ML20136B142

Calculations Re Containment Hydrogen Bubble

ML20136B142
Person / Time
Site:	Crane
Issue date:	03/30/1979
From:	Mattson R, Stello V, Tedesco R NRC OFFICE OF INSPECTION & ENFORCEMENT (IE), Office of Nuclear Reactor Regulation
To:
References
NUDOCS 7908230009
Download: ML20136B142 (105)

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RADIALYSIS INFORMATION -7 AIC TC d Y V, STELL o i l On April 1, 1979 3:00 P.M. I requested Bettis Laboratory to evaluate the potential for radielysis contributing oxygen to the bubble over the reactor core. The following people participated in the evaluation: Don Connors Lou Bogar Jim Wright Ken Vogel Bill Walker (KAPL) The following information was provided and was represented as the Bettis daboratory position. A report would be prepared if requested. I_ indicated that I would let them know if there was a need. (a) The first question I asked them to consider was if we assumed that the bubble over the reactor core is 800 cu ft, 1,000 psi and 300 F is it possible for oxygen to be added to the bubble by a radielysis process? Answer: There best estimate analysis would indicate that no oxygen would be added to the bubble. The analysis is derived from considering Henry's law they would expect that under the conditions there would be 900 ce per kilogram STP of hydrogen going into the water. Based on experimentally derived infor9 mation with a concentration of 2 cc's per kilogram of STP in water radielysis would be prevented. The experimental infor-mation was d,erived from data collected in the S7G prototype program and a reference is cited to data dating backing to_1943. 4 l l m w 3 w - r

~ (b) I requested Bettis to provide me with an estimate of the radielysis rate assuming it was no hydrogen over pressure in the bubble. Answer: Assuming no recombination was permitted they calculate that approximately 8.4 cu ft per day of oxygen at STP would be generated. This corresponds to a total radielysis rate of 29.2 cu f t per day at STP. The recombination rate was based on a defactor that was experimentally determined from S7G and boiling water reactor data. These data were stated to be conservative relative to PWR C_ conditions. Thejefactorusedwas.07 molicules of Od)g per 100 EV o'f gamma absorbed. A 1.5 x 109 NEV of gammas per second. They assumed that 1/10 of the gamma's generated in the core are absorbed in the core and that 1/15 of the gammas absorbed in the core are absorbed by water. They have had informal discussions with people like KAPL who independently determined a radialysis race in the same ballpark (estimated to be approximately 65 cu ft per day at STP). Dr. Connors is going to ask KAPL for. their view to see if their evaluation of the problem is the same. i I l \\ s s t e e u-,.-, e

/JU0TES 0v' VIL STELt0,l ^ RADIALYSTS ThTORMATION On April 1 at about 3:00 P.M. I requested the same information of the General Electric Co as I did from Bettis Laboratories. _ The CE response was that it is theoretically possible that oxygen could be added to a hydrogen bubble over the reactor core. However, they did not consider this would be likely_ and concluded that they believe that an equilibrum condition may now be present. They calculated a bounding number for the amount of radialysis that could take place assuming no hydrogen over pressure. They estimated that the boundary number is 10 cu f t per hour at STP but believe this was too conservative since it was based on BWR data . QTEDE-13148 Title KRB nadialysis Test, Nov. 1970) and that no credit was given for the effects of a back reaction and that the real number is much lower. They speculated that perhaps there is no net oxygen added. The following people participated in the evaluation: Cliff Kent, Jerry Jacobsen, Pat Marriott, Manny Ziegler, and Dor. Rockwell l 9

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Subject:

TMI-II Gas hd61e Volume Calculat Enclosed is some sumery infoneetton rweardthy our calculations of the i TMI-II gas bubble volisme. Thfs information has been trangultted (telecopy) to Dick W11sen of Met. Ed. 6perations and the NRC representative in the TMI-II control room, les believe further commamcattom are necessary to conff rw that everyone concun on the validity of the equat toni an<f the test procedure being run or to plan further testing and analys tar. $U D. W. B*reper Babcock & W1Icow t/' A/ */ 7 i o 5~ Y / 1 t l g

