3. E 01 . C

                                  . E 144                                        L.T. 1. E 02         L.T. 1.       E 02    L.T. 1    E 02 RA-226                                        L.I. 4. E 02         L.T. 3.       E 02    L.I. 3. E 02 IH-228                                        L.T. 3. E 01          L.I. 3.       E 01    L.I. 3    E 01

3 i TABLE B-13 (Cont.) BROAD LEAF VEGETATION: 10 DINE-131 AND GAleIA ISOTOPIC ANALYSES (pCl/k9 WET) STAil0N NUNSER BLK-15 NOVEMBER DATE COLLECTED: 11/26 BAORBCNENICAL A4ALYSI5: I-131 L.I. 6. E 00 GANNA SPECTAuN AWAl'f.151 SE-7 2.15 0.24E 03 4 r. E-40 7.412 0.74E 03 l c$ Ne-54 L.T. 2. E 01 C0-58 L.T. 2. E 01 FE-59 L.T. 5. E 01 CO-60 L . T . ' 2. E 01

;                                                      25-65                                              L.T.      5. E 01 2R-95/st-95                                       L.T.       2. E 01 RU-103                                            L.I.       3. E 01 20-106                                            L.T.       2. E 02 i

I-131 L.T. 6. E 01 C5-134 L.I. 2. E 01 C5-137 5.33t 2.14E 01 SA-140/LA-140 L.T. 3. E 00

                                       .               CE-141                                            L.T.      5. E 01 CE*144                                            L.T.      2. E U2 NA-226                                            L.I.      6. E U2 IH-/28                                            L.I.      h. 1 Ol

i TABLE B-14 FOOD /CARDEN CROPS: 10 DINE-131 AND GAlttA ISOTOPIC ANALYSES (pCI/kg met) I STATION - fPP 50f SEA 45 SEPTENBER DATE COLLECTES: 09/I7 j GANNA SPECT8pN ASALV515: St-7 L.T. 1. E 02 E-40 9.33 se.93E 03 Ne-54 L.T. 1. E 01

r. CO-50 1.

w L.I. E 01

       'd FE-59                                             L.T. 3. E 01 CS-60                                             L.T. 1. E 01

, 25-65 L.T. 3. E 01 2a-95/as-95 L.T. 1. E 01 RW-103 L.T. 1. E 01 tv-106 L.T. 1. E 02 1-131 L.T. 2. E 01 C5-134 1. L.1. E 01 C5-137 L.I. 1. E 01 SA-140/LA-140 L.I. 1. E 01 CE-141 2. L.I. E 01 CE-144 9. L.I. E 01 RA-226 3. L.T. E 02 I TH-228 2. L.T. E 01

J u .--.s. -.

       ..-we                           .i   2 l

h t 1 h l 6 .i ( 1 ) l 1, I l t APPENDIX C

SUMMARY

OF UNAVAIIABLE SAMPLES i AND MISSED LOWER LIMITS OF DETECTION t i s e i 1 I I

                                                                                             +

138 1 i i I { I-------.- - .._,. _ _ - _ , . . _ ,, _ _

TABLE C-1 stneeARY OF UNAVAllASE.E SAffLES AND MISSED IAWER LIMITS OF DETSCTI(NI DURIWC 13E PER100 0F i JAIBUARY I To seamal 31. 1985 Sd89LE ISBIA AA4 LYSIS 14C& Tim EErtAAATim 0F S4198.5 WhvallASILITT BATE de satsa m 143

1. Atmospiteric Crese Sete APG-1 01/22/05-01/28/85 ne semple evellebte. perticulate filter mee teet during collection by strees wiede blowing filter este ground. ,

! 2. Drinkteg/ Surface I-131 315-5/ 01/07/85-01/22/95 Water 55-5 We semple avettable. due to sempler selfunction. 3. Drinklas/serface 1-131 ass-5/ 03/03/05-03/18/05 1 Water ses-5 se semple evettable. due to eagler mettuacties. ! 4. Drinking /Serface came Bess-5/ Jemmary ! Water SMB-5 Camposite LIA met met for Be-140/La-140 due to deleyed '

      **                                                                                                 emetyste resulties from miesed osmple.

y 5. Nilk I-131. Game IEE-4 Jemmary me semples evettable goeta met lectaties.

6. Milk 1-131. Comme 355-4 February no semples evettable. goete est lectaties.

i 7. Breed 14ef Vegetaties I-131. Comme 38 4 -1 Jammary lie sample avettable due to freese. S. Breed Leaf vegetaties 1-131. comme BLa-1 Jammery me seaple'evellebte due to freese.

