ML19220B821

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Forwards Info Re Storage of Liquid Radwaste in Tankcars & Response to Request of R Vollmer Re Transuranic Concentrations in Coolant
ML19220B821
Person / Time
Site: Crane 
Issue date: 04/13/1979
From: Miraglia F
Office of Nuclear Reactor Regulation
To: Grimes B, Vollmer R
Office of Nuclear Reactor Regulation
References
NUDOCS 7904270414
Download: ML19220B821 (10)
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Central Files PSS Rdg. File April 13,1979 I

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B. K. Grimes, NRR, TMI-2 t

R. H. Vollmer, NRR, TMI-2 FROM:

F. J. Miraglia, Jr., Coordinator, Team B is infomation B. Grimes requested of S. Bland on April 12,1979. is infomation R. Vollmer requested of R. Emch on y

April 13,1979, i

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F. J. Miraglia, Jr.

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Team B l

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ATTACHMENT 1 STORAGE OF LIQUID RADWASTE IN TANKCARS B. Grimes requested on 04/12/73 that we provide an isotopic breakdown of the dose rates from a 30,000-gallon railroad tankcar containing liquid radwaste. We had sent him the dose rates on 04/11/79. The dose rate at contact was 40 R/hr as calculated by ORNL (D. Bartine).

Grimes also requested that we provide the dose rates for a 10,000-gallon tankcar.

We contacted ORNL but learned that today (04/13/79) is a state holiday in Tennessee and ORNL was not working. Therefore, we calculated the dose rates by hand in order to provide a timely response to the site.

We will follow-up on this on Monday (04/16/79) and contact ORNL agair,.

We calculated 7 R/hr at one meter from the 30,000-gallon tank and 4 P./hr at one meter from the 10,000-gallon tank. We were unsure of the dimensions of a 10,000-gallon tankcar; 4 R/hr is for a tank as-sumed to be 10 feet in diameter and 17 feet long. A tank 8 feet in diameter would give a dose rate of about 3 R/hr at one meter.

The isotopic distribution for the 7 R/hr dose rate is given below:

CONCENTRATION

% OF DOSE RATE NUCLIDE uCi/cc DUE TO NUCLIDE I-1 31 100 82 I-133 5

9 Xe-133 4

0.25 CS-134 0.4 0.5 CS-136 0.8 4

CS-137 1.4 3

La-140 1.6 1

This work was done by R. Emch and F. Akstulewicz.

83 % 1.

ATTACHMENT _2_

RESPONSE TO REOUEST OF R. VOLLMER CONCERNING TRANSURANIC CONCENTRATIONS IN COOLANT On Friday afternoon (04/13/79), R. Vollmer requested that we provide information to him on transuranic contamination of the primary coolant at PWRs other than TMI-2.

Turkey Point has reported the following measurements of transuranics in the primary coolant.

-9 Pu-238 5(+1.6) x 10 uCi/gm Pu-239 and Pu-240 4.3 x 10' uCi/gm Indian Point 1 and 2 has reported these measurements of transuranics in 1975:

Pu + AM20 + Cm242

-9

-7 10 -10 uCi/gm We called Duke Power Company today. Robert Gill informed us that the MDA for gross alpha measurements in the primary coolant at Oconee is

-6 4 x 10 uCi/cc. Oconee measurements of gross alpha in the primary

-0 coolant have always been less than 4 x 10 uCi/cc.

Generic calculations for a straight tube steam generator plant were done during the GESMO study. The calculated uranium concentrations in primary coolant were:

-12 U-235 2 x 10 uCi/cc

-5 U-237 3.8 x 10 uCi/cc

-II U-238 2 x 10 uCi/cc S3 'X2

ATTACHMENT 2 (CONT'D,)

- 2 Note that U-237 has a 6.8 day half-life. Thus, U-237 has a very high specific activity.

Printouts of calculated primary coolant concentrations for Davis-Besse and GESMO are attached.

We have estimated the concentrations of uranium in water which cor-respond to 10 ppb:

-8 10 ppb - U-235 2 x 10 pCi/gm 10 ppb - U-237 8 x 10+2 uCi/gm

-9 10 ppb - U-238 3 x 10 uCi/gm Without knowing the isotopic content of the uranium, it is impossible to supply better correlations between ppb and uCi/gm.

When LACBWR had fuel problems in 1976-1977, they measured 6 x 10~ uCi/gm of gross alpha radioactivity in the primary coolant.