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I h1 Wt Harold Denten Statement en Bubble Hazard kk l April 2 for the past several days ___we have been studying the potential hazard of the gas bubble in the reactor. There has been concern that the bubble could reach a flammable condition if exygen were being added to the hydrogen. Our earlier statement on the effects of bubble flammability on the safety of the plant.were primarily based on preliminary theeretical analysis _by the technical experts. There is also some experimental data for these conditions. After several days of intensive censideratien of the problem by these k~ w.. experts, we now believe that the hazard of hydrogen combusti:::n2in the reacter is not nearly as severe as earlier indicated. Qu'r atydy' of- / ~ ~ this problem is centinuing >and we ar~emot9bho-t:chpletely'discetiilt theTossibhi y,-oQdrotenn bur,n.ing, we nave much higher confidence today e A5 amak)(] vt-- # ht- % ~ that there is no near term hazard from th!: c u N There : n : ren 9:r piece [of new information from the plant that centribute to cur present state of cautious cptimism in this area. Measurem,nts of the size of the bubble over the last 24 hours indicate that it is not as large as originally estimated, and it may be centinuing to diminish. We are studying this new information closely to determine the effectiveness of the degassification process that has new been underway for several days and the confidence that can be placed in the bubble measurements. n r\\ p_ w w ~ -- - i t! ,, -, ~ < - -

Press Briefing 4/2 - 11:00 Three Aspects of the Bubble ouestions 1 Size Encouraging signs that it is smaller than earlier measurements indicated. 1 measurements are better degasify thru recombination letdown seal leakage in pump ' Content Our present understanding of the gas evolution and decay process says the rate of addition of oxygen is not what we originally esti-mated. There may be an equilibrium condition in which there is little or no net generation of f.ree oxygen in the reactor or even recombination (i.e., either slightly positive, sero or negative). Combustion Limits Our earlier estimates were conservative, but there is some uncertainty in the available data, so staying with the 5* and 117. limitsI ~ 1 l 1 1 3 9 = f

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W tk, kt-h 004m). ~,.' m%h Ow vwI Noise Analysis Summary M B Y N WO Ac h' ro Mer t: J. b Il O April 2, 1979 1500 hours 64-hk.Y-- { W Y-y0, ~~ ~ No significant Loose Parts noises have been detected at the bottom and top of the reactor vessel and top and bottom of steam generators. Primary Coolant pressure fluctuations have been observed with the following characteristics: 1) Increase and decreases of reactar coolant sys tem pressure , r cr MI A%1 noise were noted with nv4m 6'To~perating increases and decreases in reactor coolant system pressure.

2) The peak magnitude of the reactor coolant system pressure fluctuation increased in magnitude over a period of 18 g.,5 Q &m. ';a} %d 'i l t 9 m]

hours' reac' ing a maximum typical value of 55 psig peak.to-n peak with the maximum observed excursion of 137 psig peak-to-peak for the Reactor Coolant Loop "A" pressure signal. The typical peak to peak fluctuation for the Reactor Coolant Loop "B" pressure was 3 PSI and the maximum peak to peak l value observed over a 4 hour period was 8.5 psi peak-to-peak. l l t l l s l 0

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3) The typical peak to peck amplitude of the reactor coolant system pressure fluctuations has not increased in the last IOC

~ ~ 24 hours Ao d, G 9/1.)M y ~4) The onset of the pressure fluctuations appears to occur at a threshold value of the absolute value of the reactor coolant-system pressure. This onset pressure value has shown a slow decrease in tin.e and at 0500 hours of 4/2/79 the threshold value was approximately 850 psig.

5) After the pressure fluctuations.have increased to the typical 55 psig peak to peak values, no further increase in the fluc-tuation magnitudes have been observed with increasing reactor coolant system pressure up to 1100 psig.