9. Breed Leaf vegetettee I-131. Came 385-10 Jemmary no eenyle evellebte due to freese.
10. Breed Leaf Theatetten I-131. Game 385-10 pobruary me semple cellected elece milk eemplee were evellebte et centrel lecettee. -
11. Breed Leaf Togotetten 1-131. Comme 385-10 Iterch me semple collected elece milk ooglee were 9

4 eve 11eble et eestrel lacetten. 9 i N . i i 1

1 -

  ;                                                                          m      '

TABLE C-2~ - 4 SUtetARY OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS _ OF DETECTION 5%.ING s THE PERIOD OF - - d- APRIL 1 to JUNE 30, 1985 '

 }

SABELE MIA atrusuries op nams unmaus Lm AAALYSIS LeC& TIS BATE n e 385833 IAS i 1. Atmospheric Crees Dete AN-1 M/01/85-M/09/45 no sample ovellable, portiestate filter mee teet

                                                                         ~

during sample collecties by strees wiede blowing filter suey. +

2. Atmoseberic Crees Sete. 1-131 APC-1 M/30/85-OS/M/OS Be sample ovellable due to pump fellere.

j 3. Atmospeneric 1-131 Arc-1 95/06/05-05/98/8S

 !                                                                                                                                                                    123 met met due te les sample volme. sample pump found set rumsteg.

j 4 Ata p pberic Groes Bete. I-131 AFC-1 05/08/85-05/20/85 1 4- us semple ovellable due to peuer failure et O etaties. S. Ataseptierte 1-131 Apo.1 06/24/05-06/27/05 Lia met met due to law sample volemme. Sample peamp found met rumelag.

6. Nilk 1-131. Comme IEE-4 April Re samples ovellablog goate met lactattag.
7. Nilk 1-131. Comme 1E5-4 05/29/05 Re sample ovellable from aumer.
8. Milit 1-131. Comme IEE-4 Joe i De samples eve 11able from sener.

i 9. Breed Leaf Togetation I-131. Comme 315-10 April j to sample cellected etace milk eamples were t evettable et centrol lacettee. j 13. areed Leaf Togetaties I-131. Comme ala-It usy no sample cellected steee milk samytee were sveitable et centrol necettee. Ii 4 i I, a l 1 4

TABLE C-1 SIDMARY OF UNAVAILABLE SAMPLES AND MISSED LOWER LIMITS 0F DETECTION DURING THE PERIOD OF JULY 1 to SEPTEMBER 30. 1985 sasets impla EErtAmaTIS er SagrLE MaTAIIAstLITY amaLTsts sacatim ants a usese saa .{

1. Atarsepheric 1-131 ApC-1 07/01/05-47/03/05 122 could not be met. lasofficient semple volume cellected.
2. Ateespiseric 1-131 AFC-1 07/01/85-47/02/05 Lla could met be met. Imenfficient semple velismo cellected.
3. Milk 1-131. Ca m SEE-4 July se sempleo evettable from aumer.
4. Milk 1-131. Co m IEE-4 August no samples ovellable from aumer.
5. Milk 1-131. Comme IEE-4 3eptember me semples eve 11eble from emner.

i I H k H t l I I i e i 1 t

TABLE C-4 4 SUMARY OF UNAVAILABLE SAMPLES AND MISSED IDWER LIMITS OF DETECTION DURING THE PERIOD OF OCTOBER 1 to DECEMBER 31. 1985 SABELE I s la ANALYSIS SAC & Tim EErlAAAT1cu er SMrta MTAILABILITY R&W W 383305123

1. Atmospheric Groes Sete. 1-131 APQ-1 10/30/05-11/04/85 as sample evellables peep being repaired.
2. Atmospheric Grose Sete. 1-131 Arc-1 11/11/05-11/18/85 No sample evellable due to pump malfunction.
3. Ateespheric Groes tote. 1-131 AFC-1 11/18/05-11/25/05 i

no sample evellable. pouer to esmple pump was dioceanected due to mort at diezberes stattaa.

4. Atmospheric 1-131 APS-30 12/02/85-12/09/05 IJA could met be met due to imenfficient sample volume. Pump feed met rumming.
5. Nilk 1-131. Game MS-4 October IIe sample sweilable free aumer.

I 6. Milk 1-131. camme 3Es-4 november ne sample available from aumer.

7. Nilk I-131. Game MS-4 December No sample available from sener.

1 i

8. Milk 1-131. camme j

354-50 10/01/95 no sample cellected by state due to amergency Flameias Baercise.