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1. c c t 1. 3ci -o 3. S 3 t - c.,

PL213 a.6cL-11 2.32E-1E e.13Ed25 2.76t-23 c.34L-22 PU214 2.31 lac 4 1.02E-13 3. b b t = 2 '-

4.26E-20 e.2Lt-16 PD215 2.06F=ob b.61t-17 6.60t=2u 1.ett-22

1. cot-g3 Pu21e 1.76L-ve 1.36E-12 2.63t=19 2.07E=20 1.uBL-la PU21e 2.12E=03 1.12L-13 3.62E=20 c.2tE 20 6.2ut-to AT217
3. 79E =o7 2.37L=1b 8.3dt-25 2.61E-23 2.4cE-22 HN219 c.63E-0S 6.81L=17
e. ELE =26 1.61L-22 1.0hE-21 HN2dv 6.a6E on 1.3cE-17
2. 61 E 19 2.07t=2e 1.oot-lo Rad 22 3.82E 00 1.13E-13 2.57E-2u 0.0 0.o FR221 3.33E=03 2.37t-16 8.32L-25 2.61E=23 2.4ct-22 FP223 1.53E-02 1.57E-19 5.69E-2o 6.64E-du 2.1cE-23 RA224 3.60L 00 1.71E-1c 5.97E-21 0.0 0.0 RA226 5.8cE 05 2.51 E -19 6.76L=2e -

0.0 0.0 AC227 7.69E 03 1.12E=17 3.92E=24 0.0 0.0 AC226 2.55E=01 3.01L-23 1.06E=29 1.66E=27 6.11E=27 TM228 6.98E 02 1.70L=1a S.97E=21 6.c7E=19 0.0 TH229 2.67E 06 c.14t=19 1.4SL=25 0.0 0.0 TH230 2.92E 07 6.c7E-16 2.27E=22 3.71E-20 6.91t-20 TM231 1.07E 00 2.56E-11 6.97E=16 1.32E=16 0.0 TH232 5.15E 12 4.90E=22 1.72L-26 2.8hE-2e 6.76t=26 TH233 1.53E=02 1.73E=1a 5.96E=21 0.0 0.0 TM234 2.41E 01 2.26E-11 7.92E=16

1. 2 c E = 15,

3.05E-15 PA231 1.19L 07 5.21E=16 1.62L-22 2.80E=20 7.11L-20 PA232 1.32E 00 6.69E=12 2.34E-16 9.29E=22 0.0 i

PA233 2.70E 01 7.93L-12 2.76L-16 c.51E-16 1.06E-IS PA23am B.13E=ou 2.26t=11 7.92E=18 1.20L-15 3.07E 15 PA23c 2.81E-01 1.00E=13 3.50E=20 1.20E=16 3.07E-16 U232 2.63E 04 9.82t=1s

3. cut =20 5.50E-lb 1.35E 17 U233 5.92E 07 2.42E=15 B.47E-22 1.28E=19 3.29E-19 U23u 9.02E 07 7.40E=11 2.59E=17 3.93E=15 1.00E-14 C21_9 E
  • 171) 6.73E*19 1.32E=16 3.39E-16 G,

U235 2.59E 11 4

U236 8.73E 09 1.1_8 E = 11 4.14E-18 6.27E=16 1.60E 15 g 't/ -U237 6.7SE u0 Q 8aE=053 1.3cE=11 1.11E=10 3.13E=o'9

., i U238 1.65E 12

({J27t=113 7.95E=to 1.20E-15 1.oet-15 U239 1.63h-02 Chi 65c-057) 2.30E=11 0.0 0.6 NP236 9.17t=01 6.20E=11 2.17 E - 17 5.6eE=23 0.0 NP237 7.sdE 08 8.77E-12 3.07E=18 c.62E-te 1.21F-15 NP236 2.10E 09 G _9 %

3.49E=12 1.09E=13 2.6SL-10 NP239 2.35E 00 1.2eEo03 4.34E=10 3.06E-11 3.91L-vo

~

Pu236 1.04E 03 6.SOE=12 2.27E=1b 3.40E=16 6.buE-16 PU238 3.2SL 04 4.88t=08 1.71E=14 2.6cE-12 6.71L-12 JP U2 3_

8.91E 06 1.77E=06 6.29E=15 9.S6E=13

.2.44E-12

~

(,

PU240 2,47E 06 f.72E=06

' #R)MT 9T1-tE=13 2.33E-12 PU241 5.33E 03 dr.89t=067:>

1.01L=12 1.53E=10 3.92E O

PU242 1.38E 08

'2. 5 S t = 11 8.93E=18 1.35E-15 3.c6E-15

. Gb PU243 2.07E=01 2.89E=06 5.51E-16 1.0cE=13 2.22E-13 1.01E*12 16e 9.25E-17 A*241 1.58E 05 1.57E=u9 AM242M 5.55E 04 1.49E=10.