6) Spectral Analysis were performed and revealed that most of the pressure fluctuation amplitude power in essentially Cm Q % wyw Ww'+ hJL W O -1 \\ random fluctuations een.mupS Hz with low conerence between y the pressure fluctuations of the two reactor coolant system loops. j k .4 J J o,a J ayk 4 % W m & W J w 6. fAa& ~% d +-4 Ak P4 4 ,n- --,,a

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.~ D,., ' '} l ' ~,( u ,.. y j-,' .. r,, l m m ' 7 l rv f ry TECHNICAL UPDATE ON CURRENT SITUATION AT THREE MILE ISLAND April 2, 1979 Plant Status Reactor pressure is being held at about 1000 psi. Incore thermo-couples continue to show a decrease in fuel channel temperatures. with all measurements below about 475 degrees F as of 4:00 p.m. - ) Bulk core inlet and outlet temperatures are about 280 degrees F. At 10: 30 a.m., April 2, a containment air sample indicated about 2% hydrogen. At about 1:45 p.m. April 2 the first hydrogen re-combiner was placed in service and had reached operating tempera-tures by about 4:15. Recombiner instrumentation indicates about 2% hydrogen concentration in the containment air. r_ Further analyses and consultations with experts has led to the f development of a strong consensus that the net oxygen generation rate inside the noncendensible bubble in the reactor is much less than original conservative estimates. Also, meas urements at the ' plant appear to indicate that the volume of gases within the bubble is being signi ficantly reduced. Plant instrumentation is being closely followed to confirm these favorable indications and to better understand the characteristics of the processes cssociated k with decreasing ~ bubble size. ~ Environmental Status Thi rty-seven thermoluminescent dosimet ry (TLD) stations were established by the NRC.at distances from about one mile to about 12 miles from the plant. Multiple dosimeters are placed at each location - one will be left in place for a cumulative dose measure-ment; another is pulled and replaced each day. The highest dosimeter reading was recorded at a location 1/2 mile ENE of the plant. The dose rate of this location was 1.1 milli-roenitger per hour. The next highest was 0.4 mr. per hour 0.4 miles east of the site. All the remaining samples were 0.1 mr per hour or Imver. Aerial radiation surveys continued at three-hour intervals on April 1, and 2, 1979. The plume readings were essentially the same for all the flights. Direction of the plume varied f rom SW to WNW. The maximum level at one mile from the plant was about 3 mR/hr at an altitude of 500 feet. At three miles, the levels were f rom 0.1 to 0.5 mR/hr. Offsite ground level surveys taken between 11:00 a.m. April 1, and 4: 30 a.m. April 2, on both sides of the river in a southerly direc-tion generally showed levels of 0.01 to 0.04 mR/hr. h M 6 e 40 m e d e .e ? xpj Q.T - v c 30qpm O ' {*3 f. $ (

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Date l SW.ARY OF ELW AXA1.YSIS OF SIZE MD COMPOSITION OF H /D 2 BU3BLE M0 TMI-2 YESSEL April 2.1979 i,,m Attached is the strr.ary paper en B&W results for size and cogosition of f the bubble existing in the TMI-2 reactor vessel of This is provided in accordance with your request at 1900 hours on 4/2/79. 'h. will be happy to discuss this further with you and provide any other i details which you may require. Pteese contact me at area code 804/38?-5111 extension 219I. 9 J Attach ent i A l f, / f ,e f [l } u ,(t' y l t i li / s D. A. MItti 4/2/73 - 8:25 p.n. SIZE OF THE GAS BUBBLE IN T5E T20-2 REM ~IT.A W.5SEL The size of the gas bubbie in the iM1-2 reactor vs.nal (including any-gas trapped in the high points of the reactor coef a.c loop) was daterslaed by azeasuring systes parameters durkg airpressura-trartsient 1agxrsed on the ramctor coolant systaa. This m semryiTs'helWTsAlatitur ~~ the reactor coolanc systese, except for its letdown fiow and its reactor coolant pd seal flo.t and alicwing the pressurl ar beaters to increase :he i reactor coolant systen pressure. Cars was :akan for the reactor coolant system pressure and te=perature, the pressurizer leM x>d temerature, and the sukeup tank level and tecperature at both the start of the test period and at the end.of the test period. Using these amasured parameters and the ideal gas law, a mathematical correlation was developed to calculate the bubble ~ u~ size. This correlation =pansates for the change in pressurizer level and Qi"J.., adjusts,for the changa in specific volone between the bot fluid in the pressurizer j