9. Vegetetten 1-131. Gemme E3-10 10/30/05 No sample'evellable due to fleedtag fram marriease Juan.
10. Vegetettee 1-131. Game 38K-15 12/31/05 se emple eyeitable due to lack of venetecien.

i 6 E l 1 i ) f

TABLE C-5 SUtetARY OF UNAVAILABLE TLD MEASURDENTS DURING THE FERIOD OF JANUARY l TO DECDGER 31, 1985 LOCATION QUARTER EIP!JLMATION C-1 First TLD stolen: Replaced 3/1/85 D-5 First TLD stolen E-1 First TLD stolen: Replaced 3/1/85 E-30 First TLD stolen: Replaced 3/8/85 J-2 First TLD results affected by radiography in area; TLD results not included in Data Evaluation. N-1 First TLD stolen A-5 Second TLD stolen: Replaced 5/3/85 D-5 Second TLD stolen: Replaced 5/3/85 G-4 Second TLD stolen N-1 Second TLD stolen: Replaced 6/8/86 P-1 Second TLD stolen: Replaced 5/1/85 C-1 Fourth TLD stolen D-2 Fourth TLD stolen H-2 Fourth TLD stolen N-1 Fourth TLD stolen e i 143 l

l l D sURARY OF INTMMBORATORY COMPARISONS 144

TABLE D-1 US EPA CROSS-CHECK PROGRAM 1985 trA pate 1: nailes case trA trA 1 more gev. == uarning PREPARATION Results issued Results Media Nuclide Results(e) R e s u l t s ( h) (Known)(M) *** Action 01/04 02/01/85 04/04/85 Water Sr-89 3.0 t 8.7 L.T. 3. -- Sr-90 30. 2 2.6 29.9 t 12. -0.8 01/11 02/15/85 03/15/85 Water Pu-239 15.7 a 2.8 19. t 3. 3.6 ***(d) 01/18 02/15/85 03/15/85 Water Gross Alpha 8.7 5.0 t 5. t O. 0.. u Gross 8 eta 15.0 t 8.7 15.0 a 3. 0.1 01/25 03/08/85 04/15/85 Food Sr-89 34.0 t 8.7 17.0 1 0. -5.89 ***(e) (c) Sr-90 26.0 t 2.6 22.0 t 6. 1-131 35.0 t 10.4 26.3 a 6.2

                                                                                                                        -4.62      ***(e)
                                                                                                                        -2.50 Cs-137          29.0  t 8.7       31.0 a 10.4               0.69 K             1382.0 2207.9     1393.0 t 96.4               0.16 02/02        03/12/85        04/08/85       Water       H-3           3796. 1634. 3933.       t!74.          0.6 02/08        03/11/85        04/08/85      Water        Cr-51           48,       8.7

$ Co-60 t L.T. 57. --

20. t 8.7 19.0 t 6. -0.h 2n-65 55. t 8.7 57. t 6. 0.7 Ru-106 25. t 8.7 L.T. 40. --

Cs-134 35. t 8.7 37.0 t 12. 0.8 Cs-137 25. t 8.7 31.0 1 6. 2.0 , 02/22 04/04/85 04/15/85 Water Urantue 12.0 t 10.4 12.0 t 3. 0.3 03/01 03/20/85 06/10/85 Milk I-131 9. 1.6 t 8.0 t 3. -1.9 03/15 05/09/85 06/07/85 Water Ra-226 1.3 5.0 t 5.9 t 2.1 2.0 ** Ra-228 9.0 1 2.3 5.1 1 1.8 -5.0 ***(f) 03/29 05/13/85 01/02/85' Air Filter Gross Alpha 10.0 t 8.7 1 10.33

  • 1.7 0.11 Gross Beta 36.0 t 8.7 36.66
  • 7. 5 0.23
 s                                                         Sr-90           15.0 2     2.6     14.66 2         1.7 Cs-137                                                    -0.38 6.0 1    8.7      6.0 1         0.0       0.00 04/05        04/23/85        06/10/85     Water         1-131             7.5 t 1.4         6.67 1 1.7            -1.80 04/12        05/09/85        06/10/85     Water         H-3           3559. 1630        3367.      1963.          -0.9
                                                                                                                         .                                   TABLE D-1 US EPA CROSS-CHECK PROGRAM 1985 EPA                                                            Date TI Malled    Oate EPA                                           [PA             il          Nors Dev.           ** Warning PREPARAil0h                                                                         Results         issued Results     Media      Nuclide           Results(a)       Res ult s(b )  (Known)( dD ese Act ion 04/19                                                                               06/28/85         08/15/85      Water           Gross Alpha     32.0   t 8.7    26.33 t     1.7     -2.31               **

(Sample A) Ra-226 4.1 1 1.0 3.66 1 0.9 -1.25 Ra-228 6.2 1 1.6 6.13 2 0.7 .12 U 7.0 t 10.4 6.67 2 1.7 -0.10 04/19 06/28/85 08/15/85 Water Gross 8 eta 72.0 t 8.7 92.33 2 9.6 7.04 ***(g) (Sample 8) $r-89 10.0 t 8.7 10.0 t 0.0 0.00 Sr-90 15.0 t 2.6 13.33

  • 3.5 -1.92 Co-60 15.0 t 8.7 20.0 a 5.2 1.73 Cs-134 15.0 2 8.7 14.66 1 3.5 -0.!!