5.23L-17 7.92E=15

2. v 3 E =1 -

G)

AMau2 6.67E=01 6.66E=97

..3.03E=13 7.12E=15 7.9aE-13

-@ QS

.. _ p _.f* - [ -3

_ f.

v.s -,-

-[.s

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I G

=:

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4r L

GE S*0='Ju2 1 = T H wu=ut u Lioulp EFFLUENTS GD Ar*NDAL HEL C u t' L a N T C o r. C h i, T H A T I O N S = = = = = _= = = = = = = = = = = = = = = = = = =

dp

  • LCLIDt 'iatJ=iIFE Aw! NARY SECUNDARY BU40r, HS FLOOk DRAIN (ts a T S )

(MICNH CI/dL)(nIC40 CI/ML) (CU41tS)

(CURIES)

A 2u3 P.79t ue 2.49t=10 e 70t=17 1.32L-14 3.3BL-14 GD A*2au 1.61E=02 9.96E=09 3.4SE=14 0.0 0.0 C"2u2 1.63t 02 5.ocE=07 1.75L-13 2.3SE=11 6.e9E=11 Ce243 1.17t on 2.e9t=11 1.01E=17 1.53E-15 3.92E=15 4D CM24u 6.61t 03 2.Sut=o6 6.75E=15 1.32E=12 3.39E=.2 Cn245 5.0eE 06 2.94t=12 1.03E=18 1.56t=16 4.00L-16 Ca2ue 1.72t ao a.49E=13 1.57E=19 2.38E=17 6.10E-17 O

FISSIt'N, d w)U f. I S Z'.

7 2 1.94r 00 1.04E=09 3.64E=16 6.02E=16 2.39t=14 (D

GA 72 S.4 7t -o l 1 15t=09 4.04Ea16 8.64t=18 3.42t=14 GA 73 4 out=01 1.16t=09 4.0SE-to 0.0 2.93t=20 GA 74 S.49t=93 1.79t=10 6.05t=17 0.0 0.0 d>

et 75 5.39taud

2. Sot =09 e.71E-lo 0.0 9.99E=36 AS 76 1.tuE 00 2.76t=10 9.eSE=17 4.1 1 E = 2'1 1.72t=15 GL 77 1.71L=ul 4.17t=ub 1.4et=14 1.23E=26 5.02E=15 49 AS 77 1.61E 90 1.61t=07 5,63t=14 2.03t=16 2.90E=12 SE 77M d.95t=o4 c.62t=10 1.69E=le 6.09E=19 8.71E=15 GE 7e n.12t=u2 7.17t=0e 2.50E=14 0.0 9.44E=33

()

AS 7e e.32t =o2 1.3cE=07 4.66t=14 0.0 1.01E=30 AS 79 e.25E=93 1.92t=Gb b.51L=1b 0.0 0.0 SL 79e 7.71t=u3 2.75t=06 9.40E=1b 0.o 9.0 CD SL 79 2.37E 07 1.59t=11 4.86E=18 7.3eE=16 1.89E-15 BR 60H 1 s t=01 S.13E=07 1.79E=13 0.0 2.31E=17 e

BH 80 1.22E=02 2.e3t=oS 9.06E=1d 0.0 2.48E=17 S

SE 81M 4.9et=12 3, u.7 E = 0 6 1.21t=10 0.0 0.0 St 81 1.29t=v2 1.39t=07 4.60L-1c 0.0 0.0 dW 82M w.24E = 83 6.36t=o6 2.12E=12 0.0 0.0 BR 82 1.47E uo

4. set =0a 1.SSE=10 2.02t=12 5.93t=0e SE U3 1.7"t=02 1.64k=Q7 5.67t=10 0.0 0.4 SR 83 1.'DE=01 1.3at=u2 J,3 66E=09 0.0 0.00000 (9

BR eck 1.17t=03

3. ' i t.= 0 S 1.04E=11 0.3 0.0 Bd 64

/.21t=02 7.7ot=03 2.69E=09 0.0 0.0 Rd 86 1.9 7t al 1.o0Le04 6.24E=11 J. Set =o7 1.61E=0e 9

He 87 1.43E 13 o.ubt=12 2.52E=le 4.30E=14 o.81E=16 Sn e7M

t. tot =11 1.11E=11 3.69E=16 0.0 7.90t=27 Re 86 1.auE=e2 S.77t=01 2.23E=07 c.0 0.00000 O
  • n o9 1.07t=62 3.7tt=0?
1. sat.08 -

-o. 0

-o.o SH 89 5.20h ol 6.67t=04 2.41E=10 2.S2t=06 6.63E=0e '

3k 90

1. 9 5E ue 1.edt=0S 6.36E=12 9.62t=10 2.47E=09 '

iO Y 90M 1.29t-el 4.19t=11 2.46t=16 0.0 2.53L-25 Y 96 2.57t.> 0 3.oet=05 4.21t=09 0.conou c.00000.,'

sw g1 t 03r=31 s_cee=na

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