rnd tk raiatively cold fluid in the reactor coolant loop. A similar correction

_~ - was irwix.ded for the change in specifTc. volurse 1et.acco the bot reactor coof act ) entering and leaving the makeup tank. Adjustrents were included-for the ccx::pressibility of the reactor ecolant. fluid due to the change in pressure, J the expansion of the reactor coolant due to the change in teeperature, and fortIchac9e. In solubuity of the gas due to the change in pressure durir>p the test period. The attached figure shows the predicted bubble size for eight sets of test data analyzed tuth with and without the solubt fity correction. I These tws analyses should bound the raxtcom and ainfau bubble size. The figure shows that the bubble size approaches zero at about 1500 hours on April 1 if the solubliity of the gas is considered. Vithout the solubliity correction factor the predicted bubble s!ze is significantly larger (but exhibitch a similar .....s deceasing tendency which maid trdicate a zero volume by alsnost 12:00 hours on AprII 2,1979. The megnitude of the error ranges are ' based on tie expected repeatability of the Instruments under normal operating conditions. Under the extreme conditions icposed on the instru=entattoa in the present environ-ent, l the errer ranges cay be smewhat larger. We feel that the calculation which i includes the effects of the gas solchility is tednically core valid and feel that the conclusion of zero bubble size tends to be corroborated by the sudden l al i m-

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\\ i. : ! :. r. '4 ' : ~ ;- - D. A. Nitti April 2, 1973 - Pace Two appearance of a high frequency raise in our. pressure readings on the B-ioop pressure transmitter signals at about 15:07 on April 1st: The ~ ~ ~ -..,, appearance of th!s high frequency noise is intepreted as the point 6're mK the reactor coolire"5 once again became 1-n=pressible. i 1 m 3 /dww G ..e = ,_3.

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.,s; 1 1 4 ^ A i i l l t D. A. Mitti' = w 4/2/79 - 8:52 p.S COMPOSITION OF THE MS BUBBLE TP/# FED IN THE REACTOR CDOLMT SYSTDi 0F THE TMI-2 PLANT A review of the. postulated sequence of events on March 28 lead us.to conclude that there is no significant amount of oxygen in the beble that was I present in the reactor coolant system of the Three Mile Island Muclear Pjant. At the tir.4 of the reactor trip, the reactor coolant contained a significant axcunt of dissolved hydrogen, approximately 10 to 15 cc per kilograsa of coolant.. This annsnt dissolved hydrogen is sufficient to suppress the net production of radiolytic oxygen. When boiling occurred in the core region, hydrogen was stripped from the reactor coolant an:t sme net radiolytic oxygen production probably occurred. The estimated production rata was about 70 standard cubic feet per hour. Shortly after boiling began, a metal water reaction began and generated large anounts of hydrogen bn the order of 50,000 standard cubic feet). This Targe amount of hydro-gen apparently beca e trapped in the reactor coolant system and formed a Targe bubble in the reactor vessei bead. After the catal water reaction was quenched, this hydrogen b6ble created a hydrown overpressure sufficient to dissolve approx-icately 1,000 stardard cc's of hydrogen per kilogra= of water. This arount of dissolved hydrogen is approxicately 50 tices the ascunt required to suppress a net radiolytic generation of oxygen. A s:.all a.ount of air dissolved in the coolant water irdected into the reactor coolant systen introduced less than 200 stardard cubic feet of oxygen. Since there were no other sources of oxygen, we conclude that the hydrogen bubble never contained an oxygen concentration.of 102%. This..N '.5,. concentrationlof'oxygjn is pelf belotti$5 concentratiffi.Ng6frQ [to, support' ~ ' 7[],M. j coct:istion in hy[dFogen-o'xygeri mixtuMs.,' ' _.d* O 't'-' Independent calculations by Dr. Come.m at Bettis La.boratories sopport the conclusion that"the prtxbetfon of radiolytic oxygen was suppressed by the high hydrogen overpressure present in the TMI-2 reactor coolant systaa. DAN:dw/jws S 4 h. I f...... M i., g j ,...a ._j _.. ....j.} ..4 i.f 4I 64 ..L. .4 ,i.. J

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