Cs-137 12.0 t 8.7 16.33 2 9.6 1.50 04/26 05/13/85 , 06/13/85 Urine H-3 3056. 1622. 2833. 2345. -1.1 0!+/10 07/05/85 08/05/85 Wster Sr-89 39.0 1 8.7 35.66 i 9.2 -1.15

                                                                                                                                                           $r-90          15.0 t     2.6   12.66 1     1.7    -2.69               **

05/24 06/18/85 08/09/85 Water Gross Alpha 12.0 t 8.7 12.00 t 5.2 0.00 , Gross Seta 11.0 t 8.7 12.66 a 1.7 0.58 06/07 07/15/85 08/12/85 Water Cr-51 44.0 t 8.7 L.T. 53.3 -- Co 60 14.0 1 8.7 15.66 2 3.5 0.58 Zn-65 47.0 t 8.7 48.33 1 7.5 0.46 A u- 106 62.0 2 8.7 53.67

  • 9.6 -2.88 **

Cs-134 35.0 t 8.7 33.0 t 13.1 -0.69 Cs-137 20.0 t 8.7 23.33

  • 6.2 1.15 i

06/14 07/12/85 08/06/85 Water H-3 2416.0 2608.0 2366.66 2346.4 -0.24 06/21 08/16/85 09/19/85 Water Ra-226 3.1 2 0.7 3.86 1 0.18 2.82 ** Ra-228 4.2 1 1.0 3.66 1 2.0 -1.46 06/28 09/06/85 10/10/85 Milk Sr-89 11.00 t 8.7 11.66

  • 3.5 0.23 Sr-90 11.00 t 2.6 10.00 2 0.0 -1.15 I-131 11.00 t 10.4 9.00 1 3.0 -0.58 Cs-137 11.00 t 8.7 11.00 t 7.9 0.00 K 1525.0 2131.6 1540.0 2103.9 0.34 4

1

TABLE D-1 US EPA CROSS-CHECK P80CkAM 1985 EPA Date Tl Malled *0 ate EPA EPA il PREPARATION Results issued Results Media Nore Dev. ** Warning Nuclide Results(a) Results(b) (Known)W) *** Action 07/05 07/30/85 08/19/85 Urine H-3 2444,0 1610.0 2066.66 2624.5 -1.85 07/13 09/06/85 09/30/85 Water Pu-239 10.6 a 1.9 8.20 2 2.2 -3.78 ***(h) 07/19 08/16/85 09/19/85 Water Gross Alpha 11.0 t 8.7 Gross 8 eta 5.67 t 1. 7 -1.84 8.0 t 8.7 4.33 1 1.7 -1.27 07/26 10/04/85 12/09/85 Food Sr-89 8.7 33.0 t 25.33 t 6.2 <2.65 ** (c) Sr-90 26.0 1 2.6 28.33 a 4.6 2.69 ** l-131 35.0 t 10.4 37.33 1 4.6 0.67 Cs-137 29.0 t 8.7 31.00 2 3.0 0.69 E 1514.0 $131.6 1633.33 2154.0 2.72 ** 08/J9 09/19/85 10/10/85 Water I-131 33.0 t 10.4 36.66

  • 4.6 1.05 08/16 09/13/85 10/07/85 Water H-3 4480.0 2776.0 4433.3 1458.3 -0.18 08/23 09/19/85 11/04/85 Water U 4.0 t 10.4 4.33 2 1.7 0.10 08/30 10/30/85 12/30/85 Air Filter Gross Alpha 13.0 1 8.7 12.66 1 1.7 -0.11 Gross 8 eta 44.0 t 8.7 43.00 t 9.0 -0.34 Sr-90 18.0 t 2.6 20.00 t 3.0 2.31 **

Cs-137 8.0 a 8.7 10.00 t 3.0 0.69 09/06 10/10/85 12/24/85 Water Sr-89 Sr-90 20.0 t 8.7 18.33 t 4.6 -0.58 7.0 1 2.6 6.00 1 0.00 -1.15 09/13 11/06/85 12/16/85 Water Ra-226 2.3 8.9 t 9.23 2 1.5 0.43 Ra-228 4.6 1 1.2 4.03 1 0.6 -1.42 09/20 10/07/85 12/16/85 Water Gross Alpha 4.7 8.0 t 3.33 1 1.7 -1.61 Gross Seta 8.0 t 8.7 4.00 1 0.00 -1.38 10/04 11/14/35 01/08/86 Water Cr-51 21.004 Co-60 8.7 L.T. 63. -- 20.001 8.7 17.66 1 9.6 -0.81 2n-65 19.00t 8.7 7.5 Ru-106 25.33 t 2.19 ** 20.00* 8.7 L.T. 37 -- Cs-134 20.001 8.7 18.33 1 9.2 -0.58 Cs-137 20.002 8.7 22.33 2 3.5 0.81 10/11 11/05/85 12/24/85 Water" H-3 1974.0 1598. 2133.33 1624.5 0.8u

i l l TABLE D-1 US EPA CROSS-CHECK PROGRAM 1985 4 Collection Teledyne Date Media Nuclide EPA-Results(a) Isotopes Results(b) l NOTES: (a) EPA Results-Expected laboratory precision (3 sigma). Units are pCi/A for water, urine, and milk except K is in og/J. Units are total pCi for air particulate filters. (b) Teledyne Results - Average i three sigma. Units are PC1/4 for water, l urine, and milk except K is in og/J. Units are total pCi for air particulate filters. i (c) Units for food analysis are pC1/kg. (d) The history of this analysis indicates no problem with the chemistry. The high result is possibly technician related and sources of error have been discussed with the technician. (e) The results from the EPA were received on Agust 09, 1985 for the i analysis completed in April. The EPA had difficulty determining the correct results for this sample. It was difficult to scavenge and the results were reported as a courtesy although they were considered suspect because of the difficulty of analyzing a synthetic food sample. (f) A new chemistry was tried but did not give good results. A further refinement of the chemistry is planned. , (g) The proportional counters are calibrated for beta efficiency with Cs-137. The efficiency correction applied for the low energy beta l t anitters overcompensated because the amount of the low energy emitters 1 was small compared with the high energy emitters. (h) A new Pu-239 standard solution was prepared and a new Pu disc was ordered from N85 to check the efficiency calibration of the counters. i i 148 l

                                                     -_._ .-- _- _ __. _ _. _ _ _ - -                        a

i TABLE D-2 SEVENTW INTERNATloWAL INTERCOMPARISON OF ENVIROWNENTAL DOSINETER RESULTS DELIVER S EEPOS4mES (et) ALL PARTICIPA3rFS RESIR.TS (et) (a) LP&L'S RESag,TS (eg) (b) Botteste Macertainty steen 3D (c) I Se N (d) Egeoure llacertainty I Error (e) 3 (f) Laboratory Esseomree Free Coetum-137 (g) 75.0 3.8 73.0 11.1 15.2 185 75.0 12.0 0.0 0.70 From Cabelt-40 (b) 79.9 4.0 77.9 13.3 17.7 184 64.0 7.3 -19.9 .t.0 Field Baseeeres (b) 75.8 6.0 75.1 14.9 19.8 104 70.0 0.9 - 7.6 -0.3 e s~ (c) Results of all participante in the Intercomperison Study. (b) Results based on using Panasonic UD-814 Aq TLDe. (c) SD stande for Standard Deviation. (d) N stande for Number of results. (s) I Error is a measure of how much LP&L':. resulte differed from the estimated delivered exposures 1 Error = (LP&L's Exposure - Delivered Esposure) x 100

l. Delivered Exposure (f) ND stande for "Normalised Deviation". It to a measure of how many stendard deviatione LP&L results were from all participants' results.

ND = All participants' Results asan - LP6L Exposure , All Participants' SD (g) Results of all dosimeter types for all participants' results. (h) Results of all doetaster types for all participants' results with one outliner excluded. s.

APPENDIX E SYNOPSES OF ANALYITICAL PROCEDURES e 150

E-1.0 ANALYSIS OF SAMPLES FOR GROSS BETA ACTIVITY E-1.1 Air Particulates After a delay of three or more days, allowing for the radon-222 and radon-220 daughter products to decay, the particulate filters were counted in a gas-flow proportional counter. E-1.1 Water 1 A known volume (usually one liter) of water is evaporated to i near dryness, transferred to a two inch diameter ringed planchet, and then evaporated to dryness. The planchet was then counted for 50 minutes in an automatic alpha-beta counter. E-2.0 ANALYSIS OF WATER SAMPLES FOR TRITIUM one milliliter of water was added to 20 milliliters of liquid scintillation solution in a 25 milliliter vial. The sample was then counted for 100 minutes in a liquid scintillation counter. E-3.0 ANALYSIS OF SAMPLES FOR IODINE-131 E-3.1 Milk and Water l Two liters of sample were first equilibrated with stable iodide carrier. A batch treatment with anion exchange resin was used to remove iodine from the sample. The iodine was then stripped from the resin with sodium hypochlorite solution, reduced with hydroxylamine hydrochloride, and then

  • extracted into carbon tetrachloride as free iodine. It was then back-extracted as iodide into sodium bisulfite solution and precipitated as palladium iodide. The precipitate was l

weighed for chemical yield and mounted on a nylon planchet for low level beta counting. The chemical yield was corrected by measuring the stable iodide content of the milk or the water with a specific ion electrode. 151 l____ -__ - _ _ _ - - . - . - - _ - - - - - -- - --- --- -- - --

l E-3.2 Broad Leaf Vecetation Stable iodide carrier was first added to a measured weight of chopped sample. The sample was then leached with sodium hydroxide solution, evaporated to dryness, and fused in a muffle furnace. The melt was dissolved in water, filtered, , and treated with sodium hypochlorite. The iodine was then reduced with hydroxylamine hydrochloride and extracted into chloroform. It was then back-extracted as iodide into i sodium bisulfite solution and precipitated as palladium i iodide. The precipitate was weighed for chemical yield and mounted on a nylon planchet for low level beta counting. The chemical yield was corrected for the natural, stable iodide content of the sample by use of a specific ion electrode on a separate aliquot (without carrier added) of , the sample. ' i E-4.0 GAMMA SPECTROSCOPY ANALYSIS i E-4.1 Milk and Water  ! A one liter Marinelli beaker was filled with a representa-tive aliquot of the sample. The sample was then counted for 1000 minutes with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performed pulse height analysis. E-4.2 Vecetation. Food and Garden Crons, and Fish  ; As much as possible (without drying) of a vegetation, food, or garden crop sample was loaded into a tared one liter Marinelli beaker and weighed. The sample was then counted for 1000 minutes with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which per-formed pulse height analysis. As much as possible (up to the total sample) of the edible  ! portion of a fish was loaded into a tared Marinelli beaker and weighed. The sample was then counted for 1000 minutes i with a shielded Ge(Li) detector coupled to a mini-computer-based data acquisition system which performed pulse height analysis. 152

E-4.3 Soils and Sediment Soils and sediments were dried at low temperatures, less than 100 degrees Centigrade. The soil or sediment was loaded into a tared, standard 300 ml container and weighed. The sample was then counted for at least six hours with a shielded Ge(Li) detector coupled to a mini-computer-based l data acquisition system which performed pulse height analy-i sis. i E-4.4 Charcoal Cartridaes (Air Iodine) Charcoal cartridges were counted up to five at a time, with one positioned on the face of a Ge(Li) detector and up to four on the side of the Ge(Li) detector. Each Ge(Li) detector was calibrated for both positions. The detection limit for iodine-131 of each charcoal cartridge was deter-mined (assuming no positive iodine-131) uniquely from the volume of air which passed through it. In the event iodine-131 was observed in the initial counting of a set, each charcoal cart. ridge was then counted separately, l positioned on the face of the detector. E-4.5 Air Particulates The weekly air particulate filters for a quarterly composite ' from each field station were aligned one in front of another and then counted for at least six hours with a shielded Ge(Li) detector coupled to a mini-computer-based data 1 acquisition system which performed pulse height analysis. i , E-4.6 Connuter Software i A mini-computer software program defined peaks by certain changes in the slope of the spectrum. The program also , compared the energy of each peak with a library of peaks for isotope identification and then performed the radioactivity ' calculation using the appropriate fractional gamma ray abundance, half life, detector efficiency, and not counts in the peak region. l < 153

E-5.0 ENVIRONMENTAL DOSIMETRY Thermoluminescent Dosimeters (TLDs) manufactured by Panasonic (model UD-814AQ) were used for environmental dosimetry. The Panasonic TLDs contained one lithium borate and three calcium sulfate phosphor elements. However, only the calcium sulfate phosphor elements were used. An annealed dosimeter was placed inside a plastic bag and mounted in an aluminum frame prior to placement in the field. The dosimeters were exchanged every quarter. The exposures of the collected dosimeters were read using an automatic TLD reader manufactured by Panasonic (Model UD-710). I i

                                                                                          )

154 1

4 APPENDIX F STATISTICAL ANALYSES 155 l t.----- - . - - _ . _ . - _ _ _ _ _ _ _ _, _ __

F-1.0 CALCUIATION OF MEAN AND STANDARD DEVIATION The mean and standard deviation for different groups of analyses were calculated using the following equations: (F-1) x = I* i=1 nx

                                                              /n x                                    0.5 7

I x12_ (o x) (x)2 (F-2) s = I"I k (nx - 1) ) where: Tc = mean of sample population, s = standard deviation of sample population, nx = number of samples in sample population, and

  ,                     x1                      = value of the ith sample.

F-2.0 COMPARING TWO SAMPLE POPUIATION MEANS , The means of two sample populations can be compared for a statisical difference using the standard "t" test. The use of the test requires the assumption that the data within the populations are normally distributed and that the true standard deviations of the mean are equal for both populations. The standard "t" test tests the hypothesis that the true means of both populations are equal. The "t" value can be calculated from j the equation below (obtained from the CRC Standard Mathematical Tables, 26th Edition (1981)): i (F-3) ( ~

                                                                                           }

e, f(n x- 1)s x2 + (n y- 1)s y2 \ f1 if

                                                                                                               +
                                                                          "x + "y       -
                                                                                                          "x       "y 156

_ _ . - _ _. _ ~ - - . . _ _ _ . - , _ _ _ . . - - - _ .

where: t = calculated "t" value, x = mean of first data set,

                         ? = mean of second data set, nx   = number of variables in first data set, sx  = standard deviation of first data set,
                              = number of variables in second data set, and
                              = standard deviation of second data set.

If the data from both sample populations are treated as cor-related pairs, the difference between individual measurements can be examined using the statistical "t" test. In this case, if the true means and true standard deviations for the sample populations are equal, the difference between the correlated data points should be normally distributed about a mean of zero. The "t" value can then be calculated from the following equation (obtained from the CRC Standard Mathematical Tables, 26th Edition (1981)): (F-4) t = I (n) 0.5 sd where: dI = the average of the difference between the cor-related data points from the two sample popula-tions: N d = I (xt-yg)/N i=1 xt= the ith data point from population x, y t= N= the ith data point from population y, s= the number of correlated pairs of data points, and d the standard deviation of the difference between the correlated data points. . The calculated "t" value in both cases is used to test the hypothesis that the true mean of the first population (u x) is equal to the true mean of the second population (uy) assuming that the true standard deviations of both populatibne are equal (or " 8 y) . The calculated "t" value is compared to a tabular "t"

value such that:

a. if t>t ,n then reject the hypothesis when u x>uy, b. if t<-t ,nm then reject the hypothesis when ux<uy,

c. if ltl>tW ,n then reject the hypothesis when u xpfuy, l 157

i where t a/2 n and(5t,,n are the tabular "t" values, with a pre-selected eferor percent in this case), confidence level (1 a) l or (1 a/2), and degrees of freedon n (n=n x+n y-2 and n=N-1 for Equations F-3 and F-4, respectively). Tabular values of "t" were

obtained from the CRC Standard Mathematical Tables, 26th Edition (1981).

i F-3.0 TLD MEASUREMENTS The TLD measurements made during 1985 were grouped into cate-gories based on distance from the plant. The means and standard deviations obtained for each category are given in Table F-1. The mean dose from the stations located more than five miles away from the plant were compared to the mean dose from stations ! located within two miles from the plant and to the mean dose from stations located between two and five miles from the plant using the standard "t" test. The "t" values were calculated using Equation F-3 and are given in Table F-1. Comparing the calcula-ted and tabular "t" values show that the mean dose for stations within two miles from the plant is statistically lower than the mean dose from stations located greater than five miles from the plant. The mean dose for stations located between two and five miles from the plant is statistically the same as the mean dose j for stations located more than five miles from the plant. F-4.0 GROSS BETA ACTIVITY ON AIR PARTICULATE FILTERS The means and standard deviations for airborne gross beta results obtained during 1985 from the control and indicator stations are given in Table F-2. The mean from each indicator station was compared to the mean from the control station using the standard "t" test to determine if there was a statistical difference. The calculated (using Equation F-3) and tabular "t" values for each indicator / control station comparison are given in Table F-2. Comparing the calculated and tabular values indicate that there is no statistical difference between the means from each indicator location and the mean from the control location. F-5.0 GROSS BETA ACTIVITY IN MONTHLY DRINKING WATER COMPOSITES The means and standard deviations for gross beta activity l detected in the monthly drinking water composites obtained during i 1985 from the control and indicator stations are given in Table l F-3. The mean from each indicator station was compared to the mean from the control station using the standard "t" test to ,. l determine if there was a statistical difference. The calculpted 158 I

                     --------,.,,..-__..-_-.,--____.___,.-n.,_-,--.n,,-.,,-n---                                            n     .n m , - em mm

(using Equation F-3) and tabular "t" values for each indicator / control station comparison are given in Table F-3. Comparing the calculated and tabular values indicate that there is no statistical difference between indicator station DWE-5 and control station DWP-7 means. However, there is a statistical difference between the means from indicator station DWG-2 and control station DWP-7. In order to determine if this difference resulted from the operation of Waterford 3 SES, data obtained in 1985 were compared to data obtained in 1984. Monthly gross beta activity data from each indicator and control location were treated as correlated pairs. The differences between monthly measurements obtained from each indicator and control station samples were calculated and averaged for 1984 and 1985. The results of these calcula-tions are presented in Table F-4. The "t" values for each indicator / control station difference were calculated using Equation F-4 and are given in Table F-4. Comparing the calcula-ted "t" values to the tabular "t" values show that the means for data from station DWG-2 were statistically larger than the means from control station DWP-7 during both 1984 and 1985. The means for data from indicator location DWE-5 and control station DWP-7 were statistically the same during 1984 and 1985. As further comparison, the average of the indicator / control station differences obtained during 1984 and 1985 were compared , to each other using the standard "t" test. The "t" values were calculated using Equation F-3. The calculated and tabular "t" values are presented in Table F-4. Comparing these values indicate that there was no statistical difference between the results observed during 1984 prior to Waterford 3 SES initial criticality and the results obtained during 1985. Thus the i difference between indicator station DWG-2 and control station DWP-7 gross beta results were deemed to be unrelated to Waterford l 3 SES operation. j 159 I l 1

1 TABLE F-1 STATISTICAL COMPARISON OF TLD MEASURDENTS FROM STATIONS GROUPED BY DISTANCE FROM WATERFORD 3 SES 0-2 Miles Stations Located 2-5 Startons Located from the Plant Miles from the Plant more than 5 Miles stos the Plant j Mean (aren/std. gtr.) 16 17 4 18 i j l Standard Deviation s (aren/std. gtr.) 1.6 3.0 3.4 Os o i 4 I j Number in Sample 58 26 32 l I j Calculated "t" Value to Camparisone 4 with Statione lacated more than 5 miles from the plaat -3.794 -1.153 NA I i Tabular "t" Value at ! 95I Confidence I (t 0.025.a . a .010 m 1

s. Used value for 4.025 n, Results fadicate that the mean for station located 0-2 miles from the plant is statistically lower than
  • stations located more than 5 alles from the plant.

NA Means not applicable i i

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                                                                                    *S TABLE F-4 STATISTICAL COIWARISON OF CROSS BKTA ACTIVITT IN N00 MILT DRIIKING MATER COMPOSITES FOR 1984 and 1985 Difference of Monthly Results            Difference of Monthly Results from Stations DWG-2 and DWF-7            from Statione DUE-5 and DWP-7 for 1984             for 1985          for 1984            for 1985 i                  Mean (pC1/1)                                             1.9                 2.3              -0.1                 0.7

) Standard Deviation ! (pC1/1) 1.5 1.4 1.7 1.9 .i H

e i Neber in Sample 12 12 12 12

} l Calculated "t" Value Comparing i Control / Indicator Station Difference 4.388 4.426 -0.204 1.276 ! Tabular "t" Value Comparing { Control /lodicator Station Difference 2.201 2.201 2.201 2.201 . at 951 Confidence (t0.025.n) l Calculated "t" Value l Comparing 1984 Results -0.566 NA -1.041 NA ! to 1985 Results

!        Tabular "t" Value Comparing i         1984 Results to 1985 Results l         at 951 Confidence                                        2.074                  MA              2.074                 NA (to.025.n)
                                                                                                                                                      .i NA Meads not applicable l.

w w _a--_._m--- -

                                                            + P. O. BOX 60340
       '"4       LOUISI&ANA POWER      LIGHT/  317BARONNESTREET NEW ORLEANS, LOUISIANA 70160  *

(504) 595-3100 [Niu?$EvsM April 30, 1986 W3P86-0078 A4.05 QA Mr. Robert D. Martin Regional Administrator, Region IV U.S. Nuclear Regulatory Commission 611 Ryan Plaza Drive, Suite 1000 Arlington, TX 76011

Subject:

Waterford 3 SES Docket No. 50-382 License No. NPF-38 Radiological Environmental Monitoring Report

Dear Mr. Martin:

Enclosed is the subject 1985 annual report on radiological environmental monitoring which covers the period of January 1 through December 31, 1985. This report is submitted per Section 6.9.1.7 in the Waterford 3 Technical Specifications (NUREG-1117) of Appendix A to Facility Operating License No. o NPF-38. Vern tr"ly yours, f' K.W. Cook Nuclear Support & Licensing Manager KWC:GEW:ssf l Enclosure I cc (w/ enclosure): NRC, Director, Office of I&E l NRC, Document Control Desk, Washington, D.C. cc (w/o enclosure): C.W. Knighton, NRC-NRR J.H. Wilson, NRC-NRR N,RC Resident Inspectors Office $, B.W. Churchill V W.M. Stevenson l g( '

                              "AN EQUAL OPPORTUNITY EMPLOYER" l
                                                                             . .       _